Articles | Volume 25, issue 6
https://doi.org/10.5194/acp-25-3785-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-25-3785-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Microphysics regimes due to haze–cloud interactions: cloud oscillation and cloud collapse
Brookhaven National Laboratory, Upton, New York, USA
Hamed Fahandezh Sadi
Department of Physics, Michigan Technological University, Houghton, Michigan, USA
Raymond A. Shaw
Department of Physics, Michigan Technological University, Houghton, Michigan, USA
Fabian Hoffmann
Meteorologisches Institut, Ludwig-Maximilians-Universität München, Munich, Germany
Department of Physics, Michigan Technological University, Houghton, Michigan, USA
Department of Geological and Mining Engineering and Sciences, Michigan Technological University, Houghton, Michigan, USA
Aaron Wang
Pacific Northwest National Laboratory, Richland, Washington, USA
Mikhail Ovchinnikov
Pacific Northwest National Laboratory, Richland, Washington, USA
Related authors
Zeen Zhu, Fan Yang, Steven Krueger, and Yangang Liu
EGUsphere, https://doi.org/10.5194/egusphere-2025-3489, https://doi.org/10.5194/egusphere-2025-3489, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
To better understand cloud behavior, we used computer simulations to study how the air mix in clouds. Our results show that the pattern of mixing seen from aircraft measurements may not reflect the true mixing process happening inside clouds. This result suggests that care is needed when using aircraft data to study the cloud mixing process and that new ways of observing clouds could offer clearer insights.
Jialin Yan, Mariko Oue, Pavlos Kollias, Edward Luke, and Fan Yang
EGUsphere, https://doi.org/10.5194/egusphere-2025-2149, https://doi.org/10.5194/egusphere-2025-2149, 2025
Short summary
Short summary
In this study, we analyzed over six years of ground-based radar and weather balloon data collected in northern Alaska. We found that ice particle changes depend strongly on temperature, humidity conditions and turbulence. We also found that turbulence and the presence of supercooled liquid water often occur together, and when they do, ice particle growth is especially strong. These findings help scientists to improve weather models.
Zeen Zhu, Fan Yang, Pavlos Kollias, Raymond A. Shaw, Alex B. Kostinski, Steve Krueger, Katia Lamer, Nithin Allwayin, and Mariko Oue
Atmos. Meas. Tech., 17, 1133–1143, https://doi.org/10.5194/amt-17-1133-2024, https://doi.org/10.5194/amt-17-1133-2024, 2024
Short summary
Short summary
In this article, we demonstrate the feasibility of applying advanced radar technology to detect liquid droplets generated in the cloud chamber. Specifically, we show that using radar with centimeter-scale resolution, single drizzle drops with a diameter larger than 40 µm can be detected. This study demonstrates the applicability of remote sensing instruments in laboratory experiments and suggests new applications of ultrahigh-resolution radar for atmospheric sensing.
Damao Zhang, Andrew M. Vogelmann, Fan Yang, Edward Luke, Pavlos Kollias, Zhien Wang, Peng Wu, William I. Gustafson Jr., Fan Mei, Susanne Glienke, Jason Tomlinson, and Neel Desai
Atmos. Meas. Tech., 16, 5827–5846, https://doi.org/10.5194/amt-16-5827-2023, https://doi.org/10.5194/amt-16-5827-2023, 2023
Short summary
Short summary
Cloud droplet number concentration can be retrieved from remote sensing measurements. Aircraft measurements are used to validate four ground-based retrievals of cloud droplet number concentration. We demonstrate that retrieved cloud droplet number concentrations align well with aircraft measurements for overcast clouds, but they may substantially differ for broken clouds. The ensemble of various retrievals can help quantify retrieval uncertainties and identify reliable retrieval scenarios.
Zeen Zhu, Pavlos Kollias, and Fan Yang
Atmos. Meas. Tech., 16, 3727–3737, https://doi.org/10.5194/amt-16-3727-2023, https://doi.org/10.5194/amt-16-3727-2023, 2023
Short summary
Short summary
We show that large rain droplets, with large inertia, are unable to follow the rapid change of velocity field in a turbulent environment. A lack of consideration for this inertial effect leads to an artificial broadening of the Doppler spectrum from the conventional simulator. Based on the physics-based simulation, we propose a new approach to generate the radar Doppler spectra. This simulator provides a valuable tool to decode cloud microphysical and dynamical properties from radar observation.
Zeen Zhu, Pavlos Kollias, Edward Luke, and Fan Yang
Atmos. Chem. Phys., 22, 7405–7416, https://doi.org/10.5194/acp-22-7405-2022, https://doi.org/10.5194/acp-22-7405-2022, 2022
Short summary
Short summary
Drizzle (small rain droplets) is an important component of warm clouds; however, its existence is poorly understood. In this study, we capitalized on a machine-learning algorithm to develop a drizzle detection method. We applied this algorithm to investigate drizzle occurrence and found out that drizzle is far more ubiquitous than previously thought. This study demonstrates the ubiquitous nature of drizzle in clouds and will improve understanding of the associated microphysical process.
Fabian Hoffmann, Yao-Sheng Chen, and Graham Feingold
Atmos. Chem. Phys., 25, 8657–8670, https://doi.org/10.5194/acp-25-8657-2025, https://doi.org/10.5194/acp-25-8657-2025, 2025
Short summary
Short summary
Clouds reflect a substantial portion of the incoming solar radiation back into space. This capacity is determined by the number of cloud droplets, which in turn is influenced by the number of aerosol particles, forming the basis for aerosol–cloud–climate interactions. In this study, we use a simple entrainment parameterization to understand the effect of aerosol on cloud water in weakly and non-precipitating stratocumulus.
Zeen Zhu, Fan Yang, Steven Krueger, and Yangang Liu
EGUsphere, https://doi.org/10.5194/egusphere-2025-3489, https://doi.org/10.5194/egusphere-2025-3489, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
To better understand cloud behavior, we used computer simulations to study how the air mix in clouds. Our results show that the pattern of mixing seen from aircraft measurements may not reflect the true mixing process happening inside clouds. This result suggests that care is needed when using aircraft data to study the cloud mixing process and that new ways of observing clouds could offer clearer insights.
Prasanth Prabhakaran, Timothy A. Myers, Fabian Hoffmann, and Graham Feingold
EGUsphere, https://doi.org/10.5194/egusphere-2025-2935, https://doi.org/10.5194/egusphere-2025-2935, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
We explore how climate change and aerosol affect the evolution of marine low-clouds. Using high-resolution simulations, we find that warming has a stronger impact on these clouds, but aerosol becomes more important after the clouds form precipitation. Our results suggest that attempts to brighten these clouds using aerosol may become less effective in a warmer future due to the decrease in cloud cover.
Yao-Sheng Chen, Prasanth Prabhakaran, Fabian Hoffmann, Jan Kazil, Takanobu Yamaguchi, and Graham Feingold
Atmos. Chem. Phys., 25, 6141–6159, https://doi.org/10.5194/acp-25-6141-2025, https://doi.org/10.5194/acp-25-6141-2025, 2025
Short summary
Short summary
Injecting sea salt aerosols into marine stratiform clouds can distribute the cloud water over more droplets in smaller sizes. This process is expected to make the clouds brighter, allowing them to reflect more sunlight back to space. However, it may also cause the clouds to lose water over time, reducing their ability to reflect sunlight. We use a computer model to show that the loss of cloud water occurs relatively quickly and does not completely offset the initial brightening.
Robert Grosz, Kamal Kant Chandrakar, Raymond A. Shaw, Jesse C. Anderson, Will Cantrell, and Szymon P. Malinowski
Atmos. Meas. Tech., 18, 2619–2638, https://doi.org/10.5194/amt-18-2619-2025, https://doi.org/10.5194/amt-18-2619-2025, 2025
Short summary
Short summary
Our objective was to enhance understanding of thermally driven convection in terms of small-scale variations in the temperature scalar field. We conducted a small-scale study of the temperature field in the Π Chamber using three different temperature differences (10 K, 15 K, and 20 K). Measurements were carried out using a miniaturized UltraFast Thermometer operating at 2 kHz, allowing undisturbed vertical temperature profiling from 8 cm above the floor to 5 cm below the ceiling.
Jialin Yan, Mariko Oue, Pavlos Kollias, Edward Luke, and Fan Yang
EGUsphere, https://doi.org/10.5194/egusphere-2025-2149, https://doi.org/10.5194/egusphere-2025-2149, 2025
Short summary
Short summary
In this study, we analyzed over six years of ground-based radar and weather balloon data collected in northern Alaska. We found that ice particle changes depend strongly on temperature, humidity conditions and turbulence. We also found that turbulence and the presence of supercooled liquid water often occur together, and when they do, ice particle growth is especially strong. These findings help scientists to improve weather models.
Jung-Sub Lim, Yign Noh, Hyunho Lee, and Fabian Hoffmann
Atmos. Chem. Phys., 25, 5313–5329, https://doi.org/10.5194/acp-25-5313-2025, https://doi.org/10.5194/acp-25-5313-2025, 2025
Short summary
Short summary
Rain formation in warm clouds begins when small droplets collide, but this process can be slow without larger droplets. We used simulations to explore the role of bigger droplets, known as precipitation embryos, in triggering rain. We found that they speed up rain only when their size and number exceed a critical threshold. This threshold becomes larger when collisions are naturally efficient, such as in clouds with broad droplet size distributions or strong turbulence.
Graham Feingold, Franziska Glassmeier, Jianhao Zhang, and Fabian Hoffmann
EGUsphere, https://doi.org/10.5194/egusphere-2025-1869, https://doi.org/10.5194/egusphere-2025-1869, 2025
Short summary
Short summary
Scientists usually use snapshots of atmospheric data to glean understanding of time-evolving atmospheric processes. We examine how much can be learned about processes from snapshots using examples from cloud and atmospheric physics. We couch the analysis in terms of Boltzmann's theory of ergodic systems, space-time-exchange, and the Deborah number -- concepts that are commonly applied in other branches of physics. We discuss the reasons for the varying degrees of success.
Levin Rug, Willi Schimmel, Fabian Hoffmann, and Oswald Knoth
EGUsphere, https://doi.org/10.5194/egusphere-2025-380, https://doi.org/10.5194/egusphere-2025-380, 2025
Short summary
Short summary
We present the Chemical Mechanism Integrator (Cminor) v1.0, a tool to predict concentrations of chemical compounds undergoing arbitrary reactions. Cminor is an advanced, open-source solver to model either combustion chemistry, or atmospheric chemistry and its direct influence on condensation of cloud droplets and the subsequent processing of aerosol. It uses the superdroplet idea, making it particularly feasible for coupling with such models, which is part of future work.
Fabian Hoffmann, Franziska Glassmeier, and Graham Feingold
Atmos. Chem. Phys., 24, 13403–13412, https://doi.org/10.5194/acp-24-13403-2024, https://doi.org/10.5194/acp-24-13403-2024, 2024
Short summary
Short summary
Clouds constitute a major cooling influence on Earth's climate system by reflecting a large fraction of the incident solar radiation back to space. This ability is controlled by the number of cloud droplets, which is governed by the number of aerosol particles in the atmosphere, laying the foundation for so-called aerosol–cloud–climate interactions. In this study, a simple model to understand the effect of aerosol on cloud water is developed and applied.
Yao-Sheng Chen, Jianhao Zhang, Fabian Hoffmann, Takanobu Yamaguchi, Franziska Glassmeier, Xiaoli Zhou, and Graham Feingold
Atmos. Chem. Phys., 24, 12661–12685, https://doi.org/10.5194/acp-24-12661-2024, https://doi.org/10.5194/acp-24-12661-2024, 2024
Short summary
Short summary
Marine stratocumulus cloud is a type of shallow cloud that covers the vast areas of Earth's surface. It plays an important role in Earth's energy balance by reflecting solar radiation back to space. We used numerical models to simulate a large number of marine stratocumuli with different characteristics. We found that how the clouds develop throughout the day is affected by the level of humidity in the air above the clouds and how closely the clouds connect to the ocean surface.
Aaron Wang, Steve Krueger, Sisi Chen, Mikhail Ovchinnikov, Will Cantrell, and Raymond A. Shaw
Atmos. Chem. Phys., 24, 10245–10260, https://doi.org/10.5194/acp-24-10245-2024, https://doi.org/10.5194/acp-24-10245-2024, 2024
Short summary
Short summary
We employ two methods to examine a laboratory experiment on clouds with both ice and liquid phases. The first assumes well-mixed properties; the second resolves the spatial distribution of turbulence and cloud particles. Results show that while the trends in mean properties generally align, when turbulence is resolved, liquid droplets are not fully depleted by ice due to incomplete mixing. This underscores the threshold of ice mass fraction in distinguishing mixed-phase clouds from ice clouds.
Yu Yao, Po-Lun Ma, Yi Qin, Matthew W. Christensen, Hui Wan, Kai Zhang, Balwinder Singh, Meng Huang, and Mikhail Ovchinnikov
EGUsphere, https://doi.org/10.5194/egusphere-2024-523, https://doi.org/10.5194/egusphere-2024-523, 2024
Preprint withdrawn
Short summary
Short summary
Giant aerosols have substantial effects on warm rain formation. However, it remains challenging to quantify the impact of giant particles at global scale. In this work, we applied earth system model to investigate its impacts by implementing new giant aerosol treatments to consider its physical process. We found this approach substantially affect liquid cloud and improved model's precipitation response to aerosols. Our findings demonstrate the significant impact of giant aerosols on climate.
Zeen Zhu, Fan Yang, Pavlos Kollias, Raymond A. Shaw, Alex B. Kostinski, Steve Krueger, Katia Lamer, Nithin Allwayin, and Mariko Oue
Atmos. Meas. Tech., 17, 1133–1143, https://doi.org/10.5194/amt-17-1133-2024, https://doi.org/10.5194/amt-17-1133-2024, 2024
Short summary
Short summary
In this article, we demonstrate the feasibility of applying advanced radar technology to detect liquid droplets generated in the cloud chamber. Specifically, we show that using radar with centimeter-scale resolution, single drizzle drops with a diameter larger than 40 µm can be detected. This study demonstrates the applicability of remote sensing instruments in laboratory experiments and suggests new applications of ultrahigh-resolution radar for atmospheric sensing.
Prasanth Prabhakaran, Fabian Hoffmann, and Graham Feingold
Atmos. Chem. Phys., 24, 1919–1937, https://doi.org/10.5194/acp-24-1919-2024, https://doi.org/10.5194/acp-24-1919-2024, 2024
Short summary
Short summary
In this study, we explore the impact of deliberate aerosol perturbation in the northeast Pacific region using large-eddy simulations. Our results show that cloud reflectivity is sensitive to the aerosol sprayer arrangement in the pristine system, whereas in the polluted system it is largely proportional to the total number of aerosol particles injected. These insights would aid in assessing the efficiency of various aerosol injection strategies for climate intervention applications.
Damao Zhang, Andrew M. Vogelmann, Fan Yang, Edward Luke, Pavlos Kollias, Zhien Wang, Peng Wu, William I. Gustafson Jr., Fan Mei, Susanne Glienke, Jason Tomlinson, and Neel Desai
Atmos. Meas. Tech., 16, 5827–5846, https://doi.org/10.5194/amt-16-5827-2023, https://doi.org/10.5194/amt-16-5827-2023, 2023
Short summary
Short summary
Cloud droplet number concentration can be retrieved from remote sensing measurements. Aircraft measurements are used to validate four ground-based retrievals of cloud droplet number concentration. We demonstrate that retrieved cloud droplet number concentrations align well with aircraft measurements for overcast clouds, but they may substantially differ for broken clouds. The ensemble of various retrievals can help quantify retrieval uncertainties and identify reliable retrieval scenarios.
Elise Rosky, Will Cantrell, Tianshu Li, Issei Nakamura, and Raymond A. Shaw
Atmos. Chem. Phys., 23, 10625–10642, https://doi.org/10.5194/acp-23-10625-2023, https://doi.org/10.5194/acp-23-10625-2023, 2023
Short summary
Short summary
Using computer simulations of water, we find that water under tension freezes more easily than under normal conditions. A linear equation describes how freezing temperature increases with tension. Accordingly, simulations show that naturally occurring tension in water capillary bridges leads to higher freezing temperatures. This work is an early step in determining if atmospheric cloud droplets freeze due to naturally occurring tension, for example, during processes such as droplet collisions.
Zeen Zhu, Pavlos Kollias, and Fan Yang
Atmos. Meas. Tech., 16, 3727–3737, https://doi.org/10.5194/amt-16-3727-2023, https://doi.org/10.5194/amt-16-3727-2023, 2023
Short summary
Short summary
We show that large rain droplets, with large inertia, are unable to follow the rapid change of velocity field in a turbulent environment. A lack of consideration for this inertial effect leads to an artificial broadening of the Doppler spectrum from the conventional simulator. Based on the physics-based simulation, we propose a new approach to generate the radar Doppler spectra. This simulator provides a valuable tool to decode cloud microphysical and dynamical properties from radar observation.
Edward Gryspeerdt, Franziska Glassmeier, Graham Feingold, Fabian Hoffmann, and Rebecca J. Murray-Watson
Atmos. Chem. Phys., 22, 11727–11738, https://doi.org/10.5194/acp-22-11727-2022, https://doi.org/10.5194/acp-22-11727-2022, 2022
Short summary
Short summary
The response of clouds to changes in aerosol remains a large uncertainty in our understanding of the climate. Studies typically look at aerosol and cloud processes in snapshot images, measuring all properties at the same time. Here we use multiple images to characterise how cloud temporal development responds to aerosol. We find a reduction in liquid water path with increasing aerosol, party due to feedbacks. This suggests the aerosol impact on cloud water may be weaker than in previous studies.
Walter Hannah, Kyle Pressel, Mikhail Ovchinnikov, and Gregory Elsaesser
Geosci. Model Dev., 15, 6243–6257, https://doi.org/10.5194/gmd-15-6243-2022, https://doi.org/10.5194/gmd-15-6243-2022, 2022
Short summary
Short summary
An unphysical checkerboard signal is identified in two configurations of the atmospheric component of E3SM. The signal is very persistent and visible after averaging years of data. The signal is very difficult to study because it is often mixed with realistic weather. A method is presented to detect checkerboard patterns and compare the model with satellite observations. The causes of the signal are identified, and a solution for one configuration is discussed.
Zeen Zhu, Pavlos Kollias, Edward Luke, and Fan Yang
Atmos. Chem. Phys., 22, 7405–7416, https://doi.org/10.5194/acp-22-7405-2022, https://doi.org/10.5194/acp-22-7405-2022, 2022
Short summary
Short summary
Drizzle (small rain droplets) is an important component of warm clouds; however, its existence is poorly understood. In this study, we capitalized on a machine-learning algorithm to develop a drizzle detection method. We applied this algorithm to investigate drizzle occurrence and found out that drizzle is far more ubiquitous than previously thought. This study demonstrates the ubiquitous nature of drizzle in clouds and will improve understanding of the associated microphysical process.
Jesse C. Anderson, Subin Thomas, Prasanth Prabhakaran, Raymond A. Shaw, and Will Cantrell
Atmos. Meas. Tech., 14, 5473–5485, https://doi.org/10.5194/amt-14-5473-2021, https://doi.org/10.5194/amt-14-5473-2021, 2021
Short summary
Short summary
Fluctuations due to turbulence in Earth's atmosphere can play a role in how many droplets a cloud has and, eventually, whether that cloud rains or evaporates. We study such processes in Michigan Tech's cloud chamber. Here, we characterize the turbulent and large-scale motions of air in the chamber, measuring the spatial and temporal distributions of temperature and water vapor, which we can combine to get the distribution of relative humidity, which governs cloud formation and dissipation.
Simon Unterstrasser, Fabian Hoffmann, and Marion Lerch
Geosci. Model Dev., 13, 5119–5145, https://doi.org/10.5194/gmd-13-5119-2020, https://doi.org/10.5194/gmd-13-5119-2020, 2020
Short summary
Short summary
Particle-based cloud models use simulation particles for the representation of cloud particles like droplets or ice crystals. The collision and merging of cloud particles (i.e. collisional growth a.k.a. collection in the case of cloud droplets and aggregation in the case of ice crystals) was found to be a numerically challenging process in such models. The study presents verification exercises in a 1D column model, where sedimentation and collisional growth are the only active processes.
Cited articles
Anderson, J. C., Beeler, P., Ovchinnikov, M., Cantrell, W., Krueger, S., Shaw, R. A., Yang, F., and Fierce, L.: Enhancements in cloud condensation nuclei activity from turbulent fluctuations in supersaturation, Geophys. Res. Lett., 50, e2022GL102635, https://doi.org/10.1029/2022GL102635, 2023. a
Arabas, S. and Shima, S.: On the CCN (de)activation nonlinearities, Nonlin. Processes Geophys., 24, 535–542, https://doi.org/10.5194/npg-24-535-2017, 2017. a, b
Baker, M. B. and Charlson, R. J.: Bistability of CCN concentrations and thermodynamics in the cloud-topped boundary layer, Nature, 345, 142–145, https://doi.org/10.1038/345142a0, 1990. a
Boutle, I., Price, J., Kudzotsa, I., Kokkola, H., and Romakkaniemi, S.: Aerosol–fog interaction and the transition to well-mixed radiation fog, Atmos. Chem. Phys., 18, 7827–7840, https://doi.org/10.5194/acp-18-7827-2018, 2018. a
Brown, P. N., Byrne, G. D., and Hindmarsh, A. C.: VODE: A variable-coefficient ODE solver, SIAM journal on scientific and statistical computing, 10, 1038–1051, https://doi.org/10.1137/0910062, 1989. a
Chandrakar, K. K., Cantrell, W., Chang, K., Ciochetto, D., Niedermeier, D., Ovchinnikov, M., Shaw, R. A., and Yang, F.: Aerosol indirect effect from turbulence-induced broadening of cloud-droplet size distributions, P. Natl. Acad. Sci. USA, 113, 14243–14248, https://doi.org/10.1073/pnas.1612686113, 2016. a, b, c
Chang, K., Bench, J., Brege, M., Cantrell, W., Chandrakar, K., Ciochetto, D., Mazzoleni, C., Mazzoleni, L., Niedermeier, D., and Shaw, R.: A laboratory facility to study gas–aerosol–cloud interactions in a turbulent environment: The π chamber, B. Am. Meteorol. Soc., 97, 2343–2358, https://doi.org/10.1175/BAMS-D-15-00203.1, 2016. a
Chen, J., Liu, Y., Zhang, M., and Peng, Y.: New understanding and quantification of the regime dependence of aerosol-cloud interaction for studying aerosol indirect effects, Geophys. Res. Lett., 43, 1780–1787, https://doi.org/10.1002/2016GL067683, 2016. a
Chen, J.-P. and Lamb, D.: Simulation of cloud microphysical and chemical processes using a multicomponent framework. Part I: Description of the microphysical model, J. Atmos. Sci., 51, 2613–2630, https://doi.org/10.1175/1520-0469(1994)051<2613:SOCMAC>2.0.CO;2, 1994. a
Grabowski, W. W.: Comparison of Eulerian bin and Lagrangian particle-based schemes in simulations of Pi Chamber dynamics and microphysics, J. Atmos. Sci., 77, 1151–1165, https://doi.org/10.1175/JAS-D-19-0216.1, 2020. a
Grabowski, W. W., Morrison, H., Shima, S.-I., Abade, G. C., Dziekan, P., and Pawlowska, H.: Modeling of cloud microphysics: Can we do better?, B. Am. Meteorol. Soc., 100, 655–672, https://doi.org/10.1175/BAMS-D-18-0005.1, 2019. a
Gutiérrez, M. S., Chekroun, M. D., and Koren, I.: Dynamical regimes of CCN activation in adiabatic air parcels, arxiv [preprint], https://doi.org/10.48550/arXiv.2405.11545, 2024. a, b
Hoffmann, F.: The effect of spurious cloud edge supersaturations in Lagrangian cloud models: An analytical and numerical study, Mon. Weather Rev., 144, 107–118, https://doi.org/10.1175/MWR-D-15-0234.1, 2016. a
Hoffmann, F., Raasch, S., and Noh, Y.: Entrainment of aerosols and their activation in a shallow cumulus cloud studied with a coupled LCM–LES approach, Atmos. Res., 156, 43–57, https://doi.org/10.1016/j.atmosres.2014.12.008, 2015. a
Hoffmann, F., Mayer, B., and Feingold, G.: A parameterization of interstitial aerosol extinction and its application to marine cloud brightening, J. Atmos. Sci., 79, 2849–2862, https://doi.org/10.1175/JAS-D-22-0047.1, 2022. a
Jensen, J. B. and Nugent, A. D.: Condensational growth of drops formed on giant sea-salt aerosol particles, J. Atmos. Sci., 74, 679–697, https://doi.org/10.1175/JAS-D-15-0370.1, 2017. a
Khairoutdinov, M. F.: System for Atmospheric Modeling (SAM), Stony Brook University [code], http://rossby.msrc.sunysb.edu/SAM.html (last access: 19 March 2024), 2003. a
Khairoutdinov, M. F. and Randall, D. A.: Cloud resolving modeling of the ARM summer 1997 IOP: Model formulation, results, uncertainties, and sensitivities, J. Atmos. Sci., 60, 607–625, https://doi.org/10.1175/1520-0469(2003)060<0607:CRMOTA>2.0.CO;2, 2003. a
Khvorostyanov, V. I. and Curry, J. A.: Refinements to the Köhler's theory of aerosol equilibrium radii, size spectra, and droplet activation: Effects of humidity and insoluble fraction, J. Geophys. Res.-Atmos., 112, D5206, https://doi.org/10.1029/2006JD007672, 2007. a
Klemm, O. and Lin, N. H.: What causes observed fog trends: air quality or climate change?, Aerosol Air Qual. Res., 16, 1131–1142, https://doi.org/10.4209/aaqr.2015.05.0353, 2016. a
Koren, I. and Feingold, G.: Aerosol–cloud–precipitation system as a predator-prey problem, P. Natl. Acad. Sci. USA, 108, 12227–12232, https://doi.org/10.1073/pnas.1101777108, 2011. a
Korolev, A. V.: The influence of supersaturation fluctuations on droplet size spectra formation, J. Atmos. Sci., 52, 3620–3634, https://doi.org/10.1175/1520-0469(1995)052<3620:TIOSFO>2.0.CO;2, 1995. a
Korolev, A. V. and Mazin, I. P.: Supersaturation of water vapor in clouds, J. Atmos. Sci., 60, 2957–2974, https://doi.org/10.1175/1520-0469(2003)060<2957:SOWVIC>2.0.CO;2, 2003. a
Lai, A.: Particle deposition indoors: a review., Indoor air, 12, 211–214, https://doi.org/10.1034/j.1600-0668.2002.01159.x, 2002. a
Lehmann, K., Siebert, H., and Shaw, R. A.: Homogeneous and inhomogeneous mixing in cumulus clouds: Dependence on local turbulence structure, J. Atmos. Sci., 66, 3641–3659, https://doi.org/10.1175/2009JAS3012.1, 2009. a
Lewis, E. R.: The dependence of radius on relative humidity and solute mass at high relative humidities up to and including 100%, J. Geophys. Res.-Atmos., 124, 2105–2126, https://doi.org/10.1029/2018JD030008, 2019. a
Liu, Y. and Hallett, J.: On size distributions of cloud droplets growing by condensation: A new conceptual model, J. Atmos. Sci., 55, 527–536, https://doi.org/10.1175/1520-0469(1998)055<0527:OSDOCD>2.0.CO;2, 1998. a, b
MacMillan, T., Shaw, R. A., Cantrell, W. H., and Richter, D. H.: Direct numerical simulation of turbulence and microphysics in the Pi Chamber, Phys. Rev. Fluids, 7, 020501, https://doi.org/10.1103/PhysRevFluids.7.020501, 2022. a
McGraw, R. and Liu, Y.: Brownian drift-diffusion model for evolution of droplet size distributions in turbulent clouds, Geophys. Res. Lett., 33, L03802, https://doi.org/10.1029/2005GL023545, 2006. a
Monin, A. and Obukhov, A.: Basic laws of turbulent mixing in the atmosphere near the ground, Tr. Geofiz. Inst., Akad. Nauk SSSR, 24, 163–187, 1954. a
Morrison, H., Witte, M., Bryan, G. H., Harrington, J. Y., and Lebo, Z. J.: Broadening of modeled cloud droplet spectra using bin microphysics in an Eulerian spatial domain, J. Atmos. Sci., 75, 4005–4030, https://doi.org/10.1175/JAS-D-18-0055.1, 2018. a
Morrison, H., van Lier-Walqui, M., Fridlind, A. M., Grabowski, W. W., Harrington, J. Y., Hoose, C., Korolev, A., Kumjian, M. R., Milbrandt, J. A., Pawlowska, H., Posselt, D. J., Prat, O. P., Reimel, K. J., Shima, S. I., Diedenhoven, B., and Xue, L.: Confronting the challenge of modeling cloud and precipitation microphysics, J. Adv. Model. Earth Sy., 12, e2019MS001689, https://doi.org/10.1029/2019MS001689, 2020. a
Nenes, A., Ghan, S., Abdul-Razzak, H., Chuang, P. Y., and Seinfeld, J. H.: Kinetic limitations on cloud droplet formation and impact on cloud albedo, Tellus B, 53, 133–149, https://doi.org/10.3402/tellusb.v53i2.16569, 2001. a
Prabhakaran, P., Thomas, S., Cantrell, W., Shaw, R. A., and Yang, F.: Sources of stochasticity in the growth of cloud droplets: Supersaturation fluctuations versus turbulent transport, J. Atmos. Sci., 79, 3145–3162, https://doi.org/10.1175/JAS-D-22-0051.1, 2022. a
Richter, D. H., MacMillan, T., and Wainwright, C.: A Lagrangian cloud model for the study of marine fog, Bound.-Lay. Meteorol., 181, 523–542, https://doi.org/10.1007/s10546-020-00595-w, 2021. a
Rogers, R. R. and Yau, M. K.: A short course in cloud physics, 3rd edn., Burlington-Heinemann, MA, USA, ISBN 978-0750632157, 1989. a
Saito, I., Gotoh, T., and Watanabe, T.: Broadening of cloud droplet size distributions by condensation in turbulence, J. Meteorol. Soc. Jpn. Ser. II, 97, 867–891, https://doi.org/10.2151/jmsj.2019-049, 2019. a
Sellegri, K., Laj, P., Dupuy, R., Legrand, M., Preunkert, S., and Putaud, J.-P.: Size-dependent scavenging efficiencies of multicomponent atmospheric aerosols in clouds, J. Geophys. Res.-Atmos., 108, 4334, https://doi.org/10.1029/2002JD002749, 2003. a
Shaw, R. A., Thomas, S., Prabhakaran, P., Cantrell, W., Ovchinnikov, M., and Yang, F.: Fast and slow microphysics regimes in a minimalist model of cloudy Rayleigh-Bénard convection, Phys. Rev. Res., 5, 043018, https://doi.org/10.1103/PhysRevResearch.5.043018, 2023. a, b, c, d, e, f, g, h, i, j, k, l, m, n, o, p, q, r
Shima, S.., Kusano, K., Kawano, A., Sugiyama, T., and Kawahara, S.: The super-droplet method for the numerical simulation of clouds and precipitation: A particle-based and probabilistic microphysics model coupled with a non-hydrostatic model, Q. J. Roy. Meteor. Soc., 135, 1307–1320, https://doi.org/10.1002/qj.441, 2009. a
Thomas, S., Ovchinnikov, M., Yang, F., van der Voort, D., Cantrell, W., Krueger, S. K., and Shaw, R. A.: Scaling of an atmospheric model to simulate turbulence and cloud microphysics in the Pi Chamber, J. Adv. Model. Earth Sy., 11, 1981–1994, https://doi.org/10.1029/2019MS001670, 2019. a, b, c, d, e, f
Thomas, S., Yang, F., Ovchinnikov, M., Cantrell, W., and Shaw, R. A.: Scaling of turbulence and microphysics in a convection–cloud chamber of varying height, J. Adv. Model. Earth Sy., 15, e2022MS003304, https://doi.org/10.1029/2022MS003304, 2023. a, b
Twomey, S.: The nuclei of natural cloud formation part II: The supersaturation in natural clouds and the variation of cloud droplet concentration, Geofisica pura e applicata, 43, 243–249, https://doi.org/10.1007/BF01993560, 1959. a, b
Wang, A., Krueger, S., Chen, S., Ovchinnikov, M., Cantrell, W., and Shaw, R. A.: Glaciation of mixed-phase clouds: insights from bulk model and bin-microphysics large-eddy simulation informed by laboratory experiment, Atmos. Chem. Phys., 24, 10245–10260, https://doi.org/10.5194/acp-24-10245-2024, 2024a. a, b, c
Wang, A., Ovchinnikov, M., Yang, F., Cantrell, W., Yeom, J., and Shaw, R. A.: The Dual Nature of Entrainment-Mixing Signatures Revealed Through Large-Eddy Simulations of a Convection-Cloud Chamber, J. Atmos. Sci., https://doi.org/10.1175/JAS-D-24-0043.1, 2024b. a, b
Wang, A., Ovchinnikov, M., Yang, F., Shaw, R. A., and Schmalfuss, S.: Designing a convective cloud chamber for collision coalescence using atmospheric large-eddy simulation with bin microphysics scheme, J. Adv. Model. Earth Sy., 16, e2023MS003734, https://doi.org/10.1029/2023MS003734, 2024c. a, b, c, d, e, f, g
Wang, A., Yang, X. I. A., and Ovchinnikov, M.: An investigation of LES wall modeling for Rayleigh-Bénard convection via interpretable and physics-aware feedforward neural networks with DNS, J. Atmos. Sci., 81, 435–458, https://doi.org/10.1175/JAS-D-23-0094.1, 2024d. a
Xue, H. and Feingold, G.: A modeling study of the effect of nitric acid on cloud properties, J. Geophys. Res.-Atmos., 109, D18204, https://doi.org/10.1029/2004JD004750, 2004. a
Yang, F. and Hou, P.: Data and Code used in “Microphysics regimes due to haze-cloud interactions: cloud oscillation and cloud collapse”, Zenodo [code and data set], https://doi.org/10.5281/zenodo.14002523, 2024. a
Yang, F., Shaw, R., and Xue, H.: Conditions for super-adiabatic droplet growth after entrainment mixing, Atmos. Chem. Phys., 16, 9421–9433, https://doi.org/10.5194/acp-16-9421-2016, 2016. a
Yang, F., Kollias, P., Shaw, R. A., and Vogelmann, A. M.: Cloud droplet size distribution broadening during diffusional growth: ripening amplified by deactivation and reactivation, Atmos. Chem. Phys., 18, 7313–7328, https://doi.org/10.5194/acp-18-7313-2018, 2018. a
Yang, F., Ovchinnikov, M., Thomas, S., Khain, A., McGraw, R., Shaw, R. A., and Vogelmann, A. M.: Large-eddy simulations of a convection cloud chamber: Sensitivity to bin microphysics and advection, J. Adv. Model. Earth Sy., 14, e2021MS002895, https://doi.org/10.1029/2021MS002895, 2022. a, b, c
Yang, F., Hoffmann, F., Shaw, R. A., Ovchinnikov, M., and Vogelmann, A. M.: An intercomparison of large-eddy simulations of a convection cloud chamber using haze-capable bin and Lagrangian cloud microphysics schemes, J. Adv. Model. Earth Sy., 15, e2022MS003270, https://doi.org/10.1029/2022MS003270, 2023. a, b, c, d, e, f, g, h, i, j, k, l, m, n, o, p
Short summary
Large-eddy simulations of a convection cloud chamber show two new microphysics regimes, cloud oscillation and cloud collapse, due to haze–cloud interactions. Our results suggest that haze particles and their interactions with cloud droplets should be considered especially in polluted conditions. To properly simulate haze–cloud interactions, we need to resolve droplet activation and deactivation processes, instead of using Twomey-type activation parameterization.
Large-eddy simulations of a convection cloud chamber show two new microphysics regimes, cloud...
Altmetrics
Final-revised paper
Preprint