Articles | Volume 21, issue 11
https://doi.org/10.5194/acp-21-8377-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-8377-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
02 Jun 2021
Research article |
| 02 Jun 2021
| 02 Jun 2021
New methodology shows short atmospheric lifetimes of oxidized sulfur and nitrogen due to dry deposition
Katherine Hayden
CORRESPONDING AUTHOR
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada, M3H 5T4
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada, M3H 5T4
College of Environmental Science and Engineering, Peking University, Beijing 100871, China
Paul Makar
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada, M3H 5T4
John Liggio
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada, M3H 5T4
Samar G. Moussa
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada, M3H 5T4
Ayodeji Akingunola
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada, M3H 5T4
Robert McLaren
Center for Atmospheric Chemistry, York University, 4700 Keele Street, Toronto, Ontario, Canada
Ralf M. Staebler
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada, M3H 5T4
Andrea Darlington
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada, M3H 5T4
Jason O'Brien
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada, M3H 5T4
Junhua Zhang
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada, M3H 5T4
Mengistu Wolde
National Research Council Canada, Flight Research Laboratory, Ottawa, Canada K1A 0R6
Leiming Zhang
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada, M3H 5T4
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Cited
13 citations as recorded by crossref.
- Organic carbon dry deposition outpaces atmospheric processing with unaccounted implications for air quality and freshwater ecosystems J. Liggio et al. 10.1126/sciadv.adr0259
- Aircraft-derived CH4 emissions from surface and in-situ mining activities in the Alberta oil sands region R. Staebler et al. 10.1016/j.aeaoa.2024.100280
- Contribution of emissions from the oil sands activities in Alberta, Canada to atmospheric concentration and deposition of nitrogen and sulfur species at a downwind site Y. You et al. 10.1016/j.envpol.2024.124301
- Total organic carbon measurements reveal major gaps in petrochemical emissions reporting M. He et al. 10.1126/science.adj6233
- Quantification of Methane Emissions from Cold Heavy Oil Production with Sand Extraction in Alberta and Saskatchewan, Canada T. Han et al. 10.1021/acs.est.4c02333
- SO2 emissions derived from TROPOMI observations over India using a flux-divergence method with variable lifetimes Y. Chen et al. 10.5194/acp-25-1851-2025
- High sulfur dioxide deposition velocities measured with the flux–gradient technique in a boreal forest in the Alberta Oil Sands Region M. Gordon et al. 10.5194/acp-23-7241-2023
- A decadal synthesis of atmospheric emissions, ambient air quality, and deposition in the oil sands region E. Horb et al. 10.1002/ieam.4539
- Modeling below-cloud scavenging of size-resolved particles in GEM-MACHv3.1 R. Ghahreman et al. 10.5194/gmd-17-685-2024
- Development of a continuous UAV-mounted air sampler and application to the quantification of CO2 and CH4 emissions from a major coking plant T. Han et al. 10.5194/amt-17-677-2024
- Air Composition over the Russian Arctic–4: Atmospheric Aerosols O. Antokhina et al. 10.1134/S102485602470057X
- Ozone in the boreal forest in the Alberta Oil Sands Region X. Zhang et al. 10.5194/acp-23-13647-2023
- Contribution of Atmospheric Deposition to Nutrient Loading in Lake Taihu J. Deng et al. 10.2139/ssrn.4103358
13 citations as recorded by crossref.
- Organic carbon dry deposition outpaces atmospheric processing with unaccounted implications for air quality and freshwater ecosystems J. Liggio et al. 10.1126/sciadv.adr0259
- Aircraft-derived CH4 emissions from surface and in-situ mining activities in the Alberta oil sands region R. Staebler et al. 10.1016/j.aeaoa.2024.100280
- Contribution of emissions from the oil sands activities in Alberta, Canada to atmospheric concentration and deposition of nitrogen and sulfur species at a downwind site Y. You et al. 10.1016/j.envpol.2024.124301
- Total organic carbon measurements reveal major gaps in petrochemical emissions reporting M. He et al. 10.1126/science.adj6233
- Quantification of Methane Emissions from Cold Heavy Oil Production with Sand Extraction in Alberta and Saskatchewan, Canada T. Han et al. 10.1021/acs.est.4c02333
- SO2 emissions derived from TROPOMI observations over India using a flux-divergence method with variable lifetimes Y. Chen et al. 10.5194/acp-25-1851-2025
- High sulfur dioxide deposition velocities measured with the flux–gradient technique in a boreal forest in the Alberta Oil Sands Region M. Gordon et al. 10.5194/acp-23-7241-2023
- A decadal synthesis of atmospheric emissions, ambient air quality, and deposition in the oil sands region E. Horb et al. 10.1002/ieam.4539
- Modeling below-cloud scavenging of size-resolved particles in GEM-MACHv3.1 R. Ghahreman et al. 10.5194/gmd-17-685-2024
- Development of a continuous UAV-mounted air sampler and application to the quantification of CO2 and CH4 emissions from a major coking plant T. Han et al. 10.5194/amt-17-677-2024
- Air Composition over the Russian Arctic–4: Atmospheric Aerosols O. Antokhina et al. 10.1134/S102485602470057X
- Ozone in the boreal forest in the Alberta Oil Sands Region X. Zhang et al. 10.5194/acp-23-13647-2023
- Contribution of Atmospheric Deposition to Nutrient Loading in Lake Taihu J. Deng et al. 10.2139/ssrn.4103358
Latest update: 08 May 2025
Short summary
We developed a method using aircraft measurements to determine lifetimes with respect to dry deposition for oxidized sulfur and nitrogen compounds over the boreal forest in Alberta, Canada. Atmospheric lifetimes were significantly shorter than derived from chemical transport models with differences related to modelled dry deposition velocities. The shorter lifetimes suggest models need to reassess dry deposition treatment and predictions of sulfur and nitrogen in the atmosphere and ecosystems.
We developed a method using aircraft measurements to determine lifetimes with respect to dry...
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