Articles | Volume 21, issue 20
Atmos. Chem. Phys., 21, 15555–15567, 2021
https://doi.org/10.5194/acp-21-15555-2021

Special issue: Satellite and ground-based remote sensing of aerosol optical,...

Atmos. Chem. Phys., 21, 15555–15567, 2021
https://doi.org/10.5194/acp-21-15555-2021
Research article
18 Oct 2021
Research article | 18 Oct 2021

A black carbon peak and its sources in the free troposphere of Beijing induced by cyclone lifting and transport from central China

Zhenbin Wang et al.

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Cited articles

Bergin, M. H., Cass, G. R., Xu, J., Fang, C., Zeng, L. M., Yu, T., Salmon, L. G., Kiang, C. S., Tang, X. Y., Zhang, Y. H., and Chameides, W. L.: Aerosol radiative, physical, and chemical properties in Beijing during June 1999, J. Geophys. Res.-Atmos., 106, 17969–17980, https://doi.org/10.1029/2001JD900073, 2001. 
Bond, T. C., Streets, D. G., Yarber, K. F., Nelson, S. M., Woo, J. H., and Klimont, Z.: A technology-based global inventory of black and organic carbon emissions from combustion, J. Geophys. Res.-Atmos., 109, D14203, https://doi.org/10.1029/2003JD003697, 2004. 
Chen, F. and Dudhia, J.: Coupling an advanced land surface–hydrology model with the Penn state–NCAR MM5 modeling system. part I: model implementation and sensitivity, Mon. Weather Rev., 129, 569–585, https://doi.org/10.1175/1520-0493(2001)129<0569:CAALSH>2.0.CO;2, 2001. 
Chen, Z. H., Cheng, S. Y., Li, J. B., Guo, X. R., Wang, W. H., and Chen, D. S.: Relationship between atmospheric pollution processes and synoptic pressure patterns in northern China, Atmos. Environ., 42, 6078–6087, https://doi.org/10.1016/j.atmosenv.2008.03.043, 2008. 
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In this paper, by using WRF-Chem with a black carbon (BC) tagging technique, we investigate the formation mechanism and regional sources of a BC peak in the free troposphere observed by aircraft flights. Local sources dominated BC from the surface to about 700 m (78.5 %), while the BC peak in the free troposphere was almost entirely imported from external sources (99.8 %). Our results indicate that cyclone systems can quickly lift BC up to the free troposphere, as well as extend its lifetime.
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