Articles | Volume 18, issue 6
https://doi.org/10.5194/acp-18-3937-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-3937-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Mar 2018
Research article |
| 20 Mar 2018
| 20 Mar 2018
Secondary sulfate is internally mixed with sea spray aerosol and organic aerosol in the winter Arctic
Rachel M. Kirpes
Department of Chemistry, University of Michigan, Ann Arbor, Michigan, USA
Amy L. Bondy
Department of Chemistry, University of Michigan, Ann Arbor, Michigan, USA
Daniel Bonanno
Department of Chemistry, University of the Pacific, Stockton, California, USA
Ryan C. Moffet
Department of Chemistry, University of the Pacific, Stockton, California, USA
currently at: Sonoma Technology, Petaluma, California, USA
Bingbing Wang
Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, Washington, USA
State Key Lab of Marine and Environmental Science & College of Ocean and Earth Sciences, Xiamen University, Xiamen, China
Alexander Laskin
Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, Washington, USA
currently at: Department of Chemistry, Purdue University, West Lafayette, Indiana, USA
Department of Chemistry, University of Michigan, Ann Arbor, Michigan, USA
Department of Environmental Health Sciences, University of Michigan, Ann Arbor, Michigan, USA
Department of Chemistry, University of Michigan, Ann Arbor, Michigan, USA
Department of Earth & Environmental Sciences, University of Michigan, Ann Arbor, Michigan, USA
Viewed
Total article views: 4,665 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 01 Nov 2017)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 3,351 | 1,237 | 77 | 4,665 | 356 | 61 | 110 |
- HTML: 3,351
- PDF: 1,237
- XML: 77
- Total: 4,665
- Supplement: 356
- BibTeX: 61
- EndNote: 110
Total article views: 3,983 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 20 Mar 2018)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,948 | 968 | 67 | 3,983 | 216 | 58 | 100 |
- HTML: 2,948
- PDF: 968
- XML: 67
- Total: 3,983
- Supplement: 216
- BibTeX: 58
- EndNote: 100
Total article views: 682 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 01 Nov 2017)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 403 | 269 | 10 | 682 | 140 | 3 | 10 |
- HTML: 403
- PDF: 269
- XML: 10
- Total: 682
- Supplement: 140
- BibTeX: 3
- EndNote: 10
Viewed (geographical distribution)
Total article views: 4,665 (including HTML, PDF, and XML)
Thereof 4,660 with geography defined
and 5 with unknown origin.
Total article views: 3,983 (including HTML, PDF, and XML)
Thereof 3,984 with geography defined
and -1 with unknown origin.
Total article views: 682 (including HTML, PDF, and XML)
Thereof 676 with geography defined
and 6 with unknown origin.
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
Cited
54 citations as recorded by crossref.
- Probing Individual Particles Generated at the Freshwater–Seawater Interface through Combined Raman, Photothermal Infrared, and X-ray Spectroscopic Characterization J. Mirrielees et al. 10.1021/acsmeasuresciau.2c00041
- Characteristics of CCN activation and cloud microphysics over the east coast of India during the Northeast Monsoon onset M. Varghese et al. 10.1016/j.atmosres.2021.105589
- Sulfate Formation by Photosensitization in Mixed Incense Burning–Sodium Chloride Particles: Effects of RH, Light Intensity, and Aerosol Aging R. Tang et al. 10.1021/acs.est.3c02225
- Atmospheric nanoparticles hygroscopic growth measurement by a combined surface plasmon resonance microscope and hygroscopic tandem differential mobility analyzer Z. Xie et al. 10.5194/acp-23-2079-2023
- Differentiation of coarse-mode anthropogenic, marine and dust particles in the High Arctic islands of Svalbard C. Song et al. 10.5194/acp-21-11317-2021
- Enrichment of submicron sea-salt-containing particles in small cloud droplets based on single-particle mass spectrometry Q. Lin et al. 10.5194/acp-19-10469-2019
- Simultaneous Optical Photothermal Infrared (O-PTIR) and Raman Spectroscopy of Submicrometer Atmospheric Particles N. Olson et al. 10.1021/acs.analchem.0c01495
- Organosulfate Formation in Proxies for Aged Sea Spray Aerosol: Reactive Uptake of Isoprene Epoxydiols to Acidic Sodium Sulfate M. Cooke et al. 10.1021/acsearthspacechem.2c00156
- Overview paper: New insights into aerosol and climate in the Arctic J. Abbatt et al. 10.5194/acp-19-2527-2019
- Impact of the particle mixing state on the hygroscopicity of internally mixed sodium chloride–ammonium sulfate single droplets: a theoretical and experimental study Y. Tobon et al. 10.1039/D1CP01574E
- Marine carbohydrates in Arctic aerosol particles and fog – diversity of oceanic sources and atmospheric transformations S. Zeppenfeld et al. 10.5194/acp-23-15561-2023
- Microphysical and thermodynamic phase analyses of Arctic low-level clouds measured above the sea ice and the open ocean in spring and summer M. Moser et al. 10.5194/acp-23-7257-2023
- Existence of Crystalline Ammonium Sulfate Nuclei Affects Chemical Reactivity of Oleic Acid Particles Through Heterogeneous Nucleation W. Liu et al. 10.1029/2023JD038675
- Analysis of insoluble particles in hailstones in China H. Zhang et al. 10.5194/acp-23-13957-2023
- Untargeted Exometabolomics Provides a Powerful Approach to Investigate Biogeochemical Hotspots with Vegetation and Polygon Type in Arctic Tundra Soils M. Ladd et al. 10.3390/soilsystems5010010
- The acidity of atmospheric particles and clouds H. Pye et al. 10.5194/acp-20-4809-2020
- Emerging investigator series: influence of marine emissions and atmospheric processing on individual particle composition of summertime Arctic aerosol over the Bering Strait and Chukchi Sea R. Kirpes et al. 10.1039/C9EM00495E
- Contemporary sources dominate carbonaceous aerosol on the North Slope of Alaska C. Moffett et al. 10.1016/j.scitotenv.2022.154641
- The diverse chemical mixing state of aerosol particles in the southeastern United States A. Bondy et al. 10.5194/acp-18-12595-2018
- Comparison of operator- and computer-controlled scanning electron microscopy of particles from different atmospheric aerosol types S. Eriksen Hammer et al. 10.1007/s00216-019-01614-7
- Source apportionment of marine atmospheric aerosols in northern South China Sea during summertime 2018 B. Liang et al. 10.1016/j.envpol.2021.117948
- 基于薄膜光场调控的无标记显微成像、传感及其应用研究进展（特邀） 张. Zhang Douguo 10.3788/LOP231869
- Lake Spray Aerosol Incorporated into Great Lakes Clouds N. Olson et al. 10.1021/acsearthspacechem.9b00258
- Comparison of Different Vibrational Spectroscopic Probes (ATR-FTIR, O-PTIR, Micro-Raman, and AFM-IR) of Lipids and Other Compounds Found in Environmental Samples: Case Study of Substrate-Deposited Sea Spray Aerosols C. Molina et al. 10.1021/acsmeasuresciau.4c00033
- Measurement report: High Arctic aerosol hygroscopicity at sub- and supersaturated conditions during spring and summer A. Massling et al. 10.5194/acp-23-4931-2023
- Equal abundance of summertime natural and wintertime anthropogenic Arctic organic aerosols V. Moschos et al. 10.1038/s41561-021-00891-1
- Composition and mixing state of Arctic aerosol and cloud residual particles from long-term single-particle observations at Zeppelin Observatory, Svalbard K. Adachi et al. 10.5194/acp-22-14421-2022
- Local Arctic Air Pollution: A Neglected but Serious Problem J. Schmale et al. 10.1029/2018EF000952
- Aircraft-based measurements of High Arctic springtime aerosol show evidence for vertically varying sources, transport and composition M. Willis et al. 10.5194/acp-19-57-2019
- Sulfur aerosols in the Arctic, Antarctic, and Tibetan Plateau: Current knowledge and future perspectives Q. Pei et al. 10.1016/j.earscirev.2021.103753
- Indirect Measurements of the Composition of Ultrafine Particles in the Arctic Late‐Winter D. Myers et al. 10.1029/2021JD035428
- Atmospheric Aerosol Sulfur Distribution and Speciation in Mexico City: Sulfate, Organosulfates, and Isoprene-Derived Secondary Organic Aerosol from Low NO Pathways M. Cooke et al. 10.1021/acsestair.4c00048
- Biomass burning and marine aerosol processing over the southeast Atlantic Ocean: a TEM single-particle analysis C. Dang et al. 10.5194/acp-22-9389-2022
- Future warming exacerbated by aged-soot effect on cloud formation U. Lohmann et al. 10.1038/s41561-020-0631-0
- Atmospheric fates of SO2 at the gas–solid interface of iron oxyhydroxide (FeOOH) minerals: effects of crystal structure, oxalate coating and light irradiance W. Wang et al. 10.1039/D2EN00874B
- Molecular and physical characteristics of aerosol at a remote free troposphere site: implications for atmospheric aging S. Schum et al. 10.5194/acp-18-14017-2018
- Wintertime Arctic Sea Spray Aerosol Composition Controlled by Sea Ice Lead Microbiology R. Kirpes et al. 10.1021/acscentsci.9b00541
- Overview of the Alaskan Layered Pollution and Chemical Analysis (ALPACA) Field Experiment W. Simpson et al. 10.1021/acsestair.3c00076
- Processes Controlling the Composition and Abundance of Arctic Aerosol M. Willis et al. 10.1029/2018RG000602
- Arctic Reactive Bromine Events Occur in Two Distinct Sets of Environmental Conditions: A Statistical Analysis of 6 Years of Observations W. Swanson et al. 10.1029/2019JD032139
- Modelling wintertime sea-spray aerosols under Arctic haze conditions E. Ioannidis et al. 10.5194/acp-23-5641-2023
- A Review of the Representation of Aerosol Mixing State in Atmospheric Models R. Stevens & A. Dastoor 10.3390/atmos10040168
- Overview: Integrative and Comprehensive Understanding on Polar Environments (iCUPE) – concept and initial results T. Petäjä et al. 10.5194/acp-20-8551-2020
- Seasonal dynamics of airborne biomolecules influence the size distribution of Arctic aerosols E. Jang et al. 10.1016/j.ese.2024.100458
- Morphology and Viscosity Changes after Reactive Uptake of Isoprene Epoxydiols in Submicrometer Phase Separated Particles with Secondary Organic Aerosol Formed from Different Volatile Organic Compounds Z. Lei et al. 10.1021/acsearthspacechem.1c00156
- Atmospheric particle abundance and sea salt aerosol observations in the springtime Arctic: a focus on blowing snow and leads Q. Chen et al. 10.5194/acp-22-15263-2022
- Anthropogenic sources and liquid water drive secondary organic aerosol formation over the eastern Himalaya D. Kumar et al. 10.1016/j.scitotenv.2024.175072
- Spontaneous Water Radical Cation Oxidation at Double Bonds in Microdroplets L. Qiu et al. 10.3389/fchem.2022.903774
- Aircraft ice-nucleating particle and aerosol composition measurements in the western North American Arctic A. Sanchez-Marroquin et al. 10.5194/acp-23-13819-2023
- Marine and terrestrial influences on ice nucleating particles during continuous springtime measurements in an Arctic oilfield location J. Creamean et al. 10.5194/acp-18-18023-2018
- Aerosol Mixing State: Measurements, Modeling, and Impacts N. Riemer et al. 10.1029/2018RG000615
- Chemical composition and source attribution of sub-micrometre aerosol particles in the summertime Arctic lower troposphere F. Köllner et al. 10.5194/acp-21-6509-2021
- Organic coating on sulfate and soot particles during late summer in the Svalbard Archipelago H. Yu et al. 10.5194/acp-19-10433-2019
- Temporal variations, transport, and regional impacts of atmospheric aerosol and acid gases close to an oil and gas trading hub K. Francisco et al. 10.1007/s13762-022-04341-2
54 citations as recorded by crossref.
- Probing Individual Particles Generated at the Freshwater–Seawater Interface through Combined Raman, Photothermal Infrared, and X-ray Spectroscopic Characterization J. Mirrielees et al. 10.1021/acsmeasuresciau.2c00041
- Characteristics of CCN activation and cloud microphysics over the east coast of India during the Northeast Monsoon onset M. Varghese et al. 10.1016/j.atmosres.2021.105589
- Sulfate Formation by Photosensitization in Mixed Incense Burning–Sodium Chloride Particles: Effects of RH, Light Intensity, and Aerosol Aging R. Tang et al. 10.1021/acs.est.3c02225
- Atmospheric nanoparticles hygroscopic growth measurement by a combined surface plasmon resonance microscope and hygroscopic tandem differential mobility analyzer Z. Xie et al. 10.5194/acp-23-2079-2023
- Differentiation of coarse-mode anthropogenic, marine and dust particles in the High Arctic islands of Svalbard C. Song et al. 10.5194/acp-21-11317-2021
- Enrichment of submicron sea-salt-containing particles in small cloud droplets based on single-particle mass spectrometry Q. Lin et al. 10.5194/acp-19-10469-2019
- Simultaneous Optical Photothermal Infrared (O-PTIR) and Raman Spectroscopy of Submicrometer Atmospheric Particles N. Olson et al. 10.1021/acs.analchem.0c01495
- Organosulfate Formation in Proxies for Aged Sea Spray Aerosol: Reactive Uptake of Isoprene Epoxydiols to Acidic Sodium Sulfate M. Cooke et al. 10.1021/acsearthspacechem.2c00156
- Overview paper: New insights into aerosol and climate in the Arctic J. Abbatt et al. 10.5194/acp-19-2527-2019
- Impact of the particle mixing state on the hygroscopicity of internally mixed sodium chloride–ammonium sulfate single droplets: a theoretical and experimental study Y. Tobon et al. 10.1039/D1CP01574E
- Marine carbohydrates in Arctic aerosol particles and fog – diversity of oceanic sources and atmospheric transformations S. Zeppenfeld et al. 10.5194/acp-23-15561-2023
- Microphysical and thermodynamic phase analyses of Arctic low-level clouds measured above the sea ice and the open ocean in spring and summer M. Moser et al. 10.5194/acp-23-7257-2023
- Existence of Crystalline Ammonium Sulfate Nuclei Affects Chemical Reactivity of Oleic Acid Particles Through Heterogeneous Nucleation W. Liu et al. 10.1029/2023JD038675
- Analysis of insoluble particles in hailstones in China H. Zhang et al. 10.5194/acp-23-13957-2023
- Untargeted Exometabolomics Provides a Powerful Approach to Investigate Biogeochemical Hotspots with Vegetation and Polygon Type in Arctic Tundra Soils M. Ladd et al. 10.3390/soilsystems5010010
- The acidity of atmospheric particles and clouds H. Pye et al. 10.5194/acp-20-4809-2020
- Emerging investigator series: influence of marine emissions and atmospheric processing on individual particle composition of summertime Arctic aerosol over the Bering Strait and Chukchi Sea R. Kirpes et al. 10.1039/C9EM00495E
- Contemporary sources dominate carbonaceous aerosol on the North Slope of Alaska C. Moffett et al. 10.1016/j.scitotenv.2022.154641
- The diverse chemical mixing state of aerosol particles in the southeastern United States A. Bondy et al. 10.5194/acp-18-12595-2018
- Comparison of operator- and computer-controlled scanning electron microscopy of particles from different atmospheric aerosol types S. Eriksen Hammer et al. 10.1007/s00216-019-01614-7
- Source apportionment of marine atmospheric aerosols in northern South China Sea during summertime 2018 B. Liang et al. 10.1016/j.envpol.2021.117948
- 基于薄膜光场调控的无标记显微成像、传感及其应用研究进展（特邀） 张. Zhang Douguo 10.3788/LOP231869
- Lake Spray Aerosol Incorporated into Great Lakes Clouds N. Olson et al. 10.1021/acsearthspacechem.9b00258
- Comparison of Different Vibrational Spectroscopic Probes (ATR-FTIR, O-PTIR, Micro-Raman, and AFM-IR) of Lipids and Other Compounds Found in Environmental Samples: Case Study of Substrate-Deposited Sea Spray Aerosols C. Molina et al. 10.1021/acsmeasuresciau.4c00033
- Measurement report: High Arctic aerosol hygroscopicity at sub- and supersaturated conditions during spring and summer A. Massling et al. 10.5194/acp-23-4931-2023
- Equal abundance of summertime natural and wintertime anthropogenic Arctic organic aerosols V. Moschos et al. 10.1038/s41561-021-00891-1
- Composition and mixing state of Arctic aerosol and cloud residual particles from long-term single-particle observations at Zeppelin Observatory, Svalbard K. Adachi et al. 10.5194/acp-22-14421-2022
- Local Arctic Air Pollution: A Neglected but Serious Problem J. Schmale et al. 10.1029/2018EF000952
- Aircraft-based measurements of High Arctic springtime aerosol show evidence for vertically varying sources, transport and composition M. Willis et al. 10.5194/acp-19-57-2019
- Sulfur aerosols in the Arctic, Antarctic, and Tibetan Plateau: Current knowledge and future perspectives Q. Pei et al. 10.1016/j.earscirev.2021.103753
- Indirect Measurements of the Composition of Ultrafine Particles in the Arctic Late‐Winter D. Myers et al. 10.1029/2021JD035428
- Atmospheric Aerosol Sulfur Distribution and Speciation in Mexico City: Sulfate, Organosulfates, and Isoprene-Derived Secondary Organic Aerosol from Low NO Pathways M. Cooke et al. 10.1021/acsestair.4c00048
- Biomass burning and marine aerosol processing over the southeast Atlantic Ocean: a TEM single-particle analysis C. Dang et al. 10.5194/acp-22-9389-2022
- Future warming exacerbated by aged-soot effect on cloud formation U. Lohmann et al. 10.1038/s41561-020-0631-0
- Atmospheric fates of SO2 at the gas–solid interface of iron oxyhydroxide (FeOOH) minerals: effects of crystal structure, oxalate coating and light irradiance W. Wang et al. 10.1039/D2EN00874B
- Molecular and physical characteristics of aerosol at a remote free troposphere site: implications for atmospheric aging S. Schum et al. 10.5194/acp-18-14017-2018
- Wintertime Arctic Sea Spray Aerosol Composition Controlled by Sea Ice Lead Microbiology R. Kirpes et al. 10.1021/acscentsci.9b00541
- Overview of the Alaskan Layered Pollution and Chemical Analysis (ALPACA) Field Experiment W. Simpson et al. 10.1021/acsestair.3c00076
- Processes Controlling the Composition and Abundance of Arctic Aerosol M. Willis et al. 10.1029/2018RG000602
- Arctic Reactive Bromine Events Occur in Two Distinct Sets of Environmental Conditions: A Statistical Analysis of 6 Years of Observations W. Swanson et al. 10.1029/2019JD032139
- Modelling wintertime sea-spray aerosols under Arctic haze conditions E. Ioannidis et al. 10.5194/acp-23-5641-2023
- A Review of the Representation of Aerosol Mixing State in Atmospheric Models R. Stevens & A. Dastoor 10.3390/atmos10040168
- Overview: Integrative and Comprehensive Understanding on Polar Environments (iCUPE) – concept and initial results T. Petäjä et al. 10.5194/acp-20-8551-2020
- Seasonal dynamics of airborne biomolecules influence the size distribution of Arctic aerosols E. Jang et al. 10.1016/j.ese.2024.100458
- Morphology and Viscosity Changes after Reactive Uptake of Isoprene Epoxydiols in Submicrometer Phase Separated Particles with Secondary Organic Aerosol Formed from Different Volatile Organic Compounds Z. Lei et al. 10.1021/acsearthspacechem.1c00156
- Atmospheric particle abundance and sea salt aerosol observations in the springtime Arctic: a focus on blowing snow and leads Q. Chen et al. 10.5194/acp-22-15263-2022
- Anthropogenic sources and liquid water drive secondary organic aerosol formation over the eastern Himalaya D. Kumar et al. 10.1016/j.scitotenv.2024.175072
- Spontaneous Water Radical Cation Oxidation at Double Bonds in Microdroplets L. Qiu et al. 10.3389/fchem.2022.903774
- Aircraft ice-nucleating particle and aerosol composition measurements in the western North American Arctic A. Sanchez-Marroquin et al. 10.5194/acp-23-13819-2023
- Marine and terrestrial influences on ice nucleating particles during continuous springtime measurements in an Arctic oilfield location J. Creamean et al. 10.5194/acp-18-18023-2018
- Aerosol Mixing State: Measurements, Modeling, and Impacts N. Riemer et al. 10.1029/2018RG000615
- Chemical composition and source attribution of sub-micrometre aerosol particles in the summertime Arctic lower troposphere F. Köllner et al. 10.5194/acp-21-6509-2021
- Organic coating on sulfate and soot particles during late summer in the Svalbard Archipelago H. Yu et al. 10.5194/acp-19-10433-2019
- Temporal variations, transport, and regional impacts of atmospheric aerosol and acid gases close to an oil and gas trading hub K. Francisco et al. 10.1007/s13762-022-04341-2
Saved (final revised paper)
Discussed (final revised paper)
Latest update: 14 Dec 2024
Short summary
Arctic atmospheric particles have important climate impacts via cloud formation and precipitation, particularly in the wintertime. We show that sulfate, formed during atmospheric transport, is within individual sea spray particles and organic particles measured in the Alaskan Arctic. Greater contributions of combustion emissions were observed when the wind direction came from the Prudhoe Bay oil fields, showing its regional influence.
Arctic atmospheric particles have important climate impacts via cloud formation and...
Altmetrics
Final-revised paper
Preprint