Articles | Volume 21, issue 9
https://doi.org/10.5194/acp-21-6721-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-6721-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
04 May 2021
Research article |
| 04 May 2021
| 04 May 2021
Isotopic compositions of atmospheric total gaseous mercury in 10 Chinese cities and implications for land surface emissions
State Key Laboratory of Environmental Geochemistry, Institute of
Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China
CAS Center for Excellence in Quaternary Science and Global Change,
Xi'an 710061, China
Chen Liu
State Key Laboratory of Environmental Geochemistry, Institute of
Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China
University of Chinese Academy of Sciences, Beijing 100049, China
Hui Zhang
State Key Laboratory of Environmental Geochemistry, Institute of
Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China
University of Chinese Academy of Sciences, Beijing 100049, China
Yue Xu
State Key Laboratory of Environmental Geochemistry, Institute of
Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China
Hui Zhang
State Key Laboratory of Environmental Geochemistry, Institute of
Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of
Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Xiaopu Lyu
Department of Civil and Environmental Engineering, The Hong Kong
Polytechnic University, Hong Kong SAR, China
Gan Zhang
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of
Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Department of Civil and Environmental Engineering, The Hong Kong
Polytechnic University, Hong Kong SAR, China
State Key Laboratory of Environmental Geochemistry, Institute of
Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China
Leiming Zhang
Air Quality Research Division, Science and Technology Branch,
Environment and Climate Change Canada, Toronto, Ontario, Canada
State Key Laboratory of Environmental Geochemistry, Institute of
Geochemistry, Chinese Academy of Sciences, Guiyang 550081, China
CAS Center for Excellence in Quaternary Science and Global Change,
Xi'an 710061, China
University of Chinese Academy of Sciences, Beijing 100049, China
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25 citations as recorded by crossref.
- Applying Passive Air Sampling and Isotopic Characterization to Assess Spatial Variability of Gaseous Elemental Mercury Across Ontario, Canada N. Szponar et al. 10.1029/2022JD037361
- Isotopic investigation of sources and processes affecting gaseous and particulate bound mercury in the east coast, South Korea H. Lee et al. 10.1016/j.scitotenv.2023.164404
- Changes in Atmospheric Gaseous Elemental Mercury Concentrations and Isotopic Compositions at Mt. Changbai During 2015–2021 and Mt. Ailao During 2017–2021 in China X. Wu et al. 10.1029/2022JD037749
- Sources and Transformation Mechanisms of Atmospheric Particulate Bound Mercury Revealed by Mercury Stable Isotopes C. Liu et al. 10.1021/acs.est.1c08065
- Sustained high atmospheric Hg level in Beijing during wet seasons suggests that anthropogenic pollution is continuing: Identification of potential sources C. Wang et al. 10.1016/j.envres.2022.113814
- Three thousand years of Hg pollution recorded in mangrove wetland sediments from South China M. Chen et al. 10.1016/j.envres.2024.118866
- Using Mercury Stable Isotopes to Quantify Bidirectional Water–Atmosphere Hg(0) Exchange Fluxes and Explore Controlling Factors H. Zhang et al. 10.1021/acs.est.3c01273
- Earth system modeling of mercury using CESM2 – Part 1: Atmospheric model CAM6-Chem/Hg v1.0 P. Zhang & Y. Zhang 10.5194/gmd-15-3587-2022
- Sources and risk assessment of atmospheric Hg during the 2022 Beijing Olympic Winter Games C. Wang et al. 10.1016/j.atmosenv.2023.119718
- Modeling Mercury Isotopic Fractionation in the Atmosphere Z. Song et al. 10.2139/ssrn.3994573
- Mercury Isotope Variations in Lake Sediment Cores in Response to Direct Mercury Emissions from Non-Ferrous Metal Smelters and Legacy Mercury Remobilization R. Sun et al. 10.1021/acs.est.2c02692
- The paradigm and recent progress in studying marine mercury isotopes R. SUN et al. 10.3724/j.issn.1007-2802.20240016
- Isotope Data Constrains Redox Chemistry of Atmospheric Mercury Z. Song et al. 10.1021/acs.est.4c02600
- Spatiotemporal variations of atmospheric mercury at urban and suburban areas in Southern Vietnam megacity: A preliminary year-round measurement study T. Hien et al. 10.1016/j.atmosenv.2024.120664
- Mercury stable isotopes revealing the atmospheric mercury circulation: A review of particulate bound mercury in China X. Qin et al. 10.1016/j.earscirev.2024.104681
- Modeling mercury isotopic fractionation in the atmosphere Z. Song et al. 10.1016/j.envpol.2022.119588
- Atmospheric Mercury Isotope Shifts in Response to Mercury Emissions from Underground Coal Fires R. Sun et al. 10.1021/acs.est.2c08637
- Plant cuticle as a possible palaeo-Hg proxy: Implications from Hg concentration data of extant Ginkgo L. and extinct ginkgoaleans L. Zhang et al. 10.1016/j.palaeo.2024.112214
- Atmospheric Mercury Concentrations and Isotopic Compositions Impacted by Typical Anthropogenic Mercury Emissions Sources C. Wang et al. 10.1021/acs.est.4c07649
- Characteristics of atmospheric total gaseous mercury concentrations (TGM) and meteorological parameters observed in Chennai metropolis, South India R. Ayyamperumal et al. 10.1007/s12517-021-07803-y
- Atmospheric gaseous mercury and associated health risk assessment in the economic capital of India M. Rao et al. 10.1007/s10661-024-12679-y
- Ecosystem Mercury Recovery and Health Benefit Under the Minamata Convention in a Changing Climate Q. Wu et al. 10.1007/s44169-022-00016-8
- Isotopic Characterization of Mercury Atmosphere–Foliage and Atmosphere–Soil Exchange in a Swiss Subalpine Coniferous Forest C. Chen et al. 10.1021/acs.est.3c03576
- The Earth's atmosphere – A stable isotope perspective and review J. Hoefs & R. Harmon 10.1016/j.apgeochem.2022.105355
- Stable Isotopes Reveal Photoreduction of Particle-Bound Mercury Driven by Water-Soluble Organic Carbon during Severe Haze K. Zhang et al. 10.1021/acs.est.2c01933
25 citations as recorded by crossref.
- Applying Passive Air Sampling and Isotopic Characterization to Assess Spatial Variability of Gaseous Elemental Mercury Across Ontario, Canada N. Szponar et al. 10.1029/2022JD037361
- Isotopic investigation of sources and processes affecting gaseous and particulate bound mercury in the east coast, South Korea H. Lee et al. 10.1016/j.scitotenv.2023.164404
- Changes in Atmospheric Gaseous Elemental Mercury Concentrations and Isotopic Compositions at Mt. Changbai During 2015–2021 and Mt. Ailao During 2017–2021 in China X. Wu et al. 10.1029/2022JD037749
- Sources and Transformation Mechanisms of Atmospheric Particulate Bound Mercury Revealed by Mercury Stable Isotopes C. Liu et al. 10.1021/acs.est.1c08065
- Sustained high atmospheric Hg level in Beijing during wet seasons suggests that anthropogenic pollution is continuing: Identification of potential sources C. Wang et al. 10.1016/j.envres.2022.113814
- Three thousand years of Hg pollution recorded in mangrove wetland sediments from South China M. Chen et al. 10.1016/j.envres.2024.118866
- Using Mercury Stable Isotopes to Quantify Bidirectional Water–Atmosphere Hg(0) Exchange Fluxes and Explore Controlling Factors H. Zhang et al. 10.1021/acs.est.3c01273
- Earth system modeling of mercury using CESM2 – Part 1: Atmospheric model CAM6-Chem/Hg v1.0 P. Zhang & Y. Zhang 10.5194/gmd-15-3587-2022
- Sources and risk assessment of atmospheric Hg during the 2022 Beijing Olympic Winter Games C. Wang et al. 10.1016/j.atmosenv.2023.119718
- Modeling Mercury Isotopic Fractionation in the Atmosphere Z. Song et al. 10.2139/ssrn.3994573
- Mercury Isotope Variations in Lake Sediment Cores in Response to Direct Mercury Emissions from Non-Ferrous Metal Smelters and Legacy Mercury Remobilization R. Sun et al. 10.1021/acs.est.2c02692
- The paradigm and recent progress in studying marine mercury isotopes R. SUN et al. 10.3724/j.issn.1007-2802.20240016
- Isotope Data Constrains Redox Chemistry of Atmospheric Mercury Z. Song et al. 10.1021/acs.est.4c02600
- Spatiotemporal variations of atmospheric mercury at urban and suburban areas in Southern Vietnam megacity: A preliminary year-round measurement study T. Hien et al. 10.1016/j.atmosenv.2024.120664
- Mercury stable isotopes revealing the atmospheric mercury circulation: A review of particulate bound mercury in China X. Qin et al. 10.1016/j.earscirev.2024.104681
- Modeling mercury isotopic fractionation in the atmosphere Z. Song et al. 10.1016/j.envpol.2022.119588
- Atmospheric Mercury Isotope Shifts in Response to Mercury Emissions from Underground Coal Fires R. Sun et al. 10.1021/acs.est.2c08637
- Plant cuticle as a possible palaeo-Hg proxy: Implications from Hg concentration data of extant Ginkgo L. and extinct ginkgoaleans L. Zhang et al. 10.1016/j.palaeo.2024.112214
- Atmospheric Mercury Concentrations and Isotopic Compositions Impacted by Typical Anthropogenic Mercury Emissions Sources C. Wang et al. 10.1021/acs.est.4c07649
- Characteristics of atmospheric total gaseous mercury concentrations (TGM) and meteorological parameters observed in Chennai metropolis, South India R. Ayyamperumal et al. 10.1007/s12517-021-07803-y
- Atmospheric gaseous mercury and associated health risk assessment in the economic capital of India M. Rao et al. 10.1007/s10661-024-12679-y
- Ecosystem Mercury Recovery and Health Benefit Under the Minamata Convention in a Changing Climate Q. Wu et al. 10.1007/s44169-022-00016-8
- Isotopic Characterization of Mercury Atmosphere–Foliage and Atmosphere–Soil Exchange in a Swiss Subalpine Coniferous Forest C. Chen et al. 10.1021/acs.est.3c03576
- The Earth's atmosphere – A stable isotope perspective and review J. Hoefs & R. Harmon 10.1016/j.apgeochem.2022.105355
- Stable Isotopes Reveal Photoreduction of Particle-Bound Mercury Driven by Water-Soluble Organic Carbon during Severe Haze K. Zhang et al. 10.1021/acs.est.2c01933
Latest update: 13 Dec 2024
Short summary
TGM concentrations and isotopic compositions in 10 Chinese cities showed strong seasonality with higher TGM concentrations and Δ199Hg and lower δ202Hg in summer. We found the seasonal variations in TGM concentrations and isotopic compositions were highly related to regional surface Hg(0) emissions, suggesting land surface Hg(0) emissions are an important source of atmospheric TGM that contribute dominantly to the seasonal variations in TGM concentrations and isotopic compositions.
TGM concentrations and isotopic compositions in 10 Chinese cities showed strong seasonality with...
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