Articles | Volume 13, issue 8
https://doi.org/10.5194/acp-13-3997-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-13-3997-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
18 Apr 2013
Research article |
| 18 Apr 2013
An empirical model of global climate – Part 1: A critical evaluation of volcanic cooling
T. Canty
Department of Atmospheric and Oceanic Science, University of Maryland, College Park, MD, USA
N. R. Mascioli
now at: Department of Earth and Environmental Sciences, Columbia University, New York, NY, USA
Department of Atmospheric and Oceanic Science, University of Maryland, College Park, MD, USA
M. D. Smarte
Department of Chemistry and Biochemistry, University of Maryland, College Park, MD, USA
R. J. Salawitch
Earth System Science Interdisciplinary Center, University of Maryland, College Park, MD, USA
Department of Chemistry and Biochemistry, University of Maryland, College Park, MD, USA
Department of Atmospheric and Oceanic Science, University of Maryland, College Park, MD, USA
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T. P. Canty, L. Hembeck, T. P. Vinciguerra, D. C. Anderson, D. L. Goldberg, S. F. Carpenter, D. J. Allen, C. P. Loughner, R. J. Salawitch, and R. R. Dickerson
Atmos. Chem. Phys., 15, 10965–10982, https://doi.org/10.5194/acp-15-10965-2015, https://doi.org/10.5194/acp-15-10965-2015, 2015
J. P. Parrella, K. Chance, R. J. Salawitch, T. Canty, M. Dorf, and K. Pfeilsticker
Atmos. Meas. Tech., 6, 2549–2561, https://doi.org/10.5194/amt-6-2549-2013, https://doi.org/10.5194/amt-6-2549-2013, 2013
H. He, J. W. Stehr, J. C. Hains, D. J. Krask, B. G. Doddridge, K. Y. Vinnikov, T. P. Canty, K. M. Hosley, R. J. Salawitch, H. M. Worden, and R. R. Dickerson
Atmos. Chem. Phys., 13, 7859–7874, https://doi.org/10.5194/acp-13-7859-2013, https://doi.org/10.5194/acp-13-7859-2013, 2013
Endre Z. Farago, Laura A. McBride, Austin P. Hope, Timothy P. Canty, Brian F. Bennett, and Ross J. Salawitch
EGUsphere, https://doi.org/10.5194/egusphere-2025-342, https://doi.org/10.5194/egusphere-2025-342, 2025
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We use a reduced-complexity climate model trained by observations to compute the future rise in global mean surface temperature (GMST) for radiative forcing (RF) due to greenhouse gases (GHGs) and tropospheric aerosols, provided by the IPCC AR5 and AR6 reports. We show that the AR6 updates to RF lead to a 0.2 to 0.4 °C rise in GMST at the end of this century, for the same underlying Shared Socioeconomic Pathway emissions projections of GHGs and aerosols, relative to GMST found using RF from AR5.
Megan J. Lickley, John S. Daniel, Laura A. McBride, Ross J. Salawitch, and Guus J. M. Velders
Atmos. Chem. Phys., 24, 13081–13099, https://doi.org/10.5194/acp-24-13081-2024, https://doi.org/10.5194/acp-24-13081-2024, 2024
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The expected ozone recovery date was delayed by 17 years between the 2006 and 2022 international scientific assessments of ozone depletion. We quantify the primary drivers of this delay. Changes in the metric used to estimate ozone recovery explain ca. 5 years of this delay. Of the remaining 12 years, changes in estimated banks, atmospheric lifetimes, and emission projections explain 4, 3.5, and 3 years of this delay, respectively.
Laura A. McBride, Austin P. Hope, Timothy P. Canty, Brian F. Bennett, Walter R. Tribett, and Ross J. Salawitch
Earth Syst. Dynam., 12, 545–579, https://doi.org/10.5194/esd-12-545-2021, https://doi.org/10.5194/esd-12-545-2021, 2021
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We use a reduced-complexity climate model trained by observations to show that at the current rate of human release of CO2, total cumulative emissions will pass the 66 % likelihood of limiting warming to 1.5° or 2°C in about 10 and 35 years, respectively. We also show that complex climate models often used to guide policy tend to warm faster than observed over the past few decades. To achieve the Paris Climate Agreement, CO2 and CH4 emissions must be severely curtailed in the next decade.
Sarah E. Benish, Hao He, Xinrong Ren, Sandra J. Roberts, Ross J. Salawitch, Zhanqing Li, Fei Wang, Yuying Wang, Fang Zhang, Min Shao, Sihua Lu, and Russell R. Dickerson
Atmos. Chem. Phys., 20, 14523–14545, https://doi.org/10.5194/acp-20-14523-2020, https://doi.org/10.5194/acp-20-14523-2020, 2020
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Airborne observations of ozone and related pollutants show smog was pervasive in spring 2016 over Hebei Province, China. We find high amounts of ozone precursors throughout and even above the PBL, continuing to generate ozone at high rates to be potentially transported downwind. Concentrations even in the rural areas of this highly industrialized province promote widespread ozone production, and we show that to improve air quality over Hebei both NOx and VOCs should be targeted.
Zebedee R. J. Nicholls, Malte Meinshausen, Jared Lewis, Robert Gieseke, Dietmar Dommenget, Kalyn Dorheim, Chen-Shuo Fan, Jan S. Fuglestvedt, Thomas Gasser, Ulrich Golüke, Philip Goodwin, Corinne Hartin, Austin P. Hope, Elmar Kriegler, Nicholas J. Leach, Davide Marchegiani, Laura A. McBride, Yann Quilcaille, Joeri Rogelj, Ross J. Salawitch, Bjørn H. Samset, Marit Sandstad, Alexey N. Shiklomanov, Ragnhild B. Skeie, Christopher J. Smith, Steve Smith, Katsumasa Tanaka, Junichi Tsutsui, and Zhiang Xie
Geosci. Model Dev., 13, 5175–5190, https://doi.org/10.5194/gmd-13-5175-2020, https://doi.org/10.5194/gmd-13-5175-2020, 2020
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Computational limits mean that we cannot run our most comprehensive climate models for all applications of interest. In such cases, reduced complexity models (RCMs) are used. Here, researchers working on 15 different models present the first systematic community effort to evaluate and compare RCMs: the Reduced Complexity Model Intercomparison Project (RCMIP). Our research ensures that users of RCMs can more easily evaluate the strengths, weaknesses and limitations of their tools.
J. Eric Klobas, Debra K. Weisenstein, Ross J. Salawitch, and David M. Wilmouth
Atmos. Chem. Phys., 20, 9459–9471, https://doi.org/10.5194/acp-20-9459-2020, https://doi.org/10.5194/acp-20-9459-2020, 2020
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The rates of important ozone-destroying chemical reactions in the stratosphere are likely to change in the future. We employ a computer model to evaluate how the rates of ozone destruction by chlorine and bromine may evolve in four climate change scenarios with the introduction of the eta factor. We then show how these changing rates will impact the ozone-depleting power of the stratosphere with a new metric known as Equivalent Effective Stratospheric Benchmark-normalized Chlorine (EESBnC).
Julie M. Nicely, Bryan N. Duncan, Thomas F. Hanisco, Glenn M. Wolfe, Ross J. Salawitch, Makoto Deushi, Amund S. Haslerud, Patrick Jöckel, Béatrice Josse, Douglas E. Kinnison, Andrew Klekociuk, Michael E. Manyin, Virginie Marécal, Olaf Morgenstern, Lee T. Murray, Gunnar Myhre, Luke D. Oman, Giovanni Pitari, Andrea Pozzer, Ilaria Quaglia, Laura E. Revell, Eugene Rozanov, Andrea Stenke, Kane Stone, Susan Strahan, Simone Tilmes, Holger Tost, Daniel M. Westervelt, and Guang Zeng
Atmos. Chem. Phys., 20, 1341–1361, https://doi.org/10.5194/acp-20-1341-2020, https://doi.org/10.5194/acp-20-1341-2020, 2020
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Differences in methane lifetime among global models are large and poorly understood. We use a neural network method and simulations from the Chemistry Climate Model Initiative to quantify the factors influencing methane lifetime spread among models and variations over time. UV photolysis, tropospheric ozone, and nitrogen oxides drive large model differences, while the same factors plus specific humidity contribute to a decreasing trend in methane lifetime between 1980 and 2015.
Liang Feng, Paul I. Palmer, Robyn Butler, Stephen J. Andrews, Elliot L. Atlas, Lucy J. Carpenter, Valeria Donets, Neil R. P. Harris, Ross J. Salawitch, Laura L. Pan, and Sue M. Schauffler
Atmos. Chem. Phys., 18, 14787–14798, https://doi.org/10.5194/acp-18-14787-2018, https://doi.org/10.5194/acp-18-14787-2018, 2018
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We infer surface fluxes of bromoform (CHBr3) and dibromoform (CH2Br2) from CAST and CONTRAST aircraft observations over the western Pacific, using a tagged version of the GEOS-Chem global 3-D atmospheric chemistry model and a Maximum A Posteriori inverse model. Using the aircraft data, we estimate the regional fluxes about 20–40 % smaller than the prior inventories by Ordóñez et al. (2012). We find no evidence to support a robust linear relationship between CHBr3 and CH2Br2 oceanic emissions.
Robyn Butler, Paul I. Palmer, Liang Feng, Stephen J. Andrews, Elliot L. Atlas, Lucy J. Carpenter, Valeria Donets, Neil R. P. Harris, Stephen A. Montzka, Laura L. Pan, Ross J. Salawitch, and Sue M. Schauffler
Atmos. Chem. Phys., 18, 13135–13153, https://doi.org/10.5194/acp-18-13135-2018, https://doi.org/10.5194/acp-18-13135-2018, 2018
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Natural sources of short-lived bromoform and dibromomethane are important for determining the inorganic bromine budget in the stratosphere that drives ozone loss. Two new modelling techniques describe how different geographical source regions influence their atmospheric variability over the western Pacific. We find that it is driven primarily by open ocean sources, and we use atmospheric observations to help estimate their contributions to the upper tropospheric inorganic bromine budget.
Sandip S. Dhomse, Douglas Kinnison, Martyn P. Chipperfield, Ross J. Salawitch, Irene Cionni, Michaela I. Hegglin, N. Luke Abraham, Hideharu Akiyoshi, Alex T. Archibald, Ewa M. Bednarz, Slimane Bekki, Peter Braesicke, Neal Butchart, Martin Dameris, Makoto Deushi, Stacey Frith, Steven C. Hardiman, Birgit Hassler, Larry W. Horowitz, Rong-Ming Hu, Patrick Jöckel, Beatrice Josse, Oliver Kirner, Stefanie Kremser, Ulrike Langematz, Jared Lewis, Marion Marchand, Meiyun Lin, Eva Mancini, Virginie Marécal, Martine Michou, Olaf Morgenstern, Fiona M. O'Connor, Luke Oman, Giovanni Pitari, David A. Plummer, John A. Pyle, Laura E. Revell, Eugene Rozanov, Robyn Schofield, Andrea Stenke, Kane Stone, Kengo Sudo, Simone Tilmes, Daniele Visioni, Yousuke Yamashita, and Guang Zeng
Atmos. Chem. Phys., 18, 8409–8438, https://doi.org/10.5194/acp-18-8409-2018, https://doi.org/10.5194/acp-18-8409-2018, 2018
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We analyse simulations from the Chemistry-Climate Model Initiative (CCMI) to estimate the return dates of the stratospheric ozone layer from depletion by anthropogenic chlorine and bromine. The simulations from 20 models project that global column ozone will return to 1980 values in 2047 (uncertainty range 2042–2052). Return dates in other regions vary depending on factors related to climate change and importance of chlorine and bromine. Column ozone in the tropics may continue to decline.
Theodore K. Koenig, Rainer Volkamer, Sunil Baidar, Barbara Dix, Siyuan Wang, Daniel C. Anderson, Ross J. Salawitch, Pamela A. Wales, Carlos A. Cuevas, Rafael P. Fernandez, Alfonso Saiz-Lopez, Mathew J. Evans, Tomás Sherwen, Daniel J. Jacob, Johan Schmidt, Douglas Kinnison, Jean-François Lamarque, Eric C. Apel, James C. Bresch, Teresa Campos, Frank M. Flocke, Samuel R. Hall, Shawn B. Honomichl, Rebecca Hornbrook, Jørgen B. Jensen, Richard Lueb, Denise D. Montzka, Laura L. Pan, J. Michael Reeves, Sue M. Schauffler, Kirk Ullmann, Andrew J. Weinheimer, Elliot L. Atlas, Valeria Donets, Maria A. Navarro, Daniel Riemer, Nicola J. Blake, Dexian Chen, L. Gregory Huey, David J. Tanner, Thomas F. Hanisco, and Glenn M. Wolfe
Atmos. Chem. Phys., 17, 15245–15270, https://doi.org/10.5194/acp-17-15245-2017, https://doi.org/10.5194/acp-17-15245-2017, 2017
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Tropospheric inorganic bromine (BrO and Bry) shows a C-shaped profile over the tropical western Pacific Ocean, and supports previous speculation that marine convection is a source for inorganic bromine from sea salt to the upper troposphere. The Bry profile in the tropical tropopause layer (TTL) is complex, suggesting that the total Bry budget in the TTL is not closed without considering aerosol bromide. The implications for atmospheric composition and bromine sources are discussed.
T. P. Canty, L. Hembeck, T. P. Vinciguerra, D. C. Anderson, D. L. Goldberg, S. F. Carpenter, D. J. Allen, C. P. Loughner, R. J. Salawitch, and R. R. Dickerson
Atmos. Chem. Phys., 15, 10965–10982, https://doi.org/10.5194/acp-15-10965-2015, https://doi.org/10.5194/acp-15-10965-2015, 2015
R. P. Fernandez, R. J. Salawitch, D. E. Kinnison, J.-F. Lamarque, and A. Saiz-Lopez
Atmos. Chem. Phys., 14, 13391–13410, https://doi.org/10.5194/acp-14-13391-2014, https://doi.org/10.5194/acp-14-13391-2014, 2014
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We propose the existence of a daytime “tropical ring of atomic bromine” surrounding the tropics at a height between 15 and 19km. Our simulations show that VSL bromocarbons produce increases of 3pptv for inorganic bromine and 2pptv for organic bromine in the tropical TTL on an annual average, resulting in a total stratospheric bromine injection of 5pptv. This result suggests that the inorganic bromine injected into the stratosphere may be larger than that from VSL bromocarbons.
J. P. Parrella, K. Chance, R. J. Salawitch, T. Canty, M. Dorf, and K. Pfeilsticker
Atmos. Meas. Tech., 6, 2549–2561, https://doi.org/10.5194/amt-6-2549-2013, https://doi.org/10.5194/amt-6-2549-2013, 2013
H. He, J. W. Stehr, J. C. Hains, D. J. Krask, B. G. Doddridge, K. Y. Vinnikov, T. P. Canty, K. M. Hosley, R. J. Salawitch, H. M. Worden, and R. R. Dickerson
Atmos. Chem. Phys., 13, 7859–7874, https://doi.org/10.5194/acp-13-7859-2013, https://doi.org/10.5194/acp-13-7859-2013, 2013
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Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Regional variability of aerosol impacts on clouds and radiation in global kilometer-scale simulations
A novel method to quantify the uncertainty contribution of aerosol–radiation interaction factors
Exploring the aerosol activation properties in coastal shallow convection using cloud- and particle-resolving models
Machine-learning-assisted inference of the particle charge fraction and the ion-induced nucleation rates during new particle formation events
Modeling CMAQ dry deposition treatment over the western Pacific: a distinct characteristic of mineral dust and anthropogenic aerosols
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How to trace the origins of short-lived atmospheric species: an Arctic example
Dust-producing weather patterns of the North American Great Plains
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Interdecadal shift in the impact of winter land-sea thermal contrasts on following spring transcontinental dust transport pathways in North Africa
Anthropogenic and Natural Causes for the Interannual Variation of PM2.5 in East Asia During Summer Monsoon Periods From 2008 to 2018
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Characterization of brown carbon absorption in different European environments through source contribution analysis
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The effectiveness of solar radiation management using fine sea spray across multiple climatic regions
A global dust emission dataset for estimating dust radiative forcings in climate models
Tropospheric aerosols over the western North Atlantic Ocean during the winter and summer deployments of ACTIVATE 2020: life cycle, transport, and distribution
Spatial and temporal evolution of future atmospheric reactive nitrogen deposition in China under different climate change mitigation strategies
Steady-state mixing state of black carbon aerosols from a particle-resolved model
Direct radiative forcing of light-absorbing carbonaceous aerosol and the influencing factors over China
Distinctive dust weather intensities in North China resulted from two types of atmospheric circulation anomalies
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The effect of organic nucleation on the indirect radiative forcing with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs)
Quasi-weekly oscillation of regional PM2.5 transport over China driven by the synoptic-scale disturbance of the East Asian winter monsoon circulation
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Homogeneous ice nucleation in adsorbed water films: A theoretical approach
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The role of interfacial tension in the size-dependent phase separation of atmospheric aerosol particles
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Seasonal differences in observed versus modeled new particle formation over boreal regions
Warming effects of reduced sulfur emissions from shipping
The key role of atmospheric absorption in the Asian summer monsoon response to dust emissions in CMIP6 models
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Radiative and climate effects of aerosol scattering in long-wave radiation based on global climate modeling
Revealing dominant patterns of aerosol regimes in the lower troposphere and their evolution from preindustrial times to the future in global climate model simulations
Improving estimation of a record-breaking east Asian dust storm emission with lagged aerosol Ångström exponent observations
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Ross J. Herbert, Andrew I. L. Williams, Philipp Weiss, Duncan Watson-Parris, Elisabeth Dingley, Daniel Klocke, and Philip Stier
Atmos. Chem. Phys., 25, 7789–7814, https://doi.org/10.5194/acp-25-7789-2025, https://doi.org/10.5194/acp-25-7789-2025, 2025
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Clouds exist at scales that climate models struggle to represent, limiting our knowledge of how climate change may impact clouds. Here we use a new kilometer-scale global model representing an important step towards the necessary scale. We focus on how aerosol particles modify clouds, radiation, and precipitation. We find the magnitude and manner of responses tend to vary from region to region, highlighting the potential of global kilometer-scale simulations and a need to represent aerosols in climate models.
Bishuo He and Chunsheng Zhao
Atmos. Chem. Phys., 25, 7765–7776, https://doi.org/10.5194/acp-25-7765-2025, https://doi.org/10.5194/acp-25-7765-2025, 2025
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Factor uncertainty analysis helps us understand the impacts of factors on complex systems. Traditional methods have many limitations. This study introduces a new method to measure how each factor contributes to uncertainty. It gains insights into the role of each variable and works for all multi-factor systems. As an application, we analyzed how aerosols affect solar radiation and identified the key factors. These analyses can improve our understanding of the role of aerosols in climate change.
Ge Yu, Yueya Wang, Zhe Wang, and Xiaoming Shi
Atmos. Chem. Phys., 25, 7527–7542, https://doi.org/10.5194/acp-25-7527-2025, https://doi.org/10.5194/acp-25-7527-2025, 2025
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Studying the cloud-forming capacity of aerosols is crucial in climate research. The PartMC model can provide detailed particle information and help these studies. This model is integrated with the ideal meteorological Cloud Model 1 (CM1) to simulate the aerosols at cloud-forming locations. Significant changes are revealed in the hygroscopicity distribution of aerosols within ascending air parcels. Additionally, different ascent times also affect aerosol aging processes.
Pan Wang, Yue Zhao, Jiandong Wang, Veli-Matti Kerminen, Jingkun Jiang, and Chenxi Li
Atmos. Chem. Phys., 25, 7431–7446, https://doi.org/10.5194/acp-25-7431-2025, https://doi.org/10.5194/acp-25-7431-2025, 2025
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We developed a numerical model to investigate the evolution of the charge state of newly formed atmospheric particles. Based on the simulation results, we successfully employed neural networks to predict particle charge states and estimate ion-induced nucleation rates. This study provides new insights into the dynamics of particle charging and introduces advanced methods for evaluating ion-induced nucleation in atmospheric research.
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Atmos. Chem. Phys., 25, 7245–7268, https://doi.org/10.5194/acp-25-7245-2025, https://doi.org/10.5194/acp-25-7245-2025, 2025
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The accuracy of the chemical transport model, a key focus of our research, is strongly dependent on the dry deposition parameterization. Our findings show that the refined CMAQ dust model correlated well with ground-based and high-altitude in situ measurements by implementing the suggested dry deposition schemes. Furthermore, we reveal the mixing state of two types of aerosols at the upper level, a finding supported by both the optimized model and measurements.
Mizuo Kajino, Kentaro Ishijima, Joseph Ching, Kazuyo Yamaji, Rio Ishikawa, Tomoki Kajikawa, Tanbir Singh, Tomoki Nakayama, Yutaka Matsumi, Koyo Kojima, Taisei Machida, Takashi Maki, Prabir K. Patra, and Sachiko Hayashida
Atmos. Chem. Phys., 25, 7137–7160, https://doi.org/10.5194/acp-25-7137-2025, https://doi.org/10.5194/acp-25-7137-2025, 2025
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Air pollution in Delhi during the post-monsoon period is severe, and association with intensive crop residue burning (CRB) over Punjab state has attracted attention. However, the relationship has been unclear as the CRB emissions conventionally derived from satellites were underestimated due to clouds or thick smoke/haze over the region. We evaluated the impact of CRB on PM2.5 to be about 50 %, based on a combination of numerical modeling and an observation network using low-cost sensors we installed.
Huiyun Du, Jie Li, Xueshun Chen, Gabriele Curci, Fangqun Yu, Yele Sun, Xu Dao, Song Guo, Zhe Wang, Wenyi Yang, Lianfang Wei, and Zifa Wang
Atmos. Chem. Phys., 25, 5665–5681, https://doi.org/10.5194/acp-25-5665-2025, https://doi.org/10.5194/acp-25-5665-2025, 2025
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Inadequate consideration of mixing states and coatings on black carbon (BC) hinders aerosol radiation forcing quantification. Core–shell mixing aligns well with observations, but partial internal mixing is a more realistic representation. We used a microphysics module to determine the fraction of embedded BC and coating aerosols, constraining the mixing state. This reduced absorption enhancement by 30 %–43 % in northern China, offering insights into BC's radiative effects.
Zhixin Xue, Nair Udaysankar, and Sundar A. Christopher
Atmos. Chem. Phys., 25, 5497–5517, https://doi.org/10.5194/acp-25-5497-2025, https://doi.org/10.5194/acp-25-5497-2025, 2025
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Canadian wildfires in August 2018 significantly increased surface air pollution across the United States (US) – by up to 69 % in some areas. Using model, satellite, and ground measurements, the study highlights how weather patterns and long-range smoke transport drive pollution. The northwestern US was most affected by Canadian wildfire smoke, while the northeastern US experienced the least impact. These findings indicate the growing concern that wildfire smoke poses to air quality across the US.
Anderson Da Silva, Louis Marelle, Jean-Christophe Raut, Yvette Gramlich, Karolina Siegel, Sophie L. Haslett, Claudia Mohr, and Jennie L. Thomas
Atmos. Chem. Phys., 25, 5331–5354, https://doi.org/10.5194/acp-25-5331-2025, https://doi.org/10.5194/acp-25-5331-2025, 2025
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Particle sources in polar climates are unclear, affecting climate representation in models. This study introduces an evaluated method for tracking particles with backward modeling. Tests on simulated particles allowed us to show that traditional detection methods often misidentify sources. An improved method that accurately traces the origins of aerosol particles in the Arctic is presented. The study recommends using this enhanced method for better source identification of atmospheric species.
Stuart Evans
Atmos. Chem. Phys., 25, 4833–4845, https://doi.org/10.5194/acp-25-4833-2025, https://doi.org/10.5194/acp-25-4833-2025, 2025
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This study of the North American Great Plains identifies the various weather patterns responsible for blowing dust in all parts of the region using a weather pattern classification. In the southwestern plains passing cold fronts are the primary cause of dust; in the understudied northern plains, summertime patterns and southerly pre-frontal winds are most important in the west and east, respectively. These results are valuable to understanding and forecasting dust in this complex source region.
Camelia Talianu, Jeni Vasilescu, Doina Nicolae, Alexandru Ilie, Andrei Dandocsi, Anca Nemuc, and Livio Belegante
Atmos. Chem. Phys., 25, 4639–4654, https://doi.org/10.5194/acp-25-4639-2025, https://doi.org/10.5194/acp-25-4639-2025, 2025
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For Bucharest, Romania's capital, mobile measurements during two intensive campaigns and mixed-effect LUR (land-use regression) models to derive seasonal maps of near-surface PM10, NO2 and UFPs (ultrafine particles) have successfully been used. The model's performance was evaluated, demonstrating its potential for high-resolution mapping in other cities with well-characterized urban structures and diverse in situ monitoring stations.
Qi Wen, Yan Li, Mengying Du, Wenjun Song, Linbo Wei, Zhilan Wang, and Xu Li
EGUsphere, https://doi.org/10.5194/egusphere-2025-826, https://doi.org/10.5194/egusphere-2025-826, 2025
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We find that, through an interdecadal phase-locking effect of sea-land thermal forcing-North Atlantic Oscillation-Westerly Jet coupling, springtime dust from North Africa is more likely to be transported eastwards (extending into North America) after the late 1990s, whereas before that time westward transport paths for dust were more frequent. Subject to thermal forcing, wind speed and drought contribute to dust emissions in the two periods, respectively.
Danyang Ma, Min Xie, Huan He, Tijian Wang, Mengzhu Xi, Lingyun Feng, Shuxian Zhang, and Shitong Chen
EGUsphere, https://doi.org/10.5194/egusphere-2025-10, https://doi.org/10.5194/egusphere-2025-10, 2025
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The PM2.5 concentration in China underwent significant changes in 2013. We examined the underlying causes from three perspectives: anthropogenic pollutant emissions, meteorological conditions, and CO2 concentration variations. Our study highlighted the importance of considering the role of CO2 on vegetation when predicting PM2.5 concentrations and developing corresponding control strategies.
Jiangtao Li, Xingqin An, Zhaobin Sun, Caihua Ye, Qing Hou, Yuxin Zhao, and Zhe Liu
Atmos. Chem. Phys., 25, 3583–3602, https://doi.org/10.5194/acp-25-3583-2025, https://doi.org/10.5194/acp-25-3583-2025, 2025
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Climate change and pollution have intensified pollen allergies. We developed a pollen emissions model using phenology and random forests. Key factors affecting annual pollen emissions include temperature, relative humidity and sunshine hours. Pollen dispersal starts around 10 August, peaks around 30 August and ends by 25 September, lasting about 45 d. Over time, annual pollen emissions exhibit significant fluctuations and a downward trend.
Joe Adabouk Amooli, Marianne T. Lund, Sourangsu Chowdhury, Gunnar Myhre, Ane N. Johansen, Bjørn H. Samset, and Daniel M. Westervelt
EGUsphere, https://doi.org/10.5194/egusphere-2025-948, https://doi.org/10.5194/egusphere-2025-948, 2025
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We analyze various projections of African aerosol emissions and their potential impacts on climate and public health. We find that future emissions vary widely across emission projections, with differences in sectoral emission distributions. Using the Oslo chemical transport model, we show that air pollution exposure in some regions of Africa could increase significantly by 2050, increasing pollution-related deaths, with most scenarios projecting aerosol-induced warming over sub-Saharan Africa.
Ruth A. R. Digby, Knut von Salzen, Adam H. Monahan, Nathan P. Gillett, and Jiangnan Li
Atmos. Chem. Phys., 25, 3109–3130, https://doi.org/10.5194/acp-25-3109-2025, https://doi.org/10.5194/acp-25-3109-2025, 2025
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The refractive index of black carbon (BCRI), which determines how much energy black carbon absorbs and scatters, is difficult to measure, and different climate models use different values. We show that varying the BCRI across commonly used values can increase absorbing aerosol optical depth by 42 % and the warming effect from interactions between black carbon and radiation by 47 %, an appreciable fraction of the overall spread between models reported in recent literature assessments.
Valtteri Tikkanen, Huan Yang, Hanna Vehkamäki, and Bernhard Reischl
EGUsphere, https://doi.org/10.5194/egusphere-2025-507, https://doi.org/10.5194/egusphere-2025-507, 2025
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Collisions of neutral molecules and clusters is the prevalent pathway in atmospheric new particle formation. In heavily polluted urban areas, where clusters are formed rapidly and in large number, cluster-cluster collisions also become relevant. We calculate cluster-cluster collision rates from atomistic molecular dynamics simulations and an interacting hard sphere model. Not accounting for long-range attractive interactions underestimates collision and particle formation rates significantly.
George Jordan, Florent Malavelle, Jim Haywood, Ying Chen, Ben Johnson, Daniel Partridge, Amy Peace, Eliza Duncan, Duncan Watson-Parris, David Neubauer, Anton Laakso, Martine Michou, and Pierre Nabat
EGUsphere, https://doi.org/10.5194/egusphere-2025-835, https://doi.org/10.5194/egusphere-2025-835, 2025
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The 2014–15 Holuhraun eruption created a vast aerosol plume that acted as a natural experiment to assess how well climate models capture changes in cloud properties due to increased aerosol. We find that the models accurately represent the observed shift to smaller, more numerous cloud droplets. However, the models diverge in their aerosol induced changes to large-scale cloud properties, particularly cloud liquid water content. Our study shows that Holuhraun had a cooling effect on the Earth.
Hector Navarro-Barboza, Jordi Rovira, Vincenzo Obiso, Andrea Pozzer, Marta Via, Andres Alastuey, Xavier Querol, Noemi Perez, Marjan Savadkoohi, Gang Chen, Jesus Yus-Díez, Matic Ivancic, Martin Rigler, Konstantinos Eleftheriadis, Stergios Vratolis, Olga Zografou, Maria Gini, Benjamin Chazeau, Nicolas Marchand, Andre S. H. Prevot, Kaspar Dallenbach, Mikael Ehn, Krista Luoma, Tuukka Petäjä, Anna Tobler, Jaroslaw Necki, Minna Aurela, Hilkka Timonen, Jarkko Niemi, Olivier Favez, Jean-Eudes Petit, Jean-Philippe Putaud, Christoph Hueglin, Nicolas Pascal, Aurélien Chauvigné, Sébastien Conil, Marco Pandolfi, and Oriol Jorba
Atmos. Chem. Phys., 25, 2667–2694, https://doi.org/10.5194/acp-25-2667-2025, https://doi.org/10.5194/acp-25-2667-2025, 2025
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Brown carbon (BrC) absorbs ultraviolet (UV) and visible light, influencing climate. This study explores BrC's imaginary refractive index (k) using data from 12 European sites. Residential emissions are a major organic aerosol (OA) source in winter, while secondary organic aerosol (SOA) dominates in summer. Source-specific k values were derived, improving model accuracy. The findings highlight BrC's climate impact and emphasize source-specific constraints in atmospheric models.
Yuzhi Jin, Jiandong Wang, Chao Liu, David C. Wong, Golam Sarwar, Kathleen M. Fahey, Shang Wu, Jiaping Wang, Jing Cai, Zeyuan Tian, Zhouyang Zhang, Jia Xing, Aijun Ding, and Shuxiao Wang
Atmos. Chem. Phys., 25, 2613–2630, https://doi.org/10.5194/acp-25-2613-2025, https://doi.org/10.5194/acp-25-2613-2025, 2025
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Black carbon (BC) affects climate and the environment, and its aging process alters its properties. Current models, like WRF-CMAQ, lack full accounting for it. We developed the WRF-CMAQ-BCG model to better represent BC aging by introducing bare and coated BC species and their conversion. The WRF-CMAQ-BCG model introduces the capability to simulate BC mixing states and bare and coated BC wet deposition, and it improves the accuracy of BC mass concentration and aerosol optics.
Zhe Song, Shaocai Yu, Pengfei Li, Ningning Yao, Lang Chen, Yuhai Sun, Boqiong Jiang, and Daniel Rosenfeld
Atmos. Chem. Phys., 25, 2473–2494, https://doi.org/10.5194/acp-25-2473-2025, https://doi.org/10.5194/acp-25-2473-2025, 2025
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Our results with injected sea salt aerosols for five open oceans show that sea salt aerosols with low injection amounts dominate shortwave radiation, mainly through indirect effects. As indirect aerosol effects saturate with increasing injection rates, direct effects exceed indirect effects. This implies that marine cloud brightening is best implemented in areas with extensive cloud cover, while aerosol direct scattering effects remain dominant when clouds are scarce.
Danny M. Leung, Jasper F. Kok, Longlei Li, David M. Lawrence, Natalie M. Mahowald, Simone Tilmes, and Erik Kluzek
Atmos. Chem. Phys., 25, 2311–2331, https://doi.org/10.5194/acp-25-2311-2025, https://doi.org/10.5194/acp-25-2311-2025, 2025
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This study derives a gridded dust emission dataset for 1841–2000 by employing a combination of observed dust from core records and reanalyzed global dust cycle constraints. We evaluate the ability of global models to replicate the observed historical dust variability by using the emission dataset to force a historical simulation in an Earth system model. We show that prescribing our emissions forces the model to better match observations than other mechanistic models.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
Atmos. Chem. Phys., 25, 2087–2121, https://doi.org/10.5194/acp-25-2087-2025, https://doi.org/10.5194/acp-25-2087-2025, 2025
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We use the GEOS-Chem model to simulate aerosol distributions and properties over the western North Atlantic Ocean (WNAO) during the winter and summer deployments in 2020 of the NASA ACTIVATE mission. Model results are evaluated against aircraft, ground-based, and satellite observations. The improved understanding of life cycle, composition, transport pathways, and distribution of aerosols has important implications for characterizing aerosol–cloud–meteorology interactions over WNAO.
Mingrui Ma, Jiachen Cao, Dan Tong, Bo Zheng, and Yu Zhao
Atmos. Chem. Phys., 25, 2147–2166, https://doi.org/10.5194/acp-25-2147-2025, https://doi.org/10.5194/acp-25-2147-2025, 2025
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We combined two global climate change pathways and three national emission control scenarios to analyze the future evolution of reactive nitrogen (Nr) deposition till the 2060s in China with air quality modeling. We show China’s clean air and carbon neutrality policies would overcome the adverse effects of climate change and efficiently reduce Nr deposition. The outflow of Nr fluxes from mainland China to the west Pacific would also be clearly reduced from continuous stringent emission controls.
Zhouyang Zhang, Jiandong Wang, Jiaping Wang, Nicole Riemer, Chao Liu, Yuzhi Jin, Zeyuan Tian, Jing Cai, Yueyue Cheng, Ganzhen Chen, Bin Wang, Shuxiao Wang, and Aijun Ding
Atmos. Chem. Phys., 25, 1869–1881, https://doi.org/10.5194/acp-25-1869-2025, https://doi.org/10.5194/acp-25-1869-2025, 2025
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Black carbon (BC) exerts notable warming effects. We use a particle-resolved model to investigate the long-term behavior of the BC mixing state, revealing its compositions, coating thickness distribution, and optical properties all stabilize with a characteristic time of less than 1 d. This study can effectively simplify the description of the BC mixing state, which facilitates the precise assessment of the optical properties of BC aerosols in global and chemical transport models.
Shuangqin Yang, Yusi Liu, Li Chen, Nan Cao, Jing Wang, and Shuang Gao
EGUsphere, https://doi.org/10.5194/egusphere-2024-3705, https://doi.org/10.5194/egusphere-2024-3705, 2025
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Black carbon, primary brown carbon, and secondary brown carbon are the leading light-absorbing carbonaceous aerosols (LACs) that contribute significantly to climate change. We modified the GEOS-Chem model to simulate the climate change by LACs based on local emission inventory, and explored the impacts of LACs properties and atmospheric variables on the corresponding DRFs in seven regions of China. The study confirms the warming effect of LACs and deepens our knowledge of their climatic effects.
Qianyi Huo, Zhicong Yin, Xiaoqing Ma, and Huijun Wang
Atmos. Chem. Phys., 25, 1711–1724, https://doi.org/10.5194/acp-25-1711-2025, https://doi.org/10.5194/acp-25-1711-2025, 2025
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Dust days during the spring seasons of 2015–2023 in North China were classified into Mongolian cyclone and cold high types depending on the presence of the Mongolian cyclone. The Mongolian cyclone type led to more frequent and severe dust weather, indicated by PM10 concentrations. To comprehensively forecast the two types of dust weather, a common predictor was established based on 500 hPa anomalous circulation systems, offering insights for dust weather forecasting and climate prediction.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes W. Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
Atmos. Chem. Phys., 25, 1545–1567, https://doi.org/10.5194/acp-25-1545-2025, https://doi.org/10.5194/acp-25-1545-2025, 2025
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We compared smoke plume simulations from 11 global models to each other and to satellite smoke amount observations aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss rate assumptions vary enormously among models, causing uncertainties that require systematic in situ measurements to resolve.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Stephen R. Arnold, Leighton A. Regayre, Duseong S. Jo, Wenxiang Shen, Hao Wang, Man Yue, Jingyi Wang, Wenxin Zhang, and Ken S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2024-4135, https://doi.org/10.5194/egusphere-2024-4135, 2025
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This study uses a global chemistry-climate model to investigate how new particle formation (NPF) from highly oxygenated organic molecules (HOMs) contributes to cloud condensation nuclei (CCN) in both preindustrial (PI) and present-day (PD) environments, and its impact on aerosol indirect radiative forcing. The findings highlight the crucial role of biogenic emissions in climate change, providing new insights for carbon-neutral scenarios and enhancing understanding of aerosol-cloud interactions.
Yongqing Bai, Tianliang Zhao, Kai Meng, Yue Zhou, Jie Xiong, Xiaoyun Sun, Lijuan Shen, Yanyu Yue, Yan Zhu, Weiyang Hu, and Jingyan Yao
Atmos. Chem. Phys., 25, 1273–1287, https://doi.org/10.5194/acp-25-1273-2025, https://doi.org/10.5194/acp-25-1273-2025, 2025
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We proposed a composite statistical method to identify the quasi-weekly oscillation (QWO) of regional PM2.5 transport over China in winter from 2015 to 2019. The QWO of regional PM2.5 transport is constrained by synoptic-scale disturbances of the East Asian winter monsoon circulation with the periodic activities of the Siberian high, providing a new insight into the understanding of regional pollutant transport with meteorological drivers in atmospheric environment changes.
Léo Clauzel, Sandrine Anquetin, Christophe Lavaysse, Gilles Bergametti, Christel Bouet, Guillaume Siour, Rémy Lapere, Béatrice Marticorena, and Jennie Thomas
Atmos. Chem. Phys., 25, 997–1021, https://doi.org/10.5194/acp-25-997-2025, https://doi.org/10.5194/acp-25-997-2025, 2025
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Solar energy production in West Africa is set to rise and needs accurate solar radiation estimates which are affected by desert dust. This work analyses a March 2021 dust event using a modelling strategy incorporating desert dust. Results show that considering desert dust cuts errors in solar radiation estimates by 75 % and reduces surface solar radiation by 18 %. This highlights the importance of incorporating dust aerosols into solar forecasting for better accuracy.
Zining Yang, Qiuyan Du, Qike Yang, Chun Zhao, Gudongze Li, Zihan Xia, Mingyue Xu, Renmin Yuan, Yubin Li, Kaihui Xia, Jun Gu, and Jiawang Feng
EGUsphere, https://doi.org/10.5194/egusphere-2024-3890, https://doi.org/10.5194/egusphere-2024-3890, 2025
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This study investigates the impact of turbulent mixing on black carbon (BC) concentrations in urban areas using WRF-Chem at 25, 5, and 1 km resolutions. Significant variations in BC and turbulent mixing occur mainly at night. Higher resolutions reduce BC overestimation due to enhanced PBL mixing coefficients and vertical wind fluxes. Small-scale eddies at higher resolutions increase BC lifetime and column concentrations. Land use and terrain variations across multi-resolutions affect PBL mixing.
Ari Laaksonen, Golnaz Roudsari, Ana A. Piedehierro, and André Welti
EGUsphere, https://doi.org/10.5194/egusphere-2024-4095, https://doi.org/10.5194/egusphere-2024-4095, 2025
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The mechanisms of ice nucleation at temperatures below 235 K have remained unclear for the past century. We suggest that ice nucleation is caused by the freezing of water adsorbed on aerosol surfaces. To test this hypothesis, we derived theoretical equations to predict the exact atmospheric conditions under which ice nucleation occurs. Our predictions agree well with experiments. The new theory thus provides a basis for an improved description of ice nucleation in the atmosphere.
Ross J. Herbert, Alberto Sanchez-Marroquin, Daniel P. Grosvenor, Kirsty J. Pringle, Stephen R. Arnold, Benjamin J. Murray, and Kenneth S. Carslaw
Atmos. Chem. Phys., 25, 291–325, https://doi.org/10.5194/acp-25-291-2025, https://doi.org/10.5194/acp-25-291-2025, 2025
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Aerosol particles that help form ice in clouds vary in number and type around the world and with time. However, in many weather and climate models cloud ice is not linked to aerosols that are known to nucleate ice. Here we report the first steps towards representing ice-nucleating particles within the UK Earth System Model. We conclude that in addition to ice nucleation by sea spray and mineral components of soil dust, we also need to represent ice nucleation by the organic components of soils.
Ryan Schmedding and Andreas Zuend
Atmos. Chem. Phys., 25, 327–346, https://doi.org/10.5194/acp-25-327-2025, https://doi.org/10.5194/acp-25-327-2025, 2025
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Four different approaches for computing the interfacial tension between liquid phases in aerosol particles were tested for particles with diameters from 10 nm to more than 5 μm. Antonov's rule led to the strongest reductions in the onset relative humidity of liquid–liquid phase separation and reproduced measured interfacial tensions for highly immiscible systems. A modified form of the Butler equation was able to best reproduce measured interfacial tensions in more miscible systems.
Xinyue Huang, Wenyu Gao, and Hosein Foroutan
EGUsphere, https://doi.org/10.5194/egusphere-2024-3076, https://doi.org/10.5194/egusphere-2024-3076, 2024
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This study investigates the relationship between wind-blown dust aerosols size distribution and wind conditions over topography at a regional scale, utilizing 10 years of dust reanalysis data. Linear regression models suggest that higher wind speeds and steeper land slopes, particularly under uphill winds, are associated with increased fractions of coarser dust particles. Moreover, these positive correlations weaken during summer and afternoon events, likely related to the haboob storms.
Lulu Yuan, Wenchao Han, Jiachen Meng, Yang Wang, Haojie Yu, and Wenze Li
EGUsphere, https://doi.org/10.5194/egusphere-2024-3350, https://doi.org/10.5194/egusphere-2024-3350, 2024
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This study utilizes multi-source data to reveal the impact of various urban functional zones in China on the spatial distribution of pollutants. The findings indicate that the residential and commercial zones see notable air quality gains, but the improvement of air quality in the transportation zone is the least considerable. Moreover, the industrial zone has the most seasonal air quality variation. Therefore, air pollution prevention policies should consider differences in functional zones.
Carl Svenhag, Pontus Roldin, Tinja Olenius, Robin Wollesen de Jonge, Sara Blichner, Daniel Yazgi, and Moa Sporre
EGUsphere, https://doi.org/10.5194/egusphere-2024-3626, https://doi.org/10.5194/egusphere-2024-3626, 2024
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This study investigates the model representation of how particles are formed and grow in the atmosphere. Using modeled and observed data from two boreal forest stations in 2018, we identify key factors for NPF to improve particle-climate predictions in the global EC-Earth3 model. Comparisons with the detailed ADCHEM model show that adding ammonia improves particle growth predictions, though EC-Earth3 still highly underestimates the number of particles during warmer months.
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 13681–13692, https://doi.org/10.5194/acp-24-13681-2024, https://doi.org/10.5194/acp-24-13681-2024, 2024
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A 2020 regulation has reduced sulfur emissions from shipping by about 80 %, leading to a decrease in atmospheric aerosols that have a cooling effect primarily by affecting cloud properties and amounts. Our climate model simulations predict a global temperature increase of 0.04 K over the next 3 decades as a result, which could contribute to surpassing the Paris Agreement's 1.5 °C target. Reduced aerosols may have also contributed to the recent temperature spikes.
Alcide Zhao, Laura J. Wilcox, and Claire L. Ryder
Atmos. Chem. Phys., 24, 13385–13402, https://doi.org/10.5194/acp-24-13385-2024, https://doi.org/10.5194/acp-24-13385-2024, 2024
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Climate models include desert dust aerosols, which cause atmospheric heating and can change circulation patterns. We assess the effect of dust on the Indian and east Asian summer monsoons through multi-model experiments isolating the effect of dust in current climate models for the first time. Dust atmospheric heating results in a southward shift of western Pacific equatorial rainfall and an enhanced Indian summer monsoon. This shows the importance of accurate dust representation in models.
Ragnhild Bieltvedt Skeie, Rachael Byrom, Øivind Hodnebrog, Caroline Jouan, and Gunnar Myhre
Atmos. Chem. Phys., 24, 13361–13370, https://doi.org/10.5194/acp-24-13361-2024, https://doi.org/10.5194/acp-24-13361-2024, 2024
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In 2020, new regulations by the International Maritime Organization regarding sulfur emissions came into force, reducing emissions of SO2 from the shipping sector by approximately 80 %. In this study, we use multiple models to calculate how much the Earth energy balance changed due to the emission reduction or the so-called effective radiative forcing. The calculated effective radiative forcing is weak, comparable to the effect of the increase in CO2 over the last 2 to 3 years.
Mingxu Liu, Hitoshi Matsui, Douglas S. Hamilton, Sagar D. Rathod, Kara D. Lamb, and Natalie M. Mahowald
Atmos. Chem. Phys., 24, 13115–13127, https://doi.org/10.5194/acp-24-13115-2024, https://doi.org/10.5194/acp-24-13115-2024, 2024
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Atmospheric aerosol deposition provides bioavailable iron to promote marine primary production, yet the estimates of its fluxes remain highly uncertain. This study, by performing global aerosol simulations, demonstrates that iron-containing particle size upon emission is a critical factor in regulating soluble iron input to open oceans. Further observational constraints on this are needed to reduce modeling uncertainties.
Thomas Drugé, Pierre Nabat, Martine Michou, and Marc Mallet
EGUsphere, https://doi.org/10.5194/egusphere-2024-3659, https://doi.org/10.5194/egusphere-2024-3659, 2024
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Aerosol scattering in long-wave radiation is often neglected in climate models. In this study, we analyze its impact through a physical modeling of this process in the CNRM ARPEGE-Climat model. It mainly leads to surface LW radiation increases across Sahara, Sahel and Arabian Peninsula, resulting in daily minimum near-surface temperature rises. Other changes in atmospheric fields are also simulated.
Jingmin Li, Mattia Righi, Johannes Hendricks, Christof G. Beer, Ulrike Burkhardt, and Anja Schmidt
Atmos. Chem. Phys., 24, 12727–12747, https://doi.org/10.5194/acp-24-12727-2024, https://doi.org/10.5194/acp-24-12727-2024, 2024
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Aiming to understand underlying patterns and trends in aerosols, we characterize the spatial patterns and long-term evolution of lower tropospheric aerosols by clustering multiple aerosol properties from preindustrial times to the year 2050 under three Shared
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
Atmos. Chem. Phys., 24, 12643–12659, https://doi.org/10.5194/acp-24-12643-2024, https://doi.org/10.5194/acp-24-12643-2024, 2024
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In March 2021, east Asia experienced an outbreak of severe dust storms after an absence of 1.5 decades. Here, we innovatively used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize dust emission and reproduce the dust storm. This work is valuable for not only the quantification of health damage, aviation risks, and profound impacts on the Earth's system but also revealing the climatic driving force and the process of desertification.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
Atmos. Chem. Phys., 24, 12509–12535, https://doi.org/10.5194/acp-24-12509-2024, https://doi.org/10.5194/acp-24-12509-2024, 2024
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This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean–atmosphere–aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low-cloud fraction, decreasing the ocean and continental surface temperature and reducing the precipitation of coastal western Africa. It also highlights the role of the ocean temperature response and its feedbacks for the September–November season.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
Atmos. Chem. Phys., 24, 12341–12354, https://doi.org/10.5194/acp-24-12341-2024, https://doi.org/10.5194/acp-24-12341-2024, 2024
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The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties. This method is verified from a theoretical perspective, and it performs well for thickly coated BC at high RHs.
Catherine Anne Toolan, Joe Adabouk Amooli, Laura J. Wilcox, Bjørn H. Samset, Andrew G. Turner, and Daniel M. Westervelt
EGUsphere, https://doi.org/10.5194/egusphere-2024-3057, https://doi.org/10.5194/egusphere-2024-3057, 2024
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Our research explores how well air pollution and rainfall patterns in Africa are represented in current climate models, by comparing model data to observations from 1981 to 2023. While most models capture seasonal air quality changes well, they struggle to replicate the distribution of non-dust pollutants and certain rainfall patterns, especially over east Africa. Improving these models is crucial for better climate predictions and preparing for future risks.
Zijun Li, Angela Buchholz, and Noora Hyttinen
Atmos. Chem. Phys., 24, 11717–11725, https://doi.org/10.5194/acp-24-11717-2024, https://doi.org/10.5194/acp-24-11717-2024, 2024
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Evaluating organosulfur (OS) hygroscopicity is important for assessing aerosol–cloud climate interactions in the post-fossil-fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with (NH4)2SO4. A good agreement was observed between their model-estimated and experimental HGFs.
Jamie R. Banks, Bernd Heinold, and Kerstin Schepanski
Atmos. Chem. Phys., 24, 11451–11475, https://doi.org/10.5194/acp-24-11451-2024, https://doi.org/10.5194/acp-24-11451-2024, 2024
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The Aralkum is a new desert in Central Asia formed by the desiccation of the Aral Sea. This has created a source of atmospheric dust, with implications for the balance of solar and thermal radiation. Simulating these effects using a dust transport model, we find that Aralkum dust adds radiative cooling effects to the surface and atmosphere on average but also adds heating events. Increases in surface pressure due to Aralkum dust strengthen the Siberian High and weaken the summer Asian heat low.
Cited articles
Ammann, C. M., Meehl, G. A., Washington, W. M., and Zender, C. S.: A monthly and latitudinally varying volcanic forcing dataset in simulations of 20th century climate, Geophys. Res. Lett., 30, 1657, https://doi.org/10.1029/2003GL016875, 2003.
Ammann, C. M., Washington, W. M., Meehl, G. A., Buja, L., and Teng, H.: Climate engineering through artificial enhancement of natural forcings: magnitudes and implied consequences, J. Geophys. Res., 115, D22109, https://doi.org/10.1029/2009JD012878, 2010.
Andronova, N. G. and Schlesinger, M. E.: Causes of global temperature changes during the 19th and 20th centuries, Geophys. Res. Lett., 27, 2137–2140, https://doi.org/10.1029/2000GL006109, 2000.
Boessenkool, K. P., Hall, I. R., Elderfield, H., and Yashayaev, I.: North Atlantic climate and deep-ocean flow speed changes during the last 230 years, Geophys. Res. Lett., 34, L13614, https://doi.org/10.1029/2007GL030285, 2007.
Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T., DeAngelo, B. J., Flanner, M. G., Ghan, S., Kärcher, B., Koch, D., Kinne, S., Kondo, Y., Quinn, P. K., Sarofim, M. C., Schultz, M. G., Schulz, M., Venkataraman, C., Zhang, H., Zhang, S., Bellouin, N., Guttikunda, S. K., Hopke, P. K., Jacobson, M. Z., Kaiser, J. W., Klimont, Z., Lohmann, U., Schwarz, J. P., Shindell, D., Storelvmo, T., Warren, S. G., and Zender, C. S.: Bounding the role of black carbon in the climate system: A scientific assessment, J. Geophys. Res., in press, https://doi.org/10.1002/jgrd.50171, 2013.
Bony, S., Colman, R., Kattsov, V. M., Allan, R. P., Bretherton, C. S., Dufresne, J.-L., Hall, A., Hallegatte, S., Holland, M. M., Ingram, W., Randall, D. A., Soden, B. J., Tselioudis, G., and Webb, M. J.: How well do we understand and evaluate climate change feedback processes?, J. Clim., 19, 3445–3482, https://doi.org/10.1029/2005GL023851, 2006.
Booth, B. B. B., Dunstone, N. J., Halloran, P. R., Andrews, T., and Bellouin, N.: Aerosols implicated as a prime driver of twentieth-century North Atlantic climate variability, Nature, 484, 228–232, https://doi.org/10.1038/nature10946, 2012.
Budyko, M. I.: Climate and Life, Academic Press, New York, USA, 508 pp., 1974.
Carton, J. A. and Santorelli, A.: Global upper ocean heat content as viewed in nine analyses, J. Clim., 21, 6015–6035. https://doi.org/10.1175/2008JCLI2489.1, 2008.
Chavez, F. P., Ryan, J., Lluch-Cota, S. E., and \ {N}iquen C. M.: From anchovies to sardines and back: multidecadal change in the Pacific Ocean, Science, 299, 217–221, https://doi.org/10.1126/science.1075880, 2003.
Chiang, J. C. H. and Friedman, A. R.: Extratropical cooling, interhemispheric thermal gradients, and tropical climate change, Annu. Rev. Earth Planet. Sci., 40, 383–412, https://doi.org/:10.1146/annurev-earth-042711-105545, 2012.
Christy, J. R., Spencer, R. W., and Braswell, W. D.: MSU tropospheric temperatures: dataset construction and radiosonde comparisons, J. Atmos. Ocean. Technol., 17, 1153–1170, 2000.
Christy, J. R., Spencer, R. W., Norris, W. B., Braswell, W. D., and Parker, D. E.: Error estimates of Version 5.0 of MSU–AMSU bulk atmospheric temperatures, J. Atmos. Ocean. Technol., 20, 613–629, 2003.
Church, J. A., White, N. J., and Arblaster, J. M.: Significant decadal–scale impact of volcanic eruptions on sea level and ocean heat content, Nature, 438, 74–77, https://doi.org/10.1038/nature04237, 2005.
Church, J. A., White, N. J., Konikow, L. F., Domingues, C. M., Cogley, J. G., Rignot, E., Gregory, J. M., van den Broecke, M. R., Monaghan, A. J., and Velicogna, I.: Revisiting the Earth's sea-level and energy budgets from 1961 to 2008, Geophys. Res. Lett., 38, L18601, https://doi.org/10.1029/2011GL048794, 2011.
Crutzen, P. J.: Albedo enhancement by stratospheric sulfur injections: a contribution to resolve a policy dilemma?, Clim. Change, 77, 211–220, https://doi.org/10.1007/s10584-006-9101-y, 2006.
Davies, R. and Molloy, M.: Global cloud height fluctuations measured by MISR on Terra from 2000 to 2010, Geophys. Res. Lett., 39, L03701, https://doi.org/10.1029/2011GL050506, 2012.
DeLand, M. T. and Cebula, R. P.: Solar UV variations during the decline of cycle 23, J. Atmos. Sol. Terr. Phys., 77, 225–234, https://doi.org/10.1016/j.jastp.2012.01.007, 2012.
DelSole, T., Tippett, M. K., and Shukla, J.: A significant component of unforced multidecadal variability in the recent acceleration of global warming, J. Clim., 24, 909–926, https://doi.org/10.1175/2010JCLI3659.1, 2011.
Delworth, T. L. and Zeng, F.: Multicentennial variability of the Atlantic meridional overturning circulation and its climatic influence in a 4000 yr simulation of the GFDL CM2.1 climate model, Geophys. Res. Lett., 39, L13702, https://doi.org/10.1029/2012GL052107, 2012.
Denters, B. and van Puijenbroeck, R. A. G.:Conditional regressions analysis, Quality Quantity, 23, 83–108, https://doi.org/10.1007/BF00195408, 1989.
Dickinson, R. E.: Climate engineering: a review of aerosol approaches to changing the global energy balance, Clim. Change, 33, 279–290, https://doi.org/10.1007/BF00142576, 1996.
Dima, M. and Lohmann, G.: A Hemispheric mechanism for the Atlantic Multidecadal Oscillation, J. Clim., 20, 2706–2719, https://doi.org/10.1175/JCLI4174.1, 2007.
Domingues, C. M., Church, J. A., White, N. J., Glecker, P. J., Wijffels, S. E., Barker, P. M., and Dunn, J. R.: Improved estimates of upper-ocean warming and multidecadal sea-level rise, Nature, 453, 1090–1093, https://doi.org/10.1038/nature07080, 2008.
Douglass, D. H. and Knox, R. S.: Climate forcing by the volcanic eruption of Mount Pinatubo, Geophys. Res. Lett., 32, L05710, https://doi.org/10.1029/2004GL022119, 2005.
Douglass, D. H., Knox, R. S., Pearson, B. D., and Clark Jr, A. Clark Jr.: Thermocline flux exchange during the Pinatubo event, Geophys. Res. Lett., 33, L19711, https://doi.org/https://doi.org/10.1029/2006GL026355, 2006.
Dutton, E. G. and Bodhaine, B. A.: Solar irradiance anomalies caused by clear-sky transmission variations above Mauna Loa: 1958–1999, J. Clim., 14, 3255–3262, 2001.
Enfield, D. B., Mestas-Nuñez, A. M., and Trimble, P. J.: The Atlantic Multidecadal Oscillation and its relation to rainfall and river flows in the continental U. S., Geophys. Res. Lett. 28, 2077–2080, https://doi.org/10.1029/2000GL012745, 2001.
Eyring, V., Shepherd, T. G., and Waugh, D. W. (eds.): SPARC Report on the Evaluation of Chemistry-Climate Models, SPARC Report No. 5, WCRP-132, WMO/TD-No. 1526, 2010.
Forster, P. M. de F. and Collins, M.: Quantifying the water vapour feedback associated with post-Pinatubo global cooling, Clim. Dynam., 23, 207–214, https://doi.org/10.1007/s00382-004-0431-z, 2004.
Forster, P. M. de F. and Gregory, J. M.: The climate sensitivity and its components diagnosed from Earth radiation budget data, J. Clim., 19, 39–52, https://doi.org/10.1175/JCLI3611.1, 2006.
Foster, G. and Rahmstorf, S.: Global temperature evolution 1979–2010, Envir. Res. Lett., 6, 044022, https://doi.org/10.1088/1748-9326/6/4/044022, 2011.
Gregory, J. M.: Vertical heat transports in the ocean and their effect on time-dependent climate change, Clim. Dynam., 16, 501–515, https://doi.org/10.1007/s003820000059, 2000.
Gouretski, V. and Reseghetti, F.: On depth and temperature biases in bathythermograph data: development of a new correction scheme based on analysis of a global ocean database, Deep-Sea Res. I, 57, 812–833, https://doi.org/10.1016/j.dsr.2010.03.011, 2010.
Guan, B. and Nigam, S.: Analysis of Atlantic SST variability factoring interbasin links and the secular trend: clarified structure of the Atlantic Multidecadal Oscillation, J. Clim., 22, 4228–4240, https://doi.org/10.1175/2009JCLI2921.1, 2009.
Hansen, J., Lacis, A., Ruedy, R., Sato, M., and Wilson, H.: How sensitive is the world's climate?, Natl. Geogr. Soc. Res. Exploration, 9, 142–158, 1993.
Hansen, J., Nazarenko, L., Ruedy, R., Sato, M., Willis, J., Del Genio, A., Koch, D., Lacis, A., Lo, K., Menon, S., Novakov, T., Perlwitz, J., Russell, G., Schmidt, G. A., and Tausnev, N.: Earth's energy imbalance: confirmation and implications, Science, 309, 1431–1435, https://doi.org/10.1126/science.1110252, 2005.
Hansen, J., Sato, M., Ruedy, R., Lo, K., Lea, D. W., and Medina-Elizade, M.: Global temperature change, Proc. Nat. Acad. Sci., 103(39), 14288–14293, https://doi.org/10.1073/pnas.0606291103, 2006.
Hansen, J., Ruedy, R., Sato, M., and Lo, K.: Global surface temperature change, Rev. Geophys., 48, RG4004, https://doi.org/10.1029/2010RG000345, 2010.
Harries, J. E. and Futyan, J. M.: On the stability of the Earth's radiative energy balance: response to the Mt. Pinatubo eruption, Geophys. Res. Lett., 33, L23814, https://doi.org/10.1029/2006GL027457, 2006.
Heckendorn P., Weisenstein, D., Fueglistaler, S., Luo, B. P., Rozanov, E., Shraner, M., Thomason, L. W., and Peter, T.: The impact of geoengineering aerosols on stratospheric temperature and ozone, Environ. Res. Lett., 4, 045108, https://doi.org/10.1088/1748-9326/4/4/045108, 2009.
IPCC, 2001: Climate Change 2001: The Scientific Basis. Contribution of Working Group I to the Third Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Houghton, J. T., Ding, Y., Griggs, D. J., Noguer, M., van der Linden, P. J., Dai, X., Maskell, K., and Johnson, C. A., Cambridge University Press, Cambridge, UK and New York, NY, USA, 881 pp., 2001.
IPCC, 2007: Climate Change 2007: The Physical Science Basis. Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change edited by: Solomon, S., Qin, D., Manning, M., Chen, Z., Marquis, M., Averyt, K. B., Tignor, M., and Miller, H. L., Cambridge University Press, Cambridge, UK and New York, NY, USA, 996 pp., 2007.
Iwi, A. M., Hermanson, L., Haines, K., and Sutton, R. T.: Mechanisms linking volcanic aerosols to the Atlantic meridional overturning circulation, J. Clim., 25, 3039–3051, https://doi.org/10.1175/2011JCL04067.1, 2012.
Jones, P. D., Lister, D. H., Osborn, T. J., Harpham C., Salmon, M., and Morice, C. P.: Hemispheric and large-scale land-surface air temperature variations: an extensive revision and an update to 2010, J. Geophys. Res., 117, D05127, https://doi.org/10.1029/2011JD017139, 2012.
Kennedy, J. J., Rayner, N. A., Smith, R. O., Saunby, M., and Parker, D. E.: Reassessing biases and other uncertainties in sea-surface temperature observations since 1850 part 1: measurement and sampling errors, J. Geophys. Res., 116, D14103, https://doi.org/10.1029/2010JD015218, 2011a.
Kennedy, J. J., Rayner, N. A., Smith, R . O., Saunby, M., and Parker, D. E.: Reassessing biases and other uncertainties in sea-surface temperature observations since 1850 part 2: biases and homogenization, J. Geophys. Res., 116, D14104, https://doi.org/10.1029/2010JD015220, 2011b.
Kiehl, J. T.: Twentieth century climate model response and climate sensitivity, Geophys. Res. Lett., 34, L22710, https://doi.org/10.1029/2007GL031383, 2007.
Kinne, S., Toon, O. B., and Prather, M.: Buffering of stratospheric circulation by changing amounts of tropical ozone: a Pinatubo case study, Geophys. Res. Lett., 19, 1927–1930, https://doi.org/10.1029/92GL01937, 1992.
Kinnison, D. E., Grant, K. E., Connell, P. S., Wuebbles, D. J., and Rotman, D. A.: The chemical radiative effects of the Mt. Pinatubo eruption, J. Geophys. Res., 99, 25705–25731, https://doi.org/10.1029/94JD02318, 1994.
Knight J. R., Allan, R. J., Folland, C. K., Vellinga, M., and Mann, M. E.: A signature of persistent natural thermohaline circulation cycles in observed climate, Geophys. Res. Lett., 32, L20708, https://doi.org/10.1029/2005GL024233, 2005.
Kopp, G. and Lean, J. L.: A new, lower value of total solar irradiance: evidence and climate significance, Geophys. Res. Lett., 38, L01706, https://doi.org/10.1029/2010GL045777, 2011.
Kravitz, B., Robock, A., Boucher, O., Schmidt, H., Taylor, K. E., Stenchikov, G., and Schulz, M.: The geoengineering model intercomparison project (GeoMIP), Atmos. Sci. Lett., 12, 162–167, https://doi.org/10.1002/asl.316, 2011.
Kuhlbrodt, T., Griesel, A., Montoya, M., Levermann, A., Hofmann, M., and Rahmstorf, S.: On the driving processes of the Atlantic meridional overturning circulation, Rev. Geophys., 45, RG2001, https://doi.org/10.1029/2004RG000166, 2007.
Lacis, A. A. and Mishchenko, M. I.: Climate forcing, climate sensitivity, and climate response: a radiative modeling perspective on atmospheric aerosols, in: Aerosol Forcing of Climate: Report of the Dahlem Workshop on Aerosol Forcing of Climate, edited by: Charlson, R. J., and Heintzenberg, J., 11–42, John Wiley Sons, Chichester, England/New York, 1995.
Lamarque, J.-F., Kyle, G., Meinshausen, M., Riahi, K., Smith, S., van Vuuren, D., Conley, A., and Vitt, F.: Global and regional evolution of short-lived radiatively-active gases and aerosols in the representative concentration pathways, Climatic Change, 109, 191–212, https://doi.org/10.1007/s10584-011-0155-0, 2011.
Lean, J. L.: Evolution of the Sun's spectral irradiance since the Maunder minimum, Geophys. Res. Lett., 27, 2425–2428, https://doi.org/10.1029/2000GL000043, 2000.
Lean, J. L. and DeLand, M. T.: How does the Sun's spectrum vary?, J. Clim., 25, 2555–2560, https://doi.org/10.1175/JCLI-D-11-00571.1, 2012.
Lean, J. L. and Rind, D. H.: How natural and anthropogenic influences alter global and regional surface temperatures: 1889 to 2006, Geophys. Res. Lett., 35, L18701, https://doi.org/10.1029/2008GL034864, 2008.
Lean, J. L. and Rind, D. H.: How will Earth's surface temperature change in future decades?, Geophys. Res. Lett., 36, L15708,10.1029/2009GL038932, 2009.
Levitus, S., Antonov, J., and Boyer, T.: Warming of the world ocean, 1955–2003, Geophys. Res. Lett., 32, L02604, https://doi.org/10.1029/2004GL021592, 2005.
Mascioli, N. R., Canty, T., and Salawitch, R. J.: An empirical model of global climate: 2. Implications for future temperature, Atmos. Chem. Phys. Discuss., 12, 23913–23974, https://doi.org/10.5194/acpd-12-23913-2012, 2012.
Mass, C. F. and Portman, D. A.: Major volcanic eruptions and climate: a critical evaluation, J. Clim., 2, 566–593, 1989.
McGuffie, K. and Henderson-Sellers, A.: A Climate Modeling Primer, 3rd edn., J. Wiley and Sons, Chichester, England, 2005.
Medhaug, I. and Furevik, T.: North Atlantic 20th century multidecadal variability in coupled climate models: sea surface temperature and ocean overturning circulation, Ocean Sci., 7, 389–404, https://doi.org/10.5194/os-7-389-2011, 2011.
Meehl, G., Arblaster, J., Fasullo, J., Hu, A., and Trenberth, K.: Model-based evidence of deep-ocean heat uptake during surface-temperature hiatus periods, Nature Clim. Change, 1, 360–364. https://doi.org/10.1038/nclimate1229, 2011.
Meinshausen, M., Smith, S. J., Calvin, K. V., Daniel, J. S., Kainuma, M. L. T., Lamarque, J.-F., Matsumoto, K., Montzka, S., Raper, S., Riahi, K., Thomson, A. M., Velders, G. J. M., and van Vuuren, D. P.: The RCP greenhouse gas concentrations and their extensions from 1765 to 2300, Clim. Change, 109, 213–241, https://doi.org/10.1007/s10584-011-0156-z, 2011.
Morice, C. P., Kennedy, J. J., Rayner, N. A., and Jones, P. D., Quantifying uncertainties in global and regional temperature change using an ensemble of observational estimates: the HadCRUT4 dataset, J. Geophys. Res., 117, D08101, https://doi.org/10.1029/2011JD017187, 2012.
Murphy, D. M., Solomon, S., Portmann, R. W., Rosenlof, K. H., Forster, P. M., and Wong, T.: An observationally based energy balance for the Earth since 1950, J. Geophys. Res., 114, D17107, https://doi.org/10.1029/2009JD012105, 2009.
Myhre, G., Highwood, E. J., Shine, K. P., and Stordal, F.: New estimates of radiative forcing due to well mixed greenhouse gases, Geophys. Res. Lett., 25, 2715–2718, https://doi.org/10.1029/98GL01908, 1998.
Myhre, G., Myhre, A., and Stordal, F.: Historical evolution of radiative forcing of climate, Atmos. Environ., 35, 2361–2373, https://doi.org/10.1016/S1352-2310(00)00531-8, 2001.
National Academy of Sciences (NAS): Policy Implications of Greenhouse Warming: Mitigation, Adaptation, and the Science Base, Panel on Policy Implications of Greenhouse Warming, National Academy Press, Washington, DC, USA, 1992.
Nigam, S., Guan, B., and Ruiz-Barradas, A.: Key role of the Atlantic Multidecadal Oscillation in 20th century drought and wet periods over the Great Plains, Geophys. Res. Lett., 38, L16713, https://doi.org/10.1029/2011GL048650, 2011.
Raper, S. C. B., Gregory, J. M., and Stouffer, R. J.: The role of climate sensitivity and ocean heat uptake on AOGCM transient temperature response, J. Clim., 15, 124–130, https://doi.org/10.1175/1520-0442(2002)015<0124:TROCSA>2.0.CO;2, 2002.
Rasch, P. J., Crutzen, P. J., and Coleman, D. B.: Exploring the geoengineering of climate using stratospheric sulfate aerosols: the role of particle size, Geophys. Res. Lett., 35, L02809, https://doi.org/10.1029/2007GL032179, 2008a.
Rasch, P. J., Tilmes, S., Turco, R. P., Robock, A., Oman, L., and Chen, C.-C.: An overview of geoengineering of climate using stratospheric sulphate aerosols, Philos. Trans. R. Soc., Ser. A., 366, 4007–4037, https://doi.org/10.1098/rsta.2008.0131, 2008b.
Riahi, K., Grüber, A., and Nakicenovic, N.: Scenarios of long-term socio-economic and environmental development under climate stabilization, Technol. Forecast. Soc. Change 74, 887–935, https://doi.org/10.1016/j.techfore.2006.05.026, 2007.
Riahi, K., Rao, S., Krey, V., Cho, C., Chirkov, V., Fischer, G., Kindermann, G., Nakicenovic, N., and Rafaj, P.: RCP 8.5 – a scenario of comparatively high greenhouse gas emissions, Climatic Change, 109, 33–57, https://doi.org/10.1007/s10584-011-0149-y, 2011.
Robock, A., Oman, L., and Stenchikov, G. L.: Regional climate responses to geoengineering with tropical and Arctic SO2 injections, J. Geophys. Res., 113, D16101, https://doi.org/10.1029/2008JD010050, 2008.
Robock, A., Marquardt, A., Kravitz, B., and Stenchikov, G.: Benefits, risks, and costs of stratospheric geoengineering, Geophys. Res. Lett., 36, L19703, https://doi.org/10.1029/2009GL039209, 2009.
Rohde, R., Muller, R., Jacobsen, R., Perlmutter, S., Rosenfeld, A., Wurtele, J., Curry, J., Wickham, C., and Mosher, S.: Berkeley Earth temperature averaging process, Geoinfor. Geostat: An Overview, 1:2, https://doi.org/10.4174/gigs.1000103, 2013.
Saji, H. H., Goswami, B. N., Vinayachandran, P. H., and Yamagata, T.: A dipole mode in the tropical Indian Ocean, Nature, 401, 360–363, https://doi.org/10.1038/43854, 1999.
Salawitch, R. J., Weisenstein, D. K., Kovalenko, L. J., Sioris, C. E., Wennberg, P. O., Chance, K., Ko, M. K. W., and McLinden, C. A.: Sensitivity of ozone to bromine in the lower stratosphere, Geophys. Res. Lett., 32, L05811, https://doi.org/10.1029/2004GL021504, 2005.
Saravanan, R., and McWilliams, J. C.: Advective ocean–atmosphere interaction: an analytical stochastic model with implications for decadal variability, J. Clim., 11, 165–188, 1998.
Sato, M., Hansen, J. E., McCormick, M. P., and Pollack, J. B.: Stratospheric aerosol optical depths, 1850–1990. J. Geophys. Res., 98, 22987–22994, https://doi.org/10.1029/93JD02553, 1993.
Schlesinger, M. E. and Ramankutty, N.: An oscillation in the global climate system of period 65–70 years, Nature, 367, 723–726, https://doi.org/10.1038/367723a0, 1994.
Schmith, T., and Hansen, C.: Fram strait ice export during the nineteenth and twentieth centuries reconstructed from a multiyear sea ice index from Southwestern Greenland, J. Clim., 16, 2782–2791, https://doi.org/10.1175/1520-0442(2003)016<2782:FSIEDT>2.0.CO;2, 2003.
Schneider, S. H.: Geoengineering: could-or should-we do it?, Clim. Change, 33, 291–302, https://doi.org/10.1007/BF00142577, 1996.
Schoeberl, M. R., Bhartia, P. K., Hilsenrath, E., and Torres, O.: Tropical ozone loss following the eruption of Mt. Pinatubo, Geophys. Res. Lett., 20, 29–32, https://doi.org/10.1029/92GL02637, 1993.
Schwartz, S. E.: Determination of Earth's transient and equilibrium climate sensitivities from observations over the twentieth century: strong dependence on assumed forcing, Surv. Geophys., 33, 745–777, https://doi.org/10.1007/s10712-012-9180-4, 2012.
Semenov, V. A., Latif, M., Dommenget, D., Keenlyside, N. S., Strehz, A., Martin, T., and Park, W.: The impact of North Atlantic-Arctic multidecadal variability on Northern Hemispheric surface air temperature, 23, 5668–5677, https://doi.org/10.1175/2010JCLI3347.1, 2010.
Shindell, D., Faluvegi, G., Lacis, A., Hansen, J., Ruedy, R., and Aguilar, E.: Role of tropospheric ozone increases in 20th-century climate change, J. Geophys. Res., 111, D08302, https://doi.org/10.1029/2005JD006348, 2006.
Smith, S. J., van Aardenne, J., Klimont, Z., Andres, R. J., Volke, A., and Delgado Arias, S.: Anthropogenic sulfur dioxide emissions: 1850–2005, Atmos. Chem. Phys., 11, 1101–1116, https://doi.org/10.5194/acp-11-1101-2011, 2011.
Smith, T. M. and Reynolds, R. W.: A global merged land-air-sea surface temperature reconstruction based on historical observations (1880–1997), J. Clim., 18, 2021–2035, https://doi.org/10.1175/JCLI3362.1, 2005.
Smith, T. M., Reynolds, R. W., Peterson, T. C., and Lawrimore, J.: Improvements to NOAA's historical merged land-ocean surface temperature analysis (1880–2006), J. Clim., 21, 2283–2296, https://doi.org/10.1175/2007JCLI2100.1, 2008.
Soden, B. J. and Held, I. M.: An assessment of climate feedbacks in coupled atmosphere–ocean models, J. Clim., 19, 3354–3360, https://doi.org/10.1175/JCLI3799.1, 2006.
Soden, B. J., Wetherald, R. T., Stenchikov, G. L., and Robock A.: Global cooling after the eruption of Mount Pinatubo: a test of climate feedback by water vapor, Science, 296, 727–730, https://doi.org/10.1126/science.296.5568.727, 2002.
Srokosz, M., Baringer, M., Bryden, H., Cunningham, S., Delworth, T., Lozier, S., Marotzke, J., and Sutton, R.: Past, present, and future changes in the Atlantic meridional overturning circulation, B. AM. Meteorol. Soc., 93, 1663–1676, 10.1175/BAMS-D-11-00151.1, 2012.
Stenchikov, G., Delworth, T. L., Ramaswamy, V., Stouffer, R. J., Wittenberg, A., and Zeng, F.: Volcanic signals in oceans, J. Geophys. Res., 114, D16104, https://doi.org/10.1029/2008JD011673, 2009.
Stern, D. I.: An atmosphere-ocean time series model of global climate change, Comput. Stat. Data An., 51, 1330–1346, https://doi.org/10.1016/j.csda.2005.09.016, 2006a.
Stern, D. I.: Reversal of the trend in global anthropogenic sulfur emissions, Chemosphere, 16, 207–220, https://doi.org/10.1016/j.gloenvcha.2006.01.001, 2006b.
Stouffer, R. J., Yin, J., Gregory, J. M., Dixon, K. W., Spelman, M. J., Hurlin, W., Weaver, A. J., Eby, M., Flato, G. M., Hasumi, H., Hu, A., Jungclaus, J. H., Kamenkovich, I. V., Levermann, A., Montoya, M., Murakami, S., Nawrath, S., Oka, A., Peltier, W. R., Robitaille, D. Y., Sokolov, A., Vettoretti, G., and Webber, S. L.: Investigating the causes of the response of the thermohaline circulation to past and future climate changes, J. Clim., 19, 1365–1387, https://doi.org/10.1175/JCLI3689.1, 2006.
Sutton, R. T. and Hodson, D. L. R.: Atlantic ocean forcing of North American and European summer climate, Science, 309, 115–118, https://doi.org/10.1126/science.1109496, 2005.
Thompson, D. W. J., Kennedy, J. J., Wallace, J. M., and Jones, P. D.: A large discontinuity in the mid-twentieth century in observed global-mean surface temperature, Nature, 453, 646–649, https://doi.org/10.1038/nature06982, 2008.
Thompson, D. W. J., Wallace, J. M, Jones, P. D., and Kennedy, J. J.: Identifying signatures of natural climate variability in time series of global-mean surface temperature: methodology and insights, J. Clim., 22, 6120–6141, https://doi.org/10.1175/2009JCLI3089.1, 2009.
Thompson, R. D.: Volcanic eruptions and global temperatures, Ambio, 24, 320–321, 1995.
Tilmes, S., Müller, R., and Salawitch, R.: The sensitivity of polar ozone depletion to proposed geoengineering schemes, Science, 320, 1201–1204, https://doi.org/10.1126/science.1153966, 2008.
Tilmes, S., Garcia, R. R., Kinnison, D. E., Gettelman, A., and Rasch, R. J.: Impact of geo-engineered aerosols on the troposphere and stratosphere, J. Geophys. Res., 114, D12305, https://doi.org/10.1029/2008JD011420, 2009.
Tilmes, S., Kinnison, D. E., Garcia, R. R., Salawitch, R., Canty, T., Lee-Taylor, J., Madronich, S., and Chance, K.: Impact of very short-lived halogens on stratospheric ozone abundance and UV radiation in a geo-engineered atmosphere, Atmos. Chem. Phys. 12, 10945–10955, https://doi.org/10.5194/acpd-12-10945-2012, 2012.
Ting, M., Kushnir, Y., Seager, R., and Li, C.: Forced and internal twentieth-century SST trends in the North Atlantic, J. Clim., 22, 1469–1481, https://doi.org/10.1175/2008JCLI2561.1, 2009.
Trenberth, K. E. and Dai, A.: Effects of Mount Pinatubo volcanic eruption on the hydrological cycle as an analog of geoengineering, Geophys. Res. Lett. 34, L15702, https://doi.org/10.1029/2007GL030524, 2007.
Trenberth, K. E. and Shea, D. J.: Atlantic hurricanes and natural variability in 2005, Geophys. Res. Lett., 33, L12704, https://doi.org/10.1029/2006GL026894, 2006.
Tung, K.-K. and Zhou, J.: Using data to attribute episodes of warming and cooling in instrumental records, Proc. Natl. Acad. Sci. USA, 110, 2058–2063, https://doi.org/10.1073/pnas.1212471110, 2013.
van Oldenborgh, G. J., te Raa, L. A., Dijkstra, H. A., and Philip, S. Y.: Frequency- or amplitude-dependent effects of the Atlantic meridional overturning on the tropical Pacific Ocean, Ocean Sci., 5, 293–301, https://doi.org/10.5194/os-5-293-2009, 2009.
van Vuuren, D. P., Edmonds, J. A., Kainuma, M., Riahi, K., Thomson, A. M., Hibbard, K., Hurtt, G. C., Kram, T., Krey, V., Lamarque, J.-F., Masui, T., Meinshausen, M., Nakicenovic, N., Smith, S. J., and Rose, S: The representative concentration pathways: an overview, Climatic Change, 109, 5–31, https://doi.org/10.1007/s10584-011-0148-z, 2011.
Velders, G. J. M., Fahey, D. W., Daniel, J. S., McFarland, M., and Andersen, S. O.: The large contribution of projected HFC emissions to future climate forcing, Proc. Natl. Acad. Sci. USA, 106, 10949–10954, https://doi.org/10.1073/pnas.0902817106, 2009.
Vincze, M. and Jánosi, I. M.: Is the Atlantic multidecadal oscillation (AMO) a statistical phantom?, Nonlin. Processes Geophys., 18, 469–475, https://doi.org/https://doi.org/10.5194/npg-18-469-2011, 2011.
von Storch, H. and Zwiers, F. W.: Statistical analysis in Climate Research, Cambridge University Press, Cambridge, UK, 495 pp., 2002.
Wang, Y. M., Lean, J. L., and Sheeley Jr., N. R.: Modeling the Sun's magnetic field and irradiance since 1713, Astrophys. J., 625, 522–538, https://doi.org/10.1086/429689, 2005.
Wielicki B. A., Wong, T., Allen, R. P., Slingo, A., Kiehl, J., Soden, B. J., Gordon, C. T., Miller, A. J., Yang, S.-K., Randall, D. A., Robertson, F., Susskind, J., and Jacobowitz, H.: Evidence for large decadal variability in the tropical mean radiative energy budget, Science, 295, 841–844, https://doi.org/10.1126/science.1065837, 2002.
Wigley, T. M. L., Ammann, C. M., Santer, B. D., and Raper, S. C. D.: Effect of climate sensitivity on the response to volcanic forcing, J. Geophys. Res., 110, D09107, https://doi.org/10.1029/2004JD005557, 2005.
Wigley, T. M. L., Ammann, C. M., Santer, B. D., and Taylor, K. E.: Comment on "Climate
Willis, D. K.: Can in situ floats and satellite altimeters detect long-term changes in Atlantic Ocean overturning?, Geophys. Res. Lett., 37, L06602, https://doi.org/10.1029/2010GL042372, 2010.
WMO (World Meteorological Organization): Scientific Assessment of Ozone Depletion: 2010, Global Ozone Research and Monitoring Project – Report # 52, Geneva, 2011.
Wolter, K. and Timlin, M. S.: El Niño/Southern Oscillation behaviour since 1871 as diagnosed in an extended multivariate ENSO index (ME I.ext), Int. J. Climatol., 31, 1074–1087, https://doi.org/10.1002/joc.2336, 2011.
Wu, L. and Liu, Z.: Decadal variability in the North Pacific: the Eastern North Pacific mode, J. Clim., 16, 3111–3131, https://doi.org/10.1175/1520-0442(2003)016<311:DVITNP>2.0.CO;2, 2003.
Wu, Z., Huang, N. E., Wallace, J. M., Smoliak, B. V., and Chen, Z.: On the time varying trend in global-mean surface temperature, Clim. Dynam., 37, 759–773, https://doi.org/10.1007/s00382-011-1128-8, 2011.
Zanchettin, D., Timmreck, C., Graf, H.-F., Rubino, A., Lorenz, S., Lohmann, K., Kruger, L., and Jungclaus, J. H.: Bi-decadal variability excited in the coupled ocean-atmosphere system by strong tropical volcanic eruptions, Clim. Dynam., 39, 419–444, https://doi.org/10.1007/s00382-011-1167-1, 2012.
Zhang, R., Delworth, T. L., and Held, I. M.: Can the Atlantic Ocean drive the observed multidecadal variability in Northern Hemisphere mean temperature?, Geophys. Res. Lett., 34, L02709, https://doi.org/10.1029/2006GL028683, 2007.
Zhang, Y. and Delworth, T. L.: Impact of the Atlantic Multidecadal Oscillation on North Pacific climate variability, Geophys. Res. Lett., 34, L23708, https://doi.org/10.1029/2007GL031601, 2007.
Zhang, Y., Wallace, J. M., and Battisti, D. S.: ENSO-like interdecadal variability: 1900–93, J. Clim., 10, 1004–1020, 1997.
Zhou, J. and Tung, K.-K.: Deducing multidecadal anthropogenic global warming trends using multiple linear regression analysis, J. Atmos. Sci., 70, 3–8, https://doi.org/http://dx.doi.org/10.1175/JAS-D-12-0208.1, 2013.
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