Articles | Volume 19, issue 1
https://doi.org/10.5194/acp-19-459-2019
https://doi.org/10.5194/acp-19-459-2019
Research article
 | 
14 Jan 2019
Research article |  | 14 Jan 2019

Estimation of atmospheric total organic carbon (TOC) – paving the path towards carbon budget closure

Mingxi Yang and Zoë L. Fleming

Related authors

Sea ice concentration impacts dissolved organic gases in the Canadian Arctic
Charel Wohl, Anna E. Jones, William T. Sturges, Philip D. Nightingale, Brent Else, Brian J. Butterworth, and Mingxi Yang
Biogeosciences, 19, 1021–1045, https://doi.org/10.5194/bg-19-1021-2022,https://doi.org/10.5194/bg-19-1021-2022, 2022
Short summary
Opportunistic experiments to constrain aerosol effective radiative forcing
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022,https://doi.org/10.5194/acp-22-641-2022, 2022
Short summary
Air–sea exchange of acetone, acetaldehyde, DMS and isoprene at a UK coastal site
Daniel P. Phillips, Frances E. Hopkins, Thomas G. Bell, Peter S. Liss, Philip D. Nightingale, Claire E. Reeves, Charel Wohl, and Mingxi Yang
Atmos. Chem. Phys., 21, 10111–10132, https://doi.org/10.5194/acp-21-10111-2021,https://doi.org/10.5194/acp-21-10111-2021, 2021
Short summary
Uncertainties in eddy covariance air–sea CO2 flux measurements and implications for gas transfer velocity parameterisations
Yuanxu Dong, Mingxi Yang, Dorothee C. E. Bakker, Vassilis Kitidis, and Thomas G. Bell
Atmos. Chem. Phys., 21, 8089–8110, https://doi.org/10.5194/acp-21-8089-2021,https://doi.org/10.5194/acp-21-8089-2021, 2021
Short summary
Ozone deposition to a coastal sea: comparison of eddy covariance observations with reactive air–sea exchange models
David C. Loades, Mingxi Yang, Thomas G. Bell, Adam R. Vaughan, Ryan J. Pound, Stefan Metzger, James D. Lee, and Lucy J. Carpenter
Atmos. Meas. Tech., 13, 6915–6931, https://doi.org/10.5194/amt-13-6915-2020,https://doi.org/10.5194/amt-13-6915-2020, 2020
Short summary

Related subject area

Subject: Gases | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Measurement report: Molecular-level investigation of atmospheric cluster ions at the tropical high-altitude research station Chacaltaya (5240 m a.s.l.) in the Bolivian Andes
Qiaozhi Zha, Wei Huang, Diego Aliaga, Otso Peräkylä, Liine Heikkinen, Alkuin Maximilian Koenig, Cheng Wu, Joonas Enroth, Yvette Gramlich, Jing Cai, Samara Carbone, Armin Hansel, Tuukka Petäjä, Markku Kulmala, Douglas Worsnop, Victoria Sinclair, Radovan Krejci, Marcos Andrade, Claudia Mohr, and Federico Bianchi
Atmos. Chem. Phys., 23, 4559–4576, https://doi.org/10.5194/acp-23-4559-2023,https://doi.org/10.5194/acp-23-4559-2023, 2023
Short summary
Observations of biogenic volatile organic compounds over a mixed temperate forest during the summer to autumn transition
Michael P. Vermeuel, Gordon A. Novak, Delaney B. Kilgour, Megan S. Claflin, Brian M. Lerner, Amy M. Trowbridge, Jonathan Thom, Patricia A. Cleary, Ankur R. Desai, and Timothy H. Bertram
Atmos. Chem. Phys., 23, 4123–4148, https://doi.org/10.5194/acp-23-4123-2023,https://doi.org/10.5194/acp-23-4123-2023, 2023
Short summary
Unexpectedly high concentrations of atmospheric mercury species in Lhasa, the largest city in the Tibetan Plateau
Huiming Lin, Yindong Tong, Long Chen, Chenghao Yu, Zhaohan Chu, Qianru Zhang, Xiufeng Yin, Qianggong Zhang, Shichang Kang, Junfeng Liu, James Schauer, Benjamin de Foy, and Xuejun Wang
Atmos. Chem. Phys., 23, 3937–3953, https://doi.org/10.5194/acp-23-3937-2023,https://doi.org/10.5194/acp-23-3937-2023, 2023
Short summary
Real-time measurements of non-methane volatile organic compounds in the central Indo-Gangetic basin, Lucknow, India: source characterisation and their role in O3 and secondary organic aerosol formation
Vaishali Jain, Nidhi Tripathi, Sachchida N. Tripathi, Mansi Gupta, Lokesh K. Sahu, Vishnu Murari, Sreenivas Gaddamidi, Ashutosh K. Shukla, and Andre S. H. Prevot
Atmos. Chem. Phys., 23, 3383–3408, https://doi.org/10.5194/acp-23-3383-2023,https://doi.org/10.5194/acp-23-3383-2023, 2023
Short summary
Measurement report: Production and loss of atmospheric formaldehyde at a suburban site of Shanghai in summertime
Yizhen Wu, Juntao Huo, Gan Yang, Yuwei Wang, Lihong Wang, Shijian Wu, Lei Yao, Qingyan Fu, and Lin Wang
Atmos. Chem. Phys., 23, 2997–3014, https://doi.org/10.5194/acp-23-2997-2023,https://doi.org/10.5194/acp-23-2997-2023, 2023
Short summary

Cited articles

Ammoura, L., Xueref-Remy, I., Gros, V., Baudic, A., Bonsang, B., Petit, J.-E., Perrussel, O., Bonnaire, N., Sciare, J., and Chevallier, F.: Atmospheric measurements of ratios between CO2 and co-emitted species from traffic: a tunnel study in the Paris megacity, Atmos. Chem. Phys., 14, 12871–12882, https://doi.org/10.5194/acp-14-12871-2014, 2014. 
Andreae, M. O. and Merlet, P.: Emission of trace gases and aerosols from biomass burning, Global Biogeochem. Cy., 15, 955–966, https://doi.org/10.1029/2000GB001382, 2001. 
Chung, M. Y., Maris, C., Krischke, U., Ho, A. W., and Paulson, S. E.: An investigation of the relationship between total non-methane organic carbon and the sum of speciated hydrocarbons and carbonyls measured by standard GC/FID: measurements in the Los Angeles air basin, Atmos. Environ., 37, 159–170, https://doi.org/10.1016/S1352-2310(03)00388-1, 2003. 
Dachs, J., Calleja, M. L., Duarte, C. M., Del Vento, S., Turpin, B., Polidori, A., Herndl, G. J., and Agustí, S.: High atmosphere-ocean exchange of organic carbon in the NE subtropical Atlantic, Geophys. Res. Lett., 32, L21807, https://doi.org/10.1029/2005GL023799, 2005. 
Forster, G. L., Upstill-Goddard, R. C., Gist, N., Robinson, R., Uher, G., and Woodward, E. M. S.: Nitrous oxide and methane in the Atlantic Ocean between 501N and 521S: Latitudinal distribution and sea-to-air flux, Deep-Sea Res. Pt. II, 56, 964–976, https://doi.org/10.1016/j.dsr2.2008.12.002, 2009. 
Download
Short summary
The atmosphere contains thousands of different organic compounds but the quantification of their total burden has been a technical challenge. This hinders our understanding in atmospheric chemistry, air pollution, and global carbon cycling. Here we present a novel and robust method to measure total atmospheric organic carbon. By comparing the total organic carbon concentration in marine air to the sum of speciated organic measurements, we aim to estimate the pool of undetected organic species.
Altmetrics
Final-revised paper
Preprint