Articles | Volume 22, issue 15
https://doi.org/10.5194/acp-22-10353-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-10353-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
12 Aug 2022
Research article |
| 12 Aug 2022
| 12 Aug 2022
Disentangling the impact of air–sea interaction and boundary layer cloud formation on stable water isotope signals in the warm sector of a Southern Ocean cyclone
Institute for Atmospheric and Climate Science, ETH Zürich, Zurich, Switzerland
Geophysical Institute, University of Bergen, and Bjerknes Centre for Climate Research, Bergen, Norway
Invited contribution by Iris Thurnherr, recipient of the EGU Atmospheric Sciences Outstanding Student Poster and PICO Award 2019.
Franziska Aemisegger
Institute for Atmospheric and Climate Science, ETH Zürich, Zurich, Switzerland
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Yafei Li, Franziska Aemisegger, Andreas Riedl, Nina Buchmann, and Werner Eugster
Hydrol. Earth Syst. Sci., 25, 2617–2648, https://doi.org/10.5194/hess-25-2617-2021, https://doi.org/10.5194/hess-25-2617-2021, 2021
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During dry spells, dew and fog potentially play an increasingly important role in temperate grasslands. Research on the combined mechanisms of dew and fog inputs to ecosystems and distillation of water vapor from soil to plant surfaces is rare. Our results using stable water isotopes highlight the importance of dew and fog inputs to temperate grasslands during dry spells and reveal the complexity of the local water cycling in such conditions, including different pathways of dew and fog inputs.
Iris Thurnherr, Katharina Hartmuth, Lukas Jansing, Josué Gehring, Maxi Boettcher, Irina Gorodetskaya, Martin Werner, Heini Wernli, and Franziska Aemisegger
Weather Clim. Dynam., 2, 331–357, https://doi.org/10.5194/wcd-2-331-2021, https://doi.org/10.5194/wcd-2-331-2021, 2021
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Extratropical cyclones are important for the transport of moisture from low to high latitudes. In this study, we investigate how the isotopic composition of water vapour is affected by horizontal temperature advection associated with extratropical cyclones using measurements and modelling. It is shown that air–sea moisture fluxes induced by this horizontal temperature advection lead to the strong variability observed in the isotopic composition of water vapour in the marine boundary layer.
Franziska Aemisegger, Raphaela Vogel, Pascal Graf, Fabienne Dahinden, Leonie Villiger, Friedhelm Jansen, Sandrine Bony, Bjorn Stevens, and Heini Wernli
Weather Clim. Dynam., 2, 281–309, https://doi.org/10.5194/wcd-2-281-2021, https://doi.org/10.5194/wcd-2-281-2021, 2021
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The interaction of clouds in the trade wind region with the atmospheric flow is complex and at the heart of uncertainties associated with climate projections. In this study, a natural tracer of atmospheric circulation is used to establish a link between air originating from dry regions of the midlatitudes and the occurrence of specific cloud patterns. Two pathways involving transport within midlatitude weather systems are identified, by which air is brought into the trades within 5–10 d.
Sebastian Landwehr, Iris Thurnherr, Nicolas Cassar, Martin Gysel-Beer, and Julia Schmale
Atmos. Meas. Tech., 13, 3487–3506, https://doi.org/10.5194/amt-13-3487-2020, https://doi.org/10.5194/amt-13-3487-2020, 2020
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Shipborne wind speed measurements are relevant for field studies of air–sea interaction processes. Distortion of the airflow by the ship’s structure can, however, lead to errors. We estimate the flow distortion bias by comparing the observations to ERA-5 reanalysis data. The underlying assumptions are that the bias depends only on the relative orientation of the ship to the wind direction and that the ERA-5 wind speeds are (on average) representative of the true wind speed.
Nicolas Jullien, Étienne Vignon, Michael Sprenger, Franziska Aemisegger, and Alexis Berne
The Cryosphere, 14, 1685–1702, https://doi.org/10.5194/tc-14-1685-2020, https://doi.org/10.5194/tc-14-1685-2020, 2020
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Although snowfall is the main input of water to the Antarctic ice sheet, snowflakes are often evaporated by dry and fierce winds near the surface of the continent. The amount of snow that actually reaches the ground is therefore considerably reduced. By analyzing the position of cyclones and fronts as well as by back-tracing the atmospheric moisture pathway towards Antarctica, this study explains in which meteorological conditions snowfall is either completely evaporated or reaches the ground.
Iris Thurnherr, Anna Kozachek, Pascal Graf, Yongbiao Weng, Dimitri Bolshiyanov, Sebastian Landwehr, Stephan Pfahl, Julia Schmale, Harald Sodemann, Hans Christian Steen-Larsen, Alessandro Toffoli, Heini Wernli, and Franziska Aemisegger
Atmos. Chem. Phys., 20, 5811–5835, https://doi.org/10.5194/acp-20-5811-2020, https://doi.org/10.5194/acp-20-5811-2020, 2020
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Stable water isotopes (SWIs) are tracers of moist atmospheric processes. We analyse the impact of large- to small-scale atmospheric processes and various environmental conditions on the variability of SWIs using ship-based SWI measurement in water vapour from the Atlantic and Southern Ocean. Furthermore, simultaneous measurements of SWIs at two altitudes are used to illustrate the potential of such measurements for future research to estimate sea spray evaporation and turbulent moisture fluxes.
Andreas Schneider, Tobias Borsdorff, Joost aan de Brugh, Franziska Aemisegger, Dietrich G. Feist, Rigel Kivi, Frank Hase, Matthias Schneider, and Jochen Landgraf
Atmos. Meas. Tech., 13, 85–100, https://doi.org/10.5194/amt-13-85-2020, https://doi.org/10.5194/amt-13-85-2020, 2020
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This paper presents a new H2O/HDO data set from TROPOMI short-wave infrared measurements. It is validated against recent ground-based FTIR measurements from the TCCON network. A bias in TCCON HDO (which is not verified) is corrected by fitting a correction factor for the HDO column to match MUSICA δD for common observations. The use of the new TROPOMI data set is demonstrated using a case study of a blocking anticyclone over Europe in July 2018.
Keun-Ok Lee, Franziska Aemisegger, Stephan Pfahl, Cyrille Flamant, Jean-Lionel Lacour, and Jean-Pierre Chaboureau
Atmos. Chem. Phys., 19, 7487–7506, https://doi.org/10.5194/acp-19-7487-2019, https://doi.org/10.5194/acp-19-7487-2019, 2019
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Our study is the first study to investigate the potential benefit of stable water isotopes (SWIs) in the context of a heavy precipitation event in the Mediterranean. As such, our study provides a proof of concept of the usefulness of SWI data to understand the variety of origins and moisture processes associated with air masses feeding the convection over southern Italy.
Related subject area
Subject: Isotopes | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Estimating emissions of methane consistent with atmospheric measurements of methane and δ13C of methane
Stable water isotope signals in tropical ice clouds in the West African monsoon simulated with a regional convection-permitting model
Disentangling different moisture transport pathways over the eastern subtropical North Atlantic using multi-platform isotope observations and high-resolution numerical modelling
Firewood residential heating – local versus remote influence on the aerosol burden
Controls on the water vapor isotopic composition near the surface of tropical oceans and role of boundary layer mixing processes
Kinetic mass-transfer calculation of water isotope fractionation due to cloud microphysics in a regional meteorological model
The influence of 14CO2 releases from regional nuclear facilities at the Heidelberg 14CO2 sampling site (1986–2014)
Lagrangian process attribution of isotopic variations in near-surface water vapour in a 30-year regional climate simulation over Europe
How does sea ice influence δ18O of Arctic precipitation?
Separation of biospheric and fossil fuel fluxes of CO2 by atmospheric inversion of CO2 and 14CO2 measurements: Observation System Simulations
To what extent could water isotopic measurements help us understand model biases in the water cycle over Western Siberia
Simulating the integrated summertime Δ14CO2 signature from anthropogenic emissions over Western Europe
Variations of oxygen-18 in West Siberian precipitation during the last 50 years
Xenon-133 and caesium-137 releases into the atmosphere from the Fukushima Dai-ichi nuclear power plant: determination of the source term, atmospheric dispersion, and deposition
The isotopic composition of precipitation from a winter storm – a case study with the limited-area model COSMOiso
Theory of isotopic fractionation on facetted ice crystals
Radon activity in the lower troposphere and its impact on ionization rate: a global estimate using different radon emissions
Sourish Basu, Xin Lan, Edward Dlugokencky, Sylvia Michel, Stefan Schwietzke, John B. Miller, Lori Bruhwiler, Youmi Oh, Pieter P. Tans, Francesco Apadula, Luciana V. Gatti, Armin Jordan, Jaroslaw Necki, Motoki Sasakawa, Shinji Morimoto, Tatiana Di Iorio, Haeyoung Lee, Jgor Arduini, and Giovanni Manca
Atmos. Chem. Phys., 22, 15351–15377, https://doi.org/10.5194/acp-22-15351-2022, https://doi.org/10.5194/acp-22-15351-2022, 2022
Short summary
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Atmospheric methane (CH4) has been growing steadily since 2007 for reasons that are not well understood. Here we determine sources of methane using a technique informed by atmospheric measurements of CH4 and its isotopologue 13CH4. Measurements of 13CH4 provide for better separation of microbial, fossil, and fire sources of methane than CH4 measurements alone. Compared to previous assessments such as the Global Carbon Project, we find a larger microbial contribution to the post-2007 increase.
Andries Jan de Vries, Franziska Aemisegger, Stephan Pfahl, and Heini Wernli
Atmos. Chem. Phys., 22, 8863–8895, https://doi.org/10.5194/acp-22-8863-2022, https://doi.org/10.5194/acp-22-8863-2022, 2022
Short summary
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The Earth's water cycle contains the common H2O molecule but also the less abundant, heavier HDO. We use their different physical properties to study tropical ice clouds in model simulations of the West African monsoon. Isotope signals reveal different processes through which ice clouds form and decay in deep-convective and widespread cirrus. Previously observed variations in upper-tropospheric vapour isotopes are explained by microphysical processes in convective updraughts and downdraughts.
Fabienne Dahinden, Franziska Aemisegger, Heini Wernli, Matthias Schneider, Christopher J. Diekmann, Benjamin Ertl, Peter Knippertz, Martin Werner, and Stephan Pfahl
Atmos. Chem. Phys., 21, 16319–16347, https://doi.org/10.5194/acp-21-16319-2021, https://doi.org/10.5194/acp-21-16319-2021, 2021
Short summary
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We use high-resolution numerical isotope modelling and Lagrangian backward trajectories to identify moisture transport pathways and governing physical and dynamical processes that affect the free-tropospheric humidity and isotopic variability over the eastern subtropical North Atlantic. Furthermore, we conduct a thorough isotope modelling validation with aircraft and remote-sensing observations of water vapour isotopes.
Clara Betancourt, Christoph Küppers, Tammarat Piansawan, Uta Sager, Andrea B. Hoyer, Heinz Kaminski, Gerhard Rapp, Astrid C. John, Miriam Küpper, Ulrich Quass, Thomas Kuhlbusch, Jochen Rudolph, Astrid Kiendler-Scharr, and Iulia Gensch
Atmos. Chem. Phys., 21, 5953–5964, https://doi.org/10.5194/acp-21-5953-2021, https://doi.org/10.5194/acp-21-5953-2021, 2021
Short summary
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For the first time, we included stable isotopes in the Lagrangian particle dispersion model FLEXPART to investigate firewood home heating aerosol. This is an innovative source apportionment methodology since comparison of stable isotope ratio model predictions with observations delivers quantitative understanding of atmospheric processes. The main outcome of this study is that the home heating aerosol in residential areas was not of remote origin.
Camille Risi, Joseph Galewsky, Gilles Reverdin, and Florent Brient
Atmos. Chem. Phys., 19, 12235–12260, https://doi.org/10.5194/acp-19-12235-2019, https://doi.org/10.5194/acp-19-12235-2019, 2019
Short summary
Short summary
Water molecules can be light (one oxygen atom and two hydrogen atoms) or heavy (one hydrogen atom is replaced by a deuterium atom). These different molecules are called water isotopes. The isotopic composition of water vapor can potentially provide information about physical processes along the water cycle, but the factors controlling it are complex. As a first step, we propose an equation to predict the water vapor isotopic composition near the surface of tropical oceans.
I-Chun Tsai, Wan-Yu Chen, Jen-Ping Chen, and Mao-Chang Liang
Atmos. Chem. Phys., 19, 1753–1766, https://doi.org/10.5194/acp-19-1753-2019, https://doi.org/10.5194/acp-19-1753-2019, 2019
Short summary
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In conventional models, isotope exchange between liquid and gas phases is usually assumed to be in equilibrium, and the highly kinetic phase transformation processes inferred in clouds are yet to be fully investigated. We show that different factors controlling isotopic composition, including water vapor sources, atmospheric transport, phase transition pathways of water in clouds, and kinetic-versus-equilibrium mass transfer, contributed significantly to the variations in isotope composition.
Matthias Kuderer, Samuel Hammer, and Ingeborg Levin
Atmos. Chem. Phys., 18, 7951–7959, https://doi.org/10.5194/acp-18-7951-2018, https://doi.org/10.5194/acp-18-7951-2018, 2018
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Atmospheric 14CO2 measurements allow for estimating the regional fossil fuel CO2 component. However, results potentially need to be corrected for 14CO2 contamination from near-by nuclear facilities (NF). Our dispersion estimates of corresponding contaminations for Heidelberg, based on differently resolved wind fields, show differences of up to a factor of 2. Estimates from highly resolved models coupled with temporally resolved 14CO2 emissions from NFs are required for more accurate results.
Marina Dütsch, Stephan Pfahl, Miro Meyer, and Heini Wernli
Atmos. Chem. Phys., 18, 1653–1669, https://doi.org/10.5194/acp-18-1653-2018, https://doi.org/10.5194/acp-18-1653-2018, 2018
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Atmospheric processes are imprinted in the concentrations of stable water isotopes. Therefore, isotopes can be used to gain insight into these processes and improve our understanding of the water cycle. In this study, we present a new method that quantitatively shows which atmospheric processes influence isotope concentrations in near-surface water vapour over Europe. We found that the most important processes are evaporation from the ocean, evapotranspiration from land, and turbulent mixing.
Anne-Katrine Faber, Bo Møllesøe Vinther, Jesper Sjolte, and Rasmus Anker Pedersen
Atmos. Chem. Phys., 17, 5865–5876, https://doi.org/10.5194/acp-17-5865-2017, https://doi.org/10.5194/acp-17-5865-2017, 2017
Short summary
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The recent decades loss of Arctic sea ice provide an interesting opportunity to study the impact of sea ice changes on the isotopic composition of Arctic precipitation. Using a climate model that can simulate water isotopes, we find that reduced sea ice extent yields more enriched isotope values while increased sea ice extent yields more
depleted isotope values. Results also show that the spatial distribution of the sea ice extent are important.
Sourish Basu, John Bharat Miller, and Scott Lehman
Atmos. Chem. Phys., 16, 5665–5683, https://doi.org/10.5194/acp-16-5665-2016, https://doi.org/10.5194/acp-16-5665-2016, 2016
Short summary
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We present a dual tracer atmospheric inversion technique to separately estimate biospheric and fossil fuel CO2 fluxes from atmospheric measurements of CO2 and 14CO2. In addition to estimating monthly regional fossil fuel fluxes of CO2, this system can also reduce biases in biospheric fluxes that arise in a traditional CO2 inversion from prescribing a fixed but inaccurate fossil fuel flux.
V. Gryazin, C. Risi, J. Jouzel, N. Kurita, J. Worden, C. Frankenberg, V. Bastrikov, K. Gribanov, and O. Stukova
Atmos. Chem. Phys., 14, 9807–9830, https://doi.org/10.5194/acp-14-9807-2014, https://doi.org/10.5194/acp-14-9807-2014, 2014
D. Bozhinova, M. K. van der Molen, I. R. van der Velde, M. C. Krol, S. van der Laan, H. A. J. Meijer, and W. Peters
Atmos. Chem. Phys., 14, 7273–7290, https://doi.org/10.5194/acp-14-7273-2014, https://doi.org/10.5194/acp-14-7273-2014, 2014
M. Butzin, M. Werner, V. Masson-Delmotte, C. Risi, C. Frankenberg, K. Gribanov, J. Jouzel, and V. I. Zakharov
Atmos. Chem. Phys., 14, 5853–5869, https://doi.org/10.5194/acp-14-5853-2014, https://doi.org/10.5194/acp-14-5853-2014, 2014
A. Stohl, P. Seibert, G. Wotawa, D. Arnold, J. F. Burkhart, S. Eckhardt, C. Tapia, A. Vargas, and T. J. Yasunari
Atmos. Chem. Phys., 12, 2313–2343, https://doi.org/10.5194/acp-12-2313-2012, https://doi.org/10.5194/acp-12-2313-2012, 2012
S. Pfahl, H. Wernli, and K. Yoshimura
Atmos. Chem. Phys., 12, 1629–1648, https://doi.org/10.5194/acp-12-1629-2012, https://doi.org/10.5194/acp-12-1629-2012, 2012
J. Nelson
Atmos. Chem. Phys., 11, 11351–11360, https://doi.org/10.5194/acp-11-11351-2011, https://doi.org/10.5194/acp-11-11351-2011, 2011
K. Zhang, J. Feichter, J. Kazil, H. Wan, W. Zhuo, A. D. Griffiths, H. Sartorius, W. Zahorowski, M. Ramonet, M. Schmidt, C. Yver, R. E. M. Neubert, and E.-G. Brunke
Atmos. Chem. Phys., 11, 7817–7838, https://doi.org/10.5194/acp-11-7817-2011, https://doi.org/10.5194/acp-11-7817-2011, 2011
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Short summary
Stable water isotopes in marine boundary layer vapour are strongly influenced by the strength of air–sea fluxes. Here, we investigate a distinct vapour isotope signal observed in the warm sector of Southern Ocean cyclones. Single-process air parcel models are used together with high-resolution isotope-enabled simulations with the weather prediction model COSMOiso to improve our understanding of the importance of air–sea fluxes for the moisture cycling in the context of extratropical cyclones.
Stable water isotopes in marine boundary layer vapour are strongly influenced by the strength of...
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