Articles | Volume 22, issue 3
https://doi.org/10.5194/acp-22-1905-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-1905-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
The impact of atmospheric blocking on the compounding effect of ozone pollution and temperature: a copula-based approach
Institute for Advanced Sustainability Studies, Potsdam, Germany
Institut für Meteorologie, Freie Universität Berlin, Berlin, Germany
now at: Oeschger Centre for Climate Change Research (OCCR), Bern, Switzerland
Oscar E. Jurado
Institut für Meteorologie, Freie Universität Berlin, Berlin, Germany
Tim Butler
Institute for Advanced Sustainability Studies, Potsdam, Germany
Institut für Meteorologie, Freie Universität Berlin, Berlin, Germany
Henning W. Rust
Institut für Meteorologie, Freie Universität Berlin, Berlin, Germany
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Atmos. Chem. Phys., 22, 11675–11699, https://doi.org/10.5194/acp-22-11675-2022, https://doi.org/10.5194/acp-22-11675-2022, 2022
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Ground-level ozone is an important air pollutant that affects human health, ecosystems, and climate. Ozone is not emitted directly but rather formed in the atmosphere through chemical reactions involving two distinct precursors. Our results provide detailed information about the origin of ozone in Germany during two peak ozone events that took place in 2015 and 2018, thus improving our understanding of ground-level ozone.
Svetlana Tsyro, Wenche Aas, Augustin Colette, Camilla Andersson, Bertrand Bessagnet, Giancarlo Ciarelli, Florian Couvidat, Kees Cuvelier, Astrid Manders, Kathleen Mar, Mihaela Mircea, Noelia Otero, Maria-Teresa Pay, Valentin Raffort, Yelva Roustan, Mark R. Theobald, Marta G. Vivanco, Hilde Fagerli, Peter Wind, Gino Briganti, Andrea Cappelletti, Massimo D'Isidoro, and Mario Adani
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Particulate matter (PM) air pollution causes adverse health effects. In Europe, the emissions caused by anthropogenic activities have been reduced in the last decades. To assess the efficiency of emission reductions in improving air quality, we have studied the evolution of PM pollution in Europe. Simulations with six air quality models and observational data indicate a decrease in PM concentrations by 10 % to 30 % across Europe from 2000 to 2010, which is mainly a result of emission reductions.
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Atmos. Chem. Phys., 21, 4007–4023, https://doi.org/10.5194/acp-21-4007-2021, https://doi.org/10.5194/acp-21-4007-2021, 2021
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NO2 limit values are still regularly exceeded in many European cities despite decreasing emissions. Measurements of NOx concentrations from stations across Europe were systematically analysed to assess long-term changes observed in urban areas. We compared trends in concentration increments to trends in total and traffic emissions to find potential discrepancies. The results can help in evaluating inaccuracies in emission inventories and in improving spatial imbalances in data availability.
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This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Nat. Hazards Earth Syst. Sci., 25, 2331–2350, https://doi.org/10.5194/nhess-25-2331-2025, https://doi.org/10.5194/nhess-25-2331-2025, 2025
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Geosci. Model Dev., 18, 3265–3309, https://doi.org/10.5194/gmd-18-3265-2025, https://doi.org/10.5194/gmd-18-3265-2025, 2025
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The multi-model experiment design of the HTAP3 Fires project takes a multi-pollutant approach to improving our understanding of transboundary transport of wildland fire and agricultural burning emissions and their impacts. The experiments are designed with the goal of answering science policy questions related to fires. The options for the multi-model approach, including inputs, outputs, and model setup, are discussed, and the official recommendations for the project are presented.
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Atmos. Chem. Phys., 25, 5287–5311, https://doi.org/10.5194/acp-25-5287-2025, https://doi.org/10.5194/acp-25-5287-2025, 2025
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Deforestation has a significant impact on climate, yet its effects on drought remain less understood. This study investigates how deforestation affects drought across various climate zones and timescales. Findings indicate that deforestation leads to drier conditions in tropical regions and wetter conditions in arid areas, with minimal effects in temperate zones. Long-term drought is more affected than short-term drought, offering valuable insights into vegetation–climate interactions.
Ioannis Kioutsioukis, Christian Hogrefe, Paul A. Makar, Ummugulsun Alyuz, Jessy O. Bash, Roberto Bellasio, Roberto Bianconi, Tim Buttler, Olivia E. Clifton, Philippe Cheung, Alma Hodzic, Richard Kranenburg, Aurelia Lupascu, Kester Momoh, Juan Luis Perez-Camaño, John Pleim, Young-Hee Ryu, Robero San Jose, Donna Schwede, Ranjeet Sokhi, and Stefano Galmarini
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Edward C. Chan, Ilona J. Jäkel, Basit Khan, Martijn Schaap, Timothy M. Butler, Renate Forkel, and Sabine Banzhaf
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Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-601, https://doi.org/10.5194/essd-2024-601, 2025
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EGUsphere, https://doi.org/10.5194/egusphere-2025-225, https://doi.org/10.5194/egusphere-2025-225, 2025
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Performed under the umbrella of the fourth phase of the Air Quality Model Evaluation International Initiative (AQMEII4), this study applies AQMEII4 diagnostic tools to better characterize how dry deposition removes pollutants from the atmosphere in regional-scale models. The results also strongly suggest that improvement and harmonization of the representation of land use in these models would serve the community in their future development efforts.
Andy Richling, Jens Grieger, and Henning W. Rust
Geosci. Model Dev., 18, 361–375, https://doi.org/10.5194/gmd-18-361-2025, https://doi.org/10.5194/gmd-18-361-2025, 2025
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The performance of weather and climate prediction systems is variable in time and space. It is of interest how this performance varies in different situations. We provide a decomposition of a skill score (a measure of forecast performance) as a tool for detailed assessment of performance variability to support model development or forecast improvement. The framework is exemplified with decadal forecasts to assess the impact of different ocean states in the North Atlantic on temperature forecast.
Tabish Ansari, Aditya Nalam, Aurelia Lupaşcu, Carsten Hinz, Simon Grasse, and Tim Butler
EGUsphere, https://doi.org/10.5194/egusphere-2024-3752, https://doi.org/10.5194/egusphere-2024-3752, 2024
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Surface ozone can travel far from its sources. In recent decades, emissions of ozone-forming gases have decreased in North America and Europe but risen in Asia, alongside rising global methane levels. Using advanced modeling, this study reveals that while local reductions in nitrogen oxides have lowered summer ozone, increases in natural and foreign sources offset these gains. Methane remains important, but its ozone impact has declined with reduced local emissions.
Madlen Peter, Henning W. Rust, and Uwe Ulbrich
Nat. Hazards Earth Syst. Sci., 24, 1261–1285, https://doi.org/10.5194/nhess-24-1261-2024, https://doi.org/10.5194/nhess-24-1261-2024, 2024
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The paper introduces a statistical modeling approach describing daily extreme precipitation in Germany more accurately by including changes within the year and between the years simultaneously. The changing seasonality over years is regionally divergent and mainly weak. However, some regions stand out with a more pronounced linear rise of summer intensities, indicating a possible climate change signal. Improved modeling of extreme precipitation is beneficial for risk assessment and adaptation.
Yan Li, Bo Huang, and Henning W. Rust
Hydrol. Earth Syst. Sci., 28, 321–339, https://doi.org/10.5194/hess-28-321-2024, https://doi.org/10.5194/hess-28-321-2024, 2024
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The inconsistent changes in temperature and precipitation induced by forest cover change are very likely to affect drought condition. We use a set of statistical models to explore the relationship between forest cover change and drought change in different timescales and climate zones. We find that the influence of forest cover on droughts varies under different precipitation and temperature quantiles. Forest cover also could modulate the impacts of precipitation and temperature on drought.
Johannes Riebold, Andy Richling, Uwe Ulbrich, Henning Rust, Tido Semmler, and Dörthe Handorf
Weather Clim. Dynam., 4, 663–682, https://doi.org/10.5194/wcd-4-663-2023, https://doi.org/10.5194/wcd-4-663-2023, 2023
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Arctic sea ice loss might impact the atmospheric circulation outside the Arctic and therefore extremes over mid-latitudes. Here, we analyze model experiments to initially assess the influence of sea ice loss on occurrence frequencies of large-scale circulation patterns. Some of these detected circulation changes can be linked to changes in occurrences of European temperature extremes. Compared to future global temperature increases, the sea-ice-related impacts are however of secondary relevance.
Monica Crippa, Diego Guizzardi, Tim Butler, Terry Keating, Rosa Wu, Jacek Kaminski, Jeroen Kuenen, Junichi Kurokawa, Satoru Chatani, Tazuko Morikawa, George Pouliot, Jacinthe Racine, Michael D. Moran, Zbigniew Klimont, Patrick M. Manseau, Rabab Mashayekhi, Barron H. Henderson, Steven J. Smith, Harrison Suchyta, Marilena Muntean, Efisio Solazzo, Manjola Banja, Edwin Schaaf, Federico Pagani, Jung-Hun Woo, Jinseok Kim, Fabio Monforti-Ferrario, Enrico Pisoni, Junhua Zhang, David Niemi, Mourad Sassi, Tabish Ansari, and Kristen Foley
Earth Syst. Sci. Data, 15, 2667–2694, https://doi.org/10.5194/essd-15-2667-2023, https://doi.org/10.5194/essd-15-2667-2023, 2023
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This study responds to the global and regional atmospheric modelling community's need for a mosaic of air pollutant emissions with global coverage, long time series, spatially distributed data at a high time resolution, and a high sectoral resolution in order to enhance the understanding of transboundary air pollution. The mosaic approach to integrating official regional emission inventories with a global inventory based on a consistent methodology ensures policy-relevant results.
Edward C. Chan, Joana Leitão, Andreas Kerschbaumer, and Timothy M. Butler
Geosci. Model Dev., 16, 1427–1444, https://doi.org/10.5194/gmd-16-1427-2023, https://doi.org/10.5194/gmd-16-1427-2023, 2023
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Yeti is a Handbook Emission Factors for Road Transport-based traffic emission inventory written in the Python 3 scripting language, which adopts a generalized treatment for activity data using traffic information of varying levels of detail introduced in a systematic and consistent manner, with the ability to maximize reusability. Thus, Yeti has been conceived and implemented with a high degree of data and process symmetry, allowing scalable and flexible execution while affording ease of use.
Edmund P. Meredith, Uwe Ulbrich, and Henning W. Rust
Geosci. Model Dev., 16, 851–867, https://doi.org/10.5194/gmd-16-851-2023, https://doi.org/10.5194/gmd-16-851-2023, 2023
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Cell-tracking algorithms allow for the study of properties of a convective cell across its lifetime and, in particular, how these respond to climate change. We investigated whether the design of the algorithm can affect the magnitude of the climate-change signal. The algorithm's criteria for identifying a cell were found to have a strong impact on the warming response. The sensitivity of the warming response to different algorithm settings and cell types should thus be fully explored.
Felix Kleinert, Lukas H. Leufen, Aurelia Lupascu, Tim Butler, and Martin G. Schultz
Geosci. Model Dev., 15, 8913–8930, https://doi.org/10.5194/gmd-15-8913-2022, https://doi.org/10.5194/gmd-15-8913-2022, 2022
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We examine the effects of spatially aggregated upstream information as input for a deep learning model forecasting near-surface ozone levels. Using aggregated data from one upstream sector (45°) improves the forecast by ~ 10 % for 4 prediction days. Three upstream sectors improve the forecasts by ~ 14 % on the first 2 d only. Our results serve as an orientation for other researchers or environmental agencies focusing on pointwise time-series predictions, for example, due to regulatory purposes.
Alberto Caldas-Alvarez, Markus Augenstein, Georgy Ayzel, Klemens Barfus, Ribu Cherian, Lisa Dillenardt, Felix Fauer, Hendrik Feldmann, Maik Heistermann, Alexia Karwat, Frank Kaspar, Heidi Kreibich, Etor Emanuel Lucio-Eceiza, Edmund P. Meredith, Susanna Mohr, Deborah Niermann, Stephan Pfahl, Florian Ruff, Henning W. Rust, Lukas Schoppa, Thomas Schwitalla, Stella Steidl, Annegret H. Thieken, Jordis S. Tradowsky, Volker Wulfmeyer, and Johannes Quaas
Nat. Hazards Earth Syst. Sci., 22, 3701–3724, https://doi.org/10.5194/nhess-22-3701-2022, https://doi.org/10.5194/nhess-22-3701-2022, 2022
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In a warming climate, extreme precipitation events are becoming more frequent. To advance our knowledge on such phenomena, we present a multidisciplinary analysis of a selected case study that took place on 29 June 2017 in the Berlin metropolitan area. Our analysis provides evidence of the extremeness of the case from the atmospheric and the impacts perspectives as well as new insights on the physical mechanisms of the event at the meteorological and climate scales.
Johana Romero-Alvarez, Aurelia Lupaşcu, Douglas Lowe, Alba Badia, Scott Archer-Nicholls, Steve Dorling, Claire E. Reeves, and Tim Butler
Atmos. Chem. Phys., 22, 13797–13815, https://doi.org/10.5194/acp-22-13797-2022, https://doi.org/10.5194/acp-22-13797-2022, 2022
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As ozone can be transported across countries, efficient air quality management and regulatory policies rely on the assessment of local ozone production vs. transport. In our study, we investigate the origin of surface ozone in the UK and the contribution of the different source regions to regulatory ozone metrics. It is shown that emission controls would be necessary over western Europe to improve health-related metrics and over larger areas to reduce impacts on ecosystems.
Aurelia Lupaşcu, Noelia Otero, Andrea Minkos, and Tim Butler
Atmos. Chem. Phys., 22, 11675–11699, https://doi.org/10.5194/acp-22-11675-2022, https://doi.org/10.5194/acp-22-11675-2022, 2022
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Ground-level ozone is an important air pollutant that affects human health, ecosystems, and climate. Ozone is not emitted directly but rather formed in the atmosphere through chemical reactions involving two distinct precursors. Our results provide detailed information about the origin of ozone in Germany during two peak ozone events that took place in 2015 and 2018, thus improving our understanding of ground-level ozone.
Svetlana Tsyro, Wenche Aas, Augustin Colette, Camilla Andersson, Bertrand Bessagnet, Giancarlo Ciarelli, Florian Couvidat, Kees Cuvelier, Astrid Manders, Kathleen Mar, Mihaela Mircea, Noelia Otero, Maria-Teresa Pay, Valentin Raffort, Yelva Roustan, Mark R. Theobald, Marta G. Vivanco, Hilde Fagerli, Peter Wind, Gino Briganti, Andrea Cappelletti, Massimo D'Isidoro, and Mario Adani
Atmos. Chem. Phys., 22, 7207–7257, https://doi.org/10.5194/acp-22-7207-2022, https://doi.org/10.5194/acp-22-7207-2022, 2022
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Particulate matter (PM) air pollution causes adverse health effects. In Europe, the emissions caused by anthropogenic activities have been reduced in the last decades. To assess the efficiency of emission reductions in improving air quality, we have studied the evolution of PM pollution in Europe. Simulations with six air quality models and observational data indicate a decrease in PM concentrations by 10 % to 30 % across Europe from 2000 to 2010, which is mainly a result of emission reductions.
Robert Polzin, Annette Müller, Henning Rust, Peter Névir, and Péter Koltai
Nonlin. Processes Geophys., 29, 37–52, https://doi.org/10.5194/npg-29-37-2022, https://doi.org/10.5194/npg-29-37-2022, 2022
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In this study, a recent algorithmic framework called Direct Bayesian Model Reduction (DBMR) is applied which provides a scalable probability-preserving identification of reduced models directly from data. The stochastic method is tested in a meteorological application towards a model reduction to latent states of smaller scale convective activity conditioned on large-scale atmospheric flow.
Felix S. Fauer, Jana Ulrich, Oscar E. Jurado, and Henning W. Rust
Hydrol. Earth Syst. Sci., 25, 6479–6494, https://doi.org/10.5194/hess-25-6479-2021, https://doi.org/10.5194/hess-25-6479-2021, 2021
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Extreme rainfall events are modeled in this study for different timescales. A new parameterization of the dependence between extreme values and their timescale enables our model to estimate extremes on very short (1 min) and long (5 d) timescales simultaneously. We compare different approaches of modeling this dependence and find that our new model improves performance for timescales between 2 h and 2 d without affecting model performance on other timescales.
Jana Ulrich, Felix S. Fauer, and Henning W. Rust
Hydrol. Earth Syst. Sci., 25, 6133–6149, https://doi.org/10.5194/hess-25-6133-2021, https://doi.org/10.5194/hess-25-6133-2021, 2021
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The characteristics of extreme precipitation on different timescales as well as in different seasons are relevant information, e.g., for designing hydrological structures or managing water supplies. Therefore, our aim is to describe these characteristics simultaneously within one model. We find similar characteristics for short extreme precipitation at all considered stations in Germany but pronounced regional differences with respect to the seasonality of long-lasting extreme events.
Stefano Galmarini, Paul Makar, Olivia E. Clifton, Christian Hogrefe, Jesse O. Bash, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Tim Butler, Jason Ducker, Johannes Flemming, Alma Hodzic, Christopher D. Holmes, Ioannis Kioutsioukis, Richard Kranenburg, Aurelia Lupascu, Juan Luis Perez-Camanyo, Jonathan Pleim, Young-Hee Ryu, Roberto San Jose, Donna Schwede, Sam Silva, and Ralf Wolke
Atmos. Chem. Phys., 21, 15663–15697, https://doi.org/10.5194/acp-21-15663-2021, https://doi.org/10.5194/acp-21-15663-2021, 2021
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This technical note presents the research protocols for phase 4 of the Air Quality Model Evaluation International Initiative (AQMEII4). This initiative has three goals: (i) to define the state of wet and dry deposition in regional models, (ii) to evaluate how dry deposition influences air concentration and flux predictions, and (iii) to identify the causes for prediction differences. The evaluation compares LULC-specific dry deposition and effective conductances and fluxes.
Carola Detring, Annette Müller, Lisa Schielicke, Peter Névir, and Henning W. Rust
Weather Clim. Dynam., 2, 927–952, https://doi.org/10.5194/wcd-2-927-2021, https://doi.org/10.5194/wcd-2-927-2021, 2021
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Stationary, long-lasting blocked weather patterns can lead to extreme conditions. Within this study the temporal evolution of the occurrence probability is analyzed, and the onset, decay and transition probabilities of blocking within the past 30 years are modeled. Using Markov models combined with logistic regression, we found large changes in summer, where the probability of transitions to so-called Omega blocks increases strongly, while the unblocked state becomes less probable.
Edward C. Chan and Timothy M. Butler
Geosci. Model Dev., 14, 4555–4572, https://doi.org/10.5194/gmd-14-4555-2021, https://doi.org/10.5194/gmd-14-4555-2021, 2021
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A large-eddy simulation based chemical transport model is implemented for an idealized street canyon. The dynamics of the model are evaluated using stationary measurements. A transient model run is also conducted over a 24 h period, where variations of pollutant concentrations indicate dependence on emissions, background concentrations, and solar state. Comparison stationary model runs show changes in flow structure concentrations.
Alexander Pasternack, Jens Grieger, Henning W. Rust, and Uwe Ulbrich
Geosci. Model Dev., 14, 4335–4355, https://doi.org/10.5194/gmd-14-4335-2021, https://doi.org/10.5194/gmd-14-4335-2021, 2021
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Decadal climate ensemble forecasts are increasingly being used to guide adaptation measures. To ensure the applicability of these probabilistic predictions, inherent systematic errors of the prediction system must be adjusted. Since it is not clear which statistical model is optimal for this purpose, we propose a recalibration strategy with a systematic model selection based on non-homogeneous boosting for identifying the most relevant features for both ensemble mean and ensemble spread.
Elena Macdonald, Noelia Otero, and Tim Butler
Atmos. Chem. Phys., 21, 4007–4023, https://doi.org/10.5194/acp-21-4007-2021, https://doi.org/10.5194/acp-21-4007-2021, 2021
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NO2 limit values are still regularly exceeded in many European cities despite decreasing emissions. Measurements of NOx concentrations from stations across Europe were systematically analysed to assess long-term changes observed in urban areas. We compared trends in concentration increments to trends in total and traffic emissions to find potential discrepancies. The results can help in evaluating inaccuracies in emission inventories and in improving spatial imbalances in data availability.
Nico Becker, Henning W. Rust, and Uwe Ulbrich
Nat. Hazards Earth Syst. Sci., 20, 2857–2871, https://doi.org/10.5194/nhess-20-2857-2020, https://doi.org/10.5194/nhess-20-2857-2020, 2020
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Short summary
A set of models is developed to forecast hourly probabilities of weather-related road accidents in Germany at the spatial scale of administrative districts. Model verification shows that using precipitation and temperature data leads to the best accident forecasts. Based on weather forecast data we show that skilful predictions of accident probabilities of up to 21 h ahead are possible. The models can be used to issue impact-based warnings, which are relevant for road users and authorities.
Tim Butler, Aurelia Lupascu, and Aditya Nalam
Atmos. Chem. Phys., 20, 10707–10731, https://doi.org/10.5194/acp-20-10707-2020, https://doi.org/10.5194/acp-20-10707-2020, 2020
Short summary
Short summary
Ground-level ozone (O3) is not directly emitted; it is formed chemically in the atmosphere. Some ground-level O3 is transported from the stratosphere, but most O3 is produced from reactive precursors that are emitted by both natural and anthropogenic sources. We present the results of a novel source apportionment method for ground-level O3. Our results are consistent with previous work and also provide new insights. In particular, we highlight the roles of methane and international shipping.
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Short summary
Surface ozone and temperature are strongly dependent and their extremes might be exacerbated by underlying climatological drivers, such as atmospheric blocking. Using an observational data set, we measure the dependence structure between ozone and temperature under the influence of atmospheric blocking. Blocks enhanced the probability of occurrence of compound ozone and temperature extremes over northwestern and central Europe, leading to greater health risks.
Surface ozone and temperature are strongly dependent and their extremes might be exacerbated by...
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