Articles | Volume 21, issue 18
https://doi.org/10.5194/acp-21-14141-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-14141-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
24 Sep 2021
Research article |
| 24 Sep 2021
| 24 Sep 2021
Aerosol effects on electrification and lightning discharges in a multicell thunderstorm simulated by the WRF-ELEC model
Mengyu Sun
Key Laboratory of Middle Atmosphere and Global Environment
Observation, Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing, China
College of Earth and Planetary Sciences, University of the Chinese
Academy of Sciences, Beijing, China
Dongxia Liu
CORRESPONDING AUTHOR
Key Laboratory of Middle Atmosphere and Global Environment
Observation, Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing, China
Xiushu Qie
CORRESPONDING AUTHOR
Key Laboratory of Middle Atmosphere and Global Environment
Observation, Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing, China
College of Earth and Planetary Sciences, University of the Chinese
Academy of Sciences, Beijing, China
Edward R. Mansell
NOAA National Severe Storms Laboratory, Norman, Oklahoma, USA
Yoav Yair
School of Sustainability, Interdisciplinary Center (IDC) Herzliya,
Herzliya, Israel
Alexandre O. Fierro
NOAA National Severe Storms Laboratory, Norman, Oklahoma, USA
Cooperative Institute for Mesoscale Meteorological Studies,
University of Oklahoma, Norman, Oklahoma, USA
Department of Forecasting Models, Zentralanstalt für Meteorologie und Geodynamik (ZAMG), Vienna, Austria
Shanfeng Yuan
Key Laboratory of Middle Atmosphere and Global Environment
Observation, Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing, China
Zhixiong Chen
Key Laboratory of Middle Atmosphere and Global Environment
Observation, Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing, China
College of Earth and Planetary Sciences, University of the Chinese
Academy of Sciences, Beijing, China
Dongfang Wang
Key Laboratory of Middle Atmosphere and Global Environment
Observation, Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing, China
Related authors
No articles found.
Zhixiong Chen, Jane Liu, Xiushu Qie, Xugeng Cheng, Yukun Shen, Mengmiao Yang, Rubin Jiang, and Xiangke Liu
Atmos. Chem. Phys., 22, 8221–8240, https://doi.org/10.5194/acp-22-8221-2022, https://doi.org/10.5194/acp-22-8221-2022, 2022
Short summary
Short summary
A vigorous surface ozone surge event of stratospheric origin occurred in the North China Plain at night. Surface ozone concentrations were 40–50 ppbv higher than the corresponding monthly mean, whereas surface carbon monoxide concentrations declined abruptly, which confirmed the direct stratospheric intrusions to the surface. We further addressed the notion that a combined effect of the dying typhoon and mesoscale convective systems was responsible for this vigorous ozone surge.
Yoav Yair, Yifat Yair, Baruch Rubin, Ronit Confino-Cohen, Yosef Rosman, Eduardo Shachar, and Menachem Rottem
Nat. Hazards Earth Syst. Sci., 19, 2715–2725, https://doi.org/10.5194/nhess-19-2715-2019, https://doi.org/10.5194/nhess-19-2715-2019, 2019
Short summary
Short summary
During severe thunderstorms, cold outflows can eject pollen and dust particles from the surface, releasing allergens and causing
thunderstorm asthmaepidemics in sensitive populations. We report the first case in Israel that occurred on 25 October 2015. The emergency room presentation records from three hospitals in central Israel showed a clear increase in patients with respiratory complaints immediately after the passage of a massive super-cell thunderstorm in the area.
Bingkun Yu, Xianghui Xue, Chengling Kuo, Gaopeng Lu, Xiankang Dou, Qi Gao, Jianfei Wu, Mingjiao Jia, Chao Yu, and Xiushu Qie
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2018-1025, https://doi.org/10.5194/acp-2018-1025, 2018
Preprint withdrawn
Short summary
Short summary
This paper explores the relationship between the intensifications of atomic sodium layer and Es layer in the Mesosphere/Lower Thermosphere (MLT) region (the earth's upper atmosphere at altitudes between 90 and 130 km above ground). The multi-instrument experiment of sodium lidar observations, ionospheric observations and sodium chemical simulations advances our understanding of the dynamical and chemical coupling processes in the mesosphere and ionosphere above thunderstorms.
Y. Ben Ami, O. Altaratz, Y. Yair, and I. Koren
Nat. Hazards Earth Syst. Sci., 15, 2449–2459, https://doi.org/10.5194/nhess-15-2449-2015, https://doi.org/10.5194/nhess-15-2449-2015, 2015
Y. Yair, S. Shalev, Z. Erlich, A. Agrachov, E. Katz, H. Saaroni, C. Price, and B. Ziv
Nat. Hazards Earth Syst. Sci., 14, 165–173, https://doi.org/10.5194/nhess-14-165-2014, https://doi.org/10.5194/nhess-14-165-2014, 2014
M. Formenton, G. Panegrossi, D. Casella, S. Dietrich, A. Mugnai, P. Sanò, F. Di Paola, H.-D. Betz, C. Price, and Y. Yair
Nat. Hazards Earth Syst. Sci., 13, 1085–1104, https://doi.org/10.5194/nhess-13-1085-2013, https://doi.org/10.5194/nhess-13-1085-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Measurement report: Source attribution and estimation of black carbon levels in an urban hotspot of the central Po Valley – an integrated approach combining high-resolution dispersion modelling and micro-aethalometers
Microphysical modelling of aerosol scavenging by different types of clouds: description and validation of the approach
Insights into the sources of ultrafine particle numbers at six European urban sites obtained by investigating COVID-19 lockdowns
In-plume and out-of-plume analysis of aerosol–cloud interactions derived from the 2014–2015 Holuhraun volcanic eruption
Impacts of atmospheric circulation patterns and cloud inhibition on aerosol radiative effect and boundary layer structure during winter air pollution in Sichuan Basin, China
Investigating the sign of stratocumulus adjustments to aerosols in the ICON global storm-resolving model
A model study investigating the sensitivity of aerosol forcing to the volatilities of semi-volatile organic compounds
Decomposing the effective radiative forcing of anthropogenic aerosols based on CMIP6 Earth system models
Modeling impacts of dust mineralogy on fast climate response
Uncertainties in laboratory-measured shortwave refractive indices of mineral dust aerosols and derived optical properties: a theoretical assessment
Diagnosing uncertainties in global biomass burning emission inventories and their impact on modeled air pollutants
Role of atmospheric aerosols in severe winter fog over the Indo-Gangetic Plain of India: a case study
Long-term variability in black carbon emissions constrained by gap-filled absorption aerosol optical depth and associated premature mortality in China
Intercomparison of aerosol optical depths from four reanalyses and their multi-reanalysis consensus
Global aviation contrail climate effects from 2019 to 2021
Rapid iodine oxoacid nucleation enhanced by dimethylamine in broad marine regions
Simulations of the impact of cloud condensation nuclei and ice-nucleating particles perturbations on the microphysics and radar reflectivity factor of stratiform mixed-phase clouds
Aerosols in the central Arctic cryosphere: satellite and model integrated insights during Arctic spring and summer
Observationally constrained regional variations of shortwave absorption by iron oxides emphasize the cooling effect of dust
Droplet collection efficiencies inferred from satellite retrievals constrain effective radiative forcing of aerosol–cloud interactions
Predicting Hygroscopic Growth of Organosulfur Aerosol Particles Using COSMOtherm
Global aerosol-type classification using a new hybrid algorithm and Aerosol Robotic Network data
Simulated phase state and viscosity of secondary organic aerosols over China
Comparing the simulated influence of biomass burning plumes on low-level clouds over the southeastern Atlantic under varying smoke conditions
Improved simulations of biomass burning aerosol optical properties and lifetimes in the NASA GEOS Model during the ORACLES-I campaign
Retrieval of refractive index and water content for the coating materials of aged black carbon aerosol based on optical properties: a theoretical analysis
Revealing dominant patterns of aerosols regimes in the lower troposphere and their evolution from preindustrial times to the future in global climate model simulations
Synergistic effects of previous winter NAO and ENSO on the spring dust activities in North China
Sharp increase in Saharan dust intrusions over the western Euro-Mediterranean in February–March 2020–2022 and associated atmospheric circulation
Temporal and spatial variations in dust activity in Australia based on remote sensing and reanalysis datasets
Sensitivity of global direct aerosol shortwave radiative forcing to uncertainties in aerosol optical properties
Molecular-level study on the role of methanesulfonic acid in iodine oxoacid nucleation
Improving estimation of a record breaking East Asian dust storm emission with lagged aerosol Ångström Exponent observations
Regional to global distributions, trends, and drivers of biogenic volatile organic compound emission from 2001 to 2020
Impacts of ice-nucleating particles on cirrus clouds and radiation derived from global model simulations with MADE3 in EMAC
Seasonal characteristics of emission, distribution, and radiative effect of marine organic aerosols over the western Pacific Ocean: an investigation with a coupled regional climate aerosol model
Fire–precipitation interactions amplify the quasi-biennial variability in fires over southern Mexico and Central America
Improved estimates of smoke exposure during Australia fire seasons: importance of quantifying plume injection heights
New particle formation induced by anthropogenic–biogenic interactions on the southeastern Tibetan Plateau
Investigation of observed dust trends over the Middle East region in NASA Goddard Earth Observing System (GEOS) model simulations
Impact of Biomass Burning Aerosols (BBA) on the tropical African climate in an ocean-atmosphere-aerosols coupled climate model
A new process-based and scale-aware desert dust emission scheme for global climate models – Part II: Evaluation in the Community Earth System Model version 2 (CESM2)
How well do Earth system models reproduce the observed aerosol response to rapid emission reductions? A COVID-19 case study
Global modeling of aerosol nucleation with an explicit chemical mechanism for highly oxygenated organic molecules (HOMs)
Observationally constrained analysis of sulfur cycle in the marine atmosphere with NASA ATom measurements and AeroCom model simulations
Impact of acidity and surface-modulated acid dissociation on cloud response to organic aerosol
The contribution of residential wood combustion to the PM2.5 concentrations in the Helsinki metropolitan area
Analysis of atmospheric particle growth based on vapor concentrations measured at the high-altitude GAW station Chacaltaya in the Bolivian Andes
Expanding the simulation of East Asian super dust storms: physical transport mechanisms impacting the western Pacific
Aerosol composition, air quality, and boundary layer dynamics in the urban background of Stuttgart in winter
Giorgio Veratti, Alessandro Bigi, Michele Stortini, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 24, 10475–10512, https://doi.org/10.5194/acp-24-10475-2024, https://doi.org/10.5194/acp-24-10475-2024, 2024
Short summary
Short summary
In a study of two consecutive winter seasons, we used measurements and modelling tools to identify the levels and sources of black carbon pollution in a medium-sized urban area of the Po Valley, Italy. Our findings show that biomass burning and traffic-related emissions (especially from Euro 4 diesel cars) significantly contribute to BC concentrations. This research offers crucial insights for policymakers and urban planners aiming to improve air quality in cities.
Pascal Lemaitre, Arnaud Quérel, Alexis Dépée, Alice Guerra Devigne, Marie Monier, Thibault Hiron, Chloé Soto Minguez, Daniel Hardy, and Andrea Flossmann
Atmos. Chem. Phys., 24, 9713–9732, https://doi.org/10.5194/acp-24-9713-2024, https://doi.org/10.5194/acp-24-9713-2024, 2024
Short summary
Short summary
A new in-cloud scavenging scheme is proposed. It is based on a microphysical model of cloud formation and may be applied to long-distance atmospheric transport models (> 100 km) and climatic models. This model is applied to the two most extreme precipitating cloud types in terms of both relative humidity and vertical extension: cumulonimbus and stratus.
Alex Rowell, James Brean, David C. S. Beddows, Tuukka Petäjä, Máté Vörösmarty, Imre Salma, Jarkko V. Niemi, Hanna E. Manninen, Dominik van Pinxteren, Thomas Tuch, Kay Weinhold, Zongbo Shi, and Roy M. Harrison
Atmos. Chem. Phys., 24, 9515–9531, https://doi.org/10.5194/acp-24-9515-2024, https://doi.org/10.5194/acp-24-9515-2024, 2024
Short summary
Short summary
Different sources of airborne particles in the atmospheres of four European cities were distinguished by recognising their particle size distributions using a statistical procedure, positive matrix factorisation. The various sources responded differently to the changes in emissions associated with COVID-19 lockdowns, and the reasons are investigated. While traffic emissions generally decreased, particles formed from reactions of atmospheric gases decreased in some cities but increased in others.
Amy H. Peace, Ying Chen, George Jordan, Daniel G. Partridge, Florent Malavelle, Eliza Duncan, and Jim M. Haywood
Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
Short summary
Short summary
Natural aerosols from volcanic eruptions can help us understand how anthropogenic aerosols modify climate. We use observations and model simulations of the 2014–2015 Holuhraun eruption plume to examine aerosol–cloud interactions in September 2014. We find a shift to clouds with smaller, more numerous cloud droplets in the first 2 weeks of the eruption. In the third week, the background meteorology and previous conditions experienced by air masses modulate the aerosol perturbation to clouds.
Hua Lu, Min Xie, Bingliang Zhuang, Danyang Ma, Bojun Liu, Yangzhihao Zhan, Tijian Wang, Shu Li, Mengmeng Li, and Kuanguang Zhu
Atmos. Chem. Phys., 24, 8963–8982, https://doi.org/10.5194/acp-24-8963-2024, https://doi.org/10.5194/acp-24-8963-2024, 2024
Short summary
Short summary
To identify cloud, aerosol, and planetary boundary layer (PBL) interactions from an air quality perspective, we summarized two pollution patterns characterized by denser liquid cloud and by obvious cloud radiation interaction (CRI). Numerical simulation experiments showed CRI could cause a 50 % reduction in aerosol radiation interaction (ARI) under a low-trough system. The results emphasized the nonnegligible role of CRI and its inhibition of ARI under wet and cloudy pollution synoptic patterns.
Emilie Fons, Ann Kristin Naumann, David Neubauer, Theresa Lang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 8653–8675, https://doi.org/10.5194/acp-24-8653-2024, https://doi.org/10.5194/acp-24-8653-2024, 2024
Short summary
Short summary
Aerosols can modify the liquid water path (LWP) of stratocumulus and, thus, their radiative effect. We compare storm-resolving model and satellite data that disagree on the sign of LWP adjustments and diagnose this discrepancy with causal inference. We find that strong precipitation, the absence of wet scavenging, and cloud deepening under a weak inversion contribute to positive LWP adjustments to aerosols in the model, despite weak negative effects from cloud-top entrainment enhancement.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
Atmos. Chem. Phys., 24, 8489–8506, https://doi.org/10.5194/acp-24-8489-2024, https://doi.org/10.5194/acp-24-8489-2024, 2024
Short summary
Short summary
The study examines how the volatility of semi-volatile organic compounds affects secondary organic aerosol (SOA) formation and climate. Our simulations show that uncertainties in these volatilities influence aerosol mass and climate impacts. Accurate representation of these compounds in climate models is crucial for predicting global climate patterns.
Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, Chaincy Kuo, Sophie Szopa, Pierre Nabat, Dirk Olivié, Twan van Noije, Philippe Le Sager, David Neubauer, Naga Oshima, Jane Mulcahy, Larry W. Horowitz, and Prodromos Zanis
Atmos. Chem. Phys., 24, 7837–7872, https://doi.org/10.5194/acp-24-7837-2024, https://doi.org/10.5194/acp-24-7837-2024, 2024
Short summary
Short summary
Effective radiative forcing (ERF) is a metric for estimating how human activities and natural agents change the energy flow into and out of the Earth’s climate system. We investigate the anthropogenic aerosol ERF, and we estimate the contribution of individual processes to the total ERF using simulations from Earth system models within the Coupled Model Intercomparison Project Phase 6 (CMIP6). Our findings highlight that aerosol–cloud interactions drive ERF variability during the last 150 years.
Qianqian Song, Paul Ginoux, María Gonçalves Ageitos, Ron L. Miller, Vincenzo Obiso, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7421–7446, https://doi.org/10.5194/acp-24-7421-2024, https://doi.org/10.5194/acp-24-7421-2024, 2024
Short summary
Short summary
We implement and simulate the distribution of eight dust minerals in the GFDL AM4.0 model. We found that resolving the eight minerals reduces dust absorption compared to the homogeneous dust used in the standard GFDL AM4.0 model that assumes a globally uniform hematite content of 2.7 % by volume. Resolving dust mineralogy results in significant impacts on radiation, land surface temperature, surface winds, and precipitation over North Africa in summer.
Senyi Kong, Zheng Wang, and Lei Bi
Atmos. Chem. Phys., 24, 6911–6935, https://doi.org/10.5194/acp-24-6911-2024, https://doi.org/10.5194/acp-24-6911-2024, 2024
Short summary
Short summary
The retrieval of refractive indices of dust aerosols from laboratory optical measurements is commonly done assuming spherical particles. This paper aims to investigate the uncertainties in the shortwave refractive indices and corresponding optical properties by considering non-spherical and inhomogeneous models for dust samples. The study emphasizes the significance of using non-spherical models for simulating dust aerosols.
Wenxuan Hua, Sijia Lou, Xin Huang, Lian Xue, Ke Ding, Zilin Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 6787–6807, https://doi.org/10.5194/acp-24-6787-2024, https://doi.org/10.5194/acp-24-6787-2024, 2024
Short summary
Short summary
In this study, we diagnose uncertainties in carbon monoxide and organic carbon emissions from four inventories for seven major wildfire-prone regions. Uncertainties in vegetation classification methods, fire detection products, and cloud obscuration effects lead to bias in these biomass burning (BB) emission inventories. By comparing simulations with measurements, we provide certain inventory recommendations. Our study has implications for reducing uncertainties in emissions in further studies.
Chandrakala Bharali, Mary Barth, Rajesh Kumar, Sachin D. Ghude, Vinayak Sinha, and Baerbel Sinha
Atmos. Chem. Phys., 24, 6635–6662, https://doi.org/10.5194/acp-24-6635-2024, https://doi.org/10.5194/acp-24-6635-2024, 2024
Short summary
Short summary
This study examines the role of atmospheric aerosols in winter fog over the Indo-Gangetic Plains of India using WRF-Chem. The increase in RH with aerosol–radiation feedback (ARF) is found to be important for fog formation as it promotes the growth of aerosols in the polluted environment. Aqueous-phase chemistry in the fog increases PM2.5 concentration, further affecting ARF. ARF and aqueous-phase chemistry affect the fog intensity and the timing of fog formation by ~1–2 h.
Wenxin Zhao, Yu Zhao, Yu Zheng, Dong Chen, Jinyuan Xin, Kaitao Li, Huizheng Che, Zhengqiang Li, Mingrui Ma, and Yun Hang
Atmos. Chem. Phys., 24, 6593–6612, https://doi.org/10.5194/acp-24-6593-2024, https://doi.org/10.5194/acp-24-6593-2024, 2024
Short summary
Short summary
We evaluate the long-term (2000–2020) variabilities of aerosol absorption optical depth, black carbon emissions, and associated health risks in China with an integrated framework that combines multiple observations and modeling techniques. We demonstrate the remarkable emission abatement resulting from the implementation of national pollution controls and show how human activities affected the emissions with a spatiotemporal heterogeneity, thus supporting differentiated policy-making by region.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
Short summary
Short summary
The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc E. J. Stettler
Atmos. Chem. Phys., 24, 6071–6093, https://doi.org/10.5194/acp-24-6071-2024, https://doi.org/10.5194/acp-24-6071-2024, 2024
Short summary
Short summary
The radiative forcing (RF) due to aviation contrails is comparable to that caused by CO2. We estimate that global contrail net RF in 2019 was 62.1 mW m−2. This is ~1/2 the previous best estimate for 2018. Contrail RF varies regionally due to differences in conditions required for persistent contrails. COVID-19 reduced contrail RF by 54% in 2020 relative to 2019. Globally, 2 % of all flights account for 80 % of the annual contrail energy forcing, suggesting a opportunity to mitigate contrail RF.
Haotian Zu, Biwu Chu, Yiqun Lu, Ling Liu, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 5823–5835, https://doi.org/10.5194/acp-24-5823-2024, https://doi.org/10.5194/acp-24-5823-2024, 2024
Short summary
Short summary
The nucleation of iodic acid (HIO3) and iodous acid (HIO2) was proven to be critical in marine areas. However, HIO3–HIO2 nucleation cannot effectively derive the rapid nucleation in some polluted coasts. We find a significant enhancement of dimethylamine (DMA) on the HIO3–HIO2 nucleation in marine and polar regions with abundant DMA sources, which may establish reasonable connections between the HIO3–HIO2 nucleation and the rapid formation of new particles in polluted marine and polar regions.
Junghwa Lee, Patric Seifert, Tempei Hashino, Maximilian Maahn, Fabian Senf, and Oswald Knoth
Atmos. Chem. Phys., 24, 5737–5756, https://doi.org/10.5194/acp-24-5737-2024, https://doi.org/10.5194/acp-24-5737-2024, 2024
Short summary
Short summary
Spectral bin model simulations of an idealized supercooled stratiform cloud were performed with the AMPS model for variable CCN and INP concentrations. We performed radar forward simulations with PAMTRA to transfer the simulations into radar observational space. The derived radar reflectivity factors were compared to observational studies of stratiform mixed-phase clouds. These studies report a similar response of the radar reflectivity factor to aerosol perturbations as we found in our study.
Basudev Swain, Marco Vountas, Aishwarya Singh, Nidhi L. Anchan, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Sachin S. Gunthe, Hartmut Bösch, and John P. Burrows
Atmos. Chem. Phys., 24, 5671–5693, https://doi.org/10.5194/acp-24-5671-2024, https://doi.org/10.5194/acp-24-5671-2024, 2024
Short summary
Short summary
Arctic amplification (AA) accelerates the warming of the central Arctic cryosphere and affects aerosol dynamics. Limited observations hinder a comprehensive analysis. This study uses AEROSNOW aerosol optical density (AOD) data and GEOS-Chem simulations to assess AOD variability. Discrepancies highlight the need for improved observational integration into models to refine our understanding of aerosol effects on cloud microphysics, ice nucleation, and radiative forcing under evolving AA.
Vincenzo Obiso, María Gonçalves Ageitos, Carlos Pérez García-Pando, Jan P. Perlwitz, Gregory L. Schuster, Susanne E. Bauer, Claudia Di Biagio, Paola Formenti, Kostas Tsigaridis, and Ron L. Miller
Atmos. Chem. Phys., 24, 5337–5367, https://doi.org/10.5194/acp-24-5337-2024, https://doi.org/10.5194/acp-24-5337-2024, 2024
Short summary
Short summary
We calculate the dust direct radiative effect (DRE) in an Earth system model accounting for regionally varying soil mineralogy through a new observationally constrained method. Linking dust absorption at solar wavelengths to the varying amount of specific minerals (i.e., iron oxides) improves the modeled range of dust single scattering albedo compared to observations and increases the global cooling by dust. Our results may contribute to improved estimates of the dust DRE and its climate impact.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
Atmos. Chem. Phys., 24, 5287–5302, https://doi.org/10.5194/acp-24-5287-2024, https://doi.org/10.5194/acp-24-5287-2024, 2024
Short summary
Short summary
Single-layer warm liquid clouds cover nearly one-third of the Earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth system model estimates of the radiative forcing from the interactions of aerosols with clouds due to warm rain processes.
Zijun Li, Angela Buchholz, and Noora Hyttinen
EGUsphere, https://doi.org/10.5194/egusphere-2024-1182, https://doi.org/10.5194/egusphere-2024-1182, 2024
Short summary
Short summary
Evaluating organosulfur (OS) hygroscopicity is important for assessing the aerosol-cloud climate interactions in the post-fossil fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here, a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with AS. A good agreement was observed between their model-estimated and experimental HGFs.
Xiaoli Wei, Qian Cui, Leiming Ma, Feng Zhang, Wenwen Li, and Peng Liu
Atmos. Chem. Phys., 24, 5025–5045, https://doi.org/10.5194/acp-24-5025-2024, https://doi.org/10.5194/acp-24-5025-2024, 2024
Short summary
Short summary
A new aerosol-type classification algorithm has been proposed. It includes an optical database built by Mie scattering and a complex refractive index working as a baseline to identify different aerosol types. The new algorithm shows high accuracy and efficiency. Hence, a global map of aerosol types was generated to characterize aerosol types across the five continents. It will help improve the accuracy of aerosol inversion and determine the sources of aerosol pollution.
Zhiqiang Zhang, Ying Li, Haiyan Ran, Junling An, Yu Qu, Wei Zhou, Weiqi Xu, Weiwei Hu, Hongbin Xie, Zifa Wang, Yele Sun, and Manabu Shiraiwa
Atmos. Chem. Phys., 24, 4809–4826, https://doi.org/10.5194/acp-24-4809-2024, https://doi.org/10.5194/acp-24-4809-2024, 2024
Short summary
Short summary
Secondary organic aerosols (SOAs) can exist in liquid, semi-solid, or amorphous solid states, which are rarely accounted for in current chemical transport models. We predict the phase state of SOA particles over China and find that in northwestern China SOA particles are mostly highly viscous or glassy solid. Our results indicate that the particle phase state should be considered in SOA formation in chemical transport models for more accurate prediction of SOA mass concentrations.
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
Atmos. Chem. Phys., 24, 4591–4610, https://doi.org/10.5194/acp-24-4591-2024, https://doi.org/10.5194/acp-24-4591-2024, 2024
Short summary
Short summary
We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass burning plumes.
Sampa Das, Peter R. Colarco, Huisheng Bian, and Santiago Gassó
Atmos. Chem. Phys., 24, 4421–4449, https://doi.org/10.5194/acp-24-4421-2024, https://doi.org/10.5194/acp-24-4421-2024, 2024
Short summary
Short summary
The smoke aerosols emitted from vegetation burning can alter the regional energy budget via multiple pathways. We utilized detailed observations from the NASA ORACLES airborne campaign based in Namibia during September 2016 to improve the representation of smoke aerosol properties and lifetimes in our GEOS Earth system model. The improved model simulations are for the first time able to capture the observed changes in the smoke absorption during long-range plume transport.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
EGUsphere, https://doi.org/10.5194/egusphere-2024-1000, https://doi.org/10.5194/egusphere-2024-1000, 2024
Short summary
Short summary
The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties, and this method is verified from theoretical inspect. This method performs well for thickly coated BC at high RHs.
Jingmin Li, Mattia Righi, Johannes Hendricks, Christof G. Beer, Ulrike Burkhardt, and Anja Schmidt
EGUsphere, https://doi.org/10.5194/egusphere-2024-1024, https://doi.org/10.5194/egusphere-2024-1024, 2024
Short summary
Short summary
Aiming to understand underlying patterns and trends in aerosols, we characterize the spatial patterns and long-term evolution of lower tropospheric aerosols by clustering multiple aerosol properties from preindustrial times to the year 2050 under three SSP scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Falei Xu, Shuang Wang, Yan Li, and Juan Feng
EGUsphere, https://doi.org/10.5194/egusphere-2024-955, https://doi.org/10.5194/egusphere-2024-955, 2024
Short summary
Short summary
This study examines how the North Atlantic Oscillation (NAO) and El Niño-Southern Oscillation (ENSO) in the previous winter affect spring dust activities in North China. The results show that NAO and ENSO, particularly in their negative phases, greatly influence dust activities. When both NAO and ENSO are negative, their combined effect on dust activities is even greater. This research underscores the importance of these climate patterns in predicting spring dust activities in North China.
Emilio Cuevas-Agulló, David Barriopedro, Rosa Delia García, Silvia Alonso-Pérez, Juan Jesús González-Alemán, Ernest Werner, David Suárez, Juan José Bustos, Gerardo García-Castrillo, Omaira García, África Barreto, and Sara Basart
Atmos. Chem. Phys., 24, 4083–4104, https://doi.org/10.5194/acp-24-4083-2024, https://doi.org/10.5194/acp-24-4083-2024, 2024
Short summary
Short summary
During February–March (FM) 2020–2022, unusually intense dust storms from northern Africa hit the western Euro-Mediterranean (WEM). Using dust products from satellites and atmospheric reanalysis for 2003–2022, results show that cut-off lows and European blocking are key drivers of FM dust intrusions over the WEM. A higher frequency of cut-off lows associated with subtropical ridges is observed in the late 2020–2022 period.
Yahui Che, Bofu Yu, and Katherine Bracco
Atmos. Chem. Phys., 24, 4105–4128, https://doi.org/10.5194/acp-24-4105-2024, https://doi.org/10.5194/acp-24-4105-2024, 2024
Short summary
Short summary
Dust events occur more frequently during the Austral spring and summer in dust regions, including central Australia, the southwest of Western Australia, and the northern and southern regions of eastern Australia using remote sensing and reanalysis datasets. High-concentration dust is distributed around central Australia and in the downwind northern and southern Australia. Typically, around 50 % of the dust lifted settles on Australian land, with the remaining half being deposited in the ocean.
Jonathan Elsey, Nicolas Bellouin, and Claire Ryder
Atmos. Chem. Phys., 24, 4065–4081, https://doi.org/10.5194/acp-24-4065-2024, https://doi.org/10.5194/acp-24-4065-2024, 2024
Short summary
Short summary
Aerosols influence the Earth's energy balance. The uncertainty in this radiative forcing is large depending partly on uncertainty in measurements of aerosol optical properties. We have developed a freely available new framework of millions of radiative transfer simulations spanning aerosol uncertainty and assess the impact on radiative forcing uncertainty. We find that reducing these uncertainties would reduce radiative forcing uncertainty, but non-aerosol uncertainties must also be considered.
Jing Li, Nan Wu, Biwu Chu, An Ning, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 3989–4000, https://doi.org/10.5194/acp-24-3989-2024, https://doi.org/10.5194/acp-24-3989-2024, 2024
Short summary
Short summary
Iodic acid (HIO3) nucleates with iodous acid (HIO2) efficiently in marine areas; however, whether methanesulfonic acid (MSA) can synergistically participate in the HIO3–HIO2-based nucleation is unclear. We provide molecular-level evidence that MSA can efficiently promote the formation of HIO3–HIO2-based clusters using a theoretical approach. The proposed MSA-enhanced iodine nucleation mechanism may help us to deeply understand marine new particle formation events with bursts of iodine particles.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
EGUsphere, https://doi.org/10.5194/egusphere-2024-840, https://doi.org/10.5194/egusphere-2024-840, 2024
Short summary
Short summary
In March 2021, East Asia experienced an outbreak of severe dust storms after an absence of one and a half decades. Here, we innovative used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize the dust emission and reproduce the dust storm. This work is valuable for the quantification of health damage, aviation risks, and profound impacts on the Earth system, but also to reveal the climatic driving force and the process of desertification.
Hao Wang, Xiaohong Liu, Chenglai Wu, and Guangxing Lin
Atmos. Chem. Phys., 24, 3309–3328, https://doi.org/10.5194/acp-24-3309-2024, https://doi.org/10.5194/acp-24-3309-2024, 2024
Short summary
Short summary
We quantified different global- and regional-scale drivers of biogenic volatile organic compound (BVOC) emission trends over the past 20 years. The results show that global greening trends significantly boost BVOC emissions and deforestation reduces BVOC emissions in South America and Southeast Asia. Elevated temperature in Europe and increased soil moisture in East and South Asia enhance BVOC emissions. The results deepen our understanding of long-term BVOC emission trends in hotspots.
Christof G. Beer, Johannes Hendricks, and Mattia Righi
Atmos. Chem. Phys., 24, 3217–3240, https://doi.org/10.5194/acp-24-3217-2024, https://doi.org/10.5194/acp-24-3217-2024, 2024
Short summary
Short summary
Ice-nucleating particles (INPs) have important influences on cirrus clouds and the climate system; however, the understanding of their global impacts is still uncertain. We perform numerical simulations with a global aerosol–climate model to analyse INP-induced cirrus changes and the resulting climate impacts. We evaluate various sources of uncertainties, e.g. the ice-nucleating ability of INPs and the role of model dynamics, and provide a new estimate for the global INP–cirrus effect.
Jiawei Li, Zhiwei Han, Pingqing Fu, Xiaohong Yao, and Mingjie Liang
Atmos. Chem. Phys., 24, 3129–3161, https://doi.org/10.5194/acp-24-3129-2024, https://doi.org/10.5194/acp-24-3129-2024, 2024
Short summary
Short summary
Organic aerosols of marine origin are important for aerosol climatic effects but are poorly understood. For the first time, an online coupled regional chemistry–climate model is applied to explore the characteristics of emission, distribution, and direct and indirect radiative effects of marine organic aerosols over the western Pacific, which reveals an important role of marine organic aerosols in perturbing cloud and radiation and promotes understanding of global aerosol climatic impact.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
Short summary
Short summary
Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Xu Feng, Loretta J. Mickley, Michelle L. Bell, Tianjia Liu, Jenny A. Fisher, and Maria Val Martin
Atmos. Chem. Phys., 24, 2985–3007, https://doi.org/10.5194/acp-24-2985-2024, https://doi.org/10.5194/acp-24-2985-2024, 2024
Short summary
Short summary
During severe wildfire seasons, smoke can have a significant impact on air quality in Australia. Our study demonstrates that characterization of the smoke plume injection fractions greatly affects estimates of surface smoke PM2.5. Using the plume behavior predicted by the machine learning method leads to the best model agreement with observed surface PM2.5 in key cities across Australia, with smoke PM2.5 accounting for 5 %–52 % of total PM2.5 on average during fire seasons from 2009 to 2020.
Shiyi Lai, Ximeng Qi, Xin Huang, Sijia Lou, Xuguang Chi, Liangduo Chen, Chong Liu, Yuliang Liu, Chao Yan, Mengmeng Li, Tengyu Liu, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 24, 2535–2553, https://doi.org/10.5194/acp-24-2535-2024, https://doi.org/10.5194/acp-24-2535-2024, 2024
Short summary
Short summary
By combining in situ measurements and chemical transport modeling, this study investigates new particle formation (NPF) on the southeastern Tibetan Plateau. We found that the NPF was driven by the presence of biogenic gases and the transport of anthropogenic precursors. The NPF was vertically heterogeneous and shaped by the vertical mixing. This study highlights the importance of anthropogenic–biogenic interactions and meteorological dynamics in NPF in this climate-sensitive region.
Adriana Rocha-Lima, Peter R. Colarco, Anton S. Darmenov, Edward P. Nowottnick, Arlindo M. da Silva, and Luke D. Oman
Atmos. Chem. Phys., 24, 2443–2464, https://doi.org/10.5194/acp-24-2443-2024, https://doi.org/10.5194/acp-24-2443-2024, 2024
Short summary
Short summary
Observations show an increasing aerosol optical depth trend in the Middle East between 2003–2012. We evaluate the NASA Goddard Earth Observing System (GEOS) model's ability to capture these trends and examine the meteorological and surface parameters driving dust emissions. Our results highlight the importance of data assimilation for long-term trends of atmospheric aerosols and support the hypothesis that vegetation cover loss may have contributed to increasing dust emissions in the period.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
EGUsphere, https://doi.org/10.5194/egusphere-2024-496, https://doi.org/10.5194/egusphere-2024-496, 2024
Short summary
Short summary
This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean-atmosphere-aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low cloud fraction, decreasing the ocean and continental surface temperature and by reducing the precipitation of the coastal Western Africa. It also highlights the key role of the ocean temperature response and its feedbacks for the September to November season.
Danny M. Leung, Jasper F. Kok, Longlei Li, Natalie M. Mahowald, David M. Lawrence, Simone Tilmes, Erik Kluzek, Martina Klose, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 2287–2318, https://doi.org/10.5194/acp-24-2287-2024, https://doi.org/10.5194/acp-24-2287-2024, 2024
Short summary
Short summary
This study uses a premier Earth system model to evaluate a new desert dust emission scheme proposed in our companion paper. We show that our scheme accounts for more dust emission physics, hence matching better against observations than other existing dust emission schemes do. Our scheme's dust emissions also couple tightly with meteorology, hence likely improving the modeled dust sensitivity to climate change. We believe this work is vital for improving dust representation in climate models.
Ruth A. R. Digby, Nathan P. Gillett, Adam H. Monahan, Knut von Salzen, Antonis Gkikas, Qianqian Song, and Zhibo Zhang
Atmos. Chem. Phys., 24, 2077–2097, https://doi.org/10.5194/acp-24-2077-2024, https://doi.org/10.5194/acp-24-2077-2024, 2024
Short summary
Short summary
The COVID-19 lockdowns reduced aerosol emissions. We ask whether these reductions affected regional aerosol optical depth (AOD) and compare the observed changes to predictions from Earth system models. Only India has an observed AOD reduction outside of typical variability. Models overestimate the response in some regions, but when key biases have been addressed, the agreement is improved. Our results suggest that current models can realistically predict the effects of future emission changes.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen Arnold, Leighton Regayre, Meinrat Andreae, Mira Pöhlker, Duseong Jo, Man Yue, and Ken Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-401, https://doi.org/10.5194/egusphere-2024-401, 2024
Short summary
Short summary
Highly oxygenated organic molecules (HOMs) play an important role in atmospheric new particle formation (NPF). By explicitly coupling the chemical mechanism of HOMs and a comprehensive nucleation scheme in a global climate model. The updated model shows better agreement with measurements of nucleation rate, growth rate, NPF event frequency. Our results reveal that HOMs-driven NPF leads to a considerable increase in particle and cloud condensation nuclei burden globally.
Huisheng Bian, Mian Chin, Peter R. Colarco, Eric C. Apel, Donald R. Blake, Karl Froyd, Rebecca S. Hornbrook, Jose Jimenez, Pedro Campuzano Jost, Michael Lawler, Mingxu Liu, Marianne Tronstad Lund, Hitoshi Matsui, Benjamin A. Nault, Joyce E. Penner, Andrew W. Rollins, Gregory Schill, Ragnhild B. Skeie, Hailong Wang, Lu Xu, Kai Zhang, and Jialei Zhu
Atmos. Chem. Phys., 24, 1717–1741, https://doi.org/10.5194/acp-24-1717-2024, https://doi.org/10.5194/acp-24-1717-2024, 2024
Short summary
Short summary
This work studies sulfur in the remote troposphere at global and seasonal scales using aircraft measurements and multi-model simulations. The goal is to understand the sulfur cycle over remote oceans, spread of model simulations, and observation–model discrepancies. Such an understanding and comparison with real observations are crucial to narrow down the uncertainties in model sulfur simulations and improve understanding of the sulfur cycle in atmospheric air quality, climate, and ecosystems.
Gargi Sengupta, Minjie Zheng, and Nønne L. Prisle
Atmos. Chem. Phys., 24, 1467–1487, https://doi.org/10.5194/acp-24-1467-2024, https://doi.org/10.5194/acp-24-1467-2024, 2024
Short summary
Short summary
The effect of organic acid aerosol on sulfur chemistry and cloud properties was investigated in an atmospheric model. Organic acid dissociation was considered using both bulk and surface-related properties. We found that organic acid dissociation leads to increased hydrogen ion concentrations and sulfate aerosol mass in aqueous aerosols, increasing cloud formation. This could be important in large-scale climate models as many organic aerosol components are both acidic and surface-active.
Leena Kangas, Jaakko Kukkonen, Mari Kauhaniemi, Kari Riikonen, Mikhail Sofiev, Anu Kousa, Jarkko V. Niemi, and Ari Karppinen
Atmos. Chem. Phys., 24, 1489–1507, https://doi.org/10.5194/acp-24-1489-2024, https://doi.org/10.5194/acp-24-1489-2024, 2024
Short summary
Short summary
Residential wood combustion is a major source of fine particulate matter. This study has evaluated the contribution of residential wood combustion to fine particle concentrations and its year-to-year and seasonal variation in te Helsinki metropolitan area. The average concentrations attributed to wood combustion in winter were up to 10- or 15-fold compared to summer. Wood combustion caused 12 % to 14 % of annual fine particle concentrations. In winter, the contribution ranged from 16 % to 21 %.
Arto Heitto, Cheng Wu, Diego Aliaga, Luis Blacutt, Xuemeng Chen, Yvette Gramlich, Liine Heikkinen, Wei Huang, Radovan Krejci, Paolo Laj, Isabel Moreno, Karine Sellegri, Fernando Velarde, Kay Weinhold, Alfred Wiedensohler, Qiaozhi Zha, Federico Bianchi, Marcos Andrade, Kari E. J. Lehtinen, Claudia Mohr, and Taina Yli-Juuti
Atmos. Chem. Phys., 24, 1315–1328, https://doi.org/10.5194/acp-24-1315-2024, https://doi.org/10.5194/acp-24-1315-2024, 2024
Short summary
Short summary
Particle growth at the Chacaltaya station in Bolivia was simulated based on measured vapor concentrations and ambient conditions. Major contributors to the simulated growth were low-volatility organic compounds (LVOCs). Also, sulfuric acid had major role when volcanic activity was occurring in the area. This study provides insight on nanoparticle growth at this high-altitude Southern Hemispheric site and hence contributes to building knowledge of early growth of atmospheric particles.
Steven Soon-Kai Kong, Saginela Ravindra Babu, Sheng-Hsiang Wang, Stephen M. Griffith, Jackson Hian-Wui Chang, Ming-Tung Chuang, Guey-Rong Sheu, and Neng-Huei Lin
Atmos. Chem. Phys., 24, 1041–1058, https://doi.org/10.5194/acp-24-1041-2024, https://doi.org/10.5194/acp-24-1041-2024, 2024
Short summary
Short summary
In this study, we combined ground observations from 7-SEAS Dongsha Experiment, MERRA-2 reanalysis, and MODIS satellite images for evaluation and improvement of the CMAQ dust model for cases of East Asian Dust reaching the Taiwan region, including Dongsha in the western Pacific. We proposed a better CMAQ dust treatment over East Asia and for the first time revealed the impact of typhoons on dust transport.
Hengheng Zhang, Wei Huang, Xiaoli Shen, Ramakrishna Ramisetty, Junwei Song, Olga Kiseleva, Christopher Claus Holst, Basit Khan, Thomas Leisner, and Harald Saathoff
EGUsphere, https://doi.org/10.5194/egusphere-2024-90, https://doi.org/10.5194/egusphere-2024-90, 2024
Short summary
Short summary
Our study unravels how stagnant winter conditions elevate aerosol levels in Stuttgart. Cloud cover at night plays a pivotal role, impacting morning air quality. Validating a key model, our findings aid accurate air quality predictions, crucial for effective pollution mitigation in urban areas.
Cited articles
Altaratz, O., Koren, I., Yair, Y., and Price, C.: Lightning response to
smoke from Amazonian fires, Geophys. Res. Lett., 37, L07801,
https://doi.org/10.1029/2010GL042679, 2010.
Altaratz, O., Kucienska, B., Kostinski, A., Raga, G. B., and Koren, I.:
Global association of aerosol with flash density of intense lightning,
Environ. Res. Lett., 12, 114037, https://doi.org/10.1088/1748-9326/aa922b,
2017.
Bougeault, P. and Lacarrere, P.: Parameterization of orography-induced
turbulence in a mesobeta–scale model, Mon. Weather Rev., 117, 1872–1890,
https://doi.org/10.1175/1520-0493(1989)117<1872:POOITI>2.0.CO;2, 1989.
Brooks, I. M., Saunders, C. P. R., Mitzeva, R. P., and Peck, S. L.: The effect
on thunderstorm charging of the rate of rime accretion by graupel, Atmos.
Res., 43, 277–295, https://doi.org/10.1016/S0169-8095(96)00043-9, 1997.
Chaudhuri, S. and Middey, A.: Effect of meteorological parameters and
environmental pollution on thunderstorm and lightning activity over an urban
metropolis of India, Urban Clim., 3, 67–75,
https://doi.org/10.1016/j.uclim.2013.03.003, 2013.
Chen, F. and Dudhia, J.: Coupling an advanced land surface–hydrology model
with the Penn State–NCAR MM5 modeling system. Part I: Model implementation
and sensitivity, Mon. Weather Rev., 129, 569–585,
https://doi.org/10.1175/1520-0493(2001)129<0569:CAALSH>2.0.CO;2, 2001.
Chen, Z., Qie, X., Yair, Y., Liu, D., Xiao, X., Wang, D., and Yuan, S.:
Electrical evolution of a rapidly developing MCS during its vigorous
vertical growth phase, Atmos. Res., 246, 105201,
https://doi.org/10.1016/j.atmosres.2020.105201, 2020.
Dendy Jr., J. E.: Two multigrid methods for three-dimensional problems with
discontinuous and anisotropic coefficients, SIAM J. Sci. Stat. Comp.,
8, 673–685, https://doi.org/10.1137/0908059, 1987.
Dudhia, J.: Numerical study of convection observed during the winter monsoon
experiment using a mesoscale two-dimensional model, J. Atmos. Sci., 46,
3077–3107, https://doi.org/10.1175/1520-0469(1989)046<3077:NSOCOD>2.0.CO;2, 1989.
Dwyer, J. R.: A fundamental limit on electric fields in air, Geophys. Res.
Lett., 30, 2055, https://doi.org/10.1029/2003GL017781, 2003.
Fan, J., Zhang, R., Li, G., and Tao, W., K.: Effects of aerosols and
relative humidity on cumulus clouds, J. Geophys. Res., 112, D14204,
https://doi.org/10.1029/2006jd008136, 2007.
Fan, J., Leung, L. R., Rosenfeld, D., and DeMott, P. J.: Effects of cloud condensation nuclei and ice nucleating particles on precipitation processes and supercooled liquid in mixed-phase orographic clouds, Atmos. Chem. Phys., 17, 1017–1035, https://doi.org/10.5194/acp-17-1017-2017, 2017.
Fan, J., Rosenfeld, D., Zhang, Y., Giangrande, S., Li, Z., Machado, L., Martin, S., Yang, Y., Wang, J., Artaxo, P., Barbosa, H., Braga, R., Comstock, J., Feng, Z., Gao, W., Gomes, H., Mei, F., Pöhlker, C., Pöhlker, M., Pöschl, U., and Souza, R.: Substantial convection and precipitation enhancements by ultrafine aerosol particles, Science, 359, 411–418, https://doi.org/10.1126/science.aan8461, 2018.
Fierro, A. O., Mansell, E. R., MacGorman, D. R., and Ziegler, C. L.: The
implementation of an explicit charging and discharge lightning scheme within
the WRF-ARW model: Benchmark simulations of a continental squall line, a
tropical cyclone, and a winter storm, Mon. Weather Rev., 141, 2390–2415,
https://doi.org/10.1175/MWR-D-12-00278.1, 2013.
Guo, J., Deng, M., Lee, S.S., Wang, F., Li, Z., Zhai, P., Liu, H., Lv, W.,
Yao, W., and Li, X.: Delaying precipitation and lightning by air pollution
over the Pearl River Delta. Part I: Observational analyses, J. Geophys.
Res.-Atmos., 121, 6472–6488, https://doi.org/10.1002/2015JD023257, 2016.
Gustafsson, N., Janjić, T., Schraff, C., Leuenberger, D., Weissmann, M.,
Reich, H., et al.: Survey of data assimilation methods for convective-scale
numerical weather prediction at operational centres, Q. J. Roy. Meteor.
Soc., 144, 1218–1256, https://doi.org/10.1002/qj.3179, 2018.
Hobbs, P. V. and Rangno, A. L.: Ice particle concentrations in clouds, J.
Atmos. Sci., 42, 2523–2549,
https://doi.org/10.1175/1520-0469(1985)042<2523:IPCIC>2.0.CO;2, 1985.
Hu, J. X., Rosenfeld, D., Ryzhkov, A., Zrnic, D., Williams, E., Zhang, P.
F., Snyder, J. C., Zhang, R. Y., and Weitz, R.: Polarimetric radar
convective cell tracking reveals large sensitivity of cloud precipitation
and electrification properties to CCN, J. Geophys. Res.-Atmos., 124,
12194–12205, https://doi.org/10.1029/2019jd030857, 2019.
Jiang, M., Feng, J., Li, Z., Sun, R., Hou, Y.-T., Zhu, Y., Wan, B., Guo, J., and Cribb, M.: Potential influences of neglecting aerosol effects on the NCEP GFS precipitation forecast, Atmos. Chem. Phys., 17, 13967–13982, https://doi.org/10.5194/acp-17-13967-2017, 2017.
Kar, S. K., Liou, Y. A., and Ha, K. J.: Aerosol effects on the enhancement
of cloud-to-ground lightning over major urban areas of South Korea, Atmos.
Res., 92, 80–87, https://doi.org/10.1016/j.atmosres.2008.09.004, 2009.
Khain, A., Rosenfeld, D., and Pokrovsky, A.: Aerosol impact on the dynamics
and microphysics of deep convective clouds, Q. J. Roy. Meteor. Soc., 131,
2639–2663, https://doi.org/10.1256/qj.04.62, 2005.
Khain, A., Cohen, N., Lynn, B., and Pokrovsky, A.: Possible aerosol effects
on lightning activity and structure of hurricanes, J. Atmos. Sci., 65,
3652–3667, https://doi.org/10.1175/2008JAS2678.1, 2008.
Khain, A., Lynn, B., and Dudhia, J.: Aerosol Effects on Intensity of Landfalling Hurricanes as Seen from Simulations with the WRF Model with Spectral Bin Microphysics, J. Atmos. Sci., 67, 365–384, https://doi.org/10.1175/2009JAS3210.1, 2010.
Koren, I., Dagan, G., and Altaratz, O.: From aerosol-limited to invigoration of warm convective clouds, Science, 344, 1143–1146, https://doi.org/10.1126/science.1252595, 2014.
Kumjian, M. R., Ryzhkov, A. V., Melnikov, V. M., and Schuur, T. J.: Rapid-scan
super-resolution observations of a cyclic supercell with a dual-polarization
WSR-88D, Mon. Weather Rev., 138, 3762–3786,
https://doi.org/10.1175/2010MWR3322.1, 2010.
Li, X., Zhang, Q., and Xue, H.: The role of initial cloud condensation nuclei
concentration in hail using the WRF NSSL 2-moment microphysics scheme, Adv.
Atmos. Sci., 34, 1106–1120, https://doi.org/10.1007/s00376-017-6237-9,
2017.
Li, Z. Q., Wang, Y., Guo, J. P., Zhao, C. F., Cribb, M. C., Dong, X. Q.,
Fan, J. W., Gong, D. Y., Huang, J. P., Jiang, M. J., Jiang, Y. Q., Lee, S.
S., Li, H., Li, J. M., Liu, J. J., Qian, Y., Rosenfeld, D., Shan, S. Y.,
Sun, Y. L., Wang, H. J., Xin, J. Y., Yan, X., Yang, X., Yang, X. Q., Zhang,
F., and Zheng, Y. T.: East Asian study of tropospheric aerosols and their
impact on regional clouds, precipitation, and climate (EAST-AIR(CPC)), J.
Geophys. Res.-Atmos., 124, 13026–13054,
https://doi.org/10.1029/2019jd030758, 2019.
Liu, D., Sun, M., Su, D., Xu, W., Yu, H., and Chen, Y.: A five-year
climatological lightning characteristics of linear mesoscale convective
systems over North China, Atmos. Res., 256, 105580,
https://doi.org/10.1016/j.atmosres.2021.105580, 2021.
Liu, Z., Gao, W., Yu, Y., Hu, B., Xin, J., Sun, Y., Wang, L., Wang, G., Bi, X., Zhang, G., Xu, H., Cong, Z., He, J., Xu, J., and Wang, Y.: Characteristics of PM2.5 mass concentrations and chemical species in urban and background areas of China: emerging results from the CARE-China network, Atmos. Chem. Phys., 18, 8849–8871, https://doi.org/10.5194/acp-18-8849-2018, 2018.
Lynn, B. H., Khain, A., Rosenfeld, D., and Woodley, W. L.: Effects of
aerosols on precipitation from orographic clouds, J. Geophys. Res., 112,
D10225, https://doi.org/10.1029/2006JD007537, 2007.
Lynn, B. H., Kelman, G., and Ellrod, G.: An evaluation of the efficacy of using
observed lightning to improve convective lightning forecasts, Weather
Forecast., 30, 405–423, https://doi.org/10.1175/WAF-D-13-00028.1, 2015.
Lynn, B. H., Yair, Y., Shpund, J., Levi, Y., Qie, X., and Khain, A.: Using
factor separation to elucidate the respective contributions of desert dust
and urban pollution to the 4 January 2020 Tel Aviv lightning and flash flood
disaster, J. Geophys. Res.-Atmos., 125, e2020JD033520,
https://doi.org/10.1029/2020JD033520, 2020.
Mansell, E. R. and Ziegler, C. L.: Aerosol effects on simulated storm
electrification and precipitation in a two-moment bulk microphysics model,
J. Atmos. Sci. 70, 2032–2050, https://doi.org/10.1175/JAS-D-12-0264.1,
2013.
Mansell, E. R., MacGorman, D. R., Ziegler, C. L., and Straka, J. M.: Simulated three-dimensional branched lightning in a numerical thunderstorm model, J. Geophys. Res., 107, https://doi.org/10.1029/2000JD000244, 2002.
Mansell, E. R., MacGorman, D. R., Ziegler, C. L., and Straka, J. M.: Charge
structure and lightning sensitivity in a simulated multicell thunderstorm,
J. Geophys. Res.-Atmos., 110, D12101, https://doi.org/10.1029/2004JD005287,
2005.
Mansell, E. R., Ziegler, C. L., and Bruning, E. C.: Simulated
electrification of a small thunderstorm with two-moment bulk microphysics,
J. Atmos. Sci., 67, 171–194, https://doi.org/10.1175/2009jas2965.1, 2010.
Mitzeva, R., Latham, J., and Petrova, S.: A comparative modeling study of the
early electrical development of maritime and continental thunderstorms,
Atmos. Res., 82, 26–36, https://doi.org/10.1016/j.atmosres.2005.01.006,
2006.
Mlawer, E. J., Taubman, S. J., Brown, P. D., Iacono, M., and Clough, S.: Radiative transfer for inhomogeneous atmospheres: RRTM, a validated correlated-k model for the longwave, J. Geophys. Res.-Atmos., 102, 16663–16682, https://doi.org/10.1029/97JD00237, 1997.
Orville, R. E., Huffines, G., Nielsen-Gammon, J., Zhang, R., Ely, B.,
Steiger, S., Phillips, S., Allen, S., and Read, W.: Enhancement of
cloud-to-ground lightning over Houston, Texas, Geophys. Res. Lett., 28,
2597–2600, https://doi.org/10.1029/2001GL012990, 2001.
Price, C.: Global surface temperatures and the atmospheric electrical
circuit, Geophys. Res. Lett., 20, 1363–1366,
https://doi.org/10.1029/93GL01774, 1993.
Qie, X., Yuan, T., Xie, Y., and Ma, Y.: Spatial and temporal distribution of lightning activities on the Tibetan Plateau, Chinese J. Geophys., 47, 1122–1127, https://doi.org/10.1002/cjg2.596, 2004 (in Chinese).
Qie, K., Qie, X., and Tian, W.: Increasing trend of lightning activity in the
South Asia region, Sci. Bull., 66, 78–84,
https://doi.org/10.1016/j.scib.2020.08.033, 2021.
Qie, X., Yuan, T., Xie, Y., et al.: Spatial and temporal distribution of
lightning activities on the Tibetan Plateau, Chinese J. Geophys., 47,
1122–1127, https://doi.org/10.1002/cjg2.596, 2004 (in Chinese).
Qie, X., Yuan, S., Chen, Z., Wang, D., Liu, D., Sun, M., Sun, Z., Srivastava, A., Zhang, H., Lu, J., Xiao, H., Bi, Y., Feng, L., Tian, Y., Xu, Y., Jiang, R., Liu, M., Xiao, X., Duan, S., Su, D., Sun, C., Xu, W., Zhang, Y., Lu, G., Zhang, D., Yin, Y., and Yu, Y.: Understanding the dynamical-microphysical-electrical processes associated with severe thunderstorms over the Beijing metropolitan region, Sci. China Earth Sci., 64, 10–26, https://doi.org/10.1007/s11430-020-9656-8, 2020.
Rawlins, F.: A numerical study of thunderstorm electrification using a three dimensional model incorporating the ice phase, Quart. J. Meteor. Soc., 108, 779–800, https://doi.org/10.1002/qj.49710845804, 1982.
Rosenfeld, D., Lohmann, U., Raga, G. B., O'Dowd, C. D., Kulmala, M., Fuzzi,
S., Reissell, A., and Andreae, M. O.: Flood or Drought: How Do Aerosols
Affect Precipitation, Science, 321, 1309–1313,
https://doi.org/10.1126/science.1160606, 2008.
Saunders, C. P. R. and Peck, S. L.: Laboratory studies of the influence of the
rime accretion rate on charge transfer during crystal/graupel collisions, J.
Geophys. Res.-Atmos., 103, 13949–13956, https://doi.org/10.1029/97JD02644,
1998.
Saunders, C. P. R., Peck, S. L., Varela, G. G. A., Avila, E. E., and Castellano, N. E.: A laboratory study of the influence of water vapour and mixing on the charge transfer process during collisions between ice crystals and graupel, Atmos. Res., 58, 187–203, https://doi.org/10.1016/S0169-8095(01)00090-4, 2001.
Simpson, G. C. and Scrase, F. J.: The distribution of electricity in
thunderclouds, P. Roy. Soc. Lond. A, 161, 309–352,
https://doi.org/10.1098/rspa.1937.0148, 1937.
Srivastava, A., Tian, Y., Qie, X., Wang, D., Sun, Z., Yuan, S., Wang, Y., Chen, Z., Xu, W., Zhang, H., Jiang, R., and Su, D.: Performance assessment of Beijing Lightning Network (BLNET) and comparison with other lightning location networks across Beijing, Atmos. Res., 197, 76–83, https://doi.org/10.1016/j.atmosres.2017.06.026, 2017.
Stolz, D. C., Rutledge, S. A., and Pierce, J. R.: Simultaneous influences of
thermodynamics and aerosols on deep convection and lightning in the tropics,
J. Geophys. Res.-Atmos., 120, 6207–6231,
https://doi.org/10.1002/2014JD023033, 2015.
Storer, R. L., van den Heever, S. C., and Stephens, G. L.: Modeling aerosol
impacts on convective storms in different environments, J. Atmos. Sci., 67,
3904–3915, https://doi.org/10.1175/2010JAS3363.1, 2010.
Straka, J. M. and Mansell, E. R.: A bulk microphysics parameterization with
multiple ice precipitation categories, J. Appl. Meteorol. Clim., 44,
445–466, https://doi.org/10.1175/JAM2211.1, 2005.
Sun, J., Xue, M., Wilson, J. W., Zawadzki, I., Ballard, S. P., Onvlee-Hooimeyer, J., Joe, P., Barker, D. M., Li, P., Golding, B., Xu, M., and Pinto, J.: Use of NWP for nowcasting convective precipitation: Recent progress and challenges, Bull. Am. Meteorol. Soc., 95, 409–426, https://doi.org/10.1175/BAMS-D-11-00263.1, 2014.
Sun, M., Qie, X., Liu, D., Yair, Y., Xia, X., Yuan, S., Wang, D., Lu, J., Srivastava, A., and Ntwali, D.: Analysis of potential effects of aerosol on lightning activity in Beijing metropolitan region, Chinese J. of Geophys., 63, 1766–1774, https://doi.org/10.6038/cjg2020N0095, 2020 (in Chinese).
Takahashi, T.: Riming electrification as a charge generation mechanism in
thunderstorms, J. Atmos. Sci., 35, 1536–1548,
https://doi.org/10.1175/1520-0469(1978)035<1536:REAACG>2.0.CO;2, 1978.
Takahashi, T.: A numerical simulation of winter cumulus electrification.
Part I: Shallow cloud, J. Atmos. Sci., 40, 1257–1280,
https://doi.org/10.1175/1520-0469(1983)040<1257:ANSOWC>2.0.CO;2, 1983.
Tan, Y., Ma, X., Xiang, C., Xia, Y., and Zhang, X.: A numerical study of the effects of aerosol on electrification and lightning discharges during thunderstorms, Chinese J. Geophys., 60, 3041–3050, https://doi.org/10.6038/cjg20170812, 2017 (in Chinese).
Tao, W. K., Chen, J. P., Li, Z. Q., Wang, C., and Zhang, C. D.: Impact of
aerosols on convective clouds and precipitation, Rev. Geophys., 50, RG2001,
https://doi.org/10.1029/2011rg000369, 2012.
Thomas, R. J., Krehbiel, P. R., Rison, W., Hamlin, T., Harlin, J., and Shown, D.: Observations of VHF source powers radiated by lightning, Geophys. Res. Lett., 28, 143–146, https://doi.org/10.1029/2000GL011464, 2001.
Thornton, J. A., Virts, K. S., Holzworth, R. H., and Mitchell, T. P.:
Lightning enhancement over major oceanic shipping lanes, Geophys. Res.
Lett., 44, 9102–9111, https://doi.org/10.1002/2017GL074982, 2017.
Twomey, S.: The nuclei of natural cloud formation, Part II: The
supersaturation in natural clouds and the variation of cloud droplet
concentration, Geofis. Pura Appl., 43, 243–249,
https://doi.org/10.1007/BF01993560, 1959.
Van Den Broeke, M. S., Straka, J. M., and Rasmussen, E. N.: Polarimetric radar
observations at low levels during tornado life cycles in a small sample of
classic southern plains supercells, J. Appl. Meteorol. Clim., 47,
1232–1247, https://doi.org/10.1175/2007JAMC1714.1, 2008.
Wang, Q., Li, Z., Guo, J., Zhao, C., and Cribb, M.: The climate impact of aerosols on the lightning flash rate: is it detectable from long-term measurements?, Atmos. Chem. Phys., 18, 12797–12816, https://doi.org/10.5194/acp-18-12797-2018, 2018.
Wang, Y., Wan, Q., Meng, W., Liao, F., Tan, H., and Zhang, R.: Long-term impacts of aerosols on precipitation and lightning over the Pearl River Delta megacity area in China, Atmos. Chem. Phys., 11, 12421–12436, https://doi.org/10.5194/acp-11-12421-2011, 2011.
Wang, Y., Qie, X., Wang, D., Liu, M., Su, D., Wang, Z., Liu, D., Wu, Z., Sun, Z., and Tian, Y.: Beijing Lightning Network (BLNET) and the observation on preliminary breakdown processes, Atmos. Res., 171, 121–132, https://doi.org/10.1016/j.atmosres.2015.12.012, 2016.
Westcott, N. E.: Summertime cloud-to-ground lightning activity around major
Midwestern urban areas, J. Appl. Meteorol., 34, 1633–1642,
https://doi.org/10.1175/1520-0450-34.7.1633, 1995.
Williams, E. R.: The tripole structure of thunderstorms, J. Geophys.
Res.-Atmos., 94, 13151–13167, https://doi.org/10.1029/JD094iD11p13151,
1989.
Williams, E. R., Mushtak, V., Rosenfeld, D., Goodman, S., and Boccippio, D.:
Thermodynamic conditions favorable to superlative thunderstorm updraft,
mixed phase microphysics and lightning flash rate, Atmos. Res., 76,
288–306, https://doi.org/10.1016/j.atmosres.2004.11.009, 2005.
Xiong, Y., Qie, X., Zhou, Y., Yuan, T., and Zhang, T.: Regional responses of lightning activities to relative humidity of the surface, Chinese J. Geophys., 49, 311–318, https://doi.org/10.1002/cjg2.840, 2006 (in Chinese).
Yair, Y.: Charge generation and separation processes, Space Sci. Rev., 137,
119–131, https://doi.org/10.1007/s11214-008-9348-x, 2008.
Yair, Y.: Lightning hazards to human societies in a changing climate,
Environ. Res. Lett., 13, 123002, https://doi.org/10.1088/1748-9326/aaea86,
2018.
Yair, Y., Lynn, B., Price, C., Kotroni, V., Lagouvardos, K., Morin, E.,
Mugnai, A., and Llasat, M. D. C.: Predicting the potential for lightning
activity in Mediterranean storms based on the Weather Research and
Forecasting (WRF) model dynamic and microphysical fields, J. Geophys.
Res.-Atmos., 115, D04205, https://doi.org/10.1029/2008JD010868, 2010.
Yair, Y., Lynn, B., Yaffe, M., Ziv, B., and Shpund, J.: Observations and numerical simulations of the October 25th, 2015 super-cell thunderstorm over Central Israel, Atmos. Res., 247, 105165, https://doi.org/10.1016/j.atmosres.2020.105165, 2021.
Zhang, R., Jing, J., Tao, J., Hsu, S.-C., Wang, G., Cao, J., Lee, C. S. L., Zhu, L., Chen, Z., Zhao, Y., and Shen, Z.: Chemical characterization and source apportionment of PM2.5 in Beijing: seasonal perspective, Atmos. Chem. Phys., 13, 7053–7074, https://doi.org/10.5194/acp-13-7053-2013, 2013.
Zhang, H., Qie, X., Liu, M., Jiang, R., Lu, G., Liu, R., Liu, D., Chen, Z., Sun, Z., Li, Z., Li, J., and Ma, Z.: The charge structure in a thunderstorm based on three-dimensional electric field sonde, Chinese J. Geophys., 64, 1155–1166, https://doi.org/10.6038/cjg2021O0187, 2021 (in Chinese).
Zhao, P., Yin, Y., and Xiao, H.: The effects of aerosol on development of
thunderstorm electrification: A numerical study, Atmos. Res., 153, 376–391,
https://doi.org/10.1016/j.atmosres.2014.09.011, 2015.
Zhao, P., Li, Z., Xiao, H., Wu, F., Zheng, Y., Cribb, M. C., Jin, X., and Zhou, Y.: Distinct aerosol effects on cloud-to-ground lightning in the plateau and basin regions of Sichuan, Southwest China, Atmos. Chem. Phys., 20, 13379–13397, https://doi.org/10.5194/acp-20-13379-2020, 2020.
Ziegler, C. L.: Retrieval of thermal and microphysical variables in observed
convective storms. Part 1: Model development and preliminary testing, J.
Atmos. Sci., 42, 1487–1509,
https://doi.org/10.1175/1520-0469(1985)042<1487:ROTAMV>2.0.CO;2, 1985.
Ziegler, C. L. and MacGorman, D. R.: Observed lightning morphology relative to
modeled space charge and electric field distributions in a tornadic storm,
J. Atmos. Sci., 51, 833–851,
https://doi.org/10.1175/1520-0469(1994)051<0833:OLMRTM>2.0.CO;2, 1994.
Ziegler, C. L., MacGorman, D. R., Dye, J. E., and Ray, P. S.: A model evaluation of noninductive graupel‐ice charging in the early electrification of a mountain thunderstorm, J. Geophys. Res.-Atmos., 96, 12833–12855, https://doi.org/10.1029/91JD01246, 1991.
Zrnic, D. S., Balakrishnan, N., Ziegler, C. L., Bringi, V. N., Aydin, K., and Matejka, T.: Polarimetric signatures in the stratiform region of a mesoscale convective system, J. Appl. Meteorol. Climatol., 32, 678–693, https://doi.org/10.1175/1520-0450(1993)032<0678:PSITSR>2.0.CO;2, 1993.
Short summary
By acting as cloud condensation nuclei (CCN), increasing aerosol loading tends to enhance lightning activity through microphysical processes. We investigated the aerosol effects on the development of a thunderstorm. A two-moment bulk microphysics scheme and bulk lightning model were coupled in the WRF Model to simulate a multicell thunderstorm. Sensitivity experiments show that the enhancement of lightning activity under polluted conditions results from an increasing ice crystal number.
By acting as cloud condensation nuclei (CCN), increasing aerosol loading tends to enhance...
Altmetrics
Final-revised paper
Preprint