Articles | Volume 23, issue 8
https://doi.org/10.5194/acp-23-4663-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-4663-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Measurement report
| 
20 Apr 2023
Measurement report |
| 20 Apr 2023
| 20 Apr 2023
Measurement report: Summertime fluorescence characteristics of atmospheric water-soluble organic carbon in the marine boundary layer of the western Arctic Ocean
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Yuzo Miyazaki
Institute of Low Temperature Science, Hokkaido University, Sapporo
060-0819, Japan
Jin Hur
Department of Environment & Energy, Sejong University, 209
Neungdong-ro, Gwangjin-gu, Seoul 05006, Republic of Korea
Yun Kyung Lee
Department of Environment & Energy, Sejong University, 209
Neungdong-ro, Gwangjin-gu, Seoul 05006, Republic of Korea
Mi Hae Jeon
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Youngju Lee
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Kyoung-Ho Cho
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Hyun Young Chung
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Department of Polar Sciences, University of Science and Technology,
Incheon 21990, Republic of Korea
Kitae Kim
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Department of Polar Sciences, University of Science and Technology,
Incheon 21990, Republic of Korea
Jung-Ok Choi
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Catherine Lalande
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Joo-Hong Kim
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Taejin Choi
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Young Jun Yoon
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Eun Jin Yang
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Sung-Ho Kang
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon
21990, Republic of Korea
Related authors
Igor V. Polyakov, Andrey V. Pnyushkov, Eddy C. Carmack, Matthew Charette, Kyoung-Ho Cho, Steven Dykstra, Jari Haapala, Jinyoung Jung, Lauren Kipp, and Eun Jin Yang
EGUsphere, https://doi.org/10.5194/egusphere-2025-2316, https://doi.org/10.5194/egusphere-2025-2316, 2025
Short summary
Short summary
The Siberian Arctic Ocean greatly influences the Arctic climate system. Moreover, the region is experiencing some of the most notable Arctic climate change. In the summer, strong near-inertial currents in the upper (<30m) ocean account for more than half of the current speed and shear. In the winter, upper ocean ventilation due to atlantification distributes wind energy to far deeper (>100m) layers. Understanding the implications for mixing and halocline weakening depends on these findings.
Charlotte Eich, Mathijs van Manen, J. Scott P. McCain, Loay J. Jabre, Willem H. van de Poll, Jinyoung Jung, Sven B. E. H. Pont, Hung-An Tian, Indah Ardiningsih, Gert-Jan Reichart, Erin M. Bertrand, Corina P. D. Brussaard, and Rob Middag
Biogeosciences, 21, 4637–4663, https://doi.org/10.5194/bg-21-4637-2024, https://doi.org/10.5194/bg-21-4637-2024, 2024
Short summary
Short summary
Phytoplankton growth in the Southern Ocean (SO) is often limited by low iron (Fe) concentrations. Sea surface warming impacts Fe availability and can affect phytoplankton growth. We used shipboard Fe clean incubations to test how changes in Fe and temperature affect SO phytoplankton. Their abundances usually increased with Fe addition and temperature increase, with Fe being the major factor. These findings imply potential shifts in ecosystem structure, impacting food webs and elemental cycling.
Yange Deng, Hiroshi Tanimoto, Kohei Ikeda, Sohiko Kameyama, Sachiko Okamoto, Jinyoung Jung, Young Jun Yoon, Eun Jin Yang, and Sung-Ho Kang
Atmos. Chem. Phys., 24, 6339–6357, https://doi.org/10.5194/acp-24-6339-2024, https://doi.org/10.5194/acp-24-6339-2024, 2024
Short summary
Short summary
Black carbon (BC) aerosols play important roles in Arctic climate change, yet they are not well understood because of limited observational data. We observed BC mass concentrations (mBC) in the western Arctic Ocean during summer and early autumn 2016–2020. The mean mBC in 2019 was much higher than in other years. Biomass burning was likely the dominant BC source. Boreal fire BC transport occurring near the surface and/or in the mid-troposphere contributed to high-BC events in the Arctic Ocean.
Riku Miyase, Yuzo Miyazaki, Tomohisa Irino, and Youhei Yamashita
EGUsphere, https://doi.org/10.5194/egusphere-2025-2525, https://doi.org/10.5194/egusphere-2025-2525, 2025
Short summary
Short summary
Water-soluble pyrogenic carbon (WSPyC) is long-lived in the ocean and plays a role in regulating climate. This study observed the variations in concentration and sources of WSPyC in atmospheric aerosols. The results suggest that WSPyC can form through the oxidation of soot during atmospheric transport, highlighting this process as an important pathway before aerosols are deposited into the ocean.
Yuzo Miyazaki, Yunhan Wang, Eri Tachibana, Koji Suzuki, Youhei Yamashita, and Jun Nishioka
EGUsphere, https://doi.org/10.5194/egusphere-2025-2689, https://doi.org/10.5194/egusphere-2025-2689, 2025
Short summary
Short summary
It is essential to understand how biologically productive oceanic regions during spring phytoplankton blooms after sea ice melting contribute to the sea-to-air emission flux of atmospheric organic aerosols (OAs) in the subarctic oceans. Our shipboard measurements highlight the preferential formation of N-containing secondary water-soluble OAs associated with the predominant diatoms including ice algae during the bloom after sea ice melting/retreat in the subarctic ocean.
Shao-Min Chen, Thibaud Dezutter, David Cote, Catherine Lalande, Evan Edinger, and Owen A. Sherwood
Biogeosciences, 22, 2517–2540, https://doi.org/10.5194/bg-22-2517-2025, https://doi.org/10.5194/bg-22-2517-2025, 2025
Short summary
Short summary
The origins and composition of sinking organic matter are still understudied for the oceans, especially in ice-covered areas. We use amino acid stable isotopes combined with particle flux and plankton taxonomy to investigate the sources and composition of exported organic matter from a sediment-trap-derived time series of sinking particles in the northwestern Labrador Sea. We found that sea-ice algae and fecal pellets may be important contributors to the sinking fluxes of carbon and nitrogen.
Igor V. Polyakov, Andrey V. Pnyushkov, Eddy C. Carmack, Matthew Charette, Kyoung-Ho Cho, Steven Dykstra, Jari Haapala, Jinyoung Jung, Lauren Kipp, and Eun Jin Yang
EGUsphere, https://doi.org/10.5194/egusphere-2025-2316, https://doi.org/10.5194/egusphere-2025-2316, 2025
Short summary
Short summary
The Siberian Arctic Ocean greatly influences the Arctic climate system. Moreover, the region is experiencing some of the most notable Arctic climate change. In the summer, strong near-inertial currents in the upper (<30m) ocean account for more than half of the current speed and shear. In the winter, upper ocean ventilation due to atlantification distributes wind energy to far deeper (>100m) layers. Understanding the implications for mixing and halocline weakening depends on these findings.
Dominic Heslin-Rees, Peter Tunved, Diego Aliaga, Janne Lampilahti, Ilona Riipinen, Annica Ekman, Ki-Tae Park, Martina Mazzini, Stefania Gilardoni, Roseline Thakur, Kihong Park, Young Jun Yoon, Kitack Lee, Mikko Sipilä, Mauro Mazzola, and Radovan Krejci
Aerosol Research Discuss., https://doi.org/10.5194/ar-2025-11, https://doi.org/10.5194/ar-2025-11, 2025
Revised manuscript has not been submitted
Short summary
Short summary
New particles form in the atmosphere and can influence the climate. We studied Arctic new particle formation (NPF) from 2022 to 2024 at the Zeppelin Observatory, on Svalbard. NPF occurs from April to November, peaking in late spring as sunlight increases. Some particles measured on-site grow large enough to seed clouds. Sunlight and existing aerosol particles strongly impact the likelihood of NPF, which mainly originates from marine regions, particularly the Greenland Sea.
James Brean, David C. S. Beddows, Eija Asmi, Aki Virkkula, Lauriane L. J. Quéléver, Mikko Sipilä, Floortje Van Den Heuvel, Thomas Lachlan-Cope, Anna Jones, Markus Frey, Angelo Lupi, Jiyeon Park, Young Jun Yoon, Rolf Weller, Giselle L. Marincovich, Gabriela C. Mulena, Roy M. Harrison, and Manuel Dall'Osto
Atmos. Chem. Phys., 25, 1145–1162, https://doi.org/10.5194/acp-25-1145-2025, https://doi.org/10.5194/acp-25-1145-2025, 2025
Short summary
Short summary
Our results emphasise how understanding the geographical variation in surface types across the Antarctic is key to understanding secondary aerosol sources.
Hee-Sung Jung, Sang-Moo Lee, Joo-Hong Kim, and Kyungsoo Lee
Earth Syst. Sci. Data, 17, 233–258, https://doi.org/10.5194/essd-17-233-2025, https://doi.org/10.5194/essd-17-233-2025, 2025
Short summary
Short summary
This dataset consists of reference sea ice concentration (SIC) data records over the Arctic Ocean, which were derived from the 30 m resolution imagery from the Operational Land Imager (OLI) on board Landsat-8. Each SIC map is given in a 6.25 km polar stereographic grid and is catalogued into one of the 12 regions of the Arctic Ocean. This dataset was produced to be used as a reference in the validation of various SIC products.
Seoung Soo Lee, Chang Hoon Jung, Jinho Choi, Young Jun Yoon, Junshik Um, Youtong Zheng, Jianping Guo, Manguttathil G. Manoj, Sang-Keun Song, and Kyung-Ja Ha
Atmos. Chem. Phys., 25, 705–726, https://doi.org/10.5194/acp-25-705-2025, https://doi.org/10.5194/acp-25-705-2025, 2025
Short summary
Short summary
This study attempts to test a general factor that explains differences in the properties of different mixed-phase clouds using a modeling tool. Although this attempt is not to identify a factor that can perfectly explain and represent the properties of different mixed-phase clouds, we believe that this attempt acts as a valuable stepping stone towards a more complete, general way of using climate models to better predict climate change.
Charlotte Eich, Mathijs van Manen, J. Scott P. McCain, Loay J. Jabre, Willem H. van de Poll, Jinyoung Jung, Sven B. E. H. Pont, Hung-An Tian, Indah Ardiningsih, Gert-Jan Reichart, Erin M. Bertrand, Corina P. D. Brussaard, and Rob Middag
Biogeosciences, 21, 4637–4663, https://doi.org/10.5194/bg-21-4637-2024, https://doi.org/10.5194/bg-21-4637-2024, 2024
Short summary
Short summary
Phytoplankton growth in the Southern Ocean (SO) is often limited by low iron (Fe) concentrations. Sea surface warming impacts Fe availability and can affect phytoplankton growth. We used shipboard Fe clean incubations to test how changes in Fe and temperature affect SO phytoplankton. Their abundances usually increased with Fe addition and temperature increase, with Fe being the major factor. These findings imply potential shifts in ecosystem structure, impacting food webs and elemental cycling.
Jiao Xue, Tian Zhang, Keyhong Park, Jinpei Yan, Young Jun Yoon, Jiyeon Park, and Bingbing Wang
Atmos. Chem. Phys., 24, 7731–7754, https://doi.org/10.5194/acp-24-7731-2024, https://doi.org/10.5194/acp-24-7731-2024, 2024
Short summary
Short summary
Ice formation by particles is an important way of making mixed-phase and ice clouds. We found that particles collected in the marine atmosphere exhibit diverse ice nucleation abilities and mixing states. Sea salt mixed-sulfate particles were enriched in ice-nucleating particles. Selective aging on sea salt particles made particle populations more externally mixed. Characterizations of particles and their mixing state are needed for a better understanding of aerosol–cloud interactions.
Yange Deng, Hiroshi Tanimoto, Kohei Ikeda, Sohiko Kameyama, Sachiko Okamoto, Jinyoung Jung, Young Jun Yoon, Eun Jin Yang, and Sung-Ho Kang
Atmos. Chem. Phys., 24, 6339–6357, https://doi.org/10.5194/acp-24-6339-2024, https://doi.org/10.5194/acp-24-6339-2024, 2024
Short summary
Short summary
Black carbon (BC) aerosols play important roles in Arctic climate change, yet they are not well understood because of limited observational data. We observed BC mass concentrations (mBC) in the western Arctic Ocean during summer and early autumn 2016–2020. The mean mBC in 2019 was much higher than in other years. Biomass burning was likely the dominant BC source. Boreal fire BC transport occurring near the surface and/or in the mid-troposphere contributed to high-BC events in the Arctic Ocean.
Hannah Sharpe, Michel Gosselin, Catherine Lalande, Alexandre Normandeau, Jean-Carlos Montero-Serrano, Khouloud Baccara, Daniel Bourgault, Owen Sherwood, and Audrey Limoges
Biogeosciences, 20, 4981–5001, https://doi.org/10.5194/bg-20-4981-2023, https://doi.org/10.5194/bg-20-4981-2023, 2023
Short summary
Short summary
We studied the impact of submarine canyon processes within the Pointe-des-Monts system on biogenic matter export and phytoplankton assemblages. Using data from three oceanographic moorings, we show that the canyon experienced two low-amplitude sediment remobilization events in 2020–2021 that led to enhanced particle fluxes in the deep-water column layer > 2.6 km offshore. Sinking phytoplankton fluxes were lower near the canyon compared to background values from the lower St. Lawrence Estuary.
Yuhao Cui, Eri Tachibana, Kimitaka Kawamura, and Yuzo Miyazaki
Biogeosciences, 20, 4969–4980, https://doi.org/10.5194/bg-20-4969-2023, https://doi.org/10.5194/bg-20-4969-2023, 2023
Short summary
Short summary
Fatty alcohols (FAs) are major components of surface lipids in plant leaves and serve as surface-active aerosols. Our study on the aerosol size distributions in a forest suggests that secondary FAs (SFAs) originated from plant waxes and that leaf senescence status is likely an important factor controlling the size distribution of SFAs. This study provides new insights into the sources of primary biological aerosol particles (PBAPs) and their effects on the aerosol ice nucleation activity.
Jiyeon Park, Hyojin Kang, Yeontae Gim, Eunho Jang, Ki-Tae Park, Sangjong Park, Chang Hoon Jung, Darius Ceburnis, Colin O'Dowd, and Young Jun Yoon
Atmos. Chem. Phys., 23, 13625–13646, https://doi.org/10.5194/acp-23-13625-2023, https://doi.org/10.5194/acp-23-13625-2023, 2023
Short summary
Short summary
We measured the number size distribution of 2.5–300 nm particles and cloud condensation nuclei (CCN) number concentrations at King Sejong Station on the Antarctic Peninsula continuously from 1 January to 31 December 2018. During the pristine and clean periods, 97 new particle formation (NPF) events were detected. For 83 of these, CCN concentrations increased by 2 %–268 % (median 44 %) following 1 to 36 h (median 8 h) after NPF events.
Young-Chan Noh, Yonghan Choi, Hyo-Jong Song, Kevin Raeder, Joo-Hong Kim, and Youngchae Kwon
Geosci. Model Dev., 16, 5365–5382, https://doi.org/10.5194/gmd-16-5365-2023, https://doi.org/10.5194/gmd-16-5365-2023, 2023
Short summary
Short summary
This is the first attempt to assimilate the observations of microwave temperature sounders into the global climate forecast model in which the satellite observations have not been assimilated in the past. To do this, preprocessing schemes are developed to make the satellite observations suitable to be assimilated. In the assimilation experiments, the model analysis is significantly improved by assimilating the observations of microwave temperature sounders.
Tsukasa Dobashi, Yuzo Miyazaki, Eri Tachibana, Kazutaka Takahashi, Sachiko Horii, Fuminori Hashihama, Saori Yasui-Tamura, Yoko Iwamoto, Shu-Kuan Wong, and Koji Hamasaki
Biogeosciences, 20, 439–449, https://doi.org/10.5194/bg-20-439-2023, https://doi.org/10.5194/bg-20-439-2023, 2023
Short summary
Short summary
Water-soluble organic nitrogen (WSON) in marine aerosols is important for biogeochemical cycling of bioelements. Our shipboard measurements suggested that reactive nitrogen produced and exuded by nitrogen-fixing microorganisms in surface seawater likely contributed to the formation of WSON aerosols in the subtropical North Pacific. This study provides new implications for the role of marine microbial activity in the formation of WSON aerosols in the ocean surface.
Yange Deng, Hiroaki Fujinari, Hikari Yai, Kojiro Shimada, Yuzo Miyazaki, Eri Tachibana, Dhananjay K. Deshmukh, Kimitaka Kawamura, Tomoki Nakayama, Shiori Tatsuta, Mingfu Cai, Hanbing Xu, Fei Li, Haobo Tan, Sho Ohata, Yutaka Kondo, Akinori Takami, Shiro Hatakeyama, and Michihiro Mochida
Atmos. Chem. Phys., 22, 5515–5533, https://doi.org/10.5194/acp-22-5515-2022, https://doi.org/10.5194/acp-22-5515-2022, 2022
Short summary
Short summary
Offline analyses of the hygroscopicity and composition of atmospheric aerosols are complementary to online analyses in view of the applicability to broader sizes, specific compound groups, and investigations at remote sites. This offline study characterized the composition of water-soluble matter in aerosols and their humidity-dependent hygroscopicity on Okinawa, a receptor site of East Asian outflow. Further, comparison with online analyses showed the appropriateness of the offline method.
Stephen M. Platt, Øystein Hov, Torunn Berg, Knut Breivik, Sabine Eckhardt, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Markus Fiebig, Rebecca Fisher, Georg Hansen, Hans-Christen Hansson, Jost Heintzenberg, Ove Hermansen, Dominic Heslin-Rees, Kim Holmén, Stephen Hudson, Roland Kallenborn, Radovan Krejci, Terje Krognes, Steinar Larssen, David Lowry, Cathrine Lund Myhre, Chris Lunder, Euan Nisbet, Pernilla B. Nizzetto, Ki-Tae Park, Christina A. Pedersen, Katrine Aspmo Pfaffhuber, Thomas Röckmann, Norbert Schmidbauer, Sverre Solberg, Andreas Stohl, Johan Ström, Tove Svendby, Peter Tunved, Kjersti Tørnkvist, Carina van der Veen, Stergios Vratolis, Young Jun Yoon, Karl Espen Yttri, Paul Zieger, Wenche Aas, and Kjetil Tørseth
Atmos. Chem. Phys., 22, 3321–3369, https://doi.org/10.5194/acp-22-3321-2022, https://doi.org/10.5194/acp-22-3321-2022, 2022
Short summary
Short summary
Here we detail the history of the Zeppelin Observatory, a unique global background site and one of only a few in the high Arctic. We present long-term time series of up to 30 years of atmospheric components and atmospheric transport phenomena. Many of these time series are important to our understanding of Arctic and global atmospheric composition change. Finally, we discuss the future of the Zeppelin Observatory and emerging areas of future research on the Arctic atmosphere.
Sharmine Akter Simu, Yuzo Miyazaki, Eri Tachibana, Henning Finkenzeller, Jérôme Brioude, Aurélie Colomb, Olivier Magand, Bert Verreyken, Stephanie Evan, Rainer Volkamer, and Trissevgeni Stavrakou
Atmos. Chem. Phys., 21, 17017–17029, https://doi.org/10.5194/acp-21-17017-2021, https://doi.org/10.5194/acp-21-17017-2021, 2021
Short summary
Short summary
The tropical Indian Ocean (IO) is expected to be a significant source of water-soluble organic carbon (WSOC), which is relevant to cloud formation. Our study showed that marine secondary organic formation dominantly contributed to the aerosol WSOC mass at the high-altitude observatory in the southwest IO in the wet season in both marine boundary layer and free troposphere (FT). This suggests that the effect of marine secondary sources is important up to FT, a process missing in climate models.
Sehyun Jang, Ki-Tae Park, Kitack Lee, Young Jun Yoon, Kitae Kim, Hyun Young Chung, Eunho Jang, Silvia Becagli, Bang Yong Lee, Rita Traversi, Konstantinos Eleftheriadis, Radovan Krejci, and Ove Hermansen
Atmos. Chem. Phys., 21, 9761–9777, https://doi.org/10.5194/acp-21-9761-2021, https://doi.org/10.5194/acp-21-9761-2021, 2021
Short summary
Short summary
This study provides comprehensive datasets encompassing seasonal and interannual variations in sulfate and MSA concentration in aerosol particles in the Arctic atmosphere. As oxidation products of DMS have important roles in new particle formation and growth, we focused on factors affecting their variability and the branching ratio of DMS oxidation. We found a strong correlation between the ratio and the light condition, chemical properties of particles, and biological activities near Svalbard.
Haebum Lee, Kwangyul Lee, Chris Rene Lunder, Radovan Krejci, Wenche Aas, Jiyeon Park, Ki-Tae Park, Bang Yong Lee, Young Jun Yoon, and Kihong Park
Atmos. Chem. Phys., 20, 13425–13441, https://doi.org/10.5194/acp-20-13425-2020, https://doi.org/10.5194/acp-20-13425-2020, 2020
Short summary
Short summary
New particle formation (NPF) contributes to enhance the number of particles in the ambient atmosphere, affecting local air quality and cloud condensation nuclei (CCN) concentration. This study investigated NPF characteristics in the Arctic and showed that although formation and growth rates of nanoparticles were much lower than those in continental areas, NPF occurrence frequency was comparable and marine biogenic sources played important roles in production of condensing vapors for NPF.
Cited articles
Abbatt, J. P. D., Leaitch, W. R., Aliabadi, A. A., Bertram, A. K., Blanchet, J.-P., Boivin-Rioux, A., Bozem, H., Burkart, J., Chang, R. Y. W., Charette, J., Chaubey, J. P., Christensen, R. J., Cirisan, A., Collins, D. B., Croft, B., Dionne, J., Evans, G. J., Fletcher, C. G., Galí, M., Ghahreman, R., Girard, E., Gong, W., Gosselin, M., Gourdal, M., Hanna, S. J., Hayashida, H., Herber, A. B., Hesaraki, S., Hoor, P., Huang, L., Hussherr, R., Irish, V. E., Keita, S. A., Kodros, J. K., Köllner, F., Kolonjari, F., Kunkel, D., Ladino, L. A., Law, K., Levasseur, M., Libois, Q., Liggio, J., Lizotte, M., Macdonald, K. M., Mahmood, R., Martin, R. V., Mason, R. H., Miller, L. A., Moravek, A., Mortenson, E., Mungall, E. L., Murphy, J. G., Namazi, M., Norman, A.-L., O'Neill, N. T., Pierce, J. R., Russell, L. M., Schneider, J., Schulz, H., Sharma, S., Si, M., Staebler, R. M., Steiner, N. S., Thomas, J. L., von Salzen, K., Wentzell, J. J. B., Willis, M. D., Wentworth, G. R., Xu, J.-W., and Yakobi-Hancock, J. D.: Overview paper: New insights into aerosol and climate in the Arctic, Atmos. Chem. Phys., 19, 2527–2560, https://doi.org/10.5194/acp-19-2527-2019, 2019.
Andreae, M. O. and Crutzen, P. J.: Atmospheric aerosols: Biogeochemical
sources and role in atmospheric chemistry, Science, 276, 1052–1058,
https://doi.org/10.1126/science.276.5315.1052, 1997.
Ardyna, M. and Arrigo, K. R.: Phytoplankton dynamics in a changing Arctic
Ocean, Nat. Clim. Change, 10, 892–903,
https://doi.org/10.1038/s41558-020-0905-y, 2020.
Arrigo, K. R. and van Dijken, G. L.: Secular trends in Arctic Ocean net
primary production, J. Geophys. Res., 116, C09011,
https://doi.org/10.1029/2011JC007151, 2011.
Arrigo, K. R. and van Dijken, G. L.: Continued increases in Arctic Ocean
primary production, Prog. Oceanogr., 136, 60–70,
https://doi.org/10.1016/j.pocean.2015.05.002, 2015.
Arrigo, K. R., Lowry, K. E., and van Dijken, G. L.: Annual changes in sea
ice and phytoplankton in polynyas of the Amundsen Sea, Antarctica, Deep-Sea
Res. Part II, 71–76, 5–15, https://doi.org/10.1016/j.dsr2.2012.03.006,
2012.
Ayers, G. P., Ivey, J. P., and Gillett, R. W.: Coherence between seasonal
cycles of dimethyl sulphide, methanesulphonate and sulphate in marine air,
Nature, 349, 404–406, https://doi.org/10.1038/349404a0, 1991.
Ballinger, T. J., Overland, J. E., Wang, M., Bhatt, U. S., Hanna, E.,
Hanssen-Bauer, I., Kim, S. -J., Thomas, R. L., and Walsh, J. E.: Surface air
temperature, NOAA Arctic Report Card 2020,
https://www.arctic.noaa.gov/Report-Card (last access: 21 May 2022), 2020.
Barsotti, F., Ghigo, G., and Vione, D.: Computational assessment of the
fluorescence emission of phenol oligomers: a possible insight into the
fluorescence properties of humic-like substances (HULIS), J. Photochem.
Photobiol., A 315, 87–93, https://doi.org/10.1016/j.jphotochem.2015.09.012,
2016.
Bates, T. S., Calhoun, J. A., and Quinn, P. K.: Variations in the
methanesulfonate to sulfate molar ratio in submicrometer marine aerosol
particles over the South Pacific Ocean, J. Geophys. Res., 97, 9859–9865,
https://doi.org/10.1029/92JD00411, 1992.
Beine, H., Anastasio, C., Domine, F., Douglas, T., Barret, M., France, J.,
King, M., Hall, S., and Ullmann, K.: Soluble chromophores in marine snow,
seawater, sea ice and frost flowers near Barrow, Alaska, J. Geophys. Res.,
117, D00R15, https://doi.org/10.1029/2011JD016650, 2012.
Beine, H. J., Dominè, F., Ianniello, A., Nardino, M., Allegrini, I., Teinilä, K., and Hillamo, R.: Fluxes of nitrates between snow surfaces and the atmosphere in the European high Arctic, Atmos. Chem. Phys., 3, 335–346, https://doi.org/10.5194/acp-3-335-2003, 2003.
Bergin, M. H., Jaffrezo, J. -L., Davidson, C. I., Dibb, J. E., Pandis, S.
N., Hillamo, R., Maenhaut, W., Kuhns, H. D., and Makela, T.: The
contributions of snow, fog, and dry deposition to the summer flux of anions
and cations at Summit, Greenland, J. Geophys. Res., 100, 16275–16288,
https://doi.org/10.1029/95JD01267, 1995.
Birdwell, J. E. and Engel, A. S.: Characterization of dissolved organic
matter in cave and spring waters using UV–vis absorbance and fluorescence
spectroscopy, Org. Geochem., 41, 270–280,
https://doi.org/10.1016/j.orggeochem.2009.11.002, 2010.
Blando, J. D. and Turpin, B. J.: Secondary organic aerosol formation in
cloud and fog droplets: a literature evaluation of plausibility, Atmos.
Environ., 34, 1623–1632, https://doi.org/10.1016/S1352-2310(99)00392-1,
2000.
Brogi, S. R., Jung, J. Y., Ha, S.-Y., and Hur, J.: Seasonal differences in
dissolved organic matter properties and sources in an Arctic fjord:
Implications for future conditions, Sci. Total Environ., 694, 133740,
https://doi.org/10.1016/j.scitotenv.2019.133740, 2019.
Burrows, S. M., Ogunro, O., Frossard, A. A., Russell, L. M., Rasch, P. J., and Elliott, S. M.: A physically based framework for modeling the organic fractionation of sea spray aerosol from bubble film Langmuir equilibria, Atmos. Chem. Phys., 14, 13601–13629, https://doi.org/10.5194/acp-14-13601-2014, 2014.
Cavalieri, D. J. and Parkinson, C. L.: Arctic sea ice variability and trends, 1979–2010, The Cryosphere, 6, 881–889, https://doi.org/10.5194/tc-6-881-2012, 2012.
Cavalli, F., Facchini, M. C., Decesari, S., Mircea, M., Emblico, L., Fuzzi,
S., Ceburnis, D., Yoon, Y. J., O'Dowd, C. D., Putaud, J. -P., and
Dell'Acqua, A.: Advances in characterization of size-resolved organic matter
in marine aerosol over the North Atlantic, J. Geophys. Res., 109, D24215,
https://doi.org/10.1029/2004JD005137, 2004.
Ceburnis, D., O'Dowd, C. D., Jennings, G. S., Facchini, M. C., Emblico, L.,
Decesari, S., Fuzzi, S., and Sakalys, J.: Marine aerosol chemistry
gradients: Elucidating primary and secondary processes and fluxes, Geophys.
Res. Lett., 35, L07804, https://doi.org/10.1029/2008GL033462, 2008.
Chang, R. Y.-W., Leck, C., Graus, M., Müller, M., Paatero, J., Burkhart, J. F., Stohl, A., Orr, L. H., Hayden, K., Li, S.-M., Hansel, A., Tjernström, M., Leaitch, W. R., and Abbatt, J. P. D.: Aerosol composition and sources in the central Arctic Ocean during ASCOS, Atmos. Chem. Phys., 11, 10619–10636, https://doi.org/10.5194/acp-11-10619-2011, 2011.
Chen, Q., Miyazaki, Y., Kawamura, K., Matsumoto, K., Coburn, S., Volkamer,
R., Iwamoto, Y., Kagami, S., Deng, Y., Ogawa, S., Ramasamy, S., Kato, S.,
Ida, A., Kajii, Y., and Mochida, M.: Characterization of chromophoric
water-soluble organic matter in urban, forest, and marine aerosols by
HR-ToF-AMS analysis and excitation–emission matrix spectroscopy, Environ.
Sci. Technol., 50, 10351–10360, https://doi.org/10.1021/acs.est.6b01643,
2016.
Chen, M., Jung, J., Lee, Y. K., and Hur, J.: Surface accumulation of low
molecular weight dissolved organic matter in surface waters and horizontal
off-shelf spreading of nutrients and humic-like fluorescence in the Chukchi
Sea of the Arctic Ocean, Sci. Total Environ., 639, 624–632,
https://doi.org/10.1016/j.scitotenv.2018.05.205, 2018.
Cini, R., Innocenti, N. D., Loglio, G., Stortini, A. M., and Tesei, U.:
Spectrofluorimetric evidence of the transport of marine organic matter in
Antarctic snow via air-sea interaction, Int. J. Environ. Anal. Chem., 55,
285–295, https://doi.org/10.1080/03067319408026226, 1994.
Cini, R., Degliinnocenti, N., Loglio, G., Oppo, C., Orlandi, G., Stortini,
A. M., Tesei, U., and Udisti, R.: Air-sea exchange: Sea salt and organic
microcomponents in Antarctic Snow, Int. J. Environ. Anal. Chem., 63, 15–27,
https://doi.org/10.1080/03067319608039806, 1996.
Coble, P. G.: Characterization of marine and terrestrial DOM in seawater
using excitation-emission matrix spectroscopy, Mar. Chem., 51, 325–346,
https://doi.org/10.1016/0304-4203(95)00062-3, 1996.
Coble, P. G.: Marine optical biogeochemistry: The chemistry of ocean color,
Chem. Rev., 107, 402–418, https://doi.org/10.1021/cr050350+, 2007.
Coble, P. G., Del Castillo, C. E., and Avril, B.: Distribution and optical
properties of CDOM in the Arabian Sea during the 1995 Southwest Monsoon,
Deep-Sea Res. Part II, 45, 2195–2223,
https://doi.org/10.1016/S0967-0645(98)00068-X, 1998.
Dainard, P. G., Guéguen, C., McDonald, N., and Williams, W. J.:
Photobleaching of fluorescent dissolved organic matter in Beaufort Sea and
North Atlantic Subtropical gyre, Mar. Chem., 177, 630–637,
https://doi.org/10.1016/j.marchem.2015.10.004, 2015.
Dall'Osto, M., Ovadnevaite, J., Paglione, M., Beddows, D. C. S., Ceburnis,
D., Cree, C., Cortés, P., Zamanillo, M., Nunes, S. O., Pérez, G. L.,
Ortega-Retuerta, E., Emelianov, M., Vaqué, D., Marrasé, C., Estrada,
M., Sala, M. M., Vidal, M., Fitzsimons, M. F., Beale, R., Airs, R., Rinaldi,
M., Decesari, S., Facchini, M. C., Harrison, R. M., O'Dowd, C., and
Simó, R.: Antarctic sea ice region as a source of biogenic organic
nitrogen in aerosols, Sci. Rep., 7, 6047,
https://doi.org/10.1038/s41598-017-06188-x, 2017.
D'Andrilli, J. and McConnell, J. R.: Polar ice core organic matter
signatures reveal past atmospheric carbon composition and spatial trends
across ancient and modern timescales, J. Glaciol., 67, 1028–1042,
https://doi.org/10.1017/jog.2021.51, 2021.
Davis, J. and Benner, R.: Seasonal trends in the abundance, composition and
bioavailability of particulate and dissolved organic matter in the
Chukchi/Beaufort Seas and western Canada Basin, Deep-Sea Res. Part II, 52,
3396–3410, https://doi.org/10.1016/j.dsr2.2005.09.006, 2005.
de Leeuw, G., Andreas, E. L., Anguelova, M. D., Fairall, C. W., Lewis, E.
R., O'Dowd, C., Schulz, M., and Schwartz, S. E.: Production flux of sea
spray aerosol, Rev. Geophys., 49, RG2001,
https://doi.org/10.1029/2010RG000349, 2011.
Decesari, S., Facchini, M. C., Matta, E., Lettini, F., Mircea, M., Fuzzi,
S., Tagliavini, E., and Putaud, J. -P.: Chemical features and seasonal
variation of fine aerosol water-soluble organic compounds in the Po Valley,
Italy, Atmos. Environ., 35, 3691–3699,
https://doi.org/10.1016/S1352-2310(00)00509-4, 2001.
Duarte, R. M. B. O., Pio, C. A., and Duarte, A. C.: Synchronous scan and
excitation-emission matrix fluorescence spectroscopy of water-soluble
organic compounds in atmospheric aerosols, J. Atmos. Chem., 48, 157–171,
https://doi.org/10.1023/b:joch.0000036845.82039.8c, 2004.
Elliott, S., Burrows, S. M., Deal, C., Liu, X., Long, M., Ogunro, O.,
Russell, L. M., and Wingenter, O.: Prospects for simulating macromolecular
surfactant chemistry at the ocean–atmosphere boundary, Environ. Res. Lett.,
9, 064012, https://doi.org/10.1088/1748-9326/9/6/064012, 2014.
Ervens, B., Feingold, G., and Kreidenweis, S.: Influence of water-soluble
organic carbon on cloud drop number concentration, J. Geophys. Res., 110,
D18211, https://doi.org/10.1029/2004JD005634, 2005.
Ervens, B., Turpin, B. J., and Weber, R. J.: Secondary organic aerosol formation in cloud droplets and aqueous particles (aqSOA): a review of laboratory, field and model studies, Atmos. Chem. Phys., 11, 11069–11102, https://doi.org/10.5194/acp-11-11069-2011, 2011.
Facchini, M. C., Rinaldi, M., Decesari, S., Carbone, C., Finessi, E.,
Mircea, M., Fuzzi, S., Ceburnis, D., Flanagan, R., Nilsson, E. D., de Leeuw,
G., Martino, M., Woeltjen, J., and O'Dowd, C. D.: Primary submicron marine
aerosol dominated by insoluble organic colloids and aggregates, Geophys.
Res. Lett., 35, L17814, https://doi.org/10.1029/2008GL034210, 2008.
Fan, X., Wei, S., Zhu, M., Song, J., and Peng, P.: Comprehensive characterization of humic-like substances in smoke PM2.5 emitted from the combustion of biomass materials and fossil fuels, Atmos. Chem. Phys., 16, 13321–13340, https://doi.org/10.5194/acp-16-13321-2016, 2016.
Fellman, J. B., Spencer, R. G. M., Hernes, P. J., Edwards, R. T., D'Amore,
D. V., and Hood, E.: The impact of glacier runoff on the biodegradability
and biochemical composition of terrigenous dissolved organic matter in
near-shore marine ecosystems, Mar. Chem., 121, 112–122,
https://doi.org/10.1016/j.marchem.2010.03.009, 2010.
Frka, S., Grgić, I., Turšič, J., Gini, M. I., and Eleftheriadis,
K.: Seasonal variability of carbon in humic-like matter of ambient
size-segregated water soluble organic aerosols from urban background
environment, Atmos. Environ., 173, 239–247,
https://doi.org/10.1016/j.atmosenv.2017.11.013, 2018.
Frossard, A. A., Shaw, P. M., Russell, L. M., Kroll, J. H., Canagaratna, M.
R., Worsnop, D. R., Quinn, P. K., and Bates, T. S.: Springtime Arctic haze
contributions of submicron organic particles from European and Asian
combustion sources, J. Geophys. Res. Atmos., 116, D05205,
https://doi.org/10.1029/2010JD015178, 2011.
Frossard, A. A., Russell, L. M., Burrows, S. M., Elliott, S. M., Bates, T.
S., and Quinn, P. K.: Sources and composition of submicron organic mass in
marine aerosol particles, J. Geophys. Res.-Atmos., 119, 12977–13003,
https://doi.org/10.1002/2014JD021913, 2014.
Fu, P., Kawamura, K., and Barrie, L. A.: Photochemical and other sources of
organic compounds in the Canadian high Arctic aerosol pollution during
winter-spring, Environ. Sci. Technol., 43, 286–292,
https://doi.org/10.1021/es803046q, 2009.
Fu, P., Kawamura, K., Chen, J., Qin, M., Ren, L., Sun, Y., Wang, Z., Barrie,
L. A., Tachibana, E., Ding, A., and Yamashita, Y.: Fluorescent water-soluble
organic aerosols in the High Arctic atmosphere, Sci. Rep., 5, 9845,
https://doi.org/10.1038/srep09845, 2015.
Fu, P. Q., Kawamura, K., Chen, J., Charrière, B., and Sempéré, R.: Organic molecular composition of marine aerosols over the Arctic Ocean in summer: contributions of primary emission and secondary aerosol formation, Biogeosciences, 10, 653–667, https://doi.org/10.5194/bg-10-653-2013, 2013.
Gantt, B., Meskhidze, N., Facchini, M. C., Rinaldi, M., Ceburnis, D., and O'Dowd, C. D.: Wind speed dependent size-resolved parameterization for the organic mass fraction of sea spray aerosol, Atmos. Chem. Phys., 11, 8777–8790, https://doi.org/10.5194/acp-11-8777-2011, 2011.
Gao, Z. and Guéguen, C.: Size distribution of absorbing and fluorescing
DOM in Beaufort Sea, Canada Basin, Deep-Sea Res. Part I, 121, 30–37,
https://doi.org/10.1016/j.dsr.2016.12.014, 2017.
Gelencsér, A., Hoffer, A., Krivacsy, Z., Kiss, G., Molnár, A., and
Mészáros, E.: On the possible origin of humic matter in fine
continental aerosol, J. Geophys. Res., 107, 4137,
https://doi.org/10.1029/2001JD001299, 2002.
Gelencsér, A., Hoffer, A., Kiss, G., Tombacz, E., Kurdi, R., and Bencze,
L.: In-situ formation of light-absorbing organic matter in cloud water, J.
Atmos. Chem., 45, 25–33, https://doi.org/10.1023/A:1024060428172, 2003.
Ghahremaninezhad, R., Norman, A.-L., Abbatt, J. P. D., Levasseur, M., and Thomas, J. L.: Biogenic, anthropogenic and sea salt sulfate size-segregated aerosols in the Arctic summer, Atmos. Chem. Phys., 16, 5191–5202, https://doi.org/10.5194/acp-16-5191-2016, 2016.
Gonçalves-Araujo, R., Granskog, M. A., Bracher, A., Azetsu-Scott, K.,
Dodd, P. A., and Stedmon, C. A.: Using fluorescent dissolved organic matter
to trace and distinguish the origin of Arctic surface waters, Sci. Rep., 6,
33978, https://doi.org/10.1038/srep33978, 2016.
Graber, E. R. and Rudich, Y.: Atmospheric HULIS: How humic-like are they? A comprehensive and critical review, Atmos. Chem. Phys., 6, 729–753, https://doi.org/10.5194/acp-6-729-2006, 2006.
Grannas, A. M., Jones, A. E., Dibb, J., Ammann, M., Anastasio, C., Beine, H. J., Bergin, M., Bottenheim, J., Boxe, C. S., Carver, G., Chen, G., Crawford, J. H., Dominé, F., Frey, M. M., Guzmán, M. I., Heard, D. E., Helmig, D., Hoffmann, M. R., Honrath, R. E., Huey, L. G., Hutterli, M., Jacobi, H. W., Klán, P., Lefer, B., McConnell, J., Plane, J., Sander, R., Savarino, J., Shepson, P. B., Simpson, W. R., Sodeau, J. R., von Glasow, R., Weller, R., Wolff, E. W., and Zhu, T.: An overview of snow photochemistry: evidence, mechanisms and impacts, Atmos. Chem. Phys., 7, 4329–4373, https://doi.org/10.5194/acp-7-4329-2007, 2007.
Hara, K., Osada, K., Hayashi, M., Matsunaga, K., Shibata, T., Iwasaka, Y.,
and Furuya, K.: Fractionation of inorganic nitrates in winter Arctic
troposphere: Coarse aerosol particles containing inorganic nitrates, J.
Geophys. Res.-Atmos., 104, 23671–23679,
https://doi.org/10.1029/1999JD900348, 1999.
Hawkins, L. N. and Russell, L. M.: Polysaccharides, proteins, and
phytoplankton fragments: Four chemically distinct types of marine primary
organic aerosol classified by Single Particle spectromicroscopy, Adv.
Meteorol., 2010, 1–14, https://doi.org/10.1155/2010/612132, 2010.
Held, A., Brooks, I. M., Leck, C., and Tjernström, M.: On the potential contribution of open lead particle emissions to the central Arctic aerosol concentration, Atmos. Chem. Phys., 11, 3093–3105, https://doi.org/10.5194/acp-11-3093-2011, 2011.
Herckes, P., Chang, H., Lee, T., and Collett Jr., J. L.: Air pollution
processing by radiation fogs, Water Air Soil Pollut., 181, 65–75,
https://doi.org/10.1007/s11270-006-9276-x, 2007.
Hoffer, A., Gelencsér, A., Guyon, P., Kiss, G., Schmid, O., Frank, G. P., Artaxo, P., and Andreae, M. O.: Optical properties of humic-like substances (HULIS) in biomass-burning aerosols, Atmos. Chem. Phys., 6, 3563–3570, https://doi.org/10.5194/acp-6-3563-2006, 2006.
Hole, L. R., Christensen, J. H., Ruoho-Airola, T., Tørseth, K., Ginzburg,
V., and Glowacki, P.: Past and future trends in concentrations of sulphur
and nitrogen compounds in the Arctic, Atmos. Environ., 43, 928–939,
https://doi.org/10.1016/j.atmosenv.2008.10.043, 2009.
Holmes, R. M., McClelland, J. W., Peterson, B. J., Tank, S. E., Bulygina,
E., Eglinton, T. I., Gordeev, V. V., Gurtovaya, T. Y., Raymond, P. A.,
Repeta, D. J., Staples, R., Striegl, R. G., Zhulidov, A. V., and Zimov, S.
A.: Seasonal and annual fluxes of nutrients and organic matter from large
rivers to the Arctic Ocean and surrounding seas, Estuaries Coasts, 35,
369–382, https://doi.org/10.1007/s12237-011-9386-6, 2012.
Huguet, A., Vacher, L., Relexans, S., Saubusse, S., Froidefond, J. M., and
Parlanti, E.: Properties of fluorescent dissolved organic matter in the
Gironde Estuary, Org. Geochem., 40, 706–719,
https://doi.org/10.1016/j.orggeochem.2009.03.002, 2009.
Hynes, A. J., Wine, P. H., and Semmes, D. H.: Kinetics and mechanism of
hydroxyl reactions with organic sulfides, J. Phys. Chem., 90, 4148–4156,
https://doi.org/10.1021/j100408a062, 1986.
Ishii, S. K. L. and Boyer, T. H.: Behavior of reoccurring PARAFAC components
in fluorescent dissolved organic matter in natural and engineered systems: A
critical review, Environ. Sci. Technol., 46, 2006–2017,
https://doi.org/10.1021/es2043504, 2012.
Jacob, D. J., Waldman, J. M., Munger, J. W., and Hoffmann, M. R.: A field
investigation of physical and chemical mechanisms affecting pollutant
concentrations in fog droplets, Tellus B, 36, 272–285,
https://doi.org/10.3402/tellusb.v36i4.14909, 1984.
Jung, J., Furutani, H., Uematsu, M., Kim, S., and Yoon, S.: Atmospheric inorganic nitrogen input via dry, wet, and sea fog deposition to the subarctic western North Pacific Ocean, Atmos. Chem. Phys., 13, 411–428, https://doi.org/10.5194/acp-13-411-2013, 2013.
Jung, J., Furutani, H., Uematsu, M., and Park, J.: Distributions of
atmospheric non-sea-salt sulfate and methanesulfonic acid over the Pacific
Ocean between 48∘ N and 55∘ S during summer, Atmos.
Environ., 99, 374–384, https://doi.org/10.1016/j.atmosenv.2014.10.009,
2014.
Jung, J., Han, B., Rodriguez, B., Miyazaki, Y., Chung, H. Y., Kim, K., Choi,
J.-O., Park, K., Kim, I.-N., Kim, S., Yang, E. J., and Kang, S.-H.:
Atmospheric dry deposition of water-soluble nitrogen to the subarctic
western north Pacific Ocean during summer, Atmosphere, 10, 351,
https://doi.org/10.3390/atmos10070351, 2019.
Jung, J., Hong, S.-B., Chen, M., Hur, J., Jiao, L., Lee, Y., Park, K., Hahm, D., Choi, J.-O., Yang, E. J., Park, J., Kim, T.-W., and Lee, S.: Characteristics of methanesulfonic acid, non-sea-salt sulfate and organic carbon aerosols over the Amundsen Sea, Antarctica, Atmos. Chem. Phys., 20, 5405–5424, https://doi.org/10.5194/acp-20-5405-2020, 2020.
Jung, J., Son, J. E., Lee, Y. K., Cho, K.-H., Lee, Y., Yang, E. J., Kang,
S.-H., and Hur, J.: Tracing riverine dissolved organic carbon and its
transport to the halocline layer in the Chukchi Sea (western Arctic Ocean)
using humic-like fluorescence fingerprinting, Sci. Total Environ., 772,
145542, https://doi.org/10.1016/j.scitotenv.2021.145542, 2021.
Jung, J., Miyazaki, Y., Hur, J., Lee, Y. K., Jeon, M. H., Lee, Y., Cho, K.-H., Chung, H. Y., Kim, K., Choi, J.-O., Lalande, C., Kim, J.-H., Choi, T., Yoon, Y. J., Yang, E. J., and Kang, S.-H.: Measurement Report: Summertime fluorescence characteristics of atmospheric water-soluble organic carbon in the marine boundary layer of the western Arctic Ocean [data set], https://doi.org/10.22663/KOPRI-KPDC-00002181.1, 2023.
Kanakidou, M., Seinfeld, J. H., Pandis, S. N., Barnes, I., Dentener, F. J., Facchini, M. C., Van Dingenen, R., Ervens, B., Nenes, A., Nielsen, C. J., Swietlicki, E., Putaud, J. P., Balkanski, Y., Fuzzi, S., Horth, J., Moortgat, G. K., Winterhalter, R., Myhre, C. E. L., Tsigaridis, K., Vignati, E., Stephanou, E. G., and Wilson, J.: Organic aerosol and global climate modelling: a review, Atmos. Chem. Phys., 5, 1053–1123, https://doi.org/10.5194/acp-5-1053-2005, 2005.
Kawamura, K., Narukawa, M., Li, S.-M., and Barrie, L. A.: Size distributions
of dicarboxylic acids and inorganic ions in atmospheric aerosols collected
during polar sunrise in the Canadian high Arctic, J. Geophys. Res., 112,
D10307, https://doi.org/10.1029/2006JD008244, 2007.
Kawamura, K., Ono, K., Tachibana, E., Charriére, B., and Sempéré, R.: Distributions of low molecular weight dicarboxylic acids, ketoacids and α-dicarbonyls in the marine aerosols collected over the Arctic Ocean during late summer, Biogeosciences, 9, 4725–4737, https://doi.org/10.5194/bg-9-4725-2012, 2012.
Keene, W. C., Maring, H., Maben, J. R., Kieber, D. J., Pszenny, A. A. P.,
Dahl, E. E., Izaguirre, M. A., Davis, A. J., Long, M. S., Zhou, X.,
Smoydzin, L., and Sander, R.: Chemical and physical characteristics of
nascent aerosols produced by bursting bubbles at a model air-sea interface,
J. Geophys. Res., 112, D21202, https://doi.org/10.1029/2007JD008464, 2007.
Kerminen, V.-M. and Leck, C.: Sulfur chemistry over the central Arctic Ocean
during the summer: Gas-to-particle transformation, J. Geophys. Res., 106,
32087–32099, https://doi.org/10.1029/2000JD900604, 2001.
Kieber, R. J., Whitehead, R. F., Reid, S. N., Willey, J. D., and Seaton, P.
J.: Chromophoric dissolved organic matter (CDOM) in rainwater, southeastern
North Carolina, USA, J. Atmos. Chem., 54, 21–41,
https://doi.org/10.1007/s10874-005-9008-4, 2006.
Kiss, G., Varga, B., Galambos, I., and Ganszky, I.: Characterization of
water-soluble organic matter isolated from atmospheric fine aerosol, J.
Geophys. Res., 107, 8339, https://doi.org/10.1029/2001JD000603, 2002.
Krivácsy, Z., Kiss, Gy., Varga, B., Galambos, I., Sárvári, Z.,
Gelencsér, A., Molnár, Á., Fuzzi, S., Facchini, M. C., Zappoli,
S., Andracchio, A., Alsberg, T., Hansson, H. C., and Persson, L.: Study of
humic-like substances in fog and interstitial aerosol by size-exclusion
chromatography and capillary electrophoresis, Atmos. Environ., 34,
4273–4281, https://doi.org/10.1016/S1352-2310(00)00211-9, 2000.
Kwok, R., Spreen, G., and Pang, S.: Arctic sea ice circulation and drift
speed: Decadal trends and ocean currents, J. Geophys. Res.-Oceans, 118,
2408–2425, https://doi.org/10.1002/jgrc.20191, 2013.
Lannuzel, D., Tedesco, L., van Leeuwe, M., Campbell, K., Flores, H.,
Delille, B., Miller, L., Stefels, J., Assmy, P., Bowman, J., Brown, K.,
Castellani, G., Chierici, M., Crabeck, O., Damm, E., Else, B., Fransson, A.,
Fripiat, F., Geilfus, N.-X., Jacques, C., Jones, E., Kaartokallio, H.,
Kotovitch, M., Meiners, K., Moreau, S., Nomura, D., Peeken, I., Rintala,
J.-M., Steiner, N., Tison, J.-L., Vancoppenolle, M., Van der Linden, F.,
Vichi, M., and Wongpan, P.: The future of Arctic sea-ice biogeochemistry and
ice-associated ecosystems, Nat. Clim. Change, 10, 983–992,
https://doi.org/10.1038/s41558-020-00940-4, 2020.
Laskin, A., Laskin, J., and Nizkorodov, S. A.: Chemistry of Atmospheric
Brown Carbon, Chem. Rev., 115, 4335–4382,
https://doi.org/10.1021/cr5006167, 2015.
Lawaetz, A. J. and Stedmon, C. A.: Fluorescence intensity calibration using
the Raman scatter peak of water, Appl. Spectrosc., 63, 936–940,
https://doi.org/10.1366/000370209788964548, 2009.
Leaitch, W. R., Sharma, S., Huang, L., Toom-Sauntry, D., Chivulescu, A.,
Macdonald, A. M., von Salzen, K., Pierce, J. R., Bertram, A. K., Schroder,
J. C., Shantz, N. C., Chang, R. Y. -W., and Norman, A.-L.: Dimethyl sulfide
control of the clean summertime Arctic aerosol and cloud, Elem. Sci. Anth., 1, 17, https://doi.org/10.12952/journal.elementa.000017, 2013.
Leaitch, W. R., Russell, L. M., Liu, J., Kolonjari, F., Toom, D., Huang, L., Sharma, S., Chivulescu, A., Veber, D., and Zhang, W.: Organic functional groups in the submicron aerosol at 82.5∘ N, 62.5∘ W from 2012 to 2014, Atmos. Chem. Phys., 18, 3269–3287, https://doi.org/10.5194/acp-18-3269-2018, 2018.
Leck, C. and Persson, C.: Seasonal and short-term variability in dimethyl
sulfide, sulfur dioxide and biogenic sulfur and sea salt aerosol particles
in the arctic marine boundary layer during summer and autumn, Tellus B, 48,
272–299, https://doi.org/10.1034/j.1600-0889.48.issue2.1.x, 1996.
Lee, H. J. J., Laskin, A., Laskin, J., and Nizkorodov, S. A.:
Excitation–emission spectra and fluorescence quantum yields for fresh and
aged biogenic secondary organic aerosols, Environ. Sci. Technol., 47,
5763–5770, https://doi.org/10.1021/es400644c, 2013.
Lee, Y., Min, J. O., Yang, E. J., Cho, K.-H., Jung, J., Park, J., Moon, J.
K., and Kang, S.-H.: Influence of sea ice concentration on phytoplankton
community structure in the Chukchi and East Siberian Seas, Pacific Arctic
Ocean, Deep-Sea Res. Part I, 147, 54–64,
https://doi.org/10.1016/j.dsr.2019.04.001, 2019.
Levasseur, M.: Impact of Arctic meltdown on the microbial cycling of
sulphur, Nat. Geosci., 6, 691–700, https://doi.org/10.1038/ngeo1910, 2013.
Lewis, K. M., van Dijken, G. L., and Arrigo, K. R.: Changes in phytoplankton
concentration now drive increased Arctic Ocean primary production, Science,
369, 198–202, https://doi.org/10.1126/science.aay8380, 2020.
Matsumoto, K., Tanaka, H., Nagao, I., and Ishizaka, Y.: Contribution of
particulate sulfate and organic carbon to cloud condensation nuclei in the
marine atmosphere, Geophys. Res. Lett., 24, 655–658,
https://doi.org/10.1029/97GL00541, 1997.
McKnight, D. M., Boyer, E. W., Westerhoff, P. K., Doran, P. T., Kulbe, T.,
and Andersen, D. T.: Spectrofluorometric characterization of dissolved
organic matter for indication of precursor organic material and aromaticity,
Limnol. Oceanogr., 46, 38–48, https://doi.org/10.4319/lo.2001.46.1.0038,
2001.
McNeill, V. F., Grannas, A. M., Abbatt, J. P. D., Ammann, M., Ariya, P., Bartels-Rausch, T., Domine, F., Donaldson, D. J., Guzman, M. I., Heger, D., Kahan, T. F., Klán, P., Masclin, S., Toubin, C., and Voisin, D.: Organics in environmental ices: sources, chemistry, and impacts, Atmos. Chem. Phys., 12, 9653–9678, https://doi.org/10.5194/acp-12-9653-2012, 2012.
Millero, F. J. and Sohn, M. L.: Chemical oceanography, CRC Press, Boca
Raton, FL, 521 pp., 1992.
Miyazaki, Y., Kawamura, K., Jung, J., Furutani, H., and Uematsu, M.: Latitudinal distributions of organic nitrogen and organic carbon in marine aerosols over the western North Pacific, Atmos. Chem. Phys., 11, 3037–3049, https://doi.org/10.5194/acp-11-3037-2011, 2011.
Miyazaki, Y., Coburn, S., Ono, K., Ho, D. T., Pierce, R. B., Kawamura, K., and Volkamer, R.: Contribution of dissolved organic matter to submicron water-soluble organic aerosols in the marine boundary layer over the eastern equatorial Pacific, Atmos. Chem. Phys., 16, 7695–7707, https://doi.org/10.5194/acp-16-7695-2016, 2016.
Miyazaki, Y., Suzuki, K., Tachibana, E., Yamashita, Y., Müller, A.,
Kawana, K., and Nishioka, J.: New index of organic mass enrichment in sea
spray aerosols linked with senescent status in marine phytoplankton, Sci.
Rep., 10, 17042, https://doi.org/10.1038/s41598-020-73718-5, 2020.
Miyazaki, Y., Yamashita, Y., Kawana, K., Tachibana, E., Kagami, S., Mochida,
M., Suzuki, K., and Nishioka, J.: Chemical transfer of dissolved organic
matter from surface seawater to sea spray water-soluble organic aerosol in
the marine atmosphere, Sci. Rep., 8, 14861,
https://doi.org/10.1038/s41598-018-32864-7, 2018.
Mladenov, N., Alados-Arboledas, L., Olmo, F. J., Lyamani, H., Delgado, A.,
Molina, A., and Reche, I.: Applications of optical spectroscopy and stable
isotope analyses to organic aerosol source discrimination in an urban area,
Atmos. Environ., 45, 1960–1969,
https://doi.org/10.1016/j.atmosenv.2011.01.029, 2011.
Morin, S., Savarino, J., Frey, M. M., Yan, N., Bekki, S., Bottenheim, J. W.,
and Martins, J. M. F.: Tracing the origin and fate of NOx in the Arctic
atmosphere using stable isotopes in nitrate, Science, 322, 730–732,
https://doi.org/10.1126/science.1161910, 2008.
Mungall, E. L., Abbatt, J. P. D., Wentzell, J. J. B., Lee, A. K. Y., Thomas,
J. L., Blais, M., Gosselin, M., Miller, L. A., Papakyriakou, T., Willis, M.
D., and Liggio, J.: Microlayer source of oxygenated volatile organic
compounds in the summertime marine Arctic boundary layer, P. Natl. Acad.
Sci. USA, 114, 6203–6208, https://doi.org/10.1073/pnas.1620571114, 2017.
Murphy, K. R., Stedmon, C. A., Wenig, P., and Bro, R.: OpenFluor – an online
spectral library of auto-fluorescence by organic compounds in the
environment, Anal. Methods, 6, 658–661, https://doi.org/10.1039/C3AY41935E,
2014.
Narukawa, M., Kawamura, K., Li, S.-M., and Bottenheim, J. W.: Stable carbon
isotopic ratios and ionic composition of the high-Arctic aerosols: An
increase in δ13C values from winter to spring, J. Geophys.
Res., 113, D02312, https://doi.org/10.1029/2007JD008755, 2008.
Nielsen, I. E., Skov, H., Massling, A., Eriksson, A. C., Dall'Osto, M., Junninen, H., Sarnela, N., Lange, R., Collier, S., Zhang, Q., Cappa, C. D., and Nøjgaard, J. K.: Biogenic and anthropogenic sources of aerosols at the High Arctic site Villum Research Station, Atmos. Chem. Phys., 19, 10239–10256, https://doi.org/10.5194/acp-19-10239-2019, 2019.
Nilsson, E. D., Rannik, Ü., Swietlicki, E., Leck, C., Aalto, P. P.,
Zhou, J., and Norman, M.: Turbulent aerosol fluxes over the Arctic Ocean: 2.
Wind-driven sources from the sea, J. Geophys. Res., 106, 32139–32154,
https://doi.org/10.1029/2000JD900747, 2001.
Nozière, B., Dziedzic, P., and Córdova, A.: Formation of secondary
light-absorbing “fulvic-like” oligomers: A common process in aqueous and
ionic atmospheric particles?, Geophys. Res. Lett., 34, L21812,
https://doi.org/10.1029/2007GL031300, 2007.
O'Dowd, C. D. and De Leeuw, G.: Marine aerosol production: A review of the
current knowledge, Philos. T. R. Soc. A, 365, 1753–1774,
https://doi.org/10.1098/rsta.2007.2043, 2007.
O'Dowd, C. D., Facchini, M. C., Cavalli, F., Ceburnis, D., Mircea, M.,
Decesari, S., Fuzzi, S., Yoon, Y.-J., and Putaud, J.-P.: Biogenically driven
organic contribution to marine aerosol, Nature, 431, 676–680,
https://doi.org/10.1038/nature02959, 2004.
Osburn, C. L., Anderson, N. J., Stedmon, C. A., Giles, M. E., Whiteford, E.
J., McGenity, T. J., Dumbrell, A. J., and Underwood, G. J. C.: Shifts in the
source and composition of dissolved organic matter in Southwest Greenland
lakes along a regional hydro-climatic gradient. J. Geophys. Res.-Biogeo., 122, 3431–3445, https://doi.org/10.1002/2017JG003999, 2017.
Pani, S. K., Lee, C.-T., Griffth, S. M., and Lin, N.-H.: Humic-like
substances (HULIS) in springtime aerosols at a high-altitude background
station in the western North Pacific: Source attribution, abundance, and
light-absorption, Sci. Total Environ., 809, 151180,
https://doi.org/10.1016/j.scitotenv.2021.151180, 2022.
Park, J., Dall'Osto, M., Park, K., Kim, J.-H., Park, J., Park, K.-T., Hwang,
C. Y., Jang, G. I., Gim, Y., Kang, S., Park, S., Jin, Y. K., Yum, S. S.,
Simó, R., and Yoon, Y.-J.: Arctic primary aerosol production strongly
influenced by riverine organic matter, Environ. Sci. Technol., 53,
8621–8630, https://doi.org/10.1021/acs.est.9b03399, 2019a.
Park, K., Kim, I., Choi, J.-O., Lee, Y., Jung, J., Ha, S.-Y., Kim, J.-H.,
and Zhang, M.: Unexpectedly high dimethyl sulfide concentration in
high-latitude Arctic sea ice melt ponds, Environ. Sci.-Proc. Imp.,
21, 1642–1649, https://doi.org/10.1039/c9em00195f, 2019b.
Perovich, D., Meier, W., Tschudi, T., Hendricks, S., Petty, A. A., Divine,
D., Farrell, S., Gerland, S., Haas, C., Kaleschke, L., Pavlova, O., Ricker,
R., Tian-Kunze, X., Webster, M., and Wood, K.: Sea ice, NOAA Arctic Report
Card 2020, https://www.arctic.noaa.gov/Report-Card (last access: 21 May 2022), 2020.
Psichoudaki, M. and Pandis, S. N.: Atmospheric aerosol water-soluble organic
carbon measurement: A theoretical analysis, Environ. Sci. Technol., 47,
9791–9798, https://doi.org/10.1021/es402270y, 2013.
Qin, J., Zhang, L., Zhou, X., Duan, J., Mu, S., Xiao, K., Hu, J., and Tan,
J.: Fluorescence fingerprinting properties for exploring water-soluble
organic compounds in PM2.5 in an industrial city of northwest China, Atmos.
Environ., 184, 203–211, https://doi.org/10.1016/j.atmosenv.2018.04.049,
2018.
Quinn, P. K., Miller, T. L., Bates, T. S., Ogren, J. A., Andrews, E., and
Shaw, G. E.: A 3-year record of simultaneously measured aerosol chemical and
optical properties at Barrow, Alaska, J. Geophys. Res., 107, AAC 8-1–AAC
8-15, https://doi.org/10.1029/2001JD001248, 2002.
Quinn, P. K., Shaw, G., Andrews, E., Dutton, E. G., Ruoho-Airola, T., and
Gong, S. L.: Arctic haze: current trends and knowledge gaps, Tellus B, 59, 99–114,
https://doi.org/10.1111/j.1600-0889.2006.00236.x, 2007.
Quinn, P. K., Bates, T. S., Schulz, K., and Shaw, G. E.: Decadal trends in aerosol chemical composition at Barrow, Alaska: 1976–2008, Atmos. Chem. Phys., 9, 8883–8888, https://doi.org/10.5194/acp-9-8883-2009, 2009.
Quinn, P. K. and Bates, T. S.: The case against climate regulation via
oceanic phytoplankton sulphur emissions, Nature, 480, 51–56,
https://doi.org/10.1038/nature10580, 2011.
Quinn, P. K., Bates, T. S., Schulz, K. S., Coffman, D. J., Frossard, A. A.,
Russell, L. M., Keene, W. C., and Kieber, D. J.: Contribution of sea surface
carbon pool to organic matter enrichment in sea spray aerosol, Nat. Geosci.,
7, 228–232, https://doi.org/10.1038/NGEO2092, 2014.
Rinaldi, M., Decesari, S., Finessi, E., Giulianelli, L., Carbone, C., Fuzzi,
S., O'Dowd, C. D., Ceburnis, D., and Facchini, M. C.: Primary and secondary
organic marine aerosol and oceanic biological activity: Recent results and
new perspectives for future studies, Adv. Meteorol., 2010, 1–10,
https://doi.org/10.1155/2010/310682, 2010.
Russell, L. M., Hawkins, L. N., Frossard, A. A., Quinn, P. K., and Bates, T.
S.: Carbohydrate-like composition of submicron atmospheric particles and
their production from ocean bubble bursting, P. Natl. Acad. Sci. USA,
107, 6652–6657, https://doi.org/10.1073/pnas.0908905107, 2010.
Salma, I., Mészáros, T., and Maenhaut, W.: Mass size distribution of
carbon in atmospheric humic-like substances and water soluble organic carbon
for an urban environment, J. Aerosol Sci., 56, 53–60,
https://doi.org/10.1016/j.jaerosci.2012.06.006, 2013.
Sasakawa, M., Ooki, A., and Uematsu, M.: Aerosol size distribution during
sea fog and its scavenge process of chemical substances over the
northwestern North Pacific, J. Geophys. Res., 108, 4120,
https://doi.org/10.1029/2002JD002329, 2003.
Saxena, P., Hildemann, L. M., McMurry, P. H., and Seinfeld, J. H.: Organics
alter hygroscopic behavior of atmospheric particles, J. Geophys. Res., 100,
18755–18770, https://doi.org/10.1029/95JD01835, 1995.
Shaw, P. M., Russell, L. M., Jefferson, A., and Quinn, P. K.: Arctic organic
aerosol measurements show particles from mixed combustion in spring haze and
from frost flowers in winter, Geophys. Res. Lett., 37, L10803,
https://doi.org/10.1029/2010GL042831, 2010.
Shen, Y., Fichot, C. G., and Benner, R.: Dissolved organic matter composition and bioavailability reflect ecosystem productivity in the Western Arctic Ocean, Biogeosciences, 9, 4993–5005, https://doi.org/10.5194/bg-9-4993-2012, 2012.
Shimada, K., Kamoshida, T., Itoh, M., Nishino, S., Carmack, E., McLaughlin,
F., Zimmermann, S., and Proshutinsky, A.: Pacific Ocean inflow: Influence on
catastrophic reduction of sea ice cover in the Arctic Ocean, Geophys. Res.
Lett., 33, L08605, https://doi.org/10.1029/2005GL025624, 2006.
Sirois, A. and Barrie, L. A.: Arctic lower tropospheric aerosol trends and
composition at Alert, Canada: 1980–1995, J. Geophys. Res., 104,
11599–11618, https://doi.org/10.1029/1999JD900077, 1999.
Spreen, G., Kaleschke, L., and Heygster, G.: Sea ice remote sensing using
AMSR-E 89-GHz channels, J. Geophys. Res., 113, C02S03,
https://doi.org/10.1029/2005JC003384, 2008.
Stedmon, C. A. and Bro, R.: Characterizing dissolved organic matter
fluorescence with parallel factor analysis: a tutorial, Limnol. Oceanogr.
Methods, 6, 572–579, https://doi.org/10.4319/lom.2008.6.572, 2008.
Stedmon, C. A., Markager, S., and Bro, R.: Tracing dissolved organic matter
in aquatic environments using a new approach to fluorescence spectroscopy,
Mar. Chem., 82, 239–254, https://doi.org/10.1016/S0304-4203(03)00072-0,
2003.
Stein, A. F., Draxler, R. R., Rolph, G. D., Stunder, B. J. B, Cohen, M. D.,
and Ngan, F.: NOAA's HYSPLIT atmospheric transport and dispersion modeling
system, B. Am. Meteorol. Soc., 96, 2059–2077,
https://doi.org/10.1175/BAMS-D-14-00110.1, 2015.
Stohl, A.: Characteristics of atmospheric transport into the Arctic
troposphere, J. Geophys. Res., 111, D11306,
https://doi.org/10.1029/2005JD006888, 2006.
Sullivan, A. P., Weber, R. J., Clements, A. L., Turner, J. R., Bae, M. S.,
and Schauer, J. J.: A method for on-line measurement of water-soluble
organic carbon in ambient aerosol particles: Results from an urban site,
Geophys. Res. Lett., 31, L13105, https://doi.org/10.1029/2004GL019681, 2004.
Tang, J., Wang, J., Zhong, G., Jiang, H., Mo, Y., Zhang, B., Geng, X., Chen, Y., Tang, J., Tian, C., Bualert, S., Li, J., and Zhang, G.: Measurement report: Long-emission-wavelength chromophores dominate the light absorption of brown carbon in aerosols over Bangkok: impact from biomass burning, Atmos. Chem. Phys., 21, 11337–11352, https://doi.org/10.5194/acp-21-11337-2021, 2021.
Tsui, W. G. and McNeill, V. F.: Modeling secondary organic aerosol
production from photosensitized humic-like substances (HULIS), Environ. Sci.
Technol. Lett., 5, 255–259, https://doi.org/10.1021/acs.estlett.8b00101,
2018.
Vidovicì, K., Jurkovicì, D. L., Šala, M., Kroflič, A., and Grgic, I.:
Nighttime aqueous-phase formation of nitrocatechols in the atmospheric
condensed phase, Environ. Sci. Technol., 52, 9722–9730,
https://doi.org/10.1021/acs.est.8b01161, 2018.
Voisin, D., Jaffrezo, J.-L., Houdier, S., Barret, M., Cozic, J., King, M.
D., France, J. L., Reay, H. J., Grannas, A., Kos, G., Ariya, P. A., Beine,
H. J., and Domine, F.: Carbonaceous species and humic like substances
(HULIS) in Arctic snowpack during OASIS field campaign in Barrow, J.
Geophys. Res., 117, D00R19, https://doi.org/10.1029/2011JD016612, 2012.
Willis, M. D., Leaitch, W. R., and Abbatt, J. P. D.: Processes controlling
the composition and abundance of Arctic aerosol, Rev. Geophys., 56,
621–671, https://doi.org/10.1029/2018RG000602, 2018.
Wilson, T. W., Ladino, L. A., Alpert, P. A., Breckels, M. N., Brooks, I. M.,
Browse, J., Burrows, S. M., Carslaw, K. S., Huffman, J. A., Judd, C.,
Kilthau, W. P., Mason, R. H., McFiggans, G., Miller, L. A., Nájera, J.
J., Polishchuk, E., Rae, S., Schiller, C. L., Si, M., Temprado, J. V.,
Whale, T. F., Wong, J. P. S., Wurl, O., Yakobi-Hancock, J. D., Abbatt, J. P.
D., Aller, J. Y., Bertram, A. K., Knopf, D. A., and Murray, B. J.: A marine
biogenic source of atmospheric ice-nucleating particles, Nature, 525,
234–238, https://doi.org/10.1038/nature14986, 2015.
Wu, G., Fu, P., Ram, K., Song, J., Chen, Q., Kawamura, K., Wan, X., Kang,
S., Wang, X., Laskin, A., and Cong, Z.: Fluorescence characteristics of
water-soluble organic carbon in atmospheric aerosol, Environ. Pollut., 268,
115906, https://doi.org/10.1016/j.envpol.2020.115906, 2021.
Xie, M., Mladenov, N., Williams, M. W., Neff, J. C., Wasswa, J., and
Hannigan, M. P.: Water soluble organic aerosols in the Colorado Rocky
Mountains, USA: composition, sources and optical properties, Sci. Rep., 6,
39339, https://doi.org/10.1038/srep39339, 2016.
Yamashita, Y. and Tanoue, E.: In situ production of chromophoric dissolved
organic matter in coastal environments, Geophys. Res. Lett., 31, L14302,
https://doi.org/10.1029/2004GL019734, 2004.
Yamashita, Y. and Tanoue, E.: Production of bio-refractory fluorescent
dissolved organic matter in the ocean interior, Nat. Geosci., 1, 579–582,
https://doi.org/10.1038/ngeo279, 2008.
Yamashita, Y., Jaffé, R., Maie, N., and Tanoue, E.: Assessing the
dynamics of dissolved organic matter (DOM) in coastal environments by
excitation emission matrix fluorescence and parallel factor analysis
(EEM-PARAFAC), Limnol. Oceanogr., 53, 1900–1908,
https://doi.org/10.4319/lo.2008.53.5.1900, 2008.
Yamashita, Y., Panton, A., Mahaffey, C., and Jaffé, R.: Assessing the
spatial and temporal variability of dissolved organic matter in Liverpool
Bay using excitation–emission matrix fluorescence and parallel factor
analysis, Ocean Dynam., 61, 569–579,
https://doi.org/10.1007/s10236-010-0365-4, 2011.
Yamashita, Y., Boyer, J. N., and Jaffé, R.: Evaluating the distribution
of terrestrial dissolved organic matter in a complex coastal ecosystem using
fluorescence spectroscopy, Con. Shelf Res., 66, 136–144,
https://doi.org/10.1016/j.csr.2013.06.010, 2013.
Yang, L., Chen, W., Zhuang, W. -E., Cheng, Q., Li, W., Wang, H., Guo, W.,
Chen, C. -T. A., and Liu, M.: Characterization and bioavailability of
rainwater dissolved organic matter at the southeast coast of China using
absorption spectroscopy and fluorescence EEM-PARAFAC, Estuar. Coast.
Shelf Sci., 217, 45–55, https://doi.org/10.1016/j.ecss.2018.11.002, 2019.
Yu, C., Yan, J., Zhang, H., Lin, Q., Zheng, H., Zhong, X., Zhao, S., Zhang,
M., Zhao, S., and Li, X.: Characteristics of aerosol WSI with
high-time-resolution observation over Arctic Ocean, Earth Space Sci., 7,
e2020EA001227, https://doi.org/10.1029/2020EA001227, 2020.
Zheng, G., He, K., Duan, F., Cheng, Y., and Ma, Y.: Measurement of
humic-like substances in aerosols: A review, Environ. Pollut., 181,
301–314, https://doi.org/10.1016/j.envpol.2013.05.055, 2013.
Zsolnay, A., Baigar, E., Jimenez, M., Steinweg, B., and Saccomandi, F.:
Differentiating with fluorescence spectroscopy the sources of dissolved
organic matter in soils subjected to drying, Chemosphere, 38, 45–50,
https://doi.org/10.1016/S0045-6535(98)00166-0, 1999.
Short summary
This study examined the summertime fluorescence properties of water-soluble organic carbon (WSOC) in aerosols over the western Arctic Ocean. We found that the WSOC in fine-mode aerosols in coastal areas showed a higher polycondensation degree and aromaticity than in sea-ice-covered areas. The fluorescence properties of atmospheric WSOC in the summertime marine Arctic boundary can improve our understanding of the WSOC chemical and biological linkages at the ocean–sea-ice–atmosphere interface.
This study examined the summertime fluorescence properties of water-soluble organic carbon...
Altmetrics
Final-revised paper
Preprint