Articles | Volume 22, issue 2
https://doi.org/10.5194/acp-22-1549-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-1549-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
01 Feb 2022
Research article |
| 01 Feb 2022
| 01 Feb 2022
Exploring dimethyl sulfide (DMS) oxidation and implications for global aerosol radiative forcing
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Department of Earth, Atmospheric, and Planetary Sciences, Massachusetts Institute of Technology, Cambridge, MA, USA
Jesse H. Kroll
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Siyuan Wang
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO, USA
Chemical Sciences Laboratory, National Oceanic and Atmospheric
Administration, Boulder, CO, USA
Duseong S. Jo
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Andrew Gettelman
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Zheng Lu
Department of Atmospheric Sciences, Texas A&M University, College Station, TX, USA
Xiaohong Liu
Department of Atmospheric Sciences, Texas A&M University, College Station, TX, USA
Rahul A. Zaveri
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
Eric C. Apel
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Donald R. Blake
Department of Chemistry, University of California Irvine, Irvine, CA, USA
Jose-Luis Jimenez
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO, USA
Department of Chemistry, University of Colorado Boulder, Boulder, CO, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, CO, USA
Department of Chemistry, University of Colorado Boulder, Boulder, CO, USA
Patrick R. Veres
Chemical Sciences Laboratory, National Oceanic and Atmospheric
Administration, Boulder, CO, USA
Timothy S. Bates
The Cooperative Institute for Climate, Ocean, and Ecosystem Studies, College of the Environment, University of Washington, Seattle, WA, USA
John E. Shilling
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
Maria Zawadowicz
Environmental and Climate Sciences Department, Brookhaven National
Laboratory, Upton, NY, USA
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49 citations as recorded by crossref.
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- Dimethylsulfoniopropionate (DMSP): From Biochemistry to Global Ecological Significance C. Li et al. 10.1146/annurev-micro-041222-024055
- Assessing the Isomerization of a Primary Intermediate (CH3SCH2O2• Radical) in Dimethyl Sulfide Degradation in the Marine Boundary Layer M. Lily et al. 10.1021/acsearthspacechem.3c00209
- Marine emissions of methanethiol increase aerosol cooling in the Southern Ocean C. Wohl et al. 10.1126/sciadv.adq2465
- The Potential for Great Barrier Reef Regional Climate Regulation via Dimethylsulfide Atmospheric Oxidation Products H. Swan 10.3389/fmars.2022.869166
- Butene Emissions From Coastal Ecosystems May Contribute to New Particle Formation C. Giorio et al. 10.1029/2022GL098770
- Reactive Uptake of Hydroperoxymethyl Thioformate to Sodium Chloride and Sodium Iodide Aerosol Particles C. Jernigan et al. 10.1021/acs.jpca.2c03222
- IPB-MSA&SO4: a daily 0.25° resolution dataset of in situ-produced biogenic methanesulfonic acid and sulfate over the North Atlantic during 1998–2022 based on machine learning K. Mansour et al. 10.5194/essd-16-2717-2024
- Pan-Arctic methanesulfonic acid aerosol: source regions, atmospheric drivers, and future projections J. Pernov et al. 10.1038/s41612-024-00712-3
- Characterizing spatio-temporal variations of dimethyl sulfide in the Yellow and East China Sea based on BP neural network W. Guo et al. 10.3389/fmars.2024.1394502
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- Sulfate and Carbonyl Sulfide Production in Aqueous Reactions of Hydroperoxymethyl Thioformate C. Jernigan et al. 10.1021/acsestair.3c00098
- Chemical Fate of Particulate Sulfur from Nighttime Oxidation of Thiophene M. Lum et al. 10.1021/acsestair.4c00164
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- Molecular characteristics of sea spray aerosols during aging with the participation of marine volatile organic compounds X. Ma et al. 10.1016/j.scitotenv.2024.176380
- Influence of Air Mass Source Regions on Signatures of Surface-Active Organic Molecules in Size Resolved Atmospheric Aerosol Particles T. Burdette et al. 10.1021/acsearthspacechem.3c00161
- Atmospheric reactions of hydroperoxymethyl thioformate with sulfur trioxide catalyzed by water monomer and hydrolysis of sulfur trioxide catalyzed by hydroperoxymethyl thioformate X. Zhang et al. 10.1016/j.comptc.2024.114641
Latest update: 13 Dec 2024
Short summary
Understanding the natural aerosol burden in the preindustrial era is crucial for us to assess how atmospheric aerosols affect the Earth's radiative budgets. Our study explores how a detailed description of dimethyl sulfide (DMS) oxidation (implemented in the Community Atmospheric Model version 6 with chemistry, CAM6-chem) could help us better estimate the present-day and preindustrial concentrations of sulfate and other relevant chemicals, as well as the resulting aerosol radiative impacts.
Understanding the natural aerosol burden in the preindustrial era is crucial for us to assess...
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