Articles | Volume 24, issue 21
https://doi.org/10.5194/acp-24-12375-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-12375-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
11 Nov 2024
Research article |
| 11 Nov 2024
| 11 Nov 2024
Influence of cloudy and clear-sky partitions, aerosols, and geometry on the recent variability in surface solar irradiance components in northern France
Gabriel Chesnoiu
Université de Lille, CNRS, UMR 8518 – LOA, 59000 Lille, France
Nicolas Ferlay
CORRESPONDING AUTHOR
Université de Lille, CNRS, UMR 8518 – LOA, 59000 Lille, France
Isabelle Chiapello
Université de Lille, CNRS, UMR 8518 – LOA, 59000 Lille, France
Frédérique Auriol
Université de Lille, CNRS, UMR 8518 – LOA, 59000 Lille, France
Diane Catalfamo
Université de Lille, CNRS, UMR 8518 – LOA, 59000 Lille, France
Mathieu Compiègne
HYGEOS, Euratechnologies, Avenue de Bretagne, 59000 Lille, France
Thierry Elias
HYGEOS, Euratechnologies, Avenue de Bretagne, 59000 Lille, France
Isabelle Jankowiak
Université de Lille, CNRS, UMR 8518 – LOA, 59000 Lille, France
Related authors
Gabriel Chesnoiu, Isabelle Chiapello, Nicolas Ferlay, Pierre Nabat, Marc Mallet, and Véronique Riffault
Atmos. Chem. Phys., 25, 1307–1331, https://doi.org/10.5194/acp-25-1307-2025, https://doi.org/10.5194/acp-25-1307-2025, 2025
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The ALADIN regional climate model at 12.5 km resolution allows us to study the evolution of surface solar radiation (SSR) and key associated atmospheric parameters. Over northern France and Benelux, influenced by anthropogenic aerosols and cloudy conditions, regional evaluation of recent hindcast simulations shows satisfying results and high spatial variability. Future SSR evolution by the end of the century for two contrasting CMIP6 scenarios highlights large decreases in SSR for SSP3-7.0.
Thierry Elias, Nicolas Ferlay, Gabriel Chesnoiu, Isabelle Chiapello, and Mustapha Moulana
Atmos. Meas. Tech., 17, 4041–4063, https://doi.org/10.5194/amt-17-4041-2024, https://doi.org/10.5194/amt-17-4041-2024, 2024
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In the solar energy application field, it is key to simulate solar resources anywhere on the globe. We conceived the Solar Resource estimate (SolaRes) tool to provide precise and accurate estimates of solar resources for any solar plant technology. We present the validation of SolaRes by comparing estimates with measurements made on two ground-based platforms in northern France for 2 years at 1 min resolution. Validation is done in clear-sky conditions where aerosols are the main factors.
Adèle Georgeot, Xavier Ceamanos, Jean-Luc Attié, Daniel Juncu, Josef Gasteiger, and Mathieu Compiègne
EGUsphere, https://doi.org/10.5194/egusphere-2025-1353, https://doi.org/10.5194/egusphere-2025-1353, 2025
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This work investigates the aerosol remote sensing capabilities offered by the new Meteosat Third Generation-Imager geostationary satellite. First, aerosol load retrieval performance is demonstrated based on realistic synthetic data. Second, the potential for aerosol type characterization is proven, with the estimation of fine mode fraction. This work opens pathways for the future study of diurnal aerosol variations from space thanks to the high temporal resolution of geostationary satellites.
Gabriel Chesnoiu, Isabelle Chiapello, Nicolas Ferlay, Pierre Nabat, Marc Mallet, and Véronique Riffault
Atmos. Chem. Phys., 25, 1307–1331, https://doi.org/10.5194/acp-25-1307-2025, https://doi.org/10.5194/acp-25-1307-2025, 2025
Short summary
Short summary
The ALADIN regional climate model at 12.5 km resolution allows us to study the evolution of surface solar radiation (SSR) and key associated atmospheric parameters. Over northern France and Benelux, influenced by anthropogenic aerosols and cloudy conditions, regional evaluation of recent hindcast simulations shows satisfying results and high spatial variability. Future SSR evolution by the end of the century for two contrasting CMIP6 scenarios highlights large decreases in SSR for SSP3-7.0.
Mégane Ventura, Fabien Waquet, Isabelle Chiapello, Gérard Brogniez, Frédéric Parol, Frédérique Auriol, Rodrigue Loisil, Cyril Delegove, Luc Blarel, Oleg Dubovik, Marc Mallet, Cyrille Flamant, and Paola Formenti
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-121, https://doi.org/10.5194/amt-2024-121, 2024
Revised manuscript accepted for AMT
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Biomass burning aerosols (BBA) from Central Africa, are transported above stratocumulus clouds. The absorption of solar energy by aerosols induce warming, altering the clouds dynamics. We developed an approach that combines polarimeter and lidar to quantify it. This methodology is assessed during the AEROCLO-SA campaign. To validate it, we used flux measurements acquired during aircraft loop descents. Major perspective is the generalization of this method to the global level.
Thierry Elias, Nicolas Ferlay, Gabriel Chesnoiu, Isabelle Chiapello, and Mustapha Moulana
Atmos. Meas. Tech., 17, 4041–4063, https://doi.org/10.5194/amt-17-4041-2024, https://doi.org/10.5194/amt-17-4041-2024, 2024
Short summary
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In the solar energy application field, it is key to simulate solar resources anywhere on the globe. We conceived the Solar Resource estimate (SolaRes) tool to provide precise and accurate estimates of solar resources for any solar plant technology. We present the validation of SolaRes by comparing estimates with measurements made on two ground-based platforms in northern France for 2 years at 1 min resolution. Validation is done in clear-sky conditions where aerosols are the main factors.
Alejandra Velazquez-Garcia, Joel F. de Brito, Suzanne Crumeyrolle, Isabelle Chiapello, and Véronique Riffault
Aerosol Research, 2, 107–122, https://doi.org/10.5194/ar-2-107-2024, https://doi.org/10.5194/ar-2-107-2024, 2024
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Multi-annual in situ observations were combined with back trajectory and emissions inventories to study black and brown carbon (BC, BrC) sources in the north of France. Results show BC to be mainly originated from vehicular traffic (31 %), shipping (25 %), and residential heating (21 %). Also, a significant decrease of the BrC component from residential heating is observed after 24 h of atmospheric aging. These results should lead to better climate and air pollution mitigation strategies.
Thomas D. DeWitt, Timothy J. Garrett, Karlie N. Rees, Corey Bois, Steven K. Krueger, and Nicolas Ferlay
Atmos. Chem. Phys., 24, 109–122, https://doi.org/10.5194/acp-24-109-2024, https://doi.org/10.5194/acp-24-109-2024, 2024
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Viewed from space, a defining feature of Earth's atmosphere is the wide spectrum of cloud sizes. A recent study predicted the distribution of cloud sizes, and this paper compares the prediction to observations. Although there is nuance in viewing perspective, we find robust agreement with theory across different climatological conditions, including land–ocean contrasts, time of year, or latitude, suggesting a minor role for Coriolis forces, aerosol loading, or surface temperature.
Christian Matar, Céline Cornet, Frédéric Parol, Laurent C.-Labonnote, Frédérique Auriol, and Marc Nicolas
Atmos. Meas. Tech., 16, 3221–3243, https://doi.org/10.5194/amt-16-3221-2023, https://doi.org/10.5194/amt-16-3221-2023, 2023
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The optimal estimation formalism is applied to OSIRIS airborne high-resolution multi-angular measurements to retrieve COT and Reff. The corresponding uncertainties related to measurement errors, which are up to 6 and 12 %, the non-retrieved parameters, which are less than 0.5 %, and the cloud model assumptions show that the heterogeneous vertical profiles and the 3D radiative transfer effects lead to average uncertainties of 5 and 4 % for COT and 13 and 9 % for Reff.
Suzanne Crumeyrolle, Jenni S. S. Kontkanen, Clémence Rose, Alejandra Velazquez Garcia, Eric Bourrianne, Maxime Catalfamo, Véronique Riffault, Emmanuel Tison, Joel Ferreira de Brito, Nicolas Visez, Nicolas Ferlay, Frédérique Auriol, and Isabelle Chiapello
Atmos. Chem. Phys., 23, 183–201, https://doi.org/10.5194/acp-23-183-2023, https://doi.org/10.5194/acp-23-183-2023, 2023
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Ultrafine particles (UFPs) are particles with an aerodynamic diameter of 100 nm or less and negligible mass concentration but are the dominant contributor to the total particle number concentration. The present study aims to better understand the environmental factors favoring or inhibiting atmospheric new particle formation (NPF) over Lille, a large city in the north of France, and to analyze the impact of such an event on urban air quality using a long-term dataset (3 years).
Kostas Eleftheratos, John Kapsomenakis, Ilias Fountoulakis, Christos S. Zerefos, Patrick Jöckel, Martin Dameris, Alkiviadis F. Bais, Germar Bernhard, Dimitra Kouklaki, Kleareti Tourpali, Scott Stierle, J. Ben Liley, Colette Brogniez, Frédérique Auriol, Henri Diémoz, Stana Simic, Irina Petropavlovskikh, Kaisa Lakkala, and Kostas Douvis
Atmos. Chem. Phys., 22, 12827–12855, https://doi.org/10.5194/acp-22-12827-2022, https://doi.org/10.5194/acp-22-12827-2022, 2022
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We present the future evolution of DNA-active ultraviolet (UV) radiation in view of increasing greenhouse gases (GHGs) and decreasing ozone depleting substances (ODSs). It is shown that DNA-active UV radiation might increase after 2050 between 50° N–50° S due to GHG-induced reductions in clouds and ozone, something that is likely not to happen at high latitudes, where DNA-active UV radiation will continue its downward trend mainly due to stratospheric ozone recovery from the reduction in ODSs.
Alexandre Siméon, Fabien Waquet, Jean-Christophe Péré, Fabrice Ducos, François Thieuleux, Fanny Peers, Solène Turquety, and Isabelle Chiapello
Atmos. Chem. Phys., 21, 17775–17805, https://doi.org/10.5194/acp-21-17775-2021, https://doi.org/10.5194/acp-21-17775-2021, 2021
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For the first time, we accurately modelled the optical properties of the biomass burning aerosols (BBA) observed over the Southeast Atlantic region during their transport above clouds and over their source regions, combining a meteorology coupled with chemistry model (WRF-Chem) with innovative satellite absorbing aerosol retrievals (POLDER-3). Our results suggest a low but non-negligible brown carbon fraction (3 %) for the chemical composition of the BBA plumes observed over the source regions.
Isabelle Chiapello, Paola Formenti, Lydie Mbemba Kabuiku, Fabrice Ducos, Didier Tanré, and François Dulac
Atmos. Chem. Phys., 21, 12715–12737, https://doi.org/10.5194/acp-21-12715-2021, https://doi.org/10.5194/acp-21-12715-2021, 2021
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The Mediterranean atmosphere is impacted by a variety of particle pollution, which exerts a complex pressure on climate and air quality. We analyze the 2005–2013 POLDER-3 satellite advanced aerosol data set over the Western Mediterranean Sea. Aerosols' spatial distribution and temporal evolution suggests a large-scale improvement of air quality related to the fine aerosol component, most probably resulting from reduction of anthropogenic particle emissions in the surrounding European countries.
Aurélien Chauvigné, Fabien Waquet, Frédérique Auriol, Luc Blarel, Cyril Delegove, Oleg Dubovik, Cyrille Flamant, Marco Gaetani, Philippe Goloub, Rodrigue Loisil, Marc Mallet, Jean-Marc Nicolas, Frédéric Parol, Fanny Peers, Benjamin Torres, and Paola Formenti
Atmos. Chem. Phys., 21, 8233–8253, https://doi.org/10.5194/acp-21-8233-2021, https://doi.org/10.5194/acp-21-8233-2021, 2021
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This work presents aerosol above-cloud properties close to the Namibian coast from a combination of airborne passive remote sensing. The complete analysis of aerosol and cloud optical properties and their microphysical and radiative properties allows us to better identify the impacts of biomass burning emissions. This work also gives a complete overview of the key parameters for constraining climate models in case aerosol and cloud coexist in the troposphere.
Kaisa Lakkala, Jukka Kujanpää, Colette Brogniez, Nicolas Henriot, Antti Arola, Margit Aun, Frédérique Auriol, Alkiviadis F. Bais, Germar Bernhard, Veerle De Bock, Maxime Catalfamo, Christine Deroo, Henri Diémoz, Luca Egli, Jean-Baptiste Forestier, Ilias Fountoulakis, Katerina Garane, Rosa Delia Garcia, Julian Gröbner, Seppo Hassinen, Anu Heikkilä, Stuart Henderson, Gregor Hülsen, Bjørn Johnsen, Niilo Kalakoski, Angelos Karanikolas, Tomi Karppinen, Kevin Lamy, Sergio F. León-Luis, Anders V. Lindfors, Jean-Marc Metzger, Fanny Minvielle, Harel B. Muskatel, Thierry Portafaix, Alberto Redondas, Ricardo Sanchez, Anna Maria Siani, Tove Svendby, and Johanna Tamminen
Atmos. Meas. Tech., 13, 6999–7024, https://doi.org/10.5194/amt-13-6999-2020, https://doi.org/10.5194/amt-13-6999-2020, 2020
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The TROPOspheric Monitoring Instrument (TROPOMI) onboard the Sentinel-5 Precursor (S5P) satellite was launched on 13 October 2017 to provide the atmospheric composition for atmosphere and climate research. Ground-based data from 25 sites located in Arctic, subarctic, temperate, equatorial and Antarctic
areas were used for the validation of the TROPOMI surface ultraviolet (UV) radiation product. For most sites 60 %–80 % of TROPOMI data was within ± 20 % of ground-based data.
Marie-Thérèse El Kattar, Frédérique Auriol, and Hervé Herbin
Atmos. Meas. Tech., 13, 3769–3786, https://doi.org/10.5194/amt-13-3769-2020, https://doi.org/10.5194/amt-13-3769-2020, 2020
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This paper is submitted as part of my thesis project. It highlights the importance of ground-based measurements for future satellite validations. This paper represents the characteristics of a new prototype called CHRIS, which is the MIR version of the EM27/SUN. Our primary concern is the exploitation of the data of the MAGIC campaign, which is a French initiative in collaboration with the CoMet project, to monitor greenhouse gases.
Marie Boichu, Olivier Favez, Véronique Riffault, Jean-Eudes Petit, Yunjiang Zhang, Colette Brogniez, Jean Sciare, Isabelle Chiapello, Lieven Clarisse, Shouwen Zhang, Nathalie Pujol-Söhne, Emmanuel Tison, Hervé Delbarre, and Philippe Goloub
Atmos. Chem. Phys., 19, 14253–14287, https://doi.org/10.5194/acp-19-14253-2019, https://doi.org/10.5194/acp-19-14253-2019, 2019
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This study, benefiting especially from recently developed mass spectrometry observations of aerosols, highlights unknown properties of volcanic sulfates in the troposphere. It shows their specific chemical fingerprint, distinct from those of freshly emitted industrial sulfates and background aerosols. We also demonstrate the large-scale persistence of the volcanic sulfate pollution over weeks. Hence, these results cast light on the impact of tropospheric eruptions on air quality and climate.
Lucia T. Deaconu, Nicolas Ferlay, Fabien Waquet, Fanny Peers, François Thieuleux, and Philippe Goloub
Atmos. Chem. Phys., 19, 11613–11634, https://doi.org/10.5194/acp-19-11613-2019, https://doi.org/10.5194/acp-19-11613-2019, 2019
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We analyse and quantify the effect of above-cloud aerosol (AAC) loading on the underlying cloud properties in the South Atlantic Ocean. We use a synergy of remote sensing retrievals collocated with ERA-Interim meteorological profiles. The results show that for larger loads of AACs, clouds are optically thicker, with an increase in liquid water path by 20 g m−2 and lower cloud-top altitudes. We also observe a strong covariation between the aerosol plume and the presence of water vapour.
Marie Mazoyer, Frédéric Burnet, Cyrielle Denjean, Gregory C. Roberts, Martial Haeffelin, Jean-Charles Dupont, and Thierry Elias
Atmos. Chem. Phys., 19, 4323–4344, https://doi.org/10.5194/acp-19-4323-2019, https://doi.org/10.5194/acp-19-4323-2019, 2019
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In situ microphysical measurements collected during 23 fog events at SIRTA (south of Paris) are examined here. An original iterative method based on the κ-Köhler theory has been used to compute statistics of their activation properties. Useful information is provided to constrain and validate numerical simulations. The paper demonstrates that supersaturation encountered in these fogs is too low to observe a correlation between concentrations of aerosols > 200 nm and droplet concentrations.
Paola Formenti, Lydie Mbemba Kabuiku, Isabelle Chiapello, Fabrice Ducos, François Dulac, and Didier Tanré
Atmos. Meas. Tech., 11, 6761–6784, https://doi.org/10.5194/amt-11-6761-2018, https://doi.org/10.5194/amt-11-6761-2018, 2018
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Aerosol particles from natural and anthropogenic sources are climate regulators as they can counteract or amplify the warming effect of greenhouse gases, but are difficult to observe due to their temporal and spatial variability. Satellite sensors can provide the needed global coverage but need validation. In this paper we explore the capability of the POLDER-3 advanced space-borne sensor to observe aerosols over the western Mediterranean region.
Lucia T. Deaconu, Fabien Waquet, Damien Josset, Nicolas Ferlay, Fanny Peers, François Thieuleux, Fabrice Ducos, Nicolas Pascal, Didier Tanré, Jacques Pelon, and Philippe Goloub
Atmos. Meas. Tech., 10, 3499–3523, https://doi.org/10.5194/amt-10-3499-2017, https://doi.org/10.5194/amt-10-3499-2017, 2017
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This study presents a comparison between active (CALIOP) and passive (POLDER) remote sensing methods, developed for retrieving aerosol above-cloud optical and microphysical properties. Main results show a good agreement when the aerosol microphysics is dominated by fine-mode particles or coarse-mode dust or when the aerosol layer is well separated from the cloud below. The paper is also focused on understanding the differences between the retrievals and the limitations of each method.
Guillaume Merlin, Jérôme Riedi, Laurent C. Labonnote, Céline Cornet, Anthony B. Davis, Phillipe Dubuisson, Marine Desmons, Nicolas Ferlay, and Frédéric Parol
Atmos. Meas. Tech., 9, 4977–4995, https://doi.org/10.5194/amt-9-4977-2016, https://doi.org/10.5194/amt-9-4977-2016, 2016
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The vertical distribution of cloud cover has a significant impact on a large number of meteorological and climatic processes. Cloud top altitude (CTOP) and cloud geometrical thickness (CGT) are essential for understanding these processes. Previous studies established the possibility of retrieving those parameters from multi-angular oxygen A-band measurements. Here we perform a study and comparison of the performance of future instruments.
Jean-Baptiste Renard, François Dulac, Gwenaël Berthet, Thibaut Lurton, Damien Vignelles, Fabrice Jégou, Thierry Tonnelier, Matthieu Jeannot, Benoit Couté, Rony Akiki, Nicolas Verdier, Marc Mallet, François Gensdarmes, Patrick Charpentier, Samuel Mesmin, Vincent Duverger, Jean-Charles Dupont, Thierry Elias, Vincent Crenn, Jean Sciare, Paul Zieger, Matthew Salter, Tjarda Roberts, Jérôme Giacomoni, Matthieu Gobbi, Eric Hamonou, Haraldur Olafsson, Pavla Dagsson-Waldhauserova, Claude Camy-Peyret, Christophe Mazel, Thierry Décamps, Martin Piringer, Jérémy Surcin, and Daniel Daugeron
Atmos. Meas. Tech., 9, 3673–3686, https://doi.org/10.5194/amt-9-3673-2016, https://doi.org/10.5194/amt-9-3673-2016, 2016
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We illustrate the first Light Optical Aerosol Counter (LOAC) airborne results obtained from an unmanned aerial vehicle (UAV) and a variety of scientific balloons: tethered balloons deployed in urban environments, pressurized balloons drifting in the lower troposphere over the western Mediterranean during the Chemistry-Aerosol Mediterranean Experiment (ChArMEx), and meteorological sounding balloons launched in the western Mediterranean region and in the south-west of France.
M. Mazoyer, F. Burnet, G. C. Roberts, M. Haeffelin, J.-C Dupont, and T. Elias
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-103, https://doi.org/10.5194/acp-2016-103, 2016
Preprint withdrawn
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Comprehensive field campaigns dedicated to fog life cycle observation were conducted during the winters of 2010–2013 at the SIRTA observatory in the suburb of Paris. The objective of this paper is to evaluate the impact of aerosol particles on the fog microphysics
through an original method. We conclude that the actual supersaturations reached during these fog episodes are too low and no simultaneous increase of aerosols (D > 200 nm) and droplet concentrations can be observed.
Jean-Baptiste Renard, François Dulac, Gwenaël Berthet, Thibaut Lurton, Damien Vignelles, Fabrice Jégou, Thierry Tonnelier, Matthieu Jeannot, Benoit Couté, Rony Akiki, Nicolas Verdier, Marc Mallet, François Gensdarmes, Patrick Charpentier, Samuel Mesmin, Vincent Duverger, Jean-Charles Dupont, Thierry Elias, Vincent Crenn, Jean Sciare, Paul Zieger, Matthew Salter, Tjarda Roberts, Jérôme Giacomoni, Matthieu Gobbi, Eric Hamonou, Haraldur Olafsson, Pavla Dagsson-Waldhauserova, Claude Camy-Peyret, Christophe Mazel, Thierry Décamps, Martin Piringer, Jérémy Surcin, and Daniel Daugeron
Atmos. Meas. Tech., 9, 1721–1742, https://doi.org/10.5194/amt-9-1721-2016, https://doi.org/10.5194/amt-9-1721-2016, 2016
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LOAC is a light aerosols counter for performing measurements at the surface and under all kinds of atmospheric balloons. LOAC performs observations at two scattering angles. The first one at 12° is insensitive to the refractive index of the particles; the second one at 60° is strongly sensitive to the refractive index. By combining the measurements, it is possible to retrieve the size distribution between 0.2 and 100 micrometeres and to estimate the nature of the dominant particles.
T. Elias, J.-C. Dupont, E. Hammer, C. R. Hoyle, M. Haeffelin, F. Burnet, and D. Jolivet
Atmos. Chem. Phys., 15, 6605–6623, https://doi.org/10.5194/acp-15-6605-2015, https://doi.org/10.5194/acp-15-6605-2015, 2015
J.-B. Renard, F. Dulac, G. Berthet, T. Lurton, D. Vignelle, F. Jégou, T. Tonnelier, C. Thaury, M. Jeannot, B. Couté, R. Akiki, J.-L. Mineau, N. Verdier, M. Mallet, F. Gensdarmes, P. Charpentier, S. Mesmin, V. Duverger, J.-C. Dupont, T. Elias, V. Crenn, J. Sciare, J. Giacomoni, M. Gobbi, E. Hamonou, H. Olafsson, P. Dagsson-Waldhauserova, C. Camy-Peyret, C. Mazel, T. Décamps, M. Piringer, J. Surcin, and D. Daugeron
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amtd-8-1261-2015, https://doi.org/10.5194/amtd-8-1261-2015, 2015
Revised manuscript not accepted
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We present exemples of measurements obtained by the new light optical aerosol counter LOAC. The measurement were conducted from different kinds of balloons in the troposphre and stratosphere.
M. Desmons, N. Ferlay, F. Parol, L. Mcharek, and C. Vanbauce
Atmos. Meas. Tech., 6, 2221–2238, https://doi.org/10.5194/amt-6-2221-2013, https://doi.org/10.5194/amt-6-2221-2013, 2013
Related subject area
Subject: Radiation | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
The modulation of synoptic weather patterns and human activities on the diurnal cycle of the summertime canopy urban heat island in the Yangtze River Delta Urban Agglomeration, China
Mechanisms of surface solar irradiance variability under broken clouds
Fine and coarse dust radiative impact during an intense Saharan dust outbreak over the Iberian Peninsula – short-wave direct radiative effect
Modeling actinic flux and photolysis frequencies in dense biomass burning plumes
Regional modeling of surface solar radiation, aerosol, and cloud cover spatial variability and projections over northern France and Benelux
A numerical sensitivity study on the snow-darkening effect by black carbon deposition over the Arctic in spring
Improved calculation of single-scattering properties of frozen droplets and frozen-droplet aggregates observed in deep convective clouds
Saharan dust impact on radiative heating rate errors inherent in reanalysis data in the African easterly wave development region
Sensitivity of ice cloud radiative heating to optical, macro- and microphysical properties
Combining observations and simulations to investigate the small-scale variability of surface solar irradiance under continental cumulus clouds
The impact of coupled 3D shortwave radiative transfer on surface radiation and cumulus clouds over land
Atmospheric cloud-radiative heating in CMIP6 and observations and its response to surface warming
Responses of polar energy budget to regional SST changes in extra-polar regions
Trends in observed surface solar radiation and their causes in Brazil in the first 2 decades of the 21st century
A sensitivity study on radiative effects due to the parameterization of dust optical properties in models
Uncertainties in cloud-radiative heating within an idealized extratropical cyclone
Evaluation of downward and upward solar irradiances simulated by the Integrated Forecasting System of ECMWF using airborne observations above Arctic low-level clouds
A colorful look at climate sensitivity
Sensitivity of cirrus and contrail radiative effect on cloud microphysical and environmental parameters
Evaluation of liquid cloud albedo susceptibility in E3SM using coupled eastern North Atlantic surface and satellite retrievals
Constraints on simulated past Arctic amplification and lapse rate feedback from observations
Comparison of methods to estimate aerosol effective radiative forcings in climate models
Montreal Protocol's impact on the ozone layer and climate
Opinion: The scientific and community-building roles of the Geoengineering Model Intercomparison Project (GeoMIP) – past, present, and future
Impacts of reductions in non-methane short-lived climate forcers on future climate extremes and the resulting population exposure risks in eastern and southern Asia
Investigating the radiative effect of Arctic cirrus measured in situ during the winter 2015–2016
Dependence of strategic solar climate intervention on background scenario and model physics
Combining short-range dispersion simulations with fine-scale meteorological ensembles: probabilistic indicators and evaluation during a 85Kr field campaign
Climate consequences of hydrogen emissions
Investigating the impact of Saharan dust aerosols on analyses and forecasts of African easterly waves by constraining aerosol effects in radiance data assimilation
Distinct surface response to black carbon aerosols
Estimating the potential cooling effect of cirrus thinning achieved via the seeding approach
Impacts of multi-layer overlap on contrail radiative forcing
Bias in CMIP6 models as compared to observed regional dimming and brightening
A test of the ability of current bulk optical models to represent the radiative properties of cirrus cloud across the mid- and far-infrared
The incorporation of the Tripleclouds concept into the δ-Eddington two-stream radiation scheme: solver characterization and its application to shallow cumulus clouds
Radiative heating rate profiles over the southeast Atlantic Ocean during the 2016 and 2017 biomass burning seasons
Effective radiative forcing and adjustments in CMIP6 models
Response of surface shortwave cloud radiative effect to greenhouse gases and aerosols and its impact on summer maximum temperature
Combining atmospheric and snow radiative transfer models to assess the solar radiative effects of black carbon in the Arctic
Accurate 3-D radiative transfer simulation of spectral solar irradiance during the total solar eclipse of 21 August 2017
Quantifying the bias of radiative heating rates in numerical weather prediction models for shallow cumulus clouds
The climate effects of increasing ocean albedo: an idealized representation of solar geoengineering
Changes in clouds and thermodynamics under solar geoengineering and implications for required solar reduction
Radiative impact of an extreme Arctic biomass-burning event
Contrails and their impact on shortwave radiation and photovoltaic power production – a regional model study
The influence of internal variability on Earth's energy balance framework and implications for estimating climate sensitivity
Insights into the diurnal cycle of global Earth outgoing radiation using a numerical weather prediction model
Determining the infrared radiative effects of Saharan dust: a radiative transfer modelling study based on vertically resolved measurements at Lampedusa
The early summertime Saharan heat low: sensitivity of the radiation budget and atmospheric heating to water vapour and dust aerosol
Tao Shi, Yuanjian Yang, Lian Zong, Min Guo, Ping Qi, and Simone Lolli
Atmos. Chem. Phys., 25, 4989–5007, https://doi.org/10.5194/acp-25-4989-2025, https://doi.org/10.5194/acp-25-4989-2025, 2025
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Our study explored the daily temperature patterns in urban areas of the Yangtze River Delta, focusing on how weather and human activities impact these patterns. We found that temperatures were higher at night, and weather patterns had a bigger impact during the day, while human activities mattered more at night. This helps us understand and address urban overheating.
Wouter Mol and Chiel van Heerwaarden
Atmos. Chem. Phys., 25, 4419–4441, https://doi.org/10.5194/acp-25-4419-2025, https://doi.org/10.5194/acp-25-4419-2025, 2025
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Sunlight varies often and quickly under broken cloud cover, and every cloud field creates a unique pattern of sunlight on the surface below. These variations affect many processes in the Earth system, from photosynthesis and chemistry to cloud formation itself. The exact way in which cloud particles interact with sunlight is complex and expensive to calculate. We demonstrate a simplified framework which explains how sunlight changes for potentially any cloud field.
María-Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Michaël Sicard, Jesús Abril-Gago, Vanda Salgueiro, Adolfo Comerón, María José Granados-Muñoz, Maria João Costa, Constantino Muñoz-Porcar, Juan Antonio Bravo-Aranda, Daniele Bortoli, Alejandro Rodríguez-Gómez, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 25, 3213–3231, https://doi.org/10.5194/acp-25-3213-2025, https://doi.org/10.5194/acp-25-3213-2025, 2025
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Due to the significant radiative role of dust in climate change, vertical assessments of the short-wave dust direct radiative effect of both fine and coarse dust particles are performed separately. The study is focused on an intense Saharan dust outbreak crossing the Iberian Peninsula in springtime monitored by five Iberian lidar stations with southwest–northeast coverage. A comparative study to evaluate the differences found by considering the total dust (no separation) is also examined.
Jan-Lukas Tirpitz, Santo Fedele Colosimo, Nathaniel Brockway, Robert Spurr, Matt Christi, Samuel Hall, Kirk Ullmann, Johnathan Hair, Taylor Shingler, Rodney Weber, Jack Dibb, Richard Moore, Elizabeth Wiggins, Vijay Natraj, Nicolas Theys, and Jochen Stutz
Atmos. Chem. Phys., 25, 1989–2015, https://doi.org/10.5194/acp-25-1989-2025, https://doi.org/10.5194/acp-25-1989-2025, 2025
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We combine plume composition data from the 2019 NASA FIREX-AQ campaign with state-of-the-art radiative transfer modeling techniques to calculate distributions of actinic flux and photolysis frequencies in a wildfire plume. Excellent agreement of the model and observations demonstrates the applicability of this approach to constrain photochemistry in such plumes. We identify limiting factors for the modeling accuracy and discuss spatial and spectral features of the distributions.
Gabriel Chesnoiu, Isabelle Chiapello, Nicolas Ferlay, Pierre Nabat, Marc Mallet, and Véronique Riffault
Atmos. Chem. Phys., 25, 1307–1331, https://doi.org/10.5194/acp-25-1307-2025, https://doi.org/10.5194/acp-25-1307-2025, 2025
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The ALADIN regional climate model at 12.5 km resolution allows us to study the evolution of surface solar radiation (SSR) and key associated atmospheric parameters. Over northern France and Benelux, influenced by anthropogenic aerosols and cloudy conditions, regional evaluation of recent hindcast simulations shows satisfying results and high spatial variability. Future SSR evolution by the end of the century for two contrasting CMIP6 scenarios highlights large decreases in SSR for SSP3-7.0.
Zilu Zhang, Libo Zhou, and Meigen Zhang
Atmos. Chem. Phys., 25, 1–25, https://doi.org/10.5194/acp-25-1-2025, https://doi.org/10.5194/acp-25-1-2025, 2025
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By integrating the SNICAR model with Polar-WRF, we find that 50 ng g−1 black carbon (BC) deposition decreases snow albedo, increasing radiative forcing (RF) by 1–4 W m−2, especially in Greenland, Baffin Island, and eastern Siberia. The impact is strongly linked to BC mass, with deep snowpacks showing greater sensitivity. Snowmelt and land–atmosphere interactions are crucial. High-resolution modelling is necessary to better understand these effects on Arctic climate change.
Jeonggyu Kim, Sungmin Park, Greg M. McFarquhar, Anthony J. Baran, Joo Wan Cha, Kyoungmi Lee, Seoung Soo Lee, Chang Hoon Jung, Kyo-Sun Sunny Lim, and Junshik Um
Atmos. Chem. Phys., 24, 12707–12726, https://doi.org/10.5194/acp-24-12707-2024, https://doi.org/10.5194/acp-24-12707-2024, 2024
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We developed idealized models to represent the shapes of ice particles found in deep convective clouds and calculated their single-scattering properties. By comparing these results with in situ measurements, we discovered that a mixture of shape models matches in situ measurements more closely than single-form models or aggregate models. This finding has important implications for enhancing the simulation of single-scattering properties of ice crystals in deep convective clouds.
Ruby W. Burgess and Mayra I. Oyola-Merced
Atmos. Chem. Phys., 24, 12183–12201, https://doi.org/10.5194/acp-24-12183-2024, https://doi.org/10.5194/acp-24-12183-2024, 2024
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This study explores how aerosols affect atmospheric heating over African easterly waves (AEWs). Using data from NASA's aircraft and outputs of reanalysis models, the research focuses on days with both Saharan dust and AEWs. Using a radiative transfer model, the study reveals significant differences in heating rates, emphasizing challenges in accurately representing aerosol effects in the atmosphere and underscoring the need for improved aerosol representation in weather models.
Edgardo I. Sepulveda Araya, Sylvia C. Sullivan, and Aiko Voigt
EGUsphere, https://doi.org/10.5194/egusphere-2024-3212, https://doi.org/10.5194/egusphere-2024-3212, 2024
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Clouds composed of ice crystals are key when evaluating atmospheric radiation. The morphology of the crystals found in clouds is not clear yet, and even less clear is the impact on cloud heating rate, which is essential to describe precipitation and wind patterns. This motivated us to study how the heating rate behaves under a variety of ice complexity and environmental conditions, finding that increasing complexity in high and dense clouds weakens the heating rate.
Zili He, Quentin Libois, Najda Villefranque, Hartwig Deneke, Jonas Witthuhn, and Fleur Couvreux
Atmos. Chem. Phys., 24, 11391–11408, https://doi.org/10.5194/acp-24-11391-2024, https://doi.org/10.5194/acp-24-11391-2024, 2024
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This study uses observations and simulations to analyze how cumulus clouds affect spacial solar radiation variability on the ground. Results show that the simulations reproduce the observations well and improve understanding of cloud impacts on radiation. The research also indicates that a few strategically placed sensors, capitalizing on measurement timing, can effectively measure these variations, aiding in the development of detailed weather prediction models.
Mirjam Tijhuis, Bart J. H. van Stratum, and Chiel C. van Heerwaarden
Atmos. Chem. Phys., 24, 10567–10582, https://doi.org/10.5194/acp-24-10567-2024, https://doi.org/10.5194/acp-24-10567-2024, 2024
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Radiative transfer in the atmosphere is a 3D processes, which is often modelled in 1D for computational efficiency. We studied the differences between using 1D and 3D radiative transfer. With 3D radiation, larger clouds that contain more liquid water develop. However, they cover roughly the same part of the sky, and the average total radiation at the surface is nearly unchanged. The increase in cloud size might be important for weather models, as it can impact the formation of rain, for example.
Aiko Voigt, Stefanie North, Blaž Gasparini, and Seung-Hee Ham
Atmos. Chem. Phys., 24, 9749–9775, https://doi.org/10.5194/acp-24-9749-2024, https://doi.org/10.5194/acp-24-9749-2024, 2024
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Clouds shape weather and climate by interacting with photons, which changes temperatures within the atmosphere. We assess how well CMIP6 climate models capture this radiative heating by clouds within the atmosphere. While we find large differences among models, especially in cold regions of the atmosphere with abundant ice clouds, we also demonstrate that physical understanding allows us to predict the response of clouds and their radiative heating near the tropopause to climate change.
Qingmin Wang, Yincheng Liu, Lujun Zhang, and Chen Zhou
EGUsphere, https://doi.org/10.5194/egusphere-2024-2379, https://doi.org/10.5194/egusphere-2024-2379, 2024
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Our research explores how SST changes in non-polar regions impact the polar energy budget. Through idealized SST experiments, we found that warming in tropical and midlatitude oceans raises polar temperatures via enhanced atmospheric energy transport, leading to surface warming and top-of-atmosphere cooling in polar areas. This study highlights the distinct impacts of tropical Pacific and Indian Ocean SST changes on Arctic and Antarctic climates.
Lucas Ferreira Correa, Doris Folini, Boriana Chtirkova, and Martin Wild
Atmos. Chem. Phys., 24, 8797–8819, https://doi.org/10.5194/acp-24-8797-2024, https://doi.org/10.5194/acp-24-8797-2024, 2024
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We investigated the causes of the decadal trends of solar radiation measured at 34 stations in Brazil in the first 2 decades of the 21st century. We observed strong negative trends in north and northeast Brazil associated with changes in both atmospheric absorption (anthropogenic) and cloud cover (natural). In other parts of the country no strong trends were observed as a result of competing effects. This provides a better understanding of the energy balance in the region.
Ilias Fountoulakis, Alexandra Tsekeri, Stelios Kazadzis, Vassilis Amiridis, Angelos Nersesian, Maria Tsichla, Emmanouil Proestakis, Antonis Gkikas, Kyriakoula Papachristopoulou, Vasileios Barlakas, Claudia Emde, and Bernhard Mayer
Atmos. Chem. Phys., 24, 4915–4948, https://doi.org/10.5194/acp-24-4915-2024, https://doi.org/10.5194/acp-24-4915-2024, 2024
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In our study we provide an assessment, through a sensitivity study, of the limitations of models to calculate the dust direct radiative effect (DRE) due to the underrepresentation of its size, refractive index (RI), and shape. Our results indicate the necessity of including more realistic sizes and RIs for dust particles in dust models, in order to derive better estimations of the dust direct radiative effects.
Behrooz Keshtgar, Aiko Voigt, Bernhard Mayer, and Corinna Hoose
Atmos. Chem. Phys., 24, 4751–4769, https://doi.org/10.5194/acp-24-4751-2024, https://doi.org/10.5194/acp-24-4751-2024, 2024
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Cloud-radiative heating (CRH) affects extratropical cyclones but is uncertain in weather and climate models. We provide a framework to quantify uncertainties in CRH within an extratropical cyclone due to four factors and show that the parameterization of ice optical properties contributes significantly to uncertainty in CRH. We also argue that ice optical properties, by affecting CRH on spatial scales of 100 km, are relevant for the large-scale dynamics of extratropical cyclones.
Hanno Müller, André Ehrlich, Evelyn Jäkel, Johannes Röttenbacher, Benjamin Kirbus, Michael Schäfer, Robin J. Hogan, and Manfred Wendisch
Atmos. Chem. Phys., 24, 4157–4175, https://doi.org/10.5194/acp-24-4157-2024, https://doi.org/10.5194/acp-24-4157-2024, 2024
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A weather model is used to compare solar radiation with measurements from an aircraft campaign in the Arctic. Model and observations agree on the downward radiation but show differences in the radiation reflected by the surface and the clouds, which in the model is too low above sea ice and too high above open ocean. The model–observation bias is reduced above open ocean by a realistic fraction of clouds and less cloud liquid water and above sea ice by less dark sea ice and more cloud droplets.
Bjorn Stevens and Lukas Kluft
Atmos. Chem. Phys., 23, 14673–14689, https://doi.org/10.5194/acp-23-14673-2023, https://doi.org/10.5194/acp-23-14673-2023, 2023
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A simple model is introduced to account for the spectral diversity of radiant energy transfer. It provides an improved basis for assessing the different ways in which clouds influence Earth’s climate sensitivity, demonstrating how many cloud effects depend on the existing cloud climatology. Given existing assessments of changes in cloud albedo with warming, it is determined that clouds reduce Earth's climate sensitivity as compared to what it would be in a counterfactual world without clouds.
Kevin Wolf, Nicolas Bellouin, and Olivier Boucher
Atmos. Chem. Phys., 23, 14003–14037, https://doi.org/10.5194/acp-23-14003-2023, https://doi.org/10.5194/acp-23-14003-2023, 2023
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Cirrus and contrails considerably impact Earth's energy budget. Such ice clouds can have a positive (warming) or negative (cooling) net radiative effect (RE), which depends on cloud and ambient properties. The effect of eight parameters on the cloud RE is estimated. In total, 283 500 radiative transfer simulations have been performed, spanning the typical parameter ranges associated with cirrus and contrails. Specific cases are selected and discussed. The data set is publicly available.
Adam C. Varble, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Shuaiqi Tang, and Jerome Fast
Atmos. Chem. Phys., 23, 13523–13553, https://doi.org/10.5194/acp-23-13523-2023, https://doi.org/10.5194/acp-23-13523-2023, 2023
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We evaluate how clouds change in response to changing atmospheric particle (aerosol) concentrations in a climate model and find that the model-predicted cloud brightness increases too much as aerosols increase because the cloud drop number increases too much. Excessive drizzle in the model mutes this difference. Many differences between observational and model estimates are explained by varying assumptions of how much liquid has been lost in clouds, which impacts the estimated cloud drop number.
Olivia Linke, Johannes Quaas, Finja Baumer, Sebastian Becker, Jan Chylik, Sandro Dahlke, André Ehrlich, Dörthe Handorf, Christoph Jacobi, Heike Kalesse-Los, Luca Lelli, Sina Mehrdad, Roel A. J. Neggers, Johannes Riebold, Pablo Saavedra Garfias, Niklas Schnierstein, Matthew D. Shupe, Chris Smith, Gunnar Spreen, Baptiste Verneuil, Kameswara S. Vinjamuri, Marco Vountas, and Manfred Wendisch
Atmos. Chem. Phys., 23, 9963–9992, https://doi.org/10.5194/acp-23-9963-2023, https://doi.org/10.5194/acp-23-9963-2023, 2023
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Lapse rate feedback (LRF) is a major driver of the Arctic amplification (AA) of climate change. It arises because the warming is stronger at the surface than aloft. Several processes can affect the LRF in the Arctic, such as the omnipresent temperature inversion. Here, we compare multimodel climate simulations to Arctic-based observations from a large research consortium to broaden our understanding of these processes, find synergy among them, and constrain the Arctic LRF and AA.
Mark D. Zelinka, Christopher J. Smith, Yi Qin, and Karl E. Taylor
Atmos. Chem. Phys., 23, 8879–8898, https://doi.org/10.5194/acp-23-8879-2023, https://doi.org/10.5194/acp-23-8879-2023, 2023
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The primary uncertainty in how strongly Earth's climate has been perturbed by human activities comes from the unknown radiative impact of aerosol changes. Accurately quantifying these forcings – and their sub-components – in climate models is crucial for understanding the past and future simulated climate. In this study we describe biases in previously published estimates of aerosol radiative forcing in climate models and provide corrected estimates along with code for users to compute them.
Tatiana Egorova, Jan Sedlacek, Timofei Sukhodolov, Arseniy Karagodin-Doyennel, Franziska Zilker, and Eugene Rozanov
Atmos. Chem. Phys., 23, 5135–5147, https://doi.org/10.5194/acp-23-5135-2023, https://doi.org/10.5194/acp-23-5135-2023, 2023
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This paper describes the climate and atmosphere benefits of the Montreal Protocol, simulated with the state-of-the-art Earth system model SOCOLv4.0. We have added to and confirmed the previous studies by showing that without the Montreal Protocol by the end of the 21st century there would be a dramatic reduction in the ozone layer as well as substantial perturbation of the essential climate variables in the troposphere caused by the warming from increasing ozone-depleting substances.
Daniele Visioni, Ben Kravitz, Alan Robock, Simone Tilmes, Jim Haywood, Olivier Boucher, Mark Lawrence, Peter Irvine, Ulrike Niemeier, Lili Xia, Gabriel Chiodo, Chris Lennard, Shingo Watanabe, John C. Moore, and Helene Muri
Atmos. Chem. Phys., 23, 5149–5176, https://doi.org/10.5194/acp-23-5149-2023, https://doi.org/10.5194/acp-23-5149-2023, 2023
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Geoengineering indicates methods aiming to reduce the temperature of the planet by means of reflecting back a part of the incoming radiation before it reaches the surface or allowing more of the planetary radiation to escape into space. It aims to produce modelling experiments that are easy to reproduce and compare with different climate models, in order to understand the potential impacts of these techniques. Here we assess its past successes and failures and talk about its future.
Yingfang Li, Zhili Wang, Yadong Lei, Huizheng Che, and Xiaoye Zhang
Atmos. Chem. Phys., 23, 2499–2523, https://doi.org/10.5194/acp-23-2499-2023, https://doi.org/10.5194/acp-23-2499-2023, 2023
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Since few studies have assessed the impacts of future combined reductions in aerosols, ozone, and their precursors on future climate change, we use models with an interactive representation of tropospheric aerosols and atmospheric chemistry schemes to quantify the impact of their reductions on the Asian climate. Our results suggest that their reductions will exacerbate the warming effect caused by greenhouse gases, increasing future climate extremes and associated population exposure risk.
Andreas Marsing, Ralf Meerkötter, Romy Heller, Stefan Kaufmann, Tina Jurkat-Witschas, Martina Krämer, Christian Rolf, and Christiane Voigt
Atmos. Chem. Phys., 23, 587–609, https://doi.org/10.5194/acp-23-587-2023, https://doi.org/10.5194/acp-23-587-2023, 2023
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We employ highly resolved aircraft measurements of profiles of the ice water content (IWC) in Arctic cirrus clouds in winter and spring, when solar irradiation is low. Using radiation transfer calculations, we assess the cloud radiative effect over different surfaces like snow or ocean. The variability in the IWC of the clouds affects their overall radiative effect and drives internal processes. This helps understand the role of cirrus in a rapidly changing Arctic environment.
John T. Fasullo and Jadwiga H. Richter
Atmos. Chem. Phys., 23, 163–182, https://doi.org/10.5194/acp-23-163-2023, https://doi.org/10.5194/acp-23-163-2023, 2023
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The continued high levels of anthropogenic greenhouse gas emissions increase the likelihood that key climate warming thresholds will be exceeded in the coming decades. Here we examine a recently proposed geoengineering approach using two recently produced climate model experiments. We find the associated latitudinal distribution of aerosol mass to exhibit substantial uncertainty, suggesting the need for significant flexibility in the location and amount of aerosol delivery, if implemented.
Youness El-Ouartassy, Irène Korsakissok, Matthieu Plu, Olivier Connan, Laurent Descamps, and Laure Raynaud
Atmos. Chem. Phys., 22, 15793–15816, https://doi.org/10.5194/acp-22-15793-2022, https://doi.org/10.5194/acp-22-15793-2022, 2022
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This work investigates the potential value of using fine-scale meteorological ensembles to represent the inherent meteorological uncertainties in atmospheric dispersion model outputs. Probabilistic scores were used to evaluate the probabilistic performance of dispersion ensembles, using an original dataset of new continuous 85Kr air concentration measurements and a well-known source term. The results show that the ensemble dispersion simulations perform better than deterministic ones.
Ilissa B. Ocko and Steven P. Hamburg
Atmos. Chem. Phys., 22, 9349–9368, https://doi.org/10.5194/acp-22-9349-2022, https://doi.org/10.5194/acp-22-9349-2022, 2022
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Hydrogen is considered a key strategy to decarbonize the global economy. However, hydrogen is also a short-lived indirect greenhouse gas that can easily leak into the atmosphere. Given that the climate impacts from hydrogen emissions are not well understood, especially in the near term, we assess impacts over all timescales for plausible emissions rates. We find that hydrogen leakage can cause more warming than widely perceived; thus, attention is needed to minimize emissions.
Dustin Francis Phillip Grogan, Cheng-Hsuan Lu, Shih-Wei Wei, and Sheng-Po Chen
Atmos. Chem. Phys., 22, 2385–2398, https://doi.org/10.5194/acp-22-2385-2022, https://doi.org/10.5194/acp-22-2385-2022, 2022
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This study shows that incorporating aerosols into satellite radiance calculations affects the representation of African easterly waves (AEWs), and their environment, over North Africa and the eastern Atlantic in a numerical weather model. These changes are driven by radiative effects of Saharan dust captured by the aerosol-affected radiances, which modify the initial fields and can improve the forecasting of AEWs.
Tao Tang, Drew Shindell, Yuqiang Zhang, Apostolos Voulgarakis, Jean-Francois Lamarque, Gunnar Myhre, Gregory Faluvegi, Bjørn H. Samset, Timothy Andrews, Dirk Olivié, Toshihiko Takemura, and Xuhui Lee
Atmos. Chem. Phys., 21, 13797–13809, https://doi.org/10.5194/acp-21-13797-2021, https://doi.org/10.5194/acp-21-13797-2021, 2021
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Previous studies showed that black carbon (BC) could warm the surface with decreased incoming radiation. With climate models, we found that the surface energy redistribution plays a more crucial role in surface temperature compared with other forcing agents. Though BC could reduce the surface heating, the energy dissipates less efficiently, which is manifested by reduced convective and evaporative cooling, thereby warming the surface.
Jiaojiao Liu and Xiangjun Shi
Atmos. Chem. Phys., 21, 10609–10624, https://doi.org/10.5194/acp-21-10609-2021, https://doi.org/10.5194/acp-21-10609-2021, 2021
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Cirrus thinning, which reduces the warming effect of cirrus clouds, has been investigated as a new geoengineering approach. In this study, a flexible seeding method is used to exploit the potential cooling effect of cirrus thinning. Simulation results show that the seeding method is essential for estimating the cooling effect. Cirrus thinning with the flexible seeding method could produce a considerable cooling effect, which is much stronger than the fixed seeding method.
Inés Sanz-Morère, Sebastian D. Eastham, Florian Allroggen, Raymond L. Speth, and Steven R. H. Barrett
Atmos. Chem. Phys., 21, 1649–1681, https://doi.org/10.5194/acp-21-1649-2021, https://doi.org/10.5194/acp-21-1649-2021, 2021
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Contrails cause ~50 % of aviation climate impacts, but this is highly uncertain. This is partly due to the effect of overlap between contrails and other cloud layers. We developed a model to quantify this effect, finding that overlap with natural clouds increased contrails' radiative forcing in 2015. This suggests that cloud avoidance may help in reducing aviation's climate impacts. We also find that contrail–contrail overlap reduces impacts by ~3 %, increasing non-linearly with optical depth.
Kine Onsum Moseid, Michael Schulz, Trude Storelvmo, Ingeborg Rian Julsrud, Dirk Olivié, Pierre Nabat, Martin Wild, Jason N. S. Cole, Toshihiko Takemura, Naga Oshima, Susanne E. Bauer, and Guillaume Gastineau
Atmos. Chem. Phys., 20, 16023–16040, https://doi.org/10.5194/acp-20-16023-2020, https://doi.org/10.5194/acp-20-16023-2020, 2020
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In this study we compare solar radiation at the surface from observations and Earth system models from 1961 to 2014. We find that the models do not reproduce the so-called
global dimmingas found in observations. Only model experiments with anthropogenic aerosol emissions display any dimming at all. The discrepancies between observations and models are largest in China, which we suggest is in part due to erroneous aerosol precursor emission inventories in the emission dataset used for CMIP6.
Richard J. Bantges, Helen E. Brindley, Jonathan E. Murray, Alan E. Last, Jacqueline E. Russell, Cathryn Fox, Stuart Fox, Chawn Harlow, Sebastian J. O'Shea, Keith N. Bower, Bryan A. Baum, Ping Yang, Hilke Oetjen, and Juliet C. Pickering
Atmos. Chem. Phys., 20, 12889–12903, https://doi.org/10.5194/acp-20-12889-2020, https://doi.org/10.5194/acp-20-12889-2020, 2020
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Understanding how ice clouds influence the Earth's energy balance remains a key challenge for predicting the future climate. These clouds are ubiquitous and are composed of ice crystals that have complex shapes that are incredibly difficult to model. This work exploits new measurements of the Earth's emitted thermal energy made from instruments flown on board an aircraft to test how well the latest ice cloud models can represent these clouds. Results indicate further developments are required.
Nina Črnivec and Bernhard Mayer
Atmos. Chem. Phys., 20, 10733–10755, https://doi.org/10.5194/acp-20-10733-2020, https://doi.org/10.5194/acp-20-10733-2020, 2020
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Unresolved interaction between clouds and atmospheric radiation is a source of uncertainty in weather and climate models. The present study highlights the potential of the state-of-the-art Tripleclouds radiative solver for shallow cumulus clouds, exposing the significance of properly representing subgrid cloud horizontal heterogeneity. The Tripleclouds concept was thereby incorporated in the widely employed δ-Eddington two-stream radiation scheme within the comprehensive libRadtran library.
Allison B. Marquardt Collow, Mark A. Miller, Lynne C. Trabachino, Michael P. Jensen, and Meng Wang
Atmos. Chem. Phys., 20, 10073–10090, https://doi.org/10.5194/acp-20-10073-2020, https://doi.org/10.5194/acp-20-10073-2020, 2020
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Uncertainties in marine boundary layer clouds arise in the presence of biomass burning aerosol, as is the case over the southeast Atlantic Ocean. Heating due to this aerosol has the potential to alter the thermodynamic profile as the aerosol is transported across the Atlantic Ocean. Radiation transfer experiments indicate local shortwave aerosol heating is ~2–8 K d−1; however uncertainties in this quantity exist due to the single-scattering albedo and back trajectories of the aerosol plume.
Christopher J. Smith, Ryan J. Kramer, Gunnar Myhre, Kari Alterskjær, William Collins, Adriana Sima, Olivier Boucher, Jean-Louis Dufresne, Pierre Nabat, Martine Michou, Seiji Yukimoto, Jason Cole, David Paynter, Hideo Shiogama, Fiona M. O'Connor, Eddy Robertson, Andy Wiltshire, Timothy Andrews, Cécile Hannay, Ron Miller, Larissa Nazarenko, Alf Kirkevåg, Dirk Olivié, Stephanie Fiedler, Anna Lewinschal, Chloe Mackallah, Martin Dix, Robert Pincus, and Piers M. Forster
Atmos. Chem. Phys., 20, 9591–9618, https://doi.org/10.5194/acp-20-9591-2020, https://doi.org/10.5194/acp-20-9591-2020, 2020
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The spread in effective radiative forcing for both CO2 and aerosols is narrower in the latest CMIP6 (Coupled Model Intercomparison Project) generation than in CMIP5. For the case of CO2 it is likely that model radiation parameterisations have improved. Tropospheric and stratospheric radiative adjustments to the forcing behave differently for different forcing agents, and there is still significant diversity in how clouds respond to forcings, particularly for total anthropogenic forcing.
Tao Tang, Drew Shindell, Yuqiang Zhang, Apostolos Voulgarakis, Jean-Francois Lamarque, Gunnar Myhre, Camilla W. Stjern, Gregory Faluvegi, and Bjørn H. Samset
Atmos. Chem. Phys., 20, 8251–8266, https://doi.org/10.5194/acp-20-8251-2020, https://doi.org/10.5194/acp-20-8251-2020, 2020
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By using climate simulations, we found that both CO2 and black carbon aerosols could reduce low-level cloud cover, which is mainly due to changes in relative humidity, cloud water, dynamics, and stability. Because the impact of cloud on solar radiation is in effect only during daytime, such cloud reduction could enhance solar heating, thereby raising the daily maximum temperature by 10–50 %, varying by region, which has great implications for extreme climate events and socioeconomic activity.
Tobias Donth, Evelyn Jäkel, André Ehrlich, Bernd Heinold, Jacob Schacht, Andreas Herber, Marco Zanatta, and Manfred Wendisch
Atmos. Chem. Phys., 20, 8139–8156, https://doi.org/10.5194/acp-20-8139-2020, https://doi.org/10.5194/acp-20-8139-2020, 2020
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Solar radiative effects of Arctic black carbon (BC) particles (suspended in the atmosphere and in the surface snowpack) were quantified under cloudless and cloudy conditions. An atmospheric and a snow radiative transfer model were coupled to account for radiative interactions between both compartments. It was found that (i) the warming effect of BC in the snowpack overcompensates for the atmospheric BC cooling effect, and (ii) clouds tend to reduce the atmospheric BC cooling and snow BC warming.
Paul Ockenfuß, Claudia Emde, Bernhard Mayer, and Germar Bernhard
Atmos. Chem. Phys., 20, 1961–1976, https://doi.org/10.5194/acp-20-1961-2020, https://doi.org/10.5194/acp-20-1961-2020, 2020
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We model solar radiation as it would be measured on the Earth's surface in the core shadow of a total solar eclipse. Subsequently, we compare our results to observations during the total eclipse 2017 for ultraviolet, visible and near-infrared wavelengths. Moreover, we analyze the effect of the surface reflectance, the ozone profile, aerosol and the topography and give a visualization of the prevailing photons paths in the atmosphere during the eclipse.
Nina Črnivec and Bernhard Mayer
Atmos. Chem. Phys., 19, 8083–8100, https://doi.org/10.5194/acp-19-8083-2019, https://doi.org/10.5194/acp-19-8083-2019, 2019
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The interaction between radiation and clouds represents a source of uncertainty in numerical weather prediction (NWP), due to both intrinsic problems of one-dimensional radiation schemes and poor representation of clouds. The underlying question addressed in this study is how large the bias is of radiative heating rates in NWP models for shallow cumulus clouds and how it scales with various parameters, such as solar zenith angle, surface albedo, cloud cover and liquid water path.
Ben Kravitz, Philip J. Rasch, Hailong Wang, Alan Robock, Corey Gabriel, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Duoying Ji, Andy Jones, Andrew Lenton, John C. Moore, Helene Muri, Ulrike Niemeier, Steven Phipps, Hauke Schmidt, Shingo Watanabe, Shuting Yang, and Jin-Ho Yoon
Atmos. Chem. Phys., 18, 13097–13113, https://doi.org/10.5194/acp-18-13097-2018, https://doi.org/10.5194/acp-18-13097-2018, 2018
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Marine cloud brightening has been proposed as a means of geoengineering/climate intervention, or deliberately altering the climate system to offset anthropogenic climate change. In idealized simulations that highlight contrasts between land and ocean, we find that the globe warms, including the ocean due to transport of heat from land. This study reinforces that no net energy input into the Earth system does not mean that temperature will necessarily remain unchanged.
Rick D. Russotto and Thomas P. Ackerman
Atmos. Chem. Phys., 18, 11905–11925, https://doi.org/10.5194/acp-18-11905-2018, https://doi.org/10.5194/acp-18-11905-2018, 2018
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In simulations with different climate models in which the strength of the Sun is reduced to cancel the surface warming from a quadrupling of atmospheric carbon dioxide, low cloud cover decreases, high cloud cover increases, the upper troposphere and stratosphere cool, and water vapor concentration decreases. The stratospheric cooling and low cloud reduction result in more sunlight reduction being needed than originally thought.
Justyna Lisok, Anna Rozwadowska, Jesper G. Pedersen, Krzysztof M. Markowicz, Christoph Ritter, Jacek W. Kaminski, Joanna Struzewska, Mauro Mazzola, Roberto Udisti, Silvia Becagli, and Izabela Gorecka
Atmos. Chem. Phys., 18, 8829–8848, https://doi.org/10.5194/acp-18-8829-2018, https://doi.org/10.5194/acp-18-8829-2018, 2018
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The aim of the presented study was to investigate the impact on the radiation budget and atmospheric dynamics of a biomass-burning plume, transported from Alaska to the High Arctic region of Ny-Ålesund, Svalbard, in early July 2015. We found that the smoke plume may significantly alter radiative properties of the atmosphere. Furthermore, the simulations of atmospheric dynamics indicated a vertical positive displacement and broadening of the plume with time.
Simon Gruber, Simon Unterstrasser, Jan Bechtold, Heike Vogel, Martin Jung, Henry Pak, and Bernhard Vogel
Atmos. Chem. Phys., 18, 6393–6411, https://doi.org/10.5194/acp-18-6393-2018, https://doi.org/10.5194/acp-18-6393-2018, 2018
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A numerical model also used for operational weather forecast was applied to investigate the impact of contrails and contrail cirrus on the radiative fluxes at the earth's surface. Accounting for contrails produced by aircraft enables the model to simulate high clouds that are otherwise missing. In a case study, we find that the effect of these extra clouds is to reduce the incoming shortwave radiation at the surface as well as the production of photovoltaic power by up to 10 %.
Andrew E. Dessler, Thorsten Mauritsen, and Bjorn Stevens
Atmos. Chem. Phys., 18, 5147–5155, https://doi.org/10.5194/acp-18-5147-2018, https://doi.org/10.5194/acp-18-5147-2018, 2018
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One of the most important parameters in climate science is the equilibrium climate sensitivity (ECS). Estimates of this quantity based on 20th-century observations suggest low values of ECS (below 2 °C). We show that these calculations may be significantly in error. Together with other recent work on this problem, it seems probable that the ECS is larger than suggested by the 20th-century observations.
Jake J. Gristey, J. Christine Chiu, Robert J. Gurney, Cyril J. Morcrette, Peter G. Hill, Jacqueline E. Russell, and Helen E. Brindley
Atmos. Chem. Phys., 18, 5129–5145, https://doi.org/10.5194/acp-18-5129-2018, https://doi.org/10.5194/acp-18-5129-2018, 2018
Daniela Meloni, Alcide di Sarra, Gérard Brogniez, Cyrielle Denjean, Lorenzo De Silvestri, Tatiana Di Iorio, Paola Formenti, José L. Gómez-Amo, Julian Gröbner, Natalia Kouremeti, Giuliano Liuzzi, Marc Mallet, Giandomenico Pace, and Damiano M. Sferlazzo
Atmos. Chem. Phys., 18, 4377–4401, https://doi.org/10.5194/acp-18-4377-2018, https://doi.org/10.5194/acp-18-4377-2018, 2018
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This study examines how different aerosol optical properties determine the dust longwave radiative effects at the surface, in the atmosphere and at the top of the atmosphere, based on the combination of remote sensing and in situ observations from the ground, from airborne sensors, and from space, by means of radiative transfer modelling. The closure experiment is based on longwave irradiances and spectral brightness temperatures measured during the 2013 ChArMEx–ADRIMED campaign at Lampedusa.
Netsanet K. Alamirew, Martin C. Todd, Claire L. Ryder, John H. Marsham, and Yi Wang
Atmos. Chem. Phys., 18, 1241–1262, https://doi.org/10.5194/acp-18-1241-2018, https://doi.org/10.5194/acp-18-1241-2018, 2018
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This paper quantifies the radiative effects of dust and water vapour in the Saharan heat low. Dust has a warming effect at the top of the atmosphere while cooling the surface. Water vapour has a warming effect both at the top of atmosphere and the surface. We find dust and water vapour have similar effects in driving the variability in the top-of-atmosphere radiative budget, while dust has a stronger effect than water vapour in controlling day-to-day variability of the surface radiative budget.
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Short summary
The measured ground-based surface solar irradiance variability and its sensitivity to scene parameters are analysed with a filtering of sky conditions at a given site. Its multivariate analysis is applied to observed trends over 2010–2022. The recorded values show, in addition to the dominant effects of cloud occurrence, the variable effects of aerosol and geometry. Clear-sun-with-cloud situations are highlighted by SSI levels close to those of aerosol- and cloud-free situations.
The measured ground-based surface solar irradiance variability and its sensitivity to scene...
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