Articles | Volume 23, issue 16
https://doi.org/10.5194/acp-23-9385-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-9385-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Measurement report: New insights into the mixing structures of black carbon on the eastern Tibetan Plateau – soot redistribution and fractal dimension enhancement by liquid–liquid phase separation
Qi Yuan
Key Laboratory of Marine Environmental Science and Ecology, Ministry of Education of China, Ocean University of China, Qingdao, 266100 Shandong, China
Key Laboratory of Atmospheric Chemistry, China Meteorological Administration, 100081 Beijing, China
Yuanyuan Wang
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou, 310027 Zhejiang, China
Yixin Chen
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou, 310027 Zhejiang, China
Siyao Yue
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, 100029 Beijing, China
now at: Minerva Research Group, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Jian Zhang
School of Environmental and Material Engineering, Yantai University, Yantai, 264005 Shandong, China
Yinxiao Zhang
Flight College, Binzhou University, Binzhou, 256600 Shandong, China
Liang Xu
College of Sciences, China Jiliang University, Hangzhou, 310018 Zhejiang, China
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, 300072 Tianjin, China
Dantong Liu
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou, 310027 Zhejiang, China
Pingqing Fu
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, 300072 Tianjin, China
Huiwang Gao
Key Laboratory of Marine Environmental Science and Ecology, Ministry of Education of China, Ocean University of China, Qingdao, 266100 Shandong, China
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou, 310027 Zhejiang, China
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Cited
7 citations as recorded by crossref.
- A Framework for Quantifying the Size and Fractal Dimension of Compacting Soot Particles P. Beeler et al. 10.1021/acs.est.4c11100
- Variability in morphology of soot particles during non-cloud and in-cloud processes Y. Wang et al. 10.1016/j.atmosenv.2024.120489
- Comparative study of black carbon mixing state characterization: Evaluating Only-SP2 and CPMA-SP2 techniques for enhanced accuracy Z. Li et al. 10.1016/j.jes.2025.06.010
- Measurement report: New insights into the mixing structures of black carbon on the eastern Tibetan Plateau – soot redistribution and fractal dimension enhancement by liquid–liquid phase separation Q. Yuan et al. 10.5194/acp-23-9385-2023
- The interplay between aqueous replacement reaction and the phase state of internally mixed organic/ammonium aerosols H. Yang et al. 10.5194/acp-24-11619-2024
- Phase Transitions in Organic and Organic/Inorganic Aerosol Particles M. Freedman et al. 10.1146/annurev-physchem-083122-115909
- Measurement report: New insights into the mixing structures of black carbon on the eastern Tibetan Plateau – soot redistribution and fractal dimension enhancement by liquid–liquid phase separation Q. Yuan et al. 10.5194/acp-23-9385-2023
6 citations as recorded by crossref.
- A Framework for Quantifying the Size and Fractal Dimension of Compacting Soot Particles P. Beeler et al. 10.1021/acs.est.4c11100
- Variability in morphology of soot particles during non-cloud and in-cloud processes Y. Wang et al. 10.1016/j.atmosenv.2024.120489
- Comparative study of black carbon mixing state characterization: Evaluating Only-SP2 and CPMA-SP2 techniques for enhanced accuracy Z. Li et al. 10.1016/j.jes.2025.06.010
- Measurement report: New insights into the mixing structures of black carbon on the eastern Tibetan Plateau – soot redistribution and fractal dimension enhancement by liquid–liquid phase separation Q. Yuan et al. 10.5194/acp-23-9385-2023
- The interplay between aqueous replacement reaction and the phase state of internally mixed organic/ammonium aerosols H. Yang et al. 10.5194/acp-24-11619-2024
- Phase Transitions in Organic and Organic/Inorganic Aerosol Particles M. Freedman et al. 10.1146/annurev-physchem-083122-115909
Latest update: 30 Jun 2025
Short summary
This study for the first time found large amounts of liquid–liquid phase separation particles with soot redistributing in organic coatings instead of sulfate cores in the eastern Tibetan Plateau atmosphere. The particle size and the ratio of the organic matter coating thickness to soot size are two of the major possible factors that likely affect the soot redistribution process. The soot redistribution process promoted the morphological compaction of soot particles.
This study for the first time found large amounts of liquid–liquid phase separation particles...
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