Articles | Volume 22, issue 4
https://doi.org/10.5194/acp-22-2909-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-2909-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
03 Mar 2022
Research article |
| 03 Mar 2022
| 03 Mar 2022
Relative importance of high-latitude local and long-range-transported dust for Arctic ice-nucleating particles and impacts on Arctic mixed-phase clouds
Department of Atmospheric Sciences, Texas A&M University, College Station, TX, USA
Xiaohong Liu
CORRESPONDING AUTHOR
Department of Atmospheric Sciences, Texas A&M University, College Station, TX, USA
Mingxuan Wu
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, WA, USA
Department of Atmospheric Sciences, Texas A&M University, College Station, TX, USA
Ziming Ke
Department of Atmospheric Sciences, Texas A&M University, College Station, TX, USA
Hunter Brown
Department of Atmospheric Sciences, Texas A&M University, College Station, TX, USA
Related authors
Mingxuan Wu, Xiaohong Liu, Hongbin Yu, Hailong Wang, Yang Shi, Kang Yang, Anton Darmenov, Chenglai Wu, Zhien Wang, Tao Luo, Yan Feng, and Ziming Ke
Atmos. Chem. Phys., 20, 13835–13855, https://doi.org/10.5194/acp-20-13835-2020, https://doi.org/10.5194/acp-20-13835-2020, 2020
Short summary
Short summary
The spatiotemporal distributions of dust aerosol simulated by global climate models (GCMs) are highly uncertain. In this study, we evaluate dust extinction profiles, optical depth, and surface concentrations simulated in three GCMs and one reanalysis against multiple satellite retrievals and surface observations to gain process-level understanding. Our results highlight the importance of correctly representing dust emission, dry/wet deposition, and size distribution in GCMs.
Mingxuan Wu, Hailong Wang, Zheng Lu, Xiaohong Liu, Huisheng Bian, David Cohen, Yan Feng, Mian Chin, Didier A. Hauglustaine, Vlassis A. Karydis, Marianne T. Lund, Gunnar Myhre, Andrea Pozzer, Michael Schulz, Ragnhild B. Skeie, Alexandra P. Tsimpidi, Svetlana G. Tsyro, and Shaocheng Xie
EGUsphere, https://doi.org/10.5194/egusphere-2025-235, https://doi.org/10.5194/egusphere-2025-235, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
A key challenge in simulating the lifecycle of nitrate aerosol in global climate models is to accurately represent mass size distribution of nitrate aerosol, which lacks sufficient observational constraints. We found that most climate models underestimate the mass fraction of fine-mode nitrate at surface in all regions. Our study highlights the importance of gas-aerosol partitioning parameterization and simulation of dust and sea salt in correctly simulating mass size distribution of nitrate.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes W. Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
Atmos. Chem. Phys., 25, 1545–1567, https://doi.org/10.5194/acp-25-1545-2025, https://doi.org/10.5194/acp-25-1545-2025, 2025
Short summary
Short summary
We compared smoke plume simulations from 11 global models to each other and to satellite smoke amount observations aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss rate assumptions vary enormously among models, causing uncertainties that require systematic in situ measurements to resolve.
Kai Lyu, Xiaohong Liu, and Bernd Kärcher
EGUsphere, https://doi.org/10.5194/egusphere-2024-4144, https://doi.org/10.5194/egusphere-2024-4144, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Two nucleation schemes are used to study ice nucleation, focusing on three ice sources: mountains, turbulence and anvils. Ice from mountains is concentrated in mid- and high-latitudes, while ice from turbulence and anvils is more common in low and mid-latitudes. Both schemes simulate orographic cirrus clouds, with mountain ice as the dominant source. The schemes differ in how they handle ice source competition, causing turbulence and anvils to influence clouds differently.
Philip J. Rasch, Haruki Hirasawa, Mingxuan Wu, Sarah J. Doherty, Robert Wood, Hailong Wang, Andy Jones, James Haywood, and Hansi Singh
Geosci. Model Dev., 17, 7963–7994, https://doi.org/10.5194/gmd-17-7963-2024, https://doi.org/10.5194/gmd-17-7963-2024, 2024
Short summary
Short summary
We introduce a protocol to compare computer climate simulations to better understand a proposed strategy intended to counter warming and climate impacts from greenhouse gas increases. This slightly changes clouds in six ocean regions to reflect more sunlight and cool the Earth. Example changes in clouds and climate are shown for three climate models. Cloud changes differ between the models, but precipitation and surface temperature changes are similar when their cooling effects are made similar.
Joseph P. Hollowed, Christiane Jablonowski, Hunter Y. Brown, Benjamin R. Hillman, Diana L. Bull, and Joseph L. Hart
Geosci. Model Dev., 17, 5913–5938, https://doi.org/10.5194/gmd-17-5913-2024, https://doi.org/10.5194/gmd-17-5913-2024, 2024
Short summary
Short summary
Large volcanic eruptions deposit material in the upper atmosphere, which is capable of altering temperature and wind patterns of Earth's atmosphere for subsequent years. This research describes a new method of simulating these effects in an idealized, efficient atmospheric model. A volcanic eruption of sulfur dioxide is described with a simplified set of physical rules, which eventually cools the planetary surface. This model has been designed as a test bed for climate attribution studies.
Allen Hu, Xiaohong Liu, Ziming Ke, Benjamin Wagman, Hunter Brown, Zheng Lu, Diana Bull, and Kara Peterson
EGUsphere, https://doi.org/10.5194/egusphere-2024-2227, https://doi.org/10.5194/egusphere-2024-2227, 2024
Short summary
Short summary
Volcanic eruptions have a major effect on temperature throughout the atmosphere and can be studied as a proxy for geo-engineering. The aerosol module in the Energy Exascale Earth System Model (E3SM) was originally intended for simulation of tropospheric aerosols and has problems handling stratospheric sulfate aerosols due to volcanic eruptions. We have made alterations to the aerosol module to overcome these problems, with simulation results more closely reproducing observations.
Hunter York Brown, Benjamin Wagman, Diana Bull, Kara Peterson, Benjamin Hillman, Xiaohong Liu, Ziming Ke, and Lin Lin
Geosci. Model Dev., 17, 5087–5121, https://doi.org/10.5194/gmd-17-5087-2024, https://doi.org/10.5194/gmd-17-5087-2024, 2024
Short summary
Short summary
Explosive volcanic eruptions lead to long-lived, microscopic particles in the upper atmosphere which act to cool the Earth's surface by reflecting the Sun's light back to space. We include and test this process in a global climate model, E3SM. E3SM is tested against satellite and balloon observations of the 1991 eruption of Mt. Pinatubo, showing that with these particles in the model we reasonably recreate Pinatubo and its global effects. We also explore how particle size leads to these effects.
Johannes Mülmenstädt, Edward Gryspeerdt, Sudhakar Dipu, Johannes Quaas, Andrew S. Ackerman, Ann M. Fridlind, Florian Tornow, Susanne E. Bauer, Andrew Gettelman, Yi Ming, Youtong Zheng, Po-Lun Ma, Hailong Wang, Kai Zhang, Matthew W. Christensen, Adam C. Varble, L. Ruby Leung, Xiaohong Liu, David Neubauer, Daniel G. Partridge, Philip Stier, and Toshihiko Takemura
Atmos. Chem. Phys., 24, 7331–7345, https://doi.org/10.5194/acp-24-7331-2024, https://doi.org/10.5194/acp-24-7331-2024, 2024
Short summary
Short summary
Human activities release copious amounts of small particles called aerosols into the atmosphere. These particles change how much sunlight clouds reflect to space, an important human perturbation of the climate, whose magnitude is highly uncertain. We found that the latest climate models show a negative correlation but a positive causal relationship between aerosols and cloud water. This means we need to be very careful when we interpret observational studies that can only see correlation.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter G. Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankararaman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Johann Engelbrecht, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbigniew Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-1617, https://doi.org/10.5194/egusphere-2024-1617, 2024
Short summary
Short summary
Aerosol particles are an important part of the Earth system, but their concentrations are spatially and temporally heterogeneous, as well as variable in size and composition. Here we present a new compilation of PM2.5 and PM10 aerosol observations, focusing on the spatial variability across different observational stations, including composition, and demonstrate a method for comparing the datasets to model output.
Ziming Ke, Qi Tang, Jean-Christoophe Golaz, Xiaohong Liu, and Hailong Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1612, https://doi.org/10.5194/egusphere-2024-1612, 2024
Short summary
Short summary
By treating volcanic emission interactively, model results improve simulated temperature variability, showing better correlations for 1940–1959 and 1960–1979, and reveals how volcanic activity influences cloud behavior and climate.
Hao Wang, Xiaohong Liu, Chenglai Wu, and Guangxing Lin
Atmos. Chem. Phys., 24, 3309–3328, https://doi.org/10.5194/acp-24-3309-2024, https://doi.org/10.5194/acp-24-3309-2024, 2024
Short summary
Short summary
We quantified different global- and regional-scale drivers of biogenic volatile organic compound (BVOC) emission trends over the past 20 years. The results show that global greening trends significantly boost BVOC emissions and deforestation reduces BVOC emissions in South America and Southeast Asia. Elevated temperature in Europe and increased soil moisture in East and South Asia enhance BVOC emissions. The results deepen our understanding of long-term BVOC emission trends in hotspots.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankarararman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Hannele Hakola, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbiginiw Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-1, https://doi.org/10.5194/essd-2024-1, 2024
Preprint withdrawn
Short summary
Short summary
Aerosol particles can interact with incoming solar radiation and outgoing long wave radiation, change cloud properties, affect photochemistry, impact surface air quality, and when deposited impact surface albedo of snow and ice, and modulate carbon dioxide uptake by the land and ocean. Here we present a new compilation of aerosol observations including composition, a methodology for comparing the datasets to model output, and show the implications of these results using one model.
Hamza Ahsan, Hailong Wang, Jingbo Wu, Mingxuan Wu, Steven J. Smith, Susanne Bauer, Harrison Suchyta, Dirk Olivié, Gunnar Myhre, Hitoshi Matsui, Huisheng Bian, Jean-François Lamarque, Ken Carslaw, Larry Horowitz, Leighton Regayre, Mian Chin, Michael Schulz, Ragnhild Bieltvedt Skeie, Toshihiko Takemura, and Vaishali Naik
Atmos. Chem. Phys., 23, 14779–14799, https://doi.org/10.5194/acp-23-14779-2023, https://doi.org/10.5194/acp-23-14779-2023, 2023
Short summary
Short summary
We examine the impact of the assumed effective height of SO2 injection, SO2 and BC emission seasonality, and the assumed fraction of SO2 emissions injected as SO4 on climate and chemistry model results. We find that the SO2 injection height has a large impact on surface SO2 concentrations and, in some models, radiative flux. These assumptions are a
hiddensource of inter-model variability and may be leading to bias in some climate model results.
Simone Tilmes, Michael J. Mills, Yunqian Zhu, Charles G. Bardeen, Francis Vitt, Pengfei Yu, David Fillmore, Xiaohong Liu, Brian Toon, and Terry Deshler
Geosci. Model Dev., 16, 6087–6125, https://doi.org/10.5194/gmd-16-6087-2023, https://doi.org/10.5194/gmd-16-6087-2023, 2023
Short summary
Short summary
We implemented an alternative aerosol scheme in the high- and low-top model versions of the Community Earth System Model Version 2 (CESM2) with a more detailed description of tropospheric and stratospheric aerosol size distributions than the existing aerosol model. This development enables the comparison of different aerosol schemes with different complexity in the same model framework. It identifies improvements compared to a range of observations in both the troposphere and stratosphere.
Qi Tang, Jean-Christophe Golaz, Luke P. Van Roekel, Mark A. Taylor, Wuyin Lin, Benjamin R. Hillman, Paul A. Ullrich, Andrew M. Bradley, Oksana Guba, Jonathan D. Wolfe, Tian Zhou, Kai Zhang, Xue Zheng, Yunyan Zhang, Meng Zhang, Mingxuan Wu, Hailong Wang, Cheng Tao, Balwinder Singh, Alan M. Rhoades, Yi Qin, Hong-Yi Li, Yan Feng, Yuying Zhang, Chengzhu Zhang, Charles S. Zender, Shaocheng Xie, Erika L. Roesler, Andrew F. Roberts, Azamat Mametjanov, Mathew E. Maltrud, Noel D. Keen, Robert L. Jacob, Christiane Jablonowski, Owen K. Hughes, Ryan M. Forsyth, Alan V. Di Vittorio, Peter M. Caldwell, Gautam Bisht, Renata B. McCoy, L. Ruby Leung, and David C. Bader
Geosci. Model Dev., 16, 3953–3995, https://doi.org/10.5194/gmd-16-3953-2023, https://doi.org/10.5194/gmd-16-3953-2023, 2023
Short summary
Short summary
High-resolution simulations are superior to low-resolution ones in capturing regional climate changes and climate extremes. However, uniformly reducing the grid size of a global Earth system model is too computationally expensive. We provide an overview of the fully coupled regionally refined model (RRM) of E3SMv2 and document a first-of-its-kind set of climate production simulations using RRM at an economic cost. The key to this success is our innovative hybrid time step method.
Aishwarya Raman, Thomas Hill, Paul J. DeMott, Balwinder Singh, Kai Zhang, Po-Lun Ma, Mingxuan Wu, Hailong Wang, Simon P. Alexander, and Susannah M. Burrows
Atmos. Chem. Phys., 23, 5735–5762, https://doi.org/10.5194/acp-23-5735-2023, https://doi.org/10.5194/acp-23-5735-2023, 2023
Short summary
Short summary
Ice-nucleating particles (INPs) play an important role in cloud processes and associated precipitation. Yet, INPs are not accurately represented in climate models. This study attempts to uncover these gaps by comparing model-simulated INP concentrations against field campaign measurements in the SO for an entire year, 2017–2018. Differences in INP concentrations and variability between the model and observations have major implications for modeling cloud properties in high latitudes.
Mengjiao Jiang, Yaoting Li, Weiji Hu, Yinshan Yang, Guy Brasseur, and Xi Zhao
Atmos. Chem. Phys., 23, 4545–4557, https://doi.org/10.5194/acp-23-4545-2023, https://doi.org/10.5194/acp-23-4545-2023, 2023
Short summary
Short summary
Relatively clean background aerosol over the Tibetan Plateau makes the study of aerosol–cloud–precipitation interactions distinctive. A convection on 24 July 2014 in Naqu was selected using the Weather Research Forecasting (WRF) model, including the Thompson aerosol-aware microphysical scheme. Our study uses a compromise approach to the limited observations. We show that the transformation of cloud water to graupel and the development of convective clouds are favored in a polluted situation.
Longlei Li, Natalie M. Mahowald, Jasper F. Kok, Xiaohong Liu, Mingxuan Wu, Danny M. Leung, Douglas S. Hamilton, Louisa K. Emmons, Yue Huang, Neil Sexton, Jun Meng, and Jessica Wan
Geosci. Model Dev., 15, 8181–8219, https://doi.org/10.5194/gmd-15-8181-2022, https://doi.org/10.5194/gmd-15-8181-2022, 2022
Short summary
Short summary
This study advances mineral dust parameterizations in the Community Atmospheric Model (CAM; version 6.1). Efforts include 1) incorporating a more physically based dust emission scheme; 2) updating the dry deposition scheme; and 3) revising the gravitational settling velocity to account for dust asphericity. Substantial improvements achieved with these updates can help accurately quantify dust–climate interactions using CAM, such as the dust-radiation and dust–cloud interactions.
Kai Zhang, Wentao Zhang, Hui Wan, Philip J. Rasch, Steven J. Ghan, Richard C. Easter, Xiangjun Shi, Yong Wang, Hailong Wang, Po-Lun Ma, Shixuan Zhang, Jian Sun, Susannah M. Burrows, Manish Shrivastava, Balwinder Singh, Yun Qian, Xiaohong Liu, Jean-Christophe Golaz, Qi Tang, Xue Zheng, Shaocheng Xie, Wuyin Lin, Yan Feng, Minghuai Wang, Jin-Ho Yoon, and L. Ruby Leung
Atmos. Chem. Phys., 22, 9129–9160, https://doi.org/10.5194/acp-22-9129-2022, https://doi.org/10.5194/acp-22-9129-2022, 2022
Short summary
Short summary
Here we analyze the effective aerosol forcing simulated by E3SM version 1 using both century-long free-running and short nudged simulations. The aerosol forcing in E3SMv1 is relatively large compared to other models, mainly due to the large indirect aerosol effect. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 have a strong correlation. The aerosol forcing estimates in E3SMv1 are sensitive to the parameterization changes in both liquid and ice cloud processes.
Susannah M. Burrows, Richard C. Easter, Xiaohong Liu, Po-Lun Ma, Hailong Wang, Scott M. Elliott, Balwinder Singh, Kai Zhang, and Philip J. Rasch
Atmos. Chem. Phys., 22, 5223–5251, https://doi.org/10.5194/acp-22-5223-2022, https://doi.org/10.5194/acp-22-5223-2022, 2022
Short summary
Short summary
Sea spray particles are composed of a mixture of salts and organic substances from oceanic microorganisms. In prior work, our team developed an approach connecting sea spray chemistry to ocean biology, called OCEANFILMS. Here we describe its implementation within an Earth system model, E3SM. We show that simulated sea spray chemistry is consistent with observed seasonal cycles and that sunlight reflected by simulated Southern Ocean clouds increases, consistent with analysis of satellite data.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
Short summary
Short summary
An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Xi Zhao and Xiaohong Liu
Atmos. Chem. Phys., 22, 2585–2600, https://doi.org/10.5194/acp-22-2585-2022, https://doi.org/10.5194/acp-22-2585-2022, 2022
Short summary
Short summary
The goal of this study is to investigate the relative importance and interactions of primary and secondary ice production in the Arctic mixed-phase clouds. Our results show that the SIP is not only a result of ice crystals produced from ice nucleation, but also competes with the ice production; conversely, strong ice nucleation also suppresses SIP.
Ka Ming Fung, Colette L. Heald, Jesse H. Kroll, Siyuan Wang, Duseong S. Jo, Andrew Gettelman, Zheng Lu, Xiaohong Liu, Rahul A. Zaveri, Eric C. Apel, Donald R. Blake, Jose-Luis Jimenez, Pedro Campuzano-Jost, Patrick R. Veres, Timothy S. Bates, John E. Shilling, and Maria Zawadowicz
Atmos. Chem. Phys., 22, 1549–1573, https://doi.org/10.5194/acp-22-1549-2022, https://doi.org/10.5194/acp-22-1549-2022, 2022
Short summary
Short summary
Understanding the natural aerosol burden in the preindustrial era is crucial for us to assess how atmospheric aerosols affect the Earth's radiative budgets. Our study explores how a detailed description of dimethyl sulfide (DMS) oxidation (implemented in the Community Atmospheric Model version 6 with chemistry, CAM6-chem) could help us better estimate the present-day and preindustrial concentrations of sulfate and other relevant chemicals, as well as the resulting aerosol radiative impacts.
Zhonghua Zheng, Matthew West, Lei Zhao, Po-Lun Ma, Xiaohong Liu, and Nicole Riemer
Atmos. Chem. Phys., 21, 17727–17741, https://doi.org/10.5194/acp-21-17727-2021, https://doi.org/10.5194/acp-21-17727-2021, 2021
Short summary
Short summary
Aerosol mixing state is an important emergent property that affects aerosol radiative forcing and aerosol–cloud interactions, but it has not been easy to constrain this property globally. We present a framework for evaluating the error in aerosol mixing state induced by aerosol representation assumptions, which is one of the important contributors to structural uncertainty in aerosol models. Our study provides insights into potential improvements to model process representation for aerosols.
Xi Zhao, Xiaohong Liu, Vaughan T. J. Phillips, and Sachin Patade
Atmos. Chem. Phys., 21, 5685–5703, https://doi.org/10.5194/acp-21-5685-2021, https://doi.org/10.5194/acp-21-5685-2021, 2021
Short summary
Short summary
Arctic mixed-phase clouds significantly influence the energy budget of the Arctic. We show that a climate model considering secondary ice production (SIP) can explain the observed cloud ice number concentrations, vertical distribution pattern, and probability density distribution of ice crystal number concentrations. The mixed-phase cloud occurrence and phase partitioning are also improved.
Xi Zhao, Xiaohong Liu, Susannah M. Burrows, and Yang Shi
Atmos. Chem. Phys., 21, 2305–2327, https://doi.org/10.5194/acp-21-2305-2021, https://doi.org/10.5194/acp-21-2305-2021, 2021
Short summary
Short summary
Organic sea spray particles influence aerosol and cloud processes over the ocean. This study introduces the emission, cloud droplet activation, and ice nucleation (IN) of marine organic aerosol (MOA) into the Community Earth System Model. Our results indicate that MOA IN particles dominate primary ice nucleation below 400 hPa over the Southern Ocean and Arctic boundary layer. MOA enhances cloud forcing over the Southern Ocean in the austral winter and summer.
Ryan Patnaude, Minghui Diao, Xiaohong Liu, and Suqian Chu
Atmos. Chem. Phys., 21, 1835–1859, https://doi.org/10.5194/acp-21-1835-2021, https://doi.org/10.5194/acp-21-1835-2021, 2021
Short summary
Short summary
A comprehensive, in situ observation dataset of cirrus clouds was developed based on seven field campaigns, ranging from 87° N–75° S. The observations were compared with a global climate model. Several key factors for cirrus cloud formation were examined, including thermodynamics, dynamics, aerosol indirect effects and geographical locations. Model biases include lower ice mass concentrations, smaller ice crystals and weaker aerosol indirect effects.
Mingxuan Wu, Xiaohong Liu, Hongbin Yu, Hailong Wang, Yang Shi, Kang Yang, Anton Darmenov, Chenglai Wu, Zhien Wang, Tao Luo, Yan Feng, and Ziming Ke
Atmos. Chem. Phys., 20, 13835–13855, https://doi.org/10.5194/acp-20-13835-2020, https://doi.org/10.5194/acp-20-13835-2020, 2020
Short summary
Short summary
The spatiotemporal distributions of dust aerosol simulated by global climate models (GCMs) are highly uncertain. In this study, we evaluate dust extinction profiles, optical depth, and surface concentrations simulated in three GCMs and one reanalysis against multiple satellite retrievals and surface observations to gain process-level understanding. Our results highlight the importance of correctly representing dust emission, dry/wet deposition, and size distribution in GCMs.
Stefan Rahimi, Xiaohong Liu, Chun Zhao, Zheng Lu, and Zachary J. Lebo
Atmos. Chem. Phys., 20, 10911–10935, https://doi.org/10.5194/acp-20-10911-2020, https://doi.org/10.5194/acp-20-10911-2020, 2020
Short summary
Short summary
Dark particles emitted to the atmosphere can absorb sunlight and heat the air. As these particles settle, they may darken the surface, especially over snow-covered regions like the Rocky Mountains. This darkening of the surface may lead to changes in snowpack, affecting the local meteorology and hydrology. We seek to evaluate whether these light-absorbing particles more prominently affect this region through their atmospheric presence or their on-snow presence.
Chenglai Wu, Zhaohui Lin, and Xiaohong Liu
Atmos. Chem. Phys., 20, 10401–10425, https://doi.org/10.5194/acp-20-10401-2020, https://doi.org/10.5194/acp-20-10401-2020, 2020
Short summary
Short summary
This study provides a comprehensive evaluation of the global dust cycle in 15 models participating in the fifth phase of the Coupled Model Intercomparison Project (CMIP5). We assess the global budget and associated uncertainties. We also quantify the discrepancies in each model. The results highlight the large uncertainties in both the locations and intensities of dust emission. Our study will serve as a useful reference for model communities and help further model improvements.
Jonathon S. Wright, Xiaoyi Sun, Paul Konopka, Kirstin Krüger, Bernard Legras, Andrea M. Molod, Susann Tegtmeier, Guang J. Zhang, and Xi Zhao
Atmos. Chem. Phys., 20, 8989–9030, https://doi.org/10.5194/acp-20-8989-2020, https://doi.org/10.5194/acp-20-8989-2020, 2020
Short summary
Short summary
High clouds are influential in tropical climate. Although reanalysis cloud fields are essentially model products, they are indirectly constrained by observations and offer global coverage with direct links to advanced water and energy cycle metrics, giving them many useful applications. We describe how high cloud fields are generated in reanalyses, assess their realism and reliability in the tropics, and evaluate how differences in these fields affect other aspects of the reanalysis state.
Tongwen Wu, Fang Zhang, Jie Zhang, Weihua Jie, Yanwu Zhang, Fanghua Wu, Laurent Li, Jinghui Yan, Xiaohong Liu, Xiao Lu, Haiyue Tan, Lin Zhang, Jun Wang, and Aixue Hu
Geosci. Model Dev., 13, 977–1005, https://doi.org/10.5194/gmd-13-977-2020, https://doi.org/10.5194/gmd-13-977-2020, 2020
Short summary
Short summary
This paper describes the first version of the Beijing Climate Center (BCC) fully coupled Earth System Model with interactive atmospheric chemistry and aerosols (BCC-ESM1). It is one of the models at the BCC for the Coupled Model Intercomparison Project Phase 6 (CMIP6). The CMIP6 Aerosol Chemistry Model Intercomparison Project (AerChemMIP) experiment using BCC-ESM1 has been finished. The evaluations show an overall good agreement between BCC-ESM1 simulations and observations in the 20th century.
Fang Li, Maria Val Martin, Meinrat O. Andreae, Almut Arneth, Stijn Hantson, Johannes W. Kaiser, Gitta Lasslop, Chao Yue, Dominique Bachelet, Matthew Forrest, Erik Kluzek, Xiaohong Liu, Stephane Mangeon, Joe R. Melton, Daniel S. Ward, Anton Darmenov, Thomas Hickler, Charles Ichoku, Brian I. Magi, Stephen Sitch, Guido R. van der Werf, Christine Wiedinmyer, and Sam S. Rabin
Atmos. Chem. Phys., 19, 12545–12567, https://doi.org/10.5194/acp-19-12545-2019, https://doi.org/10.5194/acp-19-12545-2019, 2019
Short summary
Short summary
Fire emissions are critical for atmospheric composition, climate, carbon cycle, and air quality. We provide the first global multi-model fire emission reconstructions for 1700–2012, including carbon and 33 species of trace gases and aerosols, based on the nine state-of-the-art global fire models that participated in FireMIP. We also provide information on the recent status and limitations of the model-based reconstructions and identify the main uncertainty sources in their long-term changes.
Stefan Rahimi, Xiaohong Liu, Chenglai Wu, William K. Lau, Hunter Brown, Mingxuan Wu, and Yun Qian
Atmos. Chem. Phys., 19, 12025–12049, https://doi.org/10.5194/acp-19-12025-2019, https://doi.org/10.5194/acp-19-12025-2019, 2019
Short summary
Short summary
Light-absorbing particles impact the Earth system in a variety of ways. They can warm the atmosphere by their very presence, or they can warm the atmosphere after they deposit on snow, warm it, and warm the overlying atmosphere. This paper focuses on these two processes as they pertain to black carbon and dust's impacts on the South Asian monsoon. It will be shown that these two aerosols have a significant effect on the monsoon.
Douglas S. Hamilton, Rachel A. Scanza, Yan Feng, Joseph Guinness, Jasper F. Kok, Longlei Li, Xiaohong Liu, Sagar D. Rathod, Jessica S. Wan, Mingxuan Wu, and Natalie M. Mahowald
Geosci. Model Dev., 12, 3835–3862, https://doi.org/10.5194/gmd-12-3835-2019, https://doi.org/10.5194/gmd-12-3835-2019, 2019
Short summary
Short summary
MIMI v1.0 was designed for use within Earth system models to simulate the 3-D emission, atmospheric processing, and deposition of iron and its soluble fraction. Understanding the iron cycle is important due to its role as an essential micronutrient for ocean phytoplankton; its supply limits primary productivity in many of the world's oceans. Human activity has perturbed the iron cycle, and MIMI is capable of diagnosing many of these impacts; hence, it is important for future climate studies.
George S. Fanourgakis, Maria Kanakidou, Athanasios Nenes, Susanne E. Bauer, Tommi Bergman, Ken S. Carslaw, Alf Grini, Douglas S. Hamilton, Jill S. Johnson, Vlassis A. Karydis, Alf Kirkevåg, John K. Kodros, Ulrike Lohmann, Gan Luo, Risto Makkonen, Hitoshi Matsui, David Neubauer, Jeffrey R. Pierce, Julia Schmale, Philip Stier, Kostas Tsigaridis, Twan van Noije, Hailong Wang, Duncan Watson-Parris, Daniel M. Westervelt, Yang Yang, Masaru Yoshioka, Nikos Daskalakis, Stefano Decesari, Martin Gysel-Beer, Nikos Kalivitis, Xiaohong Liu, Natalie M. Mahowald, Stelios Myriokefalitakis, Roland Schrödner, Maria Sfakianaki, Alexandra P. Tsimpidi, Mingxuan Wu, and Fangqun Yu
Atmos. Chem. Phys., 19, 8591–8617, https://doi.org/10.5194/acp-19-8591-2019, https://doi.org/10.5194/acp-19-8591-2019, 2019
Short summary
Short summary
Effects of aerosols on clouds are important for climate studies but are among the largest uncertainties in climate projections. This study evaluates the skill of global models to simulate aerosol, cloud condensation nuclei (CCN) and cloud droplet number concentrations (CDNCs). Model results show reduced spread in CDNC compared to CCN due to the negative correlation between the sensitivities of CDNC to aerosol number concentration (air pollution) and updraft velocity (atmospheric dynamics).
Tongwen Wu, Yixiong Lu, Yongjie Fang, Xiaoge Xin, Laurent Li, Weiping Li, Weihua Jie, Jie Zhang, Yiming Liu, Li Zhang, Fang Zhang, Yanwu Zhang, Fanghua Wu, Jianglong Li, Min Chu, Zaizhi Wang, Xueli Shi, Xiangwen Liu, Min Wei, Anning Huang, Yaocun Zhang, and Xiaohong Liu
Geosci. Model Dev., 12, 1573–1600, https://doi.org/10.5194/gmd-12-1573-2019, https://doi.org/10.5194/gmd-12-1573-2019, 2019
Short summary
Short summary
This work presents advancements of the BCC model transition from CMIP5 to CMIP6, especially in the model resolution and its physics. Compared with BCC CMIP5 models, the BCC CMIP6 model shows significant improvements in historical simulations in many aspects including tropospheric air temperature and circulation at global and regional scales in East Asia, climate variability at different timescales (QBO, MJO, and diurnal cycle of precipitation), and the long-term trend of global air temperature.
Hunter Brown, Xiaohong Liu, Yan Feng, Yiquan Jiang, Mingxuan Wu, Zheng Lu, Chenglai Wu, Shane Murphy, and Rudra Pokhrel
Atmos. Chem. Phys., 18, 17745–17768, https://doi.org/10.5194/acp-18-17745-2018, https://doi.org/10.5194/acp-18-17745-2018, 2018
Short summary
Short summary
In climate models, organic carbon (OC) in wildfire smoke has been treated as an atmospheric cooling component by reflecting sunlight back to space. This study incorporates the observationally identified absorbing brown carbon component of OC into the Community Earth System Model, improving the agreement between the model and observations and effectively increasing absorption of solar radiation. This change contributes to altered atmospheric dynamics and changes in cloud cover in the model.
Benjamin S. Grandey, Daniel Rothenberg, Alexander Avramov, Qinjian Jin, Hsiang-He Lee, Xiaohong Liu, Zheng Lu, Samuel Albani, and Chien Wang
Atmos. Chem. Phys., 18, 15783–15810, https://doi.org/10.5194/acp-18-15783-2018, https://doi.org/10.5194/acp-18-15783-2018, 2018
Short summary
Short summary
Anthropogenic emissions of aerosol particles likely cool the climate system. We investigate the uncertainty in the strength of the cooling effect by exploring the representation of aerosols in a global climate model. We conclude that the specific representation of aerosols in global climate models has important implications for climate modelling. Important factors include the representation of aerosol mixing state, size distribution, and optical properties.
Alf Kirkevåg, Alf Grini, Dirk Olivié, Øyvind Seland, Kari Alterskjær, Matthias Hummel, Inger H. H. Karset, Anna Lewinschal, Xiaohong Liu, Risto Makkonen, Ingo Bethke, Jan Griesfeller, Michael Schulz, and Trond Iversen
Geosci. Model Dev., 11, 3945–3982, https://doi.org/10.5194/gmd-11-3945-2018, https://doi.org/10.5194/gmd-11-3945-2018, 2018
Short summary
Short summary
A new aerosol treatment is described and tested in a global climate model. With updated emissions, aerosol chemistry, and microphysics compared to its predecessor, black carbon (BC) mass concentrations aloft better fit observations, surface concentrations of BC and sea salt are less biased, and sulfate and mineral dust slightly more, while the results for organics are inconclusive. Man-made aerosols now yield a stronger cooling effect on climate that is strong compared to results from IPCC.
Tianyi Fan, Xiaohong Liu, Po-Lun Ma, Qiang Zhang, Zhanqing Li, Yiquan Jiang, Fang Zhang, Chuanfeng Zhao, Xin Yang, Fang Wu, and Yuying Wang
Atmos. Chem. Phys., 18, 1395–1417, https://doi.org/10.5194/acp-18-1395-2018, https://doi.org/10.5194/acp-18-1395-2018, 2018
Short summary
Short summary
We found that 22–28 % of the low AOD bias in eastern China simulated by the Community Atmosphere Model version 5 can be improved by using a new emission inventory. The concentrations of primary aerosols are closely related to the emission, while the seasonal variations of secondary aerosols depend more on atmospheric processes. This study highlights the importance of improving both the emission and atmospheric processes in modeling the atmospheric aerosols and their radiative effects.
Bin Zhao, Kuo-Nan Liou, Yu Gu, Jonathan H. Jiang, Qinbin Li, Rong Fu, Lei Huang, Xiaohong Liu, Xiangjun Shi, Hui Su, and Cenlin He
Atmos. Chem. Phys., 18, 1065–1078, https://doi.org/10.5194/acp-18-1065-2018, https://doi.org/10.5194/acp-18-1065-2018, 2018
Short summary
Short summary
The interactions between aerosols and ice clouds represent one of the largest uncertainties among anthropogenic forcings on climate change. We find that the responses of ice crystal effective radius, a key parameter determining ice clouds' net radiative effect, to aerosol loadings are modulated by water vapor amount and vary from a significant negative correlation in moist conditions (consistent with the “Twomey effect” for liquid clouds) to a strong positive correlation in dry conditions.
Chenglai Wu, Xiaohong Liu, Zhaohui Lin, Stefan R. Rahimi-Esfarjani, and Zheng Lu
Atmos. Chem. Phys., 18, 511–533, https://doi.org/10.5194/acp-18-511-2018, https://doi.org/10.5194/acp-18-511-2018, 2018
Short summary
Short summary
This study utilizes the newly developed variable-resolution Community Earth System Model (VR-CESM) with a refined high resolution (0.125º) to quantify the impacts of absorbing aerosol (BC and dust) deposition on snowpack and hydrologic cycles in the Rocky Mountains. BC and dust in snow significantly reduce the snowpack around the mountains. BC and dust in snow also accelerate the hydrologic cycles in the mountainous regions, with runoff increased in spring but reduced in summer.
Yawen Liu, Kai Zhang, Yun Qian, Yuhang Wang, Yufei Zou, Yongjia Song, Hui Wan, Xiaohong Liu, and Xiu-Qun Yang
Atmos. Chem. Phys., 18, 31–47, https://doi.org/10.5194/acp-18-31-2018, https://doi.org/10.5194/acp-18-31-2018, 2018
Short summary
Short summary
Fire aerosols have large impact on weather and climate through their effect on clouds and radiation, but it is difficult to quantify. Here we investigated the short-term effective radiative forcing of fire aerosols using the nudged hindcast ensemble simulations from global aerosol-climate model. Results show large effects of fire aerosols on both liquid and ice cloud and large ensemble spread of regional mean shortwave cloud radiative forcing over southern Mexico and the central US.
Maria Sand, Bjørn H. Samset, Yves Balkanski, Susanne Bauer, Nicolas Bellouin, Terje K. Berntsen, Huisheng Bian, Mian Chin, Thomas Diehl, Richard Easter, Steven J. Ghan, Trond Iversen, Alf Kirkevåg, Jean-François Lamarque, Guangxing Lin, Xiaohong Liu, Gan Luo, Gunnar Myhre, Twan van Noije, Joyce E. Penner, Michael Schulz, Øyvind Seland, Ragnhild B. Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Fangqun Yu, Kai Zhang, and Hua Zhang
Atmos. Chem. Phys., 17, 12197–12218, https://doi.org/10.5194/acp-17-12197-2017, https://doi.org/10.5194/acp-17-12197-2017, 2017
Short summary
Short summary
The role of aerosols in the changing polar climate is not well understood and the aerosols are poorly constrained in the models. In this study we have compared output from 16 different aerosol models with available observations at both poles. We show that the model median is representative of the observations, but the model spread is large. The Arctic direct aerosol radiative effect over the industrial area is positive during spring due to black carbon and negative during summer due to sulfate.
Chenglai Wu, Xiaohong Liu, Minghui Diao, Kai Zhang, Andrew Gettelman, Zheng Lu, Joyce E. Penner, and Zhaohui Lin
Atmos. Chem. Phys., 17, 4731–4749, https://doi.org/10.5194/acp-17-4731-2017, https://doi.org/10.5194/acp-17-4731-2017, 2017
Short summary
Short summary
This study utilizes a novel approach to directly compare the CAM5-simulated cloud macro- and microphysics with the collocated HIPPO observations for the period of 2009 to 2011. The model cannot capture the large spatial variabilities of observed RH, which is responsible for much of the model missing low-level warm clouds. A large portion of the RH bias results from the discrepancy in water vapor. The model underestimates the observed number concentration and ice water content.
Yiquan Jiang, Zheng Lu, Xiaohong Liu, Yun Qian, Kai Zhang, Yuhang Wang, and Xiu-Qun Yang
Atmos. Chem. Phys., 16, 14805–14824, https://doi.org/10.5194/acp-16-14805-2016, https://doi.org/10.5194/acp-16-14805-2016, 2016
Short summary
Short summary
Aerosols from open fires could significantly perturb the global radiation balance and induce climate change. In this study, the CAM5 global climate model is used to investigate the spatial and seasonal characteristics of radiative effects due to fire aerosol–radiation interactions, fire aerosol-cloud interactions and fire aerosol-surface albedo interactions, including radiative effects from all fire aerosols, fire black carbon and fire particulate organic matter.
Cheng Zhou, Joyce E. Penner, Guangxing Lin, Xiaohong Liu, and Minghuai Wang
Atmos. Chem. Phys., 16, 12411–12424, https://doi.org/10.5194/acp-16-12411-2016, https://doi.org/10.5194/acp-16-12411-2016, 2016
Short summary
Short summary
We examined the different ice nucleation parameterization factors that affect the simulated ice number concentrations in cirrus clouds in the upper troposphere using the CAM5 model. We examined the effect from three different updraft velocities (from low to high), two different water vapour accommodation coefficients (α = 0.1 or 1), the effect of including vapour deposition onto pre-existing ice particles during ice nucleation, and the effect of including SOA as heterogeneous ice nuclei.
N. I. Kristiansen, A. Stohl, D. J. L. Olivié, B. Croft, O. A. Søvde, H. Klein, T. Christoudias, D. Kunkel, S. J. Leadbetter, Y. H. Lee, K. Zhang, K. Tsigaridis, T. Bergman, N. Evangeliou, H. Wang, P.-L. Ma, R. C. Easter, P. J. Rasch, X. Liu, G. Pitari, G. Di Genova, S. Y. Zhao, Y. Balkanski, S. E. Bauer, G. S. Faluvegi, H. Kokkola, R. V. Martin, J. R. Pierce, M. Schulz, D. Shindell, H. Tost, and H. Zhang
Atmos. Chem. Phys., 16, 3525–3561, https://doi.org/10.5194/acp-16-3525-2016, https://doi.org/10.5194/acp-16-3525-2016, 2016
Short summary
Short summary
Processes affecting aerosol removal from the atmosphere are not fully understood. In this study we investigate to what extent atmospheric transport models can reproduce observed loss of aerosols. We compare measurements of radioactive isotopes, that attached to ambient sulfate aerosols during the 2011 Fukushima nuclear accident, to 19 models using identical emissions. Results indicate aerosol removal that is too fast in most models, and apply to aerosols that have undergone long-range transport.
Zak Kipling, Philip Stier, Colin E. Johnson, Graham W. Mann, Nicolas Bellouin, Susanne E. Bauer, Tommi Bergman, Mian Chin, Thomas Diehl, Steven J. Ghan, Trond Iversen, Alf Kirkevåg, Harri Kokkola, Xiaohong Liu, Gan Luo, Twan van Noije, Kirsty J. Pringle, Knut von Salzen, Michael Schulz, Øyvind Seland, Ragnhild B. Skeie, Toshihiko Takemura, Kostas Tsigaridis, and Kai Zhang
Atmos. Chem. Phys., 16, 2221–2241, https://doi.org/10.5194/acp-16-2221-2016, https://doi.org/10.5194/acp-16-2221-2016, 2016
Short summary
Short summary
The vertical distribution of atmospheric aerosol is an important factor in its effects on climate. In this study we use a sophisticated model of the many interacting processes affecting aerosol in the atmosphere to show that the vertical distribution is typically dominated by only a few of these processes. Constraining these physical processes may help to reduce the large differences between models. However, the important processes are not always the same for different types of aerosol.
Kai Zhang, Chun Zhao, Hui Wan, Yun Qian, Richard C. Easter, Steven J. Ghan, Koichi Sakaguchi, and Xiaohong Liu
Geosci. Model Dev., 9, 607–632, https://doi.org/10.5194/gmd-9-607-2016, https://doi.org/10.5194/gmd-9-607-2016, 2016
Short summary
Short summary
A sub-grid treatment based on Weibull distribution is introduced to CAM5 to take into account the impact of unresolved variability of surface wind speed on sea salt and dust emissions. Simulations show that sub-grid wind variability has relatively small impacts on the global mean sea salt emissions, but considerable influence on dust emissions. Dry convective eddies and mesoscale flows associated with complex topography are the major causes of dust emission enhancement.
X. Liu, P.-L. Ma, H. Wang, S. Tilmes, B. Singh, R. C. Easter, S. J. Ghan, and P. J. Rasch
Geosci. Model Dev., 9, 505–522, https://doi.org/10.5194/gmd-9-505-2016, https://doi.org/10.5194/gmd-9-505-2016, 2016
Short summary
Short summary
In this study, we describe and evaluate a new four-mode version of the Modal Aerosol Module (MAM4) in the Community Atmosphere Model version 5 (CAM5). Compared to the current three-mode version of MAM in CAM5, MAM4 significantly improves the simulation of seasonal variation of BC concentrations in the polar regions, by increasing the BC concentrations in all seasons and particularly in cold seasons.
S. Tilmes, J.-F. Lamarque, L. K. Emmons, D. E. Kinnison, P.-L. Ma, X. Liu, S. Ghan, C. Bardeen, S. Arnold, M. Deeter, F. Vitt, T. Ryerson, J. W. Elkins, F. Moore, J. R. Spackman, and M. Val Martin
Geosci. Model Dev., 8, 1395–1426, https://doi.org/10.5194/gmd-8-1395-2015, https://doi.org/10.5194/gmd-8-1395-2015, 2015
Short summary
Short summary
The Community Atmosphere Model (CAM), version 5, is now coupled to extensive tropospheric and stratospheric chemistry, called CAM5-chem, and is available in addition to CAM4-chem in the Community Earth System Model (CESM) version 1.2. Both configurations are well suited as tools for atmospheric chemistry modeling studies in the troposphere and lower stratosphere.
X. Shi, X. Liu, and K. Zhang
Atmos. Chem. Phys., 15, 1503–1520, https://doi.org/10.5194/acp-15-1503-2015, https://doi.org/10.5194/acp-15-1503-2015, 2015
Short summary
Short summary
The ice nucleation scheme in the Community Atmosphere Model (CAM5) was improved by considering the effects of pre-existing ice crystals and some other modifications. Subsequently, the comparison between different ice nucleation parameterizations is investigated. Experiment using the ice nucleation parameterization of Kärcher et al. (2006) predicts a much smaller anthropogenic aerosol indirect forcing than that using the parameterizations of Liu and Penner (2005) and Barahona and Nenes (2009).
R. A. Scanza, N. Mahowald, S. Ghan, C. S. Zender, J. F. Kok, X. Liu, Y. Zhang, and S. Albani
Atmos. Chem. Phys., 15, 537–561, https://doi.org/10.5194/acp-15-537-2015, https://doi.org/10.5194/acp-15-537-2015, 2015
Short summary
Short summary
The main purpose of this study was to build a framework in the Community Atmosphere Models version 4 and 5 within the Community Earth System Model to simulate dust aerosols as their component minerals. With this framework, we investigate the direct radiative forcing that results from the mineral speciation. We find that adding mineralogy results in a small positive forcing at the top of the atmosphere, while simulations without mineralogy have a small negative forcing.
S. Yu, R. Mathur, J. Pleim, D. Wong, R. Gilliam, K. Alapaty, C. Zhao, and X. Liu
Atmos. Chem. Phys., 14, 11247–11285, https://doi.org/10.5194/acp-14-11247-2014, https://doi.org/10.5194/acp-14-11247-2014, 2014
K. Tsigaridis, N. Daskalakis, M. Kanakidou, P. J. Adams, P. Artaxo, R. Bahadur, Y. Balkanski, S. E. Bauer, N. Bellouin, A. Benedetti, T. Bergman, T. K. Berntsen, J. P. Beukes, H. Bian, K. S. Carslaw, M. Chin, G. Curci, T. Diehl, R. C. Easter, S. J. Ghan, S. L. Gong, A. Hodzic, C. R. Hoyle, T. Iversen, S. Jathar, J. L. Jimenez, J. W. Kaiser, A. Kirkevåg, D. Koch, H. Kokkola, Y. H Lee, G. Lin, X. Liu, G. Luo, X. Ma, G. W. Mann, N. Mihalopoulos, J.-J. Morcrette, J.-F. Müller, G. Myhre, S. Myriokefalitakis, N. L. Ng, D. O'Donnell, J. E. Penner, L. Pozzoli, K. J. Pringle, L. M. Russell, M. Schulz, J. Sciare, Ø. Seland, D. T. Shindell, S. Sillman, R. B. Skeie, D. Spracklen, T. Stavrakou, S. D. Steenrod, T. Takemura, P. Tiitta, S. Tilmes, H. Tost, T. van Noije, P. G. van Zyl, K. von Salzen, F. Yu, Z. Wang, Z. Wang, R. A. Zaveri, H. Zhang, K. Zhang, Q. Zhang, and X. Zhang
Atmos. Chem. Phys., 14, 10845–10895, https://doi.org/10.5194/acp-14-10845-2014, https://doi.org/10.5194/acp-14-10845-2014, 2014
Y. Wang, X. Liu, C. Hoose, and B. Wang
Atmos. Chem. Phys., 14, 10411–10430, https://doi.org/10.5194/acp-14-10411-2014, https://doi.org/10.5194/acp-14-10411-2014, 2014
K. Zhang, H. Wan, X. Liu, S. J. Ghan, G. J. Kooperman, P.-L. Ma, P. J. Rasch, D. Neubauer, and U. Lohmann
Atmos. Chem. Phys., 14, 8631–8645, https://doi.org/10.5194/acp-14-8631-2014, https://doi.org/10.5194/acp-14-8631-2014, 2014
G. W. Mann, K. S. Carslaw, C. L. Reddington, K. J. Pringle, M. Schulz, A. Asmi, D. V. Spracklen, D. A. Ridley, M. T. Woodhouse, L. A. Lee, K. Zhang, S. J. Ghan, R. C. Easter, X. Liu, P. Stier, Y. H. Lee, P. J. Adams, H. Tost, J. Lelieveld, S. E. Bauer, K. Tsigaridis, T. P. C. van Noije, A. Strunk, E. Vignati, N. Bellouin, M. Dalvi, C. E. Johnson, T. Bergman, H. Kokkola, K. von Salzen, F. Yu, G. Luo, A. Petzold, J. Heintzenberg, A. Clarke, J. A. Ogren, J. Gras, U. Baltensperger, U. Kaminski, S. G. Jennings, C. D. O'Dowd, R. M. Harrison, D. C. S. Beddows, M. Kulmala, Y. Viisanen, V. Ulevicius, N. Mihalopoulos, V. Zdimal, M. Fiebig, H.-C. Hansson, E. Swietlicki, and J. S. Henzing
Atmos. Chem. Phys., 14, 4679–4713, https://doi.org/10.5194/acp-14-4679-2014, https://doi.org/10.5194/acp-14-4679-2014, 2014
P.-L. Ma, P. J. Rasch, J. D. Fast, R. C. Easter, W. I. Gustafson Jr., X. Liu, S. J. Ghan, and B. Singh
Geosci. Model Dev., 7, 755–778, https://doi.org/10.5194/gmd-7-755-2014, https://doi.org/10.5194/gmd-7-755-2014, 2014
M. S. Long, W. C. Keene, R. C. Easter, R. Sander, X. Liu, A. Kerkweg, and D. Erickson
Atmos. Chem. Phys., 14, 3397–3425, https://doi.org/10.5194/acp-14-3397-2014, https://doi.org/10.5194/acp-14-3397-2014, 2014
C. Zhao, X. Liu, Y. Qian, J. Yoon, Z. Hou, G. Lin, S. McFarlane, H. Wang, B. Yang, P.-L. Ma, H. Yan, and J. Bao
Atmos. Chem. Phys., 13, 10969–10987, https://doi.org/10.5194/acp-13-10969-2013, https://doi.org/10.5194/acp-13-10969-2013, 2013
H. Wang, R. C. Easter, P. J. Rasch, M. Wang, X. Liu, S. J. Ghan, Y. Qian, J.-H. Yoon, P.-L. Ma, and V. Vinoj
Geosci. Model Dev., 6, 765–782, https://doi.org/10.5194/gmd-6-765-2013, https://doi.org/10.5194/gmd-6-765-2013, 2013
K. Zhang, X. Liu, M. Wang, J. M. Comstock, D. L. Mitchell, S. Mishra, and G. G. Mace
Atmos. Chem. Phys., 13, 4963–4982, https://doi.org/10.5194/acp-13-4963-2013, https://doi.org/10.5194/acp-13-4963-2013, 2013
D. T. Shindell, J.-F. Lamarque, M. Schulz, M. Flanner, C. Jiao, M. Chin, P. J. Young, Y. H. Lee, L. Rotstayn, N. Mahowald, G. Milly, G. Faluvegi, Y. Balkanski, W. J. Collins, A. J. Conley, S. Dalsoren, R. Easter, S. Ghan, L. Horowitz, X. Liu, G. Myhre, T. Nagashima, V. Naik, S. T. Rumbold, R. Skeie, K. Sudo, S. Szopa, T. Takemura, A. Voulgarakis, J.-H. Yoon, and F. Lo
Atmos. Chem. Phys., 13, 2939–2974, https://doi.org/10.5194/acp-13-2939-2013, https://doi.org/10.5194/acp-13-2939-2013, 2013
B. H. Samset, G. Myhre, M. Schulz, Y. Balkanski, S. Bauer, T. K. Berntsen, H. Bian, N. Bellouin, T. Diehl, R. C. Easter, S. J. Ghan, T. Iversen, S. Kinne, A. Kirkevåg, J.-F. Lamarque, G. Lin, X. Liu, J. E. Penner, Ø. Seland, R. B. Skeie, P. Stier, T. Takemura, K. Tsigaridis, and K. Zhang
Atmos. Chem. Phys., 13, 2423–2434, https://doi.org/10.5194/acp-13-2423-2013, https://doi.org/10.5194/acp-13-2423-2013, 2013
M. S. Long, W. C. Keene, R. Easter, R. Sander, A. Kerkweg, D. Erickson, X. Liu, and S. Ghan
Geosci. Model Dev., 6, 255–262, https://doi.org/10.5194/gmd-6-255-2013, https://doi.org/10.5194/gmd-6-255-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
A global dust emission dataset for estimating dust radiative forcings in climate models
Tropospheric aerosols over the western North Atlantic Ocean during the winter and summer deployments of ACTIVATE 2020: life cycle, transport, and distribution
Spatial and temporal evolution of future atmospheric reactive nitrogen deposition in China under different climate change mitigation strategies
Steady-state mixing state of black carbon aerosols from a particle-resolved model
Distinctive dust weather intensities in North China resulted from two types of atmospheric circulation anomalies
Biomass burning emission analysis based on MODIS aerosol optical depth and AeroCom multi-model simulations: implications for model constraints and emission inventories
Quasi-weekly oscillation of regional PM2.5 transport over China driven by the synoptic-scale disturbance of the East Asian winter monsoon circulation
Solar radiation estimation in West Africa: impact of dust conditions during the 2021 dry season
Gaps in our understanding of ice-nucleating particle sources exposed by global simulation of the UK Earth System Model
The role of interfacial tension in the size-dependent phase separation of atmospheric aerosol particles
Warming effects of reduced sulfur emissions from shipping
The key role of atmospheric absorption in the Asian summer monsoon response to dust emissions in CMIP6 models
Multi-model effective radiative forcing of the 2020 sulfur cap for shipping
Representation of iron aerosol size distributions of anthropogenic emissions is critical in evaluating atmospheric soluble iron input to the ocean
High-resolution air quality maps for Bucharest using Mixed-Effects Modeling Framework
Revealing dominant patterns of aerosol regimes in the lower troposphere and their evolution from preindustrial times to the future in global climate model simulations
Improving estimation of a record-breaking east Asian dust storm emission with lagged aerosol Ångström exponent observations
Impact of biomass burning aerosols (BBA) on the tropical African climate in an ocean–atmosphere–aerosol coupled climate model
Retrieval of refractive index and water content for the coating materials of aged black carbon aerosol based on optical properties: a theoretical analysis
Predicting hygroscopic growth of organosulfur aerosol particles using COSMOtherm
Dust aerosol from the Aralkum Desert influences the radiation budget and atmospheric dynamics of Central Asia
Global modeling of aerosol nucleation with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs)
Synergistic effects of the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) on dust activities in North China during the following spring
Aerosol composition, air quality, and boundary layer dynamics in the urban background of Stuttgart in winter
Measurement report: Source attribution and estimation of black carbon levels in an urban hotspot of the central Po Valley – an integrated approach combining high-resolution dispersion modelling and micro-aethalometers
Construction and Application of a Pollen Emissions Model based on Phenology and Random Forests
Microphysical modelling of aerosol scavenging by different types of clouds: description and validation of the approach
Insights into the sources of ultrafine particle numbers at six European urban sites obtained by investigating COVID-19 lockdowns
In-plume and out-of-plume analysis of aerosol–cloud interactions derived from the 2014–2015 Holuhraun volcanic eruption
Impacts of atmospheric circulation patterns and cloud inhibition on aerosol radiative effect and boundary layer structure during winter air pollution in Sichuan Basin, China
The effectiveness of solar radiation management for marine cloud brightening geoengineering by fine sea spray in worldwide different climatic regions
Accounting for Black Carbon Aging Process in a Two-way Coupled Meteorology – Air Quality Model
Investigating the sign of stratocumulus adjustments to aerosols in the ICON global storm-resolving model
A model study investigating the sensitivity of aerosol forcing to the volatilities of semi-volatile organic compounds
Characterization of Brown Carbon absorption in different European environments through source contribution analysis
The impact of uncertainty in black carbon's refractive index on simulated optical depth and radiative forcing
Decomposing the effective radiative forcing of anthropogenic aerosols based on CMIP6 Earth system models
Modeling impacts of dust mineralogy on fast climate response
Uncertainties in laboratory-measured shortwave refractive indices of mineral dust aerosols and derived optical properties: a theoretical assessment
Diagnosing uncertainties in global biomass burning emission inventories and their impact on modeled air pollutants
Role of atmospheric aerosols in severe winter fog over the Indo-Gangetic Plain of India: a case study
Long-term variability in black carbon emissions constrained by gap-filled absorption aerosol optical depth and associated premature mortality in China
Intercomparison of aerosol optical depths from four reanalyses and their multi-reanalysis consensus
Global aviation contrail climate effects from 2019 to 2021
Rapid iodine oxoacid nucleation enhanced by dimethylamine in broad marine regions
Simulations of the impact of cloud condensation nuclei and ice-nucleating particles perturbations on the microphysics and radar reflectivity factor of stratiform mixed-phase clouds
Aerosols in the central Arctic cryosphere: satellite and model integrated insights during Arctic spring and summer
Observationally constrained regional variations of shortwave absorption by iron oxides emphasize the cooling effect of dust
Droplet collection efficiencies inferred from satellite retrievals constrain effective radiative forcing of aerosol–cloud interactions
Global aerosol-type classification using a new hybrid algorithm and Aerosol Robotic Network data
Danny M. Leung, Jasper F. Kok, Longlei Li, David M. Lawrence, Natalie M. Mahowald, Simone Tilmes, and Erik Kluzek
Atmos. Chem. Phys., 25, 2311–2331, https://doi.org/10.5194/acp-25-2311-2025, https://doi.org/10.5194/acp-25-2311-2025, 2025
Short summary
Short summary
This study derives a gridded dust emission dataset for 1841–2000 by employing a combination of observed dust from core records and reanalyzed global dust cycle constraints. We evaluate the ability of global models to replicate the observed historical dust variability by using the emission dataset to force a historical simulation in an Earth system model. We show that prescribing our emissions forces the model to better match observations than other mechanistic models.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
Atmos. Chem. Phys., 25, 2087–2121, https://doi.org/10.5194/acp-25-2087-2025, https://doi.org/10.5194/acp-25-2087-2025, 2025
Short summary
Short summary
We use the GEOS-Chem model to simulate aerosol distributions and properties over the western North Atlantic Ocean (WNAO) during the winter and summer deployments in 2020 of the NASA ACTIVATE mission. Model results are evaluated against aircraft, ground-based, and satellite observations. The improved understanding of life cycle, composition, transport pathways, and distribution of aerosols has important implications for characterizing aerosol–cloud–meteorology interactions over WNAO.
Mingrui Ma, Jiachen Cao, Dan Tong, Bo Zheng, and Yu Zhao
Atmos. Chem. Phys., 25, 2147–2166, https://doi.org/10.5194/acp-25-2147-2025, https://doi.org/10.5194/acp-25-2147-2025, 2025
Short summary
Short summary
We combined two global climate change pathways and three national emission control scenarios to analyze the future evolution of reactive nitrogen (Nr) deposition till the 2060s in China with air quality modeling. We show China’s clean air and carbon neutrality policies would overcome the adverse effects of climate change and efficiently reduce Nr deposition. The outflow of Nr fluxes from mainland China to the west Pacific would also be clearly reduced from continuous stringent emission controls.
Zhouyang Zhang, Jiandong Wang, Jiaping Wang, Nicole Riemer, Chao Liu, Yuzhi Jin, Zeyuan Tian, Jing Cai, Yueyue Cheng, Ganzhen Chen, Bin Wang, Shuxiao Wang, and Aijun Ding
Atmos. Chem. Phys., 25, 1869–1881, https://doi.org/10.5194/acp-25-1869-2025, https://doi.org/10.5194/acp-25-1869-2025, 2025
Short summary
Short summary
Black carbon (BC) exerts notable warming effects. We use a particle-resolved model to investigate the long-term behavior of the BC mixing state, revealing its compositions, coating thickness distribution, and optical properties all stabilize with a characteristic time of less than 1 d. This study can effectively simplify the description of the BC mixing state, which facilitates the precise assessment of the optical properties of BC aerosols in global and chemical transport models.
Qianyi Huo, Zhicong Yin, Xiaoqing Ma, and Huijun Wang
Atmos. Chem. Phys., 25, 1711–1724, https://doi.org/10.5194/acp-25-1711-2025, https://doi.org/10.5194/acp-25-1711-2025, 2025
Short summary
Short summary
Dust days during the spring seasons of 2015–2023 in North China were classified into Mongolian cyclone and cold high types depending on the presence of the Mongolian cyclone. The Mongolian cyclone type led to more frequent and severe dust weather, indicated by PM10 concentrations. To comprehensively forecast the two types of dust weather, a common predictor was established based on 500 hPa anomalous circulation systems, offering insights for dust weather forecasting and climate prediction.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes W. Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
Atmos. Chem. Phys., 25, 1545–1567, https://doi.org/10.5194/acp-25-1545-2025, https://doi.org/10.5194/acp-25-1545-2025, 2025
Short summary
Short summary
We compared smoke plume simulations from 11 global models to each other and to satellite smoke amount observations aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss rate assumptions vary enormously among models, causing uncertainties that require systematic in situ measurements to resolve.
Yongqing Bai, Tianliang Zhao, Kai Meng, Yue Zhou, Jie Xiong, Xiaoyun Sun, Lijuan Shen, Yanyu Yue, Yan Zhu, Weiyang Hu, and Jingyan Yao
Atmos. Chem. Phys., 25, 1273–1287, https://doi.org/10.5194/acp-25-1273-2025, https://doi.org/10.5194/acp-25-1273-2025, 2025
Short summary
Short summary
We proposed a composite statistical method to identify the quasi-weekly oscillation (QWO) of regional PM2.5 transport over China in winter from 2015 to 2019. The QWO of regional PM2.5 transport is constrained by synoptic-scale disturbances of the East Asian winter monsoon circulation with the periodic activities of the Siberian high, providing a new insight into the understanding of regional pollutant transport with meteorological drivers in atmospheric environment changes.
Léo Clauzel, Sandrine Anquetin, Christophe Lavaysse, Gilles Bergametti, Christel Bouet, Guillaume Siour, Rémy Lapere, Béatrice Marticorena, and Jennie Thomas
Atmos. Chem. Phys., 25, 997–1021, https://doi.org/10.5194/acp-25-997-2025, https://doi.org/10.5194/acp-25-997-2025, 2025
Short summary
Short summary
Solar energy production in West Africa is set to rise and needs accurate solar radiation estimates which are affected by desert dust. This work analyses a March 2021 dust event using a modelling strategy incorporating desert dust. Results show that considering desert dust cuts errors in solar radiation estimates by 75 % and reduces surface solar radiation by 18 %. This highlights the importance of incorporating dust aerosols into solar forecasting for better accuracy.
Ross J. Herbert, Alberto Sanchez-Marroquin, Daniel P. Grosvenor, Kirsty J. Pringle, Stephen R. Arnold, Benjamin J. Murray, and Kenneth S. Carslaw
Atmos. Chem. Phys., 25, 291–325, https://doi.org/10.5194/acp-25-291-2025, https://doi.org/10.5194/acp-25-291-2025, 2025
Short summary
Short summary
Aerosol particles that help form ice in clouds vary in number and type around the world and with time. However, in many weather and climate models cloud ice is not linked to aerosols that are known to nucleate ice. Here we report the first steps towards representing ice-nucleating particles within the UK Earth System Model. We conclude that in addition to ice nucleation by sea spray and mineral components of soil dust, we also need to represent ice nucleation by the organic components of soils.
Ryan Schmedding and Andreas Zuend
Atmos. Chem. Phys., 25, 327–346, https://doi.org/10.5194/acp-25-327-2025, https://doi.org/10.5194/acp-25-327-2025, 2025
Short summary
Short summary
Four different approaches for computing the interfacial tension between liquid phases in aerosol particles were tested for particles with diameters from 10 nm to more than 5 μm. Antonov's rule led to the strongest reductions in the onset relative humidity of liquid–liquid phase separation and reproduced measured interfacial tensions for highly immiscible systems. A modified form of the Butler equation was able to best reproduce measured interfacial tensions in more miscible systems.
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 13681–13692, https://doi.org/10.5194/acp-24-13681-2024, https://doi.org/10.5194/acp-24-13681-2024, 2024
Short summary
Short summary
A 2020 regulation has reduced sulfur emissions from shipping by about 80 %, leading to a decrease in atmospheric aerosols that have a cooling effect primarily by affecting cloud properties and amounts. Our climate model simulations predict a global temperature increase of 0.04 K over the next 3 decades as a result, which could contribute to surpassing the Paris Agreement's 1.5 °C target. Reduced aerosols may have also contributed to the recent temperature spikes.
Alcide Zhao, Laura J. Wilcox, and Claire L. Ryder
Atmos. Chem. Phys., 24, 13385–13402, https://doi.org/10.5194/acp-24-13385-2024, https://doi.org/10.5194/acp-24-13385-2024, 2024
Short summary
Short summary
Climate models include desert dust aerosols, which cause atmospheric heating and can change circulation patterns. We assess the effect of dust on the Indian and east Asian summer monsoons through multi-model experiments isolating the effect of dust in current climate models for the first time. Dust atmospheric heating results in a southward shift of western Pacific equatorial rainfall and an enhanced Indian summer monsoon. This shows the importance of accurate dust representation in models.
Ragnhild Bieltvedt Skeie, Rachael Byrom, Øivind Hodnebrog, Caroline Jouan, and Gunnar Myhre
Atmos. Chem. Phys., 24, 13361–13370, https://doi.org/10.5194/acp-24-13361-2024, https://doi.org/10.5194/acp-24-13361-2024, 2024
Short summary
Short summary
In 2020, new regulations by the International Maritime Organization regarding sulfur emissions came into force, reducing emissions of SO2 from the shipping sector by approximately 80 %. In this study, we use multiple models to calculate how much the Earth energy balance changed due to the emission reduction or the so-called effective radiative forcing. The calculated effective radiative forcing is weak, comparable to the effect of the increase in CO2 over the last 2 to 3 years.
Mingxu Liu, Hitoshi Matsui, Douglas S. Hamilton, Sagar D. Rathod, Kara D. Lamb, and Natalie M. Mahowald
Atmos. Chem. Phys., 24, 13115–13127, https://doi.org/10.5194/acp-24-13115-2024, https://doi.org/10.5194/acp-24-13115-2024, 2024
Short summary
Short summary
Atmospheric aerosol deposition provides bioavailable iron to promote marine primary production, yet the estimates of its fluxes remain highly uncertain. This study, by performing global aerosol simulations, demonstrates that iron-containing particle size upon emission is a critical factor in regulating soluble iron input to open oceans. Further observational constraints on this are needed to reduce modeling uncertainties.
Camelia Talianu, Jeni Vasilescu, Doina Nicolae, Alexandru Ilie, Andrei Dandocsi, Anca Nemuc, and Livio Belegante
EGUsphere, https://doi.org/10.5194/egusphere-2024-2930, https://doi.org/10.5194/egusphere-2024-2930, 2024
Short summary
Short summary
Bucharest, Romania's capital, has successfully used mobile measurements and mixed-effects LUR models to derive seasonal maps of near-surface PM10, NO2, and UFP. The data was collected during two intensive campaigns, covering high-traffic streets, residential, industrial, and commercial districts. The model's performance was evaluated, demonstrating its potential for high-resolution mapping in other cities with well-characterized urban structures and diverse in situ monitoring stations.
Jingmin Li, Mattia Righi, Johannes Hendricks, Christof G. Beer, Ulrike Burkhardt, and Anja Schmidt
Atmos. Chem. Phys., 24, 12727–12747, https://doi.org/10.5194/acp-24-12727-2024, https://doi.org/10.5194/acp-24-12727-2024, 2024
Short summary
Short summary
Aiming to understand underlying patterns and trends in aerosols, we characterize the spatial patterns and long-term evolution of lower tropospheric aerosols by clustering multiple aerosol properties from preindustrial times to the year 2050 under three Shared
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
Atmos. Chem. Phys., 24, 12643–12659, https://doi.org/10.5194/acp-24-12643-2024, https://doi.org/10.5194/acp-24-12643-2024, 2024
Short summary
Short summary
In March 2021, east Asia experienced an outbreak of severe dust storms after an absence of 1.5 decades. Here, we innovatively used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize dust emission and reproduce the dust storm. This work is valuable for not only the quantification of health damage, aviation risks, and profound impacts on the Earth's system but also revealing the climatic driving force and the process of desertification.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
Atmos. Chem. Phys., 24, 12509–12535, https://doi.org/10.5194/acp-24-12509-2024, https://doi.org/10.5194/acp-24-12509-2024, 2024
Short summary
Short summary
This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean–atmosphere–aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low-cloud fraction, decreasing the ocean and continental surface temperature and reducing the precipitation of coastal western Africa. It also highlights the role of the ocean temperature response and its feedbacks for the September–November season.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
Atmos. Chem. Phys., 24, 12341–12354, https://doi.org/10.5194/acp-24-12341-2024, https://doi.org/10.5194/acp-24-12341-2024, 2024
Short summary
Short summary
The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties. This method is verified from a theoretical perspective, and it performs well for thickly coated BC at high RHs.
Zijun Li, Angela Buchholz, and Noora Hyttinen
Atmos. Chem. Phys., 24, 11717–11725, https://doi.org/10.5194/acp-24-11717-2024, https://doi.org/10.5194/acp-24-11717-2024, 2024
Short summary
Short summary
Evaluating organosulfur (OS) hygroscopicity is important for assessing aerosol–cloud climate interactions in the post-fossil-fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with (NH4)2SO4. A good agreement was observed between their model-estimated and experimental HGFs.
Jamie R. Banks, Bernd Heinold, and Kerstin Schepanski
Atmos. Chem. Phys., 24, 11451–11475, https://doi.org/10.5194/acp-24-11451-2024, https://doi.org/10.5194/acp-24-11451-2024, 2024
Short summary
Short summary
The Aralkum is a new desert in Central Asia formed by the desiccation of the Aral Sea. This has created a source of atmospheric dust, with implications for the balance of solar and thermal radiation. Simulating these effects using a dust transport model, we find that Aralkum dust adds radiative cooling effects to the surface and atmosphere on average but also adds heating events. Increases in surface pressure due to Aralkum dust strengthen the Siberian High and weaken the summer Asian heat low.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen R. Arnold, Leighton A. Regayre, Meinrat O. Andreae, Mira L. Pöhlker, Duseong S. Jo, Man Yue, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 11365–11389, https://doi.org/10.5194/acp-24-11365-2024, https://doi.org/10.5194/acp-24-11365-2024, 2024
Short summary
Short summary
Highly oxygenated organic molecules (HOMs) play an important role in atmospheric new particle formation (NPF). By semi-explicitly coupling the chemical mechanism of HOMs and a comprehensive nucleation scheme in a global climate model, the updated model shows better agreement with measurements of nucleation rate, growth rate, and NPF event frequency. Our results reveal that HOM-driven NPF leads to a considerable increase in particle and cloud condensation nuclei burden globally.
Falei Xu, Shuang Wang, Yan Li, and Juan Feng
Atmos. Chem. Phys., 24, 10689–10705, https://doi.org/10.5194/acp-24-10689-2024, https://doi.org/10.5194/acp-24-10689-2024, 2024
Short summary
Short summary
This study examines how the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) affect dust activities in North China during the following spring. The results show that the NAO and ENSO, particularly in their negative phases, greatly influence dust activities. When both are negative, their combined effect on dust activities is even greater. This research highlights the importance of these climate patterns in predicting spring dust activities in North China.
Hengheng Zhang, Wei Huang, Xiaoli Shen, Ramakrishna Ramisetty, Junwei Song, Olga Kiseleva, Christopher Claus Holst, Basit Khan, Thomas Leisner, and Harald Saathoff
Atmos. Chem. Phys., 24, 10617–10637, https://doi.org/10.5194/acp-24-10617-2024, https://doi.org/10.5194/acp-24-10617-2024, 2024
Short summary
Short summary
Our study unravels how stagnant winter conditions elevate aerosol levels in Stuttgart. Cloud cover at night plays a pivotal role, impacting morning air quality. Validating a key model, our findings aid accurate air quality predictions, crucial for effective pollution mitigation in urban areas.
Giorgio Veratti, Alessandro Bigi, Michele Stortini, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 24, 10475–10512, https://doi.org/10.5194/acp-24-10475-2024, https://doi.org/10.5194/acp-24-10475-2024, 2024
Short summary
Short summary
In a study of two consecutive winter seasons, we used measurements and modelling tools to identify the levels and sources of black carbon pollution in a medium-sized urban area of the Po Valley, Italy. Our findings show that biomass burning and traffic-related emissions (especially from Euro 4 diesel cars) significantly contribute to BC concentrations. This research offers crucial insights for policymakers and urban planners aiming to improve air quality in cities.
Jiangtao Li, Xingqin An, Zhaobin Sun, Caihua Ye, Qing Hou, Yuxin Zhao, and Zhe Liu
EGUsphere, https://doi.org/10.5194/egusphere-2024-2000, https://doi.org/10.5194/egusphere-2024-2000, 2024
Short summary
Short summary
Climate change and pollution have intensified pollen allergies. We developed a pollen emissions model using phenology and random forests. Key factors affecting annual pollen emissions include temperature, relative humidity, and sunshine hours. Pollen dispersal starts around August 10, peaks around August 30, and ends by September 25, lasting about 45 days. Over time, annual pollen emissions exhibit significant fluctuations and a downward trend.
Pascal Lemaitre, Arnaud Quérel, Alexis Dépée, Alice Guerra Devigne, Marie Monier, Thibault Hiron, Chloé Soto Minguez, Daniel Hardy, and Andrea Flossmann
Atmos. Chem. Phys., 24, 9713–9732, https://doi.org/10.5194/acp-24-9713-2024, https://doi.org/10.5194/acp-24-9713-2024, 2024
Short summary
Short summary
A new in-cloud scavenging scheme is proposed. It is based on a microphysical model of cloud formation and may be applied to long-distance atmospheric transport models (> 100 km) and climatic models. This model is applied to the two most extreme precipitating cloud types in terms of both relative humidity and vertical extension: cumulonimbus and stratus.
Alex Rowell, James Brean, David C. S. Beddows, Tuukka Petäjä, Máté Vörösmarty, Imre Salma, Jarkko V. Niemi, Hanna E. Manninen, Dominik van Pinxteren, Thomas Tuch, Kay Weinhold, Zongbo Shi, and Roy M. Harrison
Atmos. Chem. Phys., 24, 9515–9531, https://doi.org/10.5194/acp-24-9515-2024, https://doi.org/10.5194/acp-24-9515-2024, 2024
Short summary
Short summary
Different sources of airborne particles in the atmospheres of four European cities were distinguished by recognising their particle size distributions using a statistical procedure, positive matrix factorisation. The various sources responded differently to the changes in emissions associated with COVID-19 lockdowns, and the reasons are investigated. While traffic emissions generally decreased, particles formed from reactions of atmospheric gases decreased in some cities but increased in others.
Amy H. Peace, Ying Chen, George Jordan, Daniel G. Partridge, Florent Malavelle, Eliza Duncan, and Jim M. Haywood
Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
Short summary
Short summary
Natural aerosols from volcanic eruptions can help us understand how anthropogenic aerosols modify climate. We use observations and model simulations of the 2014–2015 Holuhraun eruption plume to examine aerosol–cloud interactions in September 2014. We find a shift to clouds with smaller, more numerous cloud droplets in the first 2 weeks of the eruption. In the third week, the background meteorology and previous conditions experienced by air masses modulate the aerosol perturbation to clouds.
Hua Lu, Min Xie, Bingliang Zhuang, Danyang Ma, Bojun Liu, Yangzhihao Zhan, Tijian Wang, Shu Li, Mengmeng Li, and Kuanguang Zhu
Atmos. Chem. Phys., 24, 8963–8982, https://doi.org/10.5194/acp-24-8963-2024, https://doi.org/10.5194/acp-24-8963-2024, 2024
Short summary
Short summary
To identify cloud, aerosol, and planetary boundary layer (PBL) interactions from an air quality perspective, we summarized two pollution patterns characterized by denser liquid cloud and by obvious cloud radiation interaction (CRI). Numerical simulation experiments showed CRI could cause a 50 % reduction in aerosol radiation interaction (ARI) under a low-trough system. The results emphasized the nonnegligible role of CRI and its inhibition of ARI under wet and cloudy pollution synoptic patterns.
Zhe Song, Ningning Yao, Lang Chen, Yuhai Sun, Boqiong Jiang, Pengfei Li, Daniel Rosenfeld, and Shaocai Yu
EGUsphere, https://doi.org/10.5194/egusphere-2024-2263, https://doi.org/10.5194/egusphere-2024-2263, 2024
Short summary
Short summary
Our results with injected sea-salt aerosols for five open oceans show that the sea-salt aerosols with low injection amounts dominated the shortwave radiation mainly through the indirect effects. As indirect aerosol effects saturated with increasing injection rates, direct effects exceeded indirect effects. This implies that marine cloud brightening was best implemented in areas with extensive cloud cover, while the aerosol direct scattering effects remained dominant when clouds were scarce.
Yuzhi Jin, Jiandong Wang, David C. Wong, Chao Liu, Golam Sarwar, Kathleen M. Fahey, Shang Wu, Jiaping Wang, Jing Cai, Zeyuan Tian, Zhouyang Zhang, Jia Xing, Aijun Ding, and Shuxiao Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2372, https://doi.org/10.5194/egusphere-2024-2372, 2024
Short summary
Short summary
Black carbon (BC) affects climate and the environment, and its aging process alters its properties. Current models, like WRF-CMAQ, lack full account. We developed the WRF-CMAQ-BCG model to better represent BC aging by introducing Bare/Coated BC species and their conversion. Our findings show that BC mixing states have distinct spatiotemporal distribution characteristics, and BC wet deposition is dominated by Coated BC. Accounting for BC aging process improves aerosol optics simulation accuracy.
Emilie Fons, Ann Kristin Naumann, David Neubauer, Theresa Lang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 8653–8675, https://doi.org/10.5194/acp-24-8653-2024, https://doi.org/10.5194/acp-24-8653-2024, 2024
Short summary
Short summary
Aerosols can modify the liquid water path (LWP) of stratocumulus and, thus, their radiative effect. We compare storm-resolving model and satellite data that disagree on the sign of LWP adjustments and diagnose this discrepancy with causal inference. We find that strong precipitation, the absence of wet scavenging, and cloud deepening under a weak inversion contribute to positive LWP adjustments to aerosols in the model, despite weak negative effects from cloud-top entrainment enhancement.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
Atmos. Chem. Phys., 24, 8489–8506, https://doi.org/10.5194/acp-24-8489-2024, https://doi.org/10.5194/acp-24-8489-2024, 2024
Short summary
Short summary
The study examines how the volatility of semi-volatile organic compounds affects secondary organic aerosol (SOA) formation and climate. Our simulations show that uncertainties in these volatilities influence aerosol mass and climate impacts. Accurate representation of these compounds in climate models is crucial for predicting global climate patterns.
Hector Navarro-Barboza, Jordi Rovira, Vincenzo Obiso, Andrea Pozzer, Marta Via, Andres Alastuey, Xavier Querol, Noemi Perez, Marjan Savadkoohi, Gang Chen, Jesus Yus-Díez, Matic Ivancic, Martin Rigler, Konstantinos Eleftheriadis, Stergios Vratolis, Olga Zografou, Maria Gini, Benjamin Chazeau, Nicolas Marchand, Andre Prevot, Kaspar Dallenbach, Mikael Ehn, Krista Luoma, Tuukka Petäjä, Anna Tobler, Jaroslaw Necki, Minna Aurela, Hilkka Timonen, Jarkko Niemi, Olivier Favez, Jean-Eudes Petit, Jean-Philippe Putaud, Christoph Hueglin, Nicolas Pascal, Aurelien Chauvigné, Sebastien Conil, Marco Pandolfi, and Oriol Jorba
EGUsphere, https://doi.org/10.5194/egusphere-2024-2086, https://doi.org/10.5194/egusphere-2024-2086, 2024
Short summary
Short summary
Brown carbon (BrC) absorbs UV and visible light, affecting climate. Our study investigates BrC's imaginary refractive index (k ) using data from 12 European sites. Residential emissions are a major OA source in winter, while secondary organic aerosols (SOA) dominate in summer. We derived source-specific k values, enhancing model accuracy. This research improves understanding of BrC's climate role, emphasizing the need for source-specific constraints in atmospheric models.
Ruth A. R. Digby, Knut von Salzen, Adam H. Monahan, Nathan P. Gillett, and Jiangnan Li
EGUsphere, https://doi.org/10.5194/egusphere-2024-1796, https://doi.org/10.5194/egusphere-2024-1796, 2024
Short summary
Short summary
The refractive index of black carbon (BCRI), which determines how much energy black carbon absorbs and scatters, is difficult to measure and different climate models use different values. We show that varying the BCRI across commonly used values can increase absorbing aerosol optical depth by 42 % and the warming effect from interactions between black carbon and radiation by 47 %, an appreciable fraction of the overall spread between models reported in recent literature assessments.
Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, Chaincy Kuo, Sophie Szopa, Pierre Nabat, Dirk Olivié, Twan van Noije, Philippe Le Sager, David Neubauer, Naga Oshima, Jane Mulcahy, Larry W. Horowitz, and Prodromos Zanis
Atmos. Chem. Phys., 24, 7837–7872, https://doi.org/10.5194/acp-24-7837-2024, https://doi.org/10.5194/acp-24-7837-2024, 2024
Short summary
Short summary
Effective radiative forcing (ERF) is a metric for estimating how human activities and natural agents change the energy flow into and out of the Earth’s climate system. We investigate the anthropogenic aerosol ERF, and we estimate the contribution of individual processes to the total ERF using simulations from Earth system models within the Coupled Model Intercomparison Project Phase 6 (CMIP6). Our findings highlight that aerosol–cloud interactions drive ERF variability during the last 150 years.
Qianqian Song, Paul Ginoux, María Gonçalves Ageitos, Ron L. Miller, Vincenzo Obiso, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7421–7446, https://doi.org/10.5194/acp-24-7421-2024, https://doi.org/10.5194/acp-24-7421-2024, 2024
Short summary
Short summary
We implement and simulate the distribution of eight dust minerals in the GFDL AM4.0 model. We found that resolving the eight minerals reduces dust absorption compared to the homogeneous dust used in the standard GFDL AM4.0 model that assumes a globally uniform hematite content of 2.7 % by volume. Resolving dust mineralogy results in significant impacts on radiation, land surface temperature, surface winds, and precipitation over North Africa in summer.
Senyi Kong, Zheng Wang, and Lei Bi
Atmos. Chem. Phys., 24, 6911–6935, https://doi.org/10.5194/acp-24-6911-2024, https://doi.org/10.5194/acp-24-6911-2024, 2024
Short summary
Short summary
The retrieval of refractive indices of dust aerosols from laboratory optical measurements is commonly done assuming spherical particles. This paper aims to investigate the uncertainties in the shortwave refractive indices and corresponding optical properties by considering non-spherical and inhomogeneous models for dust samples. The study emphasizes the significance of using non-spherical models for simulating dust aerosols.
Wenxuan Hua, Sijia Lou, Xin Huang, Lian Xue, Ke Ding, Zilin Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 6787–6807, https://doi.org/10.5194/acp-24-6787-2024, https://doi.org/10.5194/acp-24-6787-2024, 2024
Short summary
Short summary
In this study, we diagnose uncertainties in carbon monoxide and organic carbon emissions from four inventories for seven major wildfire-prone regions. Uncertainties in vegetation classification methods, fire detection products, and cloud obscuration effects lead to bias in these biomass burning (BB) emission inventories. By comparing simulations with measurements, we provide certain inventory recommendations. Our study has implications for reducing uncertainties in emissions in further studies.
Chandrakala Bharali, Mary Barth, Rajesh Kumar, Sachin D. Ghude, Vinayak Sinha, and Baerbel Sinha
Atmos. Chem. Phys., 24, 6635–6662, https://doi.org/10.5194/acp-24-6635-2024, https://doi.org/10.5194/acp-24-6635-2024, 2024
Short summary
Short summary
This study examines the role of atmospheric aerosols in winter fog over the Indo-Gangetic Plains of India using WRF-Chem. The increase in RH with aerosol–radiation feedback (ARF) is found to be important for fog formation as it promotes the growth of aerosols in the polluted environment. Aqueous-phase chemistry in the fog increases PM2.5 concentration, further affecting ARF. ARF and aqueous-phase chemistry affect the fog intensity and the timing of fog formation by ~1–2 h.
Wenxin Zhao, Yu Zhao, Yu Zheng, Dong Chen, Jinyuan Xin, Kaitao Li, Huizheng Che, Zhengqiang Li, Mingrui Ma, and Yun Hang
Atmos. Chem. Phys., 24, 6593–6612, https://doi.org/10.5194/acp-24-6593-2024, https://doi.org/10.5194/acp-24-6593-2024, 2024
Short summary
Short summary
We evaluate the long-term (2000–2020) variabilities of aerosol absorption optical depth, black carbon emissions, and associated health risks in China with an integrated framework that combines multiple observations and modeling techniques. We demonstrate the remarkable emission abatement resulting from the implementation of national pollution controls and show how human activities affected the emissions with a spatiotemporal heterogeneity, thus supporting differentiated policy-making by region.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
Short summary
Short summary
The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc E. J. Stettler
Atmos. Chem. Phys., 24, 6071–6093, https://doi.org/10.5194/acp-24-6071-2024, https://doi.org/10.5194/acp-24-6071-2024, 2024
Short summary
Short summary
The radiative forcing (RF) due to aviation contrails is comparable to that caused by CO2. We estimate that global contrail net RF in 2019 was 62.1 mW m−2. This is ~1/2 the previous best estimate for 2018. Contrail RF varies regionally due to differences in conditions required for persistent contrails. COVID-19 reduced contrail RF by 54% in 2020 relative to 2019. Globally, 2 % of all flights account for 80 % of the annual contrail energy forcing, suggesting a opportunity to mitigate contrail RF.
Haotian Zu, Biwu Chu, Yiqun Lu, Ling Liu, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 5823–5835, https://doi.org/10.5194/acp-24-5823-2024, https://doi.org/10.5194/acp-24-5823-2024, 2024
Short summary
Short summary
The nucleation of iodic acid (HIO3) and iodous acid (HIO2) was proven to be critical in marine areas. However, HIO3–HIO2 nucleation cannot effectively derive the rapid nucleation in some polluted coasts. We find a significant enhancement of dimethylamine (DMA) on the HIO3–HIO2 nucleation in marine and polar regions with abundant DMA sources, which may establish reasonable connections between the HIO3–HIO2 nucleation and the rapid formation of new particles in polluted marine and polar regions.
Junghwa Lee, Patric Seifert, Tempei Hashino, Maximilian Maahn, Fabian Senf, and Oswald Knoth
Atmos. Chem. Phys., 24, 5737–5756, https://doi.org/10.5194/acp-24-5737-2024, https://doi.org/10.5194/acp-24-5737-2024, 2024
Short summary
Short summary
Spectral bin model simulations of an idealized supercooled stratiform cloud were performed with the AMPS model for variable CCN and INP concentrations. We performed radar forward simulations with PAMTRA to transfer the simulations into radar observational space. The derived radar reflectivity factors were compared to observational studies of stratiform mixed-phase clouds. These studies report a similar response of the radar reflectivity factor to aerosol perturbations as we found in our study.
Basudev Swain, Marco Vountas, Aishwarya Singh, Nidhi L. Anchan, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Sachin S. Gunthe, Hartmut Bösch, and John P. Burrows
Atmos. Chem. Phys., 24, 5671–5693, https://doi.org/10.5194/acp-24-5671-2024, https://doi.org/10.5194/acp-24-5671-2024, 2024
Short summary
Short summary
Arctic amplification (AA) accelerates the warming of the central Arctic cryosphere and affects aerosol dynamics. Limited observations hinder a comprehensive analysis. This study uses AEROSNOW aerosol optical density (AOD) data and GEOS-Chem simulations to assess AOD variability. Discrepancies highlight the need for improved observational integration into models to refine our understanding of aerosol effects on cloud microphysics, ice nucleation, and radiative forcing under evolving AA.
Vincenzo Obiso, María Gonçalves Ageitos, Carlos Pérez García-Pando, Jan P. Perlwitz, Gregory L. Schuster, Susanne E. Bauer, Claudia Di Biagio, Paola Formenti, Kostas Tsigaridis, and Ron L. Miller
Atmos. Chem. Phys., 24, 5337–5367, https://doi.org/10.5194/acp-24-5337-2024, https://doi.org/10.5194/acp-24-5337-2024, 2024
Short summary
Short summary
We calculate the dust direct radiative effect (DRE) in an Earth system model accounting for regionally varying soil mineralogy through a new observationally constrained method. Linking dust absorption at solar wavelengths to the varying amount of specific minerals (i.e., iron oxides) improves the modeled range of dust single scattering albedo compared to observations and increases the global cooling by dust. Our results may contribute to improved estimates of the dust DRE and its climate impact.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
Short summary
Short summary
Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Xiaoli Wei, Qian Cui, Leiming Ma, Feng Zhang, Wenwen Li, and Peng Liu
Atmos. Chem. Phys., 24, 5025–5045, https://doi.org/10.5194/acp-24-5025-2024, https://doi.org/10.5194/acp-24-5025-2024, 2024
Short summary
Short summary
A new aerosol-type classification algorithm has been proposed. It includes an optical database built by Mie scattering and a complex refractive index working as a baseline to identify different aerosol types. The new algorithm shows high accuracy and efficiency. Hence, a global map of aerosol types was generated to characterize aerosol types across the five continents. It will help improve the accuracy of aerosol inversion and determine the sources of aerosol pollution.
Cited articles
Albani, S., Mahowald, N. M., Perry, A. T., Scanza, R. A., Zender, C. S.,
Heavens, N. G., Maggi, V., Kok, J. F., and Otto-Bliesner, B. L.: Improved
dust representation in the Community Atmosphere Model, J. Adv. Model. Earth
Syst., 6, 541–570, https://doi.org/10.1002/2013MS000279, 2014.
Arimoto, R., Duce, R. A., Ray, B. J., Ellis Jr, W. G., Cullen, J. D., and
Merrill, J. T.: Trace elements in the atmosphere over the North Atlantic, J.
Geophys. Res.-Atmos., 100, 1199–1213,
https://doi.org/10.1029/94JD02618, 1995.
Arnalds, O., Dagsson-Waldhauserova, P., and Olafsson, H.: The Icelandic
volcanic aeolian environment: Processes and impacts – A review, Aeolian
Res., 20, 176–195, https://doi.org/10.1016/j.aeolia.2016.01.004, 2016.
Atkinson, J. D., Murray, B. J., Woodhouse, M. T., Whale, T. F., Baustian, K.
J., Carslaw, K. S., Dobbie, S., O'Sullivan, D., and Malkin, T. L.: The
importance of feldspar for ice nucleation by mineral dust in mixed-phase
clouds, Nature, 498, 355–358, https://doi.org/10.1038/nature12278, 2013.
Baddock, M. C., Mockford, T., Bullard, J. E., and Thorsteinsson, T.:
Pathways of high-latitude dust in the North Atlantic, Earth Planet. Sci.
Lett., 459, 170–182, https://doi.org/10.1016/j.epsl.2016.11.034, 2017.
Bogenschutz, P. A., Gettelman, A., Morrison, H., Larson, V. E., Craig, C.,
and Schanen, D. P.: Higher-order turbulence closure and its impact on
climate simulations in the community atmosphere model, J. Climate, 26,
9655–9676, https://doi.org/10.1175/JCLI-D-13-00075.1, 2013.
Boose, Y., Sierau, B., García, M. I., Rodríguez, S., Alastuey, A., Linke, C., Schnaiter, M., Kupiszewski, P., Kanji, Z. A., and Lohmann, U.: Ice nucleating particles in the Saharan Air Layer, Atmos. Chem. Phys., 16, 9067–9087, https://doi.org/10.5194/acp-16-9067-2016, 2016.
Bory, A. J.-M., Biscaye, P. E., Svensson, A., and Grousset, F. E.: Seasonal
variability in the origin of recent atmospheric mineral dust at NorthGRIP,
Greenland, Earth Planet. Sci. Lett., 196, 123–134,
https://doi.org/10.1016/S0012-821X(01)00609-4, 2002.
Bory, A. J.-M., Biscaye, P. E., and Grousset, F. E.: Two distinct seasonal
Asian source regions for mineral dust deposited in Greenland (NorthGRIP),
Geophys. Res. Lett., 30, 1167, https://doi.org/10.1029/2002GL016446, 2003.
Breider, T. J., Mickley, L. J., Jacob, D. J., Wang, Q., Fisher, J. A.,
Chang, R. Y.-W., and Alexander, B.: Annual distributions and sources of
Arctic aerosol components, aerosol optical depth, and aerosol absorption, J.
Geophys. Res.-Atmos., 119, 4107–4124, https://doi.org/10.1002/2013JD020996,
2014.
Bullard, J. E.: The distribution and biogeochemical importance of
high-latitude dust in the Arctic and Southern Ocean-Antarctic regions, J.
Geophys. Res.-Atmos., 122, 3098–3103, https://doi.org/10.1002/2016JD026363,
2017.
Bullard, J. E. and Austin, M. J.: Dust generation on a proglacial
floodplain, West Greenland, Aeolian Res., 3, 43–54,
https://doi.org/10.1016/j.aeolia.2011.01.002, 2011.
Bullard, J. E., Baddock, M., Bradwell, T., Crusius, J., Darlington, E.,
Gaiero, D., Gassó, S., Gisladottir, G., Hodgkins, R., McCulloch, R.,
McKenna-Neuman, C., Mockford, T., Stewart, H., and Thorsteinsson, T.:
High-latitude dust in the Earth system, Rev. Geophys., 54, 447–485,
https://doi.org/10.1002/2016RG000518, 2016.
Creamean, J. M., Kirpes, R. M., Pratt, K. A., Spada, N. J., Maahn, M., de Boer, G., Schnell, R. C., and China, S.: Marine and terrestrial influences on ice nucleating particles during continuous springtime measurements in an Arctic oilfield location, Atmos. Chem. Phys., 18, 18023–18042, https://doi.org/10.5194/acp-18-18023-2018, 2018.
Creamean, J. M., Hill, T. C. J., DeMott, P. J., Uetake, J., Kreidenweis, S.,
and Douglas, T. A.: Thawing permafrost: an overlooked source of seeds for
Arctic cloud formation, Environ. Res. Lett., 15, 084022,
https://doi.org/10.1088/1748-9326/ab87d3, 2020.
Crusius, J., Schroth, A. W., Gassó, S., Moy, C. M., Levy, R. C., and
Gatica, M.: Glacial flour dust storms in the Gulf of Alaska: Hydrologic and
meteorological controls and their importance as a source of bioavailable
iron, Geophys. Res. Lett., 38, L06602, https://doi.org/10.1029/2010GL046573,
2011.
Dagsson-Waldhauserova, P., Arnalds, O., and Olafsson, H.: Long-term variability of dust events in Iceland (1949–2011), Atmos. Chem. Phys., 14, 13411–13422, https://doi.org/10.5194/acp-14-13411-2014, 2014.
de Boer, G., Morrison, H., Shupe, M. D., and Hildner, R.: Evidence of liquid
dependent ice nucleation in high-latitude stratiform clouds from surface
remote sensors, Geophys. Res. Lett., 38, L01803,
https://doi.org/10.1029/2010GL046016, 2011.
DeMott, P. J., Sassen, K., Poellot, M. R., Baumgardner, D., Rogers, D. C.,
Brooks, S. D., Prenni, A. J., and Kreidenweis, S. M.: African dust aerosols
as atmospheric ice nuclei, Geophys. Res. Lett., 30, 1732,
https://doi.org/10.1029/2003GL017410, 2003.
DeMott, P. J., Prenni, A. J., Liu, X., Kreidenweis, S. M., Petters, M. D.,
Twohy, C. H., Richardson, M. S., Eidhammer, T., and Rogers, D. C.:
Predicting global atmospheric ice nuclei distributions and their impacts on
climate, P. Natl. Acad. Sci. USA, 107, 11217–11222,
https://doi.org/10.1073/pnas.0910818107, 2010.
DeMott, P. J., Prenni, A. J., McMeeking, G. R., Sullivan, R. C., Petters, M. D., Tobo, Y., Niemand, M., Möhler, O., Snider, J. R., Wang, Z., and Kreidenweis, S. M.: Integrating laboratory and field data to quantify the immersion freezing ice nucleation activity of mineral dust particles, Atmos. Chem. Phys., 15, 393–409, https://doi.org/10.5194/acp-15-393-2015, 2015.
Dong, X., Xi, B., Crosby, K., Long, C. N., Stone, R. S., and Shupe, M. D.: A
10 year climatology of Arctic cloud fraction and radiative forcing at
Barrow, Alaska, J. Geophys. Res.-Atmos., 115, D17212,
https://doi.org/10.1029/2009JD013489, 2010.
Dörnbrack, A., Stachlewska, I. S., Ritter, C., and Neuber, R.: Aerosol distribution around Svalbard during intense easterly winds, Atmos. Chem. Phys., 10, 1473–1490, https://doi.org/10.5194/acp-10-1473-2010, 2010.
E3SM Project: Energy Exascale Earth System Model v1.0, Computer Software, E3SM Project, DOE [code], https://doi.org/10.11578/E3SM/dc.20180418.36, 2018.
Fan, S.-M.: Modeling of observed mineral dust aerosols in the arctic and the impact on winter season low-level clouds, J. Geophys. Res.-Atmos., 118, 11161–11174, https://doi.org/10.1002/jgrd.50842, 2013.
Fenn, R. W. and Weickmann, H. K.: Some results of aerosol measurements,
Geofisica Pura e Applicata, 42, 53–61, https://doi.org/10.1007/BF02113389,
1959.
Gelaro, R., McCarty, W., Suárez, M. J., Todling, R., Molod, A., Takacs, L., Randles, C. A., Darmenov, A., Bosilovich, M. G., Reichle, R., Wargan, K., Coy, L., Cullather, R., Draper, C., Akella, S., Buchard, V., Conaty, A., Silva, A. M. da, Gu, W., Kim, G.-K., Koster, R., Lucchesi, R., Merkova, D., Nielsen, J. E., Partyka, G., Pawson, S., Putman, W., Rienecker, M., Schubert, S. D., Sienkiewicz, M., and Zhao, B.: The Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2), J. Climate, 30, 5419–5454, https://doi.org/10.1175/JCLI-D-16-0758.1, 2017.
Gettelman, A. and Morrison, H.: Advanced two-moment bulk microphysics for
global models. Part I: off-line tests and comparison with other schemes, J. Climate, 28, 1268–1287, https://doi.org/10.1175/JCLI-D-14-00102.1, 2015.
Ghan, S. J. and Zaveri, R. A.: Parameterization of optical properties for
hydrated internally mixed aerosol, J. Geophys. Res., 112, D10201,
https://doi.org/10.1029/2006JD007927, 2007.
Ginoux, P., Chin, M., Tegen, I., Prospero, J. M., Holben, B., Dubovik, O.,
and Lin, S.-J.: Sources and distributions of dust aerosols simulated with
the GOCART model, J. Geophys. Res., 106, 20255–20273,
https://doi.org/10.1029/2000JD000053, 2001.
Golaz, J.-C., Larson, V. E., and Cotton, W. R.: A PDF-based model for
boundary layer clouds. Part I: Method and model description, J. Atmos. Sci.,
59, 3540–3551, https://doi.org/10.1175/1520-0469(2002)059<3540:APBMFB>2.0.CO;2, 2002.
Groot Zwaaftink, C. D., Grythe, H., Skov, H., and Stohl, A.: Substantial
contribution of northern high-latitude sources to mineral dust in the
Arctic, J. Geophys. Res.-Atmos., 121, 13678–13697,
https://doi.org/10.1002/2016JD025482, 2016.
Hiranuma, N., Brooks, S. D., Moffet, R. C., Glen, A., Laskin, A., Gilles, M.
K.m Liu, P., Macdonald, A. M., Strapp, J. W., and McFarquhar, G. M: Chemical
characterization of individual particles and residuals of cloud droplets and
ice crystals collected on board research aircraft in the ISDAC 2008 study,
J. Geophys. Res.-Atmos., 118, 6564–6579, https://doi.org/10.1002/jgrd.50484,
2013.
Hofer, S., Tedstone, A. J., Fettweis, X., and Bamber, J. L.: Cloud
microphysics and circulation anomalies control differences in future
Greenland melt, Nat. Clim. Chang., 9, 523–528,
https://doi.org/10.1038/s41558-019-0507-8, 2019.
Holben, B. N., Eck, T. F., Slutsker, I., Tanré, D., Buis, J. P., Setzer,
A., Vermote, E., Reagan, J. A., Kaufman, Y. J., Nakajima, T., Lavenu, F.,
Jankowiak, I., and Smirnov, A.: AERONET – A Federated Instrument Network and
Data Archive for Aerosol Characterization, Remote Sens. Environ., 66, 1–16,
https://doi.org/10.1016/S0034-4257(98)00031-5, 1998.
Hoose, C. and Möhler, O.: Heterogeneous ice nucleation on atmospheric aerosols: a review of results from laboratory experiments, Atmos. Chem. Phys., 12, 9817–9854, https://doi.org/10.5194/acp-12-9817-2012, 2012.
Hoose, C., Kristjánsson, J. E., Chen, J.-P., and Hazra, A.: A classical-theory-based parameterization of heterogeneous ice nucleation by mineral dust, soot, and biological particles in a global climate model, J. Atmos. Sci., 67, 2483–2503, https://doi.org/10.1175/2010JAS3425.1, 2010.
Huang, Z., Huang, J., Hayasaka, T., Wang, S., Zhou, T., and Jin, H.:
Short-cut transport path for Asian dust directly to the Arctic: a case
study, Environ. Res. Lett., 10, 114018,
https://doi.org/10.1088/1748-9326/10/11/114018, 2015.
Huneeus, N., Schulz, M., Balkanski, Y., Griesfeller, J., Prospero, J., Kinne, S., Bauer, S., Boucher, O., Chin, M., Dentener, F., Diehl, T., Easter, R., Fillmore, D., Ghan, S., Ginoux, P., Grini, A., Horowitz, L., Koch, D., Krol, M. C., Landing, W., Liu, X., Mahowald, N., Miller, R., Morcrette, J.-J., Myhre, G., Penner, J., Perlwitz, J., Stier, P., Takemura, T., and Zender, C. S.: Global dust model intercomparison in AeroCom phase I, Atmos. Chem. Phys., 11, 7781–7816, https://doi.org/10.5194/acp-11-7781-2011, 2011 (data available at: https://aerocom-classic.met.no/DATA/download/DUST_BENCHMARK_HUNEEUS2011/, last access: December 2018).
Irish, V. E., Hanna, S. J., Willis, M. D., China, S., Thomas, J. L., Wentzell, J. J. B., Cirisan, A., Si, M., Leaitch, W. R., Murphy, J. G., Abbatt, J. P. D., Laskin, A., Girard, E., and Bertram, A. K.: Ice nucleating particles in the marine boundary layer in the Canadian Arctic during summer 2014, Atmos. Chem. Phys., 19, 1027–1039, https://doi.org/10.5194/acp-19-1027-2019, 2019.
Jacob, D. J., Crawford, J. H., Maring, H., Clarke, A. D., Dibb, J. E., Emmons, L. K., Ferrare, R. A., Hostetler, C. A., Russell, P. B., Singh, H. B., Thompson, A. M., Shaw, G. E., McCauley, E., Pederson, J. R., and Fisher, J. A.: The Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) mission: design, execution, and first results, Atmos. Chem. Phys., 10, 5191–5212, https://doi.org/10.5194/acp-10-5191-2010, 2010.
Kato, S., Rose, F. G., Rutan, D. A., Thorsen, T. E., Loeb, N. G., Doelling,
D. R., Huang, X., Smith, W. L., Su, W., and Ham, S.-H.: Surface irradiances
of Edition 4.0 Clouds and the Earth's Radiant Energy System (CERES) Energy
Balanced and Filled (EBAF) data product, J. Climate, 31, 4501–4527,
https://doi.org/10.1175/JCLI-D-17-0523.1, 2018.
Khanal, S., Wang, Z., and French, J. R.: Improving middle and high latitude
cloud liquid water path measurements from MODIS, Atmos. Res., 243, 105033,
https://doi.org/10.1016/j.atmosres.2020.105033, 2020.
Kinne, S., Schulz, M., Textor, C., Guibert, S., Balkanski, Y., Bauer, S. E., Berntsen, T., Berglen, T. F., Boucher, O., Chin, M., Collins, W., Dentener, F., Diehl, T., Easter, R., Feichter, J., Fillmore, D., Ghan, S., Ginoux, P., Gong, S., Grini, A., Hendricks, J., Herzog, M., Horowitz, L., Isaksen, I., Iversen, T., Kirkevåg, A., Kloster, S., Koch, D., Kristjansson, J. E., Krol, M., Lauer, A., Lamarque, J. F., Lesins, G., Liu, X., Lohmann, U., Montanaro, V., Myhre, G., Penner, J., Pitari, G., Reddy, S., Seland, O., Stier, P., Takemura, T., and Tie, X.: An AeroCom initial assessment – optical properties in aerosol component modules of global models, Atmos. Chem. Phys., 6, 1815–1834, https://doi.org/10.5194/acp-6-1815-2006, 2006.
Kohfeld, K. E. and Harrison, S. P.: DIRTMAP: the geological record of dust,
Earth-Sci. Rev., 54, 81–114, https://doi.org/10.1016/S0012-8252(01)00042-3,
2001.
Kok, J. F.: A scaling theory for the size distribution of emitted dust
aerosols suggests climate models underestimate the size of the global dust
cycle, P. Natl. Acad. Sci. USA, 108, 1016–1021,
https://doi.org/10.1073/pnas.1014798108, 2011.
Kok, J. F., Mahowald, N. M., Fratini, G., Gillies, J. A., Ishizuka, M., Leys, J. F., Mikami, M., Park, M.-S., Park, S.-U., Van Pelt, R. S., and Zobeck, T. M.: An improved dust emission model – Part 1: Model description and comparison against measurements, Atmos. Chem. Phys., 14, 13023–13041, https://doi.org/10.5194/acp-14-13023-2014, 2014a.
Kok, J. F., Albani, S., Mahowald, N. M., and Ward, D. S.: An improved dust emission model – Part 2: Evaluation in the Community Earth System Model, with implications for the use of dust source functions, Atmos. Chem. Phys., 14, 13043–13061, https://doi.org/10.5194/acp-14-13043-2014, 2014b.
Kok, J. F., Ridley, D. A., Zhou, Q., Miller, R. L., Zhao, C., Heald, C. L.,
Ward, D. S., Albani, S., and Haustein, K.: Smaller desert dust cooling
effect estimated from analysis of dust size and abundance, Nat. Geosci., 10,
274–278, https://doi.org/10.1038/ngeo2912, 2017.
Kulkarni, G., Sanders, C., Zhang, K., Liu, X., and Zhao, C.: Ice nucleation
of bare and sulfuric acid-coated mineral dust particles and implication for
cloud properties, J. Geophys. Res.-Atmos., 119, 9993–10011, https://doi.org/10.1002/2014JD021567,
2014.
Larson, V. E., Golaz, J.-C., and Cotton, W. R.: Small-Scale and Mesoscale
Variability in Cloudy Boundary Layers: Joint Probability Density Functions,
J. Atmos. Sci., 59, 3519–3539,
https://doi.org/10.1175/1520-0469(2002)059<3519:SSAMVI>2.0.CO;2, 2002.
Liu, X., Xie, S., Boyle, J., Klein, S. A., Shi, X., Wang, Z., Lin, W., Ghan,
S. J., Earle, M., Liu, P. S. K., and Zelenyuk, A.: Testing cloud
microphysics parameterizations in NCAR CAM5 with ISDAC and M-PACE
observations, J. Geophys. Res., 116, D00T11,
https://doi.org/10.1029/2011JD015889, 2011.
Liu, X., Ma, P.-L., Wang, H., Tilmes, S., Singh, B., Easter, R. C., Ghan, S. J., and Rasch, P. J.: Description and evaluation of a new four-mode version of the Modal Aerosol Module (MAM4) within version 5.3 of the Community Atmosphere Model, Geosci. Model Dev., 9, 505–522, https://doi.org/10.5194/gmd-9-505-2016, 2016.
Loeb, N. G., Doelling, D. R., Wang, H., Su, W., Nguyen, C., Corbett, J. G.,
Liang, L., Mitrescu, C., Rose, F. G., and Kato, S.: Clouds and the Earth's
Radiant Energy System (CERES) Energy Balanced and Filled (EBAF)
Top-of-Atmosphere (TOA) Edition-4.0 Data Product, J. Climate, 31, 895–918,
https://doi.org/10.1175/JCLI-D-17-0208.1, 2018.
Luo, C., Mahowald, N. M., and Corral, J. del: Sensitivity study of
meteorological parameters on mineral aerosol mobilization, transport, and
distribution, J. Geophys. Res., 108, 4447,
https://doi.org/10.1029/2003JD003483, 2003.
Luo, T., Wang, Z., Ferrare, R. A., Hostetler, C. A., Yuan, R., and Zhang,
D.: Vertically resolved separation of dust and other aerosol types by a new
lidar depolarization method, Opt. Express, 23, 14095–14107,
https://doi.org/10.1364/OE.23.014095, 2015a.
Luo, T., Wang, Z., Zhang, D., Liu, X., Wang, Y., and Yuan, R.: Global dust
distribution from improved thin dust layer detection using A-train satellite
lidar observations, Geophys. Res. Lett., 42, 620–628,
https://doi.org/10.1002/2014GL062111, 2015b.
Maenhaut, W., Fernandez-Jimenez, M.-T., Rajta, I., Dubtsov, S., Meixner, F.
X., Andreae, M. O., Torr, S., Hargrove, J. W., Chimanga, P., and Mlambo, J.:
Long-term aerosol composi- tion measruments and source apportionment at
Rukomechi, Zimbabwe, J. Aerosol Sci., 31, S469–S470, 2000a.
Maenhaut, W., Fernandez-Jimenez, M.-T., Vanderzalm, J. L., Hooper, B. M.,
Hooper, M. A., and Tapper, N. J.: Aerosol composition at Jabiru, Australia
and impact of biomass burning, J. Aerosol Sci., 31, S745–S746,
2000b.
Mahowald, N. M., Engelstaedter, S., Luo, C., Sealy, A., Artaxo, P.,
Benitez-Nelson, C., Bonnet, S., Chen, Y., Chuang, P. Y., Cohen, D. D.,
Dulac, F., Herut, B., Johansen, A. M., Kubilay, N., Losno, R., Maenhaut, W.,
Paytan, A., Prospero, J. M., Shank, L. M., and Siefert, R. L.: Atmospheric
iron deposition: global distribution, variability, and human perturbations,
Ann. Rev. Mar. Sci., 1, 245–278,
https://doi.org/10.1146/annurev.marine.010908.163727, 2009.
Malm, W. C., Sisler, J. F., Huffman, D., Eldred, R. A., and Cahill, T. A.: Spatial and seasonal trends in particle concentration and optical extinction in the United States, J. Geophys. Res.-Atmos., 99, 1347–1370, https://doi.org/10.1029/93JD02916, 1994 (data available at: http://vista.cira.colostate.edu/Improve/data-page/, last access: January 2021).
Mason, R. H., Si, M., Chou, C., Irish, V. E., Dickie, R., Elizondo, P., Wong, R., Brintnell, M., Elsasser, M., Lassar, W. M., Pierce, K. M., Leaitch, W. R., MacDonald, A. M., Platt, A., Toom-Sauntry, D., Sarda-Estève, R., Schiller, C. L., Suski, K. J., Hill, T. C. J., Abbatt, J. P. D., Huffman, J. A., DeMott, P. J., and Bertram, A. K.: Size-resolved measurements of ice-nucleating particles at six locations in North America and one in Europe, Atmos. Chem. Phys., 16, 1637–1651, https://doi.org/10.5194/acp-16-1637-2016, 2016.
McCluskey, C. S., Ovadnevaite, J., Rinaldi, M., Atkinson, J., Belosi, F.,
Ceburnis, D., Marullo, S., Hill, T. C. J., Lohmann, U., Kanji, Z. A.,
O'Dowd, C., Kreidenweis, S. M., and DeMott, P. J.: Marine and terrestrial
organic ice-nucleating particles in pristine marine to continentally
influenced Northeast Atlantic air masses, J. Geophys. Res.-Atmos., 123,
6196–6212, https://doi.org/10.1029/2017JD028033, 2018.
McFarquhar, G. M., Ghan, S., Verlinde, J., Korolev, A., Strapp, J. W.,
Schmid, B., Tomlinson, J. M., Wolde, M., Brooks, S. D., Cziczo, D., Dubey,
M. K., Fan, J., Flynn, C., Gultepe, I., Hubbe, J., Gilles, M. K., Laskin,
A., Lawson, P., Leaitch, W. R., Liu, P., Liu, X., Lubin, D., Mazzoleni, C.,
Macdonald, A.-M., Moffet, R. C., Morrison, H., Ovchinnikov, M., Shupe, M.
D., Turner, D. D., Xie, S., Zelenyuk, A., Bae, K., Freer, M., and Glen, A.:
Indirect and Semi-direct Aerosol Campaign: The Impact of Arctic Aerosols on
Clouds, B. Am. Meteorol. Soc., 92, 183–201,
https://doi.org/10.1175/2010BAMS2935.1, 2011.
Morrison, H., de Boer, G., Feingold, G., Harrington, J., Shupe, M. D., and
Sulia, K.: Resilience of persistent Arctic mixed-phase clouds, Nat. Geosci.,
5, 11–17, https://doi.org/10.1038/ngeo1332, 2012.
Murray, B. J., O'Sullivan, D., Atkinson, J. D., and Webb, M. E.: Ice
nucleation by particles immersed in supercooled cloud droplets, Chem. Soc.
Rev., 41, 6519–6554, https://doi.org/10.1039/c2cs35200a, 2012.
NASA: Aerosol Robotic Network (AERONET), https://aeronet.gsfc.nasa.gov, last access: December 2020.
NASA: Arctic Research of the Composition of the Troposphere from
Aircraft and Satellites (ARCTAS), https://www-air.larc.nasa.gov/missions/arctas/arctas.html, last access: August 2021a.
NASA: CERES EBAF – Level 3b, https://ceres.larc.nasa.gov/data/#ebaf-level-3, last access: November 2021b.
Paramonov, M., David, R. O., Kretzschmar, R., and Kanji, Z. A.: A laboratory investigation of the ice nucleation efficiency of three types of mineral and soil dust, Atmos. Chem. Phys., 18, 16515–16536, https://doi.org/10.5194/acp-18-16515-2018, 2018.
Platnick, S., Ackerman, S., King, M., Wind, G., Meyer, K., Menzel, P., Frey, R., Holz, R., Baum, B., and Yang, P.: MOD06_L2 – MODIS/Terra Clouds 5-Min L2 Swath 1km and 5km, NASA MODIS Adaptive Processing System, Goddard Space Flight Center [data], https://doi.org/10.5067/MODIS/MOD06_L2.061, 2017a.
Platnick, S., Ackerman, S., King, M., Wind, G., Meyer, K., Menzel, P., Frey, R., Holz, R., Baum, B., and Yang, P.: MYD06_L2 – MODIS/Aqua Clouds 5-Min L2 Swath 1km and 5km, NASA MODIS Adaptive Processing System, Goddard Space Flight Center [data], https://doi.org/10.5067/MODIS/MYD06_L2.061, 2017b.
Pincus, R., Platnick, S., Ackerman, S. A., Hemler, R. S., and Hofmann, R. J. P.: Reconciling Simulated and Observed Views of Clouds: MODIS, ISCCP, and the Limits of Instrument Simulators, J. Climate, 25, 4699–4720, https://doi.org/10.1175/JCLI-D-11-00267.1, 2012.
Prenni, A. J., Harrington, J. Y., Tjernström, M., DeMott, P. J.,
Avramov, A., Long, C. N., Kreidenweis, S. M., Olsson, P. Q., and Verlinde,
J.: Can ice-nucleating aerosols affect Arctic seasonal climate?, B. Am.
Meteorol. Soc., 88, 541–550, https://doi.org/10.1175/BAMS-88-4-541, 2007.
Prenni, A. J., Demott, P. J., Rogers, D. C., Kreidenweis, S. M., Mcfarquhar,
G. M., Zhang, G., and Poellot, M. R.: Ice nuclei characteristics from M-PACE
and their relation to ice formation in clouds, Tellus B, 61, 436–448,
https://doi.org/10.1111/j.1600-0889.2009.00415.x, 2009.
Prospero, J. M.: The Atmospheric Transport of Particles to the Ocean, in:
Particle Flux in the Ocean, edited by: Ittekkot, V., Schäfer, P., Honjo, S., and Depetris, P. J., John Wiley & Sons Ltd., New
York, ISBN 047196073X, 978-04-7196-073-7, 1996.
Prospero, J. M., Uematsu, M., and Savoie, D. L.: Mineral aerosol transport
to the Pacific Ocean, edited by: Riley, J. P., Academic Press, New
York, 187–218, ISBN 0125886101, 1989.
Prospero, J. M., Bullard, J. E., and Hodgkins, R.: High-Latitude Dust Over
the North Atlantic: Inputs from Icelandic Proglacial Dust Storms, Science,
335, 1078–1082, https://doi.org/10.1126/science.1217447, 2012.
Rasch, P. J., Xie, S., Ma, P.-L., Lin, W., Wang, H., Tang, Q., Burrows, S.
M., Caldwell, P., Zhang, K., Easter, R. C., Cameron-Smith, P., Singh, B.,
Wan, H., Golaz, J.-C., Harrop, B. E., Roesler, E., Bacmeister, J., Larson,
V. E., Evans, K. J., Qian, Y., Taylor, M., Leung, L. R., Zhang, Y., Brent,
L., Branstetter, M., Hannay, C., Mahajan, S., Mametjanov, A., Neale, R.,
Richter, J. H., Yoon, J. -H., Zender, C. S., Bader, D., Flanner, M., Foucar,
J. G., Jacob, R., Keen, N., Klein, S. A., Liu, X., Salinger, A. G.,
Shrivastava, M., and Yang, Y.: An overview of the atmospheric component of
the Energy Exascale Earth System Model, J. Adv. Model. Earth Syst., 11,
2377–2411, https://doi.org/10.1029/2019MS001629, 2019.
Ridley, D. A., Heald, C. L., Kok, J. F., and Zhao, C.: An observationally constrained estimate of global dust aerosol optical depth, Atmos. Chem. Phys., 16, 15097–15117, https://doi.org/10.5194/acp-16-15097-2016, 2016.
Sanchez-Marroquin, A., Arnalds, O., Baustian-Dorsi, K. J., Browse, J.,
Dagsson-Waldhauserova, P., Harrison, A. D., Maters, E. C., Pringle, K. J.,
Vergara-Temprado, J., Burke, I. T., McQuaid, J. B., Carslaw, K. S., and
Murray, B. J.: Iceland is an episodic source of atmospheric ice-nucleating
particles relevant for mixed-phase clouds, Sci. Adv., 6, eaba8137,
https://doi.org/10.1126/sciadv.aba8137, 2020.
Schill, G. P., DeMott, P. J., Emerson, E. W., Rauker, A. M. C., Kodros, J.
K., Suski, K. J., Hill, T. C. J., Levin, E. J. T., Pierce, J. R., Farmer, D.
K., and Kreidenweis, S. M.: The contribution of black carbon to global ice
nucleating particle concentrations relevant to mixed-phase clouds, P. Natl. Acad. Sci. USA, 117, 22705–22711, https://doi.org/10.1073/pnas.2001674117, 2020.
Schweiger, A. J., Lindsay, R. W., Vavrus, S., and Francis, J. A.:
Relationships between Arctic sea ice and clouds dusting autumn, J. Climate,
21, 4799–4810, https://doi.org/10.1175/2008JCLI2156.1, 2008.
Shao, Y., Wyrwoll, K.-H., Chappell, A., Huang, J., Lin, Z., McTainsh, G. H.,
Mikami, M., Tanaka, T. Y., Wang, X., and Yoon, S.: Dust cycle: An emerging
core theme in Earth system science, Aeolian Res., 2, 181–204,
https://doi.org/10.1016/j.aeolia.2011.02.001, 2011.
Shi, Y. and Liu, X.: Dust Radiative Effects on Climate by Glaciating
Mixed-Phase Clouds, Geophys. Res. Lett., 46, 6128–6137,
https://doi.org/10.1029/2019GL082504, 2019.
Shupe, M. D. and Intrieri, J. M.: Cloud Radiative Forcing of the Arctic
Surface: The Influence of Cloud Properties, Surface Albedo, and Solar Zenith
Angle, J. Climate, 17, 616–628,
https://doi.org/10.1175/1520-0442(2004)017<0616:CRFOTA>2.0.CO;2, 2004.
Si, M., Evoy, E., Yun, J., Xi, Y., Hanna, S. J., Chivulescu, A., Rawlings, K., Veber, D., Platt, A., Kunkel, D., Hoor, P., Sharma, S., Leaitch, W. R., and Bertram, A. K.: Concentrations, composition, and sources of ice-nucleating particles in the Canadian High Arctic during spring 2016, Atmos. Chem. Phys., 19, 3007–3024, https://doi.org/10.5194/acp-19-3007-2019, 2019.
Sirois, A. and Barrie, L. A.: Arctic lower tropospheric aerosol trends and
composition at Alert, Canada: 1980–1995, J. Geophys. Res.-Atmos., 104,
11599–11618, https://doi.org/10.1029/1999JD900077, 1999.
Smirnov, A., Holben, B. N., Eck, T. F., Dubovik, O., and Slutsker, I.: Cloud
screening and quality control algorithms for the AERONET database, Remote
Sens. Environ., 73, 337–349, https://doi.org/10.1016/S0034-4257(00)00109-7,
2000.
Stohl, A.: Characteristics of atmospheric transport into the Arctic
troposphere, J. Geophys. Res., 111, D11306,
https://doi.org/10.1029/2005JD006888, 2006.
Stone, R., Anderson, G., Andrews, E., Dutton, E., Harris, J., Shettle, E., and Berk, A.: Asian dust signatures at Barrow: observed and simulated.
Incursions and impact of Asian dust over Northern Alaska, Workshop on Remote
Sensing of Atmospheric Aerosols, IEEE Workshop on Remote Sensing of
Atmospheric Aerosols, 5–6 April 2005, Tucson, AZ, USA, 74–79, https://doi.org/10.1109/AERSOL.2005.1494152,
2005.
Tan, I. and Storelvmo, T.: Sensitivity study on the influence of cloud
microphysical parameters on mixed-phase cloud thermodynamic phase
partitioning in CAM5, J. Atmos. Sci., 73, 709–728,
https://doi.org/10.1175/JAS-D-15-0152.1, 2016.
Tan, I. and Storelvmo, T.: Evidence of Strong Contributions from Mixed-Phase
Clouds to Arctic Climate Change, Geophys. Res. Lett., 46, 2894–2902,
https://doi.org/10.1029/2018GL081871, 2019.
Tanaka, T. Y. and Chiba, M.: A numerical study of the contributions of dust
source regions to the global dust budget, Glob. Planet. Change, 52, 88–104,
https://doi.org/10.1016/j.gloplacha.2006.02.002, 2006.
Tegen, I., Harrison, S. P., Kohfeld, K., Prentice, I. C., Coe, M., and
Heimann, M.: Impact of vegetation and preferential source areas on global
dust aerosol: Results from a model study, J. Geophys. Res.-Atmos., 107, AAC
14-1–AAC 14-27, https://doi.org/10.1029/2001JD000963, 2002.
Tobo, Y., Adachi, K., DeMott, P. J., Hill, T. C. J., Hamilton, D. S.,
Mahowald, N. M., Nagatsuka, N., Ohata, S., Uetake, J., Kondo, Y., and Koike,
M.: Glacially sourced dust as a potentially significant source of ice
nucleating particles, Nat. Geosci., 12, 253–258,
https://doi.org/10.1038/s41561-019-0314-x, 2019.
Vali, G.: Nucleation terminology, B. Am. Meteorol. Soc., 66, 1426–1427,
1985.
Vali, G., DeMott, P. J., Möhler, O., and Whale, T. F.: Technical Note: A proposal for ice nucleation terminology, Atmos. Chem. Phys., 15, 10263–10270, https://doi.org/10.5194/acp-15-10263-2015, 2015.
VanCuren, R. A., Cahill, T., Burkhart, J., Barnes, D., Zhao, Y., Perry, K.,
Cliff, S., and McConnell, J.: Aerosols and their sources at Summit Greenland
– First results of continuous size- and time-resolved sampling, Atmos.
Environ., 52, 82–97, https://doi.org/10.1016/j.atmosenv.2011.10.047, 2012.
Wang, H., Rasch, P. J., Easter, R. C., Singh, B., Zhang, R., Ma, P.-L.,
Qian, Y., Ghan, S. J., and Beagley, N.: Using an explicit emission tagging
method in global modeling of source-receptor relationships for black carbon
in the Arctic: Variations, sources, and transport pathways, J. Geophys. Res.-Atmos., 119, 12888–12909, https://doi.org/10.1002/2014JD022297, 2014.
Wang, H., Easter, R. C., Zhang, R., Ma, P.-L., Singh, B., Zhang, K.,
Ganguly, D., Rasch, P. J., Burrows, S. M., Ghan, S. J., Lou, S., Qian, Y.,
Yang, Y., Feng, Y., Flanner, M., Leung, L. R., Liu, X., Shrivastava, M.,
Sun, J., Tang, Q., Xie, S., and Yoon, J.: Aerosols in the E3SM Version 1:
New Developments and Their Impacts on Radiative Forcing, J. Adv. Model.
Earth Syst., 12, e2019MS001851, https://doi.org/10.1029/2019MS001851, 2020.
Wang, Y., Liu, X., Hoose, C., and Wang, B.: Different contact angle distributions for heterogeneous ice nucleation in the Community Atmospheric Model version 5, Atmos. Chem. Phys., 14, 10411–10430, https://doi.org/10.5194/acp-14-10411-2014, 2014.
Westbrook, C. D. and Illingworth, A. J.: The formation of ice in a
long-lived supercooled layer cloud: Ice Formation in Altocumulus, Q. J. R.
Meteorol. Soc., 139, 2209–2221, https://doi.org/10.1002/qj.2096, 2013.
Wilson, T. W., Ladino, L. A., Alpert, P. A., Breckels, M. N., Brooks, I. M.,
Browse, J., Burrows, S. M., Carslaw, K. S., Huffman, J. A., Judd, C.,
Kilthau, W. P., Mason, R. H., McFiggans, G., Miller, L. A., Nájera, J.
J., Polishchuk, E., Rae, S., Schiller, C. L., Si, M., Vergara-Temprado, J.,
Whale, T. F., Wong, J. P. S., Wurl, O., Yakobi-Hancock, J. D., Abbatt, J. P.
D., Aller, J. Y., Bertram, A. K., Knopf, D. A., and Murray, B. J.: A marine
biogenic source of atmospheric ice-nucleating particles, Nature, 525,
234–238, https://doi.org/10.1038/nature14986, 2015.
Winker, D. M., Tackett, J. L., Getzewich, B. J., Liu, Z., Vaughan, M. A., and Rogers, R. R.: The global 3-D distribution of tropospheric aerosols as characterized by CALIOP, Atmos. Chem. Phys., 13, 3345–3361, https://doi.org/10.5194/acp-13-3345-2013, 2013.
Wu, M., Liu, X., Yu, H., Wang, H., Shi, Y., Yang, K., Darmenov, A., Wu, C., Wang, Z., Luo, T., Feng, Y., and Ke, Z.: Understanding processes that control dust spatial distributions with global climate models and satellite observations, Atmos. Chem. Phys., 20, 13835–13855, https://doi.org/10.5194/acp-20-13835-2020, 2020.
Yang, K., Wang, Z., Luo, T., Liu, X., and Wu, M.: Upper troposphere dust belt formation processes vary seasonally and spatially in the Northern Hemisphere, Commun. Earth Environ., 3, 24, https://doi.org/10.1038/s43247-022-00353-5, 2022.
Yang, Y., Wang, H., Smith, S. J., Easter, R., Ma, P.-L., Qian, Y., Yu, H., Li, C., and Rasch, P. J.: Global source attribution of sulfate concentration and direct and indirect radiative forcing, Atmos. Chem. Phys., 17, 8903–8922, https://doi.org/10.5194/acp-17-8903-2017, 2017a.
Yang, Y., Wang, H., Smith, S. J., Ma, P.-L., and Rasch, P. J.: Source attribution of black carbon and its direct radiative forcing in China, Atmos. Chem. Phys., 17, 4319–4336, https://doi.org/10.5194/acp-17-4319-2017, 2017b.
Yang, Y., Wang, H., Smith, S. J., Zhang, R., Lou, S., Yu, H., Li, C., and
Rasch, P. J.: Source Apportionments of Aerosols and Their Direct Radiative
Forcing and Long-Term Trends Over Continental United States, Earth's Future,
6, 793–808, https://doi.org/10.1029/2018EF000859, 2018.
Zender, C. S., Bian, H., and Newman, D.: Mineral Dust Entrainment and
Deposition (DEAD) model: Description and 1990s dust climatology, J. Geophys.
Res., 108, 4416, https://doi.org/10.1029/2002JD002775, 2003.
Zhang, G. J. and McFarlane, N. A.: Sensitivity of climate simulations to the
parameterization of cumulus convection in the Canadian climate centre
general circulation model, Atmos.-Ocean, 33, 407–446,
https://doi.org/10.1080/07055900.1995.9649539, 1995.
Zhang, K., Wan, H., Liu, X., Ghan, S. J., Kooperman, G. J., Ma, P.-L., Rasch, P. J., Neubauer, D., and Lohmann, U.: Technical Note: On the use of nudging for aerosol–climate model intercomparison studies, Atmos. Chem. Phys., 14, 8631–8645, https://doi.org/10.5194/acp-14-8631-2014, 2014.
Zhang, M., Liu, X., Diao, M., D'Alessandro, J. J., Wang, Y., Wu, C., Zhang,
D., Wang, Z., and Xie, S.: Impacts of representing heterogeneous
distribution of cloud liquid and ice on phase partitioning of Arctic
mixed-phase clouds with NCAR CAM5, J. Geophys. Res.-Atmos., 124,
13071–13090, https://doi.org/10.1029/2019JD030502, 2019.
Zhang, M., Xie, S., Liu, X., Lin, W., Zhang, K., Ma, H.-Y., Zheng, X., and
Zhang, Y.: Toward understanding the simulated phase partitioning of Arctic
single-layer mixed-phase clouds in E3SM, Earth Space Sci., 7, e2020EA001125,
https://doi.org/10.1029/2020EA001125, 2020.
Zhang, Y., Xie, S., Lin, W., Klein, S. A., Zelinka, M., Ma, P., Rasch, P.
J., Qian, Y., Tang, Q., and Ma, H.: Evaluation of clouds in version 1 of the
E3SM atmosphere model with satellite simulators, J. Adv. Model. Earth Syst.,
11, 1253–1268, https://doi.org/10.1029/2018MS001562, 2019.
Zhao, X. and Liu, X.: Global Importance of Secondary Ice Production,
Geophys. Res. Lett., 48, e2021GL092581,
https://doi.org/10.1029/2021GL092581, 2021.
Zhao, X., Liu, X., Burrows, S. M., and Shi, Y.: Effects of marine organic aerosols as sources of immersion-mode ice-nucleating particles on high-latitude mixed-phase clouds, Atmos. Chem. Phys., 21, 2305–2327, https://doi.org/10.5194/acp-21-2305-2021, 2021a.
Zhao, X., Liu, X., Phillips, V. T. J., and Patade, S.: Impacts of secondary ice production on Arctic mixed-phase clouds based on ARM observations and CAM6 single-column model simulations, Atmos. Chem. Phys., 21, 5685–5703, https://doi.org/10.5194/acp-21-5685-2021, 2021b.
Short summary
We perform a modeling study to evaluate the contribution to Arctic dust loading and ice-nucleating particle (INP) population from high-latitude local and low-latitude dust. High-latitude dust has a large contribution in the lower troposphere, while low-latitude dust dominates the upper troposphere. The high-latitude dust INPs result in a net cooling effect on the Arctic surface by glaciating mixed-phase clouds. Our results highlight the contribution of high-latitude dust to the Arctic climate.
We perform a modeling study to evaluate the contribution to Arctic dust loading and...
Altmetrics
Final-revised paper
Preprint