Articles | Volume 17, issue 15
https://doi.org/10.5194/acp-17-9585-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-9585-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
How do changes in warm-phase microphysics affect deep convective clouds?
Qian Chen
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
Key Laboratory of Meteorological Disaster, Ministry of Education (KLME); Joint International Research Laboratory of Climate and Environment Change (ILCEC); Collaborative Innovation Center on Forecast and Evaluation
of Meteorological Disasters; Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration; Nanjing University of Information Science and Technology, Nanjing, China
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
Orit Altaratz
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
Reuven H. Heiblum
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
Guy Dagan
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
Lital Pinto
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
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Shiye Huang, Jing Yang, Jiaojiao Li, Qian Chen, Qilin Zhang, and Fengxia Guo
Atmos. Chem. Phys., 25, 1831–1850, https://doi.org/10.5194/acp-25-1831-2025, https://doi.org/10.5194/acp-25-1831-2025, 2025
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Aerosol and secondary ice production are both vital to charge separation in thunderstorms, but the relative importance of different SIP processes to cloud electrification under different aerosol conditions is not well understood. In this study, we show in a clean environment, the shattering of freezing drops has the greatest effect on the charging rate, while in a polluted environment, both rime splintering and the shattering of freezing drops have a significant effect on cloud electrification.
Jing Yang, Jiaojiao Li, Meilian Chen, Xiaoqin Jing, Yan Yin, Bart Geerts, Zhien Wang, Yubao Liu, Baojun Chen, Shaofeng Hua, Hao Hu, Xiaobo Dong, Ping Tian, Qian Chen, and Yang Gao
Atmos. Chem. Phys., 24, 13833–13848, https://doi.org/10.5194/acp-24-13833-2024, https://doi.org/10.5194/acp-24-13833-2024, 2024
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Detecting unambiguous signatures is vital for examining cloud-seeding impacts, but often, seeding signatures are immersed in natural variability. In this study, reflectivity changes induced by glaciogenic seeding using different AgI concentrations are investigated under various conditions, and a method is developed to estimate the AgI concentration needed to detect unambiguous seeding signatures. The results aid in operational seeding-based decision-making regarding the amount of AgI dispersed.
Xin Zhang, Yan Yin, Ronald van der A, Jeff L. Lapierre, Qian Chen, Xiang Kuang, Shuqi Yan, Jinghua Chen, Chuan He, and Rulin Shi
Atmos. Meas. Tech., 13, 1709–1734, https://doi.org/10.5194/amt-13-1709-2020, https://doi.org/10.5194/amt-13-1709-2020, 2020
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Lightning NOx has a strong impact on ozone and the hydroxyl radical production. However, the production efficiency of lightning NOx is still quite uncertain. This work develops the algorithm of estimating lightning NOx for both clean and polluted regions and evaluates the sensitivity of estimates to the model setting of lightning NO. Results reveal that our method reduces the sensitivity to the background NO2 and includes much of the below-cloud LNO2.
Shiye Huang, Jing Yang, Jiaojiao Li, Qian Chen, Qilin Zhang, and Fengxia Guo
Atmos. Chem. Phys., 25, 1831–1850, https://doi.org/10.5194/acp-25-1831-2025, https://doi.org/10.5194/acp-25-1831-2025, 2025
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Aerosol and secondary ice production are both vital to charge separation in thunderstorms, but the relative importance of different SIP processes to cloud electrification under different aerosol conditions is not well understood. In this study, we show in a clean environment, the shattering of freezing drops has the greatest effect on the charging rate, while in a polluted environment, both rime splintering and the shattering of freezing drops have a significant effect on cloud electrification.
Jing Yang, Jiaojiao Li, Meilian Chen, Xiaoqin Jing, Yan Yin, Bart Geerts, Zhien Wang, Yubao Liu, Baojun Chen, Shaofeng Hua, Hao Hu, Xiaobo Dong, Ping Tian, Qian Chen, and Yang Gao
Atmos. Chem. Phys., 24, 13833–13848, https://doi.org/10.5194/acp-24-13833-2024, https://doi.org/10.5194/acp-24-13833-2024, 2024
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Detecting unambiguous signatures is vital for examining cloud-seeding impacts, but often, seeding signatures are immersed in natural variability. In this study, reflectivity changes induced by glaciogenic seeding using different AgI concentrations are investigated under various conditions, and a method is developed to estimate the AgI concentration needed to detect unambiguous seeding signatures. The results aid in operational seeding-based decision-making regarding the amount of AgI dispersed.
Suf Lorian and Guy Dagan
Atmos. Chem. Phys., 24, 9323–9338, https://doi.org/10.5194/acp-24-9323-2024, https://doi.org/10.5194/acp-24-9323-2024, 2024
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We examine the combined effect of aerosols and sea surface temperature (SST) on clouds under equilibrium conditions in cloud-resolving radiative–convective equilibrium simulations. We demonstrate that the aerosol–cloud interaction's effect on top-of-atmosphere energy gain strongly depends on the underlying SST, while the shortwave part of the spectrum is significantly more sensitive to SST. Furthermore, increasing aerosols influences upper-troposphere stability and thus anvil cloud fraction.
Manuel Santos Gutiérrez, Mickaël David Chekroun, and Ilan Koren
EGUsphere, https://doi.org/https://doi.org/10.48550/arXiv.2405.11545, https://doi.org/https://doi.org/10.48550/arXiv.2405.11545, 2024
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This letter explores a novel approach for the formation of cloud droplets in rising adiabatic air parcels. Our approach combines microphysical equations accounting for moisture, updrafts and concentration of aerosols. Our analysis reveals three regimes: A) Low moisture and high concentration can hinder activation; B) Droplets can activate and stabilize above critical sizes, and C) sparse clouds can have droplets exhibiting activation and deactivation cycles.
Huan Liu, Ilan Koren, Orit Altaratz, and Mickaël D. Chekroun
Atmos. Chem. Phys., 23, 6559–6569, https://doi.org/10.5194/acp-23-6559-2023, https://doi.org/10.5194/acp-23-6559-2023, 2023
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Clouds' responses to global warming contribute the largest uncertainty in climate prediction. Here, we analyze 42 years of global cloud cover in reanalysis data and show a decreasing trend over most continents and an increasing trend over the tropical and subtropical oceans. A reduction in near-surface relative humidity can explain the decreasing trend in cloud cover over land. Our results suggest potential stress on the terrestrial water cycle, associated with global warming.
Elisa T. Sena, Ilan Koren, Orit Altaratz, and Alexander B. Kostinski
Atmos. Chem. Phys., 22, 16111–16122, https://doi.org/10.5194/acp-22-16111-2022, https://doi.org/10.5194/acp-22-16111-2022, 2022
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We used record-breaking statistics together with spatial information to create record-breaking SST maps. The maps reveal warming patterns in the overwhelming majority of the ocean and coherent islands of cooling, where low records occur more frequently than high ones. Some of these cooling spots are well known; however, a surprising elliptical area in the Southern Ocean is observed as well. Similar analyses can be performed on other key climatological variables to explore their trend patterns.
Guy Dagan
Atmos. Chem. Phys., 22, 15767–15775, https://doi.org/10.5194/acp-22-15767-2022, https://doi.org/10.5194/acp-22-15767-2022, 2022
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Using idealized simulations we demonstrate that the equilibrium climate sensitivity (ECS), i.e. the increase in surface temperature under equilibrium conditions due to doubling of the CO2 concentration, increases with the aerosol concentration. The ECS increase is explained by a faster increase in precipitation efficiency with warming under high aerosol concentrations, which more efficiently depletes the water from the cloud and thus is manifested as an increase in the cloud feedback parameter.
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
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Trace gases and aerosols (tiny airborne particles) are released from a variety of point sources around the globe. Examples include volcanoes, industrial chimneys, forest fires, and ship stacks. These sources provide opportunistic experiments with which to quantify the role of aerosols in modifying cloud properties. We review the current state of understanding on the influence of aerosol on climate built from the wide range of natural and anthropogenic laboratories investigated in recent decades.
Eshkol Eytan, Ilan Koren, Orit Altaratz, Mark Pinsky, and Alexander Khain
Atmos. Chem. Phys., 21, 16203–16217, https://doi.org/10.5194/acp-21-16203-2021, https://doi.org/10.5194/acp-21-16203-2021, 2021
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Describing cloud mixing processes is among the most challenging fronts in cloud physics. Therefore, the adiabatic fraction (AF) that serves as a mixing measure is a valuable metric. We use high-resolution (10 m) simulations of single clouds with a passive tracer to test the skill of different methods used to derive AF. We highlight a method that is insensitive to the available cloud samples and allows considering microphysical effects on AF estimations in different environmental conditions.
Tom Dror, Mickaël D. Chekroun, Orit Altaratz, and Ilan Koren
Atmos. Chem. Phys., 21, 12261–12272, https://doi.org/10.5194/acp-21-12261-2021, https://doi.org/10.5194/acp-21-12261-2021, 2021
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A part of continental shallow convective cumulus (Cu) was shown to share properties such as organization and formation over vegetated areas, thus named green Cu. Mechanisms behind the formed patterns are not understood. We use different metrics and an empirical orthogonal function (EOF) to decompose the dataset and quantify organization factors (cloud streets and gravity waves). We show that clouds form a highly organized grid structure over hundreds of kilometers at the field lifetime.
Tom Dror, J. Michel Flores, Orit Altaratz, Guy Dagan, Zev Levin, Assaf Vardi, and Ilan Koren
Atmos. Chem. Phys., 20, 15297–15306, https://doi.org/10.5194/acp-20-15297-2020, https://doi.org/10.5194/acp-20-15297-2020, 2020
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We used in situ aerosol measurements over the Atlantic, Caribbean, and Pacific to initialize a cloud model and study the impact of aerosol concentration and sizes on warm clouds. We show that high aerosol concentration increases cloud mass and reduces surface rain when giant particles (diameter > 9 µm) are present. The large aerosols changed the timing and magnitude of internal cloud processes and resulted in an enhanced evaporation below cloud base and dramatically reduced surface rain.
Guy Dagan and Philip Stier
Atmos. Chem. Phys., 20, 6291–6303, https://doi.org/10.5194/acp-20-6291-2020, https://doi.org/10.5194/acp-20-6291-2020, 2020
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Ensemble daily simulations for two separate month-long periods over a region near Barbados were conducted to investigate aerosol effects on cloud properties and the atmospheric energy budget. For each day, two simulations were conducted with low and high cloud droplet number concentrations representing clean and polluted conditions, respectively. These simulations are used to distinguish between properties that are robustly affected by changes in aerosol concentrations and those that are not.
Guy Dagan, Philip Stier, Matthew Christensen, Guido Cioni, Daniel Klocke, and Axel Seifert
Atmos. Chem. Phys., 20, 4523–4544, https://doi.org/10.5194/acp-20-4523-2020, https://doi.org/10.5194/acp-20-4523-2020, 2020
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In order to better understand the physical processes behind aerosol effects on the atmospheric energy budget, we analyse numerical simulations of tropical cloud systems. Two sets of simulations, at different dates during the NARVAL 2 field campaign, are simulated with different dominant cloud modes. Our results demonstrate that under different environmental conditions, the response of the atmospheric energy budget to aerosol perturbation could be different.
Xin Zhang, Yan Yin, Ronald van der A, Jeff L. Lapierre, Qian Chen, Xiang Kuang, Shuqi Yan, Jinghua Chen, Chuan He, and Rulin Shi
Atmos. Meas. Tech., 13, 1709–1734, https://doi.org/10.5194/amt-13-1709-2020, https://doi.org/10.5194/amt-13-1709-2020, 2020
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Lightning NOx has a strong impact on ozone and the hydroxyl radical production. However, the production efficiency of lightning NOx is still quite uncertain. This work develops the algorithm of estimating lightning NOx for both clean and polluted regions and evaluates the sensitivity of estimates to the model setting of lightning NO. Results reveal that our method reduces the sensitivity to the background NO2 and includes much of the below-cloud LNO2.
George Spill, Philip Stier, Paul R. Field, and Guy Dagan
Atmos. Chem. Phys., 19, 13507–13517, https://doi.org/10.5194/acp-19-13507-2019, https://doi.org/10.5194/acp-19-13507-2019, 2019
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Shallow convective clouds are among the most common and least understood clouds in the atmosphere. Here we present simulations of realistic, shallow cloud fields in a large domain, in contrast to typical idealised simulations, and find that in these simulations the response to aerosol perturbations is different.
Reuven H. Heiblum, Lital Pinto, Orit Altaratz, Guy Dagan, and Ilan Koren
Atmos. Chem. Phys., 19, 10717–10738, https://doi.org/10.5194/acp-19-10717-2019, https://doi.org/10.5194/acp-19-10717-2019, 2019
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It is useful to divide a cloud into two regions: core and margin. Three parameters used to define a core are compared: buoyancy (B), relative humidity (RH), and vertical velocity (W). Using theoretical arguments and simulations, we show that during most of a cloud's lifetime, the cores are subsets of one another: Bcore ⊆ RHcore ⊆ Wcore. Moreover, the core–shell cloud model applies to all core definitions. Our findings can serve as a benchmark in the partition the core and margin.
Reuven H. Heiblum, Lital Pinto, Orit Altaratz, Guy Dagan, and Ilan Koren
Atmos. Chem. Phys., 19, 10739–10755, https://doi.org/10.5194/acp-19-10739-2019, https://doi.org/10.5194/acp-19-10739-2019, 2019
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The effects of aerosol concentration on a cloud's partition to core and margin are examined. The main finding from Part I (i.e. Bcore ⊆ RHcore ⊆ Wcore) is seen for all aerosol concentrations. Clouds can produce positive buoyancy due to both saturated updrafts or unsaturated downdrafts; the latter are dependent on low aerosol concentrations. We show that a cloud's mass is mainly dependent on core processes (condensation), while its volume is mainly dependent on margin processes (evaporation).
Guy Dagan, Ilan Koren, and Orit Altaratz
Atmos. Chem. Phys., 18, 6761–6769, https://doi.org/10.5194/acp-18-6761-2018, https://doi.org/10.5194/acp-18-6761-2018, 2018
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In this paper we distill the problem of aerosol–cloud interactions to an interplay between the system's two characteristic vertical velocities, i.e., the air vertical velocity and the collective droplets fall velocity. We show using theoretical considerations and cloud-resolving models that the relations between the two velocities are extremely sensitive to the cloud field's thermodynamics and microphysical properties.
Yevgeny Derimian, Marie Choël, Yinon Rudich, Karine Deboudt, Oleg Dubovik, Alexander Laskin, Michel Legrand, Bahaiddin Damiri, Ilan Koren, Florin Unga, Myriam Moreau, Meinrat O. Andreae, and Arnon Karnieli
Atmos. Chem. Phys., 17, 11331–11353, https://doi.org/10.5194/acp-17-11331-2017, https://doi.org/10.5194/acp-17-11331-2017, 2017
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We present influence of daily occurrence of the sea breeze flow from the Mediterranean Sea on physicochemical and optical properties of atmospheric aerosol deep inland in the Negev Desert of Israel. Sampled airborne dust was found be internally mixed with sea-salt particles and reacted with anthropogenic pollution, which makes the dust highly hygroscopic and a liquid coating of particles appears. These physicochemical transformations are associated with a change in aerosol radiative properties.
Guy Dagan, Ilan Koren, Orit Altaratz, and Reuven H. Heiblum
Atmos. Chem. Phys., 17, 7435–7444, https://doi.org/10.5194/acp-17-7435-2017, https://doi.org/10.5194/acp-17-7435-2017, 2017
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Large eddy simulations with bin microphysics are used to study cloud fields' sensitivity to changes in aerosol loading and the time evolution of this response. We show that the mean field properties change with a non-monotonic trend, with an optimum aerosol concentration for which the field reaches its maximal water mass or rain yield. The evolution of the mean thermodynamic properties is studied and shown to cause the migration of the optimal aerosol concentration toward higher values.
Yaniv Tubul, Ilan Koren, Orit Altaratz, and Reuven H. Heiblum
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2017-121, https://doi.org/10.5194/amt-2017-121, 2017
Revised manuscript not accepted
Chandan Sarangi, Sachchida Nand Tripathi, Vijay P. Kanawade, Ilan Koren, and D. Sivanand Pai
Atmos. Chem. Phys., 17, 5185–5204, https://doi.org/10.5194/acp-17-5185-2017, https://doi.org/10.5194/acp-17-5185-2017, 2017
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Aerosol-induced perturbations in cloud systems and rainfall are very uncertain. This study provides observational evidence of a robust positive association between aerosol–cloud–rainfall properties over the Indian summer monsoon region. Observed and modeled aerosol–cloud microphysical changes illustrate that cloud invigoration under a high AOD scenario can explain most of the aerosol-associated changes in cloud fraction, cloud top pressure, and surface rainfall over this region.
Y. Tubul, I. Koren, and O. Altaratz
Earth Syst. Dynam., 6, 781–788, https://doi.org/10.5194/esd-6-781-2015, https://doi.org/10.5194/esd-6-781-2015, 2015
Y. Ben Ami, O. Altaratz, Y. Yair, and I. Koren
Nat. Hazards Earth Syst. Sci., 15, 2449–2459, https://doi.org/10.5194/nhess-15-2449-2015, https://doi.org/10.5194/nhess-15-2449-2015, 2015
S. Fuzzi, U. Baltensperger, K. Carslaw, S. Decesari, H. Denier van der Gon, M. C. Facchini, D. Fowler, I. Koren, B. Langford, U. Lohmann, E. Nemitz, S. Pandis, I. Riipinen, Y. Rudich, M. Schaap, J. G. Slowik, D. V. Spracklen, E. Vignati, M. Wild, M. Williams, and S. Gilardoni
Atmos. Chem. Phys., 15, 8217–8299, https://doi.org/10.5194/acp-15-8217-2015, https://doi.org/10.5194/acp-15-8217-2015, 2015
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Particulate matter (PM) constitutes one of the most challenging problems both for air quality and climate change policies. This paper reviews the most recent scientific results on the issue and the policy needs that have driven much of the increase in monitoring and mechanistic research over the last 2 decades. The synthesis reveals many new processes and developments in the science underpinning climate-PM interactions and the effects of PM on human health and the environment.
G. Feingold, I. Koren, T. Yamaguchi, and J. Kazil
Atmos. Chem. Phys., 15, 7351–7367, https://doi.org/10.5194/acp-15-7351-2015, https://doi.org/10.5194/acp-15-7351-2015, 2015
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Most research on the relationship between aerosol and closed/open cell transitions tends to focus on the closed to open transition. Here we address the two-way transition between closed and open cellular states using a cloud resolving model. We find inherent asymmetry in the transitions and explain the source of the asymmetry. Results are supported by a dynamical system analogue to the full system.
G. Dagan, I. Koren, and O. Altaratz
Atmos. Chem. Phys., 15, 2749–2760, https://doi.org/10.5194/acp-15-2749-2015, https://doi.org/10.5194/acp-15-2749-2015, 2015
E. Tas, A. Teller, O. Altaratz, D. Axisa, R. Bruintjes, Z. Levin, and I. Koren
Atmos. Chem. Phys., 15, 2009–2017, https://doi.org/10.5194/acp-15-2009-2015, https://doi.org/10.5194/acp-15-2009-2015, 2015
G. Snider, C. L. Weagle, R. V. Martin, A. van Donkelaar, K. Conrad, D. Cunningham, C. Gordon, M. Zwicker, C. Akoshile, P. Artaxo, N. X. Anh, J. Brook, J. Dong, R. M. Garland, R. Greenwald, D. Griffith, K. He, B. N. Holben, R. Kahn, I. Koren, N. Lagrosas, P. Lestari, Z. Ma, J. Vanderlei Martins, E. J. Quel, Y. Rudich, A. Salam, S. N. Tripathi, C. Yu, Q. Zhang, Y. Zhang, M. Brauer, A. Cohen, M. D. Gibson, and Y. Liu
Atmos. Meas. Tech., 8, 505–521, https://doi.org/10.5194/amt-8-505-2015, https://doi.org/10.5194/amt-8-505-2015, 2015
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We have initiated a global network of ground-level monitoring stations to measure concentrations of fine aerosols in urban environments. Our findings include major ions species, total mass, and total scatter at three wavelengths. Results will be used to further evaluate and enhance satellite remote sensing estimates.
E. Hirsch, I. Koren, Z. Levin, O. Altaratz, and E. Agassi
Atmos. Chem. Phys., 14, 9001–9012, https://doi.org/10.5194/acp-14-9001-2014, https://doi.org/10.5194/acp-14-9001-2014, 2014
A. K. Mishra, K. Klingmueller, E. Fredj, J. Lelieveld, Y. Rudich, and I. Koren
Atmos. Chem. Phys., 14, 7213–7231, https://doi.org/10.5194/acp-14-7213-2014, https://doi.org/10.5194/acp-14-7213-2014, 2014
R. H. Heiblum, I. Koren, and G. Feingold
Atmos. Chem. Phys., 14, 6063–6074, https://doi.org/10.5194/acp-14-6063-2014, https://doi.org/10.5194/acp-14-6063-2014, 2014
G. Feingold and I. Koren
Nonlin. Processes Geophys., 20, 1011–1021, https://doi.org/10.5194/npg-20-1011-2013, https://doi.org/10.5194/npg-20-1011-2013, 2013
E. Hirsch, I. Koren, O. Altaratz, Z. Levin, and E. Agassi
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-28729-2013, https://doi.org/10.5194/acpd-13-28729-2013, 2013
Revised manuscript not accepted
Related subject area
Subject: Clouds and Precipitation | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Counteracting influences of gravitational settling modulate aerosol impacts on cloud-base-lowering fog characteristics
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Investigating ice formation pathways using a novel two-moment multi-class cloud microphysics scheme
Microphysics regimes due to haze–cloud interactions: cloud oscillation and cloud collapse
Impact of secondary ice production on thunderstorm electrification under different aerosol conditions
Accelerated impact of airborne glaciogenic seeding of stratiform clouds by turbulence
Model analysis of biases in the satellite-diagnosed aerosol effect on the cloud liquid water path
Evaluation of biases in mid-to-high-latitude surface snowfall and cloud phase in ERA5 and CMIP6 using satellite observations
Failed cyclogenesis of a mesoscale convective system near Cape Verde: The role of the Saharan trade wind layer among other inhibiting factors observed during the CADDIWA field campaign
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Role of a key microphysical factor in mixed-phase stratocumulus clouds and their interactions with aerosols
High-resolution modelling of early contrail evolution from hydrogen-powered aircraft
Investigating the impact of subgrid-scale aerosol-cloud interaction on mesoscale meteorology prediction
Correction of ERA5 temperature and relative humidity biases by bivariate quantile mapping for contrail formation analysis
Can pollen affect precipitation?
Potential impacts of marine fuel regulations on an Arctic stratocumulus case and its radiative response
The impact of the mesh size and microphysics scheme on the representation of mid-level clouds in the ICON model in hilly and complex terrain
The role of ascent timescales for warm conveyor belt (WCB) moisture transport into the upper troposphere and lower stratosphere (UTLS)
Magnitude and timescale of liquid water path adjustments to cloud droplet number concentration perturbations for nocturnal non-precipitating marine stratocumulus
On the Processes Determining the Slope of Cloud-Water Adjustments in Non-Precipitating Stratocumulus
Estimating the concentration of silver iodide needed to detect unambiguous signatures of glaciogenic cloud seeding
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Ice-nucleating particle concentration impacts cloud properties over Dronning Maud Land, East Antarctica, in COSMO-CLM2
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Diurnal variation in an amplified canopy urban heat island during heat wave periods in the megacity of Beijing: roles of mountain–valley breeze and urban morphology
Diurnal evolution of non-precipitating marine stratocumuli in a large-eddy simulation ensemble
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Nathan H. Pope and Adele L. Igel
Atmos. Chem. Phys., 25, 5433–5444, https://doi.org/10.5194/acp-25-5433-2025, https://doi.org/10.5194/acp-25-5433-2025, 2025
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We used an atmospheric model that simulates a single column to study the sensitivity of marine fog formed through the lowering of the base of a stratus cloud to meteorology and aerosols. We found that higher aerosol concentration reduces the likelihood and duration of fog but leads to denser fog. This overall trend was caused by multiple physical mechanisms depending on conditions.
Jung-Sub Lim, Yign Noh, Hyunho Lee, and Fabian Hoffmann
Atmos. Chem. Phys., 25, 5313–5329, https://doi.org/10.5194/acp-25-5313-2025, https://doi.org/10.5194/acp-25-5313-2025, 2025
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Rain formation in warm clouds begins when small droplets collide, but this process can be slow without larger droplets. We used simulations to explore the role of bigger droplets, known as precipitation embryos, in triggering rain. We found that they speed up rain only when their size and number exceed a critical threshold. This threshold becomes larger when collisions are naturally efficient, such as in clouds with broad droplet size distributions or strong turbulence.
Je-Yun Chun, Robert Wood, Peter N. Blossey, and Sarah J. Doherty
Atmos. Chem. Phys., 25, 5251–5271, https://doi.org/10.5194/acp-25-5251-2025, https://doi.org/10.5194/acp-25-5251-2025, 2025
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This study explores how aerosols affect clouds transitioning from stratocumulus to cumulus along trade winds under varying atmospheric conditions. We found that aerosols typically reduce precipitation and raise cloud height, but their impact changes when subsidence changes by aerosol enhancement are considered. Our findings indicate that the cooling effect of aerosols might be overestimated if these atmospheric changes are not accounted for.
Wojciech W. Grabowski and Hanna Pawlowska
Atmos. Chem. Phys., 25, 5273–5285, https://doi.org/10.5194/acp-25-5273-2025, https://doi.org/10.5194/acp-25-5273-2025, 2025
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A simple diagram to depict cloud droplets' formation via the activation of cloud condensation nuclei (CCN) as well as their subsequent growth and evaporation is presented.
Albert Ansmann, Cristofer Jimenez, Daniel A. Knopf, Johanna Roschke, Johannes Bühl, Kevin Ohneiser, and Ronny Engelmann
Atmos. Chem. Phys., 25, 4867–4884, https://doi.org/10.5194/acp-25-4867-2025, https://doi.org/10.5194/acp-25-4867-2025, 2025
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In this study, we focus on the potential impact of wildfire smoke on cirrus formation. Aerosol and cirrus observations with lidar and radar during the MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition, presented in the companion paper (Ansmann et al., 2025), are closely linked to comprehensive modeling of ice nucleation in cirrus evolution processes, presented in this article. A clear impact of wildfire smoke on cirrus formation was found.
August Mikkelsen, Daniel T. McCoy, Trude Eidhammer, Andrew Gettelman, Ci Song, Hamish Gordon, and Isabel L. McCoy
Atmos. Chem. Phys., 25, 4547–4570, https://doi.org/10.5194/acp-25-4547-2025, https://doi.org/10.5194/acp-25-4547-2025, 2025
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Whether increased aerosol increases or decreases liquid cloud mass has been a longstanding question. Observed correlations suggest that aerosols thin liquid cloud, but we are able to show that observations were consistent with an increase in liquid cloud in response to aerosols by leveraging a model where causality could be traced.
Tim Lüttmer, Peter Spichtinger, and Axel Seifert
Atmos. Chem. Phys., 25, 4505–4529, https://doi.org/10.5194/acp-25-4505-2025, https://doi.org/10.5194/acp-25-4505-2025, 2025
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We investigate ice formation pathways in idealized convective clouds using a novel microphysics scheme that distinguishes between five ice classes each with their own unique formation mechanism. Ice crystals from rime splintering form the lowermost layer of ice crystals around the updraft core. The majority of ice crystals in the anvil of the convective cloud stems from frozen droplets. Ice stemming from homogeneous and deposition nucleation was only relevant in the overshoot.
Fan Yang, Hamed Fahandezh Sadi, Raymond A. Shaw, Fabian Hoffmann, Pei Hou, Aaron Wang, and Mikhail Ovchinnikov
Atmos. Chem. Phys., 25, 3785–3806, https://doi.org/10.5194/acp-25-3785-2025, https://doi.org/10.5194/acp-25-3785-2025, 2025
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Large-eddy simulations of a convection cloud chamber show two new microphysics regimes, cloud oscillation and cloud collapse, due to haze–cloud interactions. Our results suggest that haze particles and their interactions with cloud droplets should be considered especially in polluted conditions. To properly simulate haze–cloud interactions, we need to resolve droplet activation and deactivation processes, instead of using Twomey-type activation parameterization.
Shiye Huang, Jing Yang, Jiaojiao Li, Qian Chen, Qilin Zhang, and Fengxia Guo
Atmos. Chem. Phys., 25, 1831–1850, https://doi.org/10.5194/acp-25-1831-2025, https://doi.org/10.5194/acp-25-1831-2025, 2025
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Aerosol and secondary ice production are both vital to charge separation in thunderstorms, but the relative importance of different SIP processes to cloud electrification under different aerosol conditions is not well understood. In this study, we show in a clean environment, the shattering of freezing drops has the greatest effect on the charging rate, while in a polluted environment, both rime splintering and the shattering of freezing drops have a significant effect on cloud electrification.
Meilian Chen, Xiaoqin Jing, Jiaojiao Li, Jing Yang, Xiaobo Dong, Bart Geerts, Yan Yin, Baojun Chen, Lulin Xue, Mengyu Huang, Ping Tian, and Shaofeng Hua
EGUsphere, https://doi.org/10.5194/egusphere-2025-47, https://doi.org/10.5194/egusphere-2025-47, 2025
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Several recent studies have reported complete cloud glaciation induced by airborne-based glaciogenic cloud seeding over plains. Since turbulence is an important factor to maintain clouds in mixed-phase, it is hypothesized that turbulence may have an impact on the seeding effect. This hypothesis is evident in the present study, which shows turbulence can accelerate the impact of airborne glaciogenic seeding of stratiform clouds.
Harri Kokkola, Juha Tonttila, Silvia M. Calderón, Sami Romakkaniemi, Antti Lipponen, Aapo Peräkorpi, Tero Mielonen, Edward Gryspeerdt, Timo Henrik Virtanen, Pekka Kolmonen, and Antti Arola
Atmos. Chem. Phys., 25, 1533–1543, https://doi.org/10.5194/acp-25-1533-2025, https://doi.org/10.5194/acp-25-1533-2025, 2025
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Understanding how atmospheric aerosols affect clouds is a scientific challenge. One question is how aerosols affects the amount of cloud water. We used a cloud-scale model to study these effects on marine clouds. The study showed that variations in cloud properties and instrument noise can cause bias in satellite-derived cloud water content. However, our results suggest that for similar weather conditions with well-defined aerosol concentrations, satellite data can reliably track these effects.
Franziska Hellmuth, Tim Carlsen, Anne Sophie Daloz, Robert Oscar David, Haochi Che, and Trude Storelvmo
Atmos. Chem. Phys., 25, 1353–1383, https://doi.org/10.5194/acp-25-1353-2025, https://doi.org/10.5194/acp-25-1353-2025, 2025
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This article compares the occurrence of supercooled liquid-containing clouds (sLCCs) and their link to surface snowfall in CloudSat–CALIPSO, ERA5, and the CMIP6 models. Significant discrepancies were found, with ERA5 and CMIP6 consistently overestimating sLCC and snowfall frequency. This bias is likely due to cloud microphysics parameterization. This conclusion has implications for accurately representing cloud phase and snowfall in future climate projections.
Guillaume Feger, Jean-Pierre Chaboureau, Thibaut Dauhut, Julien Delanoë, and Pierre Coutris
EGUsphere, https://doi.org/10.5194/egusphere-2025-105, https://doi.org/10.5194/egusphere-2025-105, 2025
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The Saharan air at trade wind layer, cold pools, and upper tropospheric dry air are identified as the three main factors inhibiting the cyclogenesis of the Pierre Henri mesoscale convective system. The findings were obtained trough observations made during two flights of the CADDIWA campaign and a convection-permitting simulation run with the Meso-NH model. They provide new insights into the complex dynamics of cyclogenesis in the Cape Verde region and challenge the existing model of the SAL.
Claudia Christine Stephan and Bjorn Stevens
Atmos. Chem. Phys., 25, 1209–1226, https://doi.org/10.5194/acp-25-1209-2025, https://doi.org/10.5194/acp-25-1209-2025, 2025
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Tropical precipitation cluster area and intensity distributions follow power laws, but the physical processes responsible for this behavior remain unknown. We analyze global simulations that realistically represent precipitation processes. We consider Earth-like planets as well as virtual planets to realize different types of large-scale dynamics. Our finding is that power laws in Earth’s precipitation cluster statistics stem from the robust power laws in Earth’s atmospheric wind field.
Tim Lüttmer, Annette Miltenberger, and Peter Spichtinger
EGUsphere, https://doi.org/10.5194/egusphere-2025-185, https://doi.org/10.5194/egusphere-2025-185, 2025
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We investigate ice formation pathways in a warm conveyor belt case study. We employ a multi-phase microphysics scheme that distinguishes between ice from different nucleation processes. Ice crystals in the cirrus outflow mostly stem from in-situ formation. Hence they were formed directly from the vapor phase. Sedimentational redistribution modulates cirrus properties and leads to a disagreement between cirrus origin classifications based on thermodynamic history and nucleation processes.
Seoung Soo Lee, Chang Hoon Jung, Jinho Choi, Young Jun Yoon, Junshik Um, Youtong Zheng, Jianping Guo, Manguttathil G. Manoj, Sang-Keun Song, and Kyung-Ja Ha
Atmos. Chem. Phys., 25, 705–726, https://doi.org/10.5194/acp-25-705-2025, https://doi.org/10.5194/acp-25-705-2025, 2025
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This study attempts to test a general factor that explains differences in the properties of different mixed-phase clouds using a modeling tool. Although this attempt is not to identify a factor that can perfectly explain and represent the properties of different mixed-phase clouds, we believe that this attempt acts as a valuable stepping stone towards a more complete, general way of using climate models to better predict climate change.
Annemarie Lottermoser and Simon Unterstraßer
EGUsphere, https://doi.org/10.5194/egusphere-2024-3859, https://doi.org/10.5194/egusphere-2024-3859, 2025
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Contrail-cirrus significantly contributes to aviation's overall climate impact. As hydrogen combustion and fuel cell use are emerging technologies for aircraft propulsion, we simulated individual contrails from hydrogen propulsion during the first six minutes after exhaust emission, termed the vortex phase. The ice crystal loss during that stage is crucial as the number of ice crystals has a large impact on the further evolution of contrails into contrail-cirrus and their radiative forcing.
Wenjie Zhang, Hong Wang, Xiaoye Zhang, Yue Peng, Zhaodong Liu, Deying Wang, Da Zhang, Chen Han, Yang Zhao, Junting Zhong, Wenxing Jia, Huiqiong Ning, and Huizheng Che
EGUsphere, https://doi.org/10.5194/egusphere-2024-3677, https://doi.org/10.5194/egusphere-2024-3677, 2025
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We implement a real-time subgrid-scale aerosol-cloud interaction (ACI) mechanism in a mesoscale atmospheric chemistry system and find that subgrid-scale ACI can improve meteorological factors predictions. This study demonstrates the importance of real-time subgrid-scale ACI to weather forecast and the necessity of multiscale ACI studies.
Kevin Wolf, Nicolas Bellouin, Olivier Boucher, Susanne Rohs, and Yun Li
Atmos. Chem. Phys., 25, 157–181, https://doi.org/10.5194/acp-25-157-2025, https://doi.org/10.5194/acp-25-157-2025, 2025
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ERA5 atmospheric reanalysis and airborne in situ observations from IAGOS are compared in terms of the representation of the contrail formation potential and the presence of supersaturation. Differences are traced back to biases in ERA5 relative humidity fields. Those biases are addressed by applying a quantile mapping technique that significantly improved contrail estimation based on post-processed ERA5 data.
Marje Prank, Juha Tonttila, Xiaoxia Shang, Sami Romakkaniemi, and Tomi Raatikainen
Atmos. Chem. Phys., 25, 183–197, https://doi.org/10.5194/acp-25-183-2025, https://doi.org/10.5194/acp-25-183-2025, 2025
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Large primary bioparticles such as pollen can be abundant in the atmosphere. In humid conditions pollen can rupture and release a large number of fine sub-pollen particles (SPPs). The paper investigates what kind of birch pollen concentrations are needed for the pollen and SPPs to start playing a noticeable role in cloud processes and alter precipitation formation. In the studied cases only the largest observed pollen concentrations were able to noticeably alter the precipitation formation.
Luís Filipe Escusa dos Santos, Hannah C. Frostenberg, Alejandro Baró Pérez, Annica M. L. Ekman, Luisa Ickes, and Erik S. Thomson
Atmos. Chem. Phys., 25, 119–142, https://doi.org/10.5194/acp-25-119-2025, https://doi.org/10.5194/acp-25-119-2025, 2025
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The Arctic is experiencing enhanced surface warming. The observed decline in Arctic sea-ice extent is projected to lead to an increase in Arctic shipping activity, which may lead to further climatic feedbacks. Using an atmospheric model and results from marine engine experiments that focused on fuel sulfur content reduction and exhaust wet scrubbing, we investigate how ship exhaust particles influence the properties of Arctic clouds. Implications for radiative surface processes are discussed.
Nadja Omanovic, Brigitta Goger, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 14145–14175, https://doi.org/10.5194/acp-24-14145-2024, https://doi.org/10.5194/acp-24-14145-2024, 2024
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We evaluated the numerical weather model ICON in two horizontal resolutions with two bulk microphysics schemes over hilly and complex terrain in Switzerland and Austria, respectively. We focused on the model's ability to simulate mid-level clouds in summer and winter. By combining observational data from two different field campaigns, we show that an increase in the horizontal resolution and a more advanced cloud microphysics scheme is strongly beneficial for cloud representation.
Cornelis Schwenk and Annette Miltenberger
Atmos. Chem. Phys., 24, 14073–14099, https://doi.org/10.5194/acp-24-14073-2024, https://doi.org/10.5194/acp-24-14073-2024, 2024
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Warm conveyor belts (WCBs) transport moisture into the upper atmosphere, where it acts as a greenhouse gas. This transport is not well understood, and the role of rapidly rising air is unclear. We simulate a WCB and look at fast- and slow-rising air to see how moisture is (differently) transported. We find that for fast-ascending air more ice particles reach higher into the atmosphere and that frozen cloud particles are removed differently than during slow ascent, which has more water vapour.
Yao-Sheng Chen, Prasanth Prabhakaran, Fabian Hoffmann, Jan Kazil, Takanobu Yamaguchi, and Graham Feingold
EGUsphere, https://doi.org/10.5194/egusphere-2024-3891, https://doi.org/10.5194/egusphere-2024-3891, 2024
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Injecting sea salt aerosols into marine stratiform clouds can distribute the cloud water over more droplets in smaller sizes. This process is expected to make the clouds brighter, allowing them to reflect more sunlight back to space. However, it may also cause the clouds to lose water over time, reducing their ability to reflect sunlight. We use a computer model to show that the loss of cloud water occurs relatively quickly and does not completely offset the initial brightening.
Fabian Hoffmann, Yao-Sheng Chen, and Graham Feingold
EGUsphere, https://doi.org/10.5194/egusphere-2024-3893, https://doi.org/10.5194/egusphere-2024-3893, 2024
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Clouds reflect a substantial portion of the incoming solar radiation back into space. This capacity is determined by the number of cloud droplets, which in turn is influenced by the number of aerosol particles, forming the basis for aerosol-cloud-climate interactions. In this study, we use a simple mixed-layer approach to understand the effect of aerosol on cloud water in non-precipitating stratocumulus.
Jing Yang, Jiaojiao Li, Meilian Chen, Xiaoqin Jing, Yan Yin, Bart Geerts, Zhien Wang, Yubao Liu, Baojun Chen, Shaofeng Hua, Hao Hu, Xiaobo Dong, Ping Tian, Qian Chen, and Yang Gao
Atmos. Chem. Phys., 24, 13833–13848, https://doi.org/10.5194/acp-24-13833-2024, https://doi.org/10.5194/acp-24-13833-2024, 2024
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Detecting unambiguous signatures is vital for examining cloud-seeding impacts, but often, seeding signatures are immersed in natural variability. In this study, reflectivity changes induced by glaciogenic seeding using different AgI concentrations are investigated under various conditions, and a method is developed to estimate the AgI concentration needed to detect unambiguous seeding signatures. The results aid in operational seeding-based decision-making regarding the amount of AgI dispersed.
Konstantinos Kourtidis, Stavros Stathopoulos, and Vassilis Amiridis
EGUsphere, https://doi.org/10.5194/egusphere-2024-3314, https://doi.org/10.5194/egusphere-2024-3314, 2024
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The loud sound of thunder will induce mechanical effects on cloud droplets and ice particles, causing changes in their size distribution.
Florian Sauerland, Niels Souverijns, Anna Possner, Heike Wex, Preben Van Overmeiren, Alexander Mangold, Kwinten Van Weverberg, and Nicole van Lipzig
Atmos. Chem. Phys., 24, 13751–13768, https://doi.org/10.5194/acp-24-13751-2024, https://doi.org/10.5194/acp-24-13751-2024, 2024
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We use a regional climate model, COSMO-CLM², enhanced with a module resolving aerosol processes, to study Antarctic clouds. We prescribe different concentrations of ice-nucleating particles to our model to assess how these clouds respond to concentration changes, validating results with cloud and aerosol observations from the Princess Elisabeth Antarctica station. Our results show that aerosol–cloud interactions vary with temperature, providing valuable insights into Antarctic cloud dynamics.
Yi Li, Xiaoli Liu, and Hengjia Cai
Atmos. Chem. Phys., 24, 13525–13540, https://doi.org/10.5194/acp-24-13525-2024, https://doi.org/10.5194/acp-24-13525-2024, 2024
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The influence of different aerosol modes on cloud processes remains controversial. We modified the aerosol spectra and concentrations to simulate a warm stratiform cloud process in Jiangxi, China, using the WRF-SBM scheme. Research shows that different aerosol spectra have diverse effects on cloud droplet spectra, cloud development, and the correlation between dispersion (ε) and cloud physics quantities. Compared to cloud droplet concentration, ε is more sensitive to the volume radius.
Fabian Hoffmann, Franziska Glassmeier, and Graham Feingold
Atmos. Chem. Phys., 24, 13403–13412, https://doi.org/10.5194/acp-24-13403-2024, https://doi.org/10.5194/acp-24-13403-2024, 2024
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Clouds constitute a major cooling influence on Earth's climate system by reflecting a large fraction of the incident solar radiation back to space. This ability is controlled by the number of cloud droplets, which is governed by the number of aerosol particles in the atmosphere, laying the foundation for so-called aerosol–cloud–climate interactions. In this study, a simple model to understand the effect of aerosol on cloud water is developed and applied.
Pouriya Alinaghi, Fredrik Jansson, Daniel A. Blázquez, and Franziska Glassmeier
EGUsphere, https://doi.org/10.5194/egusphere-2024-3501, https://doi.org/10.5194/egusphere-2024-3501, 2024
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Shallow clouds in the trades are a major source of uncertainty in climate projections. These clouds organize into striking mesoscale patterns that are exactly what climate models lack. This study explores the origin of such patterns and investigates how variations in microscale properties control them. The importance of microscale effects is compared to that of large-scale forcing on the mesoscale organization of trade-cumulus fields.
Andrea Mosso, Thomas Hocking, and Thorsten Mauritsen
Atmos. Chem. Phys., 24, 12793–12806, https://doi.org/10.5194/acp-24-12793-2024, https://doi.org/10.5194/acp-24-12793-2024, 2024
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Clouds play a crucial role in the Earth's energy balance, as they can either warm up or cool down the area they cover depending on their height and depth. They are expected to alter their behaviour under climate change, affecting the warming generated by greenhouse gases. This paper proposes a new method to estimate their overall effect on this warming by simulating a climate where clouds are transparent. Results show that with the model used, clouds have a stabilising effect on climate.
Tao Shi, Yuanjian Yang, Ping Qi, and Simone Lolli
Atmos. Chem. Phys., 24, 12807–12822, https://doi.org/10.5194/acp-24-12807-2024, https://doi.org/10.5194/acp-24-12807-2024, 2024
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This paper explored the formation mechanisms of the amplified canopy urban heat island intensity (ΔCUHII) during heat wave (HW) periods in the megacity of Beijing from the perspectives of mountain–valley breeze and urban morphology. During the mountain breeze phase, high-rise buildings with lower sky view factors (SVFs) had a pronounced effect on the ΔCUHII. During the valley breeze phase, high-rise buildings exerted a dual influence on the ΔCUHII.
Yao-Sheng Chen, Jianhao Zhang, Fabian Hoffmann, Takanobu Yamaguchi, Franziska Glassmeier, Xiaoli Zhou, and Graham Feingold
Atmos. Chem. Phys., 24, 12661–12685, https://doi.org/10.5194/acp-24-12661-2024, https://doi.org/10.5194/acp-24-12661-2024, 2024
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Marine stratocumulus cloud is a type of shallow cloud that covers the vast areas of Earth's surface. It plays an important role in Earth's energy balance by reflecting solar radiation back to space. We used numerical models to simulate a large number of marine stratocumuli with different characteristics. We found that how the clouds develop throughout the day is affected by the level of humidity in the air above the clouds and how closely the clouds connect to the ocean surface.
Andrew DeLaFrance, Lynn McMurdie, Angela Rowe, and Andrew Heymsfield
EGUsphere, https://doi.org/10.5194/egusphere-2024-3423, https://doi.org/10.5194/egusphere-2024-3423, 2024
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Numerical modeling simulations are used to investigate ice crystal growth and decay processes within a banded region of enhanced precipitation rates during a prominent winter storm. We identify robust primary ice growth in the upper portion of the cloud but decay exceeding 70 % during fallout through a subsaturated layer. The ice fall characteristics and decay rate are sensitive to the ambient cloud properties which has implications for radar-based measurements and precipitation accumulations.
Ehsan Erfani, Robert Wood, Peter Blossey, Sarah J. Doherty, and Ryan Eastman
EGUsphere, https://doi.org/10.5194/egusphere-2024-3232, https://doi.org/10.5194/egusphere-2024-3232, 2024
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In this study, we explore how marine clouds interact with aerosols. We introduce a novel approach to identify a reduced number of representative cases from a wide array of observed environmental conditions prevalent in the Northeast Pacific. We created over 2200 trajectories from observations and used cloud-resolving simulations to investigate how marine low clouds evolve in two different cases. It is shown that aerosols can delay cloud breakup, but their impact depends on precipitation.
Hsiang-He Lee, Xue Zheng, Shaoyue Qiu, and Yuan Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-3199, https://doi.org/10.5194/egusphere-2024-3199, 2024
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The study investigates how aerosol-cloud interactions affect warm boundary layer stratiform clouds over the Eastern North Atlantic. High-resolution WRF-Chem simulations reveal that non-rain clouds at the edges of cloud systems are prone to evaporation, leading to an aerosol drying effect and a transition of aerosols back to accumulation mode for future activation. The study emphasizes that this dynamic behavior is often not adequately represented in most previous prescribed-aerosol simulations.
Alexei Korolev, Zhipeng Qu, Jason Milbrandt, Ivan Heckman, Mélissa Cholette, Mengistu Wolde, Cuong Nguyen, Greg M. McFarquhar, Paul Lawson, and Ann M. Fridlind
Atmos. Chem. Phys., 24, 11849–11881, https://doi.org/10.5194/acp-24-11849-2024, https://doi.org/10.5194/acp-24-11849-2024, 2024
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The phenomenon of high ice water content (HIWC) occurs in mesoscale convective systems (MCSs) when a large number of small ice particles with typical sizes of a few hundred micrometers is found at high altitudes. It was found that secondary ice production in the vicinity of the melting layer plays a key role in the formation and maintenance of HIWC. This study presents a conceptual model of the formation of HIWC in tropical MCSs based on in situ observations and numerical simulation.
Puja Roy, Robert M. Rauber, and Larry Di Girolamo
Atmos. Chem. Phys., 24, 11653–11678, https://doi.org/10.5194/acp-24-11653-2024, https://doi.org/10.5194/acp-24-11653-2024, 2024
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Cloud droplet temperature and lifetime impact cloud microphysical processes such as the activation of ice-nucleating particles. We investigate the thermal and radial evolution of supercooled cloud droplets and their surrounding environments with an aim to better understand observed enhanced ice formation at supercooled cloud edges. This analysis shows that the magnitude of droplet cooling during evaporation is greater than estimated from past studies, especially for drier environments.
Mathieu Lachapelle, Mélissa Cholette, and Julie M. Thériault
Atmos. Chem. Phys., 24, 11285–11304, https://doi.org/10.5194/acp-24-11285-2024, https://doi.org/10.5194/acp-24-11285-2024, 2024
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Hazardous precipitation types such as ice pellets and freezing rain are difficult to predict because they are associated with complex microphysical processes. Using Predicted Particle Properties (P3), this work shows that secondary ice production processes increase the amount of ice pellets simulated while decreasing the amount of freezing rain. Moreover, the properties of the simulated precipitation compare well with those that were measured.
Andrew DeLaFrance, Lynn A. McMurdie, Angela K. Rowe, and Andrew J. Heymsfield
Atmos. Chem. Phys., 24, 11191–11206, https://doi.org/10.5194/acp-24-11191-2024, https://doi.org/10.5194/acp-24-11191-2024, 2024
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Using a numerical model, the process whereby falling ice crystals accumulate supercooled liquid water droplets is investigated to elucidate its effects on radar-based measurements and surface precipitation. We demonstrate that this process accounted for 55% of the precipitation during a wintertime storm and is uniquely discernable from other ice crystal growth processes in Doppler velocity measurements. These results have implications for measurements from airborne and spaceborne platforms.
Gabriella Wallentin, Annika Oertel, Luisa Ickes, Peggy Achtert, Matthias Tesche, and Corinna Hoose
EGUsphere, https://doi.org/10.5194/egusphere-2024-2988, https://doi.org/10.5194/egusphere-2024-2988, 2024
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Multilayer clouds are common in the Arctic but remain understudied. We use an atmospheric model to simulate multilayer cloud cases from the Arctic expedition MOSAiC 2019/2020. We find that it is complex to accurately model these cloud layers due to the lack of correct temperature and humidity profiles. The model also struggles to capture the observed cloud phase, the relative concentration of cloud droplets and cloud ice. We constrain our model to measured aerosols to mitigate this issue.
Toshi Matsui, Daniel Hernandez-Deckers, Scott E. Giangrande, Thiago S. Biscaro, Ann Fridlind, and Scott Braun
Atmos. Chem. Phys., 24, 10793–10814, https://doi.org/10.5194/acp-24-10793-2024, https://doi.org/10.5194/acp-24-10793-2024, 2024
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Using computer simulations and real measurements, we discovered that storms over the Amazon were narrower but more intense during the dry periods, producing heavier rain and more ice particles in the clouds. Our research showed that cumulus bubbles played a key role in creating these intense storms. This study can improve the representation of the effect of continental and ocean environments on tropical regions' rainfall patterns in simulations.
Ravi Kumar Reddy Addula, Ingrid de Almeida Ribeiro, Valeria Molinero, and Baron Peters
Atmos. Chem. Phys., 24, 10833–10848, https://doi.org/10.5194/acp-24-10833-2024, https://doi.org/10.5194/acp-24-10833-2024, 2024
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Ice nucleation from supercooled droplets is important in many weather and climate modeling efforts. For experiments where droplets are steadily supercooled from the freezing point, our work combines nucleation theory and survival probability analysis to predict the nucleation spectrum, i.e., droplet freezing probabilities vs. temperature. We use the new framework to extract approximately consistent rate parameters from experiments with different cooling rates and droplet sizes.
Jianhao Zhang, Yao-Sheng Chen, Takanobu Yamaguchi, and Graham Feingold
Atmos. Chem. Phys., 24, 10425–10440, https://doi.org/10.5194/acp-24-10425-2024, https://doi.org/10.5194/acp-24-10425-2024, 2024
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Quantifying cloud response to aerosol perturbations presents a major challenge in understanding the human impact on climate. Using a large number of process-resolving simulations of marine stratocumulus, we show that solar heating drives a negative feedback mechanism that buffers the persistent negative trend in cloud water adjustment after sunrise. This finding has implications for the dependence of the cloud cooling effect on the timing of deliberate aerosol perturbations.
Aaron Wang, Steve Krueger, Sisi Chen, Mikhail Ovchinnikov, Will Cantrell, and Raymond A. Shaw
Atmos. Chem. Phys., 24, 10245–10260, https://doi.org/10.5194/acp-24-10245-2024, https://doi.org/10.5194/acp-24-10245-2024, 2024
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We employ two methods to examine a laboratory experiment on clouds with both ice and liquid phases. The first assumes well-mixed properties; the second resolves the spatial distribution of turbulence and cloud particles. Results show that while the trends in mean properties generally align, when turbulence is resolved, liquid droplets are not fully depleted by ice due to incomplete mixing. This underscores the threshold of ice mass fraction in distinguishing mixed-phase clouds from ice clouds.
Patrick Peter, Sigrun Matthes, Christine Frömming, Patrick Jöckel, Luca Bugliaro, Andreas Giez, Martina Krämer, and Volker Grewe
EGUsphere, https://doi.org/10.5194/egusphere-2024-2142, https://doi.org/10.5194/egusphere-2024-2142, 2024
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Our study examines how temperature and humidity representations influence contrail (-cirrus) formation criteria. Using various model setups, we identified biases that lead to overestimation of contrail formation areas. By comparing simulations with in-flight and satellite observations, we confirmed that humidity threshold choices greatly affect contrail predictions. These findings can help develop strategies for climate-optimized flight routes, potentially reducing aviation's climate effect.
Theresa Kiszler, Davide Ori, and Vera Schemann
Atmos. Chem. Phys., 24, 10039–10053, https://doi.org/10.5194/acp-24-10039-2024, https://doi.org/10.5194/acp-24-10039-2024, 2024
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Microphysical processes impact the phase-partitioning of clouds. In this study we evaluate these processes while focusing on low-level Arctic clouds. To achieve this we used an extensive simulation set in combination with a new diagnostic tool. This study presents our findings on the relevance of these processes and their behaviour under different thermodynamic regimes.
Shuaiqi Tang, Hailong Wang, Xiang-Yu Li, Jingyi Chen, Armin Sorooshian, Xubin Zeng, Ewan Crosbie, Kenneth L. Thornhill, Luke D. Ziemba, and Christiane Voigt
Atmos. Chem. Phys., 24, 10073–10092, https://doi.org/10.5194/acp-24-10073-2024, https://doi.org/10.5194/acp-24-10073-2024, 2024
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We examined marine boundary layer clouds and their interactions with aerosols in the E3SM single-column model (SCM) for a case study. The SCM shows good agreement when simulating the clouds with high-resolution models. It reproduces the relationship between cloud droplet and aerosol particle number concentrations as produced in global models. However, the relationship between cloud liquid water and droplet number concentration is different, warranting further investigation.
Suf Lorian and Guy Dagan
Atmos. Chem. Phys., 24, 9323–9338, https://doi.org/10.5194/acp-24-9323-2024, https://doi.org/10.5194/acp-24-9323-2024, 2024
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We examine the combined effect of aerosols and sea surface temperature (SST) on clouds under equilibrium conditions in cloud-resolving radiative–convective equilibrium simulations. We demonstrate that the aerosol–cloud interaction's effect on top-of-atmosphere energy gain strongly depends on the underlying SST, while the shortwave part of the spectrum is significantly more sensitive to SST. Furthermore, increasing aerosols influences upper-troposphere stability and thus anvil cloud fraction.
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