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Volume 15, issue 24
Atmos. Chem. Phys., 15, 14031–14040, 2015
https://doi.org/10.5194/acp-15-14031-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 15, 14031–14040, 2015
https://doi.org/10.5194/acp-15-14031-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 21 Dec 2015

Research article | 21 Dec 2015

On the emissions and transport of bromoform: sensitivity to model resolution and emission location

M. R. Russo et al.

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Archibald, A., Levine, J., Abraham, N., Cooke, M., Edwards, P., Heard, D., Jenkin, M., Karunaharan, A., Pike, R., Monks, P., Shallcross, D., Telford, P., Whalley, L., and Pyle, J.: Impacts of HOx regeneration and recycling in the oxidation of isoprene: Consequences for the composition of past, present and future atmospheres, Geophys. Res. Lett., 38, L05804, https://doi.org/10.1029/2010GL046520, 2011.
Aschmann, J. and Sinnhuber, B.-M.: Contribution of very short-lived substances to stratospheric bromine loading: uncertainties and constraints, Atmos. Chem. Phys., 13, 1203–1219, https://doi.org/10.5194/acp-13-1203-2013, 2013.
Ashfold, M. J., Harris, N. R. P., Manning, A. J., Robinson, A. D., Warwick, N. J., and Pyle, J. A.: Estimates of tropical bromoform emissions using an inversion method, Atmos. Chem. Phys., 14, 979–994, https://doi.org/10.5194/acp-14-979-2014, 2014.
Butler, J. H., King, D. B., Lobert, J. M., Montzka, S. A., Yvon-Lewis, S. A., Hall, B. D., Warwick, N. J., Mondeel, D. J., Aydin, M., and Elkins, J. W.: Oceanic distributions and emissions of short-lived halocarbons, Global Biogeochem. Cy., 21, GB1023, https://doi.org/10.1029/2006GB002732, 2007.
Carpenter, L. J., Reimann, S., Burkholder, J. B., Clerbaux, C., Hall, B. D., Hossaini, R., Laube, J. C., and Yvon-Lewis, S. A.: Ozone-Depleting Substances (ODSs) and Other Gases of Interest to the Montreal Protocol, Chapter 1 in Scientific Assessment of Ozone Depletion: 2014, Update on Global Ozone Research and Monitoring Project – Report No. 55, World Meteorological Organization, Geneva, Switzerland, 2014.
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We find a strong regional element to the uplift of CHBr3 from the ocean to the upper troposphere and lower stratosphere. The strongest uplift occurs when the largest emission and the most intense convection are co-located which is over the Maritime Continent in northern winter. Estimates of CHBr3 emissions based on aircraft measurements will be sensitive to where the available aircraft campaigns took place.
We find a strong regional element to the uplift of CHBr3 from the ocean to the upper troposphere...
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