Articles | Volume 22, issue 11
https://doi.org/10.5194/acp-22-7681-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-7681-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Measurement report
| 
14 Jun 2022
Measurement report |
| 14 Jun 2022
| 14 Jun 2022
Measurement report: Spectral and statistical analysis of aerosol hygroscopic growth from multi-wavelength lidar measurements in Barcelona, Spain
CommSensLab, Dept. of Signal Theory and Communications, Universitat
Politècnica de Catalunya (UPC), 08034 Barcelona, Spain
Ciències i Tecnologies de l'Espai-Centre de Recerca de
l'Aeronàutica i de l'Espai/Institut d'Estudis Espacials de Catalunya
(CTE-CRAE/IEEC), Universitat Politècnica de Catalunya (UPC),
08034 Barcelona, Spain
Daniel Camilo Fortunato dos Santos Oliveira
CommSensLab, Dept. of Signal Theory and Communications, Universitat
Politècnica de Catalunya (UPC), 08034 Barcelona, Spain
Constantino Muñoz-Porcar
CommSensLab, Dept. of Signal Theory and Communications, Universitat
Politècnica de Catalunya (UPC), 08034 Barcelona, Spain
Cristina Gil-Díaz
CommSensLab, Dept. of Signal Theory and Communications, Universitat
Politècnica de Catalunya (UPC), 08034 Barcelona, Spain
Adolfo Comerón
CommSensLab, Dept. of Signal Theory and Communications, Universitat
Politècnica de Catalunya (UPC), 08034 Barcelona, Spain
Alejandro Rodríguez-Gómez
CommSensLab, Dept. of Signal Theory and Communications, Universitat
Politècnica de Catalunya (UPC), 08034 Barcelona, Spain
Federico Dios Otín
CommSensLab, Dept. of Signal Theory and Communications, Universitat
Politècnica de Catalunya (UPC), 08034 Barcelona, Spain
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Cristina Gil-Díaz, Michäel Sicard, Adolfo Comerón, Daniel Camilo Fortunato dos Santos Oliveira, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Jasper R. Lewis, Ellsworth J. Welton, and Simone Lolli
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Tristan Millet, Hassan Bencherif, Thierry Portafaix, Nelson Bègue, Alexandre Baron, Valentin Duflot, Michaël Sicard, Jean-Marc Metzger, Guillaume Payen, Nicolas Marquestaut, and Sophie Godin-Beekmann
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Preprint withdrawn
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The eruption of the Hunga Tonga volcano in January 2022 released substantial amounts of aerosols, sulfur dioxide, and water vapor into the stratosphere. Satellite and ground instruments followed the displacement of the volcanic aerosol plume and its impact on ozone levels over the Indian Ocean. Ozone data reveal the presence of a persistent ozone mini-hole structure from 17 January to 22 January, with most ozone depletion occurring within the ozone layer at the location of the aerosol plume.
Simone Lolli, Michaël Sicard, Francesco Amato, Adolfo Comeron, Cristina Gíl-Diaz, Tony C. Landi, Constantino Munoz-Porcar, Daniel Oliveira, Federico Dios Otin, Francesc Rocadenbosch, Alejandro Rodriguez-Gomez, Andrés Alastuey, Xavier Querol, and Cristina Reche
Atmos. Chem. Phys., 23, 12887–12906, https://doi.org/10.5194/acp-23-12887-2023, https://doi.org/10.5194/acp-23-12887-2023, 2023
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Adolfo Comerón, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Michaël Sicard, Federico Dios, Cristina Gil-Díaz, Daniel Camilo Fortunato dos Santos Oliveira, and Francesc Rocadenbosch
Atmos. Meas. Tech., 16, 3015–3025, https://doi.org/10.5194/amt-16-3015-2023, https://doi.org/10.5194/amt-16-3015-2023, 2023
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We derive an explicit (i.e., non-iterative) formula for the retrieval of the overlap function in an aerosol lidar with both elastic and Raman N2 and/or O2 channels used for independent measurements of aerosol backscatter and extinction coefficients. The formula requires only the measured, range-corrected elastic and the corresponding Raman signals, plus an assumed lidar ratio. We assess the influence of the lidar ratio error in the overlap function retrieval and present retrieval examples.
María Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Diego Bermejo-Pantaleón, Michaël Sicard, Vanda Salgueiro, Francisco Molero, Clara Violeta Carvajal-Pérez, María José Granados-Muñoz, Adolfo Comerón, Flavio T. Couto, Rubén Barragán, María-Paz Zorzano, Juan Antonio Bravo-Aranda, Constantino Muñoz-Porcar, María João Costa, Begoña Artíñano, Alejandro Rodríguez-Gómez, Daniele Bortoli, Manuel Pujadas, Jesús Abril-Gago, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 143–161, https://doi.org/10.5194/acp-23-143-2023, https://doi.org/10.5194/acp-23-143-2023, 2023
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An intense Saharan dust outbreak crossing the Iberian Peninsula in springtime was monitored to determinine the specific contribution of fine and coarse dust particles at five lidar stations, strategically covering its SW–central–NE pathway. Expected dust ageing along the transport started unappreciated. A different fine-dust impact on optical (~30 %) and mass (~10 %) properties was found. Use of polarized lidar measurements (mainly in elastic systems) for fine/coarse dust separation is crucial.
M. Dolores Andrés Hernández, Andreas Hilboll, Helmut Ziereis, Eric Förster, Ovid O. Krüger, Katharina Kaiser, Johannes Schneider, Francesca Barnaba, Mihalis Vrekoussis, Jörg Schmidt, Heidi Huntrieser, Anne-Marlene Blechschmidt, Midhun George, Vladyslav Nenakhov, Theresa Harlass, Bruna A. Holanda, Jennifer Wolf, Lisa Eirenschmalz, Marc Krebsbach, Mira L. Pöhlker, Anna B. Kalisz Hedegaard, Linlu Mei, Klaus Pfeilsticker, Yangzhuoran Liu, Ralf Koppmann, Hans Schlager, Birger Bohn, Ulrich Schumann, Andreas Richter, Benjamin Schreiner, Daniel Sauer, Robert Baumann, Mariano Mertens, Patrick Jöckel, Markus Kilian, Greta Stratmann, Christopher Pöhlker, Monica Campanelli, Marco Pandolfi, Michael Sicard, José L. Gómez-Amo, Manuel Pujadas, Katja Bigge, Flora Kluge, Anja Schwarz, Nikos Daskalakis, David Walter, Andreas Zahn, Ulrich Pöschl, Harald Bönisch, Stephan Borrmann, Ulrich Platt, and John P. Burrows
Atmos. Chem. Phys., 22, 5877–5924, https://doi.org/10.5194/acp-22-5877-2022, https://doi.org/10.5194/acp-22-5877-2022, 2022
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Michaël Sicard, Carmen Córdoba-Jabonero, María-Ángeles López-Cayuela, Albert Ansmann, Adolfo Comerón, María-Paz Zorzano, Alejandro Rodríguez-Gómez, and Constantino Muñoz-Porcar
Atmos. Chem. Phys., 22, 1921–1937, https://doi.org/10.5194/acp-22-1921-2022, https://doi.org/10.5194/acp-22-1921-2022, 2022
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This paper completes the companion paper of Córdoba-Jabonero et al. (2021). We estimate the total direct radiative effect produced by mineral dust particles during the June 2019 mega-heatwave at two sites in Spain and Germany. The results show that the dust particles in the atmosphere contribute to cooling the surface (less radiation reaches the surface) and that the heatwave (parametrized by high surface and air temperatures) contributes to reducing this cooling.
Jesús Abril-Gago, Juan Luis Guerrero-Rascado, Maria João Costa, Juan Antonio Bravo-Aranda, Michaël Sicard, Diego Bermejo-Pantaleón, Daniele Bortoli, María José Granados-Muñoz, Alejandro Rodríguez-Gómez, Constantino Muñoz-Porcar, Adolfo Comerón, Pablo Ortiz-Amezcua, Vanda Salgueiro, Marta María Jiménez-Martín, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 22, 1425–1451, https://doi.org/10.5194/acp-22-1425-2022, https://doi.org/10.5194/acp-22-1425-2022, 2022
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A validation of Aeolus reprocessed optical products is carried out via an intercomparison with ground-based measurements taken at several ACTRIS/EARLINET stations in western Europe. Case studies and a statistical analysis are presented. The stations are located in a hot spot between Africa and the rest of Europe, which guarantees a variety of aerosol types, from mineral dust layers to continental/anthropogenic aerosol, and allows us to test Aeolus performance under different scenarios.
Michaël Sicard, Oriol Jorba, Jiang Ji Ho, Rebeca Izquierdo, Concepción De Linares, Marta Alarcón, Adolfo Comerón, and Jordina Belmonte
Atmos. Chem. Phys., 21, 17807–17832, https://doi.org/10.5194/acp-21-17807-2021, https://doi.org/10.5194/acp-21-17807-2021, 2021
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This paper investigates the mechanisms involved in the dispersion, structure, and mixing in the vertical column of atmospheric pollen, using observations of pollen concentration obtained at the ground and its stratification in the atmosphere measured by a lidar (laser radar), as well as an atmospheric transport model and a simplified pollen module developed especially for this study. The largest pollen concentration difference between the ground and the layers above is observed during nighttime.
Mariana Adam, Iwona S. Stachlewska, Lucia Mona, Nikolaos Papagiannopoulos, Juan Antonio Bravo-Aranda, Michaël Sicard, Doina N. Nicolae, Livio Belegante, Lucja Janicka, Dominika Szczepanik, Maria Mylonaki, Christina-Anna Papanikolaou, Nikolaos Siomos, Kalliopi Artemis Voudouri, Luca Alados-Arboledas, Arnoud Apituley, Ina Mattis, Anatoli Chaikovsky, Constantino Muñoz-Porcar, Aleksander Pietruczuk, Daniele Bortoli, Holger Baars, Ivan Grigorov, and Zahary Peshev
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-759, https://doi.org/10.5194/acp-2021-759, 2021
Revised manuscript not accepted
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Results over 10 years of biomass burning events measured by EARLINET are analysed by means of the intensive parameters, based on the methodology described in Part I. Smoke type is characterized for each of the four geographical regions based on continental smoke origin. Relationships between intensive parameters or colour ratios are shown. The smoke is labelled in average as aged smoke.
Carmen Córdoba-Jabonero, Michaël Sicard, María-Ángeles López-Cayuela, Albert Ansmann, Adolfo Comerón, María-Paz Zorzano, Alejandro Rodríguez-Gómez, and Constantino Muñoz-Porcar
Atmos. Chem. Phys., 21, 6455–6479, https://doi.org/10.5194/acp-21-6455-2021, https://doi.org/10.5194/acp-21-6455-2021, 2021
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The particular pathway of dust outbreaks defines the aerosol scenario and short-wave (SW) dust direct radiative effect (DRE). The synergetic use of POLIPHON method with continuous P-MPL measurements allows SW DRE of coarse (Dc) and fine (Df) dust particles to be evaluated separately. A dust-induced cooling effect is found, and despite Dc usually being dominant in intense dust events, the Df contribution to the total DRE can be significant, being higher at the top of atmosphere than on surface.
Benjamin Torres, Luc Blarel, Philippe Goloub, Gaël Dubois, Maria Fernanda Sanchez-Barrero, Ioana Elisabeta Popovici, Fabrice Maupin, Elena Lind, Alexander Smirnov, Ilya Slutsker, Julien Chimot, Ramiro González, Michaël Sicard, Jean Marc Metzger, and Pierre Tulet
Atmos. Meas. Tech., 18, 4809–4838, https://doi.org/10.5194/amt-18-4809-2025, https://doi.org/10.5194/amt-18-4809-2025, 2025
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This study shows that it is possible to automatically monitor atmospheric aerosols from research vessels using automated instruments, following the same standards as AERONET (AErosol RObotic NETwork) land-based stations. By collecting 3 years of data in the Indian Ocean, we demonstrate that high-quality measurements can be made, even on a moving platform. These results open new possibilities for observing aerosols over the ocean and improving satellite data and climate studies.
Tristan Millet, Hassan Bencherif, Thierry Portafaix, Nelson Bègue, Alexandre Baron, Valentin Duflot, Cathy Clerbaux, Pierre-François Coheur, Andrea Pazmiño, Michaël Sicard, Anne Boynard, Jean-Marc Metzger, Guillaume Payen, Nicolas Marquestaut, and Sophie Godin-Beekmann
Atmos. Chem. Phys., 25, 10887–10905, https://doi.org/10.5194/acp-25-10887-2025, https://doi.org/10.5194/acp-25-10887-2025, 2025
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On 15 January 2022, the Hunga volcano erupted, releasing sulfur dioxide and water vapor into the stratosphere, impacting ozone levels over the Indian Ocean. Satellite data show the presence of a transient ozone depletion event related to the water vapor anomalies and sulfate aerosol clouds. Ozone reduction was confined to two distinct layers. On 21 January, the fifth percentile of total and stratospheric column ozone anomalies reached −18.6 and −14.5 DU, respectively.
Sergey Khaykin, Michael Sicard, Thierry Leblanc, Tetsu Sakai, Nickolay Balugin, Gwenael Berthet, Stéphane Chevrier, Fernando Chouza, Artem Feofilov, Dominique Gantois, Sophie Godin-Beekmann, Arezki Haddouche, Yoshitaka Jin, Isamu Morino, Nicolas Kadygrov, Thomas Lecas, Ben Liley, Richard Querel, Ghasssan Taha, and Vladimir Yushkov
EGUsphere, https://doi.org/10.5194/egusphere-2025-4377, https://doi.org/10.5194/egusphere-2025-4377, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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In April 2024, the Ruang volcano in Indonesia sent large amounts of gas and particles high into the atmosphere, which then spread worldwide. Using the new European EarthCARE satellite and its advanced laser instrument ATLID, together with ground and balloon observations, we tracked how these particles doubled levels in the tropics and spread into both hemispheres. The study shows ATLID’s power to reveal how eruptions can affect climate, clouds, and ozone for more than a year.
Maria Fernanda Sanchez-Barrero, Philippe Goloub, Luc Blarel, Ioana Elisabeta Popovici, Benjamin Torres, Gaël Dubois, Thierry Podvin, Fabrice Ducos, Romain de Filippi, Michaël Sicard, Viviane Bout Roumazeilles, and Charlotte Skonieczny
EGUsphere, https://doi.org/10.5194/egusphere-2025-3481, https://doi.org/10.5194/egusphere-2025-3481, 2025
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The TRANSAMA ship-based campaign (April–May 2023) aboard Marion Dufresne II investigated aerosols from La Réunion to Barbados using photometers and lidar. Observations revealed clean conditions over the South Atlantic, with thin transported aerosol plumes from Southern Africa. Clouds were detected in 53 % of lidar profiles with higher occurrence in the first 2 km. Results highlight aerosol-cloud interactions over remote oceans and support the development of mobile lidar-photometer systems.
África Barreto, Francisco Quirós, Omaira E. García, Jorge Pereda-de-Pablo, Daniel González-Fernández, Andrés Bedoya-Velásquez, Michael Sicard, Carmen Córdoba-Jabonero, Marco Iarlori, Vincenzo Rizi, Nickolay Krotkov, Simon Carn, Reijo Roininen, Antonio J. Molina-Arias, A. Fernando Almansa, Óscar Álvarez-Losada, Carla Aramo, Juan José Bustos, Romain Ceolato, Adolfo Comerón, Alicia Felpeto, Rosa D. García, Pablo González-Sicilia, Yenny González, Pascal Hedelt, Miguel Hernández, María-Ángeles López-Cayuela, Diego Loyola, Stavros Meletlidis, Constantino Muñoz-Porcar, Ermanno Pietropaolo, Ramón Ramos, Alejandro Rodríguez-Gómez, Roberto Román, Pedro M. Romero-Campos, Martin Stuefer, Carlos Toledano, and Elsworth Welton
EGUsphere, https://doi.org/10.5194/egusphere-2025-3164, https://doi.org/10.5194/egusphere-2025-3164, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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This manuscript describes the instrumental coverage deployed during the Tajogaite eruption (19 September–25 December 2021) by the Instituto Geográfico Nacional (IGN), the Spanish State Meteorological Agency (AEMET), and other Spanish members of ACTRIS (Aerosol, Clouds and Trace Gases Research Infrastructure) to monitor its atmospheric impact. Two complementary methods provide consistent plume height data for future operational surveillance.
Cristina Gil-Díaz, Michäel Sicard, Odran Sourdeval, Athulya Saiprakash, Constantino Muñoz-Porcar, Adolfo Comerón, Alejandro Rodríguez-Gómez, and Daniel Camilo Fortunato dos Santos Oliveira
Atmos. Chem. Phys., 25, 3445–3464, https://doi.org/10.5194/acp-25-3445-2025, https://doi.org/10.5194/acp-25-3445-2025, 2025
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This study presents a comprehensive analysis of optical scattering properties and direct radiative effects of cirrus clouds based on 4 years of continuous ground-based lidar measurements with the Barcelona MPLNET lidar. A novel approach of the self-consistent scattering model for cirrus clouds is presented to determine their optical scattering properties at different wavelengths, and their direct radiative effects are calculated with the discrete ordinates method embedded in the ARTDECO package.
María-Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Michaël Sicard, Jesús Abril-Gago, Vanda Salgueiro, Adolfo Comerón, María José Granados-Muñoz, Maria João Costa, Constantino Muñoz-Porcar, Juan Antonio Bravo-Aranda, Daniele Bortoli, Alejandro Rodríguez-Gómez, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 25, 3213–3231, https://doi.org/10.5194/acp-25-3213-2025, https://doi.org/10.5194/acp-25-3213-2025, 2025
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Due to the significant radiative role of dust in climate change, vertical assessments of the short-wave dust direct radiative effect of both fine and coarse dust particles are performed separately. The study is focused on an intense Saharan dust outbreak crossing the Iberian Peninsula in springtime monitored by five Iberian lidar stations with southwest–northeast coverage. A comparative study to evaluate the differences found by considering the total dust (no separation) is also examined.
Michaël Sicard, Alexandre Baron, Marion Ranaivombola, Dominique Gantois, Tristan Millet, Pasquale Sellitto, Nelson Bègue, Hassan Bencherif, Guillaume Payen, Nicolas Marquestaut, and Valentin Duflot
Atmos. Chem. Phys., 25, 367–381, https://doi.org/10.5194/acp-25-367-2025, https://doi.org/10.5194/acp-25-367-2025, 2025
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This study quantifies the radiative impact over Réunion Island (21° S, 55° E) of the aerosols and water vapor injected into the stratosphere by the Hunga volcano in the South Pacific. The overall aerosol and water vapor impact on the Earth’s radiation budget for the whole period is negative (cooling, -0.82 ± 0.35 W m-2) and dominated by the aerosols. At the Earth’s surface, aerosols are the main drivers and produce a negative (cooling, -1.04 ± 0.36 W m-2) radiative impact.
Dominique Gantois, Guillaume Payen, Michaël Sicard, Valentin Duflot, Nelson Bègue, Nicolas Marquestaut, Thierry Portafaix, Sophie Godin-Beekmann, Patrick Hernandez, and Eric Golubic
Earth Syst. Sci. Data, 16, 4137–4159, https://doi.org/10.5194/essd-16-4137-2024, https://doi.org/10.5194/essd-16-4137-2024, 2024
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We describe three instruments that have been measuring interactions between aerosols (particles of various origin) and light over Réunion Island since 2012. Aerosols directly or indirectly influence the temperature in the atmosphere and can interact with clouds. Details are given on how we derived aerosol properties from our measurements and how we assessed the quality of our data before sharing them with the scientific community. A good correlation was found between the three instruments.
Pierre Tulet, Joel Van Baelen, Pierre Bosser, Jérome Brioude, Aurélie Colomb, Philippe Goloub, Andrea Pazmino, Thierry Portafaix, Michel Ramonet, Karine Sellegri, Melilotus Thyssen, Léa Gest, Nicolas Marquestaut, Dominique Mékiès, Jean-Marc Metzger, Gilles Athier, Luc Blarel, Marc Delmotte, Guillaume Desprairies, Mérédith Dournaux, Gaël Dubois, Valentin Duflot, Kevin Lamy, Lionel Gardes, Jean-François Guillemot, Valérie Gros, Joanna Kolasinski, Morgan Lopez, Olivier Magand, Erwan Noury, Manuel Nunes-Pinharanda, Guillaume Payen, Joris Pianezze, David Picard, Olivier Picard, Sandrine Prunier, François Rigaud-Louise, Michael Sicard, and Benjamin Torres
Earth Syst. Sci. Data, 16, 3821–3849, https://doi.org/10.5194/essd-16-3821-2024, https://doi.org/10.5194/essd-16-3821-2024, 2024
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The MAP-IO program aims to compensate for the lack of atmospheric and oceanographic observations in the Southern Ocean by equipping the ship Marion Dufresne with a set of 17 scientific instruments. This program collected 700 d of measurements under different latitudes, seasons, sea states, and weather conditions. These new data will support the calibration and validation of numerical models and the understanding of the atmospheric composition of this region of Earth.
José Alex Zenteno-Hernández, Adolfo Comerón, Federico Dios, Alejandro Rodríguez-Gómez, Constantino Muñoz-Porcar, Michaël Sicard, Noemi Franco, Andreas Behrendt, and Paolo Di Girolamo
Atmos. Meas. Tech., 17, 4687–4694, https://doi.org/10.5194/amt-17-4687-2024, https://doi.org/10.5194/amt-17-4687-2024, 2024
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We study how the spectral characteristics of a solid-state laser in an atmospheric temperature profiling lidar using the Raman technique impact the temperature retrieval accuracy. We find that the spectral widening, with respect to a seeded laser, has virtually no impact, while crystal-rod temperature variations in the laser must be kept within a range of 1 K for the uncertainty in the atmospheric temperature below 1 K. The study is carried out through spectroscopy simulations.
Nelson Bègue, Alexandre Baron, Gisèle Krysztofiak, Gwenaël Berthet, Corinna Kloss, Fabrice Jégou, Sergey Khaykin, Marion Ranaivombola, Tristan Millet, Thierry Portafaix, Valentin Duflot, Philippe Keckhut, Hélène Vérèmes, Guillaume Payen, Mahesh Kumar Sha, Pierre-François Coheur, Cathy Clerbaux, Michaël Sicard, Tetsu Sakai, Richard Querel, Ben Liley, Dan Smale, Isamu Morino, Osamu Uchino, Tomohiro Nagai, Penny Smale, John Robinson, and Hassan Bencherif
Atmos. Chem. Phys., 24, 8031–8048, https://doi.org/10.5194/acp-24-8031-2024, https://doi.org/10.5194/acp-24-8031-2024, 2024
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During the 2020 austral summer, the pristine atmosphere of the southwest Indian Ocean basin experienced significant perturbations. Numerical models indicated that the lower-stratospheric aerosol content was influenced by the intense and persistent stratospheric aerosol layer generated during the 2019–2020 extreme Australian bushfire events. Ground-based observations at Réunion confirmed the simultaneous presence of African and Australian aerosol layers.
Cristina Gil-Díaz, Michäel Sicard, Adolfo Comerón, Daniel Camilo Fortunato dos Santos Oliveira, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Jasper R. Lewis, Ellsworth J. Welton, and Simone Lolli
Atmos. Meas. Tech., 17, 1197–1216, https://doi.org/10.5194/amt-17-1197-2024, https://doi.org/10.5194/amt-17-1197-2024, 2024
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In this paper, a statistical study of cirrus geometrical and optical properties based on 4 years of continuous ground-based lidar measurements with the Barcelona (Spain) Micro Pulse Lidar (MPL) is analysed. The cloud optical depth, effective column lidar ratio and linear cloud depolarisation ratio have been calculated by a new approach to the two-way transmittance method, which is valid for both ground-based and spaceborne lidar systems. Their associated errors are also provided.
Xiaoxia Shang, Antti Lipponen, Maria Filioglou, Anu-Maija Sundström, Mark Parrington, Virginie Buchard, Anton S. Darmenov, Ellsworth J. Welton, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Alejandro Rodríguez-Gómez, Mika Komppula, and Tero Mielonen
Atmos. Chem. Phys., 24, 1329–1344, https://doi.org/10.5194/acp-24-1329-2024, https://doi.org/10.5194/acp-24-1329-2024, 2024
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In June 2019, smoke particles from a Canadian wildfire event were transported to Europe. The long-range-transported smoke plumes were monitored with a spaceborne lidar and reanalysis models. Based on the aerosol mass concentrations estimated from the observations, the reanalysis models had difficulties in reproducing the amount and location of the smoke aerosols during the transport event. Consequently, more spaceborne lidar missions are needed for reliable monitoring of aerosol plumes.
Alexandra Tsekeri, Anna Gialitaki, Marco Di Paolantonio, Davide Dionisi, Gian Luigi Liberti, Alnilam Fernandes, Artur Szkop, Aleksander Pietruczuk, Daniel Pérez-Ramírez, Maria J. Granados Muñoz, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Diego Bermejo Pantaleón, Juan Antonio Bravo-Aranda, Anna Kampouri, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Adolfo Comerón, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Salvatore Romano, Maria Rita Perrone, Xiaoxia Shang, Mika Komppula, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Diofantos Hadjimitsis, Francisco Navas-Guzmán, Alexander Haefele, Dominika Szczepanik, Artur Tomczak, Iwona S. Stachlewska, Livio Belegante, Doina Nicolae, Kalliopi Artemis Voudouri, Dimitris Balis, Athena A. Floutsi, Holger Baars, Linda Miladi, Nicolas Pascal, Oleg Dubovik, and Anton Lopatin
Atmos. Meas. Tech., 16, 6025–6050, https://doi.org/10.5194/amt-16-6025-2023, https://doi.org/10.5194/amt-16-6025-2023, 2023
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EARLINET/ACTRIS organized an intensive observational campaign in May 2020, with the objective of monitoring the atmospheric state over Europe during the COVID-19 lockdown and relaxation period. The work presented herein focuses on deriving a common methodology for applying a synergistic retrieval that utilizes the network's ground-based passive and active remote sensing measurements and deriving the aerosols from anthropogenic activities over Europe.
Tristan Millet, Hassan Bencherif, Thierry Portafaix, Nelson Bègue, Alexandre Baron, Valentin Duflot, Michaël Sicard, Jean-Marc Metzger, Guillaume Payen, Nicolas Marquestaut, and Sophie Godin-Beekmann
EGUsphere, https://doi.org/10.5194/egusphere-2023-2645, https://doi.org/10.5194/egusphere-2023-2645, 2023
Preprint withdrawn
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The eruption of the Hunga Tonga volcano in January 2022 released substantial amounts of aerosols, sulfur dioxide, and water vapor into the stratosphere. Satellite and ground instruments followed the displacement of the volcanic aerosol plume and its impact on ozone levels over the Indian Ocean. Ozone data reveal the presence of a persistent ozone mini-hole structure from 17 January to 22 January, with most ozone depletion occurring within the ozone layer at the location of the aerosol plume.
Simone Lolli, Michaël Sicard, Francesco Amato, Adolfo Comeron, Cristina Gíl-Diaz, Tony C. Landi, Constantino Munoz-Porcar, Daniel Oliveira, Federico Dios Otin, Francesc Rocadenbosch, Alejandro Rodriguez-Gomez, Andrés Alastuey, Xavier Querol, and Cristina Reche
Atmos. Chem. Phys., 23, 12887–12906, https://doi.org/10.5194/acp-23-12887-2023, https://doi.org/10.5194/acp-23-12887-2023, 2023
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We evaluated the long-term trends and seasonal variability of the vertically resolved aerosol properties over the past 17 years in Barcelona. Results shows that air quality is improved, with a consistent drop in PM concentrations at the surface, as well as the column aerosol optical depth. The results also show that natural dust outbreaks are more likely in summer, with aerosols reaching an altitude of 5 km, while in winter, aerosols decay as an exponential with a scale height of 600 m.
Adolfo Comerón, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Michaël Sicard, Federico Dios, Cristina Gil-Díaz, Daniel Camilo Fortunato dos Santos Oliveira, and Francesc Rocadenbosch
Atmos. Meas. Tech., 16, 3015–3025, https://doi.org/10.5194/amt-16-3015-2023, https://doi.org/10.5194/amt-16-3015-2023, 2023
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We derive an explicit (i.e., non-iterative) formula for the retrieval of the overlap function in an aerosol lidar with both elastic and Raman N2 and/or O2 channels used for independent measurements of aerosol backscatter and extinction coefficients. The formula requires only the measured, range-corrected elastic and the corresponding Raman signals, plus an assumed lidar ratio. We assess the influence of the lidar ratio error in the overlap function retrieval and present retrieval examples.
María Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Diego Bermejo-Pantaleón, Michaël Sicard, Vanda Salgueiro, Francisco Molero, Clara Violeta Carvajal-Pérez, María José Granados-Muñoz, Adolfo Comerón, Flavio T. Couto, Rubén Barragán, María-Paz Zorzano, Juan Antonio Bravo-Aranda, Constantino Muñoz-Porcar, María João Costa, Begoña Artíñano, Alejandro Rodríguez-Gómez, Daniele Bortoli, Manuel Pujadas, Jesús Abril-Gago, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 143–161, https://doi.org/10.5194/acp-23-143-2023, https://doi.org/10.5194/acp-23-143-2023, 2023
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An intense Saharan dust outbreak crossing the Iberian Peninsula in springtime was monitored to determinine the specific contribution of fine and coarse dust particles at five lidar stations, strategically covering its SW–central–NE pathway. Expected dust ageing along the transport started unappreciated. A different fine-dust impact on optical (~30 %) and mass (~10 %) properties was found. Use of polarized lidar measurements (mainly in elastic systems) for fine/coarse dust separation is crucial.
M. Dolores Andrés Hernández, Andreas Hilboll, Helmut Ziereis, Eric Förster, Ovid O. Krüger, Katharina Kaiser, Johannes Schneider, Francesca Barnaba, Mihalis Vrekoussis, Jörg Schmidt, Heidi Huntrieser, Anne-Marlene Blechschmidt, Midhun George, Vladyslav Nenakhov, Theresa Harlass, Bruna A. Holanda, Jennifer Wolf, Lisa Eirenschmalz, Marc Krebsbach, Mira L. Pöhlker, Anna B. Kalisz Hedegaard, Linlu Mei, Klaus Pfeilsticker, Yangzhuoran Liu, Ralf Koppmann, Hans Schlager, Birger Bohn, Ulrich Schumann, Andreas Richter, Benjamin Schreiner, Daniel Sauer, Robert Baumann, Mariano Mertens, Patrick Jöckel, Markus Kilian, Greta Stratmann, Christopher Pöhlker, Monica Campanelli, Marco Pandolfi, Michael Sicard, José L. Gómez-Amo, Manuel Pujadas, Katja Bigge, Flora Kluge, Anja Schwarz, Nikos Daskalakis, David Walter, Andreas Zahn, Ulrich Pöschl, Harald Bönisch, Stephan Borrmann, Ulrich Platt, and John P. Burrows
Atmos. Chem. Phys., 22, 5877–5924, https://doi.org/10.5194/acp-22-5877-2022, https://doi.org/10.5194/acp-22-5877-2022, 2022
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EMeRGe provides a unique set of in situ and remote sensing airborne measurements of trace gases and aerosol particles along selected flight routes in the lower troposphere over Europe. The interpretation uses also complementary collocated ground-based and satellite measurements. The collected data help to improve the current understanding of the complex spatial distribution of trace gases and aerosol particles resulting from mixing, transport, and transformation of pollution plumes over Europe.
Michaël Sicard, Carmen Córdoba-Jabonero, María-Ángeles López-Cayuela, Albert Ansmann, Adolfo Comerón, María-Paz Zorzano, Alejandro Rodríguez-Gómez, and Constantino Muñoz-Porcar
Atmos. Chem. Phys., 22, 1921–1937, https://doi.org/10.5194/acp-22-1921-2022, https://doi.org/10.5194/acp-22-1921-2022, 2022
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This paper completes the companion paper of Córdoba-Jabonero et al. (2021). We estimate the total direct radiative effect produced by mineral dust particles during the June 2019 mega-heatwave at two sites in Spain and Germany. The results show that the dust particles in the atmosphere contribute to cooling the surface (less radiation reaches the surface) and that the heatwave (parametrized by high surface and air temperatures) contributes to reducing this cooling.
Jesús Abril-Gago, Juan Luis Guerrero-Rascado, Maria João Costa, Juan Antonio Bravo-Aranda, Michaël Sicard, Diego Bermejo-Pantaleón, Daniele Bortoli, María José Granados-Muñoz, Alejandro Rodríguez-Gómez, Constantino Muñoz-Porcar, Adolfo Comerón, Pablo Ortiz-Amezcua, Vanda Salgueiro, Marta María Jiménez-Martín, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 22, 1425–1451, https://doi.org/10.5194/acp-22-1425-2022, https://doi.org/10.5194/acp-22-1425-2022, 2022
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A validation of Aeolus reprocessed optical products is carried out via an intercomparison with ground-based measurements taken at several ACTRIS/EARLINET stations in western Europe. Case studies and a statistical analysis are presented. The stations are located in a hot spot between Africa and the rest of Europe, which guarantees a variety of aerosol types, from mineral dust layers to continental/anthropogenic aerosol, and allows us to test Aeolus performance under different scenarios.
Michaël Sicard, Oriol Jorba, Jiang Ji Ho, Rebeca Izquierdo, Concepción De Linares, Marta Alarcón, Adolfo Comerón, and Jordina Belmonte
Atmos. Chem. Phys., 21, 17807–17832, https://doi.org/10.5194/acp-21-17807-2021, https://doi.org/10.5194/acp-21-17807-2021, 2021
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This paper investigates the mechanisms involved in the dispersion, structure, and mixing in the vertical column of atmospheric pollen, using observations of pollen concentration obtained at the ground and its stratification in the atmosphere measured by a lidar (laser radar), as well as an atmospheric transport model and a simplified pollen module developed especially for this study. The largest pollen concentration difference between the ground and the layers above is observed during nighttime.
Mariana Adam, Iwona S. Stachlewska, Lucia Mona, Nikolaos Papagiannopoulos, Juan Antonio Bravo-Aranda, Michaël Sicard, Doina N. Nicolae, Livio Belegante, Lucja Janicka, Dominika Szczepanik, Maria Mylonaki, Christina-Anna Papanikolaou, Nikolaos Siomos, Kalliopi Artemis Voudouri, Luca Alados-Arboledas, Arnoud Apituley, Ina Mattis, Anatoli Chaikovsky, Constantino Muñoz-Porcar, Aleksander Pietruczuk, Daniele Bortoli, Holger Baars, Ivan Grigorov, and Zahary Peshev
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-759, https://doi.org/10.5194/acp-2021-759, 2021
Revised manuscript not accepted
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Results over 10 years of biomass burning events measured by EARLINET are analysed by means of the intensive parameters, based on the methodology described in Part I. Smoke type is characterized for each of the four geographical regions based on continental smoke origin. Relationships between intensive parameters or colour ratios are shown. The smoke is labelled in average as aged smoke.
Carmen Córdoba-Jabonero, Michaël Sicard, María-Ángeles López-Cayuela, Albert Ansmann, Adolfo Comerón, María-Paz Zorzano, Alejandro Rodríguez-Gómez, and Constantino Muñoz-Porcar
Atmos. Chem. Phys., 21, 6455–6479, https://doi.org/10.5194/acp-21-6455-2021, https://doi.org/10.5194/acp-21-6455-2021, 2021
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The particular pathway of dust outbreaks defines the aerosol scenario and short-wave (SW) dust direct radiative effect (DRE). The synergetic use of POLIPHON method with continuous P-MPL measurements allows SW DRE of coarse (Dc) and fine (Df) dust particles to be evaluated separately. A dust-induced cooling effect is found, and despite Dc usually being dominant in intense dust events, the Df contribution to the total DRE can be significant, being higher at the top of atmosphere than on surface.
Cited articles
Bedoya-Velásquez, A. E., Navas-Guzmán, F., Granados-Muñoz, M. J., Titos, G., Román, R., Casquero-Vera, J. A., Ortiz-Amezcua, P., Benavent-Oltra, J. A., de Arruda Moreira, G., Montilla-Rosero, E., Hoyos, C. D., Artiñano, B., Coz, E., Olmo-Reyes, F. J., Alados-Arboledas, L., and Guerrero-Rascado, J. L.: Hygroscopic growth study in the framework of EARLINET during the SLOPE I campaign: synergy of remote sensing and in situ instrumentation, Atmos. Chem. Phys., 18, 7001–7017, https://doi.org/10.5194/acp-18-7001-2018, 2018.
Bedoya-Velásquez, A. E., Titos, G., Bravo-Aranda, J. A., Haeffelin, M., Favez, O., Petit, J.-E., Casquero-Vera, J. A., Olmo-Reyes, F. J., Montilla-Rosero, E., Hoyos, C. D., Alados-Arboledas, L., and Guerrero-Rascado, J. L.: Long-term aerosol optical hygroscopicity study at the ACTRIS SIRTA observatory: synergy between ceilometer and in situ measurements, Atmos. Chem. Phys., 19, 7883–7896, https://doi.org/10.5194/acp-19-7883-2019, 2019.
Campbell, J. R., Hlavka, D. L., Welton, E. J., Flynn, C. J., Turner, D. D.,
Spinhirne, J. D., Scott, V. S., and Hwang, I. H.: Full-Time, Eye-Safe Cloud
and Aerosol Lidar Observation at Atmospheric Radiation Measurement Program
Sites: Instruments and Data Processing, J. Atmos. Ocean. Tech., 19,
431–442, https://doi.org/10.1175/1520-0426(2002)019<0431:FTESCA>2.0.CO;2, 2002.
Carrico, C. M., Kus, P., Rood, M. J., Quinn, P. K., and Bates, T. S.:
Mixtures of pollution, dust, sea salt, and volcanic aerosol during ACE-Asia:
Radiative properties as a function of relative humidity, J. Geophys. Res.,
108, 8650, https://doi.org/10.1029/2003JD003405, 2003.
Chatterjee, S. and Hadi, A. S. (Eds.): Simple Linear Regression, in: in Regression Analysis by Example, 4th Edition, John Wiley & Sons, ISBN 0-471-74696-7, 2006.
Chen, J., Li, Z., Lv, M., Wang, Y., Wang, W., Zhang, Y., Wang, H., Yan, X., Sun, Y., and Cribb, M.: Aerosol hygroscopic growth, contributing factors, and impact on haze events in a severely polluted region in northern China, Atmos. Chem. Phys., 19, 1327–1342, https://doi.org/10.5194/acp-19-1327-2019, 2019.
Cheung, H. C., Chou, C. C.-K., Lee, C. S. L., Kuo, W.-C., and Chang, S.-C.: Hygroscopic properties and cloud condensation nuclei activity of atmospheric aerosols under the influences of Asian continental outflow and new particle formation at a coastal site in eastern Asia, Atmos. Chem. Phys., 20, 5911–5922, https://doi.org/10.5194/acp-20-5911-2020, 2020.
Covert, D. S., Charlson, R. J., and Ahlquist, N. C.: A Study of the
Relationship of Chemical Composition and Humidity to Light Scattering by
Aerosols, J. Appl. Meteorol. Clim., 11, 968–976, https://doi.org/10.1175/1520-0450(1972)011<0968:ASOTRO>2.0.CO;2, 1972.
Cruz, C. N. and Pandis, S. N.: Deliquescence and Hygroscopic Growth of Mixed
Inorganic-Organic Atmospheric Aerosol, Environ. Sci. Technol., 34,
4313–4319, https://doi.org/10.1021/es9907109, 2000.
Cziczo, D. J., Nowak, J. B., Hu, J. H., and Abbatt, J. P. D.: Infrared
spectroscopy of model tropospheric aerosols as a function of relative
humidity: Observation of deliquescence and crystallization, J. Geophys.
Res., 102, 18843–18850, https://doi.org/10.1029/97JD01361, 1997.
Davidson, K. L., Fairall, C. W., Jones Boyle, P., and Schacher, G. E.:
Verification of an Atmospheric Mixed-Layer Model for a Coastal Region, J. Appl. Meteorol. Clim., 23,
617–636, https://doi.org/10.1175/1520-0450(1984)023<0617:VOAAML>2.0.CO;2, 1984.
Dawson, K. W., Ferrare, R. A., Moore, R. H., Clayton, M. B., Thorsen, T. J.,
and Eloranta, E. W.: Ambient Aerosol Hygroscopic Growth From Combined Raman
Lidar and HSRL, J. Geophys. Res.-Atmos., 125, e2019JD031708,
https://doi.org/10.1029/2019JD031708, 2020.
Feingold, G. and Morley, B.: Aerosol hygroscopic properties as measured by
lidar and comparison with in situ measurements, J. Geophys. Res., 108, 4327,
https://doi.org/10.1029/2002JD002842, 2003.
Fernández, A. J., Apituley, A., Veselovskii, I., Suvorina, A., Henzing,
J., Pujadas, M., and Artíñano, B.: Study of aerosol hygroscopic
events over the Cabauw experimental site for atmospheric research (CESAR)
using the multi-wavelength Raman lidar Caeli, Atmos. Environ., 120,
484–498, https://doi.org/10.1016/j.atmosenv.2015.08.079, 2015.
Gomez, S. L., Carrico, C. M., Allen, C., Lam, J., Dabli, S., Sullivan, A.
P., Aiken, A. C., Rahn, T., Romonosky, D., Chylek, P., Sevanto, S., and
Dubey, M. K.: Southwestern U.S. Biomass Burning Smoke Hygroscopicity: The
Role of Plant Phenology, Chemical Composition, and Combustion Properties, J.
Geophys. Res.-Atmos., 123, 5416–5432, https://doi.org/10.1029/2017JD028162,
2018.
Gordon, T. D., Wagner, N. L., Richardson, M. S., Law, D. C., Wolfe, D.,
Eloranta, E. W., Brock, C. A., Erdesz, F., and Murphy, D. M.: Design of a
Novel Open-Path Aerosol Extinction Cavity Ringdown Spectrometer, Aerosol
Sci. Tech., 49, 717–726,
https://doi.org/10.1080/02786826.2015.1066753, 2015.
Granados-Muñoz, M. J., Navas-Guzmán, F., Bravo-Aranda, J. A., Guerrero-Rascado, J. L., Lyamani, H., Valenzuela, A., Titos, G., Fernández-Gálvez, J., and Alados-Arboledas, L.: Hygroscopic growth of atmospheric aerosol particles based on active remote sensing and radiosounding measurements: selected cases in southeastern Spain, Atmos. Meas. Tech., 8, 705–718, https://doi.org/10.5194/amt-8-705-2015, 2015.
Gunthe, S. S., Rose, D., Su, H., Garland, R. M., Achtert, P., Nowak, A., Wiedensohler, A., Kuwata, M., Takegawa, N., Kondo, Y., Hu, M., Shao, M., Zhu, T., Andreae, M. O., and Pöschl, U.: Cloud condensation nuclei (CCN) from fresh and aged air pollution in the megacity region of Beijing, Atmos. Chem. Phys., 11, 11023–11039, https://doi.org/10.5194/acp-11-11023-2011, 2011.
Haarig, M., Ansmann, A., Gasteiger, J., Kandler, K., Althausen, D., Baars, H., Radenz, M., and Farrell, D. A.: Dry versus wet marine particle optical properties: RH dependence of depolarization ratio, backscatter, and extinction from multiwavelength lidar measurements during SALTRACE, Atmos. Chem. Phys., 17, 14199–14217, https://doi.org/10.5194/acp-17-14199-2017, 2017.
Haeffelin, M., Laffineur, Q., Bravo-Aranda, J.-A., Drouin, M.-A., Casquero-Vera, J.-A., Dupont, J.-C., and De Backer, H.: Radiation fog formation alerts using attenuated backscatter power from automatic lidars and ceilometers, Atmos. Meas. Tech., 9, 5347–5365, https://doi.org/10.5194/amt-9-5347-2016, 2016.
Hänel, G.: The Properties of Atmospheric Aerosol Particles as Functions
of the Relative Humidity at Thermodynamic Equilibrium with the Surrounding
Moist Air, Adv. Geophys., 19, 73–188, 1976.
Hansen, J., Sato, M., and Ruedy, R.: Radiative forcing and climate response, J. Geophys. Res.,
102, 6831–6864, https://doi.org/10.1029/96JD03436, 1997.
Hansson, H.-C., Rood, M. J., and Koloutsou-Vakakis, S.: NaCl Aerosol Particle
Hygroscopicity Dependence on Mixing with Organic Compounds, J. Atmos. Chem., 31, 321–346,
https://doi.org/10.1023/A:1006174514022, 1998.
Jefferson, A., Hageman, D., Morrow, H., Mei, F., and Watson, T.: Seven years
of aerosol scattering hygroscopic growth measurements from SGP: Factors
influencing water uptake, J. Geophys. Res.-Atmos., 122, 9451–9466,
https://doi.org/10.1002/2017JD026804, 2017.
Kanakidou, M., Seinfeld, J. H., Pandis, S. N., Barnes, I., Dentener, F. J., Facchini, M. C., Van Dingenen, R., Ervens, B., Nenes, A., Nielsen, C. J., Swietlicki, E., Putaud, J. P., Balkanski, Y., Fuzzi, S., Horth, J., Moortgat, G. K., Winterhalter, R., Myhre, C. E. L., Tsigaridis, K., Vignati, E., Stephanou, E. G., and Wilson, J.: Organic aerosol and global climate modelling: a review, Atmos. Chem. Phys., 5, 1053–1123, https://doi.org/10.5194/acp-5-1053-2005, 2005.
Kasten, F.: Visibility forecast in the phase of pre-condensation, Tellus A, 21,
631–635, https://doi.org/10.1111/j.2153-3490.1969.tb00469.x, 1969.
Koren, I., Kaufman, Y. J., Remer, L. A., and Martins, J. V.: Measurement of
the Effect of Amazon Smoke on Inhibition of Cloud Formation, Science, 303,
1342–1345, https://doi.org/10.1126/science.1089424, 2004.
Ku, H. H.: Notes on the use of propagation of error formulas, J. Res. Nat.
B. Stan., 70, 11, https://doi.org/10.6028/jres.070C.025, 1966.
Kumar, D., Rocadenbosch, F., Sicard, M., Comeron, A., Muñoz, C., Lange,
D., Tomás, S., and Gregorio, E.: Six-channel polychromator design and
implementation for the UPC elastic/Raman lidar, SPIE Remote Sensing, Prague,
Czech Republic, 81820W, https://doi.org/10.1117/12.896305, 2011.
Liu, H. J., Zhao, C. S., Nekat, B., Ma, N., Wiedensohler, A., van Pinxteren, D., Spindler, G., Müller, K., and Herrmann, H.: Aerosol hygroscopicity derived from size-segregated chemical composition and its parameterization in the North China Plain, Atmos. Chem. Phys., 14, 2525–2539, https://doi.org/10.5194/acp-14-2525-2014, 2014.
Liu, P., Song, M., Zhao, T., Gunthe, S. S., Ham, S., He, Y., Qin, Y. M.,
Gong, Z., Amorim, J. C., Bertram, A. K., and Martin, S. T.: Resolving the
mechanisms of hygroscopic growth and cloud condensation nuclei activity for
organic particulate matter, Nat. Commun., 9, 4076,
https://doi.org/10.1038/s41467-018-06622-2, 2018.
Lv, M., Liu, D., Li, Z., Mao, J., Sun, Y., Wang, Z., Wang, Y., and Xie, C.:
Hygroscopic growth of atmospheric aerosol particles based on lidar,
radiosonde, and in situ measurements: Case studies from the Xinzhou field
campaign, J. Quant. Spectrosc. Ra., 188,
60–70, https://doi.org/10.1016/j.jqsrt.2015.12.029, 2017.
Munoz-Porcar, C., Sicard, M., Granados-Munoz, M. J., Barragan, R., Comeron,
A., Rocadenbosch, F., Rodriguez-Gomez, A., and Garcia-Vizcaino, D.: Synergy
of Raman Lidar and Modeled Temperature for Relative Humidity Profiling:
Assessment and Uncertainty Analysis, IEEE T. Geosci. Remote, 59,
8841–8852, https://doi.org/10.1109/TGRS.2020.3039689, 2021.
Navas-Guzmán, F., Martucci, G., Collaud Coen, M., Granados-Muñoz, M. J., Hervo, M., Sicard, M., and Haefele, A.: Characterization of aerosol hygroscopicity using Raman lidar measurements at the EARLINET station of Payerne, Atmos. Chem. Phys., 19, 11651–11668, https://doi.org/10.5194/acp-19-11651-2019, 2019.
Orr, C., Hurd, F. K., and Corbett, W. J.: Aerosol size and relative
humidity, J. Colloid Sci., 13, 472–482,
https://doi.org/10.1016/0095-8522(58)90055-2, 1958.
Pandolfi, M., Martucci, G., Querol, X., Alastuey, A., Wilsenack, F., Frey, S., O'Dowd, C. D., and Dall'Osto, M.: Continuous atmospheric boundary layer observations in the coastal urban area of Barcelona during SAPUSS, Atmos. Chem. Phys., 13, 4983–4996, https://doi.org/10.5194/acp-13-4983-2013, 2013.
Papayannis, A., Argyrouli, A., Bougiatioti, A., Nenes, A., Vande Hey, J.,
Komppula, M., Kokkalis, P., Solomos, S., Banks, R. F., Labzovskii, L.,
Kalogiros, I., and Giannakaki, E.: From Hygroscopic Aerosols to Cloud
Droplets: The HygrA-CD Campaign in the Athens Basin – An Overview, in:
Perspectives on Atmospheric Sciences, edited by: Karacostas, T., Bais, A.,
and Nastos, P. T., Springer International Publishing, Cham, 781–787,
https://doi.org/10.1007/978-3-319-35095-0_112, 2017.
Pérez, C., Sicard, M., Jorba, O., Comerón, A., and Baldasano, J. M.:
Summertime re-circulations of air pollutants over the north-eastern Iberian
coast observed from systematic EARLINET lidar measurements in Barcelona,
Atmos. Environ., 38, 3983–4000,
https://doi.org/10.1016/j.atmosenv.2004.04.010, 2004.
Pérez-Ramírez, D., Whiteman, D. N., Veselovskii, I., Ferrare, R., Titos, G., Granados-Muñoz, M. J., Sánchez-Hernández, G., and Navas-Guzmán, F.: Spatiotemporal changes in aerosol properties by hygroscopic growth and impacts on radiative forcing and heating rates during DISCOVER-AQ 2011, Atmos. Chem. Phys., 21, 12021–12048, https://doi.org/10.5194/acp-21-12021-2021, 2021.
Pey, J., Querol, X., and Alastuey, A.: Discriminating the regional and urban
contributions in the North-Western Mediterranean: PM levels and composition,
Atmos. Environ., 44, 1587–1596,
https://doi.org/10.1016/j.atmosenv.2010.02.005, 2010.
Querol, X., Alastuey, A., Rodriguez, S., Plana, F., Ruiz, C. R., Cots, N.,
Massague, G., and Puig, O.: PM10 and PM2.5 source apportionment in the
Barcelona Metropolitan area, Catalonia, Spain, Atmos. Environ., 35,
6407–6419, https://doi.org/10.1016/S1352-2310(01)00361-2, 2001.
Ruehl, C. R. and Wilson, K. R.: Surface Organic Monolayers Control the
Hygroscopic Growth of Submicrometer Particles at High Relative Humidity, J.
Phys. Chem. A, 118, 3952–3966, https://doi.org/10.1021/jp502844g, 2014.
Seinfeld, J. H., Bretherton, C., Carslaw, K. S., Coe, H., DeMott, P. J.,
Dunlea, E. J., Feingold, G., Ghan, S., Guenther, A. B., Kahn, R., Kraucunas,
I., Kreidenweis, S. M., Molina, M. J., Nenes, A., Penner, J. E., Prather, K.
A., Ramanathan, V., Ramaswamy, V., Rasch, P. J., Ravishankara, A. R.,
Rosenfeld, D., Stephens, G., and Wood, R.: Improving our fundamental
understanding of the role of aerosol-cloud interactions in the climate
system, P. Natl. Acad. Sci. USA, 113, 5781–5790,
https://doi.org/10.1073/pnas.1514043113, 2016.
Sheridan, P. J., Delene, D. J., and Ogren, J. A.: Four years of continuous
surface aerosol measurements from the Department of Energy's Atmospheric
Radiation Measurement Program Southern Great Plains Cloud and Radiation
Testbed site, J. Geophys. Res., 106, 20735–20747,
https://doi.org/10.1029/2001JD000785, 2001.
Sheridan, P. J., Jefferson, A., and Ogren, J. A.: Spatial variability of
submicrometer aerosol radiative properties over the Indian Ocean during
INDOEX, J. Geophys. Res., 107, 8011, https://doi.org/10.1029/2000JD000166,
2002.
Sicard, M., Pérez, C., Rocadenbosch, F., Baldasano, J. M., and
García-Vizcaino, D.: Mixed-Layer Depth Determination in the Barcelona
Coastal Area From Regular Lidar Measurements: Methods, Results and
Limitations, Bound.-Lay. Meteorol., 119, 135–157,
https://doi.org/10.1007/s10546-005-9005-9, 2006.
Sicard, M., Rocadenbosch, F., Reba, M. N. M., Comerón, A., Tomás, S., García-Vízcaino, D., Batet, O., Barrios, R., Kumar, D., and Baldasano, J. M.: Seasonal variability of aerosol optical properties observed by means of a Raman lidar at an EARLINET site over Northeastern Spain, Atmos. Chem. Phys., 11, 175–190, https://doi.org/10.5194/acp-11-175-2011, 2011.
Sicard, M., Rodríguez-Gómez, A., Comerón, A., and
Muñoz-Porcar, C.: Calculation of the Overlap Function and Associated
Error of an Elastic Lidar or a Ceilometer: Cross-Comparison with a
Cooperative Overlap-Corrected System, Sensors, 20, 6312,
https://doi.org/10.3390/s20216312, 2020.
Sicard, M., Fortunato dos Santos Oliveira, D. C., Muñoz Porcar, C., Gil Díaz, C., Comerón Tejero, A., Rodríguez Gómez, A., and Dios Otín, F.: Barcelona MPL Backscatter profiles at 00:00 and 12:00 UTC, between 2015 and 2018, Repositori de Dades de Recerca [data set], https://doi.org/10.34810/data195, 2022a.
Sicard, M., Fortunato dos Santos Oliveira, D. C., Muñoz Porcar, C., Gil Díaz, C., Comerón Tejero, A., Rodríguez Gómez, A., and Dios Otín, F.: Barcelona radiosounding files used in identified hygroscopicity cases, between 2015 and 2018, Repositori de Dades de Recerca [data set], https://doi.org/10.34810/data194, 2022b.
Sjogren, S., Gysel, M., Weingartner, E., Baltensperger, U., Cubison, M. J.,
Coe, H., Zardini, A. A., Marcolli, C., Krieger, U. K., and Peter, T.:
Hygroscopic growth and water uptake kinetics of two-phase aerosol particles
consisting of ammonium sulfate, adipic and humic acid mixtures, J.
Aerosol Sci., 38, 157–171,
https://doi.org/10.1016/j.jaerosci.2006.11.005, 2007.
Skupin, A., Ansmann, A., Engelmann, R., Seifert, P., and Müller, T.: Four-year long-path monitoring of ambient aerosol extinction at a central European urban site: dependence on relative humidity, Atmos. Chem. Phys., 16, 1863–1876, https://doi.org/10.5194/acp-16-1863-2016, 2016.
Stein, A. F., Draxler, R. R., Rolph, G. D., Stunder, B. J. B., Cohen, M. D.,
and Ngan, F.: NOAA's HYSPLIT Atmospheric Transport and Dispersion Modeling
System, B. Am. Meteorol. Soc., 96, 2059–2077, https://doi.org/10.1175/BAMS-D-14-00110.1, 2015.
Stull, R. B.: The Energetics of Entrainment Across a Density Interface, J. Atmos. Sci., 33,
1260–1267, https://doi.org/10.1175/1520-0469(1976)033<1260:TEOEAD>2.0.CO;2, 1976.
Tang, I. N., Fung, K. H., Imre, D. G., and Munkelwitz, H. R.: Phase
Transformation and Metastability of Hygroscopic Microparticles, Aerosol
Sci. Technol., 23, 443–453,
https://doi.org/10.1080/02786829508965327, 1995.
Thorsen, T. J., Ferrare, R. A., Kato, S., and Winker, D. M.: Aerosol Direct
Radiative Effect Sensitivity Analysis, J. Climate, 33, 6119–6139,
https://doi.org/10.1175/JCLI-D-19-0669.1, 2020.
Titos, G., Cazorla, A., Zieger, P., Andrews, E., Lyamani, H.,
Granados-Muñoz, M. J., Olmo, F. J., and Alados-Arboledas, L.: Effect of
hygroscopic growth on the aerosol light-scattering coefficient: A review of
measurements, techniques and error sources, Atmos. Environ., 141,
494–507, https://doi.org/10.1016/j.atmosenv.2016.07.021, 2016.
Veselovskii, I., Whiteman, D. N., Kolgotin, A., Andrews, E., and Korenskii,
M.: Demonstration of Aerosol Property Profiling by Multiwavelength Lidar
under Varying Relative Humidity Conditions, J. Atmos. Ocean. Tech., 26, 1543–1557,
https://doi.org/10.1175/2009JTECHA1254.1, 2009.
Weather and Climate: Weather humidity in Barcelona (Catalonia),
https://weather-and-climate.com/average-monthly-Humidity-perc,barcelona,Spain,
last access: 22 October 2021.
Welton, E. J. and Campbell, J. R.: Micropulse Lidar Signals: Uncertainty
Analysis, J. Atmos. Ocean. Tech., 19, 2089–2094,
https://doi.org/10.1175/1520-0426(2002)019<2089:MLSUA>2.0.CO;2, 2002.
World Meteorological Organization and Global Atmosphere Watch: WMO/GAW aerosol measurement procedures: guidelines and recommendations, WMO/TD- No. 1178, GAW Report-No. 153, https://library.wmo.int/doc_num.php?explnum_id=9244 (last access: 23 March 2022), 2003.
Zhao, G., Zhao, C., Kuang, Y., Tao, J., Tan, W., Bian, Y., Li, J., and Li, C.: Impact of aerosol hygroscopic growth on retrieving aerosol extinction coefficient profiles from elastic-backscatter lidar signals, Atmos. Chem. Phys., 17, 12133–12143, https://doi.org/10.5194/acp-17-12133-2017, 2017.
Zieger, P., Fierz-Schmidhauser, R., Weingartner, E., and Baltensperger, U.:
Effects of relative humidity on aerosol light scattering: results from
different European sites, Atmos. Chem. Phys., 13, 10609–10631,
https://doi.org/10.5194/acp-13-10609-2013, 2013.
Short summary
Atmospheric particles can absorb water vapor, and this water uptake may change their properties, e.g., their size. In the coastal region of Barcelona, Spain, we observe that (1) smaller particles absorb more water vapor, in relative terms, than larger particles and (2) the particle capacity to absorb water vapor has no annual tendency, probably because the site background is quite constant (urban + marine aerosol regime).
Atmospheric particles can absorb water vapor, and this water uptake may change their properties,...
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