Articles | Volume 26, issue 16
https://doi.org/10.5194/acp-26-12067-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-26-12067-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Evidence of gravity wave contribution to vertical shear and mixing in the lower stratosphere
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Daniel Kunkel
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Annette Miltenberger
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Hans-Christoph Lachnitt
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Thorsten Kaluza
Department of Meteorology, University of Reading, Reading, UK
Cornelis Schwenk
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Peter Hoor
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Related authors
Madhuri Umbarkar, Daniel Kunkel, and Ulrich Achatz
EGUsphere, https://doi.org/10.5194/egusphere-2026-413, https://doi.org/10.5194/egusphere-2026-413, 2026
Short summary
Short summary
We present co-occurrence of gravity waves (GWs) and vertical shear in the North Atlantic lowermost stratosphere using ERA5 reanalysis data. Our results suggest the importance of GWs in the formation and maintenance of tropopause shear layer and ultimately to the potential turbulence occurrence in the extratropical upper troposphere lower stratosphere (UTLS). Overall, small-scale processes, and in particular, GWs can have larger implications for dynamics and composition in the UTLS.
Madhuri Umbarkar and Daniel Kunkel
Atmos. Chem. Phys., 25, 10159–10182, https://doi.org/10.5194/acp-25-10159-2025, https://doi.org/10.5194/acp-25-10159-2025, 2025
Short summary
Short summary
Atmospheric gravity waves (GWs) significantly enhance vertical shear in the lowermost stratosphere (LMS), influencing turbulence and mixing in the extratropical transition layer. Using idealized baroclinic life cycle experiments with the ICON model, this study demonstrates that moisture and cloud processes amplify GW activity, driving strong shear and turbulence in the LMS. These findings highlight the critical role of GWs in shaping the dynamics in the LMS, particularly for clear air turbulence.
Linda Smoydzin, Vera Bense, Heiko Bozem, Philipp Joppe, Daniel Kunkel, Hans-Christoph Lachnitt, Holger Tost, Andreas Zahn, Helmut Ziereis, Martin Riese, and Peter Hoor
Atmos. Chem. Phys., 26, 11857–11874, https://doi.org/10.5194/acp-26-11857-2026, https://doi.org/10.5194/acp-26-11857-2026, 2026
Short summary
Short summary
During a research flight in early October elevated upper tropospheric mixing ratios of CO, NO, NOy and O3 were observed over a distance of more than 1000 km east of the Brasilian coast. Ozone mixing ratios are 20–40 ppbv higher than during a flight in early September. By combining aircraft observations with model simulations we find that ozone production from biomass burning over Amazonia caused predominantly the ozone enhancements which have a local effect on the radiative forcing of 50 mW m−2.
Wolfgang Woiwode, Bärbel Vogel, Valentin Lauther, Jens-Uwe Grooß, Jeremy Harrison, Sören Johansson, Jörn Ungermann, Peter Braesicke, Markus Dick, Andreas Engel, Felix Friedl-Vallon, Norbert Glatthor, Thomas Gulde, Michael Höpfner, Markus Jesswein, Jan Kaumanns, Timo Keber, Anne Kleinert, Erik Kretschmer, Guido Maucher, Tom Neubert, Hans Nordmeyer, Christof Piesch, Felix Plöger, Peter Preusse, Markus Retzlaff, Sebastian Rhode, Heinz Rongen, Georg Schardt, Tanja Schuck, Björn-Martin Sinnhuber, Johannes Strobel, Franziska Trinkl, Ronja Van Luijt, Stefan Versick, C. Michael Volk, Gerald Wetzel, Peter Hoor, and Martin Riese
EGUsphere, https://doi.org/10.5194/egusphere-2026-3271, https://doi.org/10.5194/egusphere-2026-3271, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Filaments of CH2Cl2-rich air are revealed by airborne infrared limb-imaging observations in late summer 2023 above the North Pacific, Canada and Alaska and traced back to the Asian Summer Monsoon region. Involving new spectroscopic data, high CH2Cl2 levels were retrieved in the troposphere and moderate enhancements also in air masses with characteristics of the lowermost stratosphere. Mesoscale filaments are shown to transport substantial amounts of CH2Cl2 across the North Pacific.
Fatih Ekinci, Oliver Eppers, Oliver Appel, Felix Ploeger, Antonis Dragoneas, Sergej Molleker, Philipp Brauner, Hans-Christoph Lachnitt, Franziska Weyland, Linda Ort, Nicolas Emig, Hans-Christian Clemen, Laura Tomsche, Martin Ebert, Peter Hoor, Bärbel Vogel, Yafang Cheng, Johannes Schneider, Stephan Borrmann, and Franziska Köllner
Atmos. Chem. Phys., 26, 10399–10421, https://doi.org/10.5194/acp-26-10399-2026, https://doi.org/10.5194/acp-26-10399-2026, 2026
Short summary
Short summary
This study shows that aerosol transported from the Asian summer monsoon region can substantially alter the background composition of the extratropical lower stratosphere. Aircraft-based measurements and model simulations reveal a strong increase of ammonium nitrate aerosol from summer to autumn 2023 caused by transport of young air masses from South and East Asia. These particles can persist for months and undergo chemical aging.
Cornelis Schwenk and Annette Miltenberger
Atmos. Chem. Phys., 26, 7435–7462, https://doi.org/10.5194/acp-26-7435-2026, https://doi.org/10.5194/acp-26-7435-2026, 2026
Short summary
Short summary
We studied how model grid-spacing affects how moisture and ice are carried upward in large weather systems that move warm, moist air into the upper troposphere. By comparing high- and low-resolution simulations, we found that models which are able to represent convectively ascending air produce much drier air at high altitudes. This shows that model resolution strongly influences how water and clouds are transported and how they may affect climate.
Bärbel Vogel, Valentin Lauther, Franziska Köllner, Fatih Ekinci, Christian Rolf, Johannes Strobel, Ronja van Luijt, C. Michael Volk, Stephan Borrmann, Antonis Dragoneas, Oliver Eppers, Sergej Molleker, Peter Hoor, Linda Ort, Franziska Weyland, Andreas Zahn, Jan Clemens, Gebhard Günther, Oleh Kachula, Rolf Müller, Felix Ploeger, and Martin Riese
Atmos. Chem. Phys., 26, 6283–6319, https://doi.org/10.5194/acp-26-6283-2026, https://doi.org/10.5194/acp-26-6283-2026, 2026
Short summary
Short summary
This work highlights the impact of the Asian summer monsoon on the chemical composition of the upper troposphere and lower stratosphere. Measurements of trace gases and aerosol particles uplifted by the Asian summer monsoon to higher altitudes are sparse. Here, we had the opportunity to use a whole suite of different measured trace gases and the chemical composition of aerosols, in combination with simulations, to better understand the complex transport and mixing processes in this region.
Philipp Brauner, Oliver Appel, Oliver Eppers, Franziska Köllner, Hans-Christian Clemen, Tiziana Bräuer, Hans-Christoph Lachnitt, Katharina Kaiser, Johannes Schneider, Antonis Dragoneas, Andreas Hünig, Sergej Molleker, Bruce E. Anderson, Yafang Cheng, Hans Schlager, Christiane Voigt, and Stephan Borrmann
EGUsphere, https://doi.org/10.5194/egusphere-2026-2161, https://doi.org/10.5194/egusphere-2026-2161, 2026
Preprint archived
Short summary
Short summary
Airborne measurements of the aerosol chemical composition were conducted in the 2018 wintertime tropopause region over Germany using a hybrid aerosol mass spectrometer, regarding the atmospheric background and aircraft exhaust plumes. Biomass burning aerosol of North American wildfires contributes to the aerosol population. Soot and engine oil were attributed to aircraft exhaust, and were detected in contrail residuals, implying their impact on chemical processes and properties of contrails.
Chun Hang Chau, Peter Hoor, Katharina Kaiser, and Holger Tost
Atmos. Chem. Phys., 26, 3637–3652, https://doi.org/10.5194/acp-26-3637-2026, https://doi.org/10.5194/acp-26-3637-2026, 2026
Short summary
Short summary
This study examines the potential impact of different greenhouse gases to vertical mixing by clear air turbulence in the upper troposphere and lower stratosphere . We found that ozone is most sensitive to vertical mixing and could lead to cooling at the top of the atmosphere by -0.2 W/m2. We also found that the vertical mixing by clear air turbulence could lead to changes in atmospheric chemistry including changing the methane lifetime and the ozone sensitivity.
Madhuri Umbarkar, Daniel Kunkel, and Ulrich Achatz
EGUsphere, https://doi.org/10.5194/egusphere-2026-413, https://doi.org/10.5194/egusphere-2026-413, 2026
Short summary
Short summary
We present co-occurrence of gravity waves (GWs) and vertical shear in the North Atlantic lowermost stratosphere using ERA5 reanalysis data. Our results suggest the importance of GWs in the formation and maintenance of tropopause shear layer and ultimately to the potential turbulence occurrence in the extratropical upper troposphere lower stratosphere (UTLS). Overall, small-scale processes, and in particular, GWs can have larger implications for dynamics and composition in the UTLS.
Sylvia C. Sullivan, Aiko Voigt, Edgardo Sepúlveda Araya, Silvia Bucci, Annette Miltenberger, Meredith K. Kupinski, Christian Rolf, and Martina Krämer
Atmos. Chem. Phys., 26, 1685–1698, https://doi.org/10.5194/acp-26-1685-2026, https://doi.org/10.5194/acp-26-1685-2026, 2026
Short summary
Short summary
We assess the temperature, moisture, and dynamics in the upper troposphere-lower stratosphere simulated over South Asia in a high-resolution model relative to aircraft data. The lower stratosphere tends to be too warm, too dry, and too quiescent in the model, and as a result, too few ice clouds are predicted to form there. These biases could affect radiative balance and circulation in other areas also, as significant upward transport of moisture and pollutants occurs during the Asian monsoon.
Patrick Konjari, Christian Rolf, Martina Krämer, Armin Afchine, Nicole Spelten, Irene Bartolome Garcia, Annette Miltenberger, Nicolas Emig, Philipp Joppe, Johannes Schneider, Yun Li, Andreas Petzold, Heiko Bozem, and Peter Hoor
Atmos. Chem. Phys., 25, 18031–18050, https://doi.org/10.5194/acp-25-18031-2025, https://doi.org/10.5194/acp-25-18031-2025, 2025
Short summary
Short summary
We investigated how a powerful storm over southern Sweden in June 2024 transported ice particles and moist air into the normally dry stratosphere. We observed unusually high water vapor and ice levels up to 1.5 kilometers above the tropopause. Although the extra water vapor lasted only a few days to weeks, it shows how such storms can temporarily alter the upper atmosphere’s composition.
Paul Konopka, Felix Ploeger, Francesco D'Amato, Teresa Campos, Marc von Hobe, Shawn B. Honomichl, Peter Hoor, Laura L. Pan, Michelle L. Santee, Silvia Viciani, Kaley A. Walker, and Michaela I. Hegglin
Atmos. Chem. Phys., 25, 17973–17996, https://doi.org/10.5194/acp-25-17973-2025, https://doi.org/10.5194/acp-25-17973-2025, 2025
Short summary
Short summary
We present an improved version of the Chemical Lagrangian Model of the Stratosphere (CLaMS-3.0), which better represents transport from the lower atmosphere to the upper troposphere and lower stratosphere. By refining grid resolution and improving convection representation, the model more accurately simulates carbon monoxide transport. Comparisons with satellite and in situ observations highlight its ability to capture seasonal variations and improve our understanding of atmospheric transport.
Cornelis Schwenk and Annette Miltenberger
EGUsphere, https://doi.org/10.5194/egusphere-2025-5631, https://doi.org/10.5194/egusphere-2025-5631, 2025
Short summary
Short summary
We examined how model resolution affects the moisture and cloud content of large weather systems that move warm, moist air into the upper troposphere. By comparing high- and low-resolution simulations, we found that models which can resolve convectively ascending air produce drier air and more outgoing longwave radiation. This shows that model grid-spacing impacts modeled upper-level moisture and Earth's radiative balance.
Anna Breuninger, Philipp Joppe, Jonas Wilsch, Cornelis Schwenk, Heiko Bozem, Nicolas Emig, Laurin Merkel, Rainer Rossberg, Timo Keber, Arthur Kutschka, Philipp Waleska, Stefan Hofmann, Sarah Richter, Florian Ungeheuer, Konstantin Dörholt, Thorsten Hoffmann, Annette Miltenberger, Johannes Schneider, Peter Hoor, and Alexander L. Vogel
Atmos. Chem. Phys., 25, 16533–16551, https://doi.org/10.5194/acp-25-16533-2025, https://doi.org/10.5194/acp-25-16533-2025, 2025
Short summary
Short summary
This study investigates molecular organic aerosol composition in the upper troposphere and lower stratosphere from an airborne campaign over Central Europe in summer 2024. Via ultra-high-performance liquid chromatography and high-resolution mass spectrometry of tropospheric and stratospheric filter samples, we identified various organic compounds. Our findings underscore the significant cross-tropopause transport of biogenic secondary organic aerosol and anthropogenic pollutants.
Heiko Bozem, Philipp Joppe, Yun Li, Nicolas Emig, Armin Afchine, Anna Breuninger, Joachim Curtius, Stefan Hofmann, Sadath Ismayil, Konrad Kandler, Daniel Kunkel, Arthur Kutschka, Hans-Christoph Lachnitt, Andreas Petzold, Sarah Richter, Timo Röschenthaler, Christian Rolf, Lisa Schneider, Johannes Schneider, Alexander Vogel, and Peter Hoor
Atmos. Meas. Tech., 18, 6545–6568, https://doi.org/10.5194/amt-18-6545-2025, https://doi.org/10.5194/amt-18-6545-2025, 2025
Short summary
Short summary
Deployed on a Learjet as a tandem measurement platform during the TPEx I (TropoPause composition gradients and mixing Experiment) campaign in June 2024, the new TPC-TOSS (TropoPause Composition Towed Sensor Shuttle) system delivers high-resolution in situ data on ozone, aerosol, and key meteorological parameters. Laboratory and in-flight tests confirmed its precision and stability. Observed gradients near the tropopause reveal active mixing and transport processes in the tropopause region.
Philipp Joppe, Johannes Schneider, Jonas Wilsch, Heiko Bozem, Anna Breuninger, Joachim Curtius, Martin Ebert, Nicolas Emig, Peter Hoor, Sadath Ismayil, Konrad Kandler, Daniel Kunkel, Isabel Kurth, Hans-Christoph Lachnitt, Yun Li, Annette Miltenberger, Sarah Richter, Christian Rolf, Lisa Schneider, Cornelis Schwenk, Nicole Spelten, Alexander L. Vogel, Yafang Cheng, and Stephan Borrmann
Atmos. Chem. Phys., 25, 15077–15103, https://doi.org/10.5194/acp-25-15077-2025, https://doi.org/10.5194/acp-25-15077-2025, 2025
Short summary
Short summary
We show measurements of a filament with biomass burning influence transported by a warm conveyor belt (WCB) into the tropopause region over Europe. The pollution originates from Canadian forest fires and is transported in the lower troposphere towards Europe. The WCB transport is followed by mixing with air masses of stratospheric chemical signatures. We hypothesize that this mixing leads to a change in the vertical gradient of the potential temperature.
Linda Ort, Andrea Pozzer, Peter Hoor, Florian Obersteiner, Andreas Zahn, Thomas B. Ryerson, Chelsea R. Thompson, Jeff Peischl, Róisín Commane, Bruce Daube, Ilann Bourgeois, Jos Lelieveld, and Horst Fischer
Atmos. Chem. Phys., 25, 14987–15007, https://doi.org/10.5194/acp-25-14987-2025, https://doi.org/10.5194/acp-25-14987-2025, 2025
Short summary
Short summary
This study investigates the role of lightning emissions on the O3–CO ratio in the northern subtropics. We used in situ observations and a global circulation model to show an effect of up to 40 % onto the subtropical O3–CO ratio by tropical air masses transported via the Hadley cell. This influence of lightning emissions and its photochemistry has a global effect on trace and greenhouse gases and needs to be considered for global chemical distributions.
Sophie Bauchinger, Andreas Engel, Markus Jesswein, Timo Keber, Harald Bönisch, Florian Obersteiner, Andreas Zahn, Nicolas Emig, Peter Hoor, Hans-Christoph Lachnitt, Franziska Weyland, Linda Ort, and Tanja J. Schuck
Atmos. Chem. Phys., 25, 14167–14186, https://doi.org/10.5194/acp-25-14167-2025, https://doi.org/10.5194/acp-25-14167-2025, 2025
Short summary
Short summary
We compared different ways to define the upper barrier of the troposphere in the extra-tropics, the “tropopause”. By analysing ozone distributions sorted by different definitions, we found that the traditional temperature-based tropopause works less well than dynamic or tracer-based definitions. We saw a sharper transition of ozone across the tropopause using a higher value of potential vorticity than often used and recommend this value for future studies of exchange processes in this region.
Nicolas Emig, Annette K. Miltenberger, Peter M. Hoor, and Andreas Petzold
Atmos. Chem. Phys., 25, 13077–13101, https://doi.org/10.5194/acp-25-13077-2025, https://doi.org/10.5194/acp-25-13077-2025, 2025
Short summary
Short summary
This study presents in situ observations of cirrus occurrence from aircraft measurements in the extratropical transition layer (ExTL) using simultaneous measurements from two platforms. Lagrangian diagnostics based on high-resolution ICON simulations show long residence times of the cirrus in stratospheric air, allowing us to separate different diabatic processes during transit. The findings suggest that radiative diabatic cloud processes significantly impact the tropopause thermodynamic structure.
Chun Hang Chau, Peter Hoor, and Holger Tost
Atmos. Chem. Phys., 25, 13123–13140, https://doi.org/10.5194/acp-25-13123-2025, https://doi.org/10.5194/acp-25-13123-2025, 2025
Short summary
Short summary
This study examines how the turbulence in the upper troposphere/lower stratosphere (UTLS) could modify the tracer distribution under different situations. Using a multi-scale chemistry model with a novel diagnostic, we found that both the pre-existing tracer gradient and the dynamical and thermodynamical forcing play a role in modifying the tracer distribution. These results allow further research on the UTLS turbulent mixing and its implications for the climate system.
Johannes Schneider, Christiane Schulz, Florian Rubach, Anna Ludwig, Jonas Wilsch, Philipp Joppe, Christian Gurk, Sergej Molleker, Laurent Poulain, Florian Obersteiner, Torsten Gehrlein, Harald Bönisch, Andreas Zahn, Peter Hoor, Nicolas Emig, Heiko Bozem, Stephan Borrmann, and Markus Hermann
Atmos. Meas. Tech., 18, 5103–5128, https://doi.org/10.5194/amt-18-5103-2025, https://doi.org/10.5194/amt-18-5103-2025, 2025
Short summary
Short summary
An instrumented container laboratory is operated on regular commercial passenger flights to obtain a long-term representative dataset on the composition of the upper troposphere and lower stratosphere. Here we report on the development of a fully automated aerosol mass spectrometer for this project. We present technical specifications, necessary modifications for the automation, instrument calibration and comparisons, detection limits, and the first in-flight data.
Cornelis Schwenk, Annette Miltenberger, and Annika Oertel
Atmos. Chem. Phys., 25, 11333–11361, https://doi.org/10.5194/acp-25-11333-2025, https://doi.org/10.5194/acp-25-11333-2025, 2025
Short summary
Short summary
We studied how different parameter choices concerning cloud processes affect the simulated transport of water and ice into the upper atmosphere (which affects the greenhouse effect) during a weather system called a warm conveyor belt. Using a set of model experiments, we found that some parameters have a strong effect on humidity and ice, especially during fast ascents. These findings could help improve weather and climate models and may also be relevant for future climate engineering studies.
Tim Lüttmer, Annette Miltenberger, and Peter Spichtinger
Atmos. Chem. Phys., 25, 10245–10265, https://doi.org/10.5194/acp-25-10245-2025, https://doi.org/10.5194/acp-25-10245-2025, 2025
Short summary
Short summary
We investigate ice formation pathways in a warm conveyor belt case study. We employ a multi-phase microphysics scheme that distinguishes between ice from different nucleation processes. Ice crystals in the cirrus outflow mostly stem from in situ formation. Hence, they were formed directly from the vapor phase. Sedimentational redistribution modulates cirrus properties and leads to disagreement between cirrus origin classifications based on thermodynamic history and nucleation processes.
Madhuri Umbarkar and Daniel Kunkel
Atmos. Chem. Phys., 25, 10159–10182, https://doi.org/10.5194/acp-25-10159-2025, https://doi.org/10.5194/acp-25-10159-2025, 2025
Short summary
Short summary
Atmospheric gravity waves (GWs) significantly enhance vertical shear in the lowermost stratosphere (LMS), influencing turbulence and mixing in the extratropical transition layer. Using idealized baroclinic life cycle experiments with the ICON model, this study demonstrates that moisture and cloud processes amplify GW activity, driving strong shear and turbulence in the LMS. These findings highlight the critical role of GWs in shaping the dynamics in the LMS, particularly for clear air turbulence.
Rodrigo J. Seguel, Charlie Opazo, Yann Cohen, Owen R. Cooper, Laura Gallardo, Björn-Martin Sinnhuber, Florian Obersteiner, Andreas Zahn, Peter Hoor, Susanne Rohs, and Andreas Marsing
Atmos. Chem. Phys., 25, 8553–8573, https://doi.org/10.5194/acp-25-8553-2025, https://doi.org/10.5194/acp-25-8553-2025, 2025
Short summary
Short summary
We explored ozone differences between the Northern Hemisphere and Southern Hemispheres in the upper troposphere–lower stratosphere. We found lower ozone (with stratospheric origin) in the Southern Hemisphere, especially during years of severe ozone depletion. Sudden stratospheric warming events increased the ozone in each hemisphere, highlighting the relationship between stratospheric processes and ozone in the upper troposphere, where ozone is an important greenhouse gas.
Markus Jesswein, Valentin Lauther, Nicolas Emig, Peter Hoor, Timo Keber, Hans-Christoph Lachnitt, Linda Ort, Tanja Schuck, Johannes Strobel, Ronja Van Luijt, C. Michael Volk, Franziska Weyland, and Andreas Engel
Atmos. Chem. Phys., 25, 8107–8126, https://doi.org/10.5194/acp-25-8107-2025, https://doi.org/10.5194/acp-25-8107-2025, 2025
Short summary
Short summary
The study investigates transport within the Asian Summer Monsoon, focusing on how CH2Cl2 reaches the subarctic tropopause region. Using data from the PHILEAS campaign in 2023, events with increased mixing ratios were detected. Their origin, the transport paths to the tropopause region, and the potential entry into the stratosphere were analyzed. The East Asian Summer Monsoon was identified as the main transport pathway, with only a small contribution to the stratosphere in the following days.
Franziska Weyland, Peter Hoor, Daniel Kunkel, Thomas Birner, Felix Plöger, and Katharina Turhal
Atmos. Chem. Phys., 25, 1227–1252, https://doi.org/10.5194/acp-25-1227-2025, https://doi.org/10.5194/acp-25-1227-2025, 2025
Short summary
Short summary
The lowermost stratosphere (LMS) plays an important role in the Earth's climate, containing strong gradients of ozone and water vapor. Our results indicate that the thermodynamic structure of the LMS was changing between 1979–2019 in response to anthropogenic climate change and the recovery of stratospheric ozone, also indicating large-scale circulation changes. We find that both the upper and the lower LMS boundaries show an (upward) trend, which has implications for the LMS mass.
Cornelis Schwenk and Annette Miltenberger
Atmos. Chem. Phys., 24, 14073–14099, https://doi.org/10.5194/acp-24-14073-2024, https://doi.org/10.5194/acp-24-14073-2024, 2024
Short summary
Short summary
Warm conveyor belts (WCBs) transport moisture into the upper atmosphere, where it acts as a greenhouse gas. This transport is not well understood, and the role of rapidly rising air is unclear. We simulate a WCB and look at fast- and slow-rising air to see how moisture is (differently) transported. We find that for fast-ascending air more ice particles reach higher into the atmosphere and that frozen cloud particles are removed differently than during slow ascent, which has more water vapour.
Katharina Turhal, Felix Plöger, Jan Clemens, Thomas Birner, Franziska Weyland, Paul Konopka, and Peter Hoor
Atmos. Chem. Phys., 24, 13653–13679, https://doi.org/10.5194/acp-24-13653-2024, https://doi.org/10.5194/acp-24-13653-2024, 2024
Short summary
Short summary
The tropopause separates the troposphere, where many greenhouse gases originate, from the stratosphere. This study examines a tropopause defined by potential vorticity – an analogue for angular momentum that changes sharply in the subtropics, creating a transport barrier. Between 1980 and 2017, this tropopause shifted poleward at lower altitudes and equatorward above, suggesting height-dependent changes in atmospheric circulation that may affect greenhouse gas distribution and global warming.
Luis F. Millán, Peter Hoor, Michaela I. Hegglin, Gloria L. Manney, Harald Boenisch, Paul Jeffery, Daniel Kunkel, Irina Petropavlovskikh, Hao Ye, Thierry Leblanc, and Kaley Walker
Atmos. Chem. Phys., 24, 7927–7959, https://doi.org/10.5194/acp-24-7927-2024, https://doi.org/10.5194/acp-24-7927-2024, 2024
Short summary
Short summary
In the Observed Composition Trends And Variability in the UTLS (OCTAV-UTLS) Stratosphere-troposphere Processes And their Role in Climate (SPARC) activity, we have mapped multiplatform ozone datasets into coordinate systems to systematically evaluate the influence of these coordinates on binned climatological variability. This effort unifies the work of studies that focused on individual coordinate system variability. Our goal was to create the most comprehensive assessment of this topic.
Niklas Karbach, Lisa Höhler, Peter Hoor, Heiko Bozem, Nicole Bobrowski, and Thorsten Hoffmann
Atmos. Meas. Tech., 17, 4081–4086, https://doi.org/10.5194/amt-17-4081-2024, https://doi.org/10.5194/amt-17-4081-2024, 2024
Short summary
Short summary
The system presented here can accurately generate and reproduce a stable flow of gas mixtures of known concentrations over several days using ambient air as a dilution medium. In combination with the small size and low weight of the system, this enables the calibration of hydrogen sensors in the field, reducing the influence of matrix effects on the accuracy of the sensor. The system is inexpensive to assemble and easy to maintain, which is the key to reliable measurement results.
Philipp Joppe, Johannes Schneider, Katharina Kaiser, Horst Fischer, Peter Hoor, Daniel Kunkel, Hans-Christoph Lachnitt, Andreas Marsing, Lenard Röder, Hans Schlager, Laura Tomsche, Christiane Voigt, Andreas Zahn, and Stephan Borrmann
Atmos. Chem. Phys., 24, 7499–7522, https://doi.org/10.5194/acp-24-7499-2024, https://doi.org/10.5194/acp-24-7499-2024, 2024
Short summary
Short summary
From aircraft measurements in the upper troposphere/lower stratosphere, we find a correlation between the ozone and particulate sulfate in the lower stratosphere. The correlation exhibits some variability over the measurement period exceeding the background sulfate-to-ozone correlation. From our analysis, we conclude that gas-to-particle conversion of volcanic sulfur dioxide leads to observed enhanced sulfate aerosol mixing ratios.
Edward Groot, Patrick Kuntze, Annette Miltenberger, and Holger Tost
Weather Clim. Dynam., 5, 779–803, https://doi.org/10.5194/wcd-5-779-2024, https://doi.org/10.5194/wcd-5-779-2024, 2024
Short summary
Short summary
Deep convective clouds (thunderstorms), which may cause severe weather, tend to coherently organise into structured cloud systems. Accurate representation of these systems in models is difficult due to their complex dynamics and, in numerical simulations, the dependence of their dynamics on resolution. Here, the effect of convective organisation and geometry on their outflow winds (altitudes of 7–14 km) is investigated. Representation of their dynamics and outflows improves at higher resolution.
Tanja J. Schuck, Johannes Degen, Eric Hintsa, Peter Hoor, Markus Jesswein, Timo Keber, Daniel Kunkel, Fred Moore, Florian Obersteiner, Matt Rigby, Thomas Wagenhäuser, Luke M. Western, Andreas Zahn, and Andreas Engel
Atmos. Chem. Phys., 24, 689–705, https://doi.org/10.5194/acp-24-689-2024, https://doi.org/10.5194/acp-24-689-2024, 2024
Short summary
Short summary
We study the interhemispheric gradient of sulfur hexafluoride (SF6), a strong long-lived greenhouse gas. Its emissions are stronger in the Northern Hemisphere; therefore, mixing ratios in the Southern Hemisphere lag behind. Comparing the observations to a box model, the model predicts air in the Southern Hemisphere to be older. For a better agreement, the emissions used as model input need to be increased (and their spatial pattern changed), and we need to modify north–south transport.
Frederik Harzer, Hella Garny, Felix Ploeger, Harald Bönisch, Peter Hoor, and Thomas Birner
Atmos. Chem. Phys., 23, 10661–10675, https://doi.org/10.5194/acp-23-10661-2023, https://doi.org/10.5194/acp-23-10661-2023, 2023
Short summary
Short summary
We study the statistical relation between year-by-year fluctuations in winter-mean ozone and the strength of the stratospheric polar vortex. In the latitude–pressure plane, regression analysis shows that anomalously weak polar vortex years are associated with three pronounced local ozone maxima over the polar cap relative to the winter climatology. These response maxima primarily reflect the non-trivial combination of different ozone transport processes with varying relative contributions.
Annika Oertel, Annette K. Miltenberger, Christian M. Grams, and Corinna Hoose
Atmos. Chem. Phys., 23, 8553–8581, https://doi.org/10.5194/acp-23-8553-2023, https://doi.org/10.5194/acp-23-8553-2023, 2023
Short summary
Short summary
Warm conveyor belts (WCBs) are cloud- and precipitation-producing airstreams in extratropical cyclones that are important for the large-scale flow and cloud radiative forcing. We analyze cloud formation processes during WCB ascent in a two-moment microphysics scheme. Quantification of individual diabatic heating rates shows the importance of condensation, vapor deposition, rain evaporation, melting, and cloud-top radiative cooling for total heating and WCB-related potential vorticity structure.
Luis F. Millán, Gloria L. Manney, Harald Boenisch, Michaela I. Hegglin, Peter Hoor, Daniel Kunkel, Thierry Leblanc, Irina Petropavlovskikh, Kaley Walker, Krzysztof Wargan, and Andreas Zahn
Atmos. Meas. Tech., 16, 2957–2988, https://doi.org/10.5194/amt-16-2957-2023, https://doi.org/10.5194/amt-16-2957-2023, 2023
Short summary
Short summary
The determination of atmospheric composition trends in the upper troposphere and lower stratosphere (UTLS) is still highly uncertain. We present the creation of dynamical diagnostics to map several ozone datasets (ozonesondes, lidars, aircraft, and satellite measurements) in geophysically based coordinate systems. The diagnostics can also be used to analyze other greenhouse gases relevant to surface climate and UTLS chemistry.
Hans-Christoph Lachnitt, Peter Hoor, Daniel Kunkel, Martina Bramberger, Andreas Dörnbrack, Stefan Müller, Philipp Reutter, Andreas Giez, Thorsten Kaluza, and Markus Rapp
Atmos. Chem. Phys., 23, 355–373, https://doi.org/10.5194/acp-23-355-2023, https://doi.org/10.5194/acp-23-355-2023, 2023
Short summary
Short summary
We present an analysis of high-resolution airborne measurements during a flight of the DEEPWAVE 2014 campaign in New Zealand. The focus of this flight was to study the effects of enhanced mountain wave activity over the Southern Alps. We discuss changes in the upstream and downstream distributions of N2O and CO and show that these changes are related to turbulence-induced trace gas fluxes which have persistent effects on the trace gas composition in the lower stratosphere.
Paul Konopka, Mengchu Tao, Marc von Hobe, Lars Hoffmann, Corinna Kloss, Fabrizio Ravegnani, C. Michael Volk, Valentin Lauther, Andreas Zahn, Peter Hoor, and Felix Ploeger
Geosci. Model Dev., 15, 7471–7487, https://doi.org/10.5194/gmd-15-7471-2022, https://doi.org/10.5194/gmd-15-7471-2022, 2022
Short summary
Short summary
Pure trajectory-based transport models driven by meteorology derived from reanalysis products (ERA5) take into account only the resolved, advective part of transport. That means neither mixing processes nor unresolved subgrid-scale advective processes like convection are included. The Chemical Lagrangian Model of the Stratosphere (CLaMS) includes these processes. We show that isentropic mixing dominates unresolved transport. The second most important transport process is unresolved convection.
Linda Smoydzin and Peter Hoor
Atmos. Chem. Phys., 22, 7193–7206, https://doi.org/10.5194/acp-22-7193-2022, https://doi.org/10.5194/acp-22-7193-2022, 2022
Short summary
Short summary
Our study presents a detailed analysis of the spatial and temporal distribution of elevated CO level in the upper troposphere over the Pacific using 20 years of MOPITT data. We create a climatology of severe pollution episodes and use trajectory calculations to link each particular pollution event detected in MOPITT satellite data with a distinct source region. Additionally, we analyse uplift mechanisms such as WCB-related upward transport.
Helmut Ziereis, Peter Hoor, Jens-Uwe Grooß, Andreas Zahn, Greta Stratmann, Paul Stock, Michael Lichtenstern, Jens Krause, Vera Bense, Armin Afchine, Christian Rolf, Wolfgang Woiwode, Marleen Braun, Jörn Ungermann, Andreas Marsing, Christiane Voigt, Andreas Engel, Björn-Martin Sinnhuber, and Hermann Oelhaf
Atmos. Chem. Phys., 22, 3631–3654, https://doi.org/10.5194/acp-22-3631-2022, https://doi.org/10.5194/acp-22-3631-2022, 2022
Short summary
Short summary
Airborne observations were conducted in the lowermost Arctic stratosphere during the winter of 2015/2016. The observed distribution of reactive nitrogen shows clear indications of nitrification in mid-winter and denitrification in late winter. This was caused by the formation of polar stratospheric cloud particles, which were observed during several flights. The sedimentation and evaporation of these particles and the descent of air masses cause a redistribution of reactive nitrogen.
Valentin Lauther, Bärbel Vogel, Johannes Wintel, Andrea Rau, Peter Hoor, Vera Bense, Rolf Müller, and C. Michael Volk
Atmos. Chem. Phys., 22, 2049–2077, https://doi.org/10.5194/acp-22-2049-2022, https://doi.org/10.5194/acp-22-2049-2022, 2022
Short summary
Short summary
We show airborne in situ measurements of the very short-lived ozone-depleting substances CH2Cl2 and CHCl3, revealing particularly high concentrations of both species in the lower stratosphere. Back-trajectory calculations and 3D model simulations show that the air masses with high concentrations originated in the Asian boundary layer and were transported via the Asian summer monsoon. We also identify a fast transport pathway into the stratosphere via the North American monsoon and by hurricanes.
Stefan Niebler, Annette Miltenberger, Bertil Schmidt, and Peter Spichtinger
Weather Clim. Dynam., 3, 113–137, https://doi.org/10.5194/wcd-3-113-2022, https://doi.org/10.5194/wcd-3-113-2022, 2022
Short summary
Short summary
We use machine learning to create a network that detects and classifies four types of synoptic-scale weather fronts from ERA5 atmospheric reanalysis data. We present an application of our method, showing its use case in a scientific context. Additionally, our results show that multiple sources of training data are necessary to perform well on different regions, implying differences within those regions. Qualitative evaluation shows that the results are physically plausible.
Rachel E. Hawker, Annette K. Miltenberger, Jill S. Johnson, Jonathan M. Wilkinson, Adrian A. Hill, Ben J. Shipway, Paul R. Field, Benjamin J. Murray, and Ken S. Carslaw
Atmos. Chem. Phys., 21, 17315–17343, https://doi.org/10.5194/acp-21-17315-2021, https://doi.org/10.5194/acp-21-17315-2021, 2021
Short summary
Short summary
We find that ice-nucleating particles (INPs), aerosols that can initiate the freezing of cloud droplets, cause substantial changes to the properties of radiatively important convectively generated anvil cirrus. The number concentration of INPs had a large effect on ice crystal number concentration while the INP temperature dependence controlled ice crystal size and cloud fraction. The results indicate information on INP number and source is necessary for the representation of cloud glaciation.
Markus Jesswein, Heiko Bozem, Hans-Christoph Lachnitt, Peter Hoor, Thomas Wagenhäuser, Timo Keber, Tanja Schuck, and Andreas Engel
Atmos. Chem. Phys., 21, 17225–17241, https://doi.org/10.5194/acp-21-17225-2021, https://doi.org/10.5194/acp-21-17225-2021, 2021
Short summary
Short summary
This study presents and compares inorganic chlorine (Cly) derived from observations with the HALO research aircraft in the Antarctic late winter–early fall 2019 and the Arctic winter 2015–2016. Trend-corrected correlations from the Northern Hemisphere show excellent agreement with those from the Southern Hemisphere. After observation allocation inside and outside the vortex based on N2O measurements, results of the two campaigns reveal substantial differences in Cly within the respective vortex.
Meike K. Rotermund, Vera Bense, Martyn P. Chipperfield, Andreas Engel, Jens-Uwe Grooß, Peter Hoor, Tilman Hüneke, Timo Keber, Flora Kluge, Benjamin Schreiner, Tanja Schuck, Bärbel Vogel, Andreas Zahn, and Klaus Pfeilsticker
Atmos. Chem. Phys., 21, 15375–15407, https://doi.org/10.5194/acp-21-15375-2021, https://doi.org/10.5194/acp-21-15375-2021, 2021
Short summary
Short summary
Airborne total bromine (Brtot) and tracer measurements suggest Brtot-rich air masses persistently protruded into the lower stratosphere (LS), creating a high Brtot region over the North Atlantic in fall 2017. The main source is via isentropic transport by the Asian monsoon and to a lesser extent transport across the extratropical tropopause as quantified by a Lagrange model. The transport of Brtot via Central American hurricanes is also observed. Lastly, the impact of Brtot on LS O3 is assessed.
Cited articles
Achatz, U., Alexander, M. J., Becker, E., Chun, H. Y., Dörnbrack, A., Holt, L., Plougonven, R., Polichtchouk, I., Sato, K., Sheshadri, A., Stephan, C. C., Van Niekerk, A., and Wright, C. J.: Atmospheric Gravity Waves: Processes and Parameterization, J. Atmos. Sci., 81, 237–262, https://doi.org/10.1175/JAS-D-23-0210.1, 2024. a, b
Alexander, M. J. and Grimsdell, A. W.: Seasonal cycle of orographic gravity wave occurrence above small islands in the Southern Hemisphere: Implications for effects on the general circulation, J. Geophys. Res.-Atmos., 118, https://doi.org/10.1002/2013jd020526, 2013. a
Alexander, M. J., Geller, M., McLandress, C., Polavarapu, S., Preusse, P., Sassi, F., Sato, K., Eckermann, S., Ern, M., Hertzog, A., Kawatani, Y., Pulido, M., Shaw, T. A., Sigmond, M., Vincent, R., and Watanabe, S.: Recent developments in gravity-wave effects in climatemodels and the global distribution of gravity-wavemomentum flux from observations and models, Q. J. Roy. Meteor. Soc., 136, 1103–1124, https://doi.org/10.1002/qj.637, 2010. a, b
Appenzeller, C., Holton, J. R., and Rosenlof, K. H.: Seasonal variation of mass transport across the tropopause, J. Geophys. Res.-Atmos., 101, 15071–15078, https://doi.org/10.1029/96jd00821, 1996. a
Berthet, G., Esler, J. G., and Haynes, P. H.: A Lagrangian perspective of the tropopause and the ventilation of the lowermost stratosphere, J. Geophys. Res.-Atmos., 112, https://doi.org/10.1029/2006jd008295, 2007. a
Birner, T.: Fine-scale structure of the extratropical tropopause region, J. Geophys. Res.-Atmos., 111, 1–14, https://doi.org/10.1029/2005JD006301, 2006. a
Birner, T., Dörnbrack, A., and Schumann, U.: How sharp is the tropopause at midlatitudes?, Geophys. Res. Lett., 29, 1–4, https://doi.org/10.1029/2002GL015142, 2002. a
Butterworth, S.: On the theory of filter amplifiers, Experimental Wireless and the Wireless Engineer, 7, 536–541, 1930. a
Chau, C. H., Hoor, P., and Tost, H.: Simulated mixing in the UTLS by small-scale turbulence using multi-scale chemistry-climate model MECO(n), Atmos. Chem. Phys., 25, 13123–13140, https://doi.org/10.5194/acp-25-13123-2025, 2025. a
Chau, C. H., Hoor, P., Kaiser, K., and Tost, H.: Parametrizing the mixing by clear air turbulence in the chemistry climate model EMAC and its respective radiative impact, Atmos. Chem. Phys., 26, 3637–3652, https://doi.org/10.5194/acp-26-3637-2026, 2026. a
Dörnbrack, A.: Transient Tropopause Waves, J. Atmos. Sci., 81, 1647–1668, https://doi.org/10.1175/jas-d-24-0037.1, 2024. a, b
Dörnbrack, A., Bechtold, P., and Schumann, U.: High‐Resolution Aircraft Observations of Turbulence and Waves in the Free Atmosphere and Comparison With Global Model Predictions, J. Geophys. Res.-Atmos., 127, https://doi.org/10.1029/2022jd036654, 2022. a, b
Dörnbrack, A., Lachnitt, H., Hoor, P., and Imazio, P. R.: Multiscale Dynamical Processes Shaping a Mixing Line, J. Geophys. Res.-Atmos., 130, https://doi.org/10.1029/2025jd043527, 2025. a, b
Durran, D. R.: Pseudomomentum Diagnostics for Two-Dimensional Stratified Compressible Flow, J. Atmos. Sci., 52, 3997–4009, https://doi.org/10.1175/1520-0469(1995)052<3997:PDFTDS>2.0.CO;2, 1995. a
Fritts, D. C. and Alexander, M. J.: Gravity wave dynamics and effects in the middle atmosphere, Rev. Geophys., 41, 1–64, https://doi.org/10.1029/2001RG000106, 2003. a, b, c, d
Geller, M. A., Alexander, M. J., Love, P. T., Bacmeister, J., Ern, M., Hertzog, A., Manzini, E., Preusse, P., Sato, K., Scaife, A. A., and Zhou, T.: A Comparison between Gravity Wave Momentum Fluxes in Observations and Climate Models, J. Climate, 26, 6383–6405, https://doi.org/10.1175/jcli-d-12-00545.1, 2013. a
Gomes, M. B., Shapiro, A., Parsons, D. B., and Gebauer, J. G.: Using a Numerical Model to Evaluate a Proposed Mechanism for Nocturnal Low-Level Jets and Ascent over a Warm Tongue, Mon. Weather Rev., 153, 1265–1281, https://doi.org/10.1175/mwr-d-24-0111.1, 2025. a
Guest, F. M., Reeder, M. J., Marks, C. J., and Karoly, D. J.: Inertia–Gravity Waves Observed in the Lower Stratosphere over Macquarie Island, J. Atmos. Sci., 57, 737–752, https://doi.org/10.1175/1520-0469(2000)057<0737:igwoit>2.0.co;2, 2000. a
Gultepe, I., Sharman, R., Williams, P. D., Zhou, B., Ellrod, G., Minnis, P., Trier, S., Griffin, S., Yum, S. S., Gharabaghi, B., Feltz, W., Temimi, M., Pu, Z., Storer, L. N., Kneringer, P., Weston, M. J., Chuang, H.-Y., Thobois, L., Dimri, A. P., Dietz, S. J., França, G. B., Almeida, M. V., and Neto, F. L. A.: A Review of High Impact Weather for Aviation Meteorology, Pure Appl. Geophys., 176, 1869–1921, https://doi.org/10.1007/s00024-019-02168-6, 2019. a
Gupta, A., Birner, T., Dörnbrack, A., and Polichtchouk, I.: Importance of Gravity Wave Forcing for Springtime Southern Polar Vortex Breakdown as Revealed by ERA5, Geophys. Res. Lett., 48, https://doi.org/10.1029/2021GL092762, 2021. a
Gupta, A., Sheshadri, A., Alexander, M. J., and Birner, T.: Insights on Lateral Gravity Wave Propagation in the Extratropical Stratosphere From 44 Years of ERA5 Data, Geophys. Res. Lett., 51, https://doi.org/10.1029/2024gl108541, 2024. a
Hegglin, M. I., Boone, C. D., Manney, G. L., and Walker, K. A.: A global view of the extratropical tropopause transition layer from Atmospheric Chemistry Experiment Fourier Transform Spectrometer O3, H2O, and CO, J. Geophys. Res.-Atmos., 114, 1–18, https://doi.org/10.1029/2008JD009984, 2009. a
Heller, R., Voigt, C., Beaton, S., Dörnbrack, A., Giez, A., Kaufmann, S., Mallaun, C., Schlager, H., Wagner, J., Young, K., and Rapp, M.: Mountain waves modulate the water vapor distribution in the UTLS, Atmos. Chem. Phys., 17, 14853–14869, https://doi.org/10.5194/acp-17-14853-2017, 2017. a
Hersbach, H., Bell, B., Berrisford, P., Hirahara, S., Horányi, A., Muñoz‐Sabater, J., Nicolas, J., Peubey, C., Radu, R., Schepers, D., Simmons, A., Soci, C., Abdalla, S., Abellan, X., Balsamo, G., Bechtold, P., Biavati, G., Bidlot, J., Bonavita, M., De Chiara, G., Dahlgren, P., Dee, D., Diamantakis, M., Dragani, R., Flemming, J., Forbes, R., Fuentes, M., Geer, A., Haimberger, L., Healy, S., Hogan, R.J., Hólm, E., Janisková, M., Keeley, S., Laloyaux, P., Lopez, P., Lupu, C., Radnoti, G., de Rosnay, P., Rozum, I., Vamborg, F., Villaume, S., and Thépaut, J.-N.: Complete ERA5 from 1940: Fifth generation of ECMWF atmospheric reanalyses of the global climate, Copernicus Climate Change Service (C3S) Data Store (CDS) [data set], https://doi.org/10.24381/cds.143582cf, 2017. a
Hersbach, H., Bell, B., Berrisford, P., Hirahara, S., Horányi, A., Muñoz‐Sabater, J., Nicolas, J., Peubey, C., Radu, R., Schepers, D., Simmons, A., Soci, C., Abdalla, S., Abellan, X., Balsamo, G., Bechtold, P., Biavati, G., Bidlot, J., Bonavita, M., De Chiara, G., Dahlgren, P., Dee, D., Diamantakis, M., Dragani, R., Flemming, J., Forbes, R., Fuentes, M., Geer, A., Haimberger, L., Healy, S., Hogan, R. J., Hólm, E., Janisková, M., Keeley, S., Laloyaux, P., Lopez, P., Lupu, C., Radnoti, G., de Rosnay, P., Rozum, I., Vamborg, F., Villaume, S., and Thépaut, J.: The ERA5 global reanalysis, Q. J. Roy. Meteor. Soc., 146, 1999–2049, https://doi.org/10.1002/qj.3803, 2020. a
Holt, L. A., Alexander, M. J., Coy, L., Liu, C., Molod, A., Putman, W., and Pawson, S.: An evaluation of gravity waves and gravity wave sources in the Southern Hemisphere in a 7 km global climate simulation, Q. J. Roy. Meteor. Soc., 143, 2481–2495, https://doi.org/10.1002/qj.3101, 2017. a
Holton, J. R., Haynes, P. H., McIntyre, M. E., Douglass, A. R., Rood, R. B., and Pfister, L.: Stratosphere‐troposphere exchange, Rev. Geophys., 33, 403–439, https://doi.org/10.1029/95RG02097, 1995. a, b
Hooke, W. H.: Gravity Waves, p. 272–288, American Meteorological Society, ISBN 9781935704201, https://doi.org/10.1007/978-1-935704-20-1_12, 1986. a
Hoor, P., Gurk, C., Brunner, D., Hegglin, M. I., Wernli, H., and Fischer, H.: Seasonality and extent of extratropical TST derived from in-situ CO measurements during SPURT, Atmos. Chem. Phys., 4, 1427–1442, https://doi.org/10.5194/acp-4-1427-2004, 2004. a, b, c
Hoor, P., Wernli, H., Hegglin, M. I., and Bönisch, H.: Transport timescales and tracer properties in the extratropical UTLS, Atmos. Chem. Phys., 10, 7929–7944, https://doi.org/10.5194/acp-10-7929-2010, 2010. a
Jaeger, E. B. and Sprenger, M.: A Northern Hemispheric climatology of indices for clear air turbulence in the tropopause region derived from ERA40 reanalysis data, J. Geophys. Res.-Atmos., 112, 1–13, https://doi.org/10.1029/2006JD008189, 2007. a
Jewtoukoff, V., Hertzog, A., Plougonven, R., Cámara, A. D. L., and Lott, F.: Comparison of Gravity Waves in the Southern Hemisphere Derived from Balloon Observations and the ECMWF Analyses, J. Atmos. Sci., 72, 3449–3468, https://doi.org/10.1175/jas-d-14-0324.1, 2015. a, b
Jovanovic, G.: Gravity waves as a mechanism of troposphere–stratosphere–mesosphere coupling during sudden stratospheric warming, Atmos. Chem. Phys., 25, 2979–2988, https://doi.org/10.5194/acp-25-2979-2025, 2025. a
Kaluza, T., Kunkel, D., and Hoor, P.: Composite analysis of the tropopause inversion layer in extratropical baroclinic waves, Atmos. Chem. Phys., 19, 6621–6636, https://doi.org/10.5194/acp-19-6621-2019, 2019. a, b
Kaluza, T., Kunkel, D., and Hoor, P.: Analysis of Turbulence Reports and ERA5 Turbulence Diagnostics in a Tropopause‐Based Vertical Framework, Geophys. Res. Lett., 49, https://doi.org/10.1029/2022gl100036, 2022. a
Kim, J.-H. and Chun, H.-Y.: Statistics and Possible Sources of Aviation Turbulence over South Korea, J. Appl. Meteorol. Clim., 50, 311–324, https://doi.org/10.1175/2010jamc2492.1, 2011. a
Kim, J.-H., Sharman, R., Strahan, M., Scheck, J. W., Bartholomew, C., Cheung, J. C. H., Buchanan, P., and Gait, N.: Improvements in Nonconvective Aviation Turbulence Prediction for the World Area Forecast System, B. Am. Meteorol. Soc., 99, 2295–2311, https://doi.org/10.1175/bams-d-17-0117.1, 2018. a
Kim, Y., Eckermann, S. D., and Chun, H.: An overview of the past, present and future of gravity‐wave drag parametrization for numerical climate and weather prediction models, Atmosphere-Ocean, 41, 65–98, https://doi.org/10.3137/ao.410105, 2003. a
Knox, J. A.: Possible Mechanisms of Clear-Air Turbulence in Strongly Anticyclonic Flows, Mon. Weather Rev., 125, 1251–1259, https://doi.org/10.1175/1520-0493(1997)125<1251:pmocat>2.0.co;2, 1997. a
Koch, S. E., Jamison, B. D., Lu, C., Smith, T. L., Tollerud, E. I., Girz, C., Wang, N., Lane, T. P., Shapiro, M. A., Parrish, D. D., and Cooper, O. R.: Turbulence and Gravity Waves within an Upper-Level Front, J. Atmos. Sci., 62, 3885–3908, https://doi.org/10.1175/jas3574.1, 2005. a
Krautstrunk, M. and Giez, A.: The Transition From FALCON to HALO Era Airborne Atmospheric Research, Springer Berlin Heidelberg, 609–624, ISBN 9783642301834, https://doi.org/10.1007/978-3-642-30183-4_37, 2012. a
Kruse, C. G. and Smith, R. B.: Gravity Wave Diagnostics and Characteristics in Mesoscale Fields, J. Atmos. Sci., 72, 4372–4392, https://doi.org/10.1175/jas-d-15-0079.1, 2015. a
Kruse, C. G., Alexander, M. J., Hoffmann, L., van Niekerk, A., Polichtchouk, I., Bacmeister, J. T., Holt, L., Plougonven, R., Šácha, P., Wright, C., Sato, K., Shibuya, R., Gisinger, S., Ern, M., Meyer, C. I., and Stein, O.: Observed and Modeled Mountain Waves from the Surface to the Mesosphere near the Drake Passage, J. Atmos. Sci., 79, 909–932, https://doi.org/10.1175/jas-d-21-0252.1, 2022. a
Kunkel, D., Hoor, P., and Wirth, V.: Can inertia-gravity waves persistently alter the tropopause inversion layer?, Geophys. Res. Lett., 41, 7822–7829, https://doi.org/10.1002/2014GL061970, 2014. a, b, c, d
Kunkel, D., Hoor, P., and Wirth, V.: The tropopause inversion layer in baroclinic life-cycle experiments: the role of diabatic processes, Atmos. Chem. Phys., 16, 541–560, https://doi.org/10.5194/acp-16-541-2016, 2016. a
Kunkel, D., Hoor, P., Kaluza, T., Ungermann, J., Kluschat, B., Giez, A., Lachnitt, H.-C., Kaufmann, M., and Riese, M.: Evidence of small-scale quasi-isentropic mixing in ridges of extratropical baroclinic waves, Atmos. Chem. Phys., 19, 12607–12630, https://doi.org/10.5194/acp-19-12607-2019, 2019. a, b, c, d, e, f, g, h, i, j
Lachnitt, H. C.: Consistent meteorological (ERA5) and chemical (CLaMS) information across airborne measurements over the globe between 1997 and 2023, Zenodo [data set], https://doi.org/10.5281/zenodo.15076520, (last access: 08 September 2025), 2025. a
Lane, T. P. and Sharman, R. D.: Gravity wave breaking, secondary wave generation, and mixing above deep convection in a three‐dimensional cloud model, Geophys. Res. Lett., 33, https://doi.org/10.1029/2006gl027988, 2006. a, b
Lane, T. P., Reeder, M. J., and Clark, T. L.: Numerical Modeling of Gravity Wave Generation by Deep Tropical Convection, J. Atmos. Sci., 58, 1249–1274, https://doi.org/10.1175/1520-0469(2001)058<1249:nmogwg>2.0.co;2, 2001. a
Lane, T. P., Doyle, J. D., Plougonven, R., Shapiro, M. A., and Sharman, R. D.: Observations and Numerical Simulations of Inertia–Gravity Waves and Shearing Instabilities in the Vicinity of a Jet Stream, J. Atmos. Sci., 61, 2692–2706, https://doi.org/10.1175/jas3305.1, 2004. a, b, c
Lee, D.-B., Chun, H.-Y., and Kim, J.-H.: Evaluation of Multimodel-Based Ensemble Forecasts for Clear-Air Turbulence, Weather Forecast., 35, 507–521, https://doi.org/10.1175/waf-d-19-0155.1, 2019. a
Lee, J. H., Kim, J., Sharman, R. D., Kim, J., and Son, S.: Climatology of Clear‐Air Turbulence in Upper Troposphere and Lower Stratosphere in the Northern Hemisphere Using ERA5 Reanalysis Data, J. Geophys. Res.-Atmos., 128, https://doi.org/10.1029/2022jd037679, 2022. a
Lehmann, C. I., Kim, Y.-H., Preusse, P., Chun, H.-Y., Ern, M., and Kim, S.-Y.: Consistency between Fourier transform and small-volume few-wave decomposition for spectral and spatial variability of gravity waves above a typhoon, Atmos. Meas. Tech., 5, 1637–1651, https://doi.org/10.5194/amt-5-1637-2012, 2012. a
Lott, F. and Miller, M. J.: A new subgrid‐scale orographic drag parametrization: Its formulation and testing, Q. J. Roy. Meteor. Soc., 123, 101–127, https://doi.org/10.1002/qj.49712353704, 1997. a
Müller, S., Hoor, P., Berkes, F., Bozem, H., Klingebiel, M., Reutter, P., Smit, H. G. J., Wendisch, M., Spichtinger, P., and Borrmann, S.: In situ detection of stratosphere‐troposphere exchange of cirrus particles in the midlatitudes, Geophys. Res. Lett., 42, 949–955, https://doi.org/10.1002/2014gl062556, 2015. a
Olsen, M. A., Douglass, A. R., and Kaplan, T. B.: Variability of extratropical ozone stratosphere–troposphere exchange using microwave limb sounder observations, J. Geophys. Res.-Atmos., 118, 1090–1099, https://doi.org/10.1029/2012jd018465, 2013. a
Orr, A., Bechtold, P., Scinocca, J., Ern, M., and Janiskova, M.: Improved middle atmosphere climate and forecasts in the ECMWF model through a non-orographic gravity wave drag parametrization, ECMWF, https://doi.org/10.21957/DM64CMPJ, 2010. a
O'Sullivan, D. and Dunkerton, T. J.: Generation of Inertia–Gravity Waves in a Simulated Life Cycle of Baroclinic Instability, J. Atmos. Sci., 52, 3695–3716, https://doi.org/10.1175/1520-0469(1995)052<3695:GOIWIA>2.0.CO;2, 1995. a
Pan, L. L., Randel, W. J., Gary, B. L., Mahoney, M. J., and Hintsa, E. J.: Definitions and sharpness of the extratropical tropopause: A trace gas perspective, J. Geophys. Res.-Atmos., 109, https://doi.org/10.1029/2004jd004982, 2004. a
Pan, L. L., Konopka, P., and Browell, E. V.: Observations and model simulations of mixing near the extratropical tropopause, J. Geophys. Res.-Atmos., 111, 1–15, https://doi.org/10.1029/2005JD006480, 2006. a
Plougonven, R. and Snyder, C.: Gravity waves excited by jets: Propagation versus generation, Geophys. Res. Lett., 32, https://doi.org/10.1029/2005gl023730, 2005. a
Plougonven, R. and Zhang, F.: Internal gravity waves from atmospheric jets and fronts, Rev. Geophys., 52, 33–76, https://doi.org/10.1002/2012rg000419, 2014. a, b
Plougonven, R., Teitelbaum, H., and Zeitlin, V.: Inertia gravity wave generation by the tropospheric midlatitude jet as given by the Fronts and Atlantic Storm-Track Experiment radio soundings, J. Geophys. Res.-Atmos., 108, https://doi.org/10.1029/2003jd003535, 2003. a, b, c
Plougonven, R., Hertzog, A., and Teitelbaum, H.: Observations and simulations of a large-amplitude mountain wave breaking over the Antarctic Peninsula, J. Geophys. Res.-Atmos., 113, 1–17, https://doi.org/10.1029/2007JD009739, 2008. a, b
Plougonven, R., Hertzog, A., and Alexander, M. J.: Case studies of nonorographic gravity waves over the Southern Ocean emphasize the role of moisture, J. Geophys. Res.-Atmos., 120, 1278–1299, https://doi.org/10.1002/2014jd022332, 2015. a
Plougonven, R., Jewtoukoff, V., Cámara, A. d. l., Lott, F., and Hertzog, A.: On the Relation between Gravity Waves and Wind Speed in the Lower Stratosphere over the Southern Ocean, J. Atmos. Sci., 74, 1075–1093, https://doi.org/10.1175/jas-d-16-0096.1, 2017. a
Polichtchouk, I., van Niekerk, A., and Wedi, N.: Resolved Gravity Waves in the Extratropical Stratosphere: Effect of Horizontal Resolution Increase from O(10) to O(1) km, J. Atmos. Sci., 80, 473–486, https://doi.org/10.1175/jas-d-22-0138.1, 2023. a
Rapp, M., Kaifler, B., Dörnbrack, A., Gisinger, S., Mixa, T., Reichert, R., Kaifler, N., Knobloch, S., Eckert, R., Wildmann, N., Giez, A., Krasauskas, L., Preusse, P., Geldenhuys, M., Riese, M., Woiwode, W., Friedl-Vallon, F., Sinnhuber, B.-M., Torre, A. d. l., Alexander, P., Hormaechea, J. L., Janches, D., Garhammer, M., Chau, J. L., Conte, J. F., Hoor, P., and Engel, A.: SOUTHTRAC-GW: An Airborne Field Campaign to Explore Gravity Wave Dynamics at the World’s Strongest Hotspot, B. Am. Meteorol. Soc., 102, E871–E893, https://doi.org/10.1175/bams-d-20-0034.1, 2021. a
Raschendorfer, M.: The new turbulence parameterization of LM, COSMO Newsletter, 1, 89–97, http://www.cosmo-model.org (last access: 8 April 2026), 2001. a
Riese, M., Ploeger, F., Rap, A., Vogel, B., Konopka, P., Dameris, M., and Forster, P.: Impact of uncertainties in atmospheric mixing on simulated UTLS composition and related radiative effects, J. Geophys. Res.-Atmos., 117, https://doi.org/10.1029/2012jd017751, 2012. a, b
Schwenk, C. and Miltenberger, A.: The role of ascent timescales for warm conveyor belt (WCB) moisture transport into the upper troposphere and lower stratosphere (UTLS), Atmos. Chem. Phys., 24, 14073–14099, https://doi.org/10.5194/acp-24-14073-2024, 2024. a, b
Seifert, A.: On the parameterization of evaporation of raindrops as simulated by a one-dimensional rainshaft model, J. Atmos. Sci., 65, 3608–3619, https://doi.org/10.1175/2008JAS2586.1, 2008. a
Shapiro, M. A.: Further Evidence of the Mesoscale and Turbulent Structure of Upper Level Jet Stream–Frontal Zone Systems, Mon. Weather Rev., 106, 1100–1111, https://doi.org/10.1175/1520-0493(1978)106<1100:feotma>2.0.co;2, 1978. a
Shapiro, M. A.: Turbulent Mixing within Tropopause Folds as a Mechanism for the Exchange of Chemical Constituents between the Stratosphere and Troposphere, J. Atmos. Sci., 37, 994–1004, https://doi.org/10.1175/1520-0469(1980)037<0994:tmwtfa>2.0.co;2, 1980. a
Sharman, R., Tebaldi, C., Wiener, G., and Wolff, J.: An Integrated Approach to Mid- and Upper-Level Turbulence Forecasting, Weather Forecast., 21, 268–287, https://doi.org/10.1175/waf924.1, 2006. a, b, c, d
Sharman, R. D. and Pearson, J. M.: Prediction of Energy Dissipation Rates for Aviation Turbulence. Part I: Forecasting Nonconvective Turbulence, J. Appl. Meteorol. Clim., 56, 317–337, https://doi.org/10.1175/jamc-d-16-0205.1, 2017. a, b, c
Sharman, R. D., Trier, S. B., Lane, T. P., and Doyle, J. D.: Sources and dynamics of turbulence in the upper troposphere and lower stratosphere: A review, Geophys. Res. Lett., 39, 1–9, https://doi.org/10.1029/2012GL051996, 2012. a
Sharman, R. D., Cornman, L. B., Meymaris, G., Pearson, J., and Farrar, T.: Description and Derived Climatologies of Automated In Situ Eddy-Dissipation-Rate Reports of Atmospheric Turbulence, J. Appl. Meteorol. Clim., 53, 1416–1432, https://doi.org/10.1175/jamc-d-13-0329.1, 2014. a
Stephan, C. C., Strube, C., Klocke, D., Ern, M., Hoffmann, L., Preusse, P., and Schmidt, H.: Intercomparison of Gravity Waves in Global Convection-Permitting Models, J. Atmos. Sci., 76, 2739–2759, https://doi.org/10.1175/jas-d-19-0040.1, 2019a. a, b
Stephan, C. C., Strube, C., Klocke, D., Ern, M., Hoffmann, L., Preusse, P., and Schmidt, H.: Gravity Waves in Global High‐Resolution Simulations With Explicit and Parameterized Convection, J. Geophys. Res.-Atmos., 124, 4446–4459, https://doi.org/10.1029/2018jd030073, 2019b. a
Strube, C., Ern, M., Preusse, P., and Riese, M.: Removing spurious inertial instability signals from gravity wave temperature perturbations using spectral filtering methods, Atmos. Meas. Tech., 13, 4927–4945, https://doi.org/10.5194/amt-13-4927-2020, 2020. a
Thompson, C. F. and Schultz, D. M.: The Release of Inertial Instability Near an Idealized Zonal Jet, Geophys. Res. Lett., 48, https://doi.org/10.1029/2021gl092649, 2021. a, b, c, d
Toghraei, I., Lott, F., Köhler, L., Stephan, C. C., and Alexander, M. J.: Can Parameterizations Reproduce the Gravity Wave Momentum Fluxes and Drag Simulated by a Global High‐Resolution Model?, Geophys. Res. Lett., 52, https://doi.org/10.1029/2025gl115499, 2025. a
Trier, S. B., Sharman, R. D., MuñOz-Esparza, D., and Lane, T. P.: Environment and mechanisms of severe turbulence in a midlatitude cyclone, J. Atmos. Sci., 77, 3869–3889, https://doi.org/10.1175/JAS-D-20-0095.1, 2020. a, b
Umbarkar, M.: Data used for paper “Evidence of gravity wave contribution to vertical shear and mixing in the lower stratosphere: a WISE case study”, Zenodo [data set], https://doi.org/10.5281/zenodo.17227439, 2025. a
Wang, M. and Fu, Q.: Stratosphere‐Troposphere Exchange of Air Masses and Ozone Concentrations Based on Reanalyses and Observations, J. Geophys. Res.-Atmos., 126, https://doi.org/10.1029/2021jd035159, 2021. a
Wang, S. and Zhang, F.: Sensitivity of Mesoscale Gravity Waves to the Baroclinicity of Jet-Front Systems, Mon. Weather Rev., 135, 670–688, https://doi.org/10.1175/mwr3314.1, 2007. a
Wei, J. and Zhang, F.: Mesoscale gravity waves in moist baroclinic jet-front systems, J. Atmos. Sci., 71, 929–952, https://doi.org/10.1175/JAS-D-13-0171.1, 2014. a
Wei, J., Zhang, F., and Richter, J. H.: An Analysis of Gravity Wave Spectral Characteristics in Moist Baroclinic Jet–Front Systems, J. Atmos. Sci., 73, 3133–3155, https://doi.org/10.1175/jas-d-15-0316.1, 2016. a
Wei, J., Zhang, F., Richter, J. H., Alexander, M. J., and Sun, Y. Q.: Global Distributions of Tropospheric and Stratospheric Gravity Wave Momentum Fluxes Resolved by the 9-km ECMWF Experiments, J. Atmos. Sci., 79, 2621–2644, https://doi.org/10.1175/jas-d-21-0173.1, 2022. a, b, c, d
Weyland, F., Hoor, P., Kunkel, D., Birner, T., Plöger, F., and Turhal, K.: Long-term changes in the thermodynamic structure of the lowermost stratosphere inferred from reanalysis data, Atmos. Chem. Phys., 25, 1227–1252, https://doi.org/10.5194/acp-25-1227-2025, 2025. a
Whiteway, J. A., Pavelin, E. G., Busen, R., Hacker, J., and Vosper, S.: Airborne measurements of gravity wave breaking at the tropopause, Geophys. Res. Lett., 30, 2–6, https://doi.org/10.1029/2003GL018207, 2003. a
Whiteway, J. A., Klaassen, G. P., Bradshaw, N. G., and Hacker, J.: Transition to turbulence in shear above the tropopause, Geophys. Res. Lett., 31, 2–5, https://doi.org/10.1029/2003GL018509, 2004. a
Yoshida, L., Tomikawa, Y., Ejiri, M. K., Tsutsumi, M., Kohma, M., and Sato, K.: Large‐Amplitude Inertia Gravity Waves Over Syowa Station: Comparison of PANSY Radar and ERA5 Reanalysis Data, J. Geophys. Res.-Atmos., 129, https://doi.org/10.1029/2023jd040490, 2024. a
Zängl, G., Reinert, D., Rípodas, P., and Baldauf, M.: The <scp>ICON</scp> (ICOsahedral Non‐hydrostatic) modelling framework of <scp>DWD</scp> and <scp>MPI‐M</scp>: Description of the non‐hydrostatic dynamical core, Q. J. Roy. Meteor. Soc., 141, 563–579, https://doi.org/10.1002/qj.2378, 2014. a
Zhang, F., Davis, C. A., Kaplan, M. L., and Koch, S. E.: Wavelet analysis and the governing dynamics of a large‐amplitude mesoscale gravity‐wave event along the East Coast of the United States, Q. J. Roy. Meteor. Soc., 127, 2209–2245, https://doi.org/10.1002/qj.49712757702, 2001. a
Zhang, F., Wei, J., Zhang, M., Bowman, K. P., Pan, L. L., Atlas, E., and Wofsy, S. C.: Aircraft measurements of gravity waves in the upper troposphere and lower stratosphere during the START08 field experiment, Atmos. Chem. Phys., 15, 7667–7684, https://doi.org/10.5194/acp-15-7667-2015, 2015a. a, b
Zhang, W., Peng, J., Zhang, W., Wang, S., Li, Z., and Hanyan, W.: Sensitivity of Gravity Wave Momentum Flux Estimates on Separation Methods, Mon. Weather Rev., 153, 1721–1742, https://doi.org/10.1175/mwr-d-24-0272.1, 2025. a, b, c
Zhang, Y., Zhang, S., Huang, C., Huang, K., Gong, Y., and Gan, Q.: The interaction between the tropopause inversion layer and the inertial gravity wave activities revealed by radiosonde observations at a midlatitude station, J. Geophys. Res.-Atmos., 120, 8099–8111, https://doi.org/10.1002/2015jd023115, 2015b. a, b, c
Zhang, Y., Zhang, S., Huang, C., Huang, K., and Gong, Y.: The Tropopause Inversion Layer Interaction With the Inertial Gravity Wave Activities and Its Latitudinal Variability, J. Geophys. Res.-Atmos., 124, 7512–7522, https://doi.org/10.1029/2019JD030309, 2019. a
Zülicke, C. and Peters, D.: Simulation of inertia-gravity waves in a poleward-breaking Rossby wave, J. Atmos. Sci., 63, 3253–3276, https://doi.org/10.1175/JAS3805.1, 2006. a
Short summary
We present an extratropical cyclone case study over the North Atlantic focusing on the role of atmospheric gravity waves (GW) in the generation of strong vertical shear and (clear-air) turbulence (CAT), as well as their impact on tracer distribution in the lowermost stratosphere. Our findings suggest that GW related processes should be considered as a key for upper troposphere lower stratosphere (UTLS) transport and mixing, and as an important candidate for the interpretation of CAT in the UTLS.
We present an extratropical cyclone case study over the North Atlantic focusing on the role of...
Altmetrics
Final-revised paper
Preprint