Articles | Volume 23, issue 2
https://doi.org/10.5194/acp-23-1147-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-1147-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Measurement report
| 
23 Jan 2023
Measurement report |
| 23 Jan 2023
| 23 Jan 2023
Measurement report: Intensive biomass burning emissions and rapid nitrate formation drive severe haze formation in the Sichuan Basin, China – insights from aerosol mass spectrometry
Zhier Bao
Chongqing Institute of Green and Intelligent Technology, Chinese
Academy of Sciences, Chongqing, 400714, China
Xinyi Zhang
Chongqing Institute of Green and Intelligent Technology, Chinese
Academy of Sciences, Chongqing, 400714, China
Qing Li
Chongqing Institute of Green and Intelligent Technology, Chinese
Academy of Sciences, Chongqing, 400714, China
Jiawei Zhou
Chongqing Institute of Green and Intelligent Technology, Chinese
Academy of Sciences, Chongqing, 400714, China
Guangming Shi
Department of Environmental Science and Engineering, College of
Architecture and Environment, Sichuan University, Chengdu 610065, China
Li Zhou
Department of Environmental Science and Engineering, College of
Architecture and Environment, Sichuan University, Chengdu 610065, China
Fumo Yang
Department of Environmental Science and Engineering, College of
Architecture and Environment, Sichuan University, Chengdu 610065, China
Shaodong Xie
SKL-ESPC and BIC-ESAT, College of Environmental Sciences and
Engineering, Peking University, Beijing 100871, China
Dan Zhang
Research Center for Atmospheric Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 400714, China
Chongzhi Zhai
Research Center for Atmospheric Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 400714, China
Zhenliang Li
Research Center for Atmospheric Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 400714, China
Chao Peng
Research Center for Atmospheric Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 400714, China
Chongqing Institute of Green and Intelligent Technology, Chinese
Academy of Sciences, Chongqing, 400714, China
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Action Plan for the Prevention and Control of Air Pollution.
Jingsha Xu, Shaojie Song, Roy M. Harrison, Congbo Song, Lianfang Wei, Qiang Zhang, Yele Sun, Lu Lei, Chao Zhang, Xiaohong Yao, Dihui Chen, Weijun Li, Miaomiao Wu, Hezhong Tian, Lining Luo, Shengrui Tong, Weiran Li, Junling Wang, Guoliang Shi, Yanqi Huangfu, Yingze Tian, Baozhu Ge, Shaoli Su, Chao Peng, Yang Chen, Fumo Yang, Aleksandra Mihajlidi-Zelić, Dragana Đorđević, Stefan J. Swift, Imogen Andrews, Jacqueline F. Hamilton, Ye Sun, Agung Kramawijaya, Jinxiu Han, Supattarachai Saksakulkrai, Clarissa Baldo, Siqi Hou, Feixue Zheng, Kaspar R. Daellenbach, Chao Yan, Yongchun Liu, Markku Kulmala, Pingqing Fu, and Zongbo Shi
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An interlaboratory comparison was conducted for the first time to examine differences in water-soluble inorganic ions (WSIIs) measured by 10 labs using ion chromatography (IC) and by two online aerosol chemical speciation monitor (ACSM) methods. Major ions including SO42−, NO3− and NH4+ agreed well in 10 IC labs and correlated well with ACSM data. WSII interlab variability strongly affected aerosol acidity results based on ion balance, but aerosol pH computed by ISORROPIA II was very similar.
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Short summary
We characterised non-refractory fine particulate matter (PM2.5) during winter in the Sichuan Basin (SCB), Southwest China. The factors driving severe aerosol pollution were revealed, highlighting the importance of rapid nitrate formation and intensive biomass burning. Nitrate was primarily formed through gas-phase oxidation during daytime and aqueous-phase oxidation during nighttime. Controlling nitrate and biomass burning will benefit the mitigation of haze formation in the SCB.
We characterised non-refractory fine particulate matter (PM2.5) during winter in the Sichuan...
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