Articles | Volume 25, issue 22
https://doi.org/10.5194/acp-25-15953-2025
https://doi.org/10.5194/acp-25-15953-2025
Research article
 | 
18 Nov 2025
Research article |  | 18 Nov 2025

Chemical characterization and source apportionment of fine particulate matter in Kigali, Rwanda, using aerosol mass spectrometry

Theobard Habineza, Allen L. Robinson, H. Langley DeWitt, Jimmy Gasore, Philip L. Croteau, and Albert A. Presto

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Cited articles

AMS Spectral Database (Unit Mass Resolution): http://cires.colorado.edu/jimenez-group/AMSsd/, last access: 10 September 2025. 
Anand, A., Touré, N. E., Bahino, J., Gnamien, S., Hughes, A. F., Arku, R. E., Tawiah, V. O., Asfaw, A., Mamo, T., Hasheminassab, S., Bililign, S., Moschos, V., Westervelt, D. M., and Presto, A. A.: Low-Cost Hourly Ambient Black Carbon Measurements at Multiple Cities in Africa, Environ. Sci. Technol., 58, 12575–12584, https://doi.org/10.1021/acs.est.4c02297, 2024. 
Andersson, A., Kirillova, E. N., Decesari, S., DeWitt, L., Gasore, J., Potter, K. E., Prinn, R. G., Rupakheti, M., de Dieu Ndikubwimana, J., Nkusi, J., and Safari, B.: Seasonal source variability of carbonaceous aerosols at the Rwanda Climate Observatory, Atmos. Chem. Phys., 20, 4561–4573, https://doi.org/10.5194/acp-20-4561-2020, 2020. 
Brito, J., Freney, E., Dominutti, P., Borbon, A., Haslett, S. L., Batenburg, A. M., Colomb, A., Dupuy, R., Denjean, C., Burnet, F., Bourriane, T., Deroubaix, A., Sellegri, K., Borrmann, S., Coe, H., Flamant, C., Knippertz, P., and Schwarzenboeck, A.: Assessing the role of anthropogenic and biogenic sources on PM1 over southern West Africa using aircraft measurements, Atmos. Chem. Phys., 18, 757–772, https://doi.org/10.5194/acp-18-757-2018, 2018. 
Climatology of eastern Africa, http://maproom.meteorwanda.gov.rw/maproom/ (last access: 30 July 2025). 
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Short summary
This study reports year-long PM1 (particulate matter) chemical composition in Eastern Africa using aerosol mass spectrometry. Results show PM is dominated by organic aerosol (73 %), black carbon (16 %), and inorganics (11 %), with BC largely from fossil fuel (59 %) and biomass burning (41 %). Findings highlight the impact of solid fuels and aging vehicles and stress the need for regional mitigation strategies to reduce air pollution-related health risks.
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