Articles | Volume 21, issue 21
https://doi.org/10.5194/acp-21-16363-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-16363-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
08 Nov 2021
Research article |
| 08 Nov 2021
| 08 Nov 2021
Spatiotemporal variability in the oxidative potential of ambient fine particulate matter in the Midwestern United States
Haoran Yu
Department of Civil and Environmental Engineering, University of
Illinois at Urbana–Champaign, Urbana, IL 61801, USA
Joseph Varghese Puthussery
Department of Civil and Environmental Engineering, University of
Illinois at Urbana–Champaign, Urbana, IL 61801, USA
Yixiang Wang
Department of Civil and Environmental Engineering, University of
Illinois at Urbana–Champaign, Urbana, IL 61801, USA
Vishal Verma
CORRESPONDING AUTHOR
Department of Civil and Environmental Engineering, University of
Illinois at Urbana–Champaign, Urbana, IL 61801, USA
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Cited
27 citations as recorded by crossref.
- Oxidation potential of PM2.5 in a mechanical processing plant and its association with metal composition J. Ma et al. 10.1016/j.atmosenv.2023.120318
- Variations of oxidative potential of PM2.5 in a medium-sized residential city in South Korea measured using three different chemical assays P. Kim et al. 10.1016/j.scitotenv.2024.171053
- Insights the dominant contribution of biomass burning to methanol-soluble PM2.5 bounded oxidation potential based on multilayer perceptron neural network analysis in Xi'an, China Y. Luo et al. 10.1016/j.scitotenv.2023.168273
- Inter-continental variability in the relationship of oxidative potential and cytotoxicity with PM2.5 mass S. Salana et al. 10.1038/s41467-024-49649-4
- The oxidative potential of particulate matter (PM) in different regions around the world and its relation to air pollution sources V. Farahani et al. 10.1039/D2EA00043A
- Chemical and oxidative properties of fine particulate matter from near-road traffic sources N. Raparthi et al. 10.1016/j.envpol.2023.122514
- Temporal dynamics and source characteristics of fine particulate matter using Positive Matrix Factorization (PMF) V. Kumar et al. 10.1016/j.apr.2025.102539
- Sources of acellular oxidative potential of water-soluble fine ambient particulate matter in the midwestern United States H. Yu et al. 10.1016/j.jhazmat.2024.134763
- Impact of anthropogenic emission control in reducing future PM2.5 concentrations and the related oxidative potential across different regions of China J. Liu et al. 10.1016/j.scitotenv.2024.170638
- Between and within-city variations of PM2.5 oxidative potential in five cities in Colombia N. Rojas et al. 10.1007/s11869-024-01632-0
- Key toxicity enhancement effect of aqueous-phase secondary formation: Insights from hourly measurements during haze events F. Cao et al. 10.1016/j.jhazmat.2025.138139
- Linking Switzerland's PM10 and PM2.5 oxidative potential (OP) with emission sources S. Grange et al. 10.5194/acp-22-7029-2022
- Seasonal variation of driving factors of ambient PM2.5 oxidative potential in Shenzhen, China C. Xing et al. 10.1016/j.scitotenv.2022.160771
- The oxidative potential of airborne particulate matter in two urban areas of Chile: More than meets the eye C. Molina et al. 10.1016/j.envint.2023.107866
- Assessing the Oxidative Potential of Outdoor PM2.5 in Wintertime Fairbanks, Alaska Y. Yang et al. 10.1021/acsestair.3c00066
- Oxidative potential of ambient PM2.5 from São Paulo, Brazil: Variations, associations with chemical components and source apportionment E. Serafeim et al. 10.1016/j.atmosenv.2023.119593
- Residential Wood Burning and Vehicle Emissions as Major Sources of Environmentally Persistent Free Radicals in Fairbanks, Alaska K. Edwards et al. 10.1021/acs.est.4c01206
- Major source categories of PM2.5 oxidative potential in wintertime Beijing and surroundings based on online dithiothreitol-based field measurements R. Cheung et al. 10.1016/j.scitotenv.2024.172345
- Reactive oxygen species, environmentally persistent free radicals, and oxidative potential of outdoor and indoor particulate matter in Wintertime Fairbanks, Alaska S. Kapur et al. 10.1080/02786826.2024.2433656
- Assessing air quality and composition of fine particulate matter (PM 2.5 ) in Jackson, MS A. Craze Smith & C. Roper 10.1080/10934529.2025.2521899
- Monitoring of Indoor Air Quality in a Classroom Combining a Low-Cost Sensor System and Machine Learning I. Apostolopoulos et al. 10.3390/chemosensors13040148
- Effect of Biomass Burning, Diwali Fireworks, and Polluted Fog Events on the Oxidative Potential of Fine Ambient Particulate Matter in Delhi, India J. Puthussery et al. 10.1021/acs.est.2c02730
- The Influence of Different Protocols on the Application of the Dithiothreitol Assay in Determining the Oxidative Potential of Ambient Particles M. Jovanović et al. 10.3390/toxics13020113
- On the Relative Contribution of Iron and Organic Compounds, and Their Interaction in Cellular Oxidative Potential of Ambient PM2.5 Y. Wang et al. 10.1021/acs.estlett.2c00316
- Investigating PM2.5 Oxidative Potential and Its Association with Chemical Constituents Measured outside of Urban Residences in Three Metropolitan Cities of India S. Dubey et al. 10.1289/JHP1007
- Impact of meteorology and aerosol sources on PM2.5 and oxidative potential variability and levels in China J. Liu et al. 10.5194/acp-24-10849-2024
- Oxidative Potential from Common Indoor Sources of Particulate Matter P. Subramanian et al. 10.1021/acs.est.5c01696
27 citations as recorded by crossref.
- Oxidation potential of PM2.5 in a mechanical processing plant and its association with metal composition J. Ma et al. 10.1016/j.atmosenv.2023.120318
- Variations of oxidative potential of PM2.5 in a medium-sized residential city in South Korea measured using three different chemical assays P. Kim et al. 10.1016/j.scitotenv.2024.171053
- Insights the dominant contribution of biomass burning to methanol-soluble PM2.5 bounded oxidation potential based on multilayer perceptron neural network analysis in Xi'an, China Y. Luo et al. 10.1016/j.scitotenv.2023.168273
- Inter-continental variability in the relationship of oxidative potential and cytotoxicity with PM2.5 mass S. Salana et al. 10.1038/s41467-024-49649-4
- The oxidative potential of particulate matter (PM) in different regions around the world and its relation to air pollution sources V. Farahani et al. 10.1039/D2EA00043A
- Chemical and oxidative properties of fine particulate matter from near-road traffic sources N. Raparthi et al. 10.1016/j.envpol.2023.122514
- Temporal dynamics and source characteristics of fine particulate matter using Positive Matrix Factorization (PMF) V. Kumar et al. 10.1016/j.apr.2025.102539
- Sources of acellular oxidative potential of water-soluble fine ambient particulate matter in the midwestern United States H. Yu et al. 10.1016/j.jhazmat.2024.134763
- Impact of anthropogenic emission control in reducing future PM2.5 concentrations and the related oxidative potential across different regions of China J. Liu et al. 10.1016/j.scitotenv.2024.170638
- Between and within-city variations of PM2.5 oxidative potential in five cities in Colombia N. Rojas et al. 10.1007/s11869-024-01632-0
- Key toxicity enhancement effect of aqueous-phase secondary formation: Insights from hourly measurements during haze events F. Cao et al. 10.1016/j.jhazmat.2025.138139
- Linking Switzerland's PM10 and PM2.5 oxidative potential (OP) with emission sources S. Grange et al. 10.5194/acp-22-7029-2022
- Seasonal variation of driving factors of ambient PM2.5 oxidative potential in Shenzhen, China C. Xing et al. 10.1016/j.scitotenv.2022.160771
- The oxidative potential of airborne particulate matter in two urban areas of Chile: More than meets the eye C. Molina et al. 10.1016/j.envint.2023.107866
- Assessing the Oxidative Potential of Outdoor PM2.5 in Wintertime Fairbanks, Alaska Y. Yang et al. 10.1021/acsestair.3c00066
- Oxidative potential of ambient PM2.5 from São Paulo, Brazil: Variations, associations with chemical components and source apportionment E. Serafeim et al. 10.1016/j.atmosenv.2023.119593
- Residential Wood Burning and Vehicle Emissions as Major Sources of Environmentally Persistent Free Radicals in Fairbanks, Alaska K. Edwards et al. 10.1021/acs.est.4c01206
- Major source categories of PM2.5 oxidative potential in wintertime Beijing and surroundings based on online dithiothreitol-based field measurements R. Cheung et al. 10.1016/j.scitotenv.2024.172345
- Reactive oxygen species, environmentally persistent free radicals, and oxidative potential of outdoor and indoor particulate matter in Wintertime Fairbanks, Alaska S. Kapur et al. 10.1080/02786826.2024.2433656
- Assessing air quality and composition of fine particulate matter (PM 2.5 ) in Jackson, MS A. Craze Smith & C. Roper 10.1080/10934529.2025.2521899
- Monitoring of Indoor Air Quality in a Classroom Combining a Low-Cost Sensor System and Machine Learning I. Apostolopoulos et al. 10.3390/chemosensors13040148
- Effect of Biomass Burning, Diwali Fireworks, and Polluted Fog Events on the Oxidative Potential of Fine Ambient Particulate Matter in Delhi, India J. Puthussery et al. 10.1021/acs.est.2c02730
- The Influence of Different Protocols on the Application of the Dithiothreitol Assay in Determining the Oxidative Potential of Ambient Particles M. Jovanović et al. 10.3390/toxics13020113
- On the Relative Contribution of Iron and Organic Compounds, and Their Interaction in Cellular Oxidative Potential of Ambient PM2.5 Y. Wang et al. 10.1021/acs.estlett.2c00316
- Investigating PM2.5 Oxidative Potential and Its Association with Chemical Constituents Measured outside of Urban Residences in Three Metropolitan Cities of India S. Dubey et al. 10.1289/JHP1007
- Impact of meteorology and aerosol sources on PM2.5 and oxidative potential variability and levels in China J. Liu et al. 10.5194/acp-24-10849-2024
- Oxidative Potential from Common Indoor Sources of Particulate Matter P. Subramanian et al. 10.1021/acs.est.5c01696
Latest update: 10 Jul 2025
Short summary
We assessed the oxidative potential (OP) of ambient PM2.5 collected from many sites in the US Midwest through multiple acellular endpoints. Compared to homogeneously distributed PM2.5, OP showed higher spatiotemporal variation. Poor correlations for the regression between mass and OP indicated a limited role of mass in determining the OP. Moreover, weak correlations among different OP endpoints justify the need for using multiple assays to determine oxidative levels of particles.
We assessed the oxidative potential (OP) of ambient PM2.5 collected from many sites in the US...
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