Articles | Volume 21, issue 8
https://doi.org/10.5194/acp-21-5935-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-5935-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Apr 2021
Research article |
| 20 Apr 2021
| 20 Apr 2021
Parameterizing the vertical downward dispersion of ship exhaust gas in the near field
Ronny Badeke
CORRESPONDING AUTHOR
Hereon Institute of Coastal Environmental Chemistry, Helmholtz-Zentrum Hereon GmbH, 21502 Geesthacht, Germany
Volker Matthias
Hereon Institute of Coastal Environmental Chemistry, Helmholtz-Zentrum Hereon GmbH, 21502 Geesthacht, Germany
David Grawe
Center for Earth System Research and Sustainability (CEN),
Meteorological Institute, Universität Hamburg, 20146 Hamburg, Germany
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Ronny Badeke, Volker Matthias, Matthias Karl, and David Grawe
Geosci. Model Dev., 15, 4077–4103, https://doi.org/10.5194/gmd-15-4077-2022, https://doi.org/10.5194/gmd-15-4077-2022, 2022
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For air quality modeling studies, it is very important to distribute pollutants correctly into the model system. This has not yet been done for shipping pollution in great detail. We studied the effects of different vertical distributions of shipping pollutants on the urban air quality and derived advanced formulas for it. These formulas take weather conditions and ship-specific parameters like the exhaust gas temperature into account.
Volker Matthias, Markus Quante, Jan A. Arndt, Ronny Badeke, Lea Fink, Ronny Petrik, Josefine Feldner, Daniel Schwarzkopf, Eliza-Maria Link, Martin O. P. Ramacher, and Ralf Wedemann
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COVID-19 lockdown measures in spring 2020 led to cleaner air in central Europe. Densely populated areas benefitted mainly from largely reduced NO2 concentrations, while rural areas experienced lower reductions in NO2 but also lower ozone concentrations. Very low particulate matter (PM) concentrations in parts of Europe were not an effect of lockdown measures. Model simulations show that modified weather conditions are more significant for ozone and PM than severe traffic emission reductions.
Lea Fink, Matthias Karl, Volker Matthias, Sonia Oppo, Richard Kranenburg, Jeroen Kuenen, Sara Jutterström, Jana Moldanova, Elisa Majamäki, and Jukka-Pekka Jalkanen
Atmos. Chem. Phys., 23, 10163–10189, https://doi.org/10.5194/acp-23-10163-2023, https://doi.org/10.5194/acp-23-10163-2023, 2023
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The Mediterranean Sea is a heavily trafficked shipping area, and air quality monitoring stations in numerous cities along the Mediterranean coast have detected high levels of air pollutants originating from shipping emissions. The current study investigates how existing restrictions on shipping-related emissions to the atmosphere ensure compliance with legislation. Focus was laid on fine particles and particle species, which were simulated with five different chemical transport models.
Lea Fink, Matthias Karl, Volker Matthias, Sonia Oppo, Richard Kranenburg, Jeroen Kuenen, Jana Moldanova, Sara Jutterström, Jukka-Pekka Jalkanen, and Elisa Majamäki
Atmos. Chem. Phys., 23, 1825–1862, https://doi.org/10.5194/acp-23-1825-2023, https://doi.org/10.5194/acp-23-1825-2023, 2023
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Potential ship impact on air pollution in the Mediterranean Sea was simulated with five chemistry transport models. An evaluation of the results for NO2 and O3 air concentrations and dry deposition is presented. Emission data, modeled year and domain were the same. Model run outputs were compared to measurements from background stations. We focused on comparing model outputs regarding the concentration of regulatory pollutants and the relative ship impact on total air pollution concentrations.
Ronny Badeke, Volker Matthias, Matthias Karl, and David Grawe
Geosci. Model Dev., 15, 4077–4103, https://doi.org/10.5194/gmd-15-4077-2022, https://doi.org/10.5194/gmd-15-4077-2022, 2022
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For air quality modeling studies, it is very important to distribute pollutants correctly into the model system. This has not yet been done for shipping pollution in great detail. We studied the effects of different vertical distributions of shipping pollutants on the urban air quality and derived advanced formulas for it. These formulas take weather conditions and ship-specific parameters like the exhaust gas temperature into account.
Sara Jutterström, Filip Moldan, Jana Moldanová, Matthias Karl, Volker Matthias, and Maximilian Posch
Atmos. Chem. Phys., 21, 15827–15845, https://doi.org/10.5194/acp-21-15827-2021, https://doi.org/10.5194/acp-21-15827-2021, 2021
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For the Baltic Sea countries, shipping emissions are an important source of air pollution. This study investigates the contribution of shipping emissions to the acidification and eutrophication of soils and freshwater within the airshed of the Baltic Sea in the years 2012 and 2040. The implementation of emission control areas and improving energy efficiency significantly reduces the negative impact on ecosystems expressed as a decrease in the exceedance of critical loads for sulfur and nitrogen.
Volker Matthias, Markus Quante, Jan A. Arndt, Ronny Badeke, Lea Fink, Ronny Petrik, Josefine Feldner, Daniel Schwarzkopf, Eliza-Maria Link, Martin O. P. Ramacher, and Ralf Wedemann
Atmos. Chem. Phys., 21, 13931–13971, https://doi.org/10.5194/acp-21-13931-2021, https://doi.org/10.5194/acp-21-13931-2021, 2021
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COVID-19 lockdown measures in spring 2020 led to cleaner air in central Europe. Densely populated areas benefitted mainly from largely reduced NO2 concentrations, while rural areas experienced lower reductions in NO2 but also lower ozone concentrations. Very low particulate matter (PM) concentrations in parts of Europe were not an effect of lockdown measures. Model simulations show that modified weather conditions are more significant for ozone and PM than severe traffic emission reductions.
Martin O. P. Ramacher, Lin Tang, Jana Moldanová, Volker Matthias, Matthias Karl, Erik Fridell, and Lasse Johansson
Atmos. Chem. Phys., 20, 10667–10686, https://doi.org/10.5194/acp-20-10667-2020, https://doi.org/10.5194/acp-20-10667-2020, 2020
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The effects of shipping emissions on air quality and health in the harbour city of Gothenburg were simulated for different scenarios for the year 2040 with coupled regional and city-scale chemistry transport models to evaluate the impact of regional emission regulations and onshore electricity for ships at berth. The results show that contributions of shipping to exposure and associated health impacts from particulate matter and NO2 decrease significantly compared to 2012 in all scenarios.
Lin Tang, Martin O. P. Ramacher, Jana Moldanová, Volker Matthias, Matthias Karl, Lasse Johansson, Jukka-Pekka Jalkanen, Katarina Yaramenka, Armin Aulinger, and Malin Gustafsson
Atmos. Chem. Phys., 20, 7509–7530, https://doi.org/10.5194/acp-20-7509-2020, https://doi.org/10.5194/acp-20-7509-2020, 2020
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The effects of shipping emissions on air quality and health in the harbour city of Gothenburg were simulated for 2012 with coupled regional and city-scale chemistry transport models. The results show that contributions of shipping to exposure and health impacts from particulate matter and NO2 are significant and that shipping-related exposure to PM is dominated by emissions from regional shipping outside the city domain and is larger than exposure related to emissions from local road traffic.
Fan Zhang, Hai Guo, Yingjun Chen, Volker Matthias, Yan Zhang, Xin Yang, and Jianmin Chen
Atmos. Chem. Phys., 20, 1549–1564, https://doi.org/10.5194/acp-20-1549-2020, https://doi.org/10.5194/acp-20-1549-2020, 2020
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Particulate matter (PM) emitted from ships has gained more attention in recent decades. Organic matter, elemental carbon, water-soluble ions and heavy metals in PM and particle numbers are the main points. However, studies of detailed chemical compositions in particles with different size ranges emitted from ships are in shortage. This study could bring new and detailed measurement data into the field of size-segregated particles from ships and be of great source emission interest.
Daniel Neumann, Matthias Karl, Hagen Radtke, Volker Matthias, René Friedland, and Thomas Neumann
Ocean Sci., 16, 115–134, https://doi.org/10.5194/os-16-115-2020, https://doi.org/10.5194/os-16-115-2020, 2020
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The study evaluates how much bioavailable nitrogen is contributed to the nitrogen budget of the western Baltic Sea by deposition of shipping-emitted nitrogen oxides. Bioavailable nitrogen compounds are nutrients for phytoplankton (algae). Excessive input of nutrients into water bodies may lead to eutrophication: more algal blooms with subsequently more oxygen limitation at the seafloor. Hence, reducing shipping emissions might reduce the anthropogenic pressure on the marine ecosystem.
Matthias Karl, Jan Eiof Jonson, Andreas Uppstu, Armin Aulinger, Marje Prank, Mikhail Sofiev, Jukka-Pekka Jalkanen, Lasse Johansson, Markus Quante, and Volker Matthias
Atmos. Chem. Phys., 19, 7019–7053, https://doi.org/10.5194/acp-19-7019-2019, https://doi.org/10.5194/acp-19-7019-2019, 2019
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The effect of ship emissions on the regional air quality in the Baltic Sea region was investigated with three regional chemistry transport model systems. The ship influence on air quality is shown to depend on the boundary conditions, meteorological data and aerosol formation and deposition schemes that are used in these models. The study provides a reliable approach for the evaluation of policy options regarding emission regulations for ship traffic in the Baltic Sea.
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Atmos. Chem. Phys., 19, 1721–1752, https://doi.org/10.5194/acp-19-1721-2019, https://doi.org/10.5194/acp-19-1721-2019, 2019
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Air emissions of nitrogen oxides from ship traffic in the Baltic Sea are a health concern in coastal areas of the Baltic Sea region. We find that the introduction of the nitrogen emission control area (NECA) is critical for reducing ship emissions of nitrogen oxides to levels that are low enough to sustainably dampen ozone production. The decline of the ship-related nitrogen deposition to the Baltic Sea between 2012 and 2040 varies between 46 % and 78 % in different regulation scenarios.
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Geosci. Model Dev., 11, 3427–3445, https://doi.org/10.5194/gmd-11-3427-2018, https://doi.org/10.5194/gmd-11-3427-2018, 2018
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Atmos. Chem. Phys., 17, 6925–6955, https://doi.org/10.5194/acp-17-6925-2017, https://doi.org/10.5194/acp-17-6925-2017, 2017
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We conducted a multi model study to investigate our ability to reproduce the vertical distribution of mercury in the atmosphere. For this, we used observational data from over 40 aircraft flights in EU and US. We compared observations to the results of seven chemistry transport models and found that the models are able to reproduce vertical gradients of total and elemental Hg. Finally, we found that different chemical reactions seem responsible for the oxidation of Hg depending on altitude.
Oleg Travnikov, Hélène Angot, Paulo Artaxo, Mariantonia Bencardino, Johannes Bieser, Francesco D'Amore, Ashu Dastoor, Francesco De Simone, María del Carmen Diéguez, Aurélien Dommergue, Ralf Ebinghaus, Xin Bin Feng, Christian N. Gencarelli, Ian M. Hedgecock, Olivier Magand, Lynwill Martin, Volker Matthias, Nikolay Mashyanov, Nicola Pirrone, Ramesh Ramachandran, Katie Alana Read, Andrei Ryjkov, Noelle E. Selin, Fabrizio Sena, Shaojie Song, Francesca Sprovieri, Dennis Wip, Ingvar Wängberg, and Xin Yang
Atmos. Chem. Phys., 17, 5271–5295, https://doi.org/10.5194/acp-17-5271-2017, https://doi.org/10.5194/acp-17-5271-2017, 2017
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The study provides a complex analysis of processes governing Hg fate in the atmosphere involving both measurement data and simulation results of chemical transport models. Evaluation of the model simulations and numerical experiments against observations allows explaining spatial and temporal variations of Hg concentration in the near-surface atmospheric layer and shows possibility of multiple pathways of Hg oxidation occurring concurrently in various parts of the atmosphere.
Christian N. Gencarelli, Johannes Bieser, Francesco Carbone, Francesco De Simone, Ian M. Hedgecock, Volker Matthias, Oleg Travnikov, Xin Yang, and Nicola Pirrone
Atmos. Chem. Phys., 17, 627–643, https://doi.org/10.5194/acp-17-627-2017, https://doi.org/10.5194/acp-17-627-2017, 2017
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Atmospheric deposition is an important pathway by which Hg reaches marine ecosystems, where it can be methylated and enter the base of food chain. High resolution numerical experiments has been performed in order to investigate the contributions (sensitivity) of the Hg anthtropogenic emissions, speciation and atmospherical chemical reactions on Hg depositions over Europe. The comparison of wet deposition fluxes and concentrations measured on 28 monitioring sites were used to support the analysis.
Daniel Neumann, Volker Matthias, Johannes Bieser, Armin Aulinger, and Markus Quante
Atmos. Chem. Phys., 16, 9905–9933, https://doi.org/10.5194/acp-16-9905-2016, https://doi.org/10.5194/acp-16-9905-2016, 2016
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Atmospheric sea salt particles provide surface area for the condensation of gaseous substances and, thus, impact these substances' atmospheric residence time and chemical reactions. The number and size of sea salt particles govern the strength of these impacts. Therefore, these parameters should be reflected accurately in chemistry transport models. In this study, three different sea salt emission functions are compared in order to evaluate which one is best suited for the given model setup.
Fan Zhang, Yingjun Chen, Chongguo Tian, Diming Lou, Jun Li, Gan Zhang, and Volker Matthias
Atmos. Chem. Phys., 16, 6319–6334, https://doi.org/10.5194/acp-16-6319-2016, https://doi.org/10.5194/acp-16-6319-2016, 2016
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In this study, on-board tests of three offshore vessels in China have been carried out for the first time. Emission factors for gaseous species, PM, and relevant chemical components (OC, EC, metal elements, and water soluble ions) in different operating modes are given, which means a lot for estimating contributions of ships to atmosphere and calculating emission inventories of ships. Additionally, impacts of engine speed on NOx emission factors are discussed for the first time.
Daniel Neumann, Volker Matthias, Johannes Bieser, Armin Aulinger, and Markus Quante
Atmos. Chem. Phys., 16, 2921–2942, https://doi.org/10.5194/acp-16-2921-2016, https://doi.org/10.5194/acp-16-2921-2016, 2016
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Sea salt emissions were updated to be dependent on salinity which improved sodium predictions in the Baltic Sea region. The impact of sea salt on atmospheric nitrate and ammonium concentrations and on nitrogen deposition in the North and Baltic Sea region is assessed. Sea salt has a low effect on nitrate concentrations but does not improve them. 3 to 7 % of the nitrogen deposition into the North Sea is accounted to the presence of sea salt. In the Baltic Sea, the contribution is negligible.
V. Matthias, A. Aulinger, A. Backes, J. Bieser, B. Geyer, M. Quante, and M. Zeretzke
Atmos. Chem. Phys., 16, 759–776, https://doi.org/10.5194/acp-16-759-2016, https://doi.org/10.5194/acp-16-759-2016, 2016
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Scenarios for future shipping emissions in the North Sea were developed. Compared to today, the contribution of shipping to the nitrogen dioxide and ozone concentrations will increase due to the expected enhanced traffic by more than 20 % and 5 %, respectively, by 2030 if no regulation for further emission reductions is implemented. PM2.5 will decrease slightly because the sulfur content in ship fuels will be reduced.
A. Aulinger, V. Matthias, M. Zeretzke, J. Bieser, M. Quante, and A. Backes
Atmos. Chem. Phys., 16, 739–758, https://doi.org/10.5194/acp-16-739-2016, https://doi.org/10.5194/acp-16-739-2016, 2016
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A multi-model approach consisting of a bottom-up ship emissions model and a chemistry transport model was used to evaluate the impact of shipping on air quality in North Sea bordering countries. As an example, the results of the simulations indicated that the relative contribution of ships to NO2 concentration levels ashore close to the sea can reach up to 25 % in summer and 15 % in winter. Some hundred kilometers away from the sea, the contribution was about 6 % in summer and 4 % in winter.
J. Zhu, T. Wang, J. Bieser, and V. Matthias
Atmos. Chem. Phys., 15, 8767–8779, https://doi.org/10.5194/acp-15-8767-2015, https://doi.org/10.5194/acp-15-8767-2015, 2015
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This study estimated the contributions to mercury concentration and deposition in easter China from seven categories of emission sources by CMAQ-Hg. Also, this study focuses on diagnostic and process analyses for atmospheric mercury pollution formation and on identification of the dominant atmospheric processes for mercury.
E. Solazzo, R. Bianconi, G. Pirovano, M. D. Moran, R. Vautard, C. Hogrefe, K. W. Appel, V. Matthias, P. Grossi, B. Bessagnet, J. Brandt, C. Chemel, J. H. Christensen, R. Forkel, X. V. Francis, A. B. Hansen, S. McKeen, U. Nopmongcol, M. Prank, K. N. Sartelet, A. Segers, J. D. Silver, G. Yarwood, J. Werhahn, J. Zhang, S. T. Rao, and S. Galmarini
Geosci. Model Dev., 6, 791–818, https://doi.org/10.5194/gmd-6-791-2013, https://doi.org/10.5194/gmd-6-791-2013, 2013
Related subject area
Subject: Dynamics | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
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Using a numerical atmospheric model, we found that cooling sea surface temperatures along the southern coast of West Africa in July cause the “little dry season”. This effect reduces humidity and pollutant transport inland, potentially enhancing West Africa's synoptic and seasonal forecasting.
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Atmos. Chem. Phys., 23, 14451–14479, https://doi.org/10.5194/acp-23-14451-2023, https://doi.org/10.5194/acp-23-14451-2023, 2023
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Accurate fog forecasting is difficult in a complex environment. Spatial variations in soil moisture could impact fog. Here, we carried out fog simulations with spatially different soil moisture in complex topography. The soil moisture was calculated using satellite observations. The results show that the spatial variations in soil moisture do not have a significant impact on where fog occurs but do impact how long fog lasts. This finding could improve fog forecasts in the future.
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In this study, we quantitatively study the effect of the boundary layer low-level jet (BLLJ) on fast fog spatial propagation; i.e., the fog area expands very fast along a certain direction. The wind speed (10 m s−1) and direction (southeast) of the BLLJ core are consistent with fog propagation (9.6 m s−1). The BLLJ-induced temperature and moisture advections are possible reasons for fast fog propagation. The propagation speed would decrease by 6.4 m s−1 if these advections were turned off.
Miriam Saraceni, Lorenzo Silvestri, Peter Bechtold, and Paolina Bongioannini Cerlini
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This study focuses on three medicanes, tropical-like cyclones that form in the Mediterranean Sea, studied by ensemble forecasting. This involved multiple simulations of the same event by varying initial conditions and model physics parameters, especially related to convection, which showed comparable results. It is found that medicane development is influenced by the model's ability to predict precursor events and the interaction between upper and lower atmosphere dynamics and thermodynamics.
Andrew R. Jones, Susan J. Leadbetter, and Matthew C. Hort
Atmos. Chem. Phys., 23, 12477–12503, https://doi.org/10.5194/acp-23-12477-2023, https://doi.org/10.5194/acp-23-12477-2023, 2023
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The paper explores spread and calibration properties of ensemble atmospheric dispersion forecasts for hypothetical release events. Real-time forecasts from an ensemble weather prediction system were used to generate an ensemble of dispersion predictions and assessed against simulations produced using analysis meteorology. Results demonstrate good performance overall but highlight more skilful predictions for material released in the upper air compared with releases near the surface.
Jason A. Otkin, Lee M. Cronce, Jonathan L. Case, R. Bradley Pierce, Monica Harkey, Allen Lenzen, David S. Henderson, Zac Adelman, Tsengel Nergui, and Christopher R. Hain
Atmos. Chem. Phys., 23, 7935–7954, https://doi.org/10.5194/acp-23-7935-2023, https://doi.org/10.5194/acp-23-7935-2023, 2023
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We performed model simulations to assess the impact of different parameterization schemes, surface initialization datasets, and analysis nudging on lower-tropospheric conditions near Lake Michigan. Simulations were run with high-resolution, real-time datasets depicting lake surface temperatures, green vegetation fraction, and soil moisture. The most accurate results were obtained when using high-resolution sea surface temperature and soil datasets to constrain the model simulations.
Mark T. Richardson, Brian H. Kahn, and Peter Kalmus
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Convection over land often triggers hours after a satellite last passed overhead and measured the state of the atmosphere, and during those hours the atmosphere can change greatly. Here we show that it is possible to reconstruct most of those changes by using weather forecast winds to predict where warm and moist air parcels will travel. The results can be used to better predict where precipitation is likely to happen in the hours after satellite measurements.
Lars Hoffmann, Paul Konopka, Jan Clemens, and Bärbel Vogel
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Atmospheric convection plays a key role in tracer transport in the troposphere. Global meteorological forecasts and reanalyses typically have a coarse spatiotemporal resolution that does not adequately resolve the dynamics, transport, and mixing of air associated with storm systems or deep convection. We discuss the application of the extreme convection parameterization in a Lagrangian transport model to improve simulations of tracer transport from the boundary layer into the free troposphere.
Angshuman Modak and Thorsten Mauritsen
Atmos. Chem. Phys., 23, 7535–7549, https://doi.org/10.5194/acp-23-7535-2023, https://doi.org/10.5194/acp-23-7535-2023, 2023
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We provide an improved estimate of equilibrium climate sensitivity (ECS) constrained based on the instrumental temperature record including the corrections for the pattern effect. The improved estimate factors in the uncertainty caused by the underlying sea-surface temperature datasets used in the estimates of pattern effect. This together with the inter-model spread lifts the corresponding IPCC AR6 estimate to 3.2 K [1.8 to 11.0], which is lower and better constrained than in past studies.
Xiaoyu Sun, Mathias Palm, Katrin Müller, Jonas Hachmeister, and Justus Notholt
Atmos. Chem. Phys., 23, 7075–7090, https://doi.org/10.5194/acp-23-7075-2023, https://doi.org/10.5194/acp-23-7075-2023, 2023
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The tropical western Pacific (TWP) is an active interhemispheric transport region contributing significantly to the global climate. A method to determine the chemical equator was developed by model simulations of a virtual passive tracer to analyze transport in the tropics, with a focus on the TWP region. We compare the chemical equator with tropical rain belts and wind fields and obtain a vertical pattern of interhemispheric transport processes which shows tilt structure in certain seasons.
Andrew E. Schuh and Andrew R. Jacobson
Atmos. Chem. Phys., 23, 6285–6297, https://doi.org/10.5194/acp-23-6285-2023, https://doi.org/10.5194/acp-23-6285-2023, 2023
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A comparison of atmospheric carbon dioxide concentrations resulting from two different atmospheric transport models showed large differences in predicted concentrations with significant space–time correlations. The vertical mixing of long-lived trace gases by convection was determined to be the main driver of these differences. The resulting uncertainty was deemed significant to the application of using atmospheric gradients of carbon dioxide to estimate surface fluxes of carbon dioxide.
Qike Yang, Xiaoqing Wu, Xiaodan Hu, Zhiyuan Wang, Chun Qing, Tao Luo, Pengfei Wu, Xianmei Qian, and Yiming Guo
Atmos. Chem. Phys., 23, 6339–6355, https://doi.org/10.5194/acp-23-6339-2023, https://doi.org/10.5194/acp-23-6339-2023, 2023
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The AMPS-forecasted Richardson number was first comprehensively validated over the Antarctic continent. Some potential underlying reasons for the discrepancies between the forecasts and observations were analyzed. The underlying physical processes of triggering atmospheric turbulence in Antarctica were investigated. Our results suggest that the estimated Richardson number by the AMPS is reasonable and the turbulence conditions in Antarctica are well revealed.
Edward Groot and Holger Tost
Atmos. Chem. Phys., 23, 6065–6081, https://doi.org/10.5194/acp-23-6065-2023, https://doi.org/10.5194/acp-23-6065-2023, 2023
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It is shown that the outflow from cumulonimbus clouds or thunderstorms in the upper troposphere and lower stratosphere in idealized high-resolution simulations (LESs) depends linearly on the net amount of latent heat released by the cloud for fixed geometry of the clouds. However, it is shown that, in more realistic situations, convective organization and aggregation (collecting mechanisms of cumulonimbus clouds) affect the amount of outflow non-linearly through non-idealized geometry.
Robert Hanfland, Dominik Brunner, Christiane Voigt, Alina Fiehn, Anke Roiger, and Margit Pattantyús-Ábrahám
EGUsphere, https://doi.org/10.5194/egusphere-2023-245, https://doi.org/10.5194/egusphere-2023-245, 2023
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In order to simulate the 3D structure of the exhaust plume within the planetary boundary layer in agreement with real plumes, we analysed the turbulence properties of five different turbulence models to understand their abilities of mixing and compared their simulated 3D dispersion patterns with airborn in situ measurements. The deviations between simulations and observation are quantified revealing one turbulence model that agrees best under the given atmosperic conditions.
Zixuan Jia, Carlos Ordóñez, Ruth M. Doherty, Oliver Wild, Steven T. Turnock, and Fiona M. O'Connor
Atmos. Chem. Phys., 23, 2829–2842, https://doi.org/10.5194/acp-23-2829-2023, https://doi.org/10.5194/acp-23-2829-2023, 2023
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This study investigates the influence of the winter large-scale circulation on daily concentrations of PM2.5 and their sensitivity to emissions. The new proposed circulation index can effectively distinguish different levels of air pollution and explain changes in PM2.5 sensitivity to emissions from local and surrounding regions. We then project future changes in PM2.5 concentrations using this index and find an increase in PM2.5 concentrations over the region due to climate change.
Chao Lin, Yunyi Wang, Ryozo Ooka, Cédric Flageul, Youngseob Kim, Hideki Kikumoto, Zhizhao Wang, and Karine Sartelet
Atmos. Chem. Phys., 23, 1421–1436, https://doi.org/10.5194/acp-23-1421-2023, https://doi.org/10.5194/acp-23-1421-2023, 2023
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In this study, SSH-aerosol, a modular box model that simulates the evolution of gas, primary, and secondary aerosols, is coupled with the computational fluid dynamics (CFD) software, OpenFOAM and Code_Saturne. The transient dispersion of pollutants emitted from traffic in a street canyon of Greater Paris is simulated. The coupled model achieved better agreement in NO2 and PM10 with measurement data than the conventional CFD simulation which regards pollutants as passive scalars.
Johannes Mikkola, Victoria A. Sinclair, Marja Bister, and Federico Bianchi
Atmos. Chem. Phys., 23, 821–842, https://doi.org/10.5194/acp-23-821-2023, https://doi.org/10.5194/acp-23-821-2023, 2023
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Local winds in four valleys located in the Nepal Himalayas are studied by means of high-resolution meteorological modelling. Well-defined daytime up-valley winds are simulated in all of the valleys with some variation in the flow depth and strength among the valleys and their parts. Parts of the valleys with a steep valley floor inclination (2–5°) are associated with weaker and shallower daytime up-valley winds compared with the parts that have nearly flat valley floors (< 1°).
Edward Groot and Holger Tost
Atmos. Chem. Phys., 23, 565–585, https://doi.org/10.5194/acp-23-565-2023, https://doi.org/10.5194/acp-23-565-2023, 2023
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Thunderstorm systems play an important role in the dynamics of the Earth’s atmosphere, and some of them form a well-organised line: squall lines. Simulations of such squall lines with very small initial perturbations are compared to a reference simulation. The evolution of perturbations and processes amplifying them are analysed. It is shown that the formation of new secondary thunderstorm cells (after the initial primary cells) directly ahead of the line affects the spread strongly.
Matthias Nützel, Sabine Brinkop, Martin Dameris, Hella Garny, Patrick Jöckel, Laura L. Pan, and Mijeong Park
Atmos. Chem. Phys., 22, 15659–15683, https://doi.org/10.5194/acp-22-15659-2022, https://doi.org/10.5194/acp-22-15659-2022, 2022
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During the Asian summer monsoon season, a large high-pressure system is present at levels close to the tropopause above Asia. We analyse how air masses are transported from surface levels to this high-pressure system, which shows distinct features from the surrounding air masses. To this end, we employ multiannual data from two complementary models that allow us to analyse the climatology as well as the interannual and intraseasonal variability of these transport pathways.
Alice Crawford, Tianfeng Chai, Binyu Wang, Allison Ring, Barbara Stunder, Christopher P. Loughner, Michael Pavolonis, and Justin Sieglaff
Atmos. Chem. Phys., 22, 13967–13996, https://doi.org/10.5194/acp-22-13967-2022, https://doi.org/10.5194/acp-22-13967-2022, 2022
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This study describes the development of a workflow which produces probabilistic and quantitative forecasts of volcanic ash in the atmosphere. The workflow includes methods of incorporating satellite observations of the ash cloud into a modeling framework as well as verification statistics that can be used to guide further model development and provide information for risk-based approaches to flight planning.
Alessandro Carlo Maria Savazzi, Louise Nuijens, Irina Sandu, Geet George, and Peter Bechtold
Atmos. Chem. Phys., 22, 13049–13066, https://doi.org/10.5194/acp-22-13049-2022, https://doi.org/10.5194/acp-22-13049-2022, 2022
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Winds are of great importance for the transport of energy and moisture in the atmosphere. In this study we use measurements from the EUREC4A field campaign and several model experiments to understand the wind bias in the forecasts produced by the European Centre for Medium-Range Weather Forecasts. We are able to link the model errors to heights above 2 km and to the representation of the diurnal cycle of winds: the model makes the winds too slow in the morning and too strong in the evening.
Ivo Neefjes, Roope Halonen, Hanna Vehkamäki, and Bernhard Reischl
Atmos. Chem. Phys., 22, 11155–11172, https://doi.org/10.5194/acp-22-11155-2022, https://doi.org/10.5194/acp-22-11155-2022, 2022
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Collisions between ionic and dipolar molecules and clusters facilitate the formation of atmospheric aerosol particles, which affect global climate and air quality. We compared often-used classical approaches for calculating ion–dipole collision rates with robust atomistic computer simulations. While classical approaches work for simple ions and dipoles only, our modeling approach can also efficiently calculate reasonable collision properties for more complex systems.
Alice Maison, Cédric Flageul, Bertrand Carissimo, Yunyi Wang, Andrée Tuzet, and Karine Sartelet
Atmos. Chem. Phys., 22, 9369–9388, https://doi.org/10.5194/acp-22-9369-2022, https://doi.org/10.5194/acp-22-9369-2022, 2022
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This paper presents a parameterization of the tree crown effect on air flow and pollutant dispersion in a street network model used to simulate air quality at the street level. The new parameterization is built using a finer-scale model (computational fluid dynamics). The tree effect increases with the leaf area index and the crown volume fraction of the trees; the street horizontal velocity is reduced by up to 68 % and the vertical transfer into or out of the street by up to 23 %.
Natalie J. Harvey, Helen F. Dacre, Cameron Saint, Andrew T. Prata, Helen N. Webster, and Roy G. Grainger
Atmos. Chem. Phys., 22, 8529–8545, https://doi.org/10.5194/acp-22-8529-2022, https://doi.org/10.5194/acp-22-8529-2022, 2022
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In the event of a volcanic eruption, airlines need to make decisions about which routes are safe to operate and ensure that airborne aircraft land safely. The aim of this paper is to demonstrate the application of a statistical technique that best combines ash information from satellites and a suite of computer forecasts of ash concentration to provide a range of plausible estimates of how much volcanic ash emitted from a volcano is available to undergo long-range transport.
Jean-Pierre Chaboureau, Laurent Labbouz, Cyrille Flamant, and Alma Hodzic
Atmos. Chem. Phys., 22, 8639–8658, https://doi.org/10.5194/acp-22-8639-2022, https://doi.org/10.5194/acp-22-8639-2022, 2022
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Ground-based, spaceborne and rare airborne observations of biomass burning aerosols (BBAs) during the AEROCLO-sA field campaign in 2017 are complemented with convection-permitting simulations with online trajectories. The results show that the radiative effect of the BBA accelerates the southern African easterly jet and generates upward motions that transport the BBAs to higher altitudes and farther southwest.
Annika Drews, Wenjuan Huo, Katja Matthes, Kunihiko Kodera, and Tim Kruschke
Atmos. Chem. Phys., 22, 7893–7904, https://doi.org/10.5194/acp-22-7893-2022, https://doi.org/10.5194/acp-22-7893-2022, 2022
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Solar irradiance varies with a period of approximately 11 years. Using a unique large chemistry–climate model dataset, we investigate the solar surface signal in the North Atlantic and European region and find that it changes over time, depending on the strength of the solar cycle. For the first time, we estimate the potential predictability associated with including realistic solar forcing in a model. These results may improve seasonal to decadal predictions of European climate.
Shipra Jain, Ruth M. Doherty, David Sexton, Steven Turnock, Chaofan Li, Zixuan Jia, Zongbo Shi, and Lin Pei
Atmos. Chem. Phys., 22, 7443–7460, https://doi.org/10.5194/acp-22-7443-2022, https://doi.org/10.5194/acp-22-7443-2022, 2022
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We provide a range of future projections of winter haze and clear conditions over the North China Plain (NCP) using multiple simulations from a climate model for the high-emission scenario (RCP8.5). The frequency of haze conducive weather is likely to increase whereas the frequency of clear weather is likely to decrease in future. The total number of hazy days for a given winter can be as much as ˜3.5 times higher than the number of clear days over the NCP.
Antonio Capponi, Natalie J. Harvey, Helen F. Dacre, Keith Beven, Cameron Saint, Cathie Wells, and Mike R. James
Atmos. Chem. Phys., 22, 6115–6134, https://doi.org/10.5194/acp-22-6115-2022, https://doi.org/10.5194/acp-22-6115-2022, 2022
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Forecasts of the dispersal of volcanic ash in the atmosphere are hampered by uncertainties in parameters describing the characteristics of volcanic plumes. Uncertainty quantification is vital for making robust flight-planning decisions. We present a method using satellite data to refine a series of volcanic ash dispersion forecasts and quantify these uncertainties. We show how we can improve forecast accuracy and potentially reduce the regions of high risk of volcanic ash relevant to aviation.
Piyush Srivastava, Ian M. Brooks, John Prytherch, Dominic J. Salisbury, Andrew D. Elvidge, Ian A. Renfrew, and Margaret J. Yelland
Atmos. Chem. Phys., 22, 4763–4778, https://doi.org/10.5194/acp-22-4763-2022, https://doi.org/10.5194/acp-22-4763-2022, 2022
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The parameterization of surface turbulent fluxes over sea ice remains a weak point in weather forecast and climate models. Recent theoretical developments have introduced more extensive physics but these descriptions are poorly constrained due to a lack of observation data. Here we utilize a large dataset of measurements of turbulent fluxes over sea ice to tune the state-of-the-art parameterization of wind stress, and compare it with a previous scheme.
Yiqing Liu, Zhiwen Luo, and Sue Grimmond
Atmos. Chem. Phys., 22, 4721–4735, https://doi.org/10.5194/acp-22-4721-2022, https://doi.org/10.5194/acp-22-4721-2022, 2022
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Anthropogenic heat emission from buildings is important for atmospheric modelling in cities. The current building anthropogenic heat flux is simplified by building energy consumption. Our research proposes a novel approach to determine ‘real’ building anthropogenic heat emission from the changes in energy balance fluxes between occupied and unoccupied buildings. We hope to provide new insights into future parameterisations of building anthropogenic heat flux in urban climate models.
Lars Hoffmann and Reinhold Spang
Atmos. Chem. Phys., 22, 4019–4046, https://doi.org/10.5194/acp-22-4019-2022, https://doi.org/10.5194/acp-22-4019-2022, 2022
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We present an intercomparison of 2009–2018 lapse rate tropopause characteristics as derived from ECMWF's ERA5 and ERA-Interim reanalyses. Large-scale features are similar, but ERA5 shows notably larger variability, which we mainly attribute to UTLS temperature fluctuations due to gravity waves being better resolved by ECMWF's IFS forecast model. Following evaluation with radiosondes and GPS data, we conclude ERA5 will be a more suitable asset for tropopause-related studies in future work.
Linye Song, Shangfeng Chen, Wen Chen, Jianping Guo, Conglan Cheng, and Yong Wang
Atmos. Chem. Phys., 22, 1669–1688, https://doi.org/10.5194/acp-22-1669-2022, https://doi.org/10.5194/acp-22-1669-2022, 2022
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This study shows that in most years when haze pollution (HP) over the North China Plain (NCP) is more (less) serious in winter, air conditions in the following spring are also worse (better) than normal. Conversely, there are some years when HP in the following spring is opposed to that in winter. It is found that North Atlantic sea surface temperature (SST) anomalies play important roles in HP evolution over the NCP. Thus North Atlantic SST is an important preceding signal for NCP HP evolution.
Anna A. Shestakova, Dmitry G. Chechin, Christof Lüpkes, Jörg Hartmann, and Marion Maturilli
Atmos. Chem. Phys., 22, 1529–1548, https://doi.org/10.5194/acp-22-1529-2022, https://doi.org/10.5194/acp-22-1529-2022, 2022
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This article presents a comprehensive analysis of the easterly orographic wind episode which occurred over Svalbard on 30–31 May 2017. This wind caused a significant temperature rise on the lee side of the mountains and greatly intensified the snowmelt. This episode was investigated on the basis of measurements collected during the ACLOUD/PASCAL field campaigns with the help of numerical modeling.
Xiadong An, Lifang Sheng, Chun Li, Wen Chen, Yulian Tang, and Jingliang Huangfu
Atmos. Chem. Phys., 22, 725–738, https://doi.org/10.5194/acp-22-725-2022, https://doi.org/10.5194/acp-22-725-2022, 2022
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The North China Plain (NCP) suffered many periods of haze in winter during 1985–2015, related to the rainfall-induced diabatic heating over southern China. The haze over the NCP is modulated by an anomalous anticyclone caused by the Rossby wave and a north–south circulation (NSC) induced mainly by diabatic heating. As a Rossby wave source, rainfall-induced diabatic heating supports waves and finally strengthens the anticyclone over the NCP. These changes favor haze over the NCP.
Chenrui Diao, Yangyang Xu, and Shang-Ping Xie
Atmos. Chem. Phys., 21, 18499–18518, https://doi.org/10.5194/acp-21-18499-2021, https://doi.org/10.5194/acp-21-18499-2021, 2021
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Anthropogenic aerosol (AA) emission has shown a zonal redistribution since the 1980s, with a decline in the Western Hemisphere (WH) high latitudes and an increase in the Eastern Hemisphere (EH) low latitudes. This study compares the role of zonally asymmetric forcings affecting the climate. The WH aerosol reduction dominates the poleward shift of the Hadley cell and the North Pacific warming, while the EH AA forcing is largely confined to the emission domain and induces local cooling responses.
Francisco J. Pérez-Invernón, Heidi Huntrieser, Sergio Soler, Francisco J. Gordillo-Vázquez, Nicolau Pineda, Javier Navarro-González, Víctor Reglero, Joan Montanyà, Oscar van der Velde, and Nikos Koutsias
Atmos. Chem. Phys., 21, 17529–17557, https://doi.org/10.5194/acp-21-17529-2021, https://doi.org/10.5194/acp-21-17529-2021, 2021
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Lightning-ignited fires tend to occur in remote areas and can spread significantly before suppression. Long continuing current (LCC) lightning, preferably taking place in dry thunderstorms, is believed to be the main precursor of lightning-ignited fires. We analyze fire databases of lightning-ignited fires in the Mediterranean basin and report the shared meteorological conditions of fire- and LCC-lightning-producing thunderstorms. These results can be useful to improve fire forecasting methods.
Diego Aliaga, Victoria A. Sinclair, Marcos Andrade, Paulo Artaxo, Samara Carbone, Evgeny Kadantsev, Paolo Laj, Alfred Wiedensohler, Radovan Krejci, and Federico Bianchi
Atmos. Chem. Phys., 21, 16453–16477, https://doi.org/10.5194/acp-21-16453-2021, https://doi.org/10.5194/acp-21-16453-2021, 2021
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We investigate the origin of air masses sampled at Mount Chacaltaya, Bolivia. Three-quarters of the measured air has not been influenced by the surface in the previous 4 d. However, it is rare that, at any given time, the sampled air has not been influenced at all by the surface, and often the sampled air has multiple origins. The influence of the surface is more prevalent during day than night. Furthermore, during the 6-month study, one-third of the air masses originated from Amazonia.
Michael Biggart, Jenny Stocker, Ruth M. Doherty, Oliver Wild, David Carruthers, Sue Grimmond, Yiqun Han, Pingqing Fu, and Simone Kotthaus
Atmos. Chem. Phys., 21, 13687–13711, https://doi.org/10.5194/acp-21-13687-2021, https://doi.org/10.5194/acp-21-13687-2021, 2021
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Heat-related illnesses are of increasing concern in China given its rapid urbanisation and our ever-warming climate. We examine the relative impacts that land surface properties and anthropogenic heat have on the urban heat island (UHI) in Beijing using ADMS-Urban. Air temperature measurements and satellite-derived land surface temperatures provide valuable means of evaluating modelled spatiotemporal variations. This work provides critical information for urban planners and UHI mitigation.
Tobias Wolf, Lasse H. Pettersson, and Igor Esau
Atmos. Chem. Phys., 21, 12463–12477, https://doi.org/10.5194/acp-21-12463-2021, https://doi.org/10.5194/acp-21-12463-2021, 2021
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House heating by wood-burning stoves is cozy and needed in boreal cities, e.g., Bergen, Norway. But smoke (aerosols) from stoves may reduce urban air quality. It can be transported over long distance excessively polluting some neighborhoods. Who will suffer the most? Our modelling study looks at urban pollution in unprecedented meter-sized details tracing smoke pathways and turbulent dispersion in a typical city. We prototype effective policy scenarios to mitigate urban air quality problems.
Piotr Sekuła, Anita Bokwa, Jakub Bartyzel, Bogdan Bochenek, Łukasz Chmura, Michał Gałkowski, and Mirosław Zimnoch
Atmos. Chem. Phys., 21, 12113–12139, https://doi.org/10.5194/acp-21-12113-2021, https://doi.org/10.5194/acp-21-12113-2021, 2021
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The wind shear generated on a local scale by the diversified relief’s impact can be a factor which significantly modifies the spatial pattern of PM10 concentration. The vertical profile of PM10 over a city located in a large valley during the events with high surface-level PM10 concentrations may show a sudden decrease with height not only due to the increase in wind speed, but also due to the change in wind direction alone. Vertical aerosanitary urban zones can be distinguished.
Jangho Lee, Jeffrey C. Mast, and Andrew E. Dessler
Atmos. Chem. Phys., 21, 11889–11904, https://doi.org/10.5194/acp-21-11889-2021, https://doi.org/10.5194/acp-21-11889-2021, 2021
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This paper investigates the impact of global warming on heat and humidity extremes. There are three major findings in this study. We quantify how unforced variability in the climate impacts can lead to large variations where heat waves occur, we find that all heat extremes increase as the climate warms, especially between 1.5 and 2.0 °C of the average global warming, and we show that the economic inequity of facing extreme heat will worsen in a warmer world.
Hyunju Jung, Ann Kristin Naumann, and Bjorn Stevens
Atmos. Chem. Phys., 21, 10337–10345, https://doi.org/10.5194/acp-21-10337-2021, https://doi.org/10.5194/acp-21-10337-2021, 2021
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We analyze the behavior of organized convection in a large-scale flow by imposing a mean flow to idealized simulations. In the mean flow, organized convection initially propagates slower than the mean wind speed and becomes stationary. The initial upstream and downstream difference in surface fluxes becomes symmetric as the surface momentum flux acts as a drag, resulting in the stationarity. Meanwhile, the surface enthalpy flux has a minor role in the propagation of the convection.
Xueling Liu, Arthur P. Mizzi, Jeffrey L. Anderson, Inez Fung, and Ronald C. Cohen
Atmos. Chem. Phys., 21, 9573–9583, https://doi.org/10.5194/acp-21-9573-2021, https://doi.org/10.5194/acp-21-9573-2021, 2021
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Observations of winds in the planetary boundary layer remain sparse, making it challenging to simulate and predict the atmospheric conditions that are most important for describing and predicting urban air quality. Here we investigate the application of data assimilation of NO2 columns as will be observed from geostationary orbit to improve predictions and retrospective analysis of wind fields in the boundary layer.
Antara Banerjee, Amy H. Butler, Lorenzo M. Polvani, Alan Robock, Isla R. Simpson, and Lantao Sun
Atmos. Chem. Phys., 21, 6985–6997, https://doi.org/10.5194/acp-21-6985-2021, https://doi.org/10.5194/acp-21-6985-2021, 2021
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We find that simulated stratospheric sulfate geoengineering could lead to warmer Eurasian winters alongside a drier Mediterranean and wetting to the north. These effects occur due to the strengthening of the Northern Hemisphere stratospheric polar vortex, which shifts the North Atlantic Oscillation to a more positive phase. We find the effects in our simulations to be much more significant than the wintertime effects of large tropical volcanic eruptions which inject much less sulfate aerosol.
Taufiq Hassan, Robert J. Allen, Wei Liu, and Cynthia A. Randles
Atmos. Chem. Phys., 21, 5821–5846, https://doi.org/10.5194/acp-21-5821-2021, https://doi.org/10.5194/acp-21-5821-2021, 2021
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State-of-the-art climate models yield robust, externally forced changes in the Atlantic meridional overturning circulation (AMOC), the bulk of which are due to anthropogenic aerosol perturbations to net surface shortwave radiation and sea surface temperature. AMOC-related feedbacks act to reinforce this aerosol-forced response, largely due to changes in sea surface salinity (and hence sea surface density), with temperature- and cloud-related feedbacks acting to mute the initial response.
Jun-Ichi Yano and Nils P. Wedi
Atmos. Chem. Phys., 21, 4759–4778, https://doi.org/10.5194/acp-21-4759-2021, https://doi.org/10.5194/acp-21-4759-2021, 2021
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Sensitivities of forecasts of the Madden–Julian oscillation (MJO) to various different configurations of the physics are examined with the global model of ECMWF's Integrated Forecasting System (IFS). The motivation for the study was to simulate the MJO as a nonlinear free wave. To emulate free dynamics in the IFS,
various momentum dissipation terms (
friction) as well as diabatic heating were selectively turned off over the tropics for the range of the latitudes from 20° S to 20° N.
Peter Sherman, Meng Gao, Shaojie Song, Alex T. Archibald, Nathan Luke Abraham, Jean-François Lamarque, Drew Shindell, Gregory Faluvegi, and Michael B. McElroy
Atmos. Chem. Phys., 21, 3593–3605, https://doi.org/10.5194/acp-21-3593-2021, https://doi.org/10.5194/acp-21-3593-2021, 2021
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The aims here are to assess the role of aerosols in India's monsoon precipitation and to determine the relative contributions from Chinese and Indian emissions using CMIP6 models. We find that increased sulfur emissions reduce precipitation, which is primarily dynamically driven due to spatial shifts in convection over the region. A significant increase in precipitation (up to ~ 20 %) is found only when both Indian and Chinese sulfate emissions are regulated.
Melissa L. Breeden, Amy H. Butler, John R. Albers, Michael Sprenger, and Andrew O'Neil Langford
Atmos. Chem. Phys., 21, 2781–2794, https://doi.org/10.5194/acp-21-2781-2021, https://doi.org/10.5194/acp-21-2781-2021, 2021
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Prior research has found a maximum in deep stratosphere-to-troposphere mass/ozone transport over the western United States in boreal spring, which can enhance surface ozone concentrations, reducing air quality. We find that the winter-to-summer evolution of the north Pacific jet increases the frequency of stratospheric intrusions that drive transport, helping explain the observed maximum. The El Niño–Southern Oscillation affects the timing of the spring jet transition and therefore transport.
Dirk Offermann, Christoph Kalicinsky, Ralf Koppmann, and Johannes Wintel
Atmos. Chem. Phys., 21, 1593–1611, https://doi.org/10.5194/acp-21-1593-2021, https://doi.org/10.5194/acp-21-1593-2021, 2021
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Atmospheric oscillations with periods of up to several 100 years exist at altitudes up to 110 km. They are also seen in computer models (GCMs) of the atmospheric. They are often attributed to external influences from the sun, from the oceans, or from atmospheric constituents. This is difficult to verify as the atmosphere cannot be manipulated in an experiment. However, a GCM can be changed arbitrarily. Doing so, we find that long-period oscillations may be excited internally in the atmosphere.
Cited articles
Affad, E., Saadeddine, S., Assou, M., and Sbaibi, A.: Effect of the relative
humidity on an industrial plume behavior, Glob. NEST J., 8, 297–305,
https://doi.org/10.30955/gnj.000294, 2006.
Aksoyoglu, S., Baltensperger, U., and Prévôt, A. S. H.: Contribution of ship emissions to the concentration and deposition of air pollutants in Europe, Atmos. Chem. Phys., 16, 1895–1906, https://doi.org/10.5194/acp-16-1895-2016, 2016.
Aulinger, A., Matthias, V., Zeretzke, M., Bieser, J., Quante, M., and Backes, A.: The impact of shipping emissions on air pollution in the greater North Sea region – Part 1: Current emissions and concentrations, Atmos. Chem. Phys., 16, 739–758, https://doi.org/10.5194/acp-16-739-2016, 2016.
Bai, S., Wen, Y., He, L., Liu, Y., Zhang, Y., Yu, Q., and Ma, W.:
Single-Vessel Plume Dispersion Simulation: Method and a Case Study Using
CALPUFF in the Yantian Port Area, Shenzhen (China), Int. J. Env. Res.
Pub. He., 17, 1–29, https://doi.org/10.3390/ijerph17217831, 2020.
Barregard, L., Molnár, P., Jonson, J. E., and Stockfelt, L.: Impact on
population health of baltic shipping emissions, Int. J. Env. Res. Pub.
He., 16, 1954, https://doi.org/10.3390/ijerph16111954, 2019.
Bieser, J., Aulinger, A., Matthias, V., Quante, M., and van der Gon, H. A. C.
D.: Vertical emission profiles for Europe based on plume rise calculations,
Environ. Pollut., 159, 2935–2946, https://doi.org/10.1016/j.envpol.2011.04.030,
2011.
Brandt, J., Silver, J. D., Christensen, J. H., Andersen, M. S., Bønløkke, J. H., Sigsgaard, T., Geels, C., Gross, A., Hansen, A. B., Hansen, K. M., Hedegaard, G. B., Kaas, E., and Frohn, L. M.: Assessment of past, present and future health-cost externalities of air pollution in Europe and the contribution from international ship traffic using the EVA model system, Atmos. Chem. Phys., 13, 7747–7764, https://doi.org/10.5194/acp-13-7747-2013, 2013.
Briggs, G. A.: Plume rise predictions, Lect. Air Pollut. Environ. Impact
Anal., 59–111, https://doi.org/10.1007/978-1-935704-23-2_3, 1982.
Broome, R. A., Cope, M. E., Goldsworthy, B., Goldsworthy, L., Emmerson, K.,
Jegasothy, E., and Morgan, G. G.: The mortality effect of ship-related fine
particulate matter in the Sydney greater metropolitan region of NSW,
Australia, Environ. Int., 87, 85–93, https://doi.org/10.1016/j.envint.2015.11.012,
2016.
Brunner, D., Kuhlmann, G., Marshall, J., Clément, V., Fuhrer, O., Broquet, G., Löscher, A., and Meijer, Y.: Accounting for the vertical distribution of emissions in atmospheric CO2 simulations, Atmos. Chem. Phys., 19, 4541–4559, https://doi.org/10.5194/acp-19-4541-2019, 2019.
CAT: Marine Power Systems, available at: https://www.cat.com/en_GB/products/new/power-systems/marine-power-systems.html, last access: 24
July 2020.
Chosson, F., Paoli, R., and Cuenot, B.: Ship plume dispersion rates in convective boundary layers for chemistry models, Atmos. Chem. Phys., 8, 4841–4853, https://doi.org/10.5194/acp-8-4841-2008, 2008.
Corbett, J. J., Winebrake, J. J., Green, E. H., Kasibhatla, P., Eyring, V.,
and Lauer, A.: Mortality from ship emissions: A global assessment, Environ.
Sci. Technol., 41, 8512–8518, https://doi.org/10.1021/es071686z, 2007.
Eyring, V., Isaksen, I. S. A., Berntsen, T., Collins, W. J., Corbett, J. J.,
Endresen, O., Grainger, R. G., Moldanova, J., Schlager, H., and Stevenson, D.
S.: Transport impacts on atmosphere and climate: Shipping, Atmos. Environ.,
44, 4735–4771, https://doi.org/10.1016/j.atmosenv.2009.04.059, 2010.
Grawe, D., Schlünzen, K. H., and Pascheke, F.: Comparison of results of
an obstacle resolving microscale model with wind tunnel data, Atmos.
Environ., 79, 495–509, https://doi.org/10.1016/j.atmosenv.2013.06.039, 2013.
Hanna, S. R., Schulman, L. L., Paine, R. J., Pleim, J. E., and Baer, M.:
Development and evaluation of the offshore and coastal dispersion model, J.
Air Pollut. Control Assoc., 35, 1039–1047,
https://doi.org/10.1080/00022470.1985.10466003, 1985.
Hulskotte, J. H. J. and Denier van der Gon, H. A. C.: Fuel consumption and
associated emissions from seagoing ships at berth derived from an on-board
survey, Atmos. Environ., 44, 1229–1236, https://doi.org/10.1016/j.atmosenv.2009.10.018,
2010.
Huszar, P., Cariolle, D., Paoli, R., Halenka, T., Belda, M., Schlager, H.,
Miksovsky, J. and Pisoft, P.: Modeling the regional impact of ship emissions
on NOx and ozone levels over the Eastern Atlantic and Western Europe using
ship plume parameterization, Atmos. Chem. Phys., 10, 6645–6660,
https://doi.org/10.5194/acp-10-6645-2010, 2010.
ICDC: Hamburg Boundary Layer Measurement Tower, available at: https://icdc.cen.uni-hamburg.de/en/weathermast-hamburg.html, last
access: 24 July 2020.
IMO: Sulphur oxides (SOx) and Particulate Matter (PM) – Regulation 14, available at: https://www.imo.org/en/OurWork/Environment/Pages/Sulphur-oxides-(SOx)-%E2%80%93-Regulation-14.aspx, last access: 13 April 2021.
Jalkanen, J.-P., Brink, A., Kalli, J., Pettersson, H., Kukkonen, J., and Stipa, T.: A modelling system for the exhaust emissions of marine traffic and its application in the Baltic Sea area, Atmos. Chem. Phys., 9, 9209–9223, https://doi.org/10.5194/acp-9-9209-2009, 2009.
Jalkanen, J.-P., Johansson, L., Kukkonen, J., Brink, A., Kalli, J., and Stipa, T.: Extension of an assessment model of ship traffic exhaust emissions for particulate matter and carbon monoxide, Atmos. Chem. Phys., 12, 2641–2659, https://doi.org/10.5194/acp-12-2641-2012, 2012.
Janicke, U. and Janicke, L.: A three-dimensional plume rise model for dry
and wet plumes, Atmos. Environ., 35, 877–890,
https://doi.org/10.1016/S1352-2310(00)00372-1, 2001.
Johansson, L., Jalkanen, J. P., and Kukkonen, J.: Global assessment of
shipping emissions in 2015 on a high spatial and temporal resolution, Atmos.
Environ., 167, 403–415, https://doi.org/10.1016/j.atmosenv.2017.08.042, 2017.
Karl, M., Bieser, J., Geyer, B., Matthias, V., Jalkanen, J.-P., Johansson, L., and Fridell, E.: Impact of a nitrogen emission control area (NECA) on the future air quality and nitrogen deposition to seawater in the Baltic Sea region, Atmos. Chem. Phys., 19, 1721–1752, https://doi.org/10.5194/acp-19-1721-2019, 2019.
Lee, J. H. W. and Cheung, V.: Generalized lagrangian model for buoyant jets
in current, J. Environ. Eng., 116, 1085–1106,
https://doi.org/10.1061/(ASCE)0733-9372(1990)116:6(1085), 1990.
Lin, H., Tao, J., Qian, Z. (Min), Ruan, Z., Xu, Y., Hang, J., Xu, X., Liu,
T., Guo, Y., Zeng, W., Xiao, J., Guo, L., Li, X., and Ma, W.: Shipping
pollution emission associated with increased cardiovascular mortality: A
time series study in Guangzhou, China, Environ. Pollut., 241, 862–868,
https://doi.org/10.1016/j.envpol.2018.06.027, 2018.
Liu, H., Fu, M., Jin, X., Shang, Y., Shindell, D., Faluvegi, G., Shindell,
C. and He, K.: Health and climate impacts of ocean-going vessels in East
Asia, Nat. Clim. Change, 6, 1037–1041, https://doi.org/10.1038/nclimate3083, 2016.
MAN: Two-stroke project guides, available at: https://marine.man-es.com/two-stroke/project-guides, last access: 24
July 2020.
Matthias, V., Aulinger, A., Backes, A., Bieser, J., Geyer, B., Quante, M., and Zeretzke, M.: The impact of shipping emissions on air pollution in the greater North Sea region – Part 2: Scenarios for 2030, Atmos. Chem. Phys., 16, 759–776, https://doi.org/10.5194/acp-16-759-2016, 2016.
Matthias, V., Arndt, J. A., Aulinger, A., Bieser, J., Denier van der Gon,
H., Kranenburg, R., Kuenen, J., Neumann, D., Pouliot, G. and Quante, M.:
Modeling emissions for three-dimensional atmospheric chemistry transport
models, J. Air Waste Manage., 68, 763–800,
https://doi.org/10.1080/10962247.2018.1424057, 2018.
Murena, F., Mocerino, L., Quaranta, F., and Toscano, D.: Impact on air
quality of cruise ship emissions in Naples, Italy, Atmos. Environ., 187,
70–83, https://doi.org/10.1016/j.atmosenv.2018.05.056, 2018.
Murphy, S., Agrawal, H., Sorooshian, A., Padró, L. T., Gates, H.,
Hersey, S., Welch, W. A., Jung, H., Miller, J. W., Cocker, D. R., Nenes, A.,
Jonsson, H. H., Flagan, R. C., and Seinfeld, J. H.: Comprehensive
simultaneous shipboard and airborne characterization of exhaust from a
modern container ship at sea, Environ. Sci. Technol., 43, 4626–4640,
https://doi.org/10.1021/es802413j, 2009.
Port of Hamburg: Vesseltypes, available at: https://www.hafen-hamburg.de/en/vessels/, last access: 24
July 2020.
Ramacher, M. O. P., Karl, M., Bieser, J., Jalkanen, J.-P., and Johansson, L.: Urban population exposure to NOx emissions from local shipping in three Baltic Sea harbour cities – a generic approach, Atmos. Chem. Phys., 19, 9153–9179, https://doi.org/10.5194/acp-19-9153-2019, 2019.
Salim, M. H., Schlünzen, K. H., Grawe, D., Boettcher, M., Gierisch, A. M. U., and Fock, B. H.: The microscale obstacle-resolving meteorological model MITRAS v2.0: model theory, Geosci. Model Dev., 11, 3427–3445, https://doi.org/10.5194/gmd-11-3427-2018, 2018.
Schatzmann, M.: An Integral Model of Plume Rise, Atmos. Environ., 13,
721–731, https://doi.org/10.1016/0004-6981(79)90202-6, 1979.
Schlünzen, K. H., Hinneburg, D., Knoth, O., Lambrecht, M., Leitl, B.,
López, S., Lüpkes, C., Panskus, H., Renner, E., Schatzmann, M.,
Schoenemeyer, T., Trepte, S., and Wolke, R.: Flow and transport in the
obstacle layer: First results of the micro-scale model MITRAS, J. Atmos.
Chem., 44, 113–130, https://doi.org/10.1023/A:1022420130032, 2003.
Schlünzen, K. H., Boettcher, M., Fock, B. H., Gierisch, A., Grawe, D.,
and Salim, M.: Scientific Documentation of the Multiscale Model System
M-SYS, MEMI Tech. Rep. 4, CEN, Univ. Hambg., 1–153, 2018.
Sofiev, M., Winebrake, J. J., Johansson, L., Carr, E. W., Prank, M., Soares,
J., Vira, J., Kouznetsov, R., Jalkanen, J. P., and Corbett, J. J.: Cleaner
fuels for ships provide public health benefits with climate tradeoffs, Nat.
Commun., 9, 1–12, https://doi.org/10.1038/s41467-017-02774-9, 2018.
Tzannatos, E.: Ship emissions and their externalities for Greece, Atmos.
Environ., 44, 2194–2202, https://doi.org/10.1016/j.atmosenv.2010.03.018, 2010.
United Nations Conference on Trade and Development: Review of maritime
transport 2019, United Nations, Geneva, available at:
https://unctad.org/en/Pages/Publications/Review-of-Maritime-Transport-(Series).aspx (last access: 13 April 2021),
2019.
Vesseltracker: Vessels, available at: https://www.vesseltracker.com/en/vessels.html, last access:
24 July 2020.
Vinken, G. C. M., Boersma, K. F., Jacob, D. J., and Meijer, E. W.: Accounting for non-linear chemistry of ship plumes in the GEOS-Chem global chemistry transport model, Atmos. Chem. Phys., 11, 11707–11722, https://doi.org/10.5194/acp-11-11707-2011, 2011.
von Glasow, R., Lawrence, M. G., Sander, R., and Crutzen, P. J.: Modeling the chemical effects of ship exhaust in the cloud-free marine boundary layer, Atmos. Chem. Phys., 3, 233–250, https://doi.org/10.5194/acp-3-233-2003, 2003.
Wang, C., Corbett, J. J., and Firestone, J.: Improving spatial representation
of global ship emissions inventories, Environ. Sci. Technol., 42, 193–199,
https://doi.org/10.1021/es0700799, 2008.
Wärtsilä: Diesel engines, available at:
https://www.wartsila.com/marine/build/engines-and-generating-sets/diesel-engines,
last access: 24 July 2020.
Zhang, Y., Feng, J., Liu, C., Zhao, J., Ma, W., Huang, C., An, J., Shen, Y.,
Fu, Q., Wang, S., Ding, D., Ge, W., Fung, F., Manokaran, K., Patton, A. P.,
Walker, K. D., and Kan, H.: Impacts of Shipping on Air PollutantEmissions,
Air Quality, and Health in the Yangtze River Delta and Shanghai, China
Special Report 22, Heal. Eff. Inst. Spec. Rep., 22, 1–78, 2019.
Short summary
This work aims to describe the physical distribution of ship exhaust gases in the near field, e.g., inside of a harbor. Results were calculated with a mathematical model for different meteorological and technical conditions. It has been shown that large vessels like cruise ships have a significant effect of up to 55 % downward movement of exhaust gas, as they can disturb the ground near wind circulation. This needs to be considered in urban air pollution studies.
This work aims to describe the physical distribution of ship exhaust gases in the near field,...
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