Articles | Volume 24, issue 16
https://doi.org/10.5194/acp-24-9339-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-9339-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Observed and CMIP6-model-simulated organic aerosol response to drought in the contiguous United States during summertime
Department of Earth and Atmospheric Sciences, University of Houston, Houston, TX, USA
now at: Cooperative Institute for Satellite Earth System Studies, George Mason University, Fairfax, VA, USA
Department of Earth and Atmospheric Sciences, University of Houston, Houston, TX, USA
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Cited articles
Barth, M. C., Rasch, P. J., Kiehl, J. T., Benkovitz, C. M., and Schwartz, S. E.: Sulfur chemistry in the National Center for Atmospheric Research Community Climate Model: Description, evaluation, features, and sensitivity to aqueous chemistry, J. Geophys. Res.-Atmos., 105, 1387–1415, https://doi.org/10.1029/1999JD900773, 2000.
Berg, L. K., Shrivastava, M., Easter, R. C., Fast, J. D., Chapman, E. G., Liu, Y., and Ferrare, R. A.: A new WRF-Chem treatment for studying regional-scale impacts of cloud processes on aerosol and trace gases in parameterized cumuli, Geosci. Model Dev., 8, 409–429, https://doi.org/10.5194/gmd-8-409-2015, 2015.
Borlina, C. S. and Rennó, N. O.: The impact of a severe drought on dust lifting in California's Owens Lake area, Sci. Rep., 7, 1784, https://doi.org/10.1038/s41598-017-01829-7, 2017.
Brégonzio-Rozier, L., Giorio, C., Siekmann, F., Pangui, E., Morales, S. B., Temime-Roussel, B., Gratien, A., Michoud, V., Cazaunau, M., DeWitt, H. L., Tapparo, A., Monod, A., and Doussin, J.-F.: Secondary organic aerosol formation from isoprene photooxidation during cloud condensation–evaporation cycles, Atmos. Chem. Phys., 16, 1747–1760, https://doi.org/10.5194/acp-16-1747-2016, 2016.
Brilli, F., Barta, C., Fortunati, A., Lerdau, M., Loreto, F., and Centritto, M.: Response of isoprene emission and carbon metabolism to drought in white poplar (Populus alba) saplings, New Phytol., 175, 244–254, https://doi.org/10.1111/j.1469-8137.2007.02094.x, 2007.
Carslaw, K. S., Lee, L. A., Reddington, C. L., Pringle, K. J., Rap, A., Forster, P. M., Mann, G. W., Spracklen, D. V., Woodhouse, M. T., Regayre, L. A., and Pierce, J. R.: Large contribution of natural aerosols to uncertainty in indirect forcing, Nature, 503, 67–71, https://doi.org/10.1038/nature12674, 2013.
Cook, B. I., Mankin, J. S., and Anchukaitis, K. J.: Climate change and drought: From past to future, Curr. Clim. Change Rep., 4, 164–179, https://doi.org/10.1007/s40641-018-0093-2, 2018.
D'Ambro, E. L., Schobesberger, S., Gaston, C. J., Lopez-Hilfiker, F. D., Lee, B. H., Liu, J., Zelenyuk, A., Bell, D., Cappa, C. D., Helgestad, T., Li, Z., Guenther, A., Wang, J., Wise, M., Caylor, R., Surratt, J. D., Riedel, T., Hyttinen, N., Salo, V.-T., Hasan, G., Kurtén, T., Shilling, J. E., and Thornton, J. A.: Chamber-based insights into the factors controlling epoxydiol (IEPOX) secondary organic aerosol (SOA) yield, composition, and volatility, Atmos. Chem. Phys., 19, 11253–11265, https://doi.org/10.5194/acp-19-11253-2019, 2019.
Danabasoglu, G., Lamarque, J.-F., Bacmeister, J., Bailey, D. A., DuVivier, A. K., Edwards, J., Emmons, L. K., Fasullo, J., Garcia, R., Gettelman, A., Hannay, C., Holland, M. M., Large, W. G., Lauritzen, P. H., Lawrence, D. M., Lenaerts, J. T. M., Lindsay, K., Lipscomb, W. H., Mills, M. J., Neale, R., Oleson, K. W., Otto-Bliesner, B., Phillips, A. S., Sacks, W., Tilmes, S., van Kampenhout, L., Vertenstein, M., Bertini, A., Dennis, J., Deser, C., Fischer, C., Fox-Kemper, B., Kay, J. E., Kinnison, D., Kushner, P. J., Larson, V. E., Long, M. C., Mickelson, S., Moore, J. K., Nienhouse, E., Polvani, L., Rasch, P. J., and Strand, W. G.: The Community Earth System Model Version 2 (CESM2), J. Adv. Model. Earth Sy., 12, e2019MS001916, https://doi.org/10.1029/2019MS001916, 2020.
Dawson, J. P., Adams, P. J., and Pandis, S. N.: Sensitivity of PM2.5 to climate in the Eastern US: a modeling case study, Atmos. Chem. Phys., 7, 4295–4309, https://doi.org/10.5194/acp-7-4295-2007, 2007.
Dennison, P. E., Brewer, S. C., Arnold, J. D., and Moritz, M. A.: Large wildfire trends in the western United States, 1984–2011, Geophys. Res. Lett., 41, 2928–2933, https://doi.org/10.1002/2014GL059576, 2014.
Dunne, J. P., Horowitz, L. W., Adcroft, A. J., Ginoux, P., Held, I. M., John, J. G., Krasting, J. P., Malyshev, S., Naik, V., Paulot, F., Shevliakova, E., Stock, C. A., Zadeh, N., Balaji, V., Blanton, C., Dunne, K. A., Dupuis, C., Durachta, J., Dussin, R., Gauthier, P. P. G., Griffies, S. M., Guo, H., Hallberg, R. W., Harrison, M., He, J., Hurlin, W., McHugh, C., Menzel, R., Milly, P. C. D., Nikonov, S., Paynter, D. J., Ploshay, J., Radhakrishnan, A., Rand, K., Reichl, B. G., Robinson, T., Schwarzkopf, D. M., Sentman, L. T., Underwood, S., Vahlenkamp, H., Winton, M., Wittenberg, A. T., Wyman, B., Zeng, Y., and Zhao, M.: The GFDL Earth System Model Version 4.1 (GFDL-ESM 4.1): Overall Coupled Model Description and Simulation Characteristics, J. Adv. Model. Earth Sy., 12, e2019MS002015, https://doi.org/10.1029/2019MS002015, 2020.
Eyring, V., Bony, S., Meehl, G. A., Senior, C. A., Stevens, B., Stouffer, R. J., and Taylor, K. E.: Overview of the Coupled Model Intercomparison Project Phase 6 (CMIP6) experimental design and organization, Geosci. Model Dev., 9, 1937–1958, https://doi.org/10.5194/gmd-9-1937-2016, 2016.
Fang, Y., Fiore, A. M., Horowitz, L. W., Gnanadesikan, A., Held, I., Chen, G., Vecchi, G., and Levy, H.: The impacts of changing transport and precipitation on pollutant distributions in a future climate, J. Geophys. Res.-Atmos., 116, D18303, https://doi.org/10.1029/2011JD015642, 2011.
FED: The Federal Land Manager Environmental Database query wizard, FED, https://views.cira.colostate.edu/fed/QueryWizard/ (last access: 27 December 2023), 2023.
Ford, T. and Labosier, C. F.: Spatial patterns of drought persistence in the Southeastern United States, Int. J. Climatol., 34, 2229–2240, 2014.
Gaston, C. J., Riedel, T. P., Zhang, Z., Gold, A., Surratt, J. D., and Thornton, J. A.: Reactive Uptake of an Isoprene-Derived Epoxydiol to Submicron Aerosol Particles, Environ. Sci. Technol., 48, 11178–11186, https://doi.org/10.1021/es5034266, 2014.
Giglio, L., Randerson, J. T., and van der Werf, G. R.: Analysis of daily, monthly, and annual burned area using the fourth-generation global fire emissions database (GFED4), J. Geophys. Res.-Biogeo., 118, 317–328, https://doi.org/10.1002/jgrg.20042, 2013 (data available at: https://www.geo.vu.nl/~gwerf/GFED/GFED4/, last access: 21 August 2024).
Gilman, J. B., Lerner, B. M., Kuster, W. C., Goldan, P. D., Warneke, C., Veres, P. R., Roberts, J. M., de Gouw, J. A., Burling, I. R., and Yokelson, R. J.: Biomass burning emissions and potential air quality impacts of volatile organic compounds and other trace gases from fuels common in the US, Atmos. Chem. Phys., 15, 13915–13938, https://doi.org/10.5194/acp-15-13915-2015, 2015.
Gomez, J., Allen, R. J., Turnock, S. T., Horowitz, L. W., Tsigaridis, K., Bauer, S. E., Olivié, D., Thomson, E. S., and Ginoux, P.: The projected future degradation in air quality is caused by more abundant natural aerosols in a warmer world, Commun. Earth Environ., 4, 1–11, https://doi.org/10.1038/s43247-023-00688-7, 2023.
Gorham, K. A., Raffuse, S. M., Hyslop, N. P., and White, W. H.: Comparison of recent speciated PM2.5 data from collocated CSN and IMPROVE measurements, Atmos. Environ., 244, 117977, https://doi.org/10.1016/j.atmosenv.2020.117977, 2021.
Hallquist, M., Wenger, J. C., Baltensperger, U., Rudich, Y., Simpson, D., Claeys, M., Dommen, J., Donahue, N. M., George, C., Goldstein, A. H., Hamilton, J. F., Herrmann, H., Hoffmann, T., Iinuma, Y., Jang, M., Jenkin, M. E., Jimenez, J. L., Kiendler-Scharr, A., Maenhaut, W., McFiggans, G., Mentel, Th. F., Monod, A., Prévôt, A. S. H., Seinfeld, J. H., Surratt, J. D., Szmigielski, R., and Wildt, J.: The formation, properties and impact of secondary organic aerosol: current and emerging issues, Atmos. Chem. Phys., 9, 5155–5236, https://doi.org/10.5194/acp-9-5155-2009, 2009.
Hand, J. L., Schichtel, B. A., Pitchford, M., Malm, W. C., and Frank, N. H.: Seasonal composition of remote and urban fine particulate matter in the United States, J. Geophys. Res.-Atmos., 117, D05209, https://doi.org/10.1029/2011JD017122, 2012.
Hidy, G. M., Blanchard, C. L., Baumann, K., Edgerton, E., Tanenbaum, S., Shaw, S., Knipping, E., Tombach, I., Jansen, J., and Walters, J.: Chemical climatology of the southeastern United States, 1999–2013, Atmos. Chem. Phys., 14, 11893–11914, https://doi.org/10.5194/acp-14-11893-2014, 2014.
Jen, C. N., Hatch, L. E., Selimovic, V., Yokelson, R. J., Weber, R., Fernandez, A. E., Kreisberg, N. M., Barsanti, K. C., and Goldstein, A. H.: Speciated and total emission factors of particulate organics from burning western US wildland fuels and their dependence on combustion efficiency, Atmos. Chem. Phys., 19, 1013–1026, https://doi.org/10.5194/acp-19-1013-2019, 2019.
Kelley, M., Schmidt, G. A., Nazarenko, L. S., Bauer, S. E., Ruedy, R., Russell, G. L., Ackerman, A. S., Aleinov, I., Bauer, M., Bleck, R., Canuto, V., Cesana, G., Cheng, Y., Clune, T. L., Cook, B. I., Cruz, C. A., Del Genio, A. D., Elsaesser, G. S., Faluvegi, G., Kiang, N. Y., Kim, D., Lacis, A. A., Leboissetier, A., LeGrande, A. N., Lo, K. K., Marshall, J., Matthews, E. E., McDermid, S., Mezuman, K., Miller, R. L., Murray, L. T., Oinas, V., Orbe, C., García-Pando, C. P., Perlwitz, J. P., Puma, M. J., Rind, D., Romanou, A., Shindell, D. T., Sun, S., Tausnev, N., Tsigaridis, K., Tselioudis, G., Weng, E., Wu, J., and Yao, M.-S.: GISS-E2.1: Configurations and Climatology, J. Adv. Model. Earth Sy., 12, e2019MS002025, https://doi.org/10.1029/2019MS002025, 2020.
Kim, P. S., Jacob, D. J., Fisher, J. A., Travis, K., Yu, K., Zhu, L., Yantosca, R. M., Sulprizio, M. P., Jimenez, J. L., Campuzano-Jost, P., Froyd, K. D., Liao, J., Hair, J. W., Fenn, M. A., Butler, C. F., Wagner, N. L., Gordon, T. D., Welti, A., Wennberg, P. O., Crounse, J. D., St. Clair, J. M., Teng, A. P., Millet, D. B., Schwarz, J. P., Markovic, M. Z., and Perring, A. E.: Sources, seasonality, and trends of southeast US aerosol: an integrated analysis of surface, aircraft, and satellite observations with the GEOS-Chem chemical transport model, Atmos. Chem. Phys., 15, 10411–10433, https://doi.org/10.5194/acp-15-10411-2015, 2015.
Le Breton, M., Wang, Y., Hallquist, Å. M., Pathak, R. K., Zheng, J., Yang, Y., Shang, D., Glasius, M., Bannan, T. J., Liu, Q., Chan, C. K., Percival, C. J., Zhu, W., Lou, S., Topping, D., Wang, Y., Yu, J., Lu, K., Guo, S., Hu, M., and Hallquist, M.: Online gas- and particle-phase measurements of organosulfates, organosulfonates and nitrooxy organosulfates in Beijing utilizing a FIGAERO ToF-CIMS, Atmos. Chem. Phys., 18, 10355–10371, https://doi.org/10.5194/acp-18-10355-2018, 2018.
Lee, L. A., Reddington, C. L., and Carslaw, K. S.: On the relationship between aerosol model uncertainty and radiative forcing uncertainty, P. Natl. Acad. Sci. USA, 113, 5820–5827, https://doi.org/10.1073/pnas.1507050113, 2016.
Leeper, R. D., Bilotta, R., Petersen, B., Stiles, C. J., Heim, R., Fuchs, B., Prat, O. P., Palecki, M., and Ansari, S.: Characterizing U.S. drought over the past 20 years using the U.S. drought monitor, Int. J. Climatol., 42, 6616–6630, https://doi.org/10.1002/joc.7653, 2022.
Li, W. and Wang, Y.: Reduced surface fine dust under droughts over the southeastern United States during summertime: observations and CMIP6 model simulations, Atmos. Chem. Phys., 22, 7843–7859, https://doi.org/10.5194/acp-22-7843-2022, 2022.
Li, W., Wang, Y., Flynn, J., Griffin, R. J., Guo, F., and Schnell, J. L.: Spatial variation of surface O3 responses to drought over the contiguous United States during summertime: Role of precursor emissions and ozone chemistry, J. Geophys. Res.-Atmos., 127, e2021JD035607, https://doi.org/10.1029/2021JD035607, 2022.
Llusià, J., Peñuelas, J., Alessio, G. A., and Estiarte, M.: Contrasting Species-Specific, Compound-Specific, Seasonal, and Interannual Responses of Foliar Isoprenoid Emissions to Experimental Drought in a Mediterranean Shrubland, Int. J. Plant Sci., 169, 637–645, https://doi.org/10.1086/533603, 2008.
Lopez-Hilfiker, F. D., Mohr, C., D'Ambro, E. L., Lutz, A., Riedel, T. P., Gaston, C. J., Iyer, S., Zhang, Z., Gold, A., Surratt, J. D., Lee, B. H., Kurten, T., Hu, W. W., Jimenez, J., Hallquist, M., and Thornton, J. A.: Molecular composition and volatility of organic aerosol in the southeastern U.S.: Implications for IEPOX derived SOA, Environ. Sci. Technol., 50, 2200–2209, https://doi.org/10.1021/acs.est.5b04769, 2016.
Malm, W. C., Schichtel, B. A., Hand, J. L., and Collett Jr., J. L.: Concurrent temporal and spatial trends in sulfate and organic mass concentrations measured in the IMPROVE monitoring program, J. Geophys. Res.-Atmos., 122, 10462–10476, https://doi.org/10.1002/2017JD026865, 2017.
Maria, S. F., Russell, L. M., Gilles, M. K., and Myneni, S. C. B.: Organic Aerosol Growth Mechanisms and Their Climate-Forcing Implications, Science, 306, 1921–1924, https://doi.org/10.1126/science.1103491, 2004.
McClure, C. D. and Jaffe, D. A.: US particulate matter air quality improves except in wildfire-prone areas, P. Natl. Acad. Sci. USA, 115, 7901–7906, https://doi.org/10.1073/pnas.1804353115, 2018.
NASA: CERES Time-Interpolated TOA Fluxes, Clouds and Aerosols Monthly Terra Edition4A, NASA Langley Atmospheric Science Data Center DAAC [data set], https://doi.org/10.5067/TERRA/CERES/SSF1DEGMONTH_L3.004A, 2015.
Pegoraro, E., Rey, A., Barron-Gafford, G., Monson, R., Malhi, Y., and Murthy, R.: The interacting effects of elevated atmospheric CO2 concentration, drought and leaf-to-air vapour pressure deficit on ecosystem isoprene fluxes, Oecologia, 146, 120–129, https://doi.org/10.1007/s00442-005-0166-5, 2005.
Potosnak, M. J., LeStourgeon, L., Pallardy, S. G., Hosman, K. P., Gu, L., Karl, T., Geron, C., and Guenther, A. B.: Observed and modeled ecosystem isoprene fluxes from an oak-dominated temperate forest and the influence of drought stress, Atmos. Environ., 84, 314–322, https://doi.org/10.1016/j.atmosenv.2013.11.055, 2014.
Pye, H. O. T., Murphy, B. N., Xu, L., Ng, N. L., Carlton, A. G., Guo, H., Weber, R., Vasilakos, P., Appel, K. W., Budisulistiorini, S. H., Surratt, J. D., Nenes, A., Hu, W., Jimenez, J. L., Isaacman-VanWertz, G., Misztal, P. K., and Goldstein, A. H.: On the implications of aerosol liquid water and phase separation for organic aerosol mass, Atmos. Chem. Phys., 17, 343–369, https://doi.org/10.5194/acp-17-343-2017, 2017.
Pye, H. O. T., Ward-Caviness, C. K., Murphy, B. N., Appel, K. W., and Seltzer, K. M.: Secondary organic aerosol association with cardiorespiratory disease mortality in the United States, Nat. Commun., 12, 7215, https://doi.org/10.1038/s41467-021-27484-1, 2021.
Randerson, J. T., Chen, Y., van der Werf, G. R., Rogers, B. M., and Morton, D. C.: Global burned area and biomass burning emissions from small fires, J. Geophys. Res.-Biogeo., 117, G04012, https://doi.org/10.1029/2012JG002128, 2012.
Rasch, P. J., Barth, M. C., Kiehl, J. T., Schwartz, S. E., and Benkovitz, C. M.: A description of the global sulfur cycle and its controlling processes in the National Center for Atmospheric Research Community Climate Model, Version 3, J. Geophys. Res.-Atmos., 105, 1367–1385, https://doi.org/10.1029/1999JD900777, 2000.
Ridley, D. A., Heald, C. L., Ridley, K. J., and Kroll, J. H.: Causes and consequences of decreasing atmospheric organic aerosol in the United States, P. Natl. Acad. Sci. USA, 115, 290–295, https://doi.org/10.1073/pnas.1700387115, 2018.
Riva, M., Tomaz, S., Cui, T., Lin, Y.-H., Perraudin, E., Gold, A., Stone, E. A., Villenave, E., and Surratt, J. D.: Evidence for an Unrecognized Secondary Anthropogenic Source of Organosulfates and Sulfonates: Gas-Phase Oxidation of Polycyclic Aromatic Hydrocarbons in the Presence of Sulfate Aerosol, Environ. Sci. Technol., 49, 6654–6664, https://doi.org/10.1021/acs.est.5b00836, 2015.
Ruffault, J., Curt, T., Martin-StPaul, N. K., Moron, V., and Trigo, R. M.: Extreme wildfire events are linked to global-change-type droughts in the northern Mediterranean, Nat. Hazards Earth Syst. Sci., 18, 847–856, https://doi.org/10.5194/nhess-18-847-2018, 2018.
Scasta, J. D., Weir, J. R., and Stambaugh, M. C.: Droughts and wildfires in western U.S. rangelands, Rangelands, 38, 197–203, https://doi.org/10.1016/j.rala.2016.06.003, 2016.
Schnell, J. L., Holmes, C. D., Jangam, A., and Prather, M. J.: Skill in forecasting extreme ozone pollution episodes with a global atmospheric chemistry model, Atmos. Chem. Phys., 14, 7721–7739, https://doi.org/10.5194/acp-14-7721-2014, 2014.
Schroder, J. C., Campuzano-Jost, P., Day, D. A., Shah, V., Larson, K., Sommers, J. M., Sullivan, A. P., Campos, T., Reeves, J. M., Hills, A., Hornbrook, R. S., Blake, N. J., Scheuer, E., Guo, H., Fibiger, D. L., McDuffie, E. E., Hayes, P. L., Weber, R. J., Dibb, J. E., Apel, E. C., Jaeglé, L., Brown, S. S., Thornton, J. A., and Jimenez, J. L.: Sources and secondary production of organic aerosols in the northeastern United States during winter, J. Geophys. Res.-Atmos., 123, 7771–7796, https://doi.org/10.1029/2018JD028475, 2018.
Séférian, R., Nabat, P., Michou, M., Saint-Martin, D., Voldoire, A., Colin, J., Decharme, B., Delire, C., Berthet, S., Chevallier, M., Sénési, S., Franchisteguy, L., Vial, J., Mallet, M., Joetzjer, E., Geoffroy, O., Guérémy, J.-F., Moine, M.-P., Msadek, R., Ribes, A., Rocher, M., Roehrig, R., Salas-y-Mélia, D., Sanchez, E., Terray, L., Valcke, S., Waldman, R., Aumont, O., Bopp, L., Deshayes, J., Éthé, C., and Madec, G.: Evaluation of CNRM Earth System Model, CNRM-ESM2-1: Role of Earth System Processes in Present-Day and Future Climate, J. Adv. Model. Earth Sy., 11, 4182–4227, https://doi.org/10.1029/2019MS001791, 2019.
Seland, Ø., Bentsen, M., Olivié, D., Toniazzo, T., Gjermundsen, A., Graff, L. S., Debernard, J. B., Gupta, A. K., He, Y.-C., Kirkevåg, A., Schwinger, J., Tjiputra, J., Aas, K. S., Bethke, I., Fan, Y., Griesfeller, J., Grini, A., Guo, C., Ilicak, M., Karset, I. H. H., Landgren, O., Liakka, J., Moseid, K. O., Nummelin, A., Spensberger, C., Tang, H., Zhang, Z., Heinze, C., Iversen, T., and Schulz, M.: Overview of the Norwegian Earth System Model (NorESM2) and key climate response of CMIP6 DECK, historical, and scenario simulations, Geosci. Model Dev., 13, 6165–6200, https://doi.org/10.5194/gmd-13-6165-2020, 2020.
Senior, C. A., Jones, C. G., Wood, R. A., Sellar, A., Belcher, S., Klein-Tank, A., Sutton, R., Walton, J., Lawrence, B., Andrews, T., and Mulcahy, J. P.: U.K. Community Earth System Modeling for CMIP6, J. Adv. Model. Earth Sy., 12, e2019MS002004, https://doi.org/10.1029/2019MS002004, 2020.
Shrivastava, M., Cappa, C. D., Fan, J., Goldstein, A. H., Guenther, A. B., Jimenez, J. L., Kuang, C., Laskin, A., Martin, S. T., Ng, N. L., Petaja, T., Pierce, J. R., Rasch, P. J., Roldin, P., Seinfeld, J. H., Shilling, J., Smith, J. N., Thornton, J. A., Volkamer, R., Wang, J., Worsnop, D. R., Zaveri, R. A., Zelenyuk, A., and Zhang, Q.: Recent advances in understanding secondary organic aerosol: Implications for global climate forcing, Rev. Geophys., 55, 509–559, https://doi.org/10.1002/2016RG000540, 2017.
Strzepek, K., Yohe, G., Neumann, J., and Boehlert, B.: Characterizing changes in drought risk for the United States from climate change, Environ. Res. Lett., 5, 044012, https://doi.org/10.1088/1748-9326/5/4/044012, 2010.
Surratt, J. D., Chan, A. W. H., Eddingsaas, N. C., Chan, M., Loza, C. L., Kwan, A. J., Hersey, S. P., Flagan, R. C., Wennberg, P. O., and Seinfeld, J. H.: Reactive intermediates revealed in secondary organic aerosol formation from isoprene, P. Natl. Acad. Sci. USA, 107, 6640–6645, https://doi.org/10.1073/pnas.0911114107, 2010.
Tai, A. P. K., Mickley, L. J., and Jacob, D. J.: Correlations between fine particulate matter (PM2.5) and meteorological variables in the United States: Implications for the sensitivity of PM2.5 to climate change, Atmos. Environ., 44, 3976–3984, https://doi.org/10.1016/j.atmosenv.2010.06.060, 2010.
Tatebe, H., Ogura, T., Nitta, T., Komuro, Y., Ogochi, K., Takemura, T., Sudo, K., Sekiguchi, M., Abe, M., Saito, F., Chikira, M., Watanabe, S., Mori, M., Hirota, N., Kawatani, Y., Mochizuki, T., Yoshimura, K., Takata, K., O'ishi, R., Yamazaki, D., Suzuki, T., Kurogi, M., Kataoka, T., Watanabe, M., and Kimoto, M.: Description and basic evaluation of simulated mean state, internal variability, and climate sensitivity in MIROC6, Geosci. Model Dev., 12, 2727–2765, https://doi.org/10.5194/gmd-12-2727-2019, 2019.
Taufik, M., Torfs, P. J. J. F., Uijlenhoet, R., Jones, P. D., Murdiyarso, D., and Van Lanen, H. A. J.: Amplification of wildfire area burnt by hydrological drought in the humid tropics, Nat. Clim. Change, 7, 428–431, https://doi.org/10.1038/nclimate3280, 2017.
Thornhill, G., Collins, W., Olivié, D., Skeie, R. B., Archibald, A., Bauer, S., Checa-Garcia, R., Fiedler, S., Folberth, G., Gjermundsen, A., Horowitz, L., Lamarque, J.-F., Michou, M., Mulcahy, J., Nabat, P., Naik, V., O'Connor, F. M., Paulot, F., Schulz, M., Scott, C. E., Séférian, R., Smith, C., Takemura, T., Tilmes, S., Tsigaridis, K., and Weber, J.: Climate-driven chemistry and aerosol feedbacks in CMIP6 Earth system models, Atmos. Chem. Phys., 21, 1105–1126, https://doi.org/10.5194/acp-21-1105-2021, 2021.
Tsui, W. G., Woo, J. L., and McNeill, V. F.: Impact of Aerosol-Cloud Cycling on Aqueous Secondary Organic Aerosol Formation, Atmosphere, 10, 666, https://doi.org/10.3390/atmos10110666, 2019.
Turnock, S. T., Allen, R. J., Andrews, M., Bauer, S. E., Deushi, M., Emmons, L., Good, P., Horowitz, L., John, J. G., Michou, M., Nabat, P., Naik, V., Neubauer, D., O'Connor, F. M., Olivié, D., Oshima, N., Schulz, M., Sellar, A., Shim, S., Takemura, T., Tilmes, S., Tsigaridis, K., Wu, T., and Zhang, J.: Historical and future changes in air pollutants from CMIP6 models, Atmos. Chem. Phys., 20, 14547–14579, https://doi.org/10.5194/acp-20-14547-2020, 2020.
van Noije, T., Bergman, T., Le Sager, P., O'Donnell, D., Makkonen, R., Gonçalves-Ageitos, M., Döscher, R., Fladrich, U., von Hardenberg, J., Keskinen, J.-P., Korhonen, H., Laakso, A., Myriokefalitakis, S., Ollinaho, P., Pérez García-Pando, C., Reerink, T., Schrödner, R., Wyser, K., and Yang, S.: EC-Earth3-AerChem: a global climate model with interactive aerosols and atmospheric chemistry participating in CMIP6, Geosci. Model Dev., 14, 5637–5668, https://doi.org/10.5194/gmd-14-5637-2021, 2021.
Vicente-Serrano, S. M., Beguería, S., and López-Moreno, J. I.: A multiscalar drought index sensitive to global warming: The Standardized Precipitation Evapotranspiration Index, J. Climate, 23, 1696–1718, https://doi.org/10.1175/2009JCLI2909.1, 2010 (data available at: https://spei.csic.es/spei_database_2_6, last access: 21 August 2024).
Wang, Y., Xie, Y., Cai, L., Dong, W., Zhang, Q., and Zhang, L.: Impact of the 2011 southern U.S. drought on ground-level fine aerosol concentration in summertime, J. Atmos. Sci., 72, 1075–1093, https://doi.org/10.1175/JAS-D-14-0197.1, 2015.
Wang, Y., Xie, Y., Dong, W., Ming, Y., Wang, J., and Shen, L.: Adverse effects of increasing drought on air quality via natural processes, Atmos. Chem. Phys., 17, 12827–12843, https://doi.org/10.5194/acp-17-12827-2017, 2017.
Wang, Y., Wang, J., Wang, Y., and Li, W.: Drought impacts on PM2.5 composition and amount over the US during 1988–2018, J. Geophys. Res.-Atmos., 127, e2022JD037677, https://doi.org/10.1029/2022JD037677, 2022a.
Wang, Y., Lin, N., Li, W., Guenther, A., Lam, J. C. Y., Tai, A. P. K., Potosnak, M. J., and Seco, R.: Satellite-derived constraints on the effect of drought stress on biogenic isoprene emissions in the southeastern US, Atmos. Chem. Phys., 22, 14189–14208, https://doi.org/10.5194/acp-22-14189-2022, 2022b.
Wilhite, D. A., Svoboda, M. D., and Hayes, M. J.: Understanding the complex impacts of drought: A key to enhancing drought mitigation and preparedness, Water Resour. Manag., 21, 763–774, https://doi.org/10.1007/s11269-006-9076-5, 2007.
Wu, C., Pullinen, I., Andres, S., Carriero, G., Fares, S., Goldbach, H., Hacker, L., Kasal, T., Kiendler-Scharr, A., Kleist, E., Paoletti, E., Wahner, A., Wildt, J., and Mentel, Th. F.: Impacts of soil moisture on de novo monoterpene emissions from European beech, Holm oak, Scots pine, and Norway spruce, Biogeosciences, 12, 177–191, https://doi.org/10.5194/bg-12-177-2015, 2015.
Wu, T., Zhang, F., Zhang, J., Jie, W., Zhang, Y., Wu, F., Li, L., Yan, J., Liu, X., Lu, X., Tan, H., Zhang, L., Wang, J., and Hu, A.: Beijing Climate Center Earth System Model version 1 (BCC-ESM1): model description and evaluation of aerosol simulations, Geosci. Model Dev., 13, 977–1005, https://doi.org/10.5194/gmd-13-977-2020, 2020.
Xie, Y., Wang, Y., Dong, W., Wright, J. S., Shen, L., and Zhao, Z.: Evaluating the response of summertime surface sulfate to hydroclimate variations in the continental United States: Role of meteorological inputs in the GEOS-Chem model, J. Geophys. Res.-Atmos., 124, 1662–1679, https://doi.org/10.1029/2018JD029693, 2019.
Xu, L., Guo, H., Boyd, C. M., Klein, M., Bougiatioti, A., Cerully, K. M., Hite, J. R., Isaacman-VanWertz, G., Kreisberg, N. M., and Knote, C.: Effects of anthropogenic emissions on aerosol formation from isoprene and monoterpenes in the southeastern United States, P. Natl. Acad. Sci. USA, 112, 37–42, 2015.
Yli-Juuti, T., Mielonen, T., Heikkinen, L., Arola, A., Ehn, M., Isokääntä, S., Keskinen, H.-M., Kulmala, M., Laakso, A., Lipponen, A., Luoma, K., Mikkonen, S., Nieminen, T., Paasonen, P., Petäjä, T., Romakkaniemi, S., Tonttila, J., Kokkola, H., and Virtanen, A.: Significance of the organic aerosol driven climate feedback in the boreal area, Nat. Commun., 12, 5637, https://doi.org/10.1038/s41467-021-25850-7, 2021.
Yukimoto, S., Kawai, H., Koshiro, T., Oshima, N., Yoshida, K., Urakawa, S., Tsujino, H., Deushi, M., Tanaka, T., Hosaka, M., Yabu, S., Yoshimura, H., Shindo, E., Mizuta, R., Obata, A., Adachi, Y., and Ishii, M.: The Meteorological Research Institute Earth System Model Version 2.0, MRI-ESM2.0: Description and Basic Evaluation of the Physical Component, J. Meteorol. Soc. Jpn., Ser. II, 97, 931–965, https://doi.org/10.2151/jmsj.2019-051, 2019.
Zhang, Q., Jimenez, J. L., Canagaratna, M. R., Ulbrich, I. M., Ng, N. L., Worsnop, D. R., and Sun, Y.: Understanding atmospheric organic aerosols via factor analysis of aerosol mass spectrometry: a review, Anal. Bioanal. Chem., 401, 3045–3067, https://doi.org/10.1007/s00216-011-5355-y, 2011.
Zhang, X., Liu, Z., Hecobian, A., Zheng, M., Frank, N. H., Edgerton, E. S., and Weber, R. J.: Spatial and seasonal variations of fine particle water-soluble organic carbon (WSOC) over the southeastern United States: implications for secondary organic aerosol formation, Atmos. Chem. Phys., 12, 6593–6607, https://doi.org/10.5194/acp-12-6593-2012, 2012.
Zhao, Z., Wang, Y., Qin, M., Hu, Y., Xie, Y., and Russell, A. G.: Drought impacts on secondary organic aerosol: a case study in the southeast United States, Environ. Sci. Technol., 53, 242–250, https://doi.org/10.1021/acs.est.8b04842, 2019.
Zheng, Y., Thornton, J. A., Ng, N. L., Cao, H., Henze, D. K., McDuffie, E. E., Hu, W., Jimenez, J. L., Marais, E. A., Edgerton, E., and Mao, J.: Long-term observational constraints of organic aerosol dependence on inorganic species in the southeast US, Atmos. Chem. Phys., 20, 13091–13107, https://doi.org/10.5194/acp-20-13091-2020, 2020.
Short summary
Droughts immensely increased organic aerosol (OA) in the contiguous United States in summer (1998–2019), notably in the Pacific Northwest (PNW) and Southeast (SEUS). The OA rise in the SEUS is driven by the enhanced formation of epoxydiol-derived secondary organic aerosol due to the increase in biogenic volatile organic compounds and sulfate, while in the PNW, it is caused by wildfires. A total of 10 climate models captured the OA increase in the PNW yet greatly underestimated it in the SEUS.
Droughts immensely increased organic aerosol (OA) in the contiguous United States in summer...
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