Articles | Volume 20, issue 24
https://doi.org/10.5194/acp-20-16007-2020
https://doi.org/10.5194/acp-20-16007-2020
Research article
 | 
22 Dec 2020
Research article |  | 22 Dec 2020

North Atlantic marine organic aerosol characterized by novel offline thermal desorption mass spectrometry: polysaccharides, recalcitrant material, and secondary organics

Michael J. Lawler, Savannah L. Lewis, Lynn M. Russell, Patricia K. Quinn, Timothy S. Bates, Derek J. Coffman, Lucia M. Upchurch, and Eric S. Saltzman

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Cited articles

Aller, J. Y., Radway, J. A. C., Kilthau, W. P., Bothe, D. W., Wilson, T. W., Vaillancourt, R. D., Quinn, P. K., Coffman, D. J., Murray, B. J., and Knopf, D. A.: Size-resolved characterization of the polysaccharidic and proteinaceous components of sea spray aerosol, Atmos. Environ., 154, 331–347, https://doi.org/10.1016/j.atmosenv.2017.01.053, 2017. 
ASDC: North Atlantic Aerosols and Marine Ecosystems Study, NASA Langley Research Center Atmospheric Science Data Center, https://doi.org/10.5067/Suborbital/NAAMES/DATA001, 2 June 2020. 
Ault, A. P., Moffet, R. C., Baltrusaitis, J., Collins, D. B., Ruppel, M. J., Cuadra-Rodriguez, L. A., Zhao, D., Guasco, T. L., Ebben, C. J., Geiger, F. M., Bertram, T. H., Prather, K. A., and Grassian, V. H.: Size-dependent changes in sea spray aerosol composition and properties with different seawater conditions, Environ. Sci. Technol., 47, 5603–5612, https://doi.org/10.1021/es400416g, 2013. 
Bates, T. S., Coffman, D. J., Covert, D. S., and Quinn, P. K.: Regional marine boundary layer aerosol size distributions in the Indian, Atlantic, and Pacific Oceans: A comparison of INDOEX measurements with ACE-1, ACE-2, and Aerosols99, J. Geophys. Res., 107, 8026, https://doi.org/10.1029/2001JD001174, 2002. 
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This work describes new measurements of aerosol (particles) composition over the North Atlantic Ocean. It provides concentrations of polysaccharide material likely made from organisms in the surface ocean and improves our understanding of the relative importance of such fresh biogenic material compared to more recalcitrant organic carbon in forming marine organic aerosol. We aim ultimately to understand the role that ocean biology plays in cloud formation in marine regions.
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