Articles | Volume 22, issue 17
https://doi.org/10.5194/acp-22-11867-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-11867-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
14 Sep 2022
Research article |
| 14 Sep 2022
| 14 Sep 2022
Quantifying vertical wind shear effects in shallow cumulus clouds over Amazonia
Micael Amore Cecchini
CORRESPONDING AUTHOR
Institute of Astronomy, Geophysics and Atmospheric Sciences,
University of São Paulo, São Paulo, Brazil
Department of Atmospheric Science, Colorado State University, Fort
Collins, USA
Marco de Bruine
Institute for Marine and Atmospheric Research, Utrecht University,
Utrecht, the Netherlands
Jordi Vilà-Guerau de Arellano
Meteorology and Air Quality Section, Wageningen University,
Wageningen, the Netherlands
Atmospheric Chemistry Department, Max Planck Institute for Chemistry,
Mainz, Germany
Paulo Artaxo
Institute of Physics, University of São Paulo, São Paulo,
Brazil
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Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankarararman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Hannele Hakola, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbiginiw Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-1, https://doi.org/10.5194/essd-2024-1, 2024
Preprint withdrawn
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Aerosol particles can interact with incoming solar radiation and outgoing long wave radiation, change cloud properties, affect photochemistry, impact surface air quality, and when deposited impact surface albedo of snow and ice, and modulate carbon dioxide uptake by the land and ocean. Here we present a new compilation of aerosol observations including composition, a methodology for comparing the datasets to model output, and show the implications of these results using one model.
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Isotope fluxes allow for net ecosystem gas exchange fluxes to be partitioned into sub-components like plant assimilation, respiration and transpiration, which can help us better understand the environmental drivers of each partial flux. We share the results of a field campaign isotope fluxes were derived using a combination of laser spectroscopy and eddy covariance. We found lag times and high frequency signal loss in the isotope fluxes we derived and present methods to correct for both.
Xurong Wang, Qiaoqiao Wang, Maria Prass, Christopher Pöhlker, Daniel Moran-Zuloaga, Paulo Artaxo, Jianwei Gu, Ning Yang, Xiajie Yang, Jiangchuan Tao, Juan Hong, Nan Ma, Yafang Cheng, Hang Su, and Meinrat O. Andreae
Atmos. Chem. Phys., 23, 9993–10014, https://doi.org/10.5194/acp-23-9993-2023, https://doi.org/10.5194/acp-23-9993-2023, 2023
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In this work, with an optimized particle mass size distribution, we captured observed aerosol optical depth (AOD) and coarse aerosol concentrations over source and/or receptor regions well, demonstrating good performance in simulating export of African dust toward the Amazon Basin. In addition to factors controlling the transatlantic transport of African dust, the study investigated the impact of African dust over the Amazon Basin, including the nutrient inputs associated with dust deposition.
Kim A. P. Faassen, Linh N. T. Nguyen, Eadin R. Broekema, Bert A. M. Kers, Ivan Mammarella, Timo Vesala, Penelope A. Pickers, Andrew C. Manning, Jordi Vilà-Guerau de Arellano, Harro A. J. Meijer, Wouter Peters, and Ingrid T. Luijkx
Atmos. Chem. Phys., 23, 851–876, https://doi.org/10.5194/acp-23-851-2023, https://doi.org/10.5194/acp-23-851-2023, 2023
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The exchange ratio (ER) between atmospheric O2 and CO2 provides a useful tracer for separately estimating photosynthesis and respiration processes in the forest carbon balance. This is highly relevant to better understand the expected biosphere sink, which determines future atmospheric CO2 levels. We therefore measured O2, CO2, and their ER above a boreal forest in Finland and investigated their diurnal behaviour for a representative day, and we show the most suitable way to determine the ER.
Wiebke Scholz, Jiali Shen, Diego Aliaga, Cheng Wu, Samara Carbone, Isabel Moreno, Qiaozhi Zha, Wei Huang, Liine Heikkinen, Jean Luc Jaffrezo, Gaelle Uzu, Eva Partoll, Markus Leiminger, Fernando Velarde, Paolo Laj, Patrick Ginot, Paolo Artaxo, Alfred Wiedensohler, Markku Kulmala, Claudia Mohr, Marcos Andrade, Victoria Sinclair, Federico Bianchi, and Armin Hansel
Atmos. Chem. Phys., 23, 895–920, https://doi.org/10.5194/acp-23-895-2023, https://doi.org/10.5194/acp-23-895-2023, 2023
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Dimethyl sulfide (DMS), emitted from the ocean, is the most abundant biogenic sulfur emission into the atmosphere. OH radicals, among others, can oxidize DMS to sulfuric and methanesulfonic acid, which are relevant for aerosol formation. We quantified DMS and nearly all DMS oxidation products with novel mass spectrometric instruments for gas and particle phase at the high mountain station Chacaltaya (5240 m a.s.l.) in the Bolivian Andes in free tropospheric air after long-range transport.
Yunfan Liu, Hang Su, Siwen Wang, Chao Wei, Wei Tao, Mira L. Pöhlker, Christopher Pöhlker, Bruna A. Holanda, Ovid O. Krüger, Thorsten Hoffmann, Manfred Wendisch, Paulo Artaxo, Ulrich Pöschl, Meinrat O. Andreae, and Yafang Cheng
Atmos. Chem. Phys., 23, 251–272, https://doi.org/10.5194/acp-23-251-2023, https://doi.org/10.5194/acp-23-251-2023, 2023
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The origins of the abundant cloud condensation nuclei (CCN) in the upper troposphere (UT) of the Amazon remain unclear. With model developments of new secondary organic aerosol schemes and constrained by observation, we show that strong aerosol nucleation and condensation in the UT is triggered by biogenic organics, and organic condensation is key for UT CCN production. This UT CCN-producing mechanism may prevail over broader vegetation canopies and deserves emphasis in aerosol–climate feedback.
Felipe Lobos-Roco, Oscar Hartogensis, Francisco Suárez, Ariadna Huerta-Viso, Imme Benedict, Alberto de la Fuente, and Jordi Vilà-Guerau de Arellano
Hydrol. Earth Syst. Sci., 26, 3709–3729, https://doi.org/10.5194/hess-26-3709-2022, https://doi.org/10.5194/hess-26-3709-2022, 2022
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This research brings a multi-scale temporal analysis of evaporation in a saline lake of the Atacama Desert. Our findings reveal that evaporation is controlled differently depending on the timescale. Evaporation is controlled sub-diurnally by wind speed, regulated seasonally by radiation and modulated interannually by ENSO. Our research extends our understanding of evaporation, contributing to improving the climate change assessment and efficiency of water management in arid regions.
Ruben B. Schulte, Margreet C. van Zanten, Bart J. H. van Stratum, and Jordi Vilà-Guerau de Arellano
Atmos. Chem. Phys., 22, 8241–8257, https://doi.org/10.5194/acp-22-8241-2022, https://doi.org/10.5194/acp-22-8241-2022, 2022
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We present a fine-scale simulation framework, utilizing large-eddy simulations, to assess NH3 measurements influenced by boundary-layer dynamics and turbulent dispersion of a nearby emission source. The minimum required distance from an emission source differs for concentration and flux measurements, from 0.5–3.0 km and 0.75–4.5 km, respectively. The simulation framework presented here proves to be a powerful and versatile tool for future NH3 research at high spatio-temporal resolutions.
Marco A. Franco, Florian Ditas, Leslie A. Kremper, Luiz A. T. Machado, Meinrat O. Andreae, Alessandro Araújo, Henrique M. J. Barbosa, Joel F. de Brito, Samara Carbone, Bruna A. Holanda, Fernando G. Morais, Janaína P. Nascimento, Mira L. Pöhlker, Luciana V. Rizzo, Marta Sá, Jorge Saturno, David Walter, Stefan Wolff, Ulrich Pöschl, Paulo Artaxo, and Christopher Pöhlker
Atmos. Chem. Phys., 22, 3469–3492, https://doi.org/10.5194/acp-22-3469-2022, https://doi.org/10.5194/acp-22-3469-2022, 2022
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In Central Amazonia, new particle formation in the planetary boundary layer is rare. Instead, there is the appearance of sub-50 nm aerosols with diameters larger than about 20 nm that eventually grow to cloud condensation nuclei size range. Here, 254 growth events were characterized which have higher predominance in the wet season. About 70 % of them showed direct relation to convective downdrafts, while 30 % occurred partly under clear-sky conditions, evidencing still unknown particle sources.
Luiz A. T. Machado, Marco A. Franco, Leslie A. Kremper, Florian Ditas, Meinrat O. Andreae, Paulo Artaxo, Micael A. Cecchini, Bruna A. Holanda, Mira L. Pöhlker, Ivan Saraiva, Stefan Wolff, Ulrich Pöschl, and Christopher Pöhlker
Atmos. Chem. Phys., 21, 18065–18086, https://doi.org/10.5194/acp-21-18065-2021, https://doi.org/10.5194/acp-21-18065-2021, 2021
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Several studies evaluate aerosol–cloud interactions, but only a few attempted to describe how clouds modify aerosol properties. This study evaluates the effect of weather events on the particle size distribution at the ATTO, combining remote sensing and in situ data. Ultrafine, Aitken and accumulation particles modes have different behaviors for the diurnal cycle and for rainfall events. This study opens up new scientific questions that need to be pursued in detail in new field campaigns.
Diego Aliaga, Victoria A. Sinclair, Marcos Andrade, Paulo Artaxo, Samara Carbone, Evgeny Kadantsev, Paolo Laj, Alfred Wiedensohler, Radovan Krejci, and Federico Bianchi
Atmos. Chem. Phys., 21, 16453–16477, https://doi.org/10.5194/acp-21-16453-2021, https://doi.org/10.5194/acp-21-16453-2021, 2021
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We investigate the origin of air masses sampled at Mount Chacaltaya, Bolivia. Three-quarters of the measured air has not been influenced by the surface in the previous 4 d. However, it is rare that, at any given time, the sampled air has not been influenced at all by the surface, and often the sampled air has multiple origins. The influence of the surface is more prevalent during day than night. Furthermore, during the 6-month study, one-third of the air masses originated from Amazonia.
Maria Prass, Meinrat O. Andreae, Alessandro C. de Araùjo, Paulo Artaxo, Florian Ditas, Wolfgang Elbert, Jan-David Förster, Marco Aurélio Franco, Isabella Hrabe de Angelis, Jürgen Kesselmeier, Thomas Klimach, Leslie Ann Kremper, Eckhard Thines, David Walter, Jens Weber, Bettina Weber, Bernhard M. Fuchs, Ulrich Pöschl, and Christopher Pöhlker
Biogeosciences, 18, 4873–4887, https://doi.org/10.5194/bg-18-4873-2021, https://doi.org/10.5194/bg-18-4873-2021, 2021
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Bioaerosols in the atmosphere over the Amazon rain forest were analyzed by molecular biological staining and microscopy. Eukaryotic, bacterial, and archaeal aerosols were quantified in time series and altitude profiles which exhibited clear differences in number concentrations and vertical distributions. Our results provide insights into the sources and dispersion of different Amazonian bioaerosol types as a basis for a better understanding of biosphere–atmosphere interactions.
James Weber, Scott Archer-Nicholls, Nathan Luke Abraham, Youngsub M. Shin, Thomas J. Bannan, Carl J. Percival, Asan Bacak, Paulo Artaxo, Michael Jenkin, M. Anwar H. Khan, Dudley E. Shallcross, Rebecca H. Schwantes, Jonathan Williams, and Alex T. Archibald
Geosci. Model Dev., 14, 5239–5268, https://doi.org/10.5194/gmd-14-5239-2021, https://doi.org/10.5194/gmd-14-5239-2021, 2021
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The new mechanism CRI-Strat 2 features state-of-the-art isoprene chemistry not previously available in UKCA and improves UKCA's ability to reproduce observed concentrations of isoprene, monoterpenes, and OH in tropical regions. The enhanced ability to model isoprene, the most widely emitted non-methane volatile organic compound (VOC), will allow understanding of how isoprene and other biogenic VOCs affect atmospheric composition and, through biosphere–atmosphere feedbacks, climate change.
Carlos Román-Cascón, Marie Lothon, Fabienne Lohou, Oscar Hartogensis, Jordi Vila-Guerau de Arellano, David Pino, Carlos Yagüe, and Eric R. Pardyjak
Geosci. Model Dev., 14, 3939–3967, https://doi.org/10.5194/gmd-14-3939-2021, https://doi.org/10.5194/gmd-14-3939-2021, 2021
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The type of vegetation (or land cover) and its status influence the heat and water transfers between the surface and the air, affecting the processes that develop in the atmosphere at different (but connected) spatiotemporal scales. In this work, we investigate how these transfers are affected by the way the surface is represented in a widely used weather model. The results encourage including realistic high-resolution and updated land cover databases in models to improve their predictions.
Felipe Lobos-Roco, Oscar Hartogensis, Jordi Vilà-Guerau de Arellano, Alberto de la Fuente, Ricardo Muñoz, José Rutllant, and Francisco Suárez
Atmos. Chem. Phys., 21, 9125–9150, https://doi.org/10.5194/acp-21-9125-2021, https://doi.org/10.5194/acp-21-9125-2021, 2021
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We investigate the influence of regional atmospheric circulation on the evaporation of a saline lake in the Altiplano region of the Atacama Desert through a field experiment and regional modeling. Our results show that evaporation is controlled by two regimes: (1) in the morning by local conditions with low evaporation rates and low wind speed and (2) in the afternoon with high evaporation rates and high wind speed. Afternoon winds are connected to the regional Pacific Ocean–Andes flow.
Djacinto Monteiro dos Santos, Luciana Varanda Rizzo, Samara Carbone, Patrick Schlag, and Paulo Artaxo
Atmos. Chem. Phys., 21, 8761–8773, https://doi.org/10.5194/acp-21-8761-2021, https://doi.org/10.5194/acp-21-8761-2021, 2021
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The metropolitan area of São Paulo (MASP), with very extensive biofuel use, has unique atmospheric chemistry among world megacities. In this study, we examine the complex relationships between aerosol chemical composition and particle size distribution. Our findings provide a better understanding of the dynamics of the physicochemical properties of submicron particles and highlight the key role of secondary organic aerosol formation in the pollution levels in São Paulo.
Robbie Ramsay, Chiara F. Di Marco, Mathew R. Heal, Matthias Sörgel, Paulo Artaxo, Meinrat O. Andreae, and Eiko Nemitz
Biogeosciences, 18, 2809–2825, https://doi.org/10.5194/bg-18-2809-2021, https://doi.org/10.5194/bg-18-2809-2021, 2021
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The exchange of the gas ammonia between the atmosphere and the surface is an important biogeochemical process, but little is known of this exchange for certain ecosystems, such as the Amazon rainforest. This study took measurements of ammonia exchange over an Amazon rainforest site and subsequently modelled the observed deposition and emission patterns. We observed emissions of ammonia from the rainforest, which can be simulated accurately by using a canopy resistance modelling approach.
Janaína P. Nascimento, Megan M. Bela, Bruno B. Meller, Alessandro L. Banducci, Luciana V. Rizzo, Angel Liduvino Vara-Vela, Henrique M. J. Barbosa, Helber Gomes, Sameh A. A. Rafee, Marco A. Franco, Samara Carbone, Glauber G. Cirino, Rodrigo A. F. Souza, Stuart A. McKeen, and Paulo Artaxo
Atmos. Chem. Phys., 21, 6755–6779, https://doi.org/10.5194/acp-21-6755-2021, https://doi.org/10.5194/acp-21-6755-2021, 2021
Guilherme F. Camarinha-Neto, Julia C. P. Cohen, Cléo Q. Dias-Júnior, Matthias Sörgel, José Henrique Cattanio, Alessandro Araújo, Stefan Wolff, Paulo A. F. Kuhn, Rodrigo A. F. Souza, Luciana V. Rizzo, and Paulo Artaxo
Atmos. Chem. Phys., 21, 339–356, https://doi.org/10.5194/acp-21-339-2021, https://doi.org/10.5194/acp-21-339-2021, 2021
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It was observed that friagem phenomena (incursion of cold waves from the high latitudes of the Southern Hemisphere to the Amazon region), very common in the dry season of the Amazon region, produced significant changes in microclimate and atmospheric chemistry. Moreover, the effects of the friagem change the surface O3 and CO2 mixing ratios and therefore interfere deeply in the microclimatic conditions and the chemical composition of the atmosphere above the rainforest.
Jann Schrod, Erik S. Thomson, Daniel Weber, Jens Kossmann, Christopher Pöhlker, Jorge Saturno, Florian Ditas, Paulo Artaxo, Valérie Clouard, Jean-Marie Saurel, Martin Ebert, Joachim Curtius, and Heinz G. Bingemer
Atmos. Chem. Phys., 20, 15983–16006, https://doi.org/10.5194/acp-20-15983-2020, https://doi.org/10.5194/acp-20-15983-2020, 2020
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Long-term ice-nucleating particle (INP) data are presented from four semi-pristine sites located in the Amazon, the Caribbean, Germany and the Arctic. Average INP concentrations did not differ by orders of magnitude between the sites. For all sites short-term variability dominated the time series, which lacked clear trends and seasonalities. Common drivers to explain the INP levels and their variations could not be identified, illustrating the complex nature of heterogeneous ice nucleation.
Robbie Ramsay, Chiara F. Di Marco, Matthias Sörgel, Mathew R. Heal, Samara Carbone, Paulo Artaxo, Alessandro C. de Araùjo, Marta Sá, Christopher Pöhlker, Jost Lavric, Meinrat O. Andreae, and Eiko Nemitz
Atmos. Chem. Phys., 20, 15551–15584, https://doi.org/10.5194/acp-20-15551-2020, https://doi.org/10.5194/acp-20-15551-2020, 2020
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The Amazon rainforest is a unique
laboratoryto study the processes which govern the exchange of gases and aerosols to and from the atmosphere. This study investigated these processes by measuring the atmospheric concentrations of trace gases and particles at the Amazon Tall Tower Observatory. We found that the long-range transport of pollutants can affect the atmospheric composition above the Amazon rainforest and that the gases ammonia and nitrous acid can be emitted from the rainforest.
Lixia Liu, Yafang Cheng, Siwen Wang, Chao Wei, Mira L. Pöhlker, Christopher Pöhlker, Paulo Artaxo, Manish Shrivastava, Meinrat O. Andreae, Ulrich Pöschl, and Hang Su
Atmos. Chem. Phys., 20, 13283–13301, https://doi.org/10.5194/acp-20-13283-2020, https://doi.org/10.5194/acp-20-13283-2020, 2020
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This modeling paper reveals how aerosol–cloud interactions (ACIs) and aerosol–radiation interactions (ARIs) induced by biomass burning (BB) aerosols act oppositely on radiation, cloud, and precipitation in the Amazon during the dry season. The varying relative significance of ACIs and ARIs with BB aerosol concentration leads to a nonlinear dependence of the total climate response on BB aerosol loading and features the growing importance of ARIs at high aerosol loading.
Kouji Adachi, Naga Oshima, Zhaoheng Gong, Suzane de Sá, Adam P. Bateman, Scot T. Martin, Joel F. de Brito, Paulo Artaxo, Glauber G. Cirino, Arthur J. Sedlacek III, and Peter R. Buseck
Atmos. Chem. Phys., 20, 11923–11939, https://doi.org/10.5194/acp-20-11923-2020, https://doi.org/10.5194/acp-20-11923-2020, 2020
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Occurrences, size distributions, and number fractions of individual aerosol particles from the Amazon basin during the GoAmazon2014/5 campaign were analyzed using transmission electron microscopy. Aerosol particles from natural sources (e.g., mineral dust, primary biological aerosols, and sea salts) during the wet season originated from the Amazon forest and long-range transports (the Saharan desert and the Atlantic Ocean). They commonly mix at an individual particle scale during transport.
Jordi Vilà-Guerau de Arellano, Patrizia Ney, Oscar Hartogensis, Hugo de Boer, Kevin van Diepen, Dzhaner Emin, Geiske de Groot, Anne Klosterhalfen, Matthias Langensiepen, Maria Matveeva, Gabriela Miranda-García, Arnold F. Moene, Uwe Rascher, Thomas Röckmann, Getachew Adnew, Nicolas Brüggemann, Youri Rothfuss, and Alexander Graf
Biogeosciences, 17, 4375–4404, https://doi.org/10.5194/bg-17-4375-2020, https://doi.org/10.5194/bg-17-4375-2020, 2020
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The CloudRoots field experiment has obtained an open comprehensive observational data set that includes soil, plant, and atmospheric variables to investigate the interactions between a heterogeneous land surface and its overlying atmospheric boundary layer, including the rapid perturbations of clouds in evapotranspiration. Our findings demonstrate that in order to understand and represent diurnal variability, we need to measure and model processes from the leaf to the landscape scales.
Cited articles
Altaratz, O., Koren, I., Remer, L. A., and Hirsch, E.: Review: Cloud
invigoration by aerosols – Coupling between microphysics and dynamics,
Atmos. Res., 140–141, 38–60,
https://doi.org/10.1016/j.atmosres.2014.01.009, 2014.
Andreae, M. O., Afchine, A., Albrecht, R., Holanda, B. A., Artaxo, P., Barbosa, H. M. J., Borrmann, S., Cecchini, M. A., Costa, A., Dollner, M., Fütterer, D., Järvinen, E., Jurkat, T., Klimach, T., Konemann, T., Knote, C., Krämer, M., Krisna, T., Machado, L. A. T., Mertes, S., Minikin, A., Pöhlker, C., Pöhlker, M. L., Pöschl, U., Rosenfeld, D., Sauer, D., Schlager, H., Schnaiter, M., Schneider, J., Schulz, C., Spanu, A., Sperling, V. B., Voigt, C., Walser, A., Wang, J., Weinzierl, B., Wendisch, M., and Ziereis, H.: Aerosol characteristics and particle production in the upper troposphere over the Amazon Basin, Atmos. Chem. Phys., 18, 921–961, https://doi.org/10.5194/acp-18-921-2018, 2018.
Artaxo, P., Rizzo, L. V., Brito, J. F., Barbosa, H. M. J., Arana, A., Sena,
E. T., Cirino, G. G., Bastos, W., Martin, S. T., and Andreae, M. O.:
Atmospheric aerosols in Amazonia and land use change: from natural biogenic
to biomass burning conditions, Faraday Discuss., 165, 203–235,
https://doi.org/10.1039/C3FD00052D, 2013.
Asai, T.: Cumulus Convection in the Atmosphere with Vertical, Journal of the
Meteorological Society of Japan, Ser. II, 42, 245–259,
https://doi.org/10.2151/jmsj1923.42.4_245, 1964.
Betts, R. A., Malhi, Y., and Roberts, J. T.: The future of the Amazon: new
perspectives from climate, ecosystem and social sciences, Philos. Trans. R. Soc. Lond. B Biol. Sci., 363, 1729–1735, https://doi.org/10.1098/rstb.2008.0011,
2008.
Cecchini, M. A., Silva Dias, M. A. F., Machado, L. A. T., Morales Rodriguez,
C. A., and Biscaro, T.: Macrophysical and Microphysical Characteristics of
Convective Rain Cells Observed During SOS-CHUVA, J. Geophys. Res.-Atmos., 125, e2019JD031187, https://doi.org/10.1029/2019JD031187, 2020.
Chakraborty, S., Schiro, K. A., Fu, R., and Neelin, J. D.: On the role of aerosols, humidity, and vertical wind shear in the transition of shallow-to-deep convection at the Green Ocean Amazon 2014/5 site, Atmos. Chem. Phys., 18, 11135–11148, https://doi.org/10.5194/acp-18-11135-2018, 2018.
Cuijpers, J. W. M. and Duynkerke, P. G.: Large Eddy Simulation of Trade Wind
Cumulus Clouds, J. Atmos. Sci., 50, 3894–3908,
https://doi.org/10.1175/1520-0469(1993)050<3894:LESOTW>2.0.CO;2, 1993.
de Bruine, M., Krol, M., Vilà-Guerau de Arellano, J., and Röckmann, T.: Explicit aerosol–cloud interactions in the Dutch Atmospheric Large-Eddy Simulation model DALES4.1-M7, Geosci. Model Dev., 12, 5177–5196, https://doi.org/10.5194/gmd-12-5177-2019, 2019.
Drueke, S., Kirshbaum, D. J., and Kollias, P.: Environmental sensitivities of shallow-cumulus dilution – Part 2: Vertical wind profile, Atmos. Chem. Phys., 21, 14039–14058, https://doi.org/10.5194/acp-21-14039-2021, 2021.
Fan, J., Yuan, T., Comstock, J. M., Ghan, S., Khain, A., Leung, L. R., Li,
Z., Martins, V. J., and Ovchinnikov, M.: Dominant role by vertical wind
shear in regulating aerosol effects on deep convective clouds, J. Geophys. Res.-Atmos., 114, D22206,
https://doi.org/10.1029/2009JD012352, 2009.
Fu, Q. and Liou, K. N.: On the Correlated k-Distribution Method for
Radiative Transfer in Nonhomogeneous Atmospheres, J. Atmos. Sci., 49, 2139–2156, https://doi.org/10.1175/1520-0469(1992)049<2139:OTCDMF>2.0.CO;2, 1992.
Fu, Q., Liou, K. N., Cribb, M. C., Charlock, T. P., and Grossman, A.:
Multiple Scattering Parameterization in Thermal Infrared Radiative Transfer,
J. Atmos. Sci., 54, 2799–2812,
https://doi.org/10.1175/1520-0469(1997)054<2799:MSPITI>2.0.CO;2, 1997.
Heiblum, R. H., Pinto, L., Altaratz, O., Dagan, G., and Koren, I.: Core and margin in warm convective clouds – Part 1: Core types and evolution during a cloud's lifetime, Atmos. Chem. Phys., 19, 10717–10738, https://doi.org/10.5194/acp-19-10717-2019, 2019.
Helfer, K. C. and Nuijens, L.: The Morphology of Simulated Trade-Wind
Convection and Cold Pools Under Wind Shear, J. Geophys. Res.-Atmos., 126, e2021JD035148, https://doi.org/10.1029/2021JD035148, 2021.
Helfer, K. C., Nuijens, L., de Roode, S. R., and Siebesma, A. P.: How Wind
Shear Affects Trade-wind Cumulus Convection, J. Adv. Model.
Earth Sys., 12, e2020MS002183, https://doi.org/10.1029/2020MS002183,
2020.
Henkes, A., Fisch, G., Machado, L. A. T., and Chaboureau, J.-P.: Morning boundary layer conditions for shallow to deep convective cloud evolution during the dry season in the central Amazon, Atmos. Chem. Phys., 21, 13207–13225, https://doi.org/10.5194/acp-21-13207-2021, 2021.
Heus, T., van Heerwaarden, C. C., Jonker, H. J. J., Pier Siebesma, A., Axelsen, S., van den Dries, K., Geoffroy, O., Moene, A. F., Pino, D., de Roode, S. R., and Vilà-Guerau de Arellano, J.: Formulation of the Dutch Atmospheric Large-Eddy Simulation (DALES) and overview of its applications, Geosci. Model Dev., 3, 415–444, https://doi.org/10.5194/gmd-3-415-2010, 2010.
Houze, R. A.: 100 Years of Research on Mesoscale Convective Systems,
Meteorol. Monograph., 59, 17.1–17.54,
https://doi.org/10.1175/AMSMONOGRAPHS-D-18-0001.1, 2018.
Lintner, B. R., Adams, D. K., Schiro, K. A., Stansfield, A. M., Rocha, A. A.
A., and Neelin, J. D.: Relationships among climatological vertical moisture
structure, column water vapor, and precipitation over the central Amazon in
observations and CMIP5 models, Geophys. Res. Lett., 44, 1981–1989,
https://doi.org/10.1002/2016GL071923, 2017.
Lovejoy, T. E. and Nobre, C.: Amazon Tipping Point, Sci. Adv., 4, eaat2340,
https://doi.org/10.1126/sciadv.aat2340, 2018.
Machado, L. A. T., Calheiros, A. J. P., Biscaro, T., Giangrande, S., Silva Dias, M. A. F., Cecchini, M. A., Albrecht, R., Andreae, M. O., Araujo, W. F., Artaxo, P., Borrmann, S., Braga, R., Burleyson, C., Eichholz, C. W., Fan, J., Feng, Z., Fisch, G. F., Jensen, M. P., Martin, S. T., Pöschl, U., Pöhlker, C., Pöhlker, M. L., Ribaud, J.-F., Rosenfeld, D., Saraiva, J. M. B., Schumacher, C., Thalman, R., Walter, D., and Wendisch, M.: Overview: Precipitation characteristics and sensitivities to environmental conditions during GoAmazon2014/5 and ACRIDICON-CHUVA, Atmos. Chem. Phys., 18, 6461–6482, https://doi.org/10.5194/acp-18-6461-2018, 2018.
Machado, L. A. T., Franco, M. A., Kremper, L. A., Ditas, F., Andreae, M. O., Artaxo, P., Cecchini, M. A., Holanda, B. A., Pöhlker, M. L., Saraiva, I., Wolff, S., Pöschl, U., and Pöhlker, C.: How weather events modify aerosol particle size distributions in the Amazon boundary layer, Atmos. Chem. Phys., 21, 18065–18086, https://doi.org/10.5194/acp-21-18065-2021, 2021.
Malkus, J. S.: The slopes of cumulus clouds in relation to external wind
shear, Q. J. Roy. Meteor. Soc., 78, 530–542,
https://doi.org/10.1002/qj.49707833804, 1952.
Martin, S. T., Artaxo, P., Machado, L. A. T., Manzi, A. O., Souza, R. A. F., Schumacher, C., Wang, J., Andreae, M. O., Barbosa, H. M. J., Fan, J., Fisch, G., Goldstein, A. H., Guenther, A., Jimenez, J. L., Pöschl, U., Silva Dias, M. A., Smith, J. N., and Wendisch, M.: Introduction: Observations and Modeling of the Green Ocean Amazon (GoAmazon2014/5), Atmos. Chem. Phys., 16, 4785–4797, https://doi.org/10.5194/acp-16-4785-2016, 2016.
Neggers, R. A. J., Neelin, J. D., and Stevens, B.: Impact Mechanisms of
Shallow Cumulus Convection on Tropical Climate Dynamics, J. Clim.,
20, 2623–2642, https://doi.org/10.1175/JCLI4079.1, 2007.
Nobre, C. A., Obregón, G. O., Marengo, J. A., Fu, R., and Poveda, G.:
Characteristics of Amazonian Climate: Main Features, Amazonia and Global
Change, 186, 149–162, https://doi.org/10.1029/2009GM000903, 2009.
Nuijens, L. and Stevens, B.: The Influence of Wind Speed on Shallow Marine
Cumulus Convection, J. Atmos. Sci., 69, 168–184,
https://doi.org/10.1175/JAS-D-11-02.1, 2012.
Ouwersloot, H. G., Moene, A. F., Attema, J. J., and de Arellano, J. V.-G.:
Large-Eddy Simulation Comparison of Neutral Flow Over a Canopy:
Sensitivities to Physical and Numerical Conditions, and Similarity to Other
Representations, Bound.-Lay. Meteorol., 162, 71–89,
https://doi.org/10.1007/s10546-016-0182-5, 2017.
Petters, M. D. and Kreidenweis, S. M.: A single parameter representation of hygroscopic growth and cloud condensation nucleus activity, Atmos. Chem. Phys., 7, 1961–1971, https://doi.org/10.5194/acp-7-1961-2007, 2007.
Piacsek, S. A. and Williams, G. P.: Conservation properties of convection
difference schemes, J. Comput. Phys., 6, 392–405,
https://doi.org/10.1016/0021-9991(70)90038-0, 1970.
Pino, D., Vilà-Guerau de Arellano, J., and Duynkerke, P. G.: The
Contribution of Shear to the Evolution of a Convective Boundary Layer,
J. Atmos. Sci., 60, 1913–1926,
https://doi.org/10.1175/1520-0469(2003)060<1913:TCOSTT>2.0.CO;2, 2003.
Pöhlker, M. L., Ditas, F., Saturno, J., Klimach, T., Hrabě de Angelis, I., Araùjo, A. C., Brito, J., Carbone, S., Cheng, Y., Chi, X., Ditz, R., Gunthe, S. S., Holanda, B. A., Kandler, K., Kesselmeier, J., Könemann, T., Krüger, O. O., Lavrič, J. V., Martin, S. T., Mikhailov, E., Moran-Zuloaga, D., Rizzo, L. V., Rose, D., Su, H., Thalman, R., Walter, D., Wang, J., Wolff, S., Barbosa, H. M. J., Artaxo, P., Andreae, M. O., Pöschl, U., and Pöhlker, C.: Long-term observations of cloud condensation nuclei over the Amazon rain forest – Part 2: Variability and characteristics of biomass burning, long-range transport, and pristine rain forest aerosols, Atmos. Chem. Phys., 18, 10289–10331, https://doi.org/10.5194/acp-18-10289-2018, 2018.
Riehl, H., Yeh, T. C., Malkus, J. S., and la Seur, N. E.: The north-east
trade of the Pacific Ocean, Q. J. Roy. Meteor. Soc., 77, 598–626, https://doi.org/10.1002/qj.49707733405, 1951.
Schiro, K. A. and Neelin, J. D.: Deep Convective Organization, Moisture
Vertical Structure, and Convective Transition Using Deep-Inflow Mixing,
J. Atmos. Sci., 76, 965–987,
https://doi.org/10.1175/JAS-D-18-0122.1, 2019.
Schiro, K. A., Neelin, J. D., Adams, D. K., and Lintner, B. R.: Deep
Convection and Column Water Vapor over Tropical Land versus Tropical Ocean:
A Comparison between the Amazon and the Tropical Western Pacific, J. Atmos. Sci., 73, 4043–4063,
https://doi.org/10.1175/JAS-D-16-0119.1, 2016.
Seifert, A. and Beheng, K. D.: A two-moment cloud microphysics
parameterization for mixed-phase clouds. Part 1: Model description,
Meteorol. Atmos. Phys., 92, 45–66,
https://doi.org/10.1007/s00703-005-0112-4, 2006.
Silva Dias, M. A. F., Rutledge, S., Kabat, P., Silva Dias, P. L., Nobre, C.,
Fisch, G., Dolman, A. J., Zipser, E., Garstang, M., Manzi, A. O., Fuentes,
J. D., Rocha, H. R., Marengo, J., Plana-Fattori, A., Sá, L. D. A.,
Alvalá, R. C. S., Andreae, M. O., Artaxo, P., Gielow, R., and Gatti,
L.: Cloud and rain processes in a biosphere-atmosphere interaction context
in the Amazon Region, J. Geophys. Res.-Atmos., 107, LBA39-1, https://doi.org/10.1029/2001JD000335, 2002.
Sommeria, G. and Deardorff, J. W.: Subgrid-Scale Condensation in Models of
Nonprecipitating Clouds, J. Atmos. Sci., 34, 344–355,
https://doi.org/10.1175/1520-0469(1977)034<0344:SSCIMO>2.0.CO;2, 1977.
Stevens, B.: On the Growth of Layers of Nonprecipitating Cumulus Convection,
J. Atmos. Sci., 64, 2916–2931,
https://doi.org/10.1175/JAS3983.1, 2007.
Vera, C., Higgins, W., Amador, J., Ambrizzi, T., Garreaud, R., Gochis, D.,
Gutzler, D., Lettenmaier, D., Marengo, J., Mechoso, C. R., Nogues-Paegle,
J., Dias, P. L. S., and Zhang, C.: Toward a Unified View of the American
Monsoon Systems, J. Clim., 19, 4977–5000,
https://doi.org/10.1175/JCLI3896.1, 2006.
Vila, D. A., Machado, L. A. T., Laurent, H., and Velasco, I.: Forecast and
Tracking the Evolution of Cloud Clusters (ForTraCC) Using Satellite Infrared
Imagery: Methodology and Validation, Weather Forecast., 23, 233–245,
https://doi.org/10.1175/2007WAF2006121.1, 2008.
Vilà-Guerau de Arellano, J., Kim, S.-W., Barth, M. C., and Patton, E. G.: Transport and chemical transformations influenced by shallow cumulus over land, Atmos. Chem. Phys., 5, 3219–3231, https://doi.org/10.5194/acp-5-3219-2005, 2005.
Vilà-Guerau de Arellano, J., Patton, E. G., Karl, T., van den Dries, K.,
Barth, M. C., and Orlando, J. J.: The role of boundary layer dynamics on the
diurnal evolution of isoprene and the hydroxyl radical over tropical
forests, J. Geophys. Res.-Atmos., 116, D07304, https://doi.org/10.1029/2010JD014857, 2011.
Vilà-Guerau de Arellano, J., Wang, X., Pedruzo-Bagazgoitia, X., Sikma, M., Agusti-Panareda, A., Boussetta, S., Balsamo, G., Machado, L. A. T., Biscaro, T., Gentine, P., Martin, S. T., Fuentes, J. D., and
Gerken, T.: Interactions Between the Amazonian Rainforest and Cumuli Clouds: A
Large-Eddy Simulation, High-Resolution ECMWF, and Observational
Intercomparison Study, J. Adv. Model. Earth Sys., 12, e2019MS001828, https://doi.org/10.1029/2019ms001828, 2020.
Wang, J., Krejci, R., Giangrande, S., Kuang, C., Barbosa, H. M. J., Brito,
J., Carbone, S., Chi, X., Comstock, J., Ditas, F., Lavric, J., Manninen, H.
E., Mei, F., Moran-Zuloaga, D., Pöhlker, C., Pöhlker, M. L.,
Saturno, J., Schmid, B., Souza, R. A. F., Springston, S. R., Tomlinson, J.
M., Toto, T., Walter, D., Wimmer, D., Smith, J. N., Kulmala, M., Machado, L.
A. T., Artaxo, P., Andreae, M. O., Petäjä, T., and Martin, S. T.:
Amazon boundary layer aerosol concentration sustained by vertical transport
during rainfall, Nature, 539, 416–419, https://doi.org/10.1038/nature19819,
2016.
Wendisch, M., Pöschl, U., Andreae, M. O., Machado, L. A. T., Albrecht,
R., Schlager, H., Rosenfeld, D., Martin, S. T., Abdelmonem, A., Afchine, A.,
Araùjo, A. C., Artaxo, P., Aufmhoff, H., Barbosa, H. M. J., Borrmann,
S., Braga, R., Buchholz, B., Cecchini, M. A., Costa, A., Curtius, J.,
Dollner, M., Dorf, M., Dreiling, V., Ebert, V., Ehrlich, A., Ewald, F.,
Fisch, G., Fix, A., Frank, F., Fütterer, D., Heckl, C., Heidelberg, F.,
Hüneke, T., Jäkel, E., Järvinen, E., Jurkat, T., Kanter, S.,
Kästner, U., Kenntner, M., Kesselmeier, J., Klimach, T., Knecht, M.,
Kohl, R., Kölling, T., Krämer, M., Krüger, M., Krisna, T. C.,
Lavric, J. V., Longo, K., Mahnke, C., Manzi, A. O., Mayer, B., Mertes, S.,
Minikin, A., Molleker, S., Münch, S., Nillius, B., Pfeilsticker, K.,
Pöhlker, C., Roiger, A., Rose, D., Rosenow, D., Sauer, D., Schnaiter,
M., Schneider, J., Schulz, C., de Souza, R. A. F., Spanu, A., Stock, P.,
Vila, D., Voigt, C., Walser, A., Walter, D., Weigel, R., Weinzierl, B.,
Werner, F., Yamasoe, M. A., Ziereis, H., Zinner, T., and Zöger, M.:
ACRIDICON–CHUVA Campaign: Studying Tropical Deep Convective Clouds and
Precipitation over Amazonia Using the New German Research Aircraft HALO,
Bull. Am. Meteor. Soc., 97, 1885–1908,
https://doi.org/10.1175/BAMS-D-14-00255.1, 2016.
Yamaguchi, T., Feingold, G., and Kazil, J.: Aerosol-Cloud Interactions in
Trade Wind Cumulus Clouds and the Role of Vertical Wind Shear, J. Geophys. Res.-Atmos., 124, 12244–12261,
https://doi.org/10.1029/2019JD031073, 2019.
Zhou, J. and Lau, K.-M.: Does a Monsoon Climate Exist over South America?,
J. Clim., 11, 1020–1040,
https://doi.org/10.1175/1520-0442(1998)011<1020:DAMCEO>2.0.CO;2, 1998.
Zhuang, Y., Fu, R., Marengo, J. A., and Wang, H.: Seasonal variation of
shallow-to-deep convection transition and its link to the environmental
conditions over the Central Amazon, J. Geophys. Res.-Atmos., 122, 2649–2666, https://doi.org/10.1002/2016JD025993, 2017.
Short summary
Shallow clouds (vertical extent up to 3 km height) are ubiquitous throughout the Amazon and are responsible for redistributing the solar heat and moisture vertically and horizontally. They are a key component of the water cycle because they can grow past the shallow phase to contribute significantly to the precipitation formation. However, they need favourable environmental conditions to grow. In this study, we analyse how changing wind patterns affect the development of such shallow clouds.
Shallow clouds (vertical extent up to 3 km height) are ubiquitous throughout the Amazon and are...
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