Articles | Volume 23, issue 19
https://doi.org/10.5194/acp-23-10835-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-10835-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Technical note: In situ measurements and modelling of the oxidation kinetics in films of a cooking aerosol proxy using a quartz crystal microbalance with dissipation monitoring (QCM-D)
Adam Milsom
School of Geography, Earth and Environmental Sciences, University of Birmingham, Edgbaston, Birmingham, B15 2TT UK
Shaojun Qi
School of Chemical Engineering, University of Birmingham, Edgbaston, Birmingham, B15 2TT, UK
Ashmi Mishra
Multiphase Chemistry Department, Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, 55128 Mainz, Germany
Thomas Berkemeier
Multiphase Chemistry Department, Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, 55128 Mainz, Germany
Zhenyu Zhang
School of Chemical Engineering, University of Birmingham, Edgbaston, Birmingham, B15 2TT, UK
School of Geography, Earth and Environmental Sciences, University of Birmingham, Edgbaston, Birmingham, B15 2TT UK
Department of Meteorology, University of Reading, Whiteknights, Earley Gate, Reading, RG6 6BB, UK
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Short summary
Aerosols and films are found indoors and outdoors. Our study measures and models reactions of a cooking aerosol proxy with the atmospheric oxidant ozone relying on a low-cost but sensitive technique based on mass changes and film rigidity. We found that film morphology changed and film rigidity increased with evidence of surface crust formation during ozone exposure. Our modelling results demonstrate clear potential to take this robust method to the field for reaction monitoring.
Aerosols and films are found indoors and outdoors. Our study measures and models reactions of a...
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