Articles | Volume 22, issue 20
https://doi.org/10.5194/acp-22-13431-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-13431-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
18 Oct 2022
Research article |
| 18 Oct 2022
| 18 Oct 2022
Quantifying the importance of vehicle ammonia emissions in an urban area of northeastern USA utilizing nitrogen isotopes
Wendell W. Walters
CORRESPONDING AUTHOR
Department of Earth, Environmental, and Planetary Sciences, Brown
University, Providence, RI 02912, USA
Institute at Brown for Environment and Society, Brown University,
Providence, RI 02912, USA
Madeline Karod
Department of Earth, Environmental, and Planetary Sciences, Brown
University, Providence, RI 02912, USA
Chemistry and Physics Department, Simmons University, Boston, MA 02215,
USA
Emma Willcocks
Program in Biology, Division of Biology and Medicine, Brown
University, Providence, RI 02912, USA
Bok H. Baek
Center for Spatial Information, Sciences, and Systems, George Mason
University, Fairfax, VA 22030, USA
Danielle E. Blum
Institute at Brown for Environment and Society, Brown University,
Providence, RI 02912, USA
Department of Chemistry, Brown University, Providence, RI 02916, USA
Meredith G. Hastings
Department of Earth, Environmental, and Planetary Sciences, Brown
University, Providence, RI 02912, USA
Institute at Brown for Environment and Society, Brown University,
Providence, RI 02912, USA
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Cited
19 citations as recorded by crossref.
- Anthropogenic impacts and quantitative sources of nitrate in a rural-urban canal using a combined PMF, δ15N/δ18O–NO3-, and MixSIAR approach C. Zhang et al. 10.1016/j.envres.2024.118587
- Nitrogen isotopic characteristics of aerosol ammonium in a Chinese megacity indicate the reduction from vehicle emissions during the lockdown period Z. Li et al. 10.1016/j.scitotenv.2024.171265
- Large Seasonal Variation in Nitrogen Isotopic Abundances of Ammonia Volatilized from a Cropland Ecosystem and Implications for Regional NH3 Source Partitioning L. Song et al. 10.1021/acs.est.3c08800
- Monitoring gaseous pollutants using passive sampling in the Philadelphia region B. Terry & K. Shakya 10.1080/10962247.2023.2279733
- Nitrogen isotopes suggest agricultural and non-agricultural sources contribute equally to NH3 and NH4+ in urban Beijing during December 2018 N. Bhattarai et al. 10.1016/j.envpol.2023.121455
- High spatiotemporal resolution ammonia emission inventory from typical industrial and agricultural province of China from 2000 to 2020 C. Zhu et al. 10.1016/j.scitotenv.2024.170732
- Solid Phase Extraction Methodology for Robust Isotope Analysis of Atmospheric Ammonium A. MacFarland et al. 10.1021/acsearthspacechem.3c00375
- Strategic control of combustion-induced ammonia emissions: A key initiative for substantial PM2.5 reduction in Tianjin, North China Plain H. Xiao et al. 10.1016/j.scitotenv.2024.172328
- Interannual variability of atmospheric ammonia over the Sichuan Basin, southwestern China: Trend, sources, and implications on particle matter control X. Yang et al. 10.1016/j.atmosres.2023.107170
- Measurement of Light-Duty Vehicle Exhaust Emissions with Light Absorption Spectrometers B. Giechaskiel et al. 10.3390/technologies12030032
- Sensitivity of air quality to vehicle ammonia emissions in the United States C. Toro et al. 10.1016/j.atmosenv.2024.120484
- Trends of inorganic sulfur and nitrogen species at an urban site in western Canada (2004–2018) H. Wang & L. Zhang 10.1016/j.envpol.2023.122079
- Source Apportionment of Atmospheric Ammonia at 16 Sites in China Using a Bayesian Isotope Mixing Model Based on δ15N–NHx Signatures Y. Zhang et al. 10.1021/acs.est.2c09796
- Discerning the Concentration and Bi‐Directional Flux of Ammonia in an Urban Estuary Using the Relaxed Eddy Accumulation Method E. Joyce et al. 10.1029/2023JG007414
- Sources, Variations, and Effects on Air Quality of Atmospheric Ammonia Z. Lan et al. 10.1007/s40726-023-00291-6
- Impact of urbanization on fine particulate matter concentrations over central Europe P. Huszar et al. 10.5194/acp-24-397-2024
- Characteristics and sources of atmospheric ammonia at the SORPES station in the western Yangtze river delta of China R. Liu et al. 10.1016/j.atmosenv.2023.120234
- Long-term trends in inorganic aerosol chemical composition and chemistry at an urban and rural site in the northeastern US H. Kim et al. 10.1016/j.scitotenv.2023.166848
- Quantifying the importance of vehicle ammonia emissions in an urban area of northeastern USA utilizing nitrogen isotopes W. Walters et al. 10.5194/acp-22-13431-2022
18 citations as recorded by crossref.
- Anthropogenic impacts and quantitative sources of nitrate in a rural-urban canal using a combined PMF, δ15N/δ18O–NO3-, and MixSIAR approach C. Zhang et al. 10.1016/j.envres.2024.118587
- Nitrogen isotopic characteristics of aerosol ammonium in a Chinese megacity indicate the reduction from vehicle emissions during the lockdown period Z. Li et al. 10.1016/j.scitotenv.2024.171265
- Large Seasonal Variation in Nitrogen Isotopic Abundances of Ammonia Volatilized from a Cropland Ecosystem and Implications for Regional NH3 Source Partitioning L. Song et al. 10.1021/acs.est.3c08800
- Monitoring gaseous pollutants using passive sampling in the Philadelphia region B. Terry & K. Shakya 10.1080/10962247.2023.2279733
- Nitrogen isotopes suggest agricultural and non-agricultural sources contribute equally to NH3 and NH4+ in urban Beijing during December 2018 N. Bhattarai et al. 10.1016/j.envpol.2023.121455
- High spatiotemporal resolution ammonia emission inventory from typical industrial and agricultural province of China from 2000 to 2020 C. Zhu et al. 10.1016/j.scitotenv.2024.170732
- Solid Phase Extraction Methodology for Robust Isotope Analysis of Atmospheric Ammonium A. MacFarland et al. 10.1021/acsearthspacechem.3c00375
- Strategic control of combustion-induced ammonia emissions: A key initiative for substantial PM2.5 reduction in Tianjin, North China Plain H. Xiao et al. 10.1016/j.scitotenv.2024.172328
- Interannual variability of atmospheric ammonia over the Sichuan Basin, southwestern China: Trend, sources, and implications on particle matter control X. Yang et al. 10.1016/j.atmosres.2023.107170
- Measurement of Light-Duty Vehicle Exhaust Emissions with Light Absorption Spectrometers B. Giechaskiel et al. 10.3390/technologies12030032
- Sensitivity of air quality to vehicle ammonia emissions in the United States C. Toro et al. 10.1016/j.atmosenv.2024.120484
- Trends of inorganic sulfur and nitrogen species at an urban site in western Canada (2004–2018) H. Wang & L. Zhang 10.1016/j.envpol.2023.122079
- Source Apportionment of Atmospheric Ammonia at 16 Sites in China Using a Bayesian Isotope Mixing Model Based on δ15N–NHx Signatures Y. Zhang et al. 10.1021/acs.est.2c09796
- Discerning the Concentration and Bi‐Directional Flux of Ammonia in an Urban Estuary Using the Relaxed Eddy Accumulation Method E. Joyce et al. 10.1029/2023JG007414
- Sources, Variations, and Effects on Air Quality of Atmospheric Ammonia Z. Lan et al. 10.1007/s40726-023-00291-6
- Impact of urbanization on fine particulate matter concentrations over central Europe P. Huszar et al. 10.5194/acp-24-397-2024
- Characteristics and sources of atmospheric ammonia at the SORPES station in the western Yangtze river delta of China R. Liu et al. 10.1016/j.atmosenv.2023.120234
- Long-term trends in inorganic aerosol chemical composition and chemistry at an urban and rural site in the northeastern US H. Kim et al. 10.1016/j.scitotenv.2023.166848
Latest update: 01 May 2024
Short summary
Atmospheric ammonia and its products are a significant source of urban haze and nitrogen deposition. We have investigated the seasonal source contributions to a mid-sized city in the northeastern US megalopolis utilizing geospatial statistical analysis and novel isotopic constraints, which indicate that vehicle emissions were significant components of the urban-reduced nitrogen budget. Reducing vehicle ammonia emissions should be considered to improve ecosystems and human health.
Atmospheric ammonia and its products are a significant source of urban haze and nitrogen...
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