Articles | Volume 21, issue 8
https://doi.org/10.5194/acp-21-5935-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-5935-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Apr 2021
Research article |
| 20 Apr 2021
| 20 Apr 2021
Parameterizing the vertical downward dispersion of ship exhaust gas in the near field
Ronny Badeke
CORRESPONDING AUTHOR
Hereon Institute of Coastal Environmental Chemistry, Helmholtz-Zentrum Hereon GmbH, 21502 Geesthacht, Germany
Volker Matthias
Hereon Institute of Coastal Environmental Chemistry, Helmholtz-Zentrum Hereon GmbH, 21502 Geesthacht, Germany
David Grawe
Center for Earth System Research and Sustainability (CEN),
Meteorological Institute, Universität Hamburg, 20146 Hamburg, Germany
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Cited articles
Affad, E., Saadeddine, S., Assou, M., and Sbaibi, A.: Effect of the relative
humidity on an industrial plume behavior, Glob. NEST J., 8, 297–305,
https://doi.org/10.30955/gnj.000294, 2006.
Aksoyoglu, S., Baltensperger, U., and Prévôt, A. S. H.: Contribution of ship emissions to the concentration and deposition of air pollutants in Europe, Atmos. Chem. Phys., 16, 1895–1906, https://doi.org/10.5194/acp-16-1895-2016, 2016.
Aulinger, A., Matthias, V., Zeretzke, M., Bieser, J., Quante, M., and Backes, A.: The impact of shipping emissions on air pollution in the greater North Sea region – Part 1: Current emissions and concentrations, Atmos. Chem. Phys., 16, 739–758, https://doi.org/10.5194/acp-16-739-2016, 2016.
Bai, S., Wen, Y., He, L., Liu, Y., Zhang, Y., Yu, Q., and Ma, W.:
Single-Vessel Plume Dispersion Simulation: Method and a Case Study Using
CALPUFF in the Yantian Port Area, Shenzhen (China), Int. J. Env. Res.
Pub. He., 17, 1–29, https://doi.org/10.3390/ijerph17217831, 2020.
Barregard, L., Molnár, P., Jonson, J. E., and Stockfelt, L.: Impact on
population health of baltic shipping emissions, Int. J. Env. Res. Pub.
He., 16, 1954, https://doi.org/10.3390/ijerph16111954, 2019.
Bieser, J., Aulinger, A., Matthias, V., Quante, M., and van der Gon, H. A. C.
D.: Vertical emission profiles for Europe based on plume rise calculations,
Environ. Pollut., 159, 2935–2946, https://doi.org/10.1016/j.envpol.2011.04.030,
2011.
Brandt, J., Silver, J. D., Christensen, J. H., Andersen, M. S., Bønløkke, J. H., Sigsgaard, T., Geels, C., Gross, A., Hansen, A. B., Hansen, K. M., Hedegaard, G. B., Kaas, E., and Frohn, L. M.: Assessment of past, present and future health-cost externalities of air pollution in Europe and the contribution from international ship traffic using the EVA model system, Atmos. Chem. Phys., 13, 7747–7764, https://doi.org/10.5194/acp-13-7747-2013, 2013.
Briggs, G. A.: Plume rise predictions, Lect. Air Pollut. Environ. Impact
Anal., 59–111, https://doi.org/10.1007/978-1-935704-23-2_3, 1982.
Broome, R. A., Cope, M. E., Goldsworthy, B., Goldsworthy, L., Emmerson, K.,
Jegasothy, E., and Morgan, G. G.: The mortality effect of ship-related fine
particulate matter in the Sydney greater metropolitan region of NSW,
Australia, Environ. Int., 87, 85–93, https://doi.org/10.1016/j.envint.2015.11.012,
2016.
Brunner, D., Kuhlmann, G., Marshall, J., Clément, V., Fuhrer, O., Broquet, G., Löscher, A., and Meijer, Y.: Accounting for the vertical distribution of emissions in atmospheric CO2 simulations, Atmos. Chem. Phys., 19, 4541–4559, https://doi.org/10.5194/acp-19-4541-2019, 2019.
CAT: Marine Power Systems, available at: https://www.cat.com/en_GB/products/new/power-systems/marine-power-systems.html, last access: 24
July 2020.
Chosson, F., Paoli, R., and Cuenot, B.: Ship plume dispersion rates in convective boundary layers for chemistry models, Atmos. Chem. Phys., 8, 4841–4853, https://doi.org/10.5194/acp-8-4841-2008, 2008.
Corbett, J. J., Winebrake, J. J., Green, E. H., Kasibhatla, P., Eyring, V.,
and Lauer, A.: Mortality from ship emissions: A global assessment, Environ.
Sci. Technol., 41, 8512–8518, https://doi.org/10.1021/es071686z, 2007.
Eyring, V., Isaksen, I. S. A., Berntsen, T., Collins, W. J., Corbett, J. J.,
Endresen, O., Grainger, R. G., Moldanova, J., Schlager, H., and Stevenson, D.
S.: Transport impacts on atmosphere and climate: Shipping, Atmos. Environ.,
44, 4735–4771, https://doi.org/10.1016/j.atmosenv.2009.04.059, 2010.
Grawe, D., Schlünzen, K. H., and Pascheke, F.: Comparison of results of
an obstacle resolving microscale model with wind tunnel data, Atmos.
Environ., 79, 495–509, https://doi.org/10.1016/j.atmosenv.2013.06.039, 2013.
Hanna, S. R., Schulman, L. L., Paine, R. J., Pleim, J. E., and Baer, M.:
Development and evaluation of the offshore and coastal dispersion model, J.
Air Pollut. Control Assoc., 35, 1039–1047,
https://doi.org/10.1080/00022470.1985.10466003, 1985.
Hulskotte, J. H. J. and Denier van der Gon, H. A. C.: Fuel consumption and
associated emissions from seagoing ships at berth derived from an on-board
survey, Atmos. Environ., 44, 1229–1236, https://doi.org/10.1016/j.atmosenv.2009.10.018,
2010.
Huszar, P., Cariolle, D., Paoli, R., Halenka, T., Belda, M., Schlager, H.,
Miksovsky, J. and Pisoft, P.: Modeling the regional impact of ship emissions
on NOx and ozone levels over the Eastern Atlantic and Western Europe using
ship plume parameterization, Atmos. Chem. Phys., 10, 6645–6660,
https://doi.org/10.5194/acp-10-6645-2010, 2010.
ICDC: Hamburg Boundary Layer Measurement Tower, available at: https://icdc.cen.uni-hamburg.de/en/weathermast-hamburg.html, last
access: 24 July 2020.
IMO: Sulphur oxides (SOx) and Particulate Matter (PM) – Regulation 14, available at: https://www.imo.org/en/OurWork/Environment/Pages/Sulphur-oxides-(SOx)-%E2%80%93-Regulation-14.aspx, last access: 13 April 2021.
Jalkanen, J.-P., Brink, A., Kalli, J., Pettersson, H., Kukkonen, J., and Stipa, T.: A modelling system for the exhaust emissions of marine traffic and its application in the Baltic Sea area, Atmos. Chem. Phys., 9, 9209–9223, https://doi.org/10.5194/acp-9-9209-2009, 2009.
Jalkanen, J.-P., Johansson, L., Kukkonen, J., Brink, A., Kalli, J., and Stipa, T.: Extension of an assessment model of ship traffic exhaust emissions for particulate matter and carbon monoxide, Atmos. Chem. Phys., 12, 2641–2659, https://doi.org/10.5194/acp-12-2641-2012, 2012.
Janicke, U. and Janicke, L.: A three-dimensional plume rise model for dry
and wet plumes, Atmos. Environ., 35, 877–890,
https://doi.org/10.1016/S1352-2310(00)00372-1, 2001.
Johansson, L., Jalkanen, J. P., and Kukkonen, J.: Global assessment of
shipping emissions in 2015 on a high spatial and temporal resolution, Atmos.
Environ., 167, 403–415, https://doi.org/10.1016/j.atmosenv.2017.08.042, 2017.
Karl, M., Bieser, J., Geyer, B., Matthias, V., Jalkanen, J.-P., Johansson, L., and Fridell, E.: Impact of a nitrogen emission control area (NECA) on the future air quality and nitrogen deposition to seawater in the Baltic Sea region, Atmos. Chem. Phys., 19, 1721–1752, https://doi.org/10.5194/acp-19-1721-2019, 2019.
Lee, J. H. W. and Cheung, V.: Generalized lagrangian model for buoyant jets
in current, J. Environ. Eng., 116, 1085–1106,
https://doi.org/10.1061/(ASCE)0733-9372(1990)116:6(1085), 1990.
Lin, H., Tao, J., Qian, Z. (Min), Ruan, Z., Xu, Y., Hang, J., Xu, X., Liu,
T., Guo, Y., Zeng, W., Xiao, J., Guo, L., Li, X., and Ma, W.: Shipping
pollution emission associated with increased cardiovascular mortality: A
time series study in Guangzhou, China, Environ. Pollut., 241, 862–868,
https://doi.org/10.1016/j.envpol.2018.06.027, 2018.
Liu, H., Fu, M., Jin, X., Shang, Y., Shindell, D., Faluvegi, G., Shindell,
C. and He, K.: Health and climate impacts of ocean-going vessels in East
Asia, Nat. Clim. Change, 6, 1037–1041, https://doi.org/10.1038/nclimate3083, 2016.
MAN: Two-stroke project guides, available at: https://marine.man-es.com/two-stroke/project-guides, last access: 24
July 2020.
Matthias, V., Aulinger, A., Backes, A., Bieser, J., Geyer, B., Quante, M., and Zeretzke, M.: The impact of shipping emissions on air pollution in the greater North Sea region – Part 2: Scenarios for 2030, Atmos. Chem. Phys., 16, 759–776, https://doi.org/10.5194/acp-16-759-2016, 2016.
Matthias, V., Arndt, J. A., Aulinger, A., Bieser, J., Denier van der Gon,
H., Kranenburg, R., Kuenen, J., Neumann, D., Pouliot, G. and Quante, M.:
Modeling emissions for three-dimensional atmospheric chemistry transport
models, J. Air Waste Manage., 68, 763–800,
https://doi.org/10.1080/10962247.2018.1424057, 2018.
Murena, F., Mocerino, L., Quaranta, F., and Toscano, D.: Impact on air
quality of cruise ship emissions in Naples, Italy, Atmos. Environ., 187,
70–83, https://doi.org/10.1016/j.atmosenv.2018.05.056, 2018.
Murphy, S., Agrawal, H., Sorooshian, A., Padró, L. T., Gates, H.,
Hersey, S., Welch, W. A., Jung, H., Miller, J. W., Cocker, D. R., Nenes, A.,
Jonsson, H. H., Flagan, R. C., and Seinfeld, J. H.: Comprehensive
simultaneous shipboard and airborne characterization of exhaust from a
modern container ship at sea, Environ. Sci. Technol., 43, 4626–4640,
https://doi.org/10.1021/es802413j, 2009.
Port of Hamburg: Vesseltypes, available at: https://www.hafen-hamburg.de/en/vessels/, last access: 24
July 2020.
Ramacher, M. O. P., Karl, M., Bieser, J., Jalkanen, J.-P., and Johansson, L.: Urban population exposure to NOx emissions from local shipping in three Baltic Sea harbour cities – a generic approach, Atmos. Chem. Phys., 19, 9153–9179, https://doi.org/10.5194/acp-19-9153-2019, 2019.
Salim, M. H., Schlünzen, K. H., Grawe, D., Boettcher, M., Gierisch, A. M. U., and Fock, B. H.: The microscale obstacle-resolving meteorological model MITRAS v2.0: model theory, Geosci. Model Dev., 11, 3427–3445, https://doi.org/10.5194/gmd-11-3427-2018, 2018.
Schatzmann, M.: An Integral Model of Plume Rise, Atmos. Environ., 13,
721–731, https://doi.org/10.1016/0004-6981(79)90202-6, 1979.
Schlünzen, K. H., Hinneburg, D., Knoth, O., Lambrecht, M., Leitl, B.,
López, S., Lüpkes, C., Panskus, H., Renner, E., Schatzmann, M.,
Schoenemeyer, T., Trepte, S., and Wolke, R.: Flow and transport in the
obstacle layer: First results of the micro-scale model MITRAS, J. Atmos.
Chem., 44, 113–130, https://doi.org/10.1023/A:1022420130032, 2003.
Schlünzen, K. H., Boettcher, M., Fock, B. H., Gierisch, A., Grawe, D.,
and Salim, M.: Scientific Documentation of the Multiscale Model System
M-SYS, MEMI Tech. Rep. 4, CEN, Univ. Hambg., 1–153, 2018.
Sofiev, M., Winebrake, J. J., Johansson, L., Carr, E. W., Prank, M., Soares,
J., Vira, J., Kouznetsov, R., Jalkanen, J. P., and Corbett, J. J.: Cleaner
fuels for ships provide public health benefits with climate tradeoffs, Nat.
Commun., 9, 1–12, https://doi.org/10.1038/s41467-017-02774-9, 2018.
Tzannatos, E.: Ship emissions and their externalities for Greece, Atmos.
Environ., 44, 2194–2202, https://doi.org/10.1016/j.atmosenv.2010.03.018, 2010.
United Nations Conference on Trade and Development: Review of maritime
transport 2019, United Nations, Geneva, available at:
https://unctad.org/en/Pages/Publications/Review-of-Maritime-Transport-(Series).aspx (last access: 13 April 2021),
2019.
Vesseltracker: Vessels, available at: https://www.vesseltracker.com/en/vessels.html, last access:
24 July 2020.
Vinken, G. C. M., Boersma, K. F., Jacob, D. J., and Meijer, E. W.: Accounting for non-linear chemistry of ship plumes in the GEOS-Chem global chemistry transport model, Atmos. Chem. Phys., 11, 11707–11722, https://doi.org/10.5194/acp-11-11707-2011, 2011.
von Glasow, R., Lawrence, M. G., Sander, R., and Crutzen, P. J.: Modeling the chemical effects of ship exhaust in the cloud-free marine boundary layer, Atmos. Chem. Phys., 3, 233–250, https://doi.org/10.5194/acp-3-233-2003, 2003.
Wang, C., Corbett, J. J., and Firestone, J.: Improving spatial representation
of global ship emissions inventories, Environ. Sci. Technol., 42, 193–199,
https://doi.org/10.1021/es0700799, 2008.
Wärtsilä: Diesel engines, available at:
https://www.wartsila.com/marine/build/engines-and-generating-sets/diesel-engines,
last access: 24 July 2020.
Zhang, Y., Feng, J., Liu, C., Zhao, J., Ma, W., Huang, C., An, J., Shen, Y.,
Fu, Q., Wang, S., Ding, D., Ge, W., Fung, F., Manokaran, K., Patton, A. P.,
Walker, K. D., and Kan, H.: Impacts of Shipping on Air PollutantEmissions,
Air Quality, and Health in the Yangtze River Delta and Shanghai, China
Special Report 22, Heal. Eff. Inst. Spec. Rep., 22, 1–78, 2019.
Short summary
This work aims to describe the physical distribution of ship exhaust gases in the near field, e.g., inside of a harbor. Results were calculated with a mathematical model for different meteorological and technical conditions. It has been shown that large vessels like cruise ships have a significant effect of up to 55 % downward movement of exhaust gas, as they can disturb the ground near wind circulation. This needs to be considered in urban air pollution studies.
This work aims to describe the physical distribution of ship exhaust gases in the near field,...
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