Articles | Volume 20, issue 9
https://doi.org/10.5194/acp-20-5559-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-5559-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
To what extents do urbanization and air pollution affect fog?
Shuqi Yan
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Nanjing University of Information Science &
Technology, Nanjing 210044, China
Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science & Technology, Nanjing 210044, China
Key Laboratory of Meteorological Disaster, Ministry of Education
(KLME), Nanjing University of Information Science & Technology, Nanjing 210044,
China
Special Test Field of National Integrated Meteorological Observation, Nanjing University of Information Science & Technology, Nanjing 210044, China
Bin Zhu
CORRESPONDING AUTHOR
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Nanjing University of Information Science &
Technology, Nanjing 210044, China
Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science & Technology, Nanjing 210044, China
Key Laboratory of Meteorological Disaster, Ministry of Education
(KLME), Nanjing University of Information Science & Technology, Nanjing 210044,
China
Special Test Field of National Integrated Meteorological Observation, Nanjing University of Information Science & Technology, Nanjing 210044, China
Yong Huang
Anhui Meteorology Institute, Key Lab of Atmospheric Science and Remote Sensing, Hefei 230031, China
Shouxian National Climatology Observatory, Shouxian 232200, China
Jun Zhu
Xiangshan Meteorological Bureau, Xiangshan 315700, China
Hanqing Kang
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Nanjing University of Information Science &
Technology, Nanjing 210044, China
Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science & Technology, Nanjing 210044, China
Key Laboratory of Meteorological Disaster, Ministry of Education
(KLME), Nanjing University of Information Science & Technology, Nanjing 210044,
China
Special Test Field of National Integrated Meteorological Observation, Nanjing University of Information Science & Technology, Nanjing 210044, China
Chunsong Lu
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Nanjing University of Information Science &
Technology, Nanjing 210044, China
Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science & Technology, Nanjing 210044, China
Key Laboratory of Meteorological Disaster, Ministry of Education
(KLME), Nanjing University of Information Science & Technology, Nanjing 210044,
China
Special Test Field of National Integrated Meteorological Observation, Nanjing University of Information Science & Technology, Nanjing 210044, China
Tong Zhu
IMSG, NOAA/NESDIS/STAR, 5830 University Research Ct., College Park, MD 20740, USA
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Fog is an important meteorological phenomenon that affects visibility. Aerosols and the planetary boundary layer (PBL) play critical roles in the fog life cycle. In this study, aerosol-induced changes in fog properties become more remarkable in the second fog (Fog2) than in the first fog (Fog1). The reason is that aerosol–cloud interaction (ACI) delays Fog1 dissipation, leading to the PBL meteorological conditions being more conducive to Fog2 formation and to stronger ACI in Fog2.
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EGUsphere, https://doi.org/10.5194/egusphere-2023-1089, https://doi.org/10.5194/egusphere-2023-1089, 2023
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The two-moment bulk cloud microphysics scheme used in CAM6 was modified to consider the impacts of the ice-crystal size distribution shape parameter (μi). After that, how the μi impacts cloud microphysical processes and then climate simulations is clearly illustrated by offline tests and CAM6 model experiments. Our results and findings are useful for the further development of μi-related parameterizations.
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This study quantified the contribution of each urban-induced meteorological effect (temperature, humidity, and circulation) to aerosol concentration. We found that the urban heat island (UHI) circulation dominates the UHI effects on aerosol. The UHI circulation transports aerosol and its precursor gases from the warmer lower boundary layer to the colder lower free troposphere and promotes the secondary formation of ammonium nitrate aerosol in the cold atmosphere.
Zhenbin Wang, Bin Zhu, Hanqing Kang, Wen Lu, Shuqi Yan, Delong Zhao, Weihang Zhang, and Jinhui Gao
Atmos. Chem. Phys., 21, 15555–15567, https://doi.org/10.5194/acp-21-15555-2021, https://doi.org/10.5194/acp-21-15555-2021, 2021
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In this paper, by using WRF-Chem with a black carbon (BC) tagging technique, we investigate the formation mechanism and regional sources of a BC peak in the free troposphere observed by aircraft flights. Local sources dominated BC from the surface to about 700 m (78.5 %), while the BC peak in the free troposphere was almost entirely imported from external sources (99.8 %). Our results indicate that cyclone systems can quickly lift BC up to the free troposphere, as well as extend its lifetime.
Meng Gao, Yang Yang, Hong Liao, Bin Zhu, Yuxuan Zhang, Zirui Liu, Xiao Lu, Chen Wang, Qiming Zhou, Yuesi Wang, Qiang Zhang, Gregory R. Carmichael, and Jianlin Hu
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Light absorption and radiative forcing of black carbon (BC) is influenced by both BC itself and its interactions with other aerosol chemical compositions. In this study, we used the online coupled WRF-Chem model to examine how emission control measures during the Asian-Pacific Economic Cooperation (APEC) conference affect the mixing state and light absorption of BC and the associated implications for BC-PBL interactions.
Hengnan Guo, Zefeng Zhang, Lin Jiang, Junlin An, Bin Zhu, Hanqing Kang, and Jing Wang
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Visibility is an indicator of atmospheric transparency and is widely used in many research fields. Although efforts have been made to improve the performance of visibility meters, a significant error exists in measured visibility data. This is because current methods of visibility measurement include a false assumption, which leads to the long-term neglect of an important source of visibility errors. Without major adjustments to current methods, it is not possible to obtain reliable data.
Jinhui Gao, Ying Li, Bin Zhu, Bo Hu, Lili Wang, and Fangwen Bao
Atmos. Chem. Phys., 20, 10831–10844, https://doi.org/10.5194/acp-20-10831-2020, https://doi.org/10.5194/acp-20-10831-2020, 2020
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Light extinction of aerosols can decease surface ozone mainly via reducing photochemical production of ozone. However, it also leads to high levels of ozone aloft being entrained down to the surface which partly counteracts the reduction in surface ozone. The impact of aerosols is more sensitive to local ozone, which suggests that while controlling the levels of aerosols, controlling the local ozone precursors is an effective way to suppress the increase of ozone over China at present.
Zhaobing Guo, Mingyi Xu, Yuxuan He, Shuo Gao, Chenmin Xu, Bin Zhu, Qingjun Guo, Xiaoyu Shen, Shuang Zhao, and Pengxiang Qiu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-506, https://doi.org/10.5194/acp-2020-506, 2020
Revised manuscript not accepted
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In order to gain insight into the formation mechanism of sulfate, stable sulfur isotope and Rayleigh distillation were applied to investigate the isotopic fractionations controlled by the oxidation pathways. The processes of SO2 oxidation on the surface of α-Fe2O3 with different chemical condition (NOX, O3 and NH3) were conducted in laboratory to study mechanism of SO2 oxidation. It was found that nitrogen oxides contributed primarily to the formation of sulfate among NOX, O3 and NH3 pathways.
Meng Gao, Jinhui Gao, Bin Zhu, Rajesh Kumar, Xiao Lu, Shaojie Song, Yuzhong Zhang, Beixi Jia, Peng Wang, Gufran Beig, Jianlin Hu, Qi Ying, Hongliang Zhang, Peter Sherman, and Michael B. McElroy
Atmos. Chem. Phys., 20, 4399–4414, https://doi.org/10.5194/acp-20-4399-2020, https://doi.org/10.5194/acp-20-4399-2020, 2020
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A regional fully coupled meteorology–chemistry model, Weather Research and Forecasting model with Chemistry (WRF-Chem), was employed to study the seasonality of ozone (O3) pollution and its sources in both China and India.
Xin Zhang, Yan Yin, Ronald van der A, Jeff L. Lapierre, Qian Chen, Xiang Kuang, Shuqi Yan, Jinghua Chen, Chuan He, and Rulin Shi
Atmos. Meas. Tech., 13, 1709–1734, https://doi.org/10.5194/amt-13-1709-2020, https://doi.org/10.5194/amt-13-1709-2020, 2020
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Lightning NOx has a strong impact on ozone and the hydroxyl radical production. However, the production efficiency of lightning NOx is still quite uncertain. This work develops the algorithm of estimating lightning NOx for both clean and polluted regions and evaluates the sensitivity of estimates to the model setting of lightning NO. Results reveal that our method reduces the sensitivity to the background NO2 and includes much of the below-cloud LNO2.
Hanqing Kang, Bin Zhu, Jinhui Gao, Yao He, Honglei Wang, Jifeng Su, Chen Pan, Tong Zhu, and Bu Yu
Atmos. Chem. Phys., 19, 3673–3685, https://doi.org/10.5194/acp-19-3673-2019, https://doi.org/10.5194/acp-19-3673-2019, 2019
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In this study, we found that a cold front can transport air pollutants from the polluted North China Plain to the Yangtze River Delta (YRD), thereby deteriorating air quality over the YRD. Before the cold frontal passage, a warm and polluted air mass over YRD climbed to the free troposphere (1.0–2.0 km) along the frontal surface. After the cold frontal passage, high pressure behind the frontal zone resulted in a synoptic subsidence that trapped PM2.5 in the surface.
Xuezhe Xu, Weixiong Zhao, Xiaodong Qian, Shuo Wang, Bo Fang, Qilei Zhang, Weijun Zhang, Dean S. Venables, Weidong Chen, Yong Huang, Xueliang Deng, Biwen Wu, Xinfeng Lin, Sen Zhao, and Yingxiang Tong
Atmos. Chem. Phys., 18, 16829–16844, https://doi.org/10.5194/acp-18-16829-2018, https://doi.org/10.5194/acp-18-16829-2018, 2018
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We report the direct field measurement of size-resolved mixing state, Eabs, and aerosol single-scattering albedo (SSA) at λ = 532 nm at a rural site in east China in summer. Parameterization of Eabs and SSA captures much of the influence of black carbon (BC) coating and particle absorption. The results show that absorption amplification depends on the coating thickness and the absorption of coating materials, and photochemistry plays role in modifying the absorption of BC-containing particles.
Jinhui Gao, Bin Zhu, Hui Xiao, Hanqing Kang, Chen Pan, Dongdong Wang, and Honglei Wang
Atmos. Chem. Phys., 18, 7081–7094, https://doi.org/10.5194/acp-18-7081-2018, https://doi.org/10.5194/acp-18-7081-2018, 2018
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This model study is about the effect of black carbon (BC) and the boundary layer interactions on surface ozone in an area of severe haze and ozone pollution in China. It shows the following: BC not only reduces photolysis rate, but also suppresses boundary layer (BL) development, then confines more ozone precursors. The BL suppression leads to less ozone aloft being entrained downward and finally leading to surface ozone reduction before noon.
Zefeng Zhang, Yan Shen, Yanwei Li, Bin Zhu, and Xingna Yu
Atmos. Chem. Phys., 17, 4147–4157, https://doi.org/10.5194/acp-17-4147-2017, https://doi.org/10.5194/acp-17-4147-2017, 2017
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Aerosol particles and relative humidity are the main factors that affect atmospheric visibility. Due to the complexity of the physicochemical properties of aerosol particles, more and more instruments and cost were put into research, which limited the development of large area observation research. Thus, it is especially important to find the key parameters which affect the visibility and to establish the observation scheme.
Chen Pan, Bin Zhu, Jinhui Gao, and Hanqing Kang
Geosci. Model Dev., 10, 673–688, https://doi.org/10.5194/gmd-10-673-2017, https://doi.org/10.5194/gmd-10-673-2017, 2017
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This paper describes the implementation of the atmospheric water tracer (AWT) method in the NCAR Community Atmosphere Model version 5.1 (CAM5.1). Compared to other source apportionment methods, the AWT method was developed based on detailed physical parameterisations, and can therefore trace the behaviour of atmospheric water substances directly and exactly. Using this method, we quantitatively identify the dominant sources of precipitation and water vapour over East Asia.
Related subject area
Subject: Clouds and Precipitation | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
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Adiabatic and radiative cooling are both important causes of aerosol activation in simulated fog events in Europe
Estimating the concentration of silver iodide needed to detect unambiguous signatures of glaciogenic cloud seeding
Ice-nucleating particle concentration impacts cloud properties over Dronning Maud Land, East Antarctica, in COSMO-CLM2
Numerical simulation of aerosol concentration effects on cloud droplet size spectrum evolutions of warm stratiform clouds in Jiangxi, China
The impact of aerosol on cloud water: a heuristic perspective
The presence of clouds lowers climate sensitivity in the MPI-ESM1.2 climate model
Diurnal variation in an amplified canopy urban heat island during heat wave periods in the megacity of Beijing: roles of mountain–valley breeze and urban morphology
Annemarie Lottermoser and Simon Unterstrasser
Atmos. Chem. Phys., 25, 7903–7924, https://doi.org/10.5194/acp-25-7903-2025, https://doi.org/10.5194/acp-25-7903-2025, 2025
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Contrail cirrus significantly contributes to aviation's overall climate impact. As hydrogen combustion and fuel cell use are emerging technologies for aircraft propulsion, we simulated individual contrails from hydrogen propulsion during the first 6 min after exhaust emission, termed the vortex phase. The ice crystal loss during that stage is crucial, as the number of ice crystals has a large impact on the further evolution of contrails into contrail cirrus and their radiative forcing.
Meilian Chen, Xiaoqin Jing, Jiaojiao Li, Jing Yang, Xiaobo Dong, Bart Geerts, Yan Yin, Baojun Chen, Lulin Xue, Mengyu Huang, Ping Tian, and Shaofeng Hua
Atmos. Chem. Phys., 25, 7581–7596, https://doi.org/10.5194/acp-25-7581-2025, https://doi.org/10.5194/acp-25-7581-2025, 2025
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Several recent studies have reported complete cloud glaciation induced by airborne-based glaciogenic cloud seeding over plains. Since turbulence is an important factor to maintain clouds in a mixed phase, it is hypothesized that turbulence may have an impact on the seeding effect. This hypothesis is evident in the present study, which shows that turbulence can accelerate the impact of airborne glaciogenic seeding of stratiform clouds.
Guillaume Feger, Jean-Pierre Chaboureau, Thibaut Dauhut, Julien Delanoë, and Pierre Coutris
Atmos. Chem. Phys., 25, 7447–7465, https://doi.org/10.5194/acp-25-7447-2025, https://doi.org/10.5194/acp-25-7447-2025, 2025
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Saharan air at the trade wind layer, cold pools, and dry upper troposphere has these three main factors inhibiting the cyclogenesis of the Pierre Henri mesoscale convective system. The findings were obtained through observations made during two flights of the Clouds-Atmospheric Dynamics-Dust Interactions in West Africa (CADDIWA) campaign and a convection-permitting simulation run with the Meso-NH model. They provide new insights into the complex dynamics of cyclogenesis in the Cabo Verde region and challenge the existing model of the Saharan Air Layer (SAL).
Gabriella Wallentin, Annika Oertel, Luisa Ickes, Peggy Achtert, Matthias Tesche, and Corinna Hoose
Atmos. Chem. Phys., 25, 6607–6631, https://doi.org/10.5194/acp-25-6607-2025, https://doi.org/10.5194/acp-25-6607-2025, 2025
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Multilayer clouds are common in the Arctic but remain underrepresented. We use an atmospheric model to simulate multilayer cloud cases from the Arctic expedition MOSAiC 2019/2020. We find that it is complex to accurately model these cloud layers due to the lack of correct temperature profiles. The model also struggles to capture the observed cloud phase and the relative concentration of cloud droplets and cloud ice. We constrain our model to measured aerosols to mitigate this issue.
Sisi Chen, Lulin Xue, Sarah A. Tessendorf, Thomas Chubb, Andrew Peace, Suzanne Kenyon, Johanna Speirs, Jamie Wolff, and Bill Petzke
Atmos. Chem. Phys., 25, 6703–6724, https://doi.org/10.5194/acp-25-6703-2025, https://doi.org/10.5194/acp-25-6703-2025, 2025
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This study aims to investigate how cloud seeding affects snowfall in Australia's Snowy Mountains. By running simulations with different setups, we found that seeding impact varies greatly with weather conditions. Seeding increased snow in stable weather but sometimes reduced it in stormy weather. This helps us to better understand when seeding works best to boost water supplies.
Ann Kristin Naumann, Monika Esch, and Bjorn Stevens
Atmos. Chem. Phys., 25, 6429–6444, https://doi.org/10.5194/acp-25-6429-2025, https://doi.org/10.5194/acp-25-6429-2025, 2025
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This study explores how uncertainties in the representation of microphysical processes affect the tropical condensate distribution in the global storm-resolving model ICON. The results point to the importance of the fall speed of hydrometeor particles and to a simple relationship: the faster a condensate falls, the less there is of it. Implications for the energy balance and precipitation properties are discussed.
Yao-Sheng Chen, Prasanth Prabhakaran, Fabian Hoffmann, Jan Kazil, Takanobu Yamaguchi, and Graham Feingold
Atmos. Chem. Phys., 25, 6141–6159, https://doi.org/10.5194/acp-25-6141-2025, https://doi.org/10.5194/acp-25-6141-2025, 2025
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Injecting sea salt aerosols into marine stratiform clouds can distribute the cloud water over more droplets in smaller sizes. This process is expected to make the clouds brighter, allowing them to reflect more sunlight back to space. However, it may also cause the clouds to lose water over time, reducing their ability to reflect sunlight. We use a computer model to show that the loss of cloud water occurs relatively quickly and does not completely offset the initial brightening.
Pouriya Alinaghi, Fredrik Jansson, Daniel A. Blázquez, and Franziska Glassmeier
Atmos. Chem. Phys., 25, 6121–6139, https://doi.org/10.5194/acp-25-6121-2025, https://doi.org/10.5194/acp-25-6121-2025, 2025
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Shallow clouds in the trades are a major source of uncertainty in climate projections. These clouds organize into striking mesoscale patterns that are exactly what climate models lack. This study explores the origin of such patterns and investigates how variations in microscale properties control them. The importance of microscale effects is compared to that of large-scale forcing on the mesoscale organization of trade-cumulus fields.
Hsiang-He Lee, Xue Zheng, Shaoyue Qiu, and Yuan Wang
Atmos. Chem. Phys., 25, 6069–6091, https://doi.org/10.5194/acp-25-6069-2025, https://doi.org/10.5194/acp-25-6069-2025, 2025
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The study investigates how aerosol–cloud interactions affect warm boundary layer stratiform clouds over the eastern North Atlantic. High-resolution weather model simulations reveal that non-rain clouds at the edge of cloud systems are prone to evaporation, leading to an aerosol drying effect and a transition of aerosols back to the accumulation mode for future activation. The study shows that this dynamic behavior is often not adequately represented in most previous prescribed-aerosol simulations.
Patrick Peter, Sigrun Matthes, Christine Frömming, Patrick Jöckel, Luca Bugliaro, Andreas Giez, Martina Krämer, and Volker Grewe
Atmos. Chem. Phys., 25, 5911–5934, https://doi.org/10.5194/acp-25-5911-2025, https://doi.org/10.5194/acp-25-5911-2025, 2025
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Our study examines how well the global climate model EMAC (ECHAM/MESSy Atmospheric Chemistry) predicts contrail formation by analysing temperature and humidity – two key factors for contrail development and persistence. The model underestimates temperature, leading to an overprediction of contrail formation and larger ice-supersaturated regions. Adjusting the model improves temperature accuracy but adds uncertainties. Better predictions of contrail formation areas can help optimise flight tracks to reduce aviation's climate effect.
Konstantinos Kourtidis, Stavros Stathopoulos, and Vassilis Amiridis
Atmos. Chem. Phys., 25, 5935–5946, https://doi.org/10.5194/acp-25-5935-2025, https://doi.org/10.5194/acp-25-5935-2025, 2025
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The sound of thunder induces mechanical effects on cloud droplets and ice particles, causing changes in their size distribution. A shock wave near the lightning channel causes extensive shattering of cloud particles. At a distance, the audio wave will cause agglomeration of particles. So, thunder may influence the rain generation process and the radiative properties of clouds. As global warming may influence the occurrence rate of lightning, a climate feedback may be induced by these mechanisms.
Nathan H. Pope and Adele L. Igel
Atmos. Chem. Phys., 25, 5433–5444, https://doi.org/10.5194/acp-25-5433-2025, https://doi.org/10.5194/acp-25-5433-2025, 2025
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We used an atmospheric model that simulates a single column to study the sensitivity of marine fog formed through the lowering of the base of a stratus cloud to meteorology and aerosols. We found that higher aerosol concentration reduces the likelihood and duration of fog but leads to denser fog. This overall trend was caused by multiple physical mechanisms depending on conditions.
Jung-Sub Lim, Yign Noh, Hyunho Lee, and Fabian Hoffmann
Atmos. Chem. Phys., 25, 5313–5329, https://doi.org/10.5194/acp-25-5313-2025, https://doi.org/10.5194/acp-25-5313-2025, 2025
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Rain formation in warm clouds begins when small droplets collide, but this process can be slow without larger droplets. We used simulations to explore the role of bigger droplets, known as precipitation embryos, in triggering rain. We found that they speed up rain only when their size and number exceed a critical threshold. This threshold becomes larger when collisions are naturally efficient, such as in clouds with broad droplet size distributions or strong turbulence.
Je-Yun Chun, Robert Wood, Peter N. Blossey, and Sarah J. Doherty
Atmos. Chem. Phys., 25, 5251–5271, https://doi.org/10.5194/acp-25-5251-2025, https://doi.org/10.5194/acp-25-5251-2025, 2025
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This study explores how aerosols affect clouds transitioning from stratocumulus to cumulus along trade winds under varying atmospheric conditions. We found that aerosols typically reduce precipitation and raise cloud height, but their impact changes when subsidence changes by aerosol enhancement are considered. Our findings indicate that the cooling effect of aerosols might be overestimated if these atmospheric changes are not accounted for.
Wojciech W. Grabowski and Hanna Pawlowska
Atmos. Chem. Phys., 25, 5273–5285, https://doi.org/10.5194/acp-25-5273-2025, https://doi.org/10.5194/acp-25-5273-2025, 2025
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A simple diagram to depict cloud droplets' formation via the activation of cloud condensation nuclei (CCN) as well as their subsequent growth and evaporation is presented.
Albert Ansmann, Cristofer Jimenez, Daniel A. Knopf, Johanna Roschke, Johannes Bühl, Kevin Ohneiser, and Ronny Engelmann
Atmos. Chem. Phys., 25, 4867–4884, https://doi.org/10.5194/acp-25-4867-2025, https://doi.org/10.5194/acp-25-4867-2025, 2025
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In this study, we focus on the potential impact of wildfire smoke on cirrus formation. Aerosol and cirrus observations with lidar and radar during the MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition, presented in the companion paper (Ansmann et al., 2025), are closely linked to comprehensive modeling of ice nucleation in cirrus evolution processes, presented in this article. A clear impact of wildfire smoke on cirrus formation was found.
August Mikkelsen, Daniel T. McCoy, Trude Eidhammer, Andrew Gettelman, Ci Song, Hamish Gordon, and Isabel L. McCoy
Atmos. Chem. Phys., 25, 4547–4570, https://doi.org/10.5194/acp-25-4547-2025, https://doi.org/10.5194/acp-25-4547-2025, 2025
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Whether increased aerosol increases or decreases liquid cloud mass has been a longstanding question. Observed correlations suggest that aerosols thin liquid cloud, but we are able to show that observations were consistent with an increase in liquid cloud in response to aerosols by leveraging a model where causality could be traced.
Tim Lüttmer, Peter Spichtinger, and Axel Seifert
Atmos. Chem. Phys., 25, 4505–4529, https://doi.org/10.5194/acp-25-4505-2025, https://doi.org/10.5194/acp-25-4505-2025, 2025
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We investigate ice formation pathways in idealized convective clouds using a novel microphysics scheme that distinguishes between five ice classes each with their own unique formation mechanism. Ice crystals from rime splintering form the lowermost layer of ice crystals around the updraft core. The majority of ice crystals in the anvil of the convective cloud stems from frozen droplets. Ice stemming from homogeneous and deposition nucleation was only relevant in the overshoot.
Sanjeevani Panditharatne, Helen Brindley, Caroline Cox, Rui Song, Richard Siddans, Richard Bantges, Jonathan Murray, Stuart Fox, and Cathryn Fox
EGUsphere, https://doi.org/10.5194/egusphere-2025-647, https://doi.org/10.5194/egusphere-2025-647, 2025
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Upwelling radiation with wavelengths between 15 and 100 microns is theorised to be highly sensitive to the properties of ice clouds, particularly the shape of the ice crystals. We exploit this sensitivity and perform the first retrieval of ice cloud properties using these wavelengths from an observation taken on an aircraft and evaluate it against measurements of the cloud’s properties.
Fan Yang, Hamed Fahandezh Sadi, Raymond A. Shaw, Fabian Hoffmann, Pei Hou, Aaron Wang, and Mikhail Ovchinnikov
Atmos. Chem. Phys., 25, 3785–3806, https://doi.org/10.5194/acp-25-3785-2025, https://doi.org/10.5194/acp-25-3785-2025, 2025
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Large-eddy simulations of a convection cloud chamber show two new microphysics regimes, cloud oscillation and cloud collapse, due to haze–cloud interactions. Our results suggest that haze particles and their interactions with cloud droplets should be considered especially in polluted conditions. To properly simulate haze–cloud interactions, we need to resolve droplet activation and deactivation processes, instead of using Twomey-type activation parameterization.
Declan L. Finney, Alan M. Blyth, Paul R. Field, Martin I. Daily, Benjamin J. Murray, Mengyu Sun, Paul J. Connolly, Zhiqiang Cui, and Steven Böing
EGUsphere, https://doi.org/10.5194/egusphere-2025-1227, https://doi.org/10.5194/egusphere-2025-1227, 2025
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We present observation-informed modelling from the Deep Convective Microphysics Experiment to study how environmental conditions and cloud processes affect anvil cloud albedo and radiation. Aerosols influencing cloud droplets or influencing ice formation yield varying radiative effects. We introduce fingerprint metrics to discern these effects. Using detailed observations and modelling, we offer insights into high cloud radiative effects and feedbacks.
Pierre Grzegorczyk, Wolfram Wobrock, Aymeric Dziduch, and Céline Planche
EGUsphere, https://doi.org/10.5194/egusphere-2025-819, https://doi.org/10.5194/egusphere-2025-819, 2025
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The impact of secondary ice production (SIP) on a HYMEX intense precipitation event is investigated using 3D bin microphysics. Including SIP improves agreement with in situ aircraft observations (ice crystal number concentration and supercooled drop number fraction), generates small ice crystals and redistributes condensed water mass toward smaller particle sizes. As these crystals melt, the liquid precipitation flux decreases, reducing total precipitation by 8 % and heavy rainfall by 20 %.
Hairu Ding, Bjorn Stevens, and Hauke Schmidt
EGUsphere, https://doi.org/10.5194/egusphere-2025-876, https://doi.org/10.5194/egusphere-2025-876, 2025
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This study examines the physical link between subtropical highs and stratocumulus variability. Using reanalysis data, we test two proposed pathways—one at the surface and one in the free troposphere—but find that neither is a dominant mechanism for stratocumulus variability on seasonal and interannual timescales. These results challenge the assumed influence of subtropical highs on stratocumulus and highlight the need for further research into lower tropospheric stability dynamics.
Xuemei Wang, Kenneth S. Carslaw, Daniel P. Grosvenor, and Hamish Gordon
EGUsphere, https://doi.org/10.5194/egusphere-2025-132, https://doi.org/10.5194/egusphere-2025-132, 2025
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Anthropogenic emissions can influence aerosol particle number concentrations via new particle formation. Our model simulations predict around 10 % increase of the particle and cloud droplet number concentrations when doubling the emissions in the Manaus region in the Amazonian wet season. However, the corresponding changes in cloud water and rain mass are around 4 %. Such weak response implied that this convective environment is not sensitive to the localised anthropogenic emission changes here.
Shiye Huang, Jing Yang, Jiaojiao Li, Qian Chen, Qilin Zhang, and Fengxia Guo
Atmos. Chem. Phys., 25, 1831–1850, https://doi.org/10.5194/acp-25-1831-2025, https://doi.org/10.5194/acp-25-1831-2025, 2025
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Aerosol and secondary ice production are both vital to charge separation in thunderstorms, but the relative importance of different SIP processes to cloud electrification under different aerosol conditions is not well understood. In this study, we show in a clean environment, the shattering of freezing drops has the greatest effect on the charging rate, while in a polluted environment, both rime splintering and the shattering of freezing drops have a significant effect on cloud electrification.
Blaž Gasparini, Rachel Atlas, Aiko Voigt, Martina Krämer, and Peter N. Blossey
EGUsphere, https://doi.org/10.5194/egusphere-2025-203, https://doi.org/10.5194/egusphere-2025-203, 2025
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Tropical cirrus clouds, especially their evolution, are poorly understood, contributing to uncertainty in climate projections. We address this by using novel tracers in a cloud-resolving model to track the life cycle of cirrus clouds, providing insights into cloud formation, ice crystal evolution, and radiative effects. We also improve the model's cloud microphysics with a simple, computationally efficient approach that can be applied to other models.
Harri Kokkola, Juha Tonttila, Silvia M. Calderón, Sami Romakkaniemi, Antti Lipponen, Aapo Peräkorpi, Tero Mielonen, Edward Gryspeerdt, Timo Henrik Virtanen, Pekka Kolmonen, and Antti Arola
Atmos. Chem. Phys., 25, 1533–1543, https://doi.org/10.5194/acp-25-1533-2025, https://doi.org/10.5194/acp-25-1533-2025, 2025
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Understanding how atmospheric aerosols affect clouds is a scientific challenge. One question is how aerosols affects the amount of cloud water. We used a cloud-scale model to study these effects on marine clouds. The study showed that variations in cloud properties and instrument noise can cause bias in satellite-derived cloud water content. However, our results suggest that for similar weather conditions with well-defined aerosol concentrations, satellite data can reliably track these effects.
Naifang Bei, Bo Xiao, Ruonan Wang, Yuning Yang, Lang Liu, Yongming Han, and Guohui Li
EGUsphere, https://doi.org/10.5194/egusphere-2024-3558, https://doi.org/10.5194/egusphere-2024-3558, 2025
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This study uses a cloud-resolving model to examine how aerosols influence a mesoscale convective system (MCS) in central China via aerosol-radiation (ARIs) and aerosol-cloud interactions (ACIs). Without ARIs, added aerosols don’t significantly affect precipitation due to cloud competition for moisture. ARIs can stabilize or enhance convection. High aerosol levels lead to a combined ARI and ACI effect that greatly reduces precipitation.
Franziska Hellmuth, Tim Carlsen, Anne Sophie Daloz, Robert Oscar David, Haochi Che, and Trude Storelvmo
Atmos. Chem. Phys., 25, 1353–1383, https://doi.org/10.5194/acp-25-1353-2025, https://doi.org/10.5194/acp-25-1353-2025, 2025
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This article compares the occurrence of supercooled liquid-containing clouds (sLCCs) and their link to surface snowfall in CloudSat–CALIPSO, ERA5, and the CMIP6 models. Significant discrepancies were found, with ERA5 and CMIP6 consistently overestimating sLCC and snowfall frequency. This bias is likely due to cloud microphysics parameterization. This conclusion has implications for accurately representing cloud phase and snowfall in future climate projections.
Claudia Christine Stephan and Bjorn Stevens
Atmos. Chem. Phys., 25, 1209–1226, https://doi.org/10.5194/acp-25-1209-2025, https://doi.org/10.5194/acp-25-1209-2025, 2025
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Tropical precipitation cluster area and intensity distributions follow power laws, but the physical processes responsible for this behavior remain unknown. We analyze global simulations that realistically represent precipitation processes. We consider Earth-like planets as well as virtual planets to realize different types of large-scale dynamics. Our finding is that power laws in Earth’s precipitation cluster statistics stem from the robust power laws in Earth’s atmospheric wind field.
Tim Lüttmer, Annette Miltenberger, and Peter Spichtinger
EGUsphere, https://doi.org/10.5194/egusphere-2025-185, https://doi.org/10.5194/egusphere-2025-185, 2025
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We investigate ice formation pathways in a warm conveyor belt case study. We employ a multi-phase microphysics scheme that distinguishes between ice from different nucleation processes. Ice crystals in the cirrus outflow mostly stem from in-situ formation. Hence they were formed directly from the vapor phase. Sedimentational redistribution modulates cirrus properties and leads to a disagreement between cirrus origin classifications based on thermodynamic history and nucleation processes.
Seoung Soo Lee, Chang Hoon Jung, Jinho Choi, Young Jun Yoon, Junshik Um, Youtong Zheng, Jianping Guo, Manguttathil G. Manoj, Sang-Keun Song, and Kyung-Ja Ha
Atmos. Chem. Phys., 25, 705–726, https://doi.org/10.5194/acp-25-705-2025, https://doi.org/10.5194/acp-25-705-2025, 2025
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This study attempts to test a general factor that explains differences in the properties of different mixed-phase clouds using a modeling tool. Although this attempt is not to identify a factor that can perfectly explain and represent the properties of different mixed-phase clouds, we believe that this attempt acts as a valuable stepping stone towards a more complete, general way of using climate models to better predict climate change.
Wenjie Zhang, Hong Wang, Xiaoye Zhang, Yue Peng, Zhaodong Liu, Deying Wang, Da Zhang, Chen Han, Yang Zhao, Junting Zhong, Wenxing Jia, Huiqiong Ning, and Huizheng Che
EGUsphere, https://doi.org/10.5194/egusphere-2024-3677, https://doi.org/10.5194/egusphere-2024-3677, 2025
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We implement a real-time subgrid-scale aerosol-cloud interaction (ACI) mechanism in a mesoscale atmospheric chemistry system and find that subgrid-scale ACI can improve meteorological factors predictions. This study demonstrates the importance of real-time subgrid-scale ACI to weather forecast and the necessity of multiscale ACI studies.
Xinyi Huang, Paul R. Field, Benjamin J. Murray, Daniel P. Grosvenor, Floortje van den Heuvel, and Kenneth S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-4070, https://doi.org/10.5194/egusphere-2024-4070, 2025
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Cold-air outbreak (CAO) clouds play a vital role in climate prediction. This study explores the responses of CAO clouds to aerosols and ice production under different environmental conditions. We found that CAO cloud responses vary with cloud temperature and are strongly controlled by the liquid-ice partitioning in these clouds, suggesting the importance of good representations of cloud microphysics properties to predict the behaviours of CAO clouds in a warming climate.
Jordan Eissner, David Mechem, Yi Jin, Virendra Ghate, and James Booth
EGUsphere, https://doi.org/10.5194/egusphere-2024-3438, https://doi.org/10.5194/egusphere-2024-3438, 2025
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Low-level clouds have important radiative feedbacks and can occur in a range of meteorological conditions, yet our knowledge and prediction of them are insufficient. We evaluate model forecasts of low-level cloud properties across a cold front and the associated environments that they form in. The model represents the meteorological conditions well and produces broken clouds behind the cold front in areas of strong surface forcing, large stability, and large-scale subsiding motion.
Kevin Wolf, Nicolas Bellouin, Olivier Boucher, Susanne Rohs, and Yun Li
Atmos. Chem. Phys., 25, 157–181, https://doi.org/10.5194/acp-25-157-2025, https://doi.org/10.5194/acp-25-157-2025, 2025
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ERA5 atmospheric reanalysis and airborne in situ observations from IAGOS are compared in terms of the representation of the contrail formation potential and the presence of supersaturation. Differences are traced back to biases in ERA5 relative humidity fields. Those biases are addressed by applying a quantile mapping technique that significantly improved contrail estimation based on post-processed ERA5 data.
Marje Prank, Juha Tonttila, Xiaoxia Shang, Sami Romakkaniemi, and Tomi Raatikainen
Atmos. Chem. Phys., 25, 183–197, https://doi.org/10.5194/acp-25-183-2025, https://doi.org/10.5194/acp-25-183-2025, 2025
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Large primary bioparticles such as pollen can be abundant in the atmosphere. In humid conditions pollen can rupture and release a large number of fine sub-pollen particles (SPPs). The paper investigates what kind of birch pollen concentrations are needed for the pollen and SPPs to start playing a noticeable role in cloud processes and alter precipitation formation. In the studied cases only the largest observed pollen concentrations were able to noticeably alter the precipitation formation.
Luís Filipe Escusa dos Santos, Hannah C. Frostenberg, Alejandro Baró Pérez, Annica M. L. Ekman, Luisa Ickes, and Erik S. Thomson
Atmos. Chem. Phys., 25, 119–142, https://doi.org/10.5194/acp-25-119-2025, https://doi.org/10.5194/acp-25-119-2025, 2025
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The Arctic is experiencing enhanced surface warming. The observed decline in Arctic sea-ice extent is projected to lead to an increase in Arctic shipping activity, which may lead to further climatic feedbacks. Using an atmospheric model and results from marine engine experiments that focused on fuel sulfur content reduction and exhaust wet scrubbing, we investigate how ship exhaust particles influence the properties of Arctic clouds. Implications for radiative surface processes are discussed.
Julie Carles, Nicolas Bellouin, Najda Villefranque, and Jean-Louis Dufresne
EGUsphere, https://doi.org/10.5194/egusphere-2024-3642, https://doi.org/10.5194/egusphere-2024-3642, 2025
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Cirrus and contrails affect Earth’s energy balance with a lot of remaining uncertainty. The balance between solar and terrestrial radiation is delicate to calculate, and factors as cloud optical depth, shape, Sun position are crucial to estimate the effect of those clouds on radiation. Also, often neglected three dimensional paths of radiation, or 3D effects, may be important to account for at climatic scale.
Nadja Omanovic, Brigitta Goger, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 14145–14175, https://doi.org/10.5194/acp-24-14145-2024, https://doi.org/10.5194/acp-24-14145-2024, 2024
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We evaluated the numerical weather model ICON in two horizontal resolutions with two bulk microphysics schemes over hilly and complex terrain in Switzerland and Austria, respectively. We focused on the model's ability to simulate mid-level clouds in summer and winter. By combining observational data from two different field campaigns, we show that an increase in the horizontal resolution and a more advanced cloud microphysics scheme is strongly beneficial for cloud representation.
Cornelis Schwenk and Annette Miltenberger
Atmos. Chem. Phys., 24, 14073–14099, https://doi.org/10.5194/acp-24-14073-2024, https://doi.org/10.5194/acp-24-14073-2024, 2024
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Warm conveyor belts (WCBs) transport moisture into the upper atmosphere, where it acts as a greenhouse gas. This transport is not well understood, and the role of rapidly rising air is unclear. We simulate a WCB and look at fast- and slow-rising air to see how moisture is (differently) transported. We find that for fast-ascending air more ice particles reach higher into the atmosphere and that frozen cloud particles are removed differently than during slow ascent, which has more water vapour.
Fabian Hoffmann, Yao-Sheng Chen, and Graham Feingold
EGUsphere, https://doi.org/10.5194/egusphere-2024-3893, https://doi.org/10.5194/egusphere-2024-3893, 2024
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Clouds reflect a substantial portion of the incoming solar radiation back into space. This capacity is determined by the number of cloud droplets, which in turn is influenced by the number of aerosol particles, forming the basis for aerosol-cloud-climate interactions. In this study, we use a simple mixed-layer approach to understand the effect of aerosol on cloud water in non-precipitating stratocumulus.
Pratapaditya Ghosh, Ian Boutle, Paul Field, Adrian Hill, Anthony Jones, Marie Mazoyer, Katherine J. Evans, Salil Mahajan, Hyun-Gyu Kang, Min Xu, Wei Zhang, Noah Asch, and Hamish Gordon
EGUsphere, https://doi.org/10.5194/egusphere-2024-3376, https://doi.org/10.5194/egusphere-2024-3376, 2024
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We study aerosol-fog interactions near Paris using a weather and climate model with high spatial resolution. We show that our model can simulate fog lifecycle effectively. We find that the fog droplet number concentrations, the amount of liquid water in the fog, and the vertical structure of the fog are highly sensitive to the parameterization that simulates droplet formation and growth. The changes we propose could improve fog forecasts significantly without increasing computational costs.
Pratapaditya Ghosh, Ian Boutle, Paul Field, Adrian Hill, Marie Mazoyer, Katherine J. Evans, Salil Mahajan, Hyun-Gyu Kang, Min Xu, Wei Zhang, and Hamish Gordon
EGUsphere, https://doi.org/10.5194/egusphere-2024-3397, https://doi.org/10.5194/egusphere-2024-3397, 2024
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We study the lifecycle of fog events in Europe using a weather and climate model. By incorporating droplet formation and growth driven by radiative cooling, our model better simulates the total liquid water in foggy atmospheric columns. We show that both adiabatic and radiative cooling play significant, often equally important roles in driving droplet formation and growth. We discuss strategies to address droplet number overpredictions, by improving model physics and addressing model artifacts.
Jing Yang, Jiaojiao Li, Meilian Chen, Xiaoqin Jing, Yan Yin, Bart Geerts, Zhien Wang, Yubao Liu, Baojun Chen, Shaofeng Hua, Hao Hu, Xiaobo Dong, Ping Tian, Qian Chen, and Yang Gao
Atmos. Chem. Phys., 24, 13833–13848, https://doi.org/10.5194/acp-24-13833-2024, https://doi.org/10.5194/acp-24-13833-2024, 2024
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Detecting unambiguous signatures is vital for examining cloud-seeding impacts, but often, seeding signatures are immersed in natural variability. In this study, reflectivity changes induced by glaciogenic seeding using different AgI concentrations are investigated under various conditions, and a method is developed to estimate the AgI concentration needed to detect unambiguous seeding signatures. The results aid in operational seeding-based decision-making regarding the amount of AgI dispersed.
Florian Sauerland, Niels Souverijns, Anna Possner, Heike Wex, Preben Van Overmeiren, Alexander Mangold, Kwinten Van Weverberg, and Nicole van Lipzig
Atmos. Chem. Phys., 24, 13751–13768, https://doi.org/10.5194/acp-24-13751-2024, https://doi.org/10.5194/acp-24-13751-2024, 2024
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We use a regional climate model, COSMO-CLM², enhanced with a module resolving aerosol processes, to study Antarctic clouds. We prescribe different concentrations of ice-nucleating particles to our model to assess how these clouds respond to concentration changes, validating results with cloud and aerosol observations from the Princess Elisabeth Antarctica station. Our results show that aerosol–cloud interactions vary with temperature, providing valuable insights into Antarctic cloud dynamics.
Yi Li, Xiaoli Liu, and Hengjia Cai
Atmos. Chem. Phys., 24, 13525–13540, https://doi.org/10.5194/acp-24-13525-2024, https://doi.org/10.5194/acp-24-13525-2024, 2024
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The influence of different aerosol modes on cloud processes remains controversial. We modified the aerosol spectra and concentrations to simulate a warm stratiform cloud process in Jiangxi, China, using the WRF-SBM scheme. Research shows that different aerosol spectra have diverse effects on cloud droplet spectra, cloud development, and the correlation between dispersion (ε) and cloud physics quantities. Compared to cloud droplet concentration, ε is more sensitive to the volume radius.
Fabian Hoffmann, Franziska Glassmeier, and Graham Feingold
Atmos. Chem. Phys., 24, 13403–13412, https://doi.org/10.5194/acp-24-13403-2024, https://doi.org/10.5194/acp-24-13403-2024, 2024
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Clouds constitute a major cooling influence on Earth's climate system by reflecting a large fraction of the incident solar radiation back to space. This ability is controlled by the number of cloud droplets, which is governed by the number of aerosol particles in the atmosphere, laying the foundation for so-called aerosol–cloud–climate interactions. In this study, a simple model to understand the effect of aerosol on cloud water is developed and applied.
Andrea Mosso, Thomas Hocking, and Thorsten Mauritsen
Atmos. Chem. Phys., 24, 12793–12806, https://doi.org/10.5194/acp-24-12793-2024, https://doi.org/10.5194/acp-24-12793-2024, 2024
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Clouds play a crucial role in the Earth's energy balance, as they can either warm up or cool down the area they cover depending on their height and depth. They are expected to alter their behaviour under climate change, affecting the warming generated by greenhouse gases. This paper proposes a new method to estimate their overall effect on this warming by simulating a climate where clouds are transparent. Results show that with the model used, clouds have a stabilising effect on climate.
Tao Shi, Yuanjian Yang, Ping Qi, and Simone Lolli
Atmos. Chem. Phys., 24, 12807–12822, https://doi.org/10.5194/acp-24-12807-2024, https://doi.org/10.5194/acp-24-12807-2024, 2024
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This paper explored the formation mechanisms of the amplified canopy urban heat island intensity (ΔCUHII) during heat wave (HW) periods in the megacity of Beijing from the perspectives of mountain–valley breeze and urban morphology. During the mountain breeze phase, high-rise buildings with lower sky view factors (SVFs) had a pronounced effect on the ΔCUHII. During the valley breeze phase, high-rise buildings exerted a dual influence on the ΔCUHII.
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Short summary
The development of China has caused rapid urbanization and severe air pollution. However, the extent of their individual and combined effects on fog is not well understood. Through numerical experiments, we find that urbanization suppresses low-level fog but probably promotes upper-level fog. Additional aerosols generally promote fog. Urbanization affects fog to a much larger extent than aerosols do.
The development of China has caused rapid urbanization and severe air pollution. However, the...
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