Articles | Volume 21, issue 20
Atmos. Chem. Phys., 21, 15725–15753, 2021
https://doi.org/10.5194/acp-21-15725-2021
Atmos. Chem. Phys., 21, 15725–15753, 2021
https://doi.org/10.5194/acp-21-15725-2021
Technical note
21 Oct 2021
Technical note | 21 Oct 2021

Technical note: Adsorption and desorption equilibria from statistical thermodynamics and rates from transition state theory

Daniel A. Knopf and Markus Ammann

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Latest update: 07 Dec 2022
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Short summary
Adsorption on and desorption of gas molecules from solid or liquid surfaces or interfaces represent the initial interaction of gas-to-condensed-phase processes that can define the physicochemical evolution of the condensed phase. We apply a thermodynamic and microscopic treatment of these multiphase processes to evaluate how adsorption and desorption rates and surface accommodation depend on the choice of adsorption model and standard states with implications for desorption energy and lifetimes.
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