Articles | Volume 17, issue 15
https://doi.org/10.5194/acp-17-9585-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-9585-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
How do changes in warm-phase microphysics affect deep convective clouds?
Qian Chen
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
Key Laboratory of Meteorological Disaster, Ministry of Education (KLME); Joint International Research Laboratory of Climate and Environment Change (ILCEC); Collaborative Innovation Center on Forecast and Evaluation
of Meteorological Disasters; Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration; Nanjing University of Information Science and Technology, Nanjing, China
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
Orit Altaratz
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
Reuven H. Heiblum
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
Guy Dagan
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
Lital Pinto
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel
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This letter explores a novel approach for the formation of cloud droplets in rising adiabatic air parcels. Our approach combines microphysical equations accounting for moisture, updrafts and concentration of aerosols. Our analysis reveals three regimes: A) Low moisture and high concentration can hinder activation; B) Droplets can activate and stabilize above critical sizes, and C) sparse clouds can have droplets exhibiting activation and deactivation cycles.
Huan Liu, Ilan Koren, Orit Altaratz, and Mickaël D. Chekroun
Atmos. Chem. Phys., 23, 6559–6569, https://doi.org/10.5194/acp-23-6559-2023, https://doi.org/10.5194/acp-23-6559-2023, 2023
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Clouds' responses to global warming contribute the largest uncertainty in climate prediction. Here, we analyze 42 years of global cloud cover in reanalysis data and show a decreasing trend over most continents and an increasing trend over the tropical and subtropical oceans. A reduction in near-surface relative humidity can explain the decreasing trend in cloud cover over land. Our results suggest potential stress on the terrestrial water cycle, associated with global warming.
Elisa T. Sena, Ilan Koren, Orit Altaratz, and Alexander B. Kostinski
Atmos. Chem. Phys., 22, 16111–16122, https://doi.org/10.5194/acp-22-16111-2022, https://doi.org/10.5194/acp-22-16111-2022, 2022
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Guy Dagan
Atmos. Chem. Phys., 22, 15767–15775, https://doi.org/10.5194/acp-22-15767-2022, https://doi.org/10.5194/acp-22-15767-2022, 2022
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Using idealized simulations we demonstrate that the equilibrium climate sensitivity (ECS), i.e. the increase in surface temperature under equilibrium conditions due to doubling of the CO2 concentration, increases with the aerosol concentration. The ECS increase is explained by a faster increase in precipitation efficiency with warming under high aerosol concentrations, which more efficiently depletes the water from the cloud and thus is manifested as an increase in the cloud feedback parameter.
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
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Eshkol Eytan, Ilan Koren, Orit Altaratz, Mark Pinsky, and Alexander Khain
Atmos. Chem. Phys., 21, 16203–16217, https://doi.org/10.5194/acp-21-16203-2021, https://doi.org/10.5194/acp-21-16203-2021, 2021
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Tom Dror, Mickaël D. Chekroun, Orit Altaratz, and Ilan Koren
Atmos. Chem. Phys., 21, 12261–12272, https://doi.org/10.5194/acp-21-12261-2021, https://doi.org/10.5194/acp-21-12261-2021, 2021
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A part of continental shallow convective cumulus (Cu) was shown to share properties such as organization and formation over vegetated areas, thus named green Cu. Mechanisms behind the formed patterns are not understood. We use different metrics and an empirical orthogonal function (EOF) to decompose the dataset and quantify organization factors (cloud streets and gravity waves). We show that clouds form a highly organized grid structure over hundreds of kilometers at the field lifetime.
Tom Dror, J. Michel Flores, Orit Altaratz, Guy Dagan, Zev Levin, Assaf Vardi, and Ilan Koren
Atmos. Chem. Phys., 20, 15297–15306, https://doi.org/10.5194/acp-20-15297-2020, https://doi.org/10.5194/acp-20-15297-2020, 2020
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We used in situ aerosol measurements over the Atlantic, Caribbean, and Pacific to initialize a cloud model and study the impact of aerosol concentration and sizes on warm clouds. We show that high aerosol concentration increases cloud mass and reduces surface rain when giant particles (diameter > 9 µm) are present. The large aerosols changed the timing and magnitude of internal cloud processes and resulted in an enhanced evaporation below cloud base and dramatically reduced surface rain.
Guy Dagan and Philip Stier
Atmos. Chem. Phys., 20, 6291–6303, https://doi.org/10.5194/acp-20-6291-2020, https://doi.org/10.5194/acp-20-6291-2020, 2020
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Ensemble daily simulations for two separate month-long periods over a region near Barbados were conducted to investigate aerosol effects on cloud properties and the atmospheric energy budget. For each day, two simulations were conducted with low and high cloud droplet number concentrations representing clean and polluted conditions, respectively. These simulations are used to distinguish between properties that are robustly affected by changes in aerosol concentrations and those that are not.
Guy Dagan, Philip Stier, Matthew Christensen, Guido Cioni, Daniel Klocke, and Axel Seifert
Atmos. Chem. Phys., 20, 4523–4544, https://doi.org/10.5194/acp-20-4523-2020, https://doi.org/10.5194/acp-20-4523-2020, 2020
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In order to better understand the physical processes behind aerosol effects on the atmospheric energy budget, we analyse numerical simulations of tropical cloud systems. Two sets of simulations, at different dates during the NARVAL 2 field campaign, are simulated with different dominant cloud modes. Our results demonstrate that under different environmental conditions, the response of the atmospheric energy budget to aerosol perturbation could be different.
Xin Zhang, Yan Yin, Ronald van der A, Jeff L. Lapierre, Qian Chen, Xiang Kuang, Shuqi Yan, Jinghua Chen, Chuan He, and Rulin Shi
Atmos. Meas. Tech., 13, 1709–1734, https://doi.org/10.5194/amt-13-1709-2020, https://doi.org/10.5194/amt-13-1709-2020, 2020
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Lightning NOx has a strong impact on ozone and the hydroxyl radical production. However, the production efficiency of lightning NOx is still quite uncertain. This work develops the algorithm of estimating lightning NOx for both clean and polluted regions and evaluates the sensitivity of estimates to the model setting of lightning NO. Results reveal that our method reduces the sensitivity to the background NO2 and includes much of the below-cloud LNO2.
George Spill, Philip Stier, Paul R. Field, and Guy Dagan
Atmos. Chem. Phys., 19, 13507–13517, https://doi.org/10.5194/acp-19-13507-2019, https://doi.org/10.5194/acp-19-13507-2019, 2019
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Shallow convective clouds are among the most common and least understood clouds in the atmosphere. Here we present simulations of realistic, shallow cloud fields in a large domain, in contrast to typical idealised simulations, and find that in these simulations the response to aerosol perturbations is different.
Reuven H. Heiblum, Lital Pinto, Orit Altaratz, Guy Dagan, and Ilan Koren
Atmos. Chem. Phys., 19, 10717–10738, https://doi.org/10.5194/acp-19-10717-2019, https://doi.org/10.5194/acp-19-10717-2019, 2019
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It is useful to divide a cloud into two regions: core and margin. Three parameters used to define a core are compared: buoyancy (B), relative humidity (RH), and vertical velocity (W). Using theoretical arguments and simulations, we show that during most of a cloud's lifetime, the cores are subsets of one another: Bcore ⊆ RHcore ⊆ Wcore. Moreover, the core–shell cloud model applies to all core definitions. Our findings can serve as a benchmark in the partition the core and margin.
Reuven H. Heiblum, Lital Pinto, Orit Altaratz, Guy Dagan, and Ilan Koren
Atmos. Chem. Phys., 19, 10739–10755, https://doi.org/10.5194/acp-19-10739-2019, https://doi.org/10.5194/acp-19-10739-2019, 2019
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The effects of aerosol concentration on a cloud's partition to core and margin are examined. The main finding from Part I (i.e. Bcore ⊆ RHcore ⊆ Wcore) is seen for all aerosol concentrations. Clouds can produce positive buoyancy due to both saturated updrafts or unsaturated downdrafts; the latter are dependent on low aerosol concentrations. We show that a cloud's mass is mainly dependent on core processes (condensation), while its volume is mainly dependent on margin processes (evaporation).
Guy Dagan, Ilan Koren, and Orit Altaratz
Atmos. Chem. Phys., 18, 6761–6769, https://doi.org/10.5194/acp-18-6761-2018, https://doi.org/10.5194/acp-18-6761-2018, 2018
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In this paper we distill the problem of aerosol–cloud interactions to an interplay between the system's two characteristic vertical velocities, i.e., the air vertical velocity and the collective droplets fall velocity. We show using theoretical considerations and cloud-resolving models that the relations between the two velocities are extremely sensitive to the cloud field's thermodynamics and microphysical properties.
Yevgeny Derimian, Marie Choël, Yinon Rudich, Karine Deboudt, Oleg Dubovik, Alexander Laskin, Michel Legrand, Bahaiddin Damiri, Ilan Koren, Florin Unga, Myriam Moreau, Meinrat O. Andreae, and Arnon Karnieli
Atmos. Chem. Phys., 17, 11331–11353, https://doi.org/10.5194/acp-17-11331-2017, https://doi.org/10.5194/acp-17-11331-2017, 2017
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We present influence of daily occurrence of the sea breeze flow from the Mediterranean Sea on physicochemical and optical properties of atmospheric aerosol deep inland in the Negev Desert of Israel. Sampled airborne dust was found be internally mixed with sea-salt particles and reacted with anthropogenic pollution, which makes the dust highly hygroscopic and a liquid coating of particles appears. These physicochemical transformations are associated with a change in aerosol radiative properties.
Guy Dagan, Ilan Koren, Orit Altaratz, and Reuven H. Heiblum
Atmos. Chem. Phys., 17, 7435–7444, https://doi.org/10.5194/acp-17-7435-2017, https://doi.org/10.5194/acp-17-7435-2017, 2017
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Large eddy simulations with bin microphysics are used to study cloud fields' sensitivity to changes in aerosol loading and the time evolution of this response. We show that the mean field properties change with a non-monotonic trend, with an optimum aerosol concentration for which the field reaches its maximal water mass or rain yield. The evolution of the mean thermodynamic properties is studied and shown to cause the migration of the optimal aerosol concentration toward higher values.
Yaniv Tubul, Ilan Koren, Orit Altaratz, and Reuven H. Heiblum
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2017-121, https://doi.org/10.5194/amt-2017-121, 2017
Revised manuscript not accepted
Chandan Sarangi, Sachchida Nand Tripathi, Vijay P. Kanawade, Ilan Koren, and D. Sivanand Pai
Atmos. Chem. Phys., 17, 5185–5204, https://doi.org/10.5194/acp-17-5185-2017, https://doi.org/10.5194/acp-17-5185-2017, 2017
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Aerosol-induced perturbations in cloud systems and rainfall are very uncertain. This study provides observational evidence of a robust positive association between aerosol–cloud–rainfall properties over the Indian summer monsoon region. Observed and modeled aerosol–cloud microphysical changes illustrate that cloud invigoration under a high AOD scenario can explain most of the aerosol-associated changes in cloud fraction, cloud top pressure, and surface rainfall over this region.
Y. Tubul, I. Koren, and O. Altaratz
Earth Syst. Dynam., 6, 781–788, https://doi.org/10.5194/esd-6-781-2015, https://doi.org/10.5194/esd-6-781-2015, 2015
Y. Ben Ami, O. Altaratz, Y. Yair, and I. Koren
Nat. Hazards Earth Syst. Sci., 15, 2449–2459, https://doi.org/10.5194/nhess-15-2449-2015, https://doi.org/10.5194/nhess-15-2449-2015, 2015
S. Fuzzi, U. Baltensperger, K. Carslaw, S. Decesari, H. Denier van der Gon, M. C. Facchini, D. Fowler, I. Koren, B. Langford, U. Lohmann, E. Nemitz, S. Pandis, I. Riipinen, Y. Rudich, M. Schaap, J. G. Slowik, D. V. Spracklen, E. Vignati, M. Wild, M. Williams, and S. Gilardoni
Atmos. Chem. Phys., 15, 8217–8299, https://doi.org/10.5194/acp-15-8217-2015, https://doi.org/10.5194/acp-15-8217-2015, 2015
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Particulate matter (PM) constitutes one of the most challenging problems both for air quality and climate change policies. This paper reviews the most recent scientific results on the issue and the policy needs that have driven much of the increase in monitoring and mechanistic research over the last 2 decades. The synthesis reveals many new processes and developments in the science underpinning climate-PM interactions and the effects of PM on human health and the environment.
G. Feingold, I. Koren, T. Yamaguchi, and J. Kazil
Atmos. Chem. Phys., 15, 7351–7367, https://doi.org/10.5194/acp-15-7351-2015, https://doi.org/10.5194/acp-15-7351-2015, 2015
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Most research on the relationship between aerosol and closed/open cell transitions tends to focus on the closed to open transition. Here we address the two-way transition between closed and open cellular states using a cloud resolving model. We find inherent asymmetry in the transitions and explain the source of the asymmetry. Results are supported by a dynamical system analogue to the full system.
G. Dagan, I. Koren, and O. Altaratz
Atmos. Chem. Phys., 15, 2749–2760, https://doi.org/10.5194/acp-15-2749-2015, https://doi.org/10.5194/acp-15-2749-2015, 2015
E. Tas, A. Teller, O. Altaratz, D. Axisa, R. Bruintjes, Z. Levin, and I. Koren
Atmos. Chem. Phys., 15, 2009–2017, https://doi.org/10.5194/acp-15-2009-2015, https://doi.org/10.5194/acp-15-2009-2015, 2015
G. Snider, C. L. Weagle, R. V. Martin, A. van Donkelaar, K. Conrad, D. Cunningham, C. Gordon, M. Zwicker, C. Akoshile, P. Artaxo, N. X. Anh, J. Brook, J. Dong, R. M. Garland, R. Greenwald, D. Griffith, K. He, B. N. Holben, R. Kahn, I. Koren, N. Lagrosas, P. Lestari, Z. Ma, J. Vanderlei Martins, E. J. Quel, Y. Rudich, A. Salam, S. N. Tripathi, C. Yu, Q. Zhang, Y. Zhang, M. Brauer, A. Cohen, M. D. Gibson, and Y. Liu
Atmos. Meas. Tech., 8, 505–521, https://doi.org/10.5194/amt-8-505-2015, https://doi.org/10.5194/amt-8-505-2015, 2015
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We have initiated a global network of ground-level monitoring stations to measure concentrations of fine aerosols in urban environments. Our findings include major ions species, total mass, and total scatter at three wavelengths. Results will be used to further evaluate and enhance satellite remote sensing estimates.
E. Hirsch, I. Koren, Z. Levin, O. Altaratz, and E. Agassi
Atmos. Chem. Phys., 14, 9001–9012, https://doi.org/10.5194/acp-14-9001-2014, https://doi.org/10.5194/acp-14-9001-2014, 2014
A. K. Mishra, K. Klingmueller, E. Fredj, J. Lelieveld, Y. Rudich, and I. Koren
Atmos. Chem. Phys., 14, 7213–7231, https://doi.org/10.5194/acp-14-7213-2014, https://doi.org/10.5194/acp-14-7213-2014, 2014
R. H. Heiblum, I. Koren, and G. Feingold
Atmos. Chem. Phys., 14, 6063–6074, https://doi.org/10.5194/acp-14-6063-2014, https://doi.org/10.5194/acp-14-6063-2014, 2014
G. Feingold and I. Koren
Nonlin. Processes Geophys., 20, 1011–1021, https://doi.org/10.5194/npg-20-1011-2013, https://doi.org/10.5194/npg-20-1011-2013, 2013
E. Hirsch, I. Koren, O. Altaratz, Z. Levin, and E. Agassi
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-28729-2013, https://doi.org/10.5194/acpd-13-28729-2013, 2013
Revised manuscript not accepted
Related subject area
Subject: Clouds and Precipitation | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
The impact of the mesh size and microphysics scheme on the representation of mid-level clouds in the ICON model in hilly and complex terrain
The role of ascent timescales for warm conveyor belt (WCB) moisture transport into the upper troposphere and lower stratosphere (UTLS)
Estimating the concentration of silver iodide needed to detect unambiguous signatures of glaciogenic cloud seeding
Ice-nucleating particle concentration impacts cloud properties over Dronning Maud Land, East Antarctica, in COSMO-CLM2
Numerical simulation of aerosol concentration effects on cloud droplet size spectrum evolutions of warm stratiform clouds in Jiangxi, China
The impact of aerosol on cloud water: a heuristic perspective
The presence of clouds lowers climate sensitivity in the MPI-ESM1.2 climate model
Diurnal variation in an amplified canopy urban heat island during heat wave periods in the megacity of Beijing: roles of mountain–valley breeze and urban morphology
Diurnal evolution of non-precipitating marine stratocumuli in a large-eddy simulation ensemble
High ice water content in tropical mesoscale convective systems (a conceptual model)
Evolution of cloud droplet temperature and lifetime in spatiotemporally varying subsaturated environments with implications for ice nucleation at cloud edges
Effect of secondary ice production processes on the simulation of ice pellets using the Predicted Particle Properties microphysics scheme
Simulated particle evolution within a winter storm: contributions of riming to radar moments and precipitation fallout
A thermal-driven graupel generation process to explain dry-season convective vigor over the Amazon
Modeling homogeneous ice nucleation from drop-freezing experiments: impact of droplet volume dispersion and cooling rates
Cloud water adjustments to aerosol perturbations are buffered by solar heating in non-precipitating marine stratocumuli
Glaciation of mixed-phase clouds: insights from bulk model and bin-microphysics large-eddy simulation informed by laboratory experiment
Microphysical processes involving the vapour phase dominate in simulated low-level Arctic clouds
Understanding aerosol–cloud interactions using a single-column model for a cold-air outbreak case during the ACTIVATE campaign
On the sensitivity of aerosol–cloud interactions to changes in sea surface temperature in radiative–convective equilibrium
Exploring aerosol–cloud interactions in liquid-phase clouds over eastern China and its adjacent ocean using the WRF-Chem–SBM model
Impact of secondary ice production on thunderstorm electrification under different aerosol conditions
Finite domains cause bias in measured and modeled distributions of cloud sizes
A systematic evaluation of high-cloud controlling factors
Tracking precipitation features and associated large-scale environments over southeastern Texas
Revisiting the evolution of downhill thunderstorms over Beijing: a new perspective from a radar wind profiler mesonet
How well can persistent contrails be predicted? An update
Model analysis of biases in satellite diagnosed aerosol effect on cloud liquid water path
Dynamical imprints on precipitation cluster statistics across a hierarchy of high-resolution simulations
Potential impacts of marine fuel regulations on Arctic clouds and radiative feedbacks
Present-day correlations are insufficient to predict cloud albedo change by anthropogenic aerosols in E3SM v2
Simulations of primary and secondary ice production during an Arctic mixed-phase cloud case from the Ny-Ålesund Aerosol Cloud Experiment (NASCENT) campaign
Microphysical characteristics of precipitation within convective overshooting over East China observed by GPM DPR and ERA5
Effects of radiative cooling on advection fog over the northwest Pacific Ocean: observations and large-eddy simulations
Evaluating the Wegener–Bergeron–Findeisen process in ICON in large-eddy mode with in situ observations from the CLOUDLAB project
Aerosol-induced closure of marine cloud cells: enhanced effects in the presence of precipitation
Impact of ice multiplication on the cloud electrification of a cold-season thunderstorm: a numerical case study
Developing a climatological simplification of aerosols to enter the cloud microphysics of a global climate model
Interactions between trade wind clouds and local forcings over the Great Barrier Reef: a case study using convection-permitting simulations
Variability in the properties of the distribution of the relative humidity with respect to ice: implications for contrail formation
Simulating the seeder–feeder impacts on cloud ice and precipitation over the Alps
Can pollen affect precipitation?
Cloud response to co-condensation of water and organic vapors over the boreal forest
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Nadja Omanovic, Brigitta Goger, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 14145–14175, https://doi.org/10.5194/acp-24-14145-2024, https://doi.org/10.5194/acp-24-14145-2024, 2024
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We evaluated the numerical weather model ICON in two horizontal resolutions with two bulk microphysics schemes over hilly and complex terrain in Switzerland and Austria, respectively. We focused on the model's ability to simulate mid-level clouds in summer and winter. By combining observational data from two different field campaigns, we show that an increase in the horizontal resolution and a more advanced cloud microphysics scheme is strongly beneficial for cloud representation.
Cornelis Schwenk and Annette Miltenberger
Atmos. Chem. Phys., 24, 14073–14099, https://doi.org/10.5194/acp-24-14073-2024, https://doi.org/10.5194/acp-24-14073-2024, 2024
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Warm conveyor belts (WCBs) transport moisture into the upper atmosphere, where it acts as a greenhouse gas. This transport is not well understood, and the role of rapidly rising air is unclear. We simulate a WCB and look at fast- and slow-rising air to see how moisture is (differently) transported. We find that for fast-ascending air more ice particles reach higher into the atmosphere and that frozen cloud particles are removed differently than during slow ascent, which has more water vapour.
Jing Yang, Jiaojiao Li, Meilian Chen, Xiaoqin Jing, Yan Yin, Bart Geerts, Zhien Wang, Yubao Liu, Baojun Chen, Shaofeng Hua, Hao Hu, Xiaobo Dong, Ping Tian, Qian Chen, and Yang Gao
Atmos. Chem. Phys., 24, 13833–13848, https://doi.org/10.5194/acp-24-13833-2024, https://doi.org/10.5194/acp-24-13833-2024, 2024
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Detecting unambiguous signatures is vital for examining cloud-seeding impacts, but often, seeding signatures are immersed in natural variability. In this study, reflectivity changes induced by glaciogenic seeding using different AgI concentrations are investigated under various conditions, and a method is developed to estimate the AgI concentration needed to detect unambiguous seeding signatures. The results aid in operational seeding-based decision-making regarding the amount of AgI dispersed.
Florian Sauerland, Niels Souverijns, Anna Possner, Heike Wex, Preben Van Overmeiren, Alexander Mangold, Kwinten Van Weverberg, and Nicole van Lipzig
Atmos. Chem. Phys., 24, 13751–13768, https://doi.org/10.5194/acp-24-13751-2024, https://doi.org/10.5194/acp-24-13751-2024, 2024
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We use a regional climate model, COSMO-CLM², enhanced with a module resolving aerosol processes, to study Antarctic clouds. We prescribe different concentrations of ice-nucleating particles to our model to assess how these clouds respond to concentration changes, validating results with cloud and aerosol observations from the Princess Elisabeth Antarctica station. Our results show that aerosol–cloud interactions vary with temperature, providing valuable insights into Antarctic cloud dynamics.
Yi Li, Xiaoli Liu, and Hengjia Cai
Atmos. Chem. Phys., 24, 13525–13540, https://doi.org/10.5194/acp-24-13525-2024, https://doi.org/10.5194/acp-24-13525-2024, 2024
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The influence of different aerosol modes on cloud processes remains controversial. We modified the aerosol spectra and concentrations to simulate a warm stratiform cloud process in Jiangxi, China, using the WRF-SBM scheme. Research shows that different aerosol spectra have diverse effects on cloud droplet spectra, cloud development, and the correlation between dispersion (ε) and cloud physics quantities. Compared to cloud droplet concentration, ε is more sensitive to the volume radius.
Fabian Hoffmann, Franziska Glassmeier, and Graham Feingold
Atmos. Chem. Phys., 24, 13403–13412, https://doi.org/10.5194/acp-24-13403-2024, https://doi.org/10.5194/acp-24-13403-2024, 2024
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Clouds constitute a major cooling influence on Earth's climate system by reflecting a large fraction of the incident solar radiation back to space. This ability is controlled by the number of cloud droplets, which is governed by the number of aerosol particles in the atmosphere, laying the foundation for so-called aerosol–cloud–climate interactions. In this study, a simple model to understand the effect of aerosol on cloud water is developed and applied.
Andrea Mosso, Thomas Hocking, and Thorsten Mauritsen
Atmos. Chem. Phys., 24, 12793–12806, https://doi.org/10.5194/acp-24-12793-2024, https://doi.org/10.5194/acp-24-12793-2024, 2024
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Clouds play a crucial role in the Earth's energy balance, as they can either warm up or cool down the area they cover depending on their height and depth. They are expected to alter their behaviour under climate change, affecting the warming generated by greenhouse gases. This paper proposes a new method to estimate their overall effect on this warming by simulating a climate where clouds are transparent. Results show that with the model used, clouds have a stabilising effect on climate.
Tao Shi, Yuanjian Yang, Ping Qi, and Simone Lolli
Atmos. Chem. Phys., 24, 12807–12822, https://doi.org/10.5194/acp-24-12807-2024, https://doi.org/10.5194/acp-24-12807-2024, 2024
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This paper explored the formation mechanisms of the amplified canopy urban heat island intensity (ΔCUHII) during heat wave (HW) periods in the megacity of Beijing from the perspectives of mountain–valley breeze and urban morphology. During the mountain breeze phase, high-rise buildings with lower sky view factors (SVFs) had a pronounced effect on the ΔCUHII. During the valley breeze phase, high-rise buildings exerted a dual influence on the ΔCUHII.
Yao-Sheng Chen, Jianhao Zhang, Fabian Hoffmann, Takanobu Yamaguchi, Franziska Glassmeier, Xiaoli Zhou, and Graham Feingold
Atmos. Chem. Phys., 24, 12661–12685, https://doi.org/10.5194/acp-24-12661-2024, https://doi.org/10.5194/acp-24-12661-2024, 2024
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Marine stratocumulus cloud is a type of shallow cloud that covers the vast areas of Earth's surface. It plays an important role in Earth's energy balance by reflecting solar radiation back to space. We used numerical models to simulate a large number of marine stratocumuli with different characteristics. We found that how the clouds develop throughout the day is affected by the level of humidity in the air above the clouds and how closely the clouds connect to the ocean surface.
Alexei Korolev, Zhipeng Qu, Jason Milbrandt, Ivan Heckman, Mélissa Cholette, Mengistu Wolde, Cuong Nguyen, Greg M. McFarquhar, Paul Lawson, and Ann M. Fridlind
Atmos. Chem. Phys., 24, 11849–11881, https://doi.org/10.5194/acp-24-11849-2024, https://doi.org/10.5194/acp-24-11849-2024, 2024
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The phenomenon of high ice water content (HIWC) occurs in mesoscale convective systems (MCSs) when a large number of small ice particles with typical sizes of a few hundred micrometers is found at high altitudes. It was found that secondary ice production in the vicinity of the melting layer plays a key role in the formation and maintenance of HIWC. This study presents a conceptual model of the formation of HIWC in tropical MCSs based on in situ observations and numerical simulation.
Puja Roy, Robert M. Rauber, and Larry Di Girolamo
Atmos. Chem. Phys., 24, 11653–11678, https://doi.org/10.5194/acp-24-11653-2024, https://doi.org/10.5194/acp-24-11653-2024, 2024
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Cloud droplet temperature and lifetime impact cloud microphysical processes such as the activation of ice-nucleating particles. We investigate the thermal and radial evolution of supercooled cloud droplets and their surrounding environments with an aim to better understand observed enhanced ice formation at supercooled cloud edges. This analysis shows that the magnitude of droplet cooling during evaporation is greater than estimated from past studies, especially for drier environments.
Mathieu Lachapelle, Mélissa Cholette, and Julie M. Thériault
Atmos. Chem. Phys., 24, 11285–11304, https://doi.org/10.5194/acp-24-11285-2024, https://doi.org/10.5194/acp-24-11285-2024, 2024
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Hazardous precipitation types such as ice pellets and freezing rain are difficult to predict because they are associated with complex microphysical processes. Using Predicted Particle Properties (P3), this work shows that secondary ice production processes increase the amount of ice pellets simulated while decreasing the amount of freezing rain. Moreover, the properties of the simulated precipitation compare well with those that were measured.
Andrew DeLaFrance, Lynn A. McMurdie, Angela K. Rowe, and Andrew J. Heymsfield
Atmos. Chem. Phys., 24, 11191–11206, https://doi.org/10.5194/acp-24-11191-2024, https://doi.org/10.5194/acp-24-11191-2024, 2024
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Using a numerical model, the process whereby falling ice crystals accumulate supercooled liquid water droplets is investigated to elucidate its effects on radar-based measurements and surface precipitation. We demonstrate that this process accounted for 55% of the precipitation during a wintertime storm and is uniquely discernable from other ice crystal growth processes in Doppler velocity measurements. These results have implications for measurements from airborne and spaceborne platforms.
Toshi Matsui, Daniel Hernandez-Deckers, Scott E. Giangrande, Thiago S. Biscaro, Ann Fridlind, and Scott Braun
Atmos. Chem. Phys., 24, 10793–10814, https://doi.org/10.5194/acp-24-10793-2024, https://doi.org/10.5194/acp-24-10793-2024, 2024
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Using computer simulations and real measurements, we discovered that storms over the Amazon were narrower but more intense during the dry periods, producing heavier rain and more ice particles in the clouds. Our research showed that cumulus bubbles played a key role in creating these intense storms. This study can improve the representation of the effect of continental and ocean environments on tropical regions' rainfall patterns in simulations.
Ravi Kumar Reddy Addula, Ingrid de Almeida Ribeiro, Valeria Molinero, and Baron Peters
Atmos. Chem. Phys., 24, 10833–10848, https://doi.org/10.5194/acp-24-10833-2024, https://doi.org/10.5194/acp-24-10833-2024, 2024
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Ice nucleation from supercooled droplets is important in many weather and climate modeling efforts. For experiments where droplets are steadily supercooled from the freezing point, our work combines nucleation theory and survival probability analysis to predict the nucleation spectrum, i.e., droplet freezing probabilities vs. temperature. We use the new framework to extract approximately consistent rate parameters from experiments with different cooling rates and droplet sizes.
Jianhao Zhang, Yao-Sheng Chen, Takanobu Yamaguchi, and Graham Feingold
Atmos. Chem. Phys., 24, 10425–10440, https://doi.org/10.5194/acp-24-10425-2024, https://doi.org/10.5194/acp-24-10425-2024, 2024
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Quantifying cloud response to aerosol perturbations presents a major challenge in understanding the human impact on climate. Using a large number of process-resolving simulations of marine stratocumulus, we show that solar heating drives a negative feedback mechanism that buffers the persistent negative trend in cloud water adjustment after sunrise. This finding has implications for the dependence of the cloud cooling effect on the timing of deliberate aerosol perturbations.
Aaron Wang, Steve Krueger, Sisi Chen, Mikhail Ovchinnikov, Will Cantrell, and Raymond A. Shaw
Atmos. Chem. Phys., 24, 10245–10260, https://doi.org/10.5194/acp-24-10245-2024, https://doi.org/10.5194/acp-24-10245-2024, 2024
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We employ two methods to examine a laboratory experiment on clouds with both ice and liquid phases. The first assumes well-mixed properties; the second resolves the spatial distribution of turbulence and cloud particles. Results show that while the trends in mean properties generally align, when turbulence is resolved, liquid droplets are not fully depleted by ice due to incomplete mixing. This underscores the threshold of ice mass fraction in distinguishing mixed-phase clouds from ice clouds.
Theresa Kiszler, Davide Ori, and Vera Schemann
Atmos. Chem. Phys., 24, 10039–10053, https://doi.org/10.5194/acp-24-10039-2024, https://doi.org/10.5194/acp-24-10039-2024, 2024
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Microphysical processes impact the phase-partitioning of clouds. In this study we evaluate these processes while focusing on low-level Arctic clouds. To achieve this we used an extensive simulation set in combination with a new diagnostic tool. This study presents our findings on the relevance of these processes and their behaviour under different thermodynamic regimes.
Shuaiqi Tang, Hailong Wang, Xiang-Yu Li, Jingyi Chen, Armin Sorooshian, Xubin Zeng, Ewan Crosbie, Kenneth L. Thornhill, Luke D. Ziemba, and Christiane Voigt
Atmos. Chem. Phys., 24, 10073–10092, https://doi.org/10.5194/acp-24-10073-2024, https://doi.org/10.5194/acp-24-10073-2024, 2024
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We examined marine boundary layer clouds and their interactions with aerosols in the E3SM single-column model (SCM) for a case study. The SCM shows good agreement when simulating the clouds with high-resolution models. It reproduces the relationship between cloud droplet and aerosol particle number concentrations as produced in global models. However, the relationship between cloud liquid water and droplet number concentration is different, warranting further investigation.
Suf Lorian and Guy Dagan
Atmos. Chem. Phys., 24, 9323–9338, https://doi.org/10.5194/acp-24-9323-2024, https://doi.org/10.5194/acp-24-9323-2024, 2024
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We examine the combined effect of aerosols and sea surface temperature (SST) on clouds under equilibrium conditions in cloud-resolving radiative–convective equilibrium simulations. We demonstrate that the aerosol–cloud interaction's effect on top-of-atmosphere energy gain strongly depends on the underlying SST, while the shortwave part of the spectrum is significantly more sensitive to SST. Furthermore, increasing aerosols influences upper-troposphere stability and thus anvil cloud fraction.
Jianqi Zhao, Xiaoyan Ma, Johannes Quaas, and Hailing Jia
Atmos. Chem. Phys., 24, 9101–9118, https://doi.org/10.5194/acp-24-9101-2024, https://doi.org/10.5194/acp-24-9101-2024, 2024
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We explore aerosol–cloud interactions in liquid-phase clouds over eastern China and its adjacent ocean in winter based on the WRF-Chem–SBM model, which couples a spectral-bin microphysics scheme and an online aerosol module. Our study highlights the differences in aerosol–cloud interactions between land and ocean and between precipitation clouds and non-precipitation clouds, and it differentiates and quantifies their underlying mechanisms.
Shiye Huang, Jing Yang, Qian Chen, Jiaojiao Li, Qilin Zhang, and Fengxia Guo
EGUsphere, https://doi.org/10.5194/egusphere-2024-2013, https://doi.org/10.5194/egusphere-2024-2013, 2024
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Aerosol and secondary ice production are both vital to charge separation in thunderstorms, but the relative importance of different SIP processes to cloud electrification under different aerosol conditions is not well understood. In this study, we show in a clean environment, the shattering of freezing drops has the greatest effect on the charging rate, while in a polluted environment, both rime splintering and the shattering of freezing drops have a significant effect on cloud electrification.
Thomas D. DeWitt and Timothy J. Garrett
Atmos. Chem. Phys., 24, 8457–8472, https://doi.org/10.5194/acp-24-8457-2024, https://doi.org/10.5194/acp-24-8457-2024, 2024
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There is considerable disagreement on mathematical parameters that describe the number of clouds of different sizes as well as the size of the largest clouds. Both are key defining characteristics of Earth's atmosphere. A previous study provided an incorrect explanation for the disagreement. Instead, the disagreement may be explained by prior studies not properly accounting for the size of their measurement domain. We offer recommendations for how the domain size can be accounted for.
Sarah Wilson Kemsley, Paulo Ceppi, Hendrik Andersen, Jan Cermak, Philip Stier, and Peer Nowack
Atmos. Chem. Phys., 24, 8295–8316, https://doi.org/10.5194/acp-24-8295-2024, https://doi.org/10.5194/acp-24-8295-2024, 2024
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Aiming to inform parameter selection for future observational constraint analyses, we incorporate five candidate meteorological drivers specifically targeting high clouds into a cloud controlling factor framework within a range of spatial domain sizes. We find a discrepancy between optimal domain size for predicting locally and globally aggregated cloud radiative anomalies and identify upper-tropospheric static stability as an important high-cloud controlling factor.
Ye Liu, Yun Qian, Larry K. Berg, Zhe Feng, Jianfeng Li, Jingyi Chen, and Zhao Yang
Atmos. Chem. Phys., 24, 8165–8181, https://doi.org/10.5194/acp-24-8165-2024, https://doi.org/10.5194/acp-24-8165-2024, 2024
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Deep convection under various large-scale meteorological patterns (LSMPs) shows distinct precipitation features. In southeastern Texas, mesoscale convective systems (MCSs) contribute significantly to precipitation year-round, while isolated deep convection (IDC) is prominent in summer and fall. Self-organizing maps (SOMs) reveal convection can occur without large-scale lifting or moisture convergence. MCSs and IDC events have distinct life cycles influenced by specific LSMPs.
Xiaoran Guo, Jianping Guo, Tianmeng Chen, Ning Li, Fan Zhang, and Yuping Sun
Atmos. Chem. Phys., 24, 8067–8083, https://doi.org/10.5194/acp-24-8067-2024, https://doi.org/10.5194/acp-24-8067-2024, 2024
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The prediction of downhill thunderstorms (DSs) remains elusive. We propose an objective method to identify DSs, based on which enhanced and dissipated DSs are discriminated. A radar wind profiler (RWP) mesonet is used to derive divergence and vertical velocity. The mid-troposphere divergence and prevailing westerlies enhance the intensity of DSs, whereas low-level divergence is observed when the DS dissipates. The findings highlight the key role that an RWP mesonet plays in the evolution of DSs.
Sina Hofer, Klaus Gierens, and Susanne Rohs
Atmos. Chem. Phys., 24, 7911–7925, https://doi.org/10.5194/acp-24-7911-2024, https://doi.org/10.5194/acp-24-7911-2024, 2024
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We try to improve the forecast of ice supersaturation (ISS) and potential persistent contrails using data on dynamical quantities in addition to temperature and relative humidity in a modern kind of regression model. Although the results are improved, they are not good enough for flight routing. The origin of the problem is the strong overlap of probability densities conditioned on cases with and without ice-supersaturated regions (ISSRs) in the important range of 70–100 %.
Harri Kokkola, Juha Tonttila, Silvia Calderón, Sami Romakkaniemi, Antti Lipponen, Aapo Peräkorpi, Tero Mielonen, Edward Gryspeerdt, Timo H. Virtanen, Pekka Kolmonen, and Antti Arola
EGUsphere, https://doi.org/10.5194/egusphere-2024-1964, https://doi.org/10.5194/egusphere-2024-1964, 2024
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Understanding how atmospheric aerosols affect clouds is a scientific challenge. One question is how aerosols affects the amount cloud water. We used a cloud-scale model to study these effects on marine clouds. The study showed that variations in cloud properties and instrument noise can cause bias in satellite derived cloud water content. However, our results suggest that for similar weather conditions with well-defined aerosol concentrations, satellite data can reliably track these effects.
Claudia Christine Stephan and Bjorn Stevens
EGUsphere, https://doi.org/10.5194/egusphere-2024-2020, https://doi.org/10.5194/egusphere-2024-2020, 2024
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Tropical precipitation cluster area and intensity distributions follow power laws, but the physical processes responsible for this behavior remain unknown. We analyze global simulations that realistically represent precipitation processes. We consider Earth-like planets as well as virtual planets to realize different types of large-scale dynamics. Our finding is that power laws in Earth’s precipitation cluster statistics stem from the robust power laws in Earth’s atmospheric wind field.
Luís Filipe Escusa dos Santos, Hannah C. Frostenberg, Alejandro Baró Pérez, Annica M. L. Ekman, Luisa Ickes, and Erik S. Thomson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1891, https://doi.org/10.5194/egusphere-2024-1891, 2024
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The Arctic is experiencing enhanced surface warming. The observed decline in Arctic sea-ice extent is projected to lead to an increase in Arctic shipping activity which may lead to further climatic feedbacks. We investigate, using an atmospheric model and results from marine engine experiments which focused on fuel sulfur content reduction and exhaust wet scrubbing, how ship exhaust particles influence the properties of Arctic clouds. Implications for radiative surface processes are discussed.
Naser Mahfouz, Johannes Mülmenstädt, and Susannah Burrows
Atmos. Chem. Phys., 24, 7253–7260, https://doi.org/10.5194/acp-24-7253-2024, https://doi.org/10.5194/acp-24-7253-2024, 2024
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Climate models are our primary tool to probe past, present, and future climate states unlike the more recent observation record. By constructing a hypothetical model configuration, we show that present-day correlations are insufficient to predict a persistent uncertainty in climate projection (how much sun because clouds will reflect in a changing climate). We hope our result will contribute to the scholarly conversation on better utilizing observations to constrain climate uncertainties.
Britta Schäfer, Robert Oscar David, Paraskevi Georgakaki, Julie Thérèse Pasquier, Georgia Sotiropoulou, and Trude Storelvmo
Atmos. Chem. Phys., 24, 7179–7202, https://doi.org/10.5194/acp-24-7179-2024, https://doi.org/10.5194/acp-24-7179-2024, 2024
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Mixed-phase clouds, i.e., clouds consisting of ice and supercooled water, are very common in the Arctic. However, how these clouds form is often not correctly represented in standard weather models. We show that both ice crystal concentrations in the cloud and precipitation from the cloud can be improved in the model when aerosol concentrations are prescribed from observations and when more processes for ice multiplication, i.e., the production of new ice particles from existing ice, are added.
Nan Sun, Gaopeng Lu, and Yunfei Fu
Atmos. Chem. Phys., 24, 7123–7135, https://doi.org/10.5194/acp-24-7123-2024, https://doi.org/10.5194/acp-24-7123-2024, 2024
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Microphysical characteristics of convective overshooting are essential but poorly understood, and we examine them by using the latest data. (1) Convective overshooting events mainly occur over NC (Northeast China) and northern MEC (Middle and East China). (2) Radar reflectivity of convective overshooting over NC accounts for a higher proportion below the zero level, while the opposite is the case for MEC and SC (South China). (3) Droplets of convective overshooting are large but sparse.
Liu Yang, Saisai Ding, Jing-Wu Liu, and Su-Ping Zhang
Atmos. Chem. Phys., 24, 6809–6824, https://doi.org/10.5194/acp-24-6809-2024, https://doi.org/10.5194/acp-24-6809-2024, 2024
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Advection fog occurs when warm and moist air moves over a cold sea surface. In this situation, the temperature of the foggy air usually drops below the sea surface temperature (SST), particularly at night. High-resolution simulations show that the cooling effect of longwave radiation from the top of the fog layer permeates through the fog, resulting in a cooling of the surface air below SST. This study emphasizes the significance of monitoring air temperature to enhance sea fog forecasting.
Nadja Omanovic, Sylvaine Ferrachat, Christopher Fuchs, Jan Henneberger, Anna J. Miller, Kevin Ohneiser, Fabiola Ramelli, Patric Seifert, Robert Spirig, Huiying Zhang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 6825–6844, https://doi.org/10.5194/acp-24-6825-2024, https://doi.org/10.5194/acp-24-6825-2024, 2024
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We present simulations with a high-resolution numerical weather prediction model to study the growth of ice crystals in low clouds following glaciogenic seeding. We show that the simulated ice crystals grow slower than observed and do not consume as many cloud droplets as measured in the field. This may have implications for forecasting precipitation, as the ice phase is crucial for precipitation at middle and high latitudes.
Matthew W. Christensen, Peng Wu, Adam C. Varble, Heng Xiao, and Jerome D. Fast
Atmos. Chem. Phys., 24, 6455–6476, https://doi.org/10.5194/acp-24-6455-2024, https://doi.org/10.5194/acp-24-6455-2024, 2024
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Clouds are essential to keep Earth cooler by reflecting sunlight back to space. We show that an increase in aerosol concentration suppresses precipitation in clouds, causing them to accumulate water and expand in a polluted environment with stronger turbulence and radiative cooling. This process enhances their reflectance by 51 %. It is therefore prudent to account for cloud fraction changes in assessments of aerosol–cloud interactions to improve predictions of climate change.
Jing Yang, Shiye Huang, Tianqi Yang, Qilin Zhang, Yuting Deng, and Yubao Liu
Atmos. Chem. Phys., 24, 5989–6010, https://doi.org/10.5194/acp-24-5989-2024, https://doi.org/10.5194/acp-24-5989-2024, 2024
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This study contributes to filling the dearth of understanding the impacts of different secondary ice production (SIP) processes on the cloud electrification in cold-season thunderstorms. The results suggest that SIP, especially the rime-splintering process and the shattering of freezing drops, has significant impacts on the charge structure of the storm. In addition, the modeled radar composite reflectivity and flash rate are improved after implementing the SIP processes in the model.
Ulrike Proske, Sylvaine Ferrachat, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 5907–5933, https://doi.org/10.5194/acp-24-5907-2024, https://doi.org/10.5194/acp-24-5907-2024, 2024
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Climate models include treatment of aerosol particles because these influence clouds and radiation. Over time their representation has grown increasingly detailed. This complexity may hinder our understanding of model behaviour. Thus here we simplify the aerosol representation of our climate model by prescribing mean concentrations, which saves run time and helps to discover unexpected model behaviour. We conclude that simplifications provide a new perspective for model study and development.
Wenhui Zhao, Yi Huang, Steven Siems, Michael Manton, and Daniel Harrison
Atmos. Chem. Phys., 24, 5713–5736, https://doi.org/10.5194/acp-24-5713-2024, https://doi.org/10.5194/acp-24-5713-2024, 2024
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We studied how shallow clouds and rain behave over the Great Barrier Reef (GBR) using a detailed weather model. We found that the shape of the land, especially mountains, and particles in the air play big roles in influencing these clouds. Surprisingly, the sea's temperature had a smaller effect. Our research helps us understand the GBR's climate and how various factors can influence it, where the importance of the local cloud in thermal coral bleaching has recently been identified.
Sidiki Sanogo, Olivier Boucher, Nicolas Bellouin, Audran Borella, Kevin Wolf, and Susanne Rohs
Atmos. Chem. Phys., 24, 5495–5511, https://doi.org/10.5194/acp-24-5495-2024, https://doi.org/10.5194/acp-24-5495-2024, 2024
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Relative humidity relative to ice (RHi) is a key variable in the formation of cirrus clouds and contrails. This study shows that the properties of the probability density function of RHi differ between the tropics and higher latitudes. In line with RHi and temperature variability, aircraft are likely to produce more contrails with bioethanol and liquid hydrogen as fuel. The impact of this fuel change decreases with decreasing pressure levels but increases from high latitudes to the tropics.
Zane Dedekind, Ulrike Proske, Sylvaine Ferrachat, Ulrike Lohmann, and David Neubauer
Atmos. Chem. Phys., 24, 5389–5404, https://doi.org/10.5194/acp-24-5389-2024, https://doi.org/10.5194/acp-24-5389-2024, 2024
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Ice particles precipitating into lower clouds from an upper cloud, the seeder–feeder process, can enhance precipitation. A numerical modeling study conducted in the Swiss Alps found that 48 % of observed clouds were overlapping, with the seeder–feeder process occurring in 10 % of these clouds. Inhibiting the seeder–feeder process reduced the surface precipitation and ice particle growth rates, which were further reduced when additional ice multiplication processes were included in the model.
Marje Prank, Juha Tonttila, Xiaoxia Shang, Sami Romakkaniemi, and Tomi Raatikainen
EGUsphere, https://doi.org/10.5194/egusphere-2024-876, https://doi.org/10.5194/egusphere-2024-876, 2024
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Large primary bioparticles such as pollen can be abundant in the atmosphere. In humid conditions pollens can rupture and release a large number of fine sub-pollen particles (SPPs). The paper investigates what kind of birch pollen concentrations are needed for the pollen and SPPs to start playing a noticeable role in cloud processes and alter precipitation formation. In the studied cases only the largest observed pollen concentrations were able to noticeably alter the precipitation formation.
Liine Heikkinen, Daniel G. Partridge, Sara Blichner, Wei Huang, Rahul Ranjan, Paul Bowen, Emanuele Tovazzi, Tuukka Petäjä, Claudia Mohr, and Ilona Riipinen
Atmos. Chem. Phys., 24, 5117–5147, https://doi.org/10.5194/acp-24-5117-2024, https://doi.org/10.5194/acp-24-5117-2024, 2024
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The organic vapor condensation with water vapor (co-condensation) in rising air below clouds is modeled in this work over the boreal forest because the forest air is rich in organic vapors. We show that the number of cloud droplets can increase by 20 % if considering co-condensation. The enhancements are even larger if the air contains many small, naturally produced aerosol particles. Such conditions are most frequently met in spring in the boreal forest.
Kevin Wolf, Nicolas Bellouin, and Olivier Boucher
Atmos. Chem. Phys., 24, 5009–5024, https://doi.org/10.5194/acp-24-5009-2024, https://doi.org/10.5194/acp-24-5009-2024, 2024
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The contrail formation potential and its tempo-spatial distribution are estimated for the North Atlantic flight corridor. Meteorological conditions of temperature and relative humidity are taken from the ERA5 re-analysis and IAGOS. Based on IAGOS flight tracks, crossing length, size, orientation, frequency of occurrence, and overlap of persistent contrail formation areas are determined. The presented conclusions might provide a guide for statistical flight track optimization to reduce contrails.
Franziska Hellmuth, Tim Carlsen, Anne Sophie Daloz, Robert Oscar David, and Trude Storelvmo
EGUsphere, https://doi.org/10.5194/egusphere-2024-754, https://doi.org/10.5194/egusphere-2024-754, 2024
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This article compares the occurrence of supercooled liquid-containing clouds (sLCCs) and their link to surface snowfall in CloudSat-CALIPSO, ERA5, and CMIP6 models. Significant discrepancies were found, with ERA5 and CMIP6 consistently overestimating sLCC and snowfall frequency. This bias is likely due to cloud microphysics parameterization. This conclusion has implications for accurately representing cloud phase and snowfall in future climate projections.
Lucas J. Sterzinger and Adele L. Igel
Atmos. Chem. Phys., 24, 3529–3540, https://doi.org/10.5194/acp-24-3529-2024, https://doi.org/10.5194/acp-24-3529-2024, 2024
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Using idealized large eddy simulations, we find that clouds forming in the Arctic in environments with low concentrations of aerosol particles may be sustained by mixing in new particles through the cloud top. Observations show that higher concentrations of these particles regularly exist above cloud top in concentrations that are sufficient to promote this sustenance.
Andreas Bier, Simon Unterstrasser, Josef Zink, Dennis Hillenbrand, Tina Jurkat-Witschas, and Annemarie Lottermoser
Atmos. Chem. Phys., 24, 2319–2344, https://doi.org/10.5194/acp-24-2319-2024, https://doi.org/10.5194/acp-24-2319-2024, 2024
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Using hydrogen as aviation fuel affects contrails' climate impact. We study contrail formation behind aircraft with H2 combustion. Due to the absence of soot emissions, contrail ice crystals are assumed to form only on ambient particles mixed into the plume. The ice crystal number, which strongly varies with temperature and aerosol number density, is decreased by more than 80 %–90 % compared to kerosene contrails. However H2 contrails can form at lower altitudes due to higher H2O emissions.
Prasanth Prabhakaran, Fabian Hoffmann, and Graham Feingold
Atmos. Chem. Phys., 24, 1919–1937, https://doi.org/10.5194/acp-24-1919-2024, https://doi.org/10.5194/acp-24-1919-2024, 2024
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In this study, we explore the impact of deliberate aerosol perturbation in the northeast Pacific region using large-eddy simulations. Our results show that cloud reflectivity is sensitive to the aerosol sprayer arrangement in the pristine system, whereas in the polluted system it is largely proportional to the total number of aerosol particles injected. These insights would aid in assessing the efficiency of various aerosol injection strategies for climate intervention applications.
Lisa Bock and Axel Lauer
Atmos. Chem. Phys., 24, 1587–1605, https://doi.org/10.5194/acp-24-1587-2024, https://doi.org/10.5194/acp-24-1587-2024, 2024
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Climate model simulations still show a large range of effective climate sensitivity (ECS) with high uncertainties. An important contribution to ECS is cloud climate feedback. We investigate the representation of cloud physical and radiative properties from Coupled Model Intercomparison Project models grouped by ECS. We compare the simulated cloud properties of today’s climate from three ECS groups and quantify how the projected changes in cloud properties and cloud radiative effects differ.
Leonie Villiger and Franziska Aemisegger
Atmos. Chem. Phys., 24, 957–976, https://doi.org/10.5194/acp-24-957-2024, https://doi.org/10.5194/acp-24-957-2024, 2024
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Three numerical simulations performed with an isotope-enabled weather forecast model are used to investigate the cloud–circulation coupling between shallow trade-wind cumulus clouds and atmospheric circulations on different scales. It is shown that stable water isotopes near cloud base in the tropics reflect (1) the diel cycle of the atmospheric circulation, which drives the formation and dissipation of clouds, and (2) changes in the large-scale circulation over the North Atlantic.
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