Articles | Volume 21, issue 8
https://doi.org/10.5194/acp-21-5847-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-5847-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Apr 2021
Research article |
| 19 Apr 2021
| 19 Apr 2021
Ozone variability induced by synoptic weather patterns in warm seasons of 2014–2018 over the Yangtze River Delta region, China
Da Gao
School of Atmospheric Sciences, Joint Center for Atmospheric Radar
Research of CMA/NJU, CMA-NJU Joint Laboratory for Climate Prediction
Studies, Jiangsu Collaborative Innovation Center for Climate Change, Nanjing
University, Nanjing 210023, China
School of Atmospheric Sciences, Joint Center for Atmospheric Radar
Research of CMA/NJU, CMA-NJU Joint Laboratory for Climate Prediction
Studies, Jiangsu Collaborative Innovation Center for Climate Change, Nanjing
University, Nanjing 210023, China
College of Geographic Sciences, Fujian Normal University, Fuzhou
350007, China
Department of Geography and Planning, University of Toronto, Toronto, M5S 3G3, Canada
Tijian Wang
School of Atmospheric Sciences, Joint Center for Atmospheric Radar
Research of CMA/NJU, CMA-NJU Joint Laboratory for Climate Prediction
Studies, Jiangsu Collaborative Innovation Center for Climate Change, Nanjing
University, Nanjing 210023, China
Chaoqun Ma
School of Atmospheric Sciences, Joint Center for Atmospheric Radar
Research of CMA/NJU, CMA-NJU Joint Laboratory for Climate Prediction
Studies, Jiangsu Collaborative Innovation Center for Climate Change, Nanjing
University, Nanjing 210023, China
now at:
Minerva Research Group, Max Planck Institute for Chemistry, Mainz, Germany
Haokun Bai
School of Atmospheric Sciences, Joint Center for Atmospheric Radar
Research of CMA/NJU, CMA-NJU Joint Laboratory for Climate Prediction
Studies, Jiangsu Collaborative Innovation Center for Climate Change, Nanjing
University, Nanjing 210023, China
Xing Chen
School of Atmospheric Sciences, Joint Center for Atmospheric Radar
Research of CMA/NJU, CMA-NJU Joint Laboratory for Climate Prediction
Studies, Jiangsu Collaborative Innovation Center for Climate Change, Nanjing
University, Nanjing 210023, China
Mengmeng Li
School of Atmospheric Sciences, Joint Center for Atmospheric Radar
Research of CMA/NJU, CMA-NJU Joint Laboratory for Climate Prediction
Studies, Jiangsu Collaborative Innovation Center for Climate Change, Nanjing
University, Nanjing 210023, China
Bingliang Zhuang
School of Atmospheric Sciences, Joint Center for Atmospheric Radar
Research of CMA/NJU, CMA-NJU Joint Laboratory for Climate Prediction
Studies, Jiangsu Collaborative Innovation Center for Climate Change, Nanjing
University, Nanjing 210023, China
Shu Li
School of Atmospheric Sciences, Joint Center for Atmospheric Radar
Research of CMA/NJU, CMA-NJU Joint Laboratory for Climate Prediction
Studies, Jiangsu Collaborative Innovation Center for Climate Change, Nanjing
University, Nanjing 210023, China
Related authors
Lei Shu, Min Xie, Da Gao, Tijian Wang, Dexian Fang, Qian Liu, Anning Huang, and Liwen Peng
Atmos. Chem. Phys., 17, 12871–12891, https://doi.org/10.5194/acp-17-12871-2017, https://doi.org/10.5194/acp-17-12871-2017, 2017
Short summary
Short summary
Based on 1-year in situ monitoring data of 16 cities, this paper can enhance the understanding of the pollution characteristics of particles (PM2.5 and PM10) in the Yangtze River Delta region, China. Based on NCEP reanalysis data, the establishment of the potential links between different levels of particle pollution and predominant synoptic patterns can provide an insightful view on formulating pollution control and mitigation strategies.
Min Xie, Lei Shu, Tijian Wang, Da Gao, Shu Li, Bingliang Zhuang, Anning Huang, Dexian Fang, Yong Han, Mengmeng Li, Pulong Chen, Zhijun Liu, Zheng Wu, and Hua Lu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-500, https://doi.org/10.5194/acp-2017-500, 2017
Preprint withdrawn
Short summary
Short summary
The spatial distribution of aerosol can be affected by monsoon circulation. With the aid of a EAWM index, the stong and the weak EAWM years are identified. The long-term trend of weakening EAWM may potentially increase the aerosol loading in YRD, BTH and SCB but decrease AOD in PRD. By using RegCCMS, we further prove that the intensity of EAWM has great impacts on the spatial distribution of aerosols. The change pattern is mainly decided by the change of aerosols in lower troposphere.
Lei Shu, Min Xie, Tijian Wang, Da Gao, Pulong Chen, Yong Han, Shu Li, Bingliang Zhuang, and Mengmeng Li
Atmos. Chem. Phys., 16, 15801–15819, https://doi.org/10.5194/acp-16-15801-2016, https://doi.org/10.5194/acp-16-15801-2016, 2016
Short summary
Short summary
Severe high ozone episodes usually have close relations to synoptic systems. A regional continuous ozone pollution episode is detected over the Yangtze River Delta region in August 2013. By means of observational analysis and model simulations, it is found that the western Pacific subtropical high and Typhoon Utor play an important role.
Min Xie, Kuanguang Zhu, Tijian Wang, Wen Feng, Da Gao, Mengmeng Li, Shu Li, Bingliang Zhuang, Yong Han, Pulong Chen, and Jingbiao Liao
Atmos. Chem. Phys., 16, 15011–15031, https://doi.org/10.5194/acp-16-15011-2016, https://doi.org/10.5194/acp-16-15011-2016, 2016
Short summary
Short summary
In this paper, we present our new findings on (1) the spatial and temporal characteristics of AH emissions in South China, (2) how to implement the inhomogeneous AH data into the air quality model WRF/Chem, (3) the impacts of AH fluxes on meteorological fields, and (4) the impacts of meteorology changes on the air quality in different cities in South China. Our results show that the meteorology and air pollution predictions in and around big cities are highly sensitive to AH.
Hua Lu, Min Xie, Bingliang Zhuang, Danyang Ma, Bojun Liu, Yangzhihao Zhan, Tijian Wang, Shu Li, Mengmeng Li, and Kuanguang Zhu
Atmos. Chem. Phys., 24, 8963–8982, https://doi.org/10.5194/acp-24-8963-2024, https://doi.org/10.5194/acp-24-8963-2024, 2024
Short summary
Short summary
To identify cloud, aerosol, and planetary boundary layer (PBL) interactions from an air quality perspective, we summarized two pollution patterns characterized by denser liquid cloud and by obvious cloud radiation interaction (CRI). Numerical simulation experiments showed CRI could cause a 50 % reduction in aerosol radiation interaction (ARI) under a low-trough system. The results emphasized the nonnegligible role of CRI and its inhibition of ARI under wet and cloudy pollution synoptic patterns.
Honglei Wang, David W. Tarasick, Jane Liu, Herman G. J. Smit, Roeland Van Malderen, Lijuan Shen, and Tianliang Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-1015, https://doi.org/10.5194/egusphere-2024-1015, 2024
Short summary
Short summary
In this study, we identify 23 suitable pairs of sites in the WOUDC and IAGOS datasets from 1995 to 2021, compare the average vertical distribution of tropospheric O3 shown by ozonesonde and aircraft measurements, and analyze their differences by ozonesonde type and by station-airport distance.
Nanhong Xie, Tijian Wang, Xiaodong Xie, Xu Yue, Filippo Giorgi, Qian Zhang, Danyang Ma, Rong Song, Beiyao Xu, Shu Li, Bingliang Zhuang, Mengmeng Li, Min Xie, Natalya Andreeva Kilifarska, Georgi Gadzhev, and Reneta Dimitrova
Geosci. Model Dev., 17, 3259–3277, https://doi.org/10.5194/gmd-17-3259-2024, https://doi.org/10.5194/gmd-17-3259-2024, 2024
Short summary
Short summary
For the first time, we coupled a regional climate chemistry model, RegCM-Chem, with a dynamic vegetation model, YIBs, to create a regional climate–chemistry–ecology model, RegCM-Chem–YIBs. We applied it to simulate climatic, chemical, and ecological parameters in East Asia and fully validated it on a variety of observational data. Results show that RegCM-Chem–YIBs model is a valuable tool for studying the terrestrial carbon cycle, atmospheric chemistry, and climate change on a regional scale.
Zhou Zang, Jane Liu, David Tarasick, Omid Moeini, Jianchun Bian, Jinqiang Zhang, Anne M. Thompson, Roeland Van Malderen, Herman G. J. Smit, Ryan M. Stauffer, Bryan J. Johnson, and Debra E. Kollonige
EGUsphere, https://doi.org/10.5194/egusphere-2024-800, https://doi.org/10.5194/egusphere-2024-800, 2024
Short summary
Short summary
The Trajectory-mapped Ozonesonde dataset for the Stratosphere and Troposphere (TOST) provides a global-scale, long-term ozone climatology that is horizontally- and vertically-resolved. In this study, we improved, updated, and validated the TOST from 1970 to 2021. Based on this TOST dataset, we characterized global ozone variations spatially in both the troposphere and stratosphere and temporally by season and decade. We also showed a stagnant stratospheric ozone variation since the late 1990s.
Jiye Leng, Jing M. Chen, Wenyu Li, Xiangzhong Luo, Mingzhu Xu, Jane Liu, Rong Wang, Cheryl Rogers, Bolun Li, and Yulin Yan
Earth Syst. Sci. Data, 16, 1283–1300, https://doi.org/10.5194/essd-16-1283-2024, https://doi.org/10.5194/essd-16-1283-2024, 2024
Short summary
Short summary
We produced a long-term global two-leaf gross primary productivity (GPP) and evapotranspiration (ET) dataset at the hourly time step by integrating a diagnostic process-based model with dynamic parameterizations. The new dataset provides us with a unique opportunity to study carbon and water fluxes at sub-daily time scales and advance our understanding of ecosystem functions in response to transient environmental changes.
Shiyi Lai, Ximeng Qi, Xin Huang, Sijia Lou, Xuguang Chi, Liangduo Chen, Chong Liu, Yuliang Liu, Chao Yan, Mengmeng Li, Tengyu Liu, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 24, 2535–2553, https://doi.org/10.5194/acp-24-2535-2024, https://doi.org/10.5194/acp-24-2535-2024, 2024
Short summary
Short summary
By combining in situ measurements and chemical transport modeling, this study investigates new particle formation (NPF) on the southeastern Tibetan Plateau. We found that the NPF was driven by the presence of biogenic gases and the transport of anthropogenic precursors. The NPF was vertically heterogeneous and shaped by the vertical mixing. This study highlights the importance of anthropogenic–biogenic interactions and meteorological dynamics in NPF in this climate-sensitive region.
Hua Lu, Min Xie, Wei Zhao, Bojun Liu, Tijian Wang, and Bingliang Zhuang
Atmos. Meas. Tech., 17, 167–179, https://doi.org/10.5194/amt-17-167-2024, https://doi.org/10.5194/amt-17-167-2024, 2024
Short summary
Short summary
Observations of vertical wind in regions with complex terrain are essential, but they are always sparse and have poor representation. Data verification and quality control are conducted on the wind profile radar and Aeolus wind products in this study, trying to compensate for the limitations of wind field observations. The results shed light on the comprehensive applications of multi-source wind profile data in complicated terrain regions with sparse ground-based wind observations.
Siyu Zhu, Peipei Wu, Siyi Zhang, Oliver Jahn, Shu Li, and Yanxu Zhang
Geosci. Model Dev., 16, 5915–5929, https://doi.org/10.5194/gmd-16-5915-2023, https://doi.org/10.5194/gmd-16-5915-2023, 2023
Short summary
Short summary
In this study, we estimate the global biogeochemical cycling of Hg in a state-of-the-art physical-ecosystem ocean model (high-resolution-MITgcm/Hg), providing a more accurate portrayal of surface Hg concentrations in estuarine and coastal areas, strong western boundary flow and upwelling areas, and concentration diffusion as vortex shapes. The high-resolution model can help us better predict the transport and fate of Hg in the ocean and its impact on the global Hg cycle.
Yangzhihao Zhan, Min Xie, Wei Zhao, Tijian Wang, Da Gao, Pulong Chen, Jun Tian, Kuanguang Zhu, Shu Li, Bingliang Zhuang, Mengmeng Li, Yi Luo, and Runqi Zhao
Atmos. Chem. Phys., 23, 9837–9852, https://doi.org/10.5194/acp-23-9837-2023, https://doi.org/10.5194/acp-23-9837-2023, 2023
Short summary
Short summary
Although the main source contribution of pollution is secondary inorganic aerosols in Nanjing, health risks mainly come from industry sources and vehicle emissions. Therefore, the development of megacities should pay more attention to the health burden of vehicle emissions, coal combustion, and industrial processes. This study provides new insight into assessing the relationship between source apportionment and health risks and can provide valuable insight into air pollution strategies.
Danyang Ma, Tijian Wang, Hao Wu, Yawei Qu, Jian Liu, Jane Liu, Shu Li, Bingliang Zhuang, Mengmeng Li, and Min Xie
Atmos. Chem. Phys., 23, 6525–6544, https://doi.org/10.5194/acp-23-6525-2023, https://doi.org/10.5194/acp-23-6525-2023, 2023
Short summary
Short summary
Increasing surface ozone (O3) concentrations have long been a significant environmental issue in China, despite the Clean Air Action Plan launched in 2013. Most previous research ignores the contributions of CO2 variations. Our study comprehensively analyzed O3 variation across China from various perspectives and highlighted the importance of considering CO2 variations when designing long-term O3 control policies, especially in high-vegetation-coverage areas.
Chenchao Zhan, Min Xie, Hua Lu, Bojun Liu, Zheng Wu, Tijian Wang, Bingliang Zhuang, Mengmeng Li, and Shu Li
Atmos. Chem. Phys., 23, 771–788, https://doi.org/10.5194/acp-23-771-2023, https://doi.org/10.5194/acp-23-771-2023, 2023
Short summary
Short summary
With the development of urbanization, urban land use and anthropogenic
emissions increase, affecting urban air quality and, in turn, the health risks associated with air pollutants. In this study, we systematically evaluate the impacts of urbanization on air quality and the corresponding health risks in a highly urbanized city with severe air pollution and complex terrain. This work focuses on the health risks caused by urbanization and can provide valuable insight for air pollution strategies.
Shiyue Zhang, Gang Zeng, Tijian Wang, Xiaoye Yang, and Vedaste Iyakaremye
Atmos. Chem. Phys., 22, 16017–16030, https://doi.org/10.5194/acp-22-16017-2022, https://doi.org/10.5194/acp-22-16017-2022, 2022
Short summary
Short summary
Severe haze days in eastern China (HDEC) are affected by the atmospheric circulation variations on a synoptic scale, while the dominant atmospheric circulation patterns influencing HDEC and the differences between them are still unclear. This study obtains three dominant circulation types that could lead to severe HDEC and investigates the differences between them. The results provide a basis for establishing applicable haze prediction and management policies.
Zhixiong Chen, Jane Liu, Xiushu Qie, Xugeng Cheng, Yukun Shen, Mengmiao Yang, Rubin Jiang, and Xiangke Liu
Atmos. Chem. Phys., 22, 8221–8240, https://doi.org/10.5194/acp-22-8221-2022, https://doi.org/10.5194/acp-22-8221-2022, 2022
Short summary
Short summary
A vigorous surface ozone surge event of stratospheric origin occurred in the North China Plain at night. Surface ozone concentrations were 40–50 ppbv higher than the corresponding monthly mean, whereas surface carbon monoxide concentrations declined abruptly, which confirmed the direct stratospheric intrusions to the surface. We further addressed the notion that a combined effect of the dying typhoon and mesoscale convective systems was responsible for this vigorous ozone surge.
Chenchao Zhan and Min Xie
Atmos. Chem. Phys., 22, 1351–1371, https://doi.org/10.5194/acp-22-1351-2022, https://doi.org/10.5194/acp-22-1351-2022, 2022
Short summary
Short summary
The changes of land use and anthropogenic heat (AH) derived from urbanization can affect meteorology and in turn O3 evolution. In this study, we briefly describe the general features of O3 pollution in the Yangtze River Delta (YRD) based on in situ observational data. Then, the impacts of land use and anthropogenic heat on O3 via changing the meteorological factors and local circulations are investigated in this region using the WRF-Chem model.
Zhixiong Chen, Jane Liu, Xugeng Cheng, Mengmiao Yang, and Hong Wang
Atmos. Chem. Phys., 21, 16911–16923, https://doi.org/10.5194/acp-21-16911-2021, https://doi.org/10.5194/acp-21-16911-2021, 2021
Short summary
Short summary
Using a large ensemble of typhoons, we investigate the impacts of evolving typhoons on tropospheric ozone and address the linkages between typhoon-affected meteorological conditions and ozone variations. The influences of typhoon-induced stratospheric intrusions on lower-troposphere ozone are also quantified. Thus, the results obtained in this study have important implications for a full understanding of the multifaced roles of typhoons in modulating tropospheric ozone variation.
Mengmeng Li, Zihan Zhang, Quan Yao, Tijian Wang, Min Xie, Shu Li, Bingliang Zhuang, and Yong Han
Atmos. Chem. Phys., 21, 15135–15152, https://doi.org/10.5194/acp-21-15135-2021, https://doi.org/10.5194/acp-21-15135-2021, 2021
Short summary
Short summary
We establish the nonlinear responses between nitrate and NOx in China. Reduction of NOx results in linearly lower nitrate in summer–autumn whereas an increase of winter nitrate until an inflexion point at 40–50 % reduction due to the excess oxidants. NH3 and VOCs are effective in controlling nitrate pollution, whereas decreasing the SO2 and NOx emissions may have counterintuitive effects on nitrate aerosols. This paper helps understand the nonlinear aerosol and photochemistry feedback.
Yawei Qu, Apostolos Voulgarakis, Tijian Wang, Matthew Kasoar, Chris Wells, Cheng Yuan, Sunil Varma, and Laura Mansfield
Atmos. Chem. Phys., 21, 5705–5718, https://doi.org/10.5194/acp-21-5705-2021, https://doi.org/10.5194/acp-21-5705-2021, 2021
Short summary
Short summary
The meteorological effect of aerosols on tropospheric ozone is investigated using global atmospheric modelling. We found that aerosol-induced meteorological effects act to reduce modelled ozone concentrations over China, which brings the simulation closer to observed levels. Our work sheds light on understudied processes affecting the levels of tropospheric gaseous pollutants and provides a basis for evaluating such processes using a combination of observations and model sensitivity experiments.
Paul T. Griffiths, Lee T. Murray, Guang Zeng, Youngsub Matthew Shin, N. Luke Abraham, Alexander T. Archibald, Makoto Deushi, Louisa K. Emmons, Ian E. Galbally, Birgit Hassler, Larry W. Horowitz, James Keeble, Jane Liu, Omid Moeini, Vaishali Naik, Fiona M. O'Connor, Naga Oshima, David Tarasick, Simone Tilmes, Steven T. Turnock, Oliver Wild, Paul J. Young, and Prodromos Zanis
Atmos. Chem. Phys., 21, 4187–4218, https://doi.org/10.5194/acp-21-4187-2021, https://doi.org/10.5194/acp-21-4187-2021, 2021
Short summary
Short summary
We analyse the CMIP6 Historical and future simulations for tropospheric ozone, a species which is important for many aspects of atmospheric chemistry. We show that the current generation of models agrees well with observations, being particularly successful in capturing trends in surface ozone and its vertical distribution in the troposphere. We analyse the factors that control ozone and show that they evolve over the period of the CMIP6 experiments.
Chenchao Zhan, Min Xie, Chongwu Huang, Jane Liu, Tijian Wang, Meng Xu, Chaoqun Ma, Jianwei Yu, Yumeng Jiao, Mengmeng Li, Shu Li, Bingliang Zhuang, Ming Zhao, and Dongyang Nie
Atmos. Chem. Phys., 20, 13781–13799, https://doi.org/10.5194/acp-20-13781-2020, https://doi.org/10.5194/acp-20-13781-2020, 2020
Short summary
Short summary
The Yangtze River Delta (YRD) region has been suffering from severe ozone (O3) pollution in recent years. Synoptic systems, like typhoons, can have a significant effect on O3 episodes. However, research on landfall typhoons affecting O3 in the YRD is limited. This work aims to reveal the main processes of landfall typhoons affecting surface O3 and estimate health impacts of O3 during the study period in the YRD, which can be useful for taking reasonable pollution control measures in this area.
Han Han, Yue Wu, Jane Liu, Tianliang Zhao, Bingliang Zhuang, Honglei Wang, Yichen Li, Huimin Chen, Ye Zhu, Hongnian Liu, Qin'geng Wang, Shu Li, Tijian Wang, Min Xie, and Mengmeng Li
Atmos. Chem. Phys., 20, 13591–13610, https://doi.org/10.5194/acp-20-13591-2020, https://doi.org/10.5194/acp-20-13591-2020, 2020
Short summary
Short summary
Combining simulations from a global chemical transport model and a trajectory model, we find that black carbon aerosols from South Asia and East Asia contribute 77 % of the surface black carbon in the Tibetan Plateau. The Asian monsoon largely modulates inter-annual transport of black carbon from non-local regions to the Tibetan Plateau surface in most seasons, while inter-annual fire activities in South Asia influence black carbon concentration over the Tibetan Plateau surface mainly in spring.
Meng Gao, Zhiwei Han, Zhining Tao, Jiawei Li, Jeong-Eon Kang, Kan Huang, Xinyi Dong, Bingliang Zhuang, Shu Li, Baozhu Ge, Qizhong Wu, Hyo-Jung Lee, Cheol-Hee Kim, Joshua S. Fu, Tijian Wang, Mian Chin, Meng Li, Jung-Hun Woo, Qiang Zhang, Yafang Cheng, Zifa Wang, and Gregory R. Carmichael
Atmos. Chem. Phys., 20, 1147–1161, https://doi.org/10.5194/acp-20-1147-2020, https://doi.org/10.5194/acp-20-1147-2020, 2020
Short summary
Short summary
Topic 3 of the Model Inter-Comparison Study for Asia (MICS-Asia) Phase III examines how online coupled air quality models perform in simulating high aerosol pollution in the North China Plain region during wintertime haze events and evaluates the importance of aerosol radiative feedbacks. This paper discusses the estimates of aerosol radiative forcing, aerosol feedbacks, and possible causes for the differences among the models.
Han Han, Jane Liu, Lei Shu, Tijian Wang, and Huiling Yuan
Atmos. Chem. Phys., 20, 203–222, https://doi.org/10.5194/acp-20-203-2020, https://doi.org/10.5194/acp-20-203-2020, 2020
Short summary
Short summary
We statistically assessed the impacts of local and synoptic meteorology on daily surface ozone in eastern China in summer during 2013–2018. The results show that the meteorology described by a multiple linear regression model explains 43 % of variations in surface ozone. The most important local meteorological factors vary with location in eastern China. The maximum impact of the predominant synoptic pattern on surface ozone can reach ± 8 µg m-3 or ± 16 % of the daily mean over some regions.
Lifei Yin, Zhenying Xu, Mingxu Liu, Tingting Xu, Tiantian Wang, Wenling Liao, Mengmeng Li, Xuhui Cai, Ling Kang, Hongsheng Zhang, and Yu Song
Biogeosciences Discuss., https://doi.org/10.5194/bg-2019-458, https://doi.org/10.5194/bg-2019-458, 2020
Manuscript not accepted for further review
Short summary
Short summary
Biogenic Volatile Organic Compounds (BVOCs) emission of terrestrial vegetation is an important part of biogeochemical cycle. Compared with previous studies which calculate regional BVOC emissions independently, the coupled model WRF-CLM-MEGAN achieves an integrated parameterization of BVOC emissions and other land surface processes, and therefore provides a more reasonable estimate. The model could be further coupled with chemistry module to fully investigate the land-atmosphere interactions.
Han Han, Jane Liu, Huiling Yuan, Tijian Wang, Bingliang Zhuang, and Xun Zhang
Atmos. Chem. Phys., 19, 12495–12514, https://doi.org/10.5194/acp-19-12495-2019, https://doi.org/10.5194/acp-19-12495-2019, 2019
Short summary
Short summary
In the East Asian middle and upper troposphere, foreign ozone is 0.8–4.8 times more than its native counterpart in all the seasons. At the East Asian surface, the annual mean concentrations of foreign ozone and native ozone are comparable, being approximately 20 ppbv. The seasonal and interannual variations in foreign ozone over East Asia are closely related to the East Asian monsoon.
Huimin Chen, Bingliang Zhuang, Jane Liu, Tijian Wang, Shu Li, Min Xie, Mengmeng Li, Pulong Chen, and Ming Zhao
Atmos. Chem. Phys., 19, 4153–4175, https://doi.org/10.5194/acp-19-4153-2019, https://doi.org/10.5194/acp-19-4153-2019, 2019
Short summary
Short summary
To better understand the characteristics of air pollutants and their interactions in the highly polluted region of eastern China, continuous measurements of particles and trace gases were made during cold seasons in 2016. We found 48 days with excess of PM2.5, 14 with excess of PM10, and 40 with excess of O3. Results further reveal the formation of secondary aerosols under high-O3 and temperature conditions and suggest a VOC-sensitive regime for photochemical production of O3 in urban Nanjing.
Junting Zhong, Xiaoye Zhang, Yaqiang Wang, Jizhi Wang, Xiaojing Shen, Hongsheng Zhang, Tijian Wang, Zhouqing Xie, Cheng Liu, Hengde Zhang, Tianliang Zhao, Junying Sun, Shaojia Fan, Zhiqiu Gao, Yubin Li, and Linlin Wang
Atmos. Chem. Phys., 19, 3287–3306, https://doi.org/10.5194/acp-19-3287-2019, https://doi.org/10.5194/acp-19-3287-2019, 2019
Short summary
Short summary
In various haze regions in China, including the Guanzhong Plain, the middle and lower reaches of the Yangtze River, the Pearl River Delta, the Sichuan Basin, and the Northeast China Plain, heavy aerosol pollution episodes include inter-/trans-regional transport stages and cumulative stages (CSs). During CSs a two-way feedback mechanism exists between unfavorable meteorological conditions and cumulative aerosol pollution. This two-way feedback is further quantified and its magnitude is compared.
Cheng Yuan, William K. M. Lau, Zhanqing Li, and Maureen Cribb
Atmos. Chem. Phys., 19, 1901–1913, https://doi.org/10.5194/acp-19-1901-2019, https://doi.org/10.5194/acp-19-1901-2019, 2019
Short summary
Short summary
Using MERRA-2 reanalysis daily data from 2001 to 2015, we found that during strong South Asian summer monsoon years, the Asian monsoon anticyclone is more expansive and shifted northward. All the CO, carbonaceous aerosols and dust are found to be more abundant in the Asian Tropopause Aerosol Layer (ATAL). ATAL trends are associated with increasing strength of the AMA, with earlier and enhanced vertical transport of ATAL constituents by enhanced overshooting convection over the transport regions.
Debora Griffin, Kaley A. Walker, Ingo Wohltmann, Sandip S. Dhomse, Markus Rex, Martyn P. Chipperfield, Wuhu Feng, Gloria L. Manney, Jane Liu, and David Tarasick
Atmos. Chem. Phys., 19, 577–601, https://doi.org/10.5194/acp-19-577-2019, https://doi.org/10.5194/acp-19-577-2019, 2019
Short summary
Short summary
Ozone in the stratosphere is important to protect the Earth from UV radiation. Using measurements taken by the Atmospheric Chemistry Experiment satellite between 2005 and 2013, we examine different methods to calculate the ozone loss in the high Arctic and establish the altitude at which most of the ozone is destroyed. Our results show that the different methods agree within the uncertainties. Recommendations are made on which methods are most appropriate to use.
Jun Hu, Yichen Li, Tianliang Zhao, Jane Liu, Xiao-Ming Hu, Duanyang Liu, Yongcheng Jiang, Jianming Xu, and Luyu Chang
Atmos. Chem. Phys., 18, 16239–16251, https://doi.org/10.5194/acp-18-16239-2018, https://doi.org/10.5194/acp-18-16239-2018, 2018
Short summary
Short summary
Using observational and modeling studies, the importance of the mechanism driving regional O3 transport in the residual layer (RL) with respect to summer smog over the Yangtze River Delta region in eastern China was revealed. This mechanism was also examined in association with diurnal change in the atmospheric boundary layer. Regional O3 transport through the nocturnal RL is believed to have great implications for understanding urban and regional O3 pollution in this area.
Meng Gao, Zhiwei Han, Zirui Liu, Meng Li, Jinyuan Xin, Zhining Tao, Jiawei Li, Jeong-Eon Kang, Kan Huang, Xinyi Dong, Bingliang Zhuang, Shu Li, Baozhu Ge, Qizhong Wu, Yafang Cheng, Yuesi Wang, Hyo-Jung Lee, Cheol-Hee Kim, Joshua S. Fu, Tijian Wang, Mian Chin, Jung-Hun Woo, Qiang Zhang, Zifa Wang, and Gregory R. Carmichael
Atmos. Chem. Phys., 18, 4859–4884, https://doi.org/10.5194/acp-18-4859-2018, https://doi.org/10.5194/acp-18-4859-2018, 2018
Short summary
Short summary
Topic 3 of the Model Inter-Comparison Study for Asia (MICS-Asia) Phase III examines how online coupled air quality models perform in simulating high aerosol pollution in the North China Plain region during wintertime haze events and evaluates the importance of aerosol radiative and microphysical feedbacks. A comprehensive overview of the MICS-ASIA III Topic 3 study design is presented.
Han Han, Jane Liu, Huiling Yuan, Bingliang Zhuang, Ye Zhu, Yue Wu, Yuhan Yan, and Aijun Ding
Atmos. Chem. Phys., 18, 4251–4276, https://doi.org/10.5194/acp-18-4251-2018, https://doi.org/10.5194/acp-18-4251-2018, 2018
Short summary
Short summary
Imported African ozone peaks in the Asian middle and upper troposphere in March. The seasonality of African ozone influence on Asia is mainly driven by the seasonal swing of the ITCZ, the Hadley circulation, and the northern subtropical westerlies. The stronger the ITCZ over Africa in a boreal winter is, the more African ozone is transported to Asia that winter. The convective divergence over the ITCZ and the Somali jet are drivers of interhemispheric transport of African ozone.
Bingliang Zhuang, Tijian Wang, Jane Liu, Huizheng Che, Yong Han, Yu Fu, Shu Li, Min Xie, Mengmeng Li, Pulong Chen, Huimin Chen, Xiu-qun Yang, and Jianning Sun
Atmos. Chem. Phys., 18, 1419–1436, https://doi.org/10.5194/acp-18-1419-2018, https://doi.org/10.5194/acp-18-1419-2018, 2018
Short summary
Short summary
Aerosols have a significant influence on climate changes. Their uncertainties could be substantially reduced if observation data were used. The properties and the DRF of fractionated aerosols in the western Yangtze River Delta are investigated based on measurements. Results reveal the characteristics of the optical properties and DRFs of different types of fractionated aerosols, which can be further used to improve aerosol modelling performance in the eastern regions of China.
Qian Huang, Tijian Wang, Pulong Chen, Xiaoxian Huang, Jialei Zhu, and Bingliang Zhuang
Atmos. Chem. Phys., 17, 13457–13471, https://doi.org/10.5194/acp-17-13457-2017, https://doi.org/10.5194/acp-17-13457-2017, 2017
Short summary
Short summary
This paper investigate the important factor contributing to the improvement of air quality of Nanjing, China, during the 2nd Youth Olympic Games, held in August, 2014. The interesting finding is that meteorological factors are not beneficial to air quality during the YOG. However, emission reduction plays a more important role, which suggest that emission reduction is an effective way to cut air pollution levels for social events.
Lei Shu, Min Xie, Da Gao, Tijian Wang, Dexian Fang, Qian Liu, Anning Huang, and Liwen Peng
Atmos. Chem. Phys., 17, 12871–12891, https://doi.org/10.5194/acp-17-12871-2017, https://doi.org/10.5194/acp-17-12871-2017, 2017
Short summary
Short summary
Based on 1-year in situ monitoring data of 16 cities, this paper can enhance the understanding of the pollution characteristics of particles (PM2.5 and PM10) in the Yangtze River Delta region, China. Based on NCEP reanalysis data, the establishment of the potential links between different levels of particle pollution and predominant synoptic patterns can provide an insightful view on formulating pollution control and mitigation strategies.
Min Xie, Lei Shu, Tijian Wang, Da Gao, Shu Li, Bingliang Zhuang, Anning Huang, Dexian Fang, Yong Han, Mengmeng Li, Pulong Chen, Zhijun Liu, Zheng Wu, and Hua Lu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-500, https://doi.org/10.5194/acp-2017-500, 2017
Preprint withdrawn
Short summary
Short summary
The spatial distribution of aerosol can be affected by monsoon circulation. With the aid of a EAWM index, the stong and the weak EAWM years are identified. The long-term trend of weakening EAWM may potentially increase the aerosol loading in YRD, BTH and SCB but decrease AOD in PRD. By using RegCCMS, we further prove that the intensity of EAWM has great impacts on the spatial distribution of aerosols. The change pattern is mainly decided by the change of aerosols in lower troposphere.
Bingliang Zhuang, Tijian Wang, Jane Liu, Shu Li, Min Xie, Yong Han, Pulong Chen, Qiduo Hu, Xiu-qun Yang, Congbin Fu, and Jialei Zhu
Atmos. Chem. Phys., 17, 1143–1160, https://doi.org/10.5194/acp-17-1143-2017, https://doi.org/10.5194/acp-17-1143-2017, 2017
Short summary
Short summary
The observed near-surface aerosol optical properties in urban Nanjing are analysed from March 2014 to February 2016. Substantial analysis in the key optical properties of the surface aerosol fill the gaps in the study on aerosols in Nanjing, even in the Yangtze River Delta (YRD). Relationships between the aerosol extinction coefficient (single scattering albedo) and atmospheric visibility are also carried out in different seasons to figure out the effect of aerosol on the visibility in Nanjing, YRD.
Lei Shu, Min Xie, Tijian Wang, Da Gao, Pulong Chen, Yong Han, Shu Li, Bingliang Zhuang, and Mengmeng Li
Atmos. Chem. Phys., 16, 15801–15819, https://doi.org/10.5194/acp-16-15801-2016, https://doi.org/10.5194/acp-16-15801-2016, 2016
Short summary
Short summary
Severe high ozone episodes usually have close relations to synoptic systems. A regional continuous ozone pollution episode is detected over the Yangtze River Delta region in August 2013. By means of observational analysis and model simulations, it is found that the western Pacific subtropical high and Typhoon Utor play an important role.
Min Xie, Kuanguang Zhu, Tijian Wang, Wen Feng, Da Gao, Mengmeng Li, Shu Li, Bingliang Zhuang, Yong Han, Pulong Chen, and Jingbiao Liao
Atmos. Chem. Phys., 16, 15011–15031, https://doi.org/10.5194/acp-16-15011-2016, https://doi.org/10.5194/acp-16-15011-2016, 2016
Short summary
Short summary
In this paper, we present our new findings on (1) the spatial and temporal characteristics of AH emissions in South China, (2) how to implement the inhomogeneous AH data into the air quality model WRF/Chem, (3) the impacts of AH fluxes on meteorological fields, and (4) the impacts of meteorology changes on the air quality in different cities in South China. Our results show that the meteorology and air pollution predictions in and around big cities are highly sensitive to AH.
Mohammed K. Osman, David W. Tarasick, Jane Liu, Omid Moeini, Valerie Thouret, Vitali E. Fioletov, Mark Parrington, and Philippe Nédélec
Atmos. Chem. Phys., 16, 10263–10282, https://doi.org/10.5194/acp-16-10263-2016, https://doi.org/10.5194/acp-16-10263-2016, 2016
Short summary
Short summary
A new 3-D gridded climatology of CO has been developed by trajectory mapping of global MOZAIC-IAGOS in situ aircraft measurements. The dataset is archived monthly from 2001–2012 on a grid of 5 × 5deg × 1 km altitude. The dataset facilitates comparison of different years and seasons and offers insight into the global variation and trends of CO. Major CO sources are clearly visible. The dataset can be used as an a priori data for satellite retrieval and for air quality model validation and initialization.
Zhe Jiang, Kazuyuki Miyazaki, John R. Worden, Jane J. Liu, Dylan B. A. Jones, and Daven K. Henze
Atmos. Chem. Phys., 16, 6537–6546, https://doi.org/10.5194/acp-16-6537-2016, https://doi.org/10.5194/acp-16-6537-2016, 2016
Short summary
Short summary
We quantify the impacts of anthropogenic and natural sources on free tropospheric ozone over the Middle East, using the adjoint of the GEOS-Chem model with updated NOx emissions estimates from an ensemble Kalman filter. We show that the global total contribution of lightning NOx on free tropospheric O3 over the Middle East is about 2 times larger than that from global anthropogenic sources. The summertime free tropospheric O3 enhancement is primarily due to Asian NOx emissions.
Min Xie, Jingbiao Liao, Tijian Wang, Kuanguang Zhu, Bingliang Zhuang, Yong Han, Mengmeng Li, and Shu Li
Atmos. Chem. Phys., 16, 6071–6089, https://doi.org/10.5194/acp-16-6071-2016, https://doi.org/10.5194/acp-16-6071-2016, 2016
Short summary
Short summary
The spatial and temporal distribution of anthropogenic heat emissions over the YRD region was developed. These gridded AH emissions were incorporated into the modified WRF/Chem model with the seasonal and diurnal variation. The impacts of AH on meteorology and chemical variables were evaluated. The results show that the anthropogenic heat inputs improved the meteorology and air pollution predictions from WRF/Chem in and around large urban areas.
B. L. Zhuang, T. J. Wang, J. Liu, Y. Ma, C. Q. Yin, S. Li, M. Xie, Y. Han, J. L. Zhu, X. Q. Yang, and C. B. Fu
Atmos. Chem. Phys., 15, 13633–13646, https://doi.org/10.5194/acp-15-13633-2015, https://doi.org/10.5194/acp-15-13633-2015, 2015
Short summary
Short summary
The aerosol absorbing coefficient (AAC) assesses the direct radiative forcing of absorbing aerosols. The corrected AAC and absorption Ångström exponent (AAE) in Nanjing, YRD, are characterized using AE-31. Schmid-corrected AAC at 532nm and the AAE at 660/470nm are about 43.23±28.13 Mm-1 and 1.56, both with strong seasonal and diurnal variations. A high AAC is mostly resultant of local and subregional emissions in Nanjing. It peaks at RH values of 40, 65, and 80% at different AAE levels.
Y. C. Jiang, T. L. Zhao, J. Liu, X. D. Xu, C. H. Tan, X. H. Cheng, X. Y. Bi, J. B. Gan, J. F. You, and S. Z. Zhao
Atmos. Chem. Phys., 15, 13331–13338, https://doi.org/10.5194/acp-15-13331-2015, https://doi.org/10.5194/acp-15-13331-2015, 2015
Short summary
Short summary
An O3 episode with high night-time O3 was observed before typhoon landing over southeastern China. Variations in the observed O3, NO2, CO and meteorology during Typhoon Hagibis event clearly suggest a substantial impact of the peripheral downdrafts in the tropical cyclone on the high O3 episode. This study provides observational evidence of typhoon-driven intrusion of O3 from the upper troposphere and lower stratosphere to surface air threatening to ambient air quality.
Y. Zhou, H. Mao, K. Demerjian, C. Hogrefe, and J. Liu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-27253-2015, https://doi.org/10.5194/acpd-15-27253-2015, 2015
Revised manuscript not accepted
Short summary
Short summary
Baseline carbon monoxide (CO) and ozone (O3) were studied at seven rural sites in the Northeast U.S. during varying periods over 2001 – 2010. Baseline CO at all sites decreased significantly at a rate between -4.3 – -2.3 ppbv yr-1, while baseline O3 was relatively constant. Interannual and seasonal variations of baseline CO and O3 were related to increasing Asian emissions, NOx emissions reduction in urban areas, global biomass burning emissions, and meteorological conditions.
J. Zhu, T. Wang, J. Bieser, and V. Matthias
Atmos. Chem. Phys., 15, 8767–8779, https://doi.org/10.5194/acp-15-8767-2015, https://doi.org/10.5194/acp-15-8767-2015, 2015
Short summary
Short summary
This study estimated the contributions to mercury concentration and deposition in easter China from seven categories of emission sources by CMAQ-Hg. Also, this study focuses on diagnostic and process analyses for atmospheric mercury pollution formation and on identification of the dominant atmospheric processes for mercury.
H. Che, X.-Y. Zhang, X. Xia, P. Goloub, B. Holben, H. Zhao, Y. Wang, X.-C. Zhang, H. Wang, L. Blarel, B. Damiri, R. Zhang, X. Deng, Y. Ma, T. Wang, F. Geng, B. Qi, J. Zhu, J. Yu, Q. Chen, and G. Shi
Atmos. Chem. Phys., 15, 7619–7652, https://doi.org/10.5194/acp-15-7619-2015, https://doi.org/10.5194/acp-15-7619-2015, 2015
Short summary
Short summary
This work studied more than 10 years of measurements of aerosol optical depths (AODs) made for 50 sites of CARSNET compiled into a climatology of aerosol optical properties for China. It lets us see a detailed full-scale description of AOD observations over China. The results would benefit us a lot in comprehending the temporal and special distribution aerosol optical property over China. Also the data would be valuable to communities of aerosol satellite retrieval, modelling, etc.
K. Ding, J. Liu, A. Ding, Q. Liu, T. L. Zhao, J. Shi, Y. Han, H. Wang, and F. Jiang
Atmos. Chem. Phys., 15, 2843–2866, https://doi.org/10.5194/acp-15-2843-2015, https://doi.org/10.5194/acp-15-2843-2015, 2015
Short summary
Short summary
1. High CO abundances of 300-550 ppbv is shown in aircraft MOZAIC data between 700 and 300 hPa over East Asia in three episodes. Correspondingly, elevated CO is observed in satellite MOPITT data at similar altitudes.
2. GEOS-Chem and FLEXPART simulations reveal distinct uplifting processes for CO from fires and anthropogenic sources in the cases.
3. Topography in East Asia affects uplifting of CO in different ways.
4. The new version 5 MOPITT data can help diagnose vertical transport of CO.
J. Zhu, T. Wang, R. Talbot, H. Mao, X. Yang, C. Fu, J. Sun, B. Zhuang, S. Li, Y. Han, and M. Xie
Atmos. Chem. Phys., 14, 2233–2244, https://doi.org/10.5194/acp-14-2233-2014, https://doi.org/10.5194/acp-14-2233-2014, 2014
J. Liu, D. W. Tarasick, V. E. Fioletov, C. McLinden, T. Zhao, S. Gong, C. Sioris, J. J. Jin, G. Liu, and O. Moeini
Atmos. Chem. Phys., 13, 11441–11464, https://doi.org/10.5194/acp-13-11441-2013, https://doi.org/10.5194/acp-13-11441-2013, 2013
G. Liu, J. Liu, D. W. Tarasick, V. E. Fioletov, J. J. Jin, O. Moeini, X. Liu, C. E. Sioris, and M. Osman
Atmos. Chem. Phys., 13, 10659–10675, https://doi.org/10.5194/acp-13-10659-2013, https://doi.org/10.5194/acp-13-10659-2013, 2013
L. Xing, T.-M. Fu, J. J. Cao, S. C. Lee, G. H. Wang, K. F. Ho, M.-C. Cheng, C.-F. You, and T. J. Wang
Atmos. Chem. Phys., 13, 4307–4318, https://doi.org/10.5194/acp-13-4307-2013, https://doi.org/10.5194/acp-13-4307-2013, 2013
J. Zhu, T. Wang, R. Talbot, H. Mao, C. B. Hall, X. Yang, C. Fu, B. Zhuang, S. Li, Y. Han, and X. Huang
Atmos. Chem. Phys., 12, 12103–12118, https://doi.org/10.5194/acp-12-12103-2012, https://doi.org/10.5194/acp-12-12103-2012, 2012
Related subject area
Subject: Gases | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
How rainfall events modify trace gas mixing ratios in central Amazonia
Uncertainty in continuous ΔCO-based ΔffCO2 estimates derived from 14C flask and bottom-up ΔCO ∕ ΔffCO2 ratios
Dynamical drivers of free-tropospheric ozone increases over equatorial Southeast Asia
Air mass transport to the tropical western Pacific troposphere inferred from ozone and relative humidity balloon observations above Palau
Atmospheric NH3 in urban Beijing: long-term variations and implications for secondary inorganic aerosol control
Mixing-layer-height-referenced ozone vertical distribution in the lower troposphere of Chinese megacities: stratification, classification, and meteorological and photochemical mechanisms
Six years of continuous carbon isotope composition measurements of methane in Heidelberg (Germany) – a study of source contributions and comparison to emission inventories
What caused large ozone variabilities in three megacity clusters in eastern China during 2015–2020?
Atmospheric turbulence observed during a fuel-bed-scale low-intensity surface fire
Interannual variations in the Δ(17O) signature of atmospheric CO2 at two mid-latitude sites suggest a close link to stratosphere-troposphere exchange
Fingerprints of the COVID-19 economic downturn and recovery on ozone anomalies at high-elevation sites in North America and western Europe
Ozone in the boreal forest in the Alberta Oil Sands Region
Zugspitze ozone 1970–2020: the role of stratosphere–troposphere transport
High sulfur dioxide deposition velocities measured with the flux–gradient technique in a boreal forest in the Alberta Oil Sands Region
Quantification of methane emissions in Hamburg using a network of FTIR spectrometers and an inverse modeling approach
Local-to-regional methane emissions from the Upper Silesian Coal Basin (USCB) quantified using UAV-based atmospheric measurements
Transport pathways of carbon monoxide from Indonesian fire pollution to a subtropical high-altitude mountain site in the western North Pacific
Global warming will largely increase waste treatment CH4 emissions in Chinese megacities: insight from the first city-scale CH4 concentration observation network in Hangzhou, China
Disentangling methane and carbon dioxide sources and transport across the Russian Arctic from aircraft measurements
Airborne glyoxal measurements in the marine and continental atmosphere: comparison with TROPOMI observations and EMAC simulations
Mercury in the free troposphere and bidirectional atmosphere–vegetation exchanges – insights from Maïdo mountain observatory in the Southern Hemisphere tropics
Diurnal variability of atmospheric O2, CO2, and their exchange ratio above a boreal forest in southern Finland
How adequately are elevated moist layers represented in reanalysis and satellite observations?
Quantitative impacts of vertical transport on the long-term trend of nocturnal ozone increase over the Pearl River Delta region during 2006–2019
Factors influencing the temporal variability of atmospheric methane emissions from Upper Silesia coal mines: a case study from the CoMet mission
Enhanced natural releases of mercury in response to the reduction in anthropogenic emissions during the COVID-19 lockdown by explainable machine learning
Temporal variability of tropospheric ozone and ozone profiles in the Korean Peninsula during the East Asian summer monsoon: insights from multiple measurements and reanalysis datasets
Retrieving CH4-emission rates from coal mine ventilation shafts using UAV-based AirCore observations and the genetic algorithm–interior point penalty function (GA-IPPF) model
Measurement report: Atmospheric mercury in a coastal city of Southeast China – inter-annual variations and influencing factors
Tropospheric and stratospheric ozone profiles during the 2019 TROpomi vaLIdation eXperiment (TROLIX-19)
Evaluation of correlated Pandora column NO2 and in situ surface NO2 measurements during GMAP campaign
Transport of substantial stratospheric ozone to the surface by a dying typhoon and shallow convection
Observational constraints on methane emissions from Polish coal mines using a ground-based remote sensing network
Continuous CH4 and δ13CH4 measurements in London demonstrate under-reported natural gas leakage
Long-term fluxes of carbonyl sulfide and their seasonality and interannual variability in a boreal forest
Declines and peaks in NO2 pollution during the multiple waves of the COVID-19 pandemic in the New York metropolitan area
Measurement report: Characterization of uncertainties in fluxes and fuel sulfur content from ship emissions in the Baltic Sea
Limitations of the radon tracer method (RTM) to estimate regional greenhouse gas (GHG) emissions – a case study for methane in Heidelberg
Positive and negative influences of typhoons on tropospheric ozone over southern China
Spatial and temporal variations of CO2 mole fractions observed at Beijing, Xianghe, and Xinglong in North China
The CO2 integral emission by the megacity of St Petersburg as quantified from ground-based FTIR measurements combined with dispersion modelling
Anthropogenic and natural controls on atmospheric δ13C-CO2 variations in the Yangtze River delta: insights from a carbon isotope modeling framework
Quantifying variability, source, and transport of CO in the urban areas over the Himalayas and Tibetan Plateau
New methodology shows short atmospheric lifetimes of oxidized sulfur and nitrogen due to dry deposition
Uncertainties in eddy covariance air–sea CO2 flux measurements and implications for gas transfer velocity parameterisations
Convergent evidence for the pervasive but limited contribution of biomass burning to atmospheric ammonia in peninsular Southeast Asia
Concurrent variation in oil and gas methane emissions and oil price during the COVID-19 pandemic
Seasonal patterns of atmospheric mercury in tropical South America as inferred by a continuous total gaseous mercury record at Chacaltaya station (5240 m) in Bolivia
A mass-weighted isentropic coordinate for mapping chemical tracers and computing atmospheric inventories
Methane mapping, emission quantification, and attribution in two European cities: Utrecht (NL) and Hamburg (DE)
Luiz A. T. Machado, Jürgen Kesselmeier, Santiago Botía, Hella van Asperen, Meinrat O. Andreae, Alessandro C. de Araújo, Paulo Artaxo, Achim Edtbauer, Rosaria R. Ferreira, Marco A. Franco, Hartwig Harder, Sam P. Jones, Cléo Q. Dias-Júnior, Guido G. Haytzmann, Carlos A. Quesada, Shujiro Komiya, Jost Lavric, Jos Lelieveld, Ingeborg Levin, Anke Nölscher, Eva Pfannerstill, Mira L. Pöhlker, Ulrich Pöschl, Akima Ringsdorf, Luciana Rizzo, Ana M. Yáñez-Serrano, Susan Trumbore, Wanda I. D. Valenti, Jordi Vila-Guerau de Arellano, David Walter, Jonathan Williams, Stefan Wolff, and Christopher Pöhlker
Atmos. Chem. Phys., 24, 8893–8910, https://doi.org/10.5194/acp-24-8893-2024, https://doi.org/10.5194/acp-24-8893-2024, 2024
Short summary
Short summary
Composite analysis of gas concentration before and after rainfall, during the day and night, gives insight into the complex relationship between trace gas variability and precipitation. The analysis helps us to understand the sources and sinks of trace gases within a forest ecosystem. It elucidates processes that are not discernible under undisturbed conditions and contributes to a deeper understanding of the trace gas life cycle and its intricate interactions with cloud dynamics in the Amazon.
Fabian Maier, Ingeborg Levin, Sébastien Conil, Maksym Gachkivskyi, Hugo Denier van der Gon, and Samuel Hammer
Atmos. Chem. Phys., 24, 8205–8223, https://doi.org/10.5194/acp-24-8205-2024, https://doi.org/10.5194/acp-24-8205-2024, 2024
Short summary
Short summary
We assess the uncertainty in continuous fossil fuel carbon dioxide (ffCO2) estimates derived from carbon monoxide (CO) observations and radiocarbon (14CO2) flask measurements from an urban and a rural site. This study provides the basis for using continuous CO-based ffCO2 observations in atmospheric transport inversion frameworks to derive ffCO2 emission estimates. We also compare the flask-based CO / ffCO2 ratios with modeled ratios to validate an emission inventory for central Europe.
Ryan M. Stauffer, Anne M. Thompson, Debra E. Kollonige, Ninong Komala, Habib Khirzin Al-Ghazali, Dian Yudha Risdianto, Ambun Dindang, Ahmad Fairudz bin Jamaluddin, Mohan Kumar Sammathuria, Norazura Binti Zakaria, Bryan J. Johnson, and Patrick D. Cullis
Atmos. Chem. Phys., 24, 5221–5234, https://doi.org/10.5194/acp-24-5221-2024, https://doi.org/10.5194/acp-24-5221-2024, 2024
Short summary
Short summary
SHADOZ balloon-borne ozone measurements over equatorial Southeast Asia from 1998–2022 reveal that ozone increases during the early months of the year are linked to reduced convective storm activity, which typically redistributes and cleans the atmosphere of ozone. These findings challenge models to replicate the trends produced by the SHADOZ and meteorological observations and emphasize the importance of studying monthly or seasonal instead of annual changes for understanding ozone trends.
Katrin Müller, Peter von der Gathen, and Markus Rex
Atmos. Chem. Phys., 24, 4693–4716, https://doi.org/10.5194/acp-24-4693-2024, https://doi.org/10.5194/acp-24-4693-2024, 2024
Short summary
Short summary
The transport history of tropospheric air masses above the tropical western Pacific is studied by local ozone and relative humidity profile measurements from Palau. A prominent anti-correlation between both tracers separates air masses of different origin and genesis. Back trajectories confirm a local convective origin of the year-round humid ozone-poor background. Anomalously dry ozone-rich air is generated in tropical Asia by pollution and dehydrated during transport via radiative cooling.
Ziru Lan, Xiaoyi Zhang, Weili Lin, Xiaobin Xu, Zhiqiang Ma, Jun Jin, Lingyan Wu, and Yangmei Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2024-375, https://doi.org/10.5194/egusphere-2024-375, 2024
Short summary
Short summary
Our study examined the long-term trends of atmospheric ammonia in urban Beijing from 2009 to 2020. We found that the trends didn't match satellite data or emissions estimates, revealing complexities in ammonia sources. While seasonal variations in ammonia were temperature-dependent, daily variations were correlated with water vapor. We also found an increasing contribution of ammonia reduction, emphasizing its importance in mitigating fine particulate matter in Beijing.
Zhiheng Liao, Meng Gao, Jinqiang Zhang, Jiaren Sun, Jiannong Quan, Xingcan Jia, Yubing Pan, and Shaojia Fan
Atmos. Chem. Phys., 24, 3541–3557, https://doi.org/10.5194/acp-24-3541-2024, https://doi.org/10.5194/acp-24-3541-2024, 2024
Short summary
Short summary
This study collected 1897 ozonesondes from two Chinese megacities (Beijing and Hong Kong) in 2000–2022 to investigate the climatological vertical heterogeneity of lower-tropospheric ozone distribution with a mixing-layer-height-referenced (h-referenced) vertical coordinate system. This vertical coordinate system highlighted O3 stratification features existing at the mixing layer–free troposphere interface and provided a better understanding of O3 pollution in urban regions.
Antje Hoheisel and Martina Schmidt
Atmos. Chem. Phys., 24, 2951–2969, https://doi.org/10.5194/acp-24-2951-2024, https://doi.org/10.5194/acp-24-2951-2024, 2024
Short summary
Short summary
In Heidelberg, Germany, methane and its stable carbon isotope composition have been measured continuously with a cavity ring-down spectroscopy (CRDS) analyser since April 2014. These 6-year time series are analysed with the Keeling plot method for the isotopic composition of the sources, as well as seasonal variations and trends in methane emissions. The source contributions derived from atmospheric measurements were used to evaluate global and regional emission inventories of methane.
Tingting Hu, Yu Lin, Run Liu, Yuepeng Xu, Shanshan Ouyang, Boguang Wang, Yuanhang Zhang, and Shaw Chen Liu
Atmos. Chem. Phys., 24, 1607–1626, https://doi.org/10.5194/acp-24-1607-2024, https://doi.org/10.5194/acp-24-1607-2024, 2024
Short summary
Short summary
We hypothesize that the cause of the worsening O3 trends in the Beijing–Tianjin–Hebei region, the Yangtze River Delta, and Pearl River Delta from 2015 to 2020 is attributable to the increased occurrence of meteorological conditions of high solar radiation and a positive temperature anomaly under the influence of West Pacific subtropical high, tropical cyclones, and mid–high-latitude wave activities.
Joseph Seitz, Shiyuan Zhong, Joseph J. Charney, Warren E. Heilman, Kenneth L. Clark, Xindi Bian, Nicholas S. Skowronski, Michael R. Gallagher, Matthew Patterson, Jason Cole, Michael T. Kiefer, Rory Hadden, and Eric Mueller
Atmos. Chem. Phys., 24, 1119–1142, https://doi.org/10.5194/acp-24-1119-2024, https://doi.org/10.5194/acp-24-1119-2024, 2024
Short summary
Short summary
Atmospheric turbulence affects wildland fire behaviors and heat and smoke transfer. Turbulence data collected during an experimental fire on a 10 m x 10 m densely instrumented burn plot are analyzed, and the results reveal substantial heterogeneity in fire-induced turbulence characteristics across the small plot, which highlights the necessity for coupled atmosphere–fire behavior models to have 1–2 m grid spacing so that adequate simulations of fire behavior and smoke transfer can be achieved.
Pharahilda M. Steur, Hubertus A. Scheeren, Gerbrand Koren, Getachew A. Adnew, Wouter Peters, and Harro A. J. Meijer
EGUsphere, https://doi.org/10.5194/egusphere-2023-2924, https://doi.org/10.5194/egusphere-2023-2924, 2024
Short summary
Short summary
We present records of the triple oxygen isotope signature (Δ(17O)) of atmospheric CO2 conducted with laser absorption spectroscopy from two mid-latitude stations. Significant interannual variability is observed in both records. A model sensitivity study suggests that stratosphere-troposphere exchange, carrying high Δ(17O) CO2 from the stratosphere into the troposphere, causes most of the variability. This makes Δ(17O) a potential tracer for stratospheric intrusions in the troposphere.
Davide Putero, Paolo Cristofanelli, Kai-Lan Chang, Gaëlle Dufour, Gregory Beachley, Cédric Couret, Peter Effertz, Daniel A. Jaffe, Dagmar Kubistin, Jason Lynch, Irina Petropavlovskikh, Melissa Puchalski, Timothy Sharac, Barkley C. Sive, Martin Steinbacher, Carlos Torres, and Owen R. Cooper
Atmos. Chem. Phys., 23, 15693–15709, https://doi.org/10.5194/acp-23-15693-2023, https://doi.org/10.5194/acp-23-15693-2023, 2023
Short summary
Short summary
We investigated the impact of societal restriction measures during the COVID-19 pandemic on surface ozone at 41 high-elevation sites worldwide. Negative ozone anomalies were observed for spring and summer 2020 for all of the regions considered. In 2021, negative anomalies continued for Europe and partially for the eastern US, while western US sites showed positive anomalies due to wildfires. IASI satellite data and the Carbon Monitor supported emission reductions as a cause of the anomalies.
Xuanyi Zhang, Mark Gordon, Paul A. Makar, Timothy Jiang, Jonathan Davies, and David Tarasick
Atmos. Chem. Phys., 23, 13647–13664, https://doi.org/10.5194/acp-23-13647-2023, https://doi.org/10.5194/acp-23-13647-2023, 2023
Short summary
Short summary
Measurements of ozone in the atmosphere were made in a forest downwind of oil sands mining and production facilities in northern Alberta. These measurements show that the emissions of other pollutants from oil sands production and processing reduce the amount of ozone in the forest. By using an atmospheric model combined with measurements, we find that the rate at which ozone is absorbed by the forest is lower than typical rates from similar measurements in other forests.
Thomas Trickl, Cédric Couret, Ludwig Ries, and Hannes Vogelmann
Atmos. Chem. Phys., 23, 8403–8427, https://doi.org/10.5194/acp-23-8403-2023, https://doi.org/10.5194/acp-23-8403-2023, 2023
Short summary
Short summary
Downward atmospheric transport from the stratosphere (STT) is the most important natural source of tropospheric ozone. We analyse the stratospheric influence on the long-term series of ozone and carbon monoxide measured on the Zugspitze in the Bavarian Alps (2962 m a.s.l.). Since the 1970s, there has been a pronounced ozone rise that has been ascribed to an increase in STT. We determine the stratospheric influence from the observational data alone (humidity and 7Be).
Mark Gordon, Dane Blanchard, Timothy Jiang, Paul A. Makar, Ralf M. Staebler, Julian Aherne, Cris Mihele, and Xuanyi Zhang
Atmos. Chem. Phys., 23, 7241–7255, https://doi.org/10.5194/acp-23-7241-2023, https://doi.org/10.5194/acp-23-7241-2023, 2023
Short summary
Short summary
Measurements of the gas sulfur dioxide (SO2) were made in a forest downwind of oil sands mining and production facilities in northern Alberta. These measurements tell us the rate at which SO2 is absorbed by the forest. The measured rate is much higher than what is currently used by air quality models, which is supported by a previous study in this region. This suggests that SO2 may have a much shorter lifetime in the atmosphere at this location than currently predicted by models.
Andreas Forstmaier, Jia Chen, Florian Dietrich, Juan Bettinelli, Hossein Maazallahi, Carsten Schneider, Dominik Winkler, Xinxu Zhao, Taylor Jones, Carina van der Veen, Norman Wildmann, Moritz Makowski, Aydin Uzun, Friedrich Klappenbach, Hugo Denier van der Gon, Stefan Schwietzke, and Thomas Röckmann
Atmos. Chem. Phys., 23, 6897–6922, https://doi.org/10.5194/acp-23-6897-2023, https://doi.org/10.5194/acp-23-6897-2023, 2023
Short summary
Short summary
Large cities emit greenhouse gases which contribute to global warming. In this study, we measured the release of one important green house gas, methane, in Hamburg. Multiple sources that contribute to methane emissions were located and quantified. Methane sources were found to be mainly caused by human activity (e.g., by release from oil and gas refineries). Moreover, potential natural sources have been located, such as the Elbe River and lakes.
Truls Andersen, Zhao Zhao, Marcel de Vries, Jaroslaw Necki, Justyna Swolkien, Malika Menoud, Thomas Röckmann, Anke Roiger, Andreas Fix, Wouter Peters, and Huilin Chen
Atmos. Chem. Phys., 23, 5191–5216, https://doi.org/10.5194/acp-23-5191-2023, https://doi.org/10.5194/acp-23-5191-2023, 2023
Short summary
Short summary
The Upper Silesian Coal Basin, Poland, is one of the hot spots of methane emissions in Europe. Using an uncrewed aerial vehicle (UAV), we performed atmospheric measurements of methane concentrations downwind of five ventilation shafts in this region and determined the emission rates from the individual shafts. We found a strong correlation between quantified shaft-averaged emission rates and hourly inventory data, which also allows us to estimate the methane emissions from the entire region.
Saginela Ravindra Babu, Chang-Feng Ou-Yang, Stephen M. Griffith, Shantanu Kumar Pani, Steven Soon-Kai Kong, and Neng-Huei Lin
Atmos. Chem. Phys., 23, 4727–4740, https://doi.org/10.5194/acp-23-4727-2023, https://doi.org/10.5194/acp-23-4727-2023, 2023
Short summary
Short summary
In October 2006 and 2015, extensive fire episodes occurred in Indonesia, releasing an enormous amount of CO emissions. By combining in situ and satellite CO measurements and reanalysis products, we reported plausible transport pathways of CO from Indonesia to the Lulin Atmospheric Background Station (LABS; 23.47° N, 120.87° E; 2862 m a.s.l.) in Taiwan. We identified (i) horizontal transport in the free troposphere and (ii) vertical transport through the Hadley circulation.
Cheng Hu, Junqing Zhang, Bing Qi, Rongguang Du, Xiaofei Xu, Haoyu Xiong, Huili Liu, Xinyue Ai, Yiyi Peng, and Wei Xiao
Atmos. Chem. Phys., 23, 4501–4520, https://doi.org/10.5194/acp-23-4501-2023, https://doi.org/10.5194/acp-23-4501-2023, 2023
Short summary
Short summary
We build the first city-scale tower-based atmospheric CH4 concentration observation network in China. The a priori total annual anthropogenic CH4 emissions and emissions from waste treatment were overestimated by 36.0 % and 47.1 %, respectively, in Hangzhou. Global warming will largely enhance the CH4 emission factor of waste treatment, which will increase by 17.6 %, 9.6 %, 5.6 % and 4.0 % for Representative Concentration Pathway (RCP) 8.5, RCP6.0, RCP4.5 and RCP2.6, respectively, by 2100.
Clément Narbaud, Jean-Daniel Paris, Sophie Wittig, Antoine Berchet, Marielle Saunois, Philippe Nédélec, Boris D. Belan, Mikhail Y. Arshinov, Sergei B. Belan, Denis Davydov, Alexander Fofonov, and Artem Kozlov
Atmos. Chem. Phys., 23, 2293–2314, https://doi.org/10.5194/acp-23-2293-2023, https://doi.org/10.5194/acp-23-2293-2023, 2023
Short summary
Short summary
We measured CH4 and CO2 from aircraft over the Russian Arctic. Analyzing our data with the Lagrangian model FLEXPART, we find a sharp east–west gradient in atmospheric composition. Western Siberia is influenced by strong wetland CH4 emissions, deep CO2 gradient from biospheric uptake, and long-range transport from Europe and North America. Eastern flights document less variability. Over the Arctic Ocean, we find a small influence from marine CH4 emissions compatible with reasonable inventories.
Flora Kluge, Tilman Hüneke, Christophe Lerot, Simon Rosanka, Meike K. Rotermund, Domenico Taraborrelli, Benjamin Weyland, and Klaus Pfeilsticker
Atmos. Chem. Phys., 23, 1369–1401, https://doi.org/10.5194/acp-23-1369-2023, https://doi.org/10.5194/acp-23-1369-2023, 2023
Short summary
Short summary
Using airborne glyoxal concentration and vertical column density measurements, vertical profiles are inferred for eight global regions in aged biomass burning plumes and the tropical marine boundary layer. Using TROPOMI observations, an analysis of space- and airborne measurements is performed. A comparison to EMAC simulations shows a general glyoxal underprediction, which points to various missing sources and precursors from anthropogenic activities, biomass burning, and the sea surface.
Alkuin M. Koenig, Olivier Magand, Bert Verreyken, Jerome Brioude, Crist Amelynck, Niels Schoon, Aurélie Colomb, Beatriz Ferreira Araujo, Michel Ramonet, Mahesh K. Sha, Jean-Pierre Cammas, Jeroen E. Sonke, and Aurélien Dommergue
Atmos. Chem. Phys., 23, 1309–1328, https://doi.org/10.5194/acp-23-1309-2023, https://doi.org/10.5194/acp-23-1309-2023, 2023
Short summary
Short summary
The global distribution of mercury, a potent neurotoxin, depends on atmospheric transport, chemistry, and interactions between the Earth’s surface and the air. Our understanding of these processes is still hampered by insufficient observations. Here, we present new data from a mountain observatory in the Southern Hemisphere. We give insights into mercury concentrations in air masses coming from aloft, and we show that tropical mountain vegetation may be a daytime source of mercury to the air.
Kim A. P. Faassen, Linh N. T. Nguyen, Eadin R. Broekema, Bert A. M. Kers, Ivan Mammarella, Timo Vesala, Penelope A. Pickers, Andrew C. Manning, Jordi Vilà-Guerau de Arellano, Harro A. J. Meijer, Wouter Peters, and Ingrid T. Luijkx
Atmos. Chem. Phys., 23, 851–876, https://doi.org/10.5194/acp-23-851-2023, https://doi.org/10.5194/acp-23-851-2023, 2023
Short summary
Short summary
The exchange ratio (ER) between atmospheric O2 and CO2 provides a useful tracer for separately estimating photosynthesis and respiration processes in the forest carbon balance. This is highly relevant to better understand the expected biosphere sink, which determines future atmospheric CO2 levels. We therefore measured O2, CO2, and their ER above a boreal forest in Finland and investigated their diurnal behaviour for a representative day, and we show the most suitable way to determine the ER.
Marc Prange, Stefan A. Buehler, and Manfred Brath
Atmos. Chem. Phys., 23, 725–741, https://doi.org/10.5194/acp-23-725-2023, https://doi.org/10.5194/acp-23-725-2023, 2023
Short summary
Short summary
We investigate the representation of elevated moist layers (EMLs) in two satellite retrieval products and ERA5 reanalysis. EMLs occur in the vicinity of tropical convective storms and are thought to have an impact on their evolution through radiative heating. We provide a first dedicated assessment of EMLs in long-term data products in terms of moist layer strength, vertical thickness and altitude by comparing to collocated radiosondes over the western Pacific, a region where EMLs often occur.
Yongkang Wu, Weihua Chen, Yingchang You, Qianqian Xie, Shiguo Jia, and Xuemei Wang
Atmos. Chem. Phys., 23, 453–469, https://doi.org/10.5194/acp-23-453-2023, https://doi.org/10.5194/acp-23-453-2023, 2023
Short summary
Short summary
Relying on observed and simulated data, we determine the spatiotemporal characteristics of nocturnal O3 increase (NOI) events in the Pearl River Delta region during 2006–2019. Low-level jets and convective storms are the main meteorological processes causing NOI. Daytime O3 is another essential influencing factor. More importantly, a more prominent role of meteorological processes in NOI has been demonstrated. Our study highlights the important role of meteorology in nocturnal O3 pollution.
Justyna Swolkień, Andreas Fix, and Michał Gałkowski
Atmos. Chem. Phys., 22, 16031–16052, https://doi.org/10.5194/acp-22-16031-2022, https://doi.org/10.5194/acp-22-16031-2022, 2022
Short summary
Short summary
Determination of emissions from coal mines on a local scale requires instantaneous data. We analysed temporal emission data for ventilation shafts and factors influencing their variability. They were saturation of the seams with methane, the permeability of the rock mass, and coal output. The data for the verification should reflect the actual values of emissions from point sources. It is recommended to achieve this by using a standardised emission measurement system for all coal mines.
Xiaofei Qin, Shengqian Zhou, Hao Li, Guochen Wang, Cheng Chen, Chengfeng Liu, Xiaohao Wang, Juntao Huo, Yanfen Lin, Jia Chen, Qingyan Fu, Yusen Duan, Kan Huang, and Congrui Deng
Atmos. Chem. Phys., 22, 15851–15865, https://doi.org/10.5194/acp-22-15851-2022, https://doi.org/10.5194/acp-22-15851-2022, 2022
Short summary
Short summary
Using artificial neural network modeling and an explainable analysis approach, natural surface emissions (NSEs) were identified as a main driver of gaseous elemental mercury (GEM) variations during the COVID-19 lockdown. A sharp drop in GEM concentrations due to a significant reduction in anthropogenic emissions may disrupt the surface–air exchange balance of Hg, leading to increases in NSEs. This implies that NSEs may pose challenges to the future control of Hg pollution.
Juseon Bak, Eun-Ji Song, Hyo-Jung Lee, Xiong Liu, Ja-Ho Koo, Joowan Kim, Wonbae Jeon, Jae-Hwan Kim, and Cheol-Hee Kim
Atmos. Chem. Phys., 22, 14177–14187, https://doi.org/10.5194/acp-22-14177-2022, https://doi.org/10.5194/acp-22-14177-2022, 2022
Short summary
Short summary
Our study investigates the temporal variations of ozone profiles at Pohang in the Korean Peninsula from multiple ozone products. We discuss the quantitative relationships between daily surface measurements and key meteorological variables, different seasonality of ozone between the troposphere and stratosphere, and interannual changes in the lower tropospheric ozone, linked by the weather pattern driven by the East Asian summer monsoon.
Tianqi Shi, Zeyu Han, Ge Han, Xin Ma, Huilin Chen, Truls Andersen, Huiqin Mao, Cuihong Chen, Haowei Zhang, and Wei Gong
Atmos. Chem. Phys., 22, 13881–13896, https://doi.org/10.5194/acp-22-13881-2022, https://doi.org/10.5194/acp-22-13881-2022, 2022
Short summary
Short summary
CH4 works as the second-most important greenhouse gas, its reported emission inventories being far less than CO2. In this study, we developed a self-adjusted model to estimate the CH4 emission rate from strong point sources by the UAV-based AirCore system. This model would reduce the uncertainty in CH4 emission rate quantification accrued by errors in measurements of wind and concentration. Actual measurements on Pniówek coal demonstrate the high accuracy and stability of our developed model.
Jiayan Shi, Yuping Chen, Lingling Xu, Youwei Hong, Mengren Li, Xiaolong Fan, Liqian Yin, Yanting Chen, Chen Yang, Gaojie Chen, Taotao Liu, Xiaoting Ji, and Jinsheng Chen
Atmos. Chem. Phys., 22, 11187–11202, https://doi.org/10.5194/acp-22-11187-2022, https://doi.org/10.5194/acp-22-11187-2022, 2022
Short summary
Short summary
Gaseous elemental mercury (GEM) was observed in Southeast China over the period 2012–2020. The observed GEM concentrations showed no distinct inter-annual variation trends. The interpretation rate of transportation and meteorology on GEM variations displayed an increasing trend. In contrast, anthropogenic emissions have shown a decreasing interpretation rate since 2012, indicating the effectiveness of emission mitigation measures in reducing GEM concentrations in the study region.
John T. Sullivan, Arnoud Apituley, Nora Mettig, Karin Kreher, K. Emma Knowland, Marc Allaart, Ankie Piters, Michel Van Roozendael, Pepijn Veefkind, Jerry R. Ziemke, Natalya Kramarova, Mark Weber, Alexei Rozanov, Laurence Twigg, Grant Sumnicht, and Thomas J. McGee
Atmos. Chem. Phys., 22, 11137–11153, https://doi.org/10.5194/acp-22-11137-2022, https://doi.org/10.5194/acp-22-11137-2022, 2022
Short summary
Short summary
A TROPOspheric Monitoring Instrument (TROPOMI) validation campaign (TROLIX-19) was held in the Netherlands in September 2019. The research presented here focuses on using ozone lidars from NASA’s Goddard Space Flight Center to better evaluate the characterization of ozone throughout TROLIX-19 as compared to balloon-borne, space-borne and ground-based passive measurements, as well as a global coupled chemistry meteorology model.
Lim-Seok Chang, Donghee Kim, Hyunkee Hong, Deok-Rae Kim, Jeong-Ah Yu, Kwangyul Lee, Hanlim Lee, Daewon Kim, Jinkyu Hong, Hyun-Young Jo, and Cheol-Hee Kim
Atmos. Chem. Phys., 22, 10703–10720, https://doi.org/10.5194/acp-22-10703-2022, https://doi.org/10.5194/acp-22-10703-2022, 2022
Short summary
Short summary
Our study explored the synergy of combined column and surface measurements during GMAP (GEMS Map of Air Pollution) campaign. It has several points to note for vertical distribution analysis. Particularly under prevailing local wind meteorological conditions, Pandora-based vertical structures sometimes showed negative correlations between column and surface measurements. Vertical analysis should be done carefully in some local meteorological conditions when employing either surface or columns.
Zhixiong Chen, Jane Liu, Xiushu Qie, Xugeng Cheng, Yukun Shen, Mengmiao Yang, Rubin Jiang, and Xiangke Liu
Atmos. Chem. Phys., 22, 8221–8240, https://doi.org/10.5194/acp-22-8221-2022, https://doi.org/10.5194/acp-22-8221-2022, 2022
Short summary
Short summary
A vigorous surface ozone surge event of stratospheric origin occurred in the North China Plain at night. Surface ozone concentrations were 40–50 ppbv higher than the corresponding monthly mean, whereas surface carbon monoxide concentrations declined abruptly, which confirmed the direct stratospheric intrusions to the surface. We further addressed the notion that a combined effect of the dying typhoon and mesoscale convective systems was responsible for this vigorous ozone surge.
Andreas Luther, Julian Kostinek, Ralph Kleinschek, Sara Defratyka, Mila Stanisavljević, Andreas Forstmaier, Alexandru Dandocsi, Leon Scheidweiler, Darko Dubravica, Norman Wildmann, Frank Hase, Matthias M. Frey, Jia Chen, Florian Dietrich, Jarosław Nȩcki, Justyna Swolkień, Christoph Knote, Sanam N. Vardag, Anke Roiger, and André Butz
Atmos. Chem. Phys., 22, 5859–5876, https://doi.org/10.5194/acp-22-5859-2022, https://doi.org/10.5194/acp-22-5859-2022, 2022
Short summary
Short summary
Coal mining is an extensive source of anthropogenic methane emissions. In order to reduce and mitigate methane emissions, it is important to know how much and where the methane is emitted. We estimated coal mining methane emissions in Poland based on atmospheric methane measurements and particle dispersion modeling. In general, our emission estimates suggest higher emissions than expected by previous annual emission reports.
Eric Saboya, Giulia Zazzeri, Heather Graven, Alistair J. Manning, and Sylvia Englund Michel
Atmos. Chem. Phys., 22, 3595–3613, https://doi.org/10.5194/acp-22-3595-2022, https://doi.org/10.5194/acp-22-3595-2022, 2022
Short summary
Short summary
Continuous measurements of atmospheric methane concentrations and its carbon-13 isotope have been made in central London since early 2018. These measurements were used to evaluate methane emissions reported in global and UK-specific emission inventories for the London area. Compared to atmospheric methane measurements from March 2018 to October 2020, both inventories are under-reporting natural gas leakage for the London area.
Timo Vesala, Kukka-Maaria Kohonen, Linda M. J. Kooijmans, Arnaud P. Praplan, Lenka Foltýnová, Pasi Kolari, Markku Kulmala, Jaana Bäck, David Nelson, Dan Yakir, Mark Zahniser, and Ivan Mammarella
Atmos. Chem. Phys., 22, 2569–2584, https://doi.org/10.5194/acp-22-2569-2022, https://doi.org/10.5194/acp-22-2569-2022, 2022
Short summary
Short summary
Carbonyl sulfide (COS) provides new insights into carbon cycle research. We present an easy-to-use flux parameterization and the longest existing time series of forest–atmosphere COS exchange measurements, which allow us to study both seasonal and interannual variability. We observed only uptake of COS by the forest on an annual basis, with 37 % variability between years. Upscaling the boreal COS uptake using a biosphere model indicates a significant missing COS sink at high latitudes.
Maria Tzortziou, Charlotte F. Kwong, Daniel Goldberg, Luke Schiferl, Róisín Commane, Nader Abuhassan, James J. Szykman, and Lukas C. Valin
Atmos. Chem. Phys., 22, 2399–2417, https://doi.org/10.5194/acp-22-2399-2022, https://doi.org/10.5194/acp-22-2399-2022, 2022
Short summary
Short summary
The COVID-19 pandemic created an extreme natural experiment in which sudden changes in human behavior significantly impacted urban air quality. Using a combination of model, satellite, and ground-based data, we examine the impact of multiple waves and phases of the pandemic on atmospheric nitrogen pollution in the New York metropolitan area, and address the role of weather as a key driver of high pollution episodes observed even during – and despite – the stringent early lockdowns.
Jari Walden, Liisa Pirjola, Tuomas Laurila, Juha Hatakka, Heidi Pettersson, Tuomas Walden, Jukka-Pekka Jalkanen, Harri Nordlund, Toivo Truuts, Miika Meretoja, and Kimmo K. Kahma
Atmos. Chem. Phys., 21, 18175–18194, https://doi.org/10.5194/acp-21-18175-2021, https://doi.org/10.5194/acp-21-18175-2021, 2021
Short summary
Short summary
Ship emissions play an important role in the deposition of gaseous compounds and nanoparticles (Ntot), affecting climate, human health (especially in coastal areas), and eutrophication. Micrometeorological methods showed that ship emissions were mainly responsible for the deposition of Ntot, whereas they only accounted for a minor proportion of CO2 deposition. An uncertainty analysis applied to the fluxes and fuel sulfur content results demonstrated the reliability of the results.
Ingeborg Levin, Ute Karstens, Samuel Hammer, Julian DellaColetta, Fabian Maier, and Maksym Gachkivskyi
Atmos. Chem. Phys., 21, 17907–17926, https://doi.org/10.5194/acp-21-17907-2021, https://doi.org/10.5194/acp-21-17907-2021, 2021
Short summary
Short summary
The radon tracer method is applied to atmospheric methane and radon observations from the upper Rhine valley to independently estimate methane emissions from the region. Comparison of our top-down results with bottom-up inventory data requires high-resolution footprint modelling and representative radon flux data. In agreement with inventories, observed emissions decreased, but only until 2005. A limitation of this method is that point-source emissions are not captured or not fully captured.
Zhixiong Chen, Jane Liu, Xugeng Cheng, Mengmiao Yang, and Hong Wang
Atmos. Chem. Phys., 21, 16911–16923, https://doi.org/10.5194/acp-21-16911-2021, https://doi.org/10.5194/acp-21-16911-2021, 2021
Short summary
Short summary
Using a large ensemble of typhoons, we investigate the impacts of evolving typhoons on tropospheric ozone and address the linkages between typhoon-affected meteorological conditions and ozone variations. The influences of typhoon-induced stratospheric intrusions on lower-troposphere ozone are also quantified. Thus, the results obtained in this study have important implications for a full understanding of the multifaced roles of typhoons in modulating tropospheric ozone variation.
Yang Yang, Minqiang Zhou, Ting Wang, Bo Yao, Pengfei Han, Denghui Ji, Wei Zhou, Yele Sun, Gengchen Wang, and Pucai Wang
Atmos. Chem. Phys., 21, 11741–11757, https://doi.org/10.5194/acp-21-11741-2021, https://doi.org/10.5194/acp-21-11741-2021, 2021
Short summary
Short summary
This study introduces the in situ CO2 measurement system installed in Beijing (urban), Xianghe (suburban), and Xinglong (rural) in North China for the first time. The spatial and temporal variations in CO2 mole fractions at the three sites between June 2018 and April 2020 are discussed on both seasonal and diurnal scales.
Dmitry V. Ionov, Maria V. Makarova, Frank Hase, Stefani C. Foka, Vladimir S. Kostsov, Carlos Alberti, Thomas Blumenstock, Thorsten Warneke, and Yana A. Virolainen
Atmos. Chem. Phys., 21, 10939–10963, https://doi.org/10.5194/acp-21-10939-2021, https://doi.org/10.5194/acp-21-10939-2021, 2021
Short summary
Short summary
Megacities are a significant source of emissions of various substances in the atmosphere, including carbon dioxide, which is the most important anthropogenic greenhouse gas. In 2019–2020, the Emission Monitoring Mobile Experiment was carried out in St Petersburg, which is the second-largest industrial city in Russia. The results of this experiment, coupled with numerical modelling, helped to estimate the amount of CO2 emitted by the city. This value was twice as high as predicted.
Cheng Hu, Jiaping Xu, Cheng Liu, Yan Chen, Dong Yang, Wenjing Huang, Lichen Deng, Shoudong Liu, Timothy J. Griffis, and Xuhui Lee
Atmos. Chem. Phys., 21, 10015–10037, https://doi.org/10.5194/acp-21-10015-2021, https://doi.org/10.5194/acp-21-10015-2021, 2021
Short summary
Short summary
Seventy percent of global CO2 emissions were emitted from urban landscapes. The Yangtze River delta (YRD) ranks as one of the most densely populated regions in the world and is an anthropogenic CO2 hotspot. Besides anthropogenic factors, natural ecosystems and croplands act as significant CO2 sinks and sources. Independent quantification of the fossil and cement CO2 emission and assessment of their impact on atmospheric δ13C-CO2 have potential to improve our understanding of urban CO2 cycling.
Youwen Sun, Hao Yin, Yuan Cheng, Qianggong Zhang, Bo Zheng, Justus Notholt, Xiao Lu, Cheng Liu, Yuan Tian, and Jianguo Liu
Atmos. Chem. Phys., 21, 9201–9222, https://doi.org/10.5194/acp-21-9201-2021, https://doi.org/10.5194/acp-21-9201-2021, 2021
Short summary
Short summary
We quantified the variability, source, and transport of urban CO over the Himalayas and Tibetan Plateau (HTP) by using measurement, model simulation, and the analysis of meteorological fields. Urban CO over the HTP is dominated by anthropogenic and biomass burning emissions from local, South Asia and East Asia, and oxidation sources. The decreasing trends in surface CO since 2015 in most cities over the HTP are attributed to the reduction in local and transported CO emissions in recent years.
Katherine Hayden, Shao-Meng Li, Paul Makar, John Liggio, Samar G. Moussa, Ayodeji Akingunola, Robert McLaren, Ralf M. Staebler, Andrea Darlington, Jason O'Brien, Junhua Zhang, Mengistu Wolde, and Leiming Zhang
Atmos. Chem. Phys., 21, 8377–8392, https://doi.org/10.5194/acp-21-8377-2021, https://doi.org/10.5194/acp-21-8377-2021, 2021
Short summary
Short summary
We developed a method using aircraft measurements to determine lifetimes with respect to dry deposition for oxidized sulfur and nitrogen compounds over the boreal forest in Alberta, Canada. Atmospheric lifetimes were significantly shorter than derived from chemical transport models with differences related to modelled dry deposition velocities. The shorter lifetimes suggest models need to reassess dry deposition treatment and predictions of sulfur and nitrogen in the atmosphere and ecosystems.
Yuanxu Dong, Mingxi Yang, Dorothee C. E. Bakker, Vassilis Kitidis, and Thomas G. Bell
Atmos. Chem. Phys., 21, 8089–8110, https://doi.org/10.5194/acp-21-8089-2021, https://doi.org/10.5194/acp-21-8089-2021, 2021
Short summary
Short summary
Eddy covariance (EC) is the most direct method for measuring air–sea CO2 flux from ships. However, uncertainty in EC air–sea CO2 fluxes has not been well quantified. Here we show that with the state-of-the-art gas analysers, instrumental noise no longer contributes significantly to the CO2 flux uncertainty. Applying an appropriate averaging timescale (1–3 h) and suitable air–sea CO2 fugacity threshold (at least 20 µatm) to EC flux data enables an optimal analysis of the gas transfer velocity.
Yunhua Chang, Yan-Lin Zhang, Sawaeng Kawichai, Qian Wang, Martin Van Damme, Lieven Clarisse, Tippawan Prapamontol, and Moritz F. Lehmann
Atmos. Chem. Phys., 21, 7187–7198, https://doi.org/10.5194/acp-21-7187-2021, https://doi.org/10.5194/acp-21-7187-2021, 2021
Short summary
Short summary
In this study, we integrated satellite constraints on atmospheric NH3 levels and fire intensity, discrete NH3 concentration measurement, and N isotopic analysis of NH3 in order to assess the regional-scale contribution of biomass burning to ambient atmospheric NH3 in the heartland of Southeast Asia. The combined approach provides a valuable cross-validation framework for source apportioning of NH3 in the lower atmosphere and will thus help to ameliorate predictions of biomass burning emissions.
David R. Lyon, Benjamin Hmiel, Ritesh Gautam, Mark Omara, Katherine A. Roberts, Zachary R. Barkley, Kenneth J. Davis, Natasha L. Miles, Vanessa C. Monteiro, Scott J. Richardson, Stephen Conley, Mackenzie L. Smith, Daniel J. Jacob, Lu Shen, Daniel J. Varon, Aijun Deng, Xander Rudelis, Nikhil Sharma, Kyle T. Story, Adam R. Brandt, Mary Kang, Eric A. Kort, Anthony J. Marchese, and Steven P. Hamburg
Atmos. Chem. Phys., 21, 6605–6626, https://doi.org/10.5194/acp-21-6605-2021, https://doi.org/10.5194/acp-21-6605-2021, 2021
Short summary
Short summary
The Permian Basin (USA) is the world’s largest oil field. We use tower- and aircraft-based approaches to measure how methane emissions in the Permian Basin changed throughout 2020. In early 2020, 3.3 % of the region’s gas was emitted; then in spring 2020, the loss rate temporarily dropped to 1.9 % as oil price crashed. We find this short-term reduction to be a result of reduced well development, less gas flaring, and fewer abnormal events despite minimal reductions in oil and gas production.
Alkuin Maximilian Koenig, Olivier Magand, Paolo Laj, Marcos Andrade, Isabel Moreno, Fernando Velarde, Grover Salvatierra, René Gutierrez, Luis Blacutt, Diego Aliaga, Thomas Reichler, Karine Sellegri, Olivier Laurent, Michel Ramonet, and Aurélien Dommergue
Atmos. Chem. Phys., 21, 3447–3472, https://doi.org/10.5194/acp-21-3447-2021, https://doi.org/10.5194/acp-21-3447-2021, 2021
Short summary
Short summary
The environmental cycling of atmospheric mercury, a harmful global contaminant, is still not sufficiently constrained, partly due to missing data in remote regions. Here, we address this issue by presenting 20 months of atmospheric mercury measurements, sampled in the Bolivian Andes. We observe a significant seasonal pattern, whose key features we explore. Moreover, we deduce ratios to constrain South American biomass burning mercury emissions and the mercury uptake by the Amazon rainforest.
Yuming Jin, Ralph F. Keeling, Eric J. Morgan, Eric Ray, Nicholas C. Parazoo, and Britton B. Stephens
Atmos. Chem. Phys., 21, 217–238, https://doi.org/10.5194/acp-21-217-2021, https://doi.org/10.5194/acp-21-217-2021, 2021
Short summary
Short summary
We propose a new atmospheric coordinate (Mθe) based on equivalent potential temperature (θe) but with mass as the unit. This coordinate is useful in studying the spatial and temporal distribution of long-lived chemical tracers (CO2, CH4, O2 / N2, etc.) from sparse data, like airborne observation. Using this coordinate and sparse airborne observation (HIPPO and ATom), we resolve the Northern Hemisphere mass-weighted average CO2 seasonal cycle with high accuracy.
Hossein Maazallahi, Julianne M. Fernandez, Malika Menoud, Daniel Zavala-Araiza, Zachary D. Weller, Stefan Schwietzke, Joseph C. von Fischer, Hugo Denier van der Gon, and Thomas Röckmann
Atmos. Chem. Phys., 20, 14717–14740, https://doi.org/10.5194/acp-20-14717-2020, https://doi.org/10.5194/acp-20-14717-2020, 2020
Short summary
Short summary
Methane accounts for ∼ 25 % of current climate warming. The current lack of methane measurements is a barrier for tracking major sources, which are key for near-term climate mitigation. We use mobile measurements to identify and quantify methane emission sources in Utrecht (NL) and Hamburg (DE) with a focus on natural gas pipeline leaks. The measurements resulted in fixing the major leaks by the local utility, but coordinated efforts are needed at national levels for further emission reductions.
Cited articles
Barnes, E. A. and Fiore, A. M.: Surface ozone variability and the jet
position: Implications for projecting future air quality, Geophys. Res. Lett.,
40, 2839–2844, https://doi.org/10.1002/grl.50411, 2013.
Cooper, O. R., Schultz, M. G., Schroder, S., Chang, K. L., Gaudel, A.,
Benitez, G. C., Cuevas, E., Frohlich, M., Galbally, I. E., Molloy, S.,
Kubistin, D., Lu, X., McClure-Begley, A., Nedelec, P., O'Brien, J., Oltmans,
S. J., Petropavlovskikh, I., Ries, L., Senik, I., Sjoberg, K., Solberg, S.,
Spain, G. T., Spangl, W., Steinbacher, M., Tarasick, D., Thouret, V., and
Xu, X. B.: Multi-decadal surface ozone trends at globally distributed remote
locations, Elementa-Sci. Anthrop., 8, 23, https://doi.org/10.1525/Elementa.420, 2020.
Day, D. B., Xiang, J., and Mo, J.: Association of ozone exposure with
cardiorespiratory pathophysiologic mechanisms in healthy adults, Jama Intern. Med., 177, 1400–1400,
https://doi.org/10.1001/jamainternmed.2017.4605, 2017.
Doherty, R. M., Wild, O., Shindell, D. T., Zeng, G., MacKenzie, I. A.,
Collins, W. J., Fiore, A. M., Stevenson, D. S., Dentener, F. J., Schultz, M.
G., Hess, P., Derwent, R. G., and Keating, T. J.: Impacts of climate change
on surface ozone and intercontinental ozone pollution: A multi-model study,
J. Geophys. Res.-Atmos., 118, 3744–3763, https://doi.org/10.1002/jgrd.50266, 2013.
Eskridge, R. E., Ku, J. Y., Rao, S. T., Porter, P. S., and Zurbenko, I. G.:
Separating different scales of motion in time series of meteorological
variables, B. Am. Meteorol. Soc., 78, 1473–1483, https://doi.org/10.1175/1520-0477(1997)078<1473:Sdsomi>2.0.Co;2, 1997.
Fiore, A. M., Jacob, D. J., Mathur, R., and Martin, R. V.: Application of
empirical orthogonal functions to evaluate ozone simulations with regional
and global models, J. Geophys. Res.-Atmos., 108, 4431,
https://doi.org/10.1029/2002jd003151, 2003.
Gao, D., Xie, M., Chen, X., Wang, T. J., Liu, J., Xu, Q., Mu, X. Y., Chen, F., Li, S., Zhuang, B. L., Li, M. M., Zhao, M., and Ren, J. Y.: Systematic classification of circulation patterns and integrated analysis of their effects on different ozone pollution levels in the Yangtze River Delta Region, China, Atmos. Environ., 242, 117760, https://doi.org/10.1016/j.atmosenv.2020.117760, 2020.
Gao, W., Tie, X. X., Xu, J. M., Huang, R. J., Mao, X. Q., Zhou, G. Q., and
Chang, L. Y.: Long-term trend of O3 in a mega City (Shanghai), China:
Characteristics, causes, and interactions with precursors, Sci. Total
Environ., 603, 425–433, https://doi.org/10.1016/j.scitotenv.2017.06.099, 2017.
Han, H., Liu, J., Shu, L., Wang, T., and Yuan, H.: Local and synoptic meteorological influences on daily variability in summertime surface ozone in eastern China, Atmos. Chem. Phys., 20, 203–222, https://doi.org/10.5194/acp-20-203-2020, 2020.
Hegarty, J., Mao, H., and Talbot, R.: Synoptic controls on summertime
surface ozone in the northeastern United States, J. Geophys. Res.-Atmos., 112,
D14306, https://doi.org/10.1029/2006jd008170, 2007.
Hou, X. W., Zhu, B., Kumar, K. R., and Lu, W.: Inter-annual variability in
fine particulate matter pollution over China during 2013-2018: Role of
meteorology, Atmos. Environ., 214, 116842, https://doi.org/10.1016/j.atmosenv.2019.116842,
2019.
Jacob, D. J. and Winner, D. A.: Effect of climate change on air quality,
Atmos. Environ., 43, 51–63, https://doi.org/10.1016/j.atmosenv.2008.09.051, 2009.
Jerrett, M., Burnett, R. T., Pope, C. A., Ito, K., Thurston, G., Krewski,
D., Shi, Y. L., Calle, E., and Thun, M.: Long-Term Ozone Exposure and
Mortality., New Engl. J. Med., 360, 1085–1095, https://doi.org/10.1056/Nejmoa0803894, 2009.
Leibensperger, E. M., Mickley, L. J., and Jacob, D. J.: Sensitivity of US air quality to mid-latitude cyclone frequency and implications of 1980–2006 climate change, Atmos. Chem. Phys., 8, 7075–7086, https://doi.org/10.5194/acp-8-7075-2008, 2008.
Li, K., Jacob, D. J., Liao, H., Shen, L., Zhang, Q., and Bates, K. H.:
Anthropogenic drivers of 2013–2017 trends in summer surface ozone in China,
P. Natl. Acad. Sci. USA, 116, 422–427, 2019.
Liu, J., Wang, L., Li, M., Liao, Z., Sun, Y., Song, T., Gao, W., Wang, Y., Li, Y., Ji, D., Hu, B., Kerminen, V.-M., Wang, Y., and Kulmala, M.: Quantifying the impact of synoptic circulation patterns on ozone variability in northern China from April to October 2013–2017, Atmos. Chem. Phys., 19, 14477–14492, https://doi.org/10.5194/acp-19-14477-2019, 2019.
Lu, X., Hong, J. Y., Zhang, L., Cooper, O. R., Schultz, M. G., Xu, X. B.,
Wang, T., Gao, M., Zhao, Y. H., and Zhang, Y. H.: Severe Surface Ozone
Pollution in China: A Global Perspective, Environ. Sci. Tech. Lett., 5, 487–494,
https://doi.org/10.1021/acs.estlett.8b00366, 2018.
Lu, X., Zhang, L., Wang, X. L., Gao, M., Li, K., Zhang, Y. Z., Yue, X., and
Zhang, Y. H.: Rapid Increases in Warm-Season Surface Ozone and Resulting
Health Impact in China Since 2013, Environ. Sci. Tech. Lett., 7, 240–247,
https://doi.org/10.1021/acs.estlett.0c00171, 2020.
Milanchus, M. L., Rao, S. T., and Zurbenko, I. G.: Evaluating the
effectiveness of ozone management efforts in the presence of meteorological
variability, J. Air Waste Manage., 48, 201–215, https://doi.org/10.1080/10473289.1998.10463673, 1998.
Papanastasiou, D. K., Melas, D., Bartzanas, T., and Kittas, C.: Estimation
of Ozone Trend in Central Greece, Based on Meteorologically Adjusted Time
Series, Environ. Model. Assess., 17, 353–361, https://doi.org/10.1007/s10666-011-9299-6, 2012.
Philipp, A., Beck, C., Huth, R., and Jacobeit, J.: Development and
comparison of circulation type classifications using the COST 733 dataset
and software, Int. J. Climatol., 36, 2673–2691, https://doi.org/10.1002/joc.3920, 2016.
Pu, X., Wang, T. J., Huang, X., Melas, D., Zanis, P., Papanastasiou, D. K.,
and Poupkou, A.: Enhanced surface ozone during the heat wave of 2013 in
Yangtze River Delta region, China, Sci. Total Environ., 603, 807–816,
https://doi.org/10.1016/j.scitotenv.2017.03.056, 2017.
Rao, S. T. and Zurbenko, I. G.: Detecting And Tracking Changes In Ozone
Air-Quality, J. Air Waste Manage., 44, 1089–1092, https://doi.org/10.1080/10473289.1994.10467303, 1994.
Santurtun, A., Gonzalez-Hidalgo, J. C., Sanchez-Lorenzo, A., and
Zarrabeitia, M. T.: Surface ozone concentration trends and its relationship
with weather types in Spain (2001–2010), Atmos. Environ., 101, 10–22,
https://doi.org/10.1016/j.atmosenv.2014.11.005, 2015.
Shu, L., Xie, M., Wang, T., Gao, D., Chen, P., Han, Y., Li, S., Zhuang, B., and Li, M.: Integrated studies of a regional ozone pollution synthetically affected by subtropical high and typhoon system in the Yangtze River Delta region, China, Atmos. Chem. Phys., 16, 15801–15819, https://doi.org/10.5194/acp-16-15801-2016, 2016.
Shu, L., Xie, M., Gao, D., Wang, T., Fang, D., Liu, Q., Huang, A., and Peng, L.: Regional severe particle pollution and its association with synoptic weather patterns in the Yangtze River Delta region, China, Atmos. Chem. Phys., 17, 12871–12891, https://doi.org/10.5194/acp-17-12871-2017, 2017.
Shu, L., Wang, T., Han, H., Xie, M., Chen, P., Li, M., and Wu, H.: Summertime
ozone pollution in the Yangtze River Delta of eastern China during 2013–2017:
Synoptic impacts and source apportionment, Environ. Pollut., 257, 113631, https://doi.org/10.1016/j.envpol.2019.113631, 2020.
Wang, B. and Fan, Z.: Choice of south Asian summer monsoon indices, B. Am.
Meteorol. Soc., 80, 629–638, https://doi.org/10.1175/1520-0477(1999)080<0629:Cosasm>2.0.Co;2, 1999.
Wang, B., Wu, Z. W., Li, J. P., Liu, J., Chang, C. P., Ding, Y. H., and Wu,
G. X.: How to measure the strength of the East Asian summer monsoon, J.
Climate, 21, 4449–4463, https://doi.org/10.1175/2008JCLI2183.1, 2008.
Wang, T., Xue, L. K., Brimblecombe, P., Lam, Y. F., Li, L., and Zhang, L.:
Ozone pollution in China: A review of concentrations, meteorological
influences, chemical precursors, and effects, Sci. Total Environ., 575,
1582–1596, https://doi.org/10.1016/j.scitotenv.2016.10.081, 2017.
Wise, E. K. and Comrie, A. C.: Extending the Kolmogorov-Zurbenko filter:
Application to ozone, particulate matter, and meteorological trends, J. Air
Waste Manage., 55, 1208–1216, https://doi.org/10.1080/10473289.2005.10464718, 2005.
Xie, M., Zhu, K. G., Wang, T. J., Yang, H. M., Zhuang, B. L., Li, S., Li, M.
G., Zhu, X. S., and Ouyang, Y.: Application of photochemical indicators to
evaluate ozone nonlinear chemistry and pollution control countermeasure in
China, Atmos. Environ., 99, 466–473, https://doi.org/10.1016/j.atmosenv.2014.10.013, 2014.
Xie, M., Liao, J., Wang, T., Zhu, K., Zhuang, B., Han, Y., Li, M., and Li, S.: Modeling of the anthropogenic heat flux and its effect on regional meteorology and air quality over the Yangtze River Delta region, China, Atmos. Chem. Phys., 16, 6071–6089, https://doi.org/10.5194/acp-16-6071-2016, 2016a.
Xie, M., Zhu, K., Wang, T., Chen, P., Han, Y., Li, S., Zhuang, B., and Shu,
L.: Temporal characterization and regional contribution to O3 and NOx at an
urban and a suburban site in Nanjing, China, Sci. Total
Environ., 551–552, 533–545, https://doi.org/10.1016/j.scitotenv.2016.02.047, 2016b.
Xie, M., Shu, L., Wang, T.-j., Liu, Q., Gao, D., Li, S., Zhuang, B.-l., Han,
Y., Li, M.-M., and Chen, P.-l.: Natural emissions under future climate
condition and their effects on surface ozone in the Yangtze River Delta
region, China, Atmos. Environ., 150, 162–180,
https://doi.org/10.1016/j.atmosenv.2016.11.053, 2017.
Yang, L., Luo, H., Yuan, Z., Zheng, J., Huang, Z., Li, C., Lin, X., Louie, P. K. K., Chen, D., and Bian, Y.: Quantitative impacts of meteorology and precursor emission changes on the long-term trend of ambient ozone over the Pearl River Delta, China, and implications for ozone control strategy, Atmos. Chem. Phys., 19, 12901–12916, https://doi.org/10.5194/acp-19-12901-2019, 2019.
Yang, Y., Liao, H., and Li, J.: Impacts of the East Asian summer monsoon on interannual variations of summertime surface-layer ozone concentrations over China, Atmos. Chem. Phys., 14, 6867–6879, https://doi.org/10.5194/acp-14-6867-2014, 2014.
Yarnal, B.: Synoptic Climatology in Environmental Analysis A Primer, Journal
of Preventive Medicine Information, 347, 170–180, 1993.
Yin, Z., Cao, B., and Wang, H.: Dominant patterns of summer ozone pollution in eastern China and associated atmospheric circulations, Atmos. Chem. Phys., 19, 13933–13943, https://doi.org/10.5194/acp-19-13933-2019, 2019.
Yue, X., Unger, N., Harper, K., Xia, X., Liao, H., Zhu, T., Xiao, J., Feng, Z., and Li, J.: Ozone and haze pollution weakens net primary productivity in China, Atmos. Chem. Phys., 17, 6073–6089, https://doi.org/10.5194/acp-17-6073-2017, 2017.
Zhang, J., Gao, Y., Luo, K., Leung, L. R., Zhang, Y., Wang, K., and Fan, J.: Impacts of compound extreme weather events on ozone in the present and future, Atmos. Chem. Phys., 18, 9861–9877, https://doi.org/10.5194/acp-18-9861-2018, 2018.
Zhao, Z. J. and Wang, Y. X.: Influence of the West Pacific subtropical high
on surface ozone daily variability in summertime over eastern China, Atmos.
Environ., 170, 197–204, 2017.
Short summary
O3 has been increasing in recent years over the Yangtze River Delta region of China and is closely associated with dominant weather systems. Still, the study on the impact of changes in synoptic weather patterns (SWPs) on O3 variation is quite limited. This work aims to reveal the unique features of changes in each SWP under O3 variation and quantifies the effects of meteorological conditions on O3 variation. Our findings could be helpful in strategy planning for O3 pollution control.
O3 has been increasing in recent years over the Yangtze River Delta region of China and is...
Altmetrics
Final-revised paper
Preprint