Articles | Volume 24, issue 5
https://doi.org/10.5194/acp-24-3197-2024
https://doi.org/10.5194/acp-24-3197-2024
Research article
 | 
14 Mar 2024
Research article |  | 14 Mar 2024

Contribution of brown carbon to light absorption in emissions of European residential biomass combustion appliances

Satish Basnet, Anni Hartikainen, Aki Virkkula, Pasi Yli-Pirilä, Miika Kortelainen, Heikki Suhonen, Laura Kilpeläinen, Mika Ihalainen, Sampsa Väätäinen, Juho Louhisalmi, Markus Somero, Jarkko Tissari, Gert Jakobi, Ralf Zimmermann, Antti Kilpeläinen, and Olli Sippula

Related authors

The role of fuel and environmental conditions on the amount and composition of primary, fresh, and aged aerosol emissions originating from diesel- and gasoline-operated auxiliary heaters of passenger cars
Henri Oikarinen, Anni Hartikainen, Pauli Simonen, Miska Olin, Ukko-Ville Mäkinen, Petteri Marjanen, Laura Salo, Ville Silvonen, Sampsa Martikainen, Jussi Hoivala, Mika Ihalainen, Pasi Miettinen, Pasi Yli-Pirilä, Olli Sippula, Santtu Mikkonen, and Panu Karjalainen
EGUsphere, https://doi.org/10.5194/egusphere-2025-540,https://doi.org/10.5194/egusphere-2025-540, 2025
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
Short summary
Field-deployable cantilever-enhanced photoacoustic instrument for aerosol light absorption measurement at three wavelengths
Juho Karhu, Tommi Mikkonen, Joel Kuula, Aki Virkkula, Erkki Ikonen, Markku Vainio, Hilkka Timonen, and Tuomas Hieta
Aerosol Research, 3, 113–124, https://doi.org/10.5194/ar-3-113-2025,https://doi.org/10.5194/ar-3-113-2025, 2025
Short summary
Multiple eco-regions contribute to the seasonal cycle of Antarctic aerosol size distributions
James Brean, David C. S. Beddows, Eija Asmi, Aki Virkkula, Lauriane L. J. Quéléver, Mikko Sipilä, Floortje Van Den Heuvel, Thomas Lachlan-Cope, Anna Jones, Markus Frey, Angelo Lupi, Jiyeon Park, Young Jun Yoon, Rolf Weller, Giselle L. Marincovich, Gabriela C. Mulena, Roy M. Harrison, and Manuel Dall'Osto
Atmos. Chem. Phys., 25, 1145–1162, https://doi.org/10.5194/acp-25-1145-2025,https://doi.org/10.5194/acp-25-1145-2025, 2025
Short summary
Validation of cantilever-enhanced photoacoustic particle-size-resolved light absorption measurement using nigrosin reference particles and Mie modelling
Joel Kuula, Juho Karhu, Tommi Mikkonen, Patrick Grahn, Aki Virkkula, Hilkka Timonen, Tuomas Hieta, and Markku Vainio
Aerosol Research, 3, 1–13, https://doi.org/10.5194/ar-3-1-2025,https://doi.org/10.5194/ar-3-1-2025, 2025
Short summary
Photochemical aging of aviation emissions: transformation of chemical and physical properties of exhaust emissions from a laboratory-scale jet engine combustion chamber
Anni Hartikainen, Mika Ihalainen, Deeksha Shukla, Marius Rohkamp, Arya Mukherjee, Quanfu He, Sandra Piel, Aki Virkkula, Delun Li, Tuukka Kokkola, Seongho Jeong, Hanna Koponen, Uwe Etzien, Anusmita Das, Krista Luoma, Lukas Schwalb, Thomas Gröger, Alexandre Barth, Martin Sklorz, Thorsten Streibel, Hendryk Czech, Benedikt Gündling, Markus Kalberer, Bert Buchholz, Andreas Hupfer, Thomas Adam, Thorsten Hohaus, Johan Øvrevik, Ralf Zimmermann, and Olli Sippula
EGUsphere, https://doi.org/10.5194/egusphere-2024-3836,https://doi.org/10.5194/egusphere-2024-3836, 2025
Short summary

Related subject area

Subject: Aerosols | Research Activity: Laboratory Studies | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Wind-driven emission of marine ice-nucleating particles in the Scripps Ocean-Atmosphere Research Simulator (SOARS)
Kathryn A. Moore, Thomas C. J. Hill, Chamika K. Madawala, Raymond J. Leibensperger III, Samantha Greeney, Christopher D. Cappa, M. Dale Stokes, Grant B. Deane, Christopher Lee, Alexei V. Tivanski, Kimberly A. Prather, and Paul J. DeMott
Atmos. Chem. Phys., 25, 3131–3159, https://doi.org/10.5194/acp-25-3131-2025,https://doi.org/10.5194/acp-25-3131-2025, 2025
Short summary
Measurement report: The ice-nucleating activity of lichen sampled in a northern European boreal forest
Ulrike Proske, Michael P. Adams, Grace C. E. Porter, Mark A. Holden, Jaana Bäck, and Benjamin J. Murray
Atmos. Chem. Phys., 25, 979–995, https://doi.org/10.5194/acp-25-979-2025,https://doi.org/10.5194/acp-25-979-2025, 2025
Short summary
Insights into the real part of natural sea spray aerosol refractive index in the Pacific Ocean
Chengyi Fan, Bishuo He, Shuqi Guo, Jie Qiu, and Chunsheng Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-3527,https://doi.org/10.5194/egusphere-2024-3527, 2025
Short summary
Partitioning of ionic surfactants in aerosol droplets containing glutaric acid, sodium chloride, or sea salts
Alison Bain, Kunal Ghosh, Konstantin Tumashevich, Nonne L. Prisle, and Bryan R. Bzdek
EGUsphere, https://doi.org/10.5194/egusphere-2024-3993,https://doi.org/10.5194/egusphere-2024-3993, 2025
Short summary
Viscosity of aqueous ammonium nitrate–organic particles: equilibrium partitioning may be a reasonable assumption for most tropospheric conditions
Liviana K. Klein, Allan K. Bertram, Andreas Zuend, Florence Gregson, and Ulrich K. Krieger
Atmos. Chem. Phys., 24, 13341–13359, https://doi.org/10.5194/acp-24-13341-2024,https://doi.org/10.5194/acp-24-13341-2024, 2024
Short summary

Cited articles

Andreae, M. O.: Emission of trace gases and aerosols from biomass burning – an updated assessment, Atmos. Chem. Phys., 19, 8523–8546, https://doi.org/10.5194/acp-19-8523-2019, 2019. 
Backman, J., Schmeisser, L., Virkkula, A., Ogren, J. A., Asmi, E., Starkweather, S., Sharma, S., Eleftheriadis, K., Uttal, T., Jefferson, A., Bergin, M., Makshtas, A., Tunved, P., and Fiebig, M.: On Aethalometer measurement uncertainties and an instrument correction factor for the Arctic, Atmos. Meas. Tech., 10, 5039–5062, https://doi.org/10.5194/amt-10-5039-2017, 2017. 
Bahadur, R., Praveen, P. S., Xu, Y., and Ramanathan, V.: Solar absorption by elemental and brown carbon determined from spectral observations, P. Natl. Acad. Sci. USA, 109, 17366–17371, https://doi.org/10.1073/pnas.1205910109, 2012. 
Bernardoni, V., Pileci, R. E., Caponi, L., and Massabò, D.: The multi-wavelength absorption analyzer (MWAA) model as a tool for source and component apportionment based on aerosol absorption properties: Application to samples collected in different environments, Atmosphere, 8, 218, https://doi.org/10.3390/atmos8110218, 2017. 
Bond, T. C., Habib, G., and Bergstrom, R. W.: Limitations in the enhancement of visible light absorption due to mixing state, J. Geophys. Res.-Atmos., 111, 20211, https://doi.org/10.1029/2006JD007315, 2006. 
Download
Short summary
Brown carbon (BrC) emissions were estimated, for residential wood combustion (RWC) from various northern European appliances, utilizing an extensive seven-wavelength aethalometer dataset and thermal–optical carbon analysis. The contribution of BrC370–950 to the absorption of visible light varied between 1 % and 21 %, and was linked with fuel moisture content and combustion efficiency. This study provides important information required for assessing the climate effects of RWC emissions.
Share
Altmetrics
Final-revised paper
Preprint