Articles | Volume 24, issue 14
https://doi.org/10.5194/acp-24-8363-2024
https://doi.org/10.5194/acp-24-8363-2024
Research article
 | 
25 Jul 2024
Research article |  | 25 Jul 2024

Source-resolved atmospheric metal emissions, concentrations, and deposition fluxes into the East Asian seas

Shenglan Jiang, Yan Zhang, Guangyuan Yu, Zimin Han, Junri Zhao, Tianle Zhang, and Mei Zheng

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This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Cited articles

Alexander, B., Park, R. J., Jacob, D. J., and Gong, S.: Transition metal-catalyzed oxidation of atmospheric sulfur: Global implications for the sulfur budget, J. Geophys. Res.-Atmos., 114, D02309, https://doi.org/10.1029/2008JD010486, 2009. 
Amedro, D., Berasategui, M., Bunkan, A. J. C., Pozzer, A., Lelieveld, J., and Crowley, J. N.: Kinetics of the OH+NO2 reaction: effect of water vapour and new parameterization for global modelling, Atmos. Chem. Phys., 20, 3091–3105, https://doi.org/10.5194/acp-20-3091-2020, 2020. 
Bai, X., Luo, L., Tian, H., Liu, S., Hao, Y., Zhao, S., Lin, S., Zhu, C., Guo, Z., and Lv, Y.: Atmospheric Vanadium Emission Inventory from Both Anthropogenic and Natural Sources in China, Environ. Sci. Technol., 55, 11568–11578, https://doi.org/10.1021/acs.est.1c04766, 2021. 
Baker, A. R. and Jickells, T. D.: Atmospheric deposition of soluble trace elements along the Atlantic Meridional Transect (AMT), Prog. Oceanogr., 158, 41–51, https://doi.org/10.1016/j.pocean.2016.10.002, 2017. 
Baker, A. R., Li, M., and Chance, R.: Trace Metal Fractional Solubility in Size-Segregated Aerosols From the Tropical Eastern Atlantic Ocean, Global Biogeochem. Cy., 34, e2019GB006510, https://doi.org/10.1029/2019GB006510, 2020. 
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This study aims to provide gridded data on sea-wide concentrations, deposition fluxes, and soluble deposition fluxes with detailed source categories of metals using the modified CMAQ model. We developed a monthly emission inventory of six metals – Fe, Al, V, Ni, Zn, and Cu – from terrestrial anthropogenic, ship, and dust sources in East Asia in 2017. Our results reveal the contribution of each source to the emissions, concentrations, and deposition fluxes of metals in the East Asian seas.
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