Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics
ACP
Articles | Volume 21, issue 20
Articles | Volume 21, issue 20
https://doi.org/10.5194/acp-21-15725-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-15725-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
Articles | Volume 21, issue 20
Technical note
 | 
21 Oct 2021
Technical note |  | 21 Oct 2021

Technical note: Adsorption and desorption equilibria from statistical thermodynamics and rates from transition state theory

Daniel A. Knopf and Markus Ammann

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Short summary
Adsorption on and desorption of gas molecules from solid or liquid surfaces or interfaces represent the initial interaction of gas-to-condensed-phase processes that can define the physicochemical evolution of the condensed phase. We apply a thermodynamic and microscopic treatment of these multiphase processes to evaluate how adsorption and desorption rates and surface accommodation depend on the choice of adsorption model and standard states with implications for desorption energy and lifetimes.
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