Articles | Volume 21, issue 5
https://doi.org/10.5194/acp-21-4103-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-4103-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
18 Mar 2021
Research article |
| 18 Mar 2021
| 18 Mar 2021
Simulations of anthropogenic bromoform indicate high emissions at the coast of East Asia
Josefine Maas
GEOMAR Helmholtz Centre for Ocean Research Kiel, Kiel, Germany
now at: Helmholtz-Zentrum Geesthacht, Institute of Coastal Research, Geesthacht, Germany
Susann Tegtmeier
CORRESPONDING AUTHOR
GEOMAR Helmholtz Centre for Ocean Research Kiel, Kiel, Germany
Institute of Space and Atmospheric Studies, University of
Saskatchewan, Saskatoon, Canada
GEOMAR Helmholtz Centre for Ocean Research Kiel, Kiel, Germany
Institute of Space and Atmospheric Studies, University of
Saskatchewan, Saskatoon, Canada
Birgit Quack
GEOMAR Helmholtz Centre for Ocean Research Kiel, Kiel, Germany
Jonathan V. Durgadoo
GEOMAR Helmholtz Centre for Ocean Research Kiel, Kiel, Germany
Faculty of Mathematics and Natural Sciences, Kiel University, Kiel, Germany
Arne Biastoch
GEOMAR Helmholtz Centre for Ocean Research Kiel, Kiel, Germany
Faculty of Mathematics and Natural Sciences, Kiel University, Kiel, Germany
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Nigel A. D. Richards, Natalya A. Kramarova, Stacey M. Frith, Sean M. Davis, and Yue Jia
Atmos. Meas. Tech., 19, 529–547, https://doi.org/10.5194/amt-19-529-2026, https://doi.org/10.5194/amt-19-529-2026, 2026
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The Montreal Protocol has led to a slow recovery in the Earth's ozone layer. To detect such changes, and to monitor the health of the ozone layer, long term global observations are needed. The OMPS Limb Profiler (LP) series of satellite sensors are designed to meet this need. We validate the latest version OMPS LP ozone profiles against other satellite and ground based measurements. We find that OMPS LP ozone is consistent with other data sources and is suitable for use in ozone trend studies.
Yannick Wölker, Willi Rath, Matthias Renz, and Arne Biastoch
Ocean Sci., 21, 3541–3562, https://doi.org/10.5194/os-21-3541-2025, https://doi.org/10.5194/os-21-3541-2025, 2025
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The Atlantic Meridional Overturning Circulation (AMOC) is a large current system that helps regulating Earth's climate. Monitoring the AMOC relies on fixed instruments anchored to the seafloor. This study explores, in a high-resolution model, whether data from Argo floats, autonomous drifters collecting hydrographic profiles, can be used to monitor the AMOC cost-effectively with the help of Machine Learning. Results suggest that Argo floats can extend AMOC monitoring beyond current fixed arrays.
Kimberlee Dubé, Adam Bourassa, Susann Tegtmeier, Daniel Zawada, and Douglas Degenstein
EGUsphere, https://doi.org/10.5194/egusphere-2025-5470, https://doi.org/10.5194/egusphere-2025-5470, 2025
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The stratopause, the boundary between the stratosphere and the mesosphere, is projected to cool and drop in response to anthropogenic greenhouse gas emissions. We use observations from two satellite instruments to assess the annual and inter-annual variability and to quantify trends in the stratopause temperature and height. We find that the stratopause cooled by ~0.5–1 K per decade and that the tropical stratopause moved lower by 300–475 m per decade during 2005–2021.
Gokhan Danabasoglu, Frederic S. Castruccio, Burcu Boza, Alice M. Barthel, Arne Biastoch, Adam Blaker, Alexandra Bozec, Diego Bruciaferri, Frank O. Bryan, Eric P. Chassignet, Yao Fu, Ian Grooms, Catherine Guiavarc'h, Hakase Hayashida, Andrew McC. Hogg, Ryan M. Holmes, Doroteaciro Iovino, Andrew E. Kiss, M. Susan Lozier, Gustavo Marques, Alex Megann, Franziska U. Schwarzkopf, Dave Storkey, Luke van Roekel, Jon Wolfe, Xiaobiao Xu, and Rong Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2025-5406, https://doi.org/10.5194/egusphere-2025-5406, 2025
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A comparison of simulated and observed overturning transports across the Overturning in the Subpolar North Atlantic Program sections for the 2014–2022 period is presented. Eighteen ocean simulations participate in the study. The simulated transports are in general agreement with observations. Analyzing overturning circulations in both depth and density space together provides a more complete picture of the overturning properties. The study serves as a benchmark for evaluation of ocean models.
Tobias Schulzki, Franziska U. Schwarzkopf, and Arne Biastoch
Ocean Sci., 21, 2481–2504, https://doi.org/10.5194/os-21-2481-2025, https://doi.org/10.5194/os-21-2481-2025, 2025
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Exceptionally high ocean temperatures can cause long-lasting damage to marine ecosystems. Most existing knowledge about such temperature extremes is focused on near-surface waters, yet ecosystems also thrive at greater depths. In this study, we present a comprehensive analysis of temperature extremes across the entire Atlantic Ocean, from the surface to the seafloor. Our findings underscore the importance of the ocean circulation in driving extreme temperature events.
Mona Zolghadrshojaee, Susann Tegtmeier, Sean M. Davis, Robin Pilch Kedzierski, and Leopold Haimberger
Atmos. Chem. Phys., 25, 12213–12232, https://doi.org/10.5194/acp-25-12213-2025, https://doi.org/10.5194/acp-25-12213-2025, 2025
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The tropical tropopause layer (TTL) is a crucial region where the troposphere transitions into the stratosphere, influencing air mass transport. This study examines temperature trends in the TTL and lower stratosphere using data from weather balloons, satellites and reanalysis datasets. We found cooling trends in the TTL from 1980 to 2001, followed by warming from 2002 to 2023. These shifts are linked to changes in atmospheric circulation and impact water vapour transport into the stratosphere.
Meghan Brehon, Susann Tegtmeier, Adam Bourassa, Sean M. Davis, Udo Grabowski, Tobias Kerzenmacher, and Gabriele Stiller
EGUsphere, https://doi.org/10.5194/egusphere-2025-4457, https://doi.org/10.5194/egusphere-2025-4457, 2025
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We used satellite-based water vapour data to estimate vertical transport rates in the tropical stratosphere for 1995 to 2020. These estimates were compared with other upwelling datasets and used to analyze stratospheric variability. Our results find good agreement between the datasets and reveal that variability in upwelling is mainly driven by known climate patterns like the QBO and ENSO with a clear signal in the upwelling time series coinciding with the QBO disruptions of 2015/16 and 2019/20.
Shenglong Zhang, Jiao Chen, Jonathon S. Wright, Sean M. Davis, Jie Gao, Paul Konopka, Ninghui Li, Mengqian Lu, Susann Tegtmeier, Xiaolu Yan, Guang J. Zhang, and Nuanliang Zhu
Atmos. Chem. Phys., 25, 10109–10139, https://doi.org/10.5194/acp-25-10109-2025, https://doi.org/10.5194/acp-25-10109-2025, 2025
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Swirling above summer storms, the Asian monsoon anticyclone functions as both gateway and gatekeeper to moisture entering the stratosphere. Although well monitored from space since 2005, many details of the anticyclone and the air that flows through it remain mysterious. Reanalyses, which combine model output and observations, may help to address how and why but only if they reliably capture the what and where of water vapor variations. Current reanalyses are beginning to meet these criteria.
Miming Zhang, Haipeng Gao, Shanshan Wang, Yue Jia, Shibo Yan, Rong Tian, Jinpei Yan, and Yanfang Wu
EGUsphere, https://doi.org/10.5194/egusphere-2025-1622, https://doi.org/10.5194/egusphere-2025-1622, 2025
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Under cold and clean conditions in the free troposphere, oceanic dimethyl sulfide (DMS) can form new particles. Using data from the field observation and Lana climatology with the FLEXPART model, we evaluated DMS contribution from surface ocean to the free troposphere. We found that cyclone enhances the contribution of oceanic dimethyl sulfide to the free troposphere over the Southern Ocean, suggesting significant DMS-derived new particles likely occurred at high altitudes in the Southern Ocean.
Matthew Toohey, Yue Jia, Sujan Khanal, and Susann Tegtmeier
Atmos. Chem. Phys., 25, 3821–3839, https://doi.org/10.5194/acp-25-3821-2025, https://doi.org/10.5194/acp-25-3821-2025, 2025
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The climate impact of volcanic eruptions depends in part on how long aerosols spend in the stratosphere. We develop a conceptual model for stratospheric aerosol lifetime in terms of production and decay timescales, as well as a lag between injection and decay. We find residence time depends strongly on injection height in the lower stratosphere. We show that the lifetime of stratospheric aerosol from the 1991 Pinatubo eruption is around 22 months, significantly longer than is commonly reported.
Zirui Zhang, Kaiming Huang, Fan Yi, Wei Cheng, Fuchao Liu, Jian Zhang, and Yue Jia
Atmos. Chem. Phys., 25, 3347–3361, https://doi.org/10.5194/acp-25-3347-2025, https://doi.org/10.5194/acp-25-3347-2025, 2025
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The height of the convective boundary layer (CBLH) is related to our health due to its crucial role in pollutant dispersion. The variance of vertical velocity from millimeter wave cloud radar (MMCR) can accurately capture the diurnal evolution of the CBLH, due to a small blind range and less impact by the residual layer. The CBLH is affected by radiation, humidity, cloud, and precipitation; thus, the MMCR is suitable for monitoring the CBLH, owing to its observation capability in various weather conditions.
Léo C. Aroucha, Joke F. Lübbecke, Peter Brandt, Franziska U. Schwarzkopf, and Arne Biastoch
Ocean Sci., 21, 661–678, https://doi.org/10.5194/os-21-661-2025, https://doi.org/10.5194/os-21-661-2025, 2025
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The west African coastal region sustains highly productive fisheries and marine ecosystems influenced by sea surface temperature. We use oceanic models to show that the freshwater input from land to ocean strengthens a surface northward (southward) coastal current north (south) of the Congo River mouth, promoting a transfer of cooler (warmer) waters to north (south) of the Congo discharge location. We highlight the significant impact of river discharge on ocean temperatures and circulation.
Kimberlee Dubé, Susann Tegtmeier, Felix Ploeger, and Kaley A. Walker
Atmos. Chem. Phys., 25, 1433–1447, https://doi.org/10.5194/acp-25-1433-2025, https://doi.org/10.5194/acp-25-1433-2025, 2025
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The transport rate of air in the stratosphere has changed in response to human emissions of greenhouse gases and ozone-depleting substances. This transport rate can be approximated using measurements of long-lived trace gases. We use observations and model results to derive anomalies and trends in the mean rate of stratospheric air transport. We find that air in the Northern Hemisphere aged by up to 0.3 years per decade relative to air in the Southern Hemisphere over 2004–2017.
Hendrik Großelindemann, Frederic S. Castruccio, Gokhan Danabasoglu, and Arne Biastoch
Ocean Sci., 21, 93–112, https://doi.org/10.5194/os-21-93-2025, https://doi.org/10.5194/os-21-93-2025, 2025
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This study investigates the Agulhas Leakage and examines its role in the global ocean circulation. It utilises a high-resolution Earth system model and a preindustrial climate to look at the response of the Agulhas Leakage to the wind field and the Atlantic Meridional Overturning Circulation (AMOC) and its evolution under climate change. The Agulhas Leakage could influence the stability of the AMOC, whose possible collapse would impact the climate in the Northern Hemisphere.
Kimberlee Dubé, Susann Tegtmeier, Adam Bourassa, Daniel Zawada, Douglas Degenstein, William Randel, Sean Davis, Michael Schwartz, Nathaniel Livesey, and Anne Smith
Atmos. Chem. Phys., 24, 12925–12941, https://doi.org/10.5194/acp-24-12925-2024, https://doi.org/10.5194/acp-24-12925-2024, 2024
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Greenhouse gas emissions that warm the troposphere also result in stratospheric cooling. The cooling rate is difficult to quantify above 35 km due to a deficit of long-term observational data with high vertical resolution in this region. We use satellite observations from several instruments, including a new temperature product from OSIRIS, to show that the upper stratosphere, from 35–60 km, cooled by 0.5 to 1 K per decade over 2005–2021 and by 0.6 K per decade over 1979–2021.
Mona Zolghadrshojaee, Susann Tegtmeier, Sean M. Davis, and Robin Pilch Kedzierski
Atmos. Chem. Phys., 24, 7405–7419, https://doi.org/10.5194/acp-24-7405-2024, https://doi.org/10.5194/acp-24-7405-2024, 2024
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Satellite data challenge the idea of an overall cooling trend in the tropical tropopause layer. From 2002 to 2022, a warming trend was observed, diverging from earlier findings. Tropopause height changes indicate dynamic processes alongside radiative effects. Upper-tropospheric warming contrasts with lower-stratosphere temperatures. The study highlights the complex interplay of factors shaping temperature trends.
Dennis Booge, Jerry F. Tjiputra, Dirk J. L. Olivié, Birgit Quack, and Kirstin Krüger
Earth Syst. Dynam., 15, 801–816, https://doi.org/10.5194/esd-15-801-2024, https://doi.org/10.5194/esd-15-801-2024, 2024
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Oceanic bromoform, produced by algae, is an important precursor of atmospheric bromine, highlighting the importance of implementing these emissions in climate models. The simulated mean oceanic concentrations align well with observations, while the mean atmospheric values are lower than the observed ones. Modelled annual mean emissions mostly occur from the sea to the air and are driven by oceanic concentrations, sea surface temperature, and wind speed, which depend on season and location.
Bjorn Stevens, Stefan Adami, Tariq Ali, Hartwig Anzt, Zafer Aslan, Sabine Attinger, Jaana Bäck, Johanna Baehr, Peter Bauer, Natacha Bernier, Bob Bishop, Hendryk Bockelmann, Sandrine Bony, Guy Brasseur, David N. Bresch, Sean Breyer, Gilbert Brunet, Pier Luigi Buttigieg, Junji Cao, Christelle Castet, Yafang Cheng, Ayantika Dey Choudhury, Deborah Coen, Susanne Crewell, Atish Dabholkar, Qing Dai, Francisco Doblas-Reyes, Dale Durran, Ayoub El Gaidi, Charlie Ewen, Eleftheria Exarchou, Veronika Eyring, Florencia Falkinhoff, David Farrell, Piers M. Forster, Ariane Frassoni, Claudia Frauen, Oliver Fuhrer, Shahzad Gani, Edwin Gerber, Debra Goldfarb, Jens Grieger, Nicolas Gruber, Wilco Hazeleger, Rolf Herken, Chris Hewitt, Torsten Hoefler, Huang-Hsiung Hsu, Daniela Jacob, Alexandra Jahn, Christian Jakob, Thomas Jung, Christopher Kadow, In-Sik Kang, Sarah Kang, Karthik Kashinath, Katharina Kleinen-von Königslöw, Daniel Klocke, Uta Kloenne, Milan Klöwer, Chihiro Kodama, Stefan Kollet, Tobias Kölling, Jenni Kontkanen, Steve Kopp, Michal Koran, Markku Kulmala, Hanna Lappalainen, Fakhria Latifi, Bryan Lawrence, June Yi Lee, Quentin Lejeun, Christian Lessig, Chao Li, Thomas Lippert, Jürg Luterbacher, Pekka Manninen, Jochem Marotzke, Satoshi Matsouoka, Charlotte Merchant, Peter Messmer, Gero Michel, Kristel Michielsen, Tomoki Miyakawa, Jens Müller, Ramsha Munir, Sandeep Narayanasetti, Ousmane Ndiaye, Carlos Nobre, Achim Oberg, Riko Oki, Tuba Özkan-Haller, Tim Palmer, Stan Posey, Andreas Prein, Odessa Primus, Mike Pritchard, Julie Pullen, Dian Putrasahan, Johannes Quaas, Krishnan Raghavan, Venkatachalam Ramaswamy, Markus Rapp, Florian Rauser, Markus Reichstein, Aromar Revi, Sonakshi Saluja, Masaki Satoh, Vera Schemann, Sebastian Schemm, Christina Schnadt Poberaj, Thomas Schulthess, Cath Senior, Jagadish Shukla, Manmeet Singh, Julia Slingo, Adam Sobel, Silvina Solman, Jenna Spitzer, Philip Stier, Thomas Stocker, Sarah Strock, Hang Su, Petteri Taalas, John Taylor, Susann Tegtmeier, Georg Teutsch, Adrian Tompkins, Uwe Ulbrich, Pier-Luigi Vidale, Chien-Ming Wu, Hao Xu, Najibullah Zaki, Laure Zanna, Tianjun Zhou, and Florian Ziemen
Earth Syst. Sci. Data, 16, 2113–2122, https://doi.org/10.5194/essd-16-2113-2024, https://doi.org/10.5194/essd-16-2113-2024, 2024
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To manage Earth in the Anthropocene, new tools, new institutions, and new forms of international cooperation will be required. Earth Virtualization Engines is proposed as an international federation of centers of excellence to empower all people to respond to the immense and urgent challenges posed by climate change.
Daniel Zawada, Kimberlee Dubé, Taran Warnock, Adam Bourassa, Susann Tegtmeier, and Douglas Degenstein
Atmos. Meas. Tech., 17, 1995–2010, https://doi.org/10.5194/amt-17-1995-2024, https://doi.org/10.5194/amt-17-1995-2024, 2024
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There remain large uncertainties in long-term changes of stratospheric–atmospheric temperatures. We have produced a time series of more than 20 years of satellite-based temperature measurements from the OSIRIS instrument in the upper–middle stratosphere. The dataset is publicly available and intended to be used for a better understanding of changes in stratospheric temperatures.
Kristin Burmeister, Franziska U. Schwarzkopf, Willi Rath, Arne Biastoch, Peter Brandt, Joke F. Lübbecke, and Mark Inall
Ocean Sci., 20, 307–339, https://doi.org/10.5194/os-20-307-2024, https://doi.org/10.5194/os-20-307-2024, 2024
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We apply two different forcing products to a high-resolution ocean model to investigate their impact on the simulated upper-current field in the tropical Atlantic. Where possible, we compare the simulated results to long-term observations. We find large discrepancies between the two simulations regarding the wind and current fields. We propose that long-term observations, once they have reached a critical length, need to be used to test the quality of wind-driven simulations.
Kimberlee Dubé, Susann Tegtmeier, Adam Bourassa, Daniel Zawada, Douglas Degenstein, Patrick E. Sheese, Kaley A. Walker, and William Randel
Atmos. Chem. Phys., 23, 13283–13300, https://doi.org/10.5194/acp-23-13283-2023, https://doi.org/10.5194/acp-23-13283-2023, 2023
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This paper presents a technique for understanding the causes of long-term changes in stratospheric composition. By using N2O as a proxy for stratospheric circulation in the model used to calculated trends, it is possible to separate the effects of dynamics and chemistry on observed trace gas trends. We find that observed HCl increases are due to changes in the stratospheric circulation, as are O3 decreases above 30 hPa in the Northern Hemisphere.
Torge Martin and Arne Biastoch
Ocean Sci., 19, 141–167, https://doi.org/10.5194/os-19-141-2023, https://doi.org/10.5194/os-19-141-2023, 2023
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How is the ocean affected by continued Greenland Ice Sheet mass loss? We show in a systematic set of model experiments that atmospheric feedback needs to be accounted for as the large-scale ocean circulation is more than twice as sensitive to the meltwater otherwise. Coastal winds, boundary currents, and ocean eddies play a key role in redistributing the meltwater. Eddy paramterization helps the coarse simulation to perform better in the Labrador Sea but not in the North Atlantic Current region.
Alan D. Fox, Patricia Handmann, Christina Schmidt, Neil Fraser, Siren Rühs, Alejandra Sanchez-Franks, Torge Martin, Marilena Oltmanns, Clare Johnson, Willi Rath, N. Penny Holliday, Arne Biastoch, Stuart A. Cunningham, and Igor Yashayaev
Ocean Sci., 18, 1507–1533, https://doi.org/10.5194/os-18-1507-2022, https://doi.org/10.5194/os-18-1507-2022, 2022
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Observations of the eastern subpolar North Atlantic in the 2010s show exceptional freshening and cooling of the upper ocean, peaking in 2016 with the lowest salinities recorded for 120 years. Using results from a high-resolution ocean model, supported by observations, we propose that the leading cause is reduced surface cooling over the preceding decade in the Labrador Sea, leading to increased outflow of less dense water and so to freshening and cooling of the eastern subpolar North Atlantic.
Jörg Fröhle, Patricia V. K. Handmann, and Arne Biastoch
Ocean Sci., 18, 1431–1450, https://doi.org/10.5194/os-18-1431-2022, https://doi.org/10.5194/os-18-1431-2022, 2022
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Three deep-water masses pass the southern exit of the Labrador Sea. Usually they are defined by explicit density intervals linked to the formation region. We evaluate this relation in an ocean model by backtracking the paths the water follows for 40 years: 48 % densify without contact to the atmosphere, 24 % densify in contact with the atmosphere, and 19 % are from the Nordic Seas. All three contribute to a similar density range at 53° N with weak specific formation location characteristics.
Takaya Uchida, Julien Le Sommer, Charles Stern, Ryan P. Abernathey, Chris Holdgraf, Aurélie Albert, Laurent Brodeau, Eric P. Chassignet, Xiaobiao Xu, Jonathan Gula, Guillaume Roullet, Nikolay Koldunov, Sergey Danilov, Qiang Wang, Dimitris Menemenlis, Clément Bricaud, Brian K. Arbic, Jay F. Shriver, Fangli Qiao, Bin Xiao, Arne Biastoch, René Schubert, Baylor Fox-Kemper, William K. Dewar, and Alan Wallcraft
Geosci. Model Dev., 15, 5829–5856, https://doi.org/10.5194/gmd-15-5829-2022, https://doi.org/10.5194/gmd-15-5829-2022, 2022
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Ocean and climate scientists have used numerical simulations as a tool to examine the ocean and climate system since the 1970s. Since then, owing to the continuous increase in computational power and advances in numerical methods, we have been able to simulate increasing complex phenomena. However, the fidelity of the simulations in representing the phenomena remains a core issue in the ocean science community. Here we propose a cloud-based framework to inter-compare and assess such simulations.
Kristof Bognar, Susann Tegtmeier, Adam Bourassa, Chris Roth, Taran Warnock, Daniel Zawada, and Doug Degenstein
Atmos. Chem. Phys., 22, 9553–9569, https://doi.org/10.5194/acp-22-9553-2022, https://doi.org/10.5194/acp-22-9553-2022, 2022
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We quantify recent changes in stratospheric ozone (outside the polar regions) using a combination of three satellite datasets. We find that upper stratospheric ozone have increased significantly since 2000, although the recovery shows an unexpected pause in the Northern Hemisphere. Combined with the likely decrease in ozone in the lower stratosphere, this presents an interesting challenge for predicting the future of the ozone layer.
Jens Zinke, Takaaki K. Watanabe, Siren Rühs, Miriam Pfeiffer, Stefan Grab, Dieter Garbe-Schönberg, and Arne Biastoch
Clim. Past, 18, 1453–1474, https://doi.org/10.5194/cp-18-1453-2022, https://doi.org/10.5194/cp-18-1453-2022, 2022
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Salinity is an important and integrative measure of changes to the water cycle steered by changes to the balance between rainfall and evaporation and by vertical and horizontal movements of water parcels by ocean currents. However, salinity measurements in our oceans are extremely sparse. To fill this gap, we have developed a 334-year coral record of seawater oxygen isotopes that reflects salinity changes in the globally important Agulhas Current system and reveals its main oceanic drivers.
Yue Jia, Birgit Quack, Robert D. Kinley, Ignacio Pisso, and Susann Tegtmeier
Atmos. Chem. Phys., 22, 7631–7646, https://doi.org/10.5194/acp-22-7631-2022, https://doi.org/10.5194/acp-22-7631-2022, 2022
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In this study, we assessed the potential risks of bromoform released from Asparagopsis farming near Australia for the stratospheric ozone layer by analyzing different cultivation scenarios. We conclude that the intended operation of Asparagopsis seaweed cultivation farms with an annual yield to meet the needs of 50 % of feedlots and cattle in either open-ocean or terrestrial cultures in Australia will not impact the ozone layer under normal operating conditions.
Susann Tegtmeier, Christa Marandino, Yue Jia, Birgit Quack, and Anoop S. Mahajan
Atmos. Chem. Phys., 22, 6625–6676, https://doi.org/10.5194/acp-22-6625-2022, https://doi.org/10.5194/acp-22-6625-2022, 2022
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In the atmosphere over the Indian Ocean, intense anthropogenic pollution from Southeast Asia mixes with pristine oceanic air. During the winter monsoon, high pollution levels are regularly observed over the entire northern Indian Ocean, while during the summer monsoon, clean air dominates. Here, we review current progress in detecting and understanding atmospheric gas-phase composition over the Indian Ocean and its impacts on the upper atmosphere, oceanic biogeochemistry, and marine ecosystems.
Ioana Ivanciu, Katja Matthes, Arne Biastoch, Sebastian Wahl, and Jan Harlaß
Weather Clim. Dynam., 3, 139–171, https://doi.org/10.5194/wcd-3-139-2022, https://doi.org/10.5194/wcd-3-139-2022, 2022
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Greenhouse gas concentrations continue to increase, while the Antarctic ozone hole is expected to recover during the twenty-first century. We separate the effects of ozone recovery and of greenhouse gases on the Southern Hemisphere atmospheric and oceanic circulation, and we find that ozone recovery is generally reducing the impact of greenhouse gases, with the exception of certain regions of the stratosphere during spring, where the two effects reinforce each other.
Arne Biastoch, Franziska U. Schwarzkopf, Klaus Getzlaff, Siren Rühs, Torge Martin, Markus Scheinert, Tobias Schulzki, Patricia Handmann, Rebecca Hummels, and Claus W. Böning
Ocean Sci., 17, 1177–1211, https://doi.org/10.5194/os-17-1177-2021, https://doi.org/10.5194/os-17-1177-2021, 2021
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The Atlantic Meridional Overturning Circulation (AMOC) quantifies the impact of the ocean on climate and climate change. Here we show that a high-resolution ocean model is able to realistically simulate ocean currents. While the mean representation of the AMOC depends on choices made for the model and on the atmospheric forcing, the temporal variability is quite robust. Comparing the ocean model with ocean observations, we able to identify that the AMOC has declined over the past two decades.
Christina Schmidt, Franziska U. Schwarzkopf, Siren Rühs, and Arne Biastoch
Ocean Sci., 17, 1067–1080, https://doi.org/10.5194/os-17-1067-2021, https://doi.org/10.5194/os-17-1067-2021, 2021
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We estimate Agulhas leakage, water flowing from the Indian Ocean to the South Atlantic, in an ocean model with two different tools. The mean transport, variability and trend of Agulhas leakage is simulated comparably with both tools, emphasising the robustness of our method. If the experiments are designed differently, the mean transport of Agulhas leakage is altered, but not the trend. Agulhas leakage waters cool and become less salty south of Africa resulting in a density increase.
Michaela I. Hegglin, Susann Tegtmeier, John Anderson, Adam E. Bourassa, Samuel Brohede, Doug Degenstein, Lucien Froidevaux, Bernd Funke, John Gille, Yasuko Kasai, Erkki T. Kyrölä, Jerry Lumpe, Donal Murtagh, Jessica L. Neu, Kristell Pérot, Ellis E. Remsberg, Alexei Rozanov, Matthew Toohey, Joachim Urban, Thomas von Clarmann, Kaley A. Walker, Hsiang-Jui Wang, Carlo Arosio, Robert Damadeo, Ryan A. Fuller, Gretchen Lingenfelser, Christopher McLinden, Diane Pendlebury, Chris Roth, Niall J. Ryan, Christopher Sioris, Lesley Smith, and Katja Weigel
Earth Syst. Sci. Data, 13, 1855–1903, https://doi.org/10.5194/essd-13-1855-2021, https://doi.org/10.5194/essd-13-1855-2021, 2021
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An overview of the SPARC Data Initiative is presented, to date the most comprehensive assessment of stratospheric composition measurements spanning 1979–2018. Measurements of 26 chemical constituents obtained from an international suite of space-based limb sounders were compiled into vertically resolved, zonal monthly mean time series. The quality and consistency of these gridded datasets are then evaluated using a climatological validation approach and a range of diagnostics.
Ioana Ivanciu, Katja Matthes, Sebastian Wahl, Jan Harlaß, and Arne Biastoch
Atmos. Chem. Phys., 21, 5777–5806, https://doi.org/10.5194/acp-21-5777-2021, https://doi.org/10.5194/acp-21-5777-2021, 2021
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The Antarctic ozone hole has driven substantial dynamical changes in the Southern Hemisphere atmosphere over the past decades. This study separates the historical impacts of ozone depletion from those of rising levels of greenhouse gases and investigates how these impacts are captured in two types of climate models: one using interactive atmospheric chemistry and one prescribing the CMIP6 ozone field. The effects of ozone depletion are more pronounced in the model with interactive chemistry.
Josefine Herrford, Peter Brandt, Torsten Kanzow, Rebecca Hummels, Moacyr Araujo, and Jonathan V. Durgadoo
Ocean Sci., 17, 265–284, https://doi.org/10.5194/os-17-265-2021, https://doi.org/10.5194/os-17-265-2021, 2021
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The Atlantic Meridional Overturning Circulation (AMOC) is an important component of the climate system. Understanding its structure and variability is a key priority for many scientists. Here, we present the first estimate of AMOC variations for the tropical South Atlantic from the TRACOS array at 11° S. Over the observed period, the AMOC was dominated by seasonal variability. We investigate the respective mechanisms with an ocean model and find that different wind-forced waves play a big role.
Cited articles
Allonier, A.-S., Khalanski, M., Camel, V., and Bermond, A.: Characterization
of Chlorination By-products in Cooling Effluents of Coastal Nuclear Power
Stations, Mar. Pollut. Bull., 38, 1232–1241,
https://doi.org/10.1016/S0025-326X(99)00168-X, 1999.
Aschmann, J. and Sinnhuber, B.-M.: Contribution of very short-lived substances to stratospheric bromine loading: uncertainties and constraints, Atmos. Chem. Phys., 13, 1203–1219, https://doi.org/10.5194/acp-13-1203-2013, 2013.
Aschmann, J., Sinnhuber, B.-M., Atlas, E. L., and Schauffler, S. M.: Modeling the transport of very short-lived substances into the tropical upper troposphere and lower stratosphere, Atmos. Chem. Phys., 9, 9237–9247, https://doi.org/10.5194/acp-9-9237-2009, 2009.
Blanke, B., Arhan, M., Madec, G., and Roche, S.: Warm Water Paths in the
Equatorial Atlantic as Diagnosed with a General Circulation Model, J. Phys.
Oceanogr., 29, 2753–2768, https://doi.org/10.1175/1520-0485(1999)029<2753:WWPITE>2.0.CO;2, 1999.
Boudjellaba, D., Dron, J., Revenko, G., Démelas, C., and Boudenne, J.-L.:
Chlorination by-product concentration levels in seawater and fish of an
industrialised bay (Gulf of Fos, France) exposed to multiple chlorinated
effluents, Sci. Total Environ., 541, 391–399, https://doi.org/10.1016/j.scitotenv.2015.09.046, 2016.
Butler, J. H., King, D. B., Lobert, J. M., Montzka, S. A., Yvon-Lewis, S. A., Hall, B. D., Warwick, N. J., Mondeel, D. J., Aydin, M., and Elkins, J. W.: Oceanic distributions and emissions of short-lived halocarbons, Global
Biogeochem. Cy., 21, GB1023, https://doi.org/10.1029/2006GB002732, 2007.
Davis, C., Chmieliauskas, A., Dijkema, G., and Nikolic, I.: Enipedia, Energy and Industry group Faculty of Technology Policy and Managment, TU Delft, Delft, the Netherlands, available at: http://enipedia.tudelft.nl,Technical report (last access: 1 March 2021), 2012.
Davis, C. B.: Making sense of open data: from raw data to actionable insight, TU Delft, Delft, the Netherlands, https://doi.org/10.4233/uuid:88c3c6f9-d6a2-4a82-9353-884a3b77b6ed, 2012.
Dee, D. P., Uppala, S. M., Simmons, A. J., Berrisford, P., Poli, P.,
Kobayashi, S., Andrae, U., Balmaseda, M. A., Balsamo, G., Bauer, P.,
Bechtold, P., Beljaars, A. C. M., van de Berg, L., Bidlot, J., Bormann, N.,
Delsol, C., Dragani, R., Fuentes, M., Geer, A. J., Haimberger, L., Healy, S. B., Hersbach, H., Hólm, E. V., Isaksen, L., Kållberg, P.,
Köhler, M., Matricardi, M., McNally, A. P., Monge-Sanz, B. M.,
Morcrette, J.-J., Park, B.-K., Peubey, C., de Rosnay, P., Tavolato, C.,
Thépaut, J.-N., and Vitart, F.: The ERA-Interim reanalysis: configuration
and performance of the data assimilation system, Q. J. Roy. Meteorol. Soc., 137, 553–597, https://doi.org/10.1002/qj.828, 2011.
Dussin, R., Barnier, B., Brodeau, L., and Molines, J. M.: The Making Of the
DRAKKAR FORCING SET DFS5, DRAKKAR/MyOcean Rep. 01-04-16, 1–34, 2016.
Engel, A. and Rigby, M. (Lead Authors), Burkholder, J. B., Fernandez, R. P., Froidevaux, L., Hall, B. D., Hossaini, R., Saito, T., Vollmer, M. K., and Yao, B.: Update on Ozone-Depleting Substances (ODSs) and Other Gases of Interest to the Montreal Protocol, Chapter 1, in: Scientific Assessment of Ozone Depletion: 2018, Global Ozone Research and Monitoring Project – Report No. 58, World Meteorological Organization, Geneva, Switzerland, 2018.
Fiehn, A., Quack, B., Hepach, H., Fuhlbrügge, S., Tegtmeier, S., Toohey, M., Atlas, E., and Krüger, K.: Delivery of halogenated very short-lived substances from the west Indian Ocean to the stratosphere during the Asian summer monsoon, Atmos. Chem. Phys., 17, 6723–6741, https://doi.org/10.5194/acp-17-6723-2017, 2017.
Fiehn, A., Quack, B., Stemmler, I., Ziska, F., and Krüger, K.: Importance of seasonally resolved oceanic emissions for bromoform delivery from the tropical Indian Ocean and west Pacific to the stratosphere, Atmos. Chem. Phys., 18, 11973–11990, https://doi.org/10.5194/acp-18-11973-2018, 2018a.
Fiehn, A., Quack, B., Marandino, C. A., and Krüger, K.: Transport
Variability of Very Short Lived Substances From the West Indian Ocean to the
Stratosphere, J. Geophys. Res.-Atmos., 123, 5720–5738,
https://doi.org/10.1029/2017JD027563, 2018b.
Fogelqvist, E. and Krysell, M.: Naturally and anthropogenically produced
bromoform in the Kattegatt, a semi-enclosed oceanic basin, J. Atmos. Chem., 13, 315–324, https://doi.org/10.1007/BF00057749, 1991.
Forster, C., Stohl, A., and Seibert, P.: Parameterization of convective
transport in a Lagrangian particle dispersion model and its evaluation, J.
Appl. Meteorol. Clim., 46, 403–422, https://doi.org/10.1175/JAM2470.1, 2007.
Fuhlbrügge, S., Quack, B., Tegtmeier, S., Atlas, E., Hepach, H., Shi, Q., Raimund, S., and Krüger, K.: The contribution of oceanic halocarbons to marine and free tropospheric air over the tropical West Pacific, Atmos. Chem. Phys., 16, 7569–7585, https://doi.org/10.5194/acp-16-7569-2016, 2016.
He, Z., Yang, G.-P., Lu, X.-L., and Zhang, H.-H.: Distributions and
sea-to-air fluxes of chloroform, trichloroethylene, tetrachloroethylene,
chlorodibromomethane and bromoform in the Yellow Sea and the East China Sea
during spring, Environ. Pollut., 177, 28–37, https://doi.org/10.1016/j.envpol.2013.02.008, 2013a.
He, Z., Yang, G.-P., and Lu, X.-L.: Distributions and sea-to-air fluxes of
volatile halocarbons in the East China Sea in early winter, Chemosphere, 90, 747–757, https://doi.org/10.1016/j.chemosphere.2012.09.067, 2013b.
Helz, G. R., Sugam, R., and Sigleo, A. C.: Chemical modifications of
estuarine water by a power plant using continuous chlorination, Environ.
Sci. Technol., 18, 192–199, https://doi.org/10.1021/es00121a011, 1984.
Hossaini, R., Mantle, H., Chipperfield, M. P., Montzka, S. A., Hamer, P., Ziska, F., Quack, B., Krüger, K., Tegtmeier, S., Atlas, E., Sala, S., Engel, A., Bönisch, H., Keber, T., Oram, D., Mills, G., Ordóñez, C., Saiz-Lopez, A., Warwick, N., Liang, Q., Feng, W., Moore, F., Miller, B. R., Marécal, V., Richards, N. A. D., Dorf, M., and Pfeilsticker, K.: Evaluating global emission inventories of biogenic bromocarbons, Atmos. Chem. Phys., 13, 11819–11838, https://doi.org/10.5194/acp-13-11819-2013, 2013.
Hossaini, R., Chipperfield, M. P., Montzka, S. A., Rap, A., Dhomse, S., and
Feng, W.: Efficiency of short-lived halogens at influencing climate through
depletion of stratospheric ozone, Nat. Geosci., 8, 186–190,
https://doi.org/10.1038/ngeo2363, 2015.
Hossaini, R., Patra, P. K., Leeson, A. A., Krysztofiak, G., Abraham, N. L., Andrews, S. J., Archibald, A. T., Aschmann, J., Atlas, E. L., Belikov, D. A., Bönisch, H., Carpenter, L. J., Dhomse, S., Dorf, M., Engel, A., Feng, W., Fuhlbrügge, S., Griffiths, P. T., Harris, N. R. P., Hommel, R., Keber, T., Krüger, K., Lennartz, S. T., Maksyutov, S., Mantle, H., Mills, G. P., Miller, B., Montzka, S. A., Moore, F., Navarro, M. A., Oram, D. E., Pfeilsticker, K., Pyle, J. A., Quack, B., Robinson, A. D., Saikawa, E., Saiz-Lopez, A., Sala, S., Taguchi, S., Tegtmeier, S., Lidster, R. T., Wilson, C., and Ziska, F.: A multi-model intercomparison of halogenated very short-lived substances (TransCom-VSLS): linking oceanic emissions and tropospheric transport for a reconciled estimate of the stratospheric source gas injection of bromine, Atmos. Chem. Phys., 16, 9163–9187, https://doi.org/10.5194/acp-16-9163-2016, 2016.
IEA: Key world energy statistics 2005, Int. Energy Agency, Paris, 2005.
IEA: Key world energy statistics 2018, Int. Energy Agency, Paris, 2018.
Jenner, H. A., Taylor, C. J. L., van Donk, M., and Khalanski, M.:
Chlorination by-products in chlorinated cooling water of some European
coastal power stations, Mar. Environ. Res., 43, 279–293,
https://doi.org/10.1016/S0141-1136(96)00091-8, 1997.
Jia, Y., Tegtmeier, S., Atlas, E., and Quack, B.: How marine emissions of bromoform impact the remote atmosphere, Atmos. Chem. Phys., 19, 11089–11103, https://doi.org/10.5194/acp-19-11089-2019, 2019.
Joint Research Council: Integrated Pollution Prevention and Control (IPPC) Reference Document on the application of Best Available Techniques to Industrial Cooling Systems, December 2001, Eur. Comm. Sev., I–313, 2001.
Jones, E., Qadir, M., van Vliet, M. T. H., Smakhtin, V., and Kang, S.: The
state of desalination and brine production: A global outlook, Sci. Total
Environ., 657, 1343–1356, https://doi.org/10.1016/j.scitotenv.2018.12.076, 2019.
Khalanski, M. and Jenner, H. A.: Chlorination Chemistry and Ecotoxicology of
the Marine Cooling Water Systems, Chapt. 9, in: Operational and Environmental
Consequences of Large Industrial Cooling Water Systems, chap. 9, Springer, Boston, 183–226, 2012.
Liang, Q., Stolarski, R. S., Kawa, S. R., Nielsen, J. E., Douglass, A. R., Rodriguez, J. M., Blake, D. R., Atlas, E. L., and Ott, L. E.: Finding the missing stratospheric Bry: a global modeling study of CHBr3 and CH2Br2, Atmos. Chem. Phys., 10, 2269–2286, https://doi.org/10.5194/acp-10-2269-2010, 2010.
Liu, Z., Wang, X., Luo, Z., Huo, M., Wu, J., Huo, H., and Yang, W.: Removing
of Disinfection By-Product Precursors from Surface Water by Using Magnetic
Graphene Oxide, edited by: Mishra, Y. K., PLoS One, 10, e0143819,
https://doi.org/10.1371/journal.pone.0143819, 2015.
Maas, J., Tegtmeier, S., Quack, B., Biastoch, A., Durgadoo, J. V., Rühs, S., Gollasch, S., and David, M.: Simulating the spread of disinfection by-products and anthropogenic bromoform emissions from ballast water discharge in Southeast Asia, Ocean Sci., 15, 891–904, https://doi.org/10.5194/os-15-891-2019, 2019.
Madec, G. and the N. T.: NEMO ocean engine, Note du Pôle
modélisation l'Institut Pierre-Simon Laplace No. 27, l'Institut Pierre-Simon Laplace, France, 2008.
Marandino, C. A., Tegtmeier, S., Krüger, K., Zindler, C., Atlas, E. L., Moore, F., and Bange, H. W.: Dimethylsulphide (DMS) emissions from the western Pacific Ocean: a potential marine source for stratospheric sulphur?, Atmos. Chem. Phys., 13, 8427–8437, https://doi.org/10.5194/acp-13-8427-2013, 2013.
Moat, B. I., Josey, S. A., Sinha, B., Blaker, A. T., Smeed, D. A., McCarthy, G. D., Johns, W. E., Hirschi, J. J. M., Frajka-Williams, E., Rayner, D., Duchez, A., and Coward, A. C.: Major variations in subtropical North Atlantic heat transport at short (5 day) timescales and their causes, J. Geophys. Res.-Oceans, 121, 3237–3249, https://doi.org/10.1002/2016JC011660, 2016.
Mohd Nadzir, M. S., Phang, S. M., Abas, M. R., Abdul Rahman, N., Abu Samah, A., Sturges, W. T., Oram, D. E., Mills, G. P., Leedham, E. C., Pyle, J. A., Harris, N. R. P., Robinson, A. D., Ashfold, M. J., Mead, M. I., Latif, M. T., Khan, M. F., Amiruddin, A. M., Banan, N., and Hanafiah, M. M.: Bromocarbons in the tropical coastal and open ocean atmosphere during the 2009 Prime Expedition Scientific Cruise (PESC-09), Atmos. Chem. Phys., 14, 8137–8148, https://doi.org/10.5194/acp-14-8137-2014, 2014.
Montzka, S. A. and Reimann, S.: Ozone-Depleting Substances (ODSs) and
Related Chemicals, Chapt. 1, in: Sci. Assess. Ozone Deplet. 2010, 1–108,
2010.
Nightingale, D., Malin, G., Law, C. S., Watson, A. J., Liss, P. S.,
Liddicoat, M. I., Boutin, J., and Upstill-Goddard, R. C.: In situ evaluation
of air-sea gas exchange parameterizations using novel conservative and
volatile tracers, Global Biogeochem. Cy., 14, 373–387, 2000.
Ordóñez, C., Lamarque, J.-F., Tilmes, S., Kinnison, D. E., Atlas, E. L., Blake, D. R., Sousa Santos, G., Brasseur, G., and Saiz-Lopez, A.: Bromine and iodine chemistry in a global chemistry-climate model: description and evaluation of very short-lived oceanic sources, Atmos. Chem. Phys., 12, 1423–1447, https://doi.org/10.5194/acp-12-1423-2012, 2012.
Padhi, R. K., Subramanian, S., Mohanty, A. K., Bramha, S. N., Prasad, M. V. R. R., and Satpathy, K. K.: Trihalomethanes in the Cooling Discharge of a Power Plant on Chlorination of Intake Seawater, Environ. Eng. Res., 17, 57–62, https://doi.org/10.4491/eer.2012.17.S1.S57, 2012.
Pisso, I., Haynes, P. H., and Law, K. S.: Emission location dependent ozone depletion potentials for very short-lived halogenated species, Atmos. Chem. Phys., 10, 12025–12036, https://doi.org/10.5194/acp-10-12025-2010, 2010.
Quack, B. and Wallace, D. W. R.: Air-sea flux of bromoform: Controls, rates,
and implications, Global Biogeochem. Cy., 17, 1023,
https://doi.org/10.1029/2002GB001890, 2003.
Rajamohan, R., Vinnitha, E., Venugopalan, V. P., and Narasimhan, S. V:
Chlorination by-products and their discharge from the cooling water system
of a coastal electric plant, Curr. Sci. India, 93, 1608–1612, 2007.
Randel, W. J., Park, M., Emmons, L., Kinnison, D., Bernath, P., Walker, K. A., Boone, C., and Pumphrey, H.: Asian monsoon transport of pollution to the stratosphere, Science, 328, 611–613, https://doi.org/10.1126/science.1182274, 2010.
Saiz-Lopez, A. and von Glasow, R.: Reactive halogen chemistry in the
troposphere, Chem. Soc. Rev., 41, 6448, https://doi.org/10.1039/c2cs35208g, 2012.
Sherwen, T., Schmidt, J. A., Evans, M. J., Carpenter, L. J., Großmann, K., Eastham, S. D., Jacob, D. J., Dix, B., Koenig, T. K., Sinreich, R., Ortega, I., Volkamer, R., Saiz-Lopez, A., Prados-Roman, C., Mahajan, A. S., and Ordóñz, C.: Global impacts of tropospheric halogens (Cl, Br, I) on oxidants and composition in GEOS-Chem, Atmos. Chem. Phys., 16, 12239–12271, https://doi.org/10.5194/acp-16-12239-2016, 2016.
Stemmler, I., Hense, I., and Quack, B.: Marine sources of bromoform in the
global open ocean – global patterns and emissions, Biogeosciences, 12, 1967–1981, https://doi.org/10.5194/bg-12-1967-2015, 2015.
Stohl, A. and Thomson, D. J.: A density correction for Lagrangian particle
dispersion models, Bound.-Lay. Meteorol., 90, 155–167, https://doi.org/10.1023/A:1001741110696, 1999.
Stohl, A., Forster, C., Frank, A., Seibert, P., and Wotawa, G.: Technical note: The Lagrangian particle dispersion model FLEXPART version 6.2, Atmos. Chem. Phys., 5, 2461–2474, https://doi.org/10.5194/acp-5-2461-2005, 2005.
Tamelander, J., Riddering, L., Haag, F., and Matheickal, J.: Guidelines for development of a national ballast water management strategy, GEF-UNDP-IMO Glob. London, GloBallast No. 18, UK IUCN, Gland. Switz., 2010.
Taylor, C. J. L.: The effects of biological fouling control at coastal and
estuarine power stations, Mar. Pollut. Bull., 53, 30–48,
https://doi.org/10.1016/j.marpolbul.2006.01.004, 2006.
Tegtmeier, S., Ziska, F., Pisso, I., Quack, B., Velders, G. J. M., Yang, X.,
and Krüer, K.: Oceanic bromoform emissions weighted by their ozone depletion potential, Atmos. Chem. Phys., 15, 13647–13663,
https://doi.org/10.5194/acp-15-13647-2015, 2015.
Tegtmeier, S., Atlas, E., Quack, B., Ziska, F., and Krüger, K.: Variability and past long-term changes of brominated very short-lived substances at the tropical tropopause, Atmos. Chem. Phys., 20, 7103–7123, https://doi.org/10.5194/acp-20-7103-2020, 2020a.
Tegtmeier, S., Anstey, J., Davis, S., Dragani, R., Harada, Y., Ivanciu, I., Pilch Kedzierski, R., Krüger, K., Legras, B., Long, C., Wang, J. S., Wargan, K., and Wright, J. S.: Temperature and tropopause characteristics from reanalyses data in the tropical tropopause layer, Atmos. Chem. Phys., 20, 753–770, https://doi.org/10.5194/acp-20-753-2020, 2020b.
The DRAKKAR Group: Eddy permitting ocean circulation hindcasts of past
decades, CLIVAR Exch., 42, 8–10, 2007.
Wales, P. A., Salawitch, R. J., Nicely, J. M., Anderson, D. C., Canty, T. P., Baidar, S., Dix, B., Koenig, T. K., Volkamer, R., Chen, D., Huey, L. G., Tanner, D. J., Cuevas, C. A., Fernandez, R. P., Kinnison, D. E., Lamarque, J.-F., Saiz-Lopez, A., Atlas, E. L., Hall, S. R., Navarro, M. A., Pan, L. L., Schauffler, S. M., Stell, M., Tilmes, S., Ullmann, K., Weinheimer, A. J., Akiyoshi, H., Chipperfield, M. P., Deushi, M., Dhomse, S. S., Feng, W., Graf, P., Hossaini, R., Jöckel, P., Mancini, E., Michou, M., Morgenstern, O., Oman, L. D., Pitari, G., Plummer, D. A., Revell, L. E., Rozanov, E., Saint-Martin, D., Schofield, R., Stenke, A., Stone, K. A., Visioni, D., Yamashita, Y., and Zeng,G.: Stratospheric injection of brominated very short-lived substances: Aircraft observations in the Western Pacific and representation in global models, J. Geophys. Res.-Atmos., 123, 5690–5719, https://doi.org/10.1029/2017JD027978, 2018.
Waliser, D. E. and Gautier, C.: A satellite-derived climatology of the ITCZ, J. Climate, 6, 2162–2174, https://doi.org/10.1175/1520-0442(1993)006<2162:ASDCOT>2.0.CO;2, 1993.
Yang, B., Yang, G.-P., Lu, X.-L., Li, L., and He, Z.: Distributions and
sources of volatile chlorocarbons and bromocarbons in the Yellow Sea and
East China Sea, Mar. Pollut. Bull., 95, 491–502,
https://doi.org/10.1016/j.marpolbul.2015.03.009, 2015.
Yang, G.-P., Yang, B., Lu, X.-L., Ding, H.-B., and He, Z.: Spatio-temporal
variations of sea surface halocarbon concentrations and fluxes from southern
Yellow Sea, Biogeochemistry, 121, 369–388,
https://doi.org/10.1007/s10533-014-0007-x, 2014.
Yang, J. S.: Bromoform in the effluents of a nuclear power plant: A
potential tracer of coastal water masses, Hydrobiologia, 464, 99–105,
https://doi.org/10.1023/A:1013922731434, 2001.
Yokouchi, Y., Saito, T., Zeng, J., Mukai, H., and Montzka, S.: Seasonal
variation of bromocarbons at Hateruma Island, Japan: implications for global
sources, J. Atmos. Chem., 74, 171–185, https://doi.org/10.1007/s10874-016-9333-9, 2017.
Ziska, F., Quack, B., Abrahamsson, K., Archer, S. D., Atlas, E., Bell, T., Butler, J. H., Carpenter, L. J., Jones, C. E., Harris, N. R. P., Hepach, H., Heumann, K. G., Hughes, C., Kuss, J., Krüger, K., Liss, P., Moore, R. M., Orlikowska, A., Raimund, S., Reeves, C. E., Reifenhäuser, W., Robinson, A. D., Schall, C., Tanhua, T., Tegtmeier, S., Turner, S., Wang, L., Wallace, D., Williams, J., Yamamoto, H., Yvon-Lewis, S., and Yokouchi, Y.: Global sea-to-air flux climatology for bromoform, dibromomethane and methyl iodide, Atmos. Chem. Phys., 13, 8915–8934, https://doi.org/10.5194/acp-13-8915-2013, 2013.
Short summary
Cooling-water disinfection at coastal power plants is a known source of atmospheric bromoform. A large source of anthropogenic bromoform is the industrial regions in East Asia. In current bottom-up flux estimates, these anthropogenic emissions are missing, underestimating the global air–sea flux of bromoform. With transport simulations, we show that by including anthropogenic bromoform from cooling-water treatment, the bottom-up flux estimates significantly improve in East and Southeast Asia.
Cooling-water disinfection at coastal power plants is a known source of atmospheric bromoform. A...
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