Articles | Volume 22, issue 13
https://doi.org/10.5194/acp-22-9011-2022
https://doi.org/10.5194/acp-22-9011-2022
Technical note
 | 
13 Jul 2022
Technical note |  | 13 Jul 2022

Technical note: Entrainment-limited kinetics of bimolecular reactions in clouds

Christopher D. Holmes

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Cited articles

Alexander, B., Sherwen, T., Holmes, C. D., Fisher, J. A., Chen, Q., Evans, M. J., and Kasibhatla, P.: Global inorganic nitrate production mechanisms: comparison of a global model with nitrate isotope observations, Atmos. Chem. Phys., 20, 3859–3877, https://doi.org/10.5194/acp-20-3859-2020, 2020. 
Chameides, W. L: The photochemistry of a remote marine stratiform cloud, J. Geophys. Res., 89, 4739–4755, https://doi.org/10.1029/JD089iD03p04739, 1984. 
Chan, Y.-C., Evans, M. J., He, P., Holmes, C. D., Jaegle, L., Kasibhatla, P., Liu, X.-Y., Sherwen, T., Thornton, J. A., Wang, X., Xie, Z., Zhai, S., and Alexander, B.: Heterogeneous nitrate production mechanisms in intense haze events in North China, J. Geophys. Res., 126, e2021JD034688, https://doi.org/10.1029/2021JD034688, 2021. 
Holmes, C. D., Bertram, T. H., Confer, K. L., Graham, K. A., Ronan, A. C., Wirks, C. K., and Shah, V.: The role of clouds in the tropospheric NOx cycle: A new modeling approach for cloud chemistry and its global implications, Geophys. Res. Lett., 46, 4980–4990, https://doi.org/10.1029/2019GL081990, 2019.  
Jernigan, C. M., Fite, C. H., Vereecken, L., Berkelhammer, M. B., Rollins, A. W., Rickly, P. S., Novelli, A., Taraborrelli, D., Holmes, C. D., and Bertram, T. H.: Efficient Production of Carbonyl Sulfide in the Low-NOx Oxidation of Dimethyl Sulfide, Geophys. Res. Lett., 49, e2021GL096838, https://doi.org/10.1029/2021GL096838, 2022. 
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Short summary
Cloud water and ice enable reactions that lead to acid rain and alter atmospheric oxidants, among other impacts. This work develops and evaluates an efficient method of simulating cloud chemistry within global and regional atmospheric models in order to better understand the role of clouds in atmospheric chemistry.
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