Articles | Volume 21, issue 16 
            
                
                    
            
            
            https://doi.org/10.5194/acp-21-12595-2021
                    © Author(s) 2021. This work is distributed under 
the Creative Commons Attribution 4.0 License.
                the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-12595-2021
                    © Author(s) 2021. This work is distributed under 
the Creative Commons Attribution 4.0 License.
                the Creative Commons Attribution 4.0 License.
Aerosol formation and growth rates from chamber experiments using Kalman smoothing
Matthew Ozon
                                            Department of Applied Physics, University of Eastern Finland, 70210 Kuopio, Finland
                                        
                                    Dominik Stolzenburg
                                            Institute for Atmospheric and Earth System Research/ Physics,
University of Helsinki, 00014 Helsinki, Finland
                                        
                                    Lubna Dada
                                            Institute for Atmospheric and Earth System Research/ Physics,
University of Helsinki, 00014 Helsinki, Finland
                                        
                                    
                                            EPFL, School of Architecture, Civil and Environmental Engineering,
1951 Sion, Switzerland
                                        
                                    
                                            Paul Scherrer Institute, Laboratory of Atmospheric Chemistry, 5232
Villigen PSI, Switzerland
                                        
                                    Aku Seppänen
                                            Department of Applied Physics, University of Eastern Finland, 70210 Kuopio, Finland
                                        
                                    Kari E. J. Lehtinen
CORRESPONDING AUTHOR
                                            
                                    
                                            Department of Applied Physics, University of Eastern Finland, 70210 Kuopio, Finland
                                        
                                    
                                            Atmospheric Research Centre of Eastern Finland, Finnish
Meteorological Institute, 70210 Kuopio, Finland
                                        
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                            Cited
11 citations as recorded by crossref.
- Survival of newly formed particles in haze conditions R. Marten et al. 10.1039/D2EA00007E
- What controls the observed size-dependency of the growth rates of sub-10 nm atmospheric particles? J. Kontkanen et al. 10.1039/D1EA00103E
- Role of sesquiterpenes in biogenic new particle formation L. Dada et al. 10.1126/sciadv.adi5297
- Combining instrument inversions for sub-10 nm aerosol number size-distribution measurements D. Stolzenburg et al. 10.1016/j.jaerosci.2021.105862
- Improved counting statistics of an ultrafine differential mobility particle size spectrometer system D. Stolzenburg et al. 10.5194/amt-16-2471-2023
- Revisiting matrix-based inversion of scanning mobility particle sizer (SMPS) and humidified tandem differential mobility analyzer (HTDMA) data M. Petters 10.5194/amt-14-7909-2021
- Global modeling of aerosol nucleation with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs) X. Shao et al. 10.5194/acp-24-11365-2024
- Assessing pH- and temperature-dependence in the aqueous phase partitioning of organic acids and bases in the atmosphere O. Driessen & J. Murphy 10.1039/D5EA00034C
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
- Opinion: Should high-resolution differential mobility analyzers be used in mainstream aerosol studies? J. Fernandez de la Mora 10.5194/ar-2-21-2024
- Efficacy of a portable, moderate-resolution, fast-scanning differential mobility analyzer for ambient aerosol size distribution measurements S. Amanatidis et al. 10.5194/amt-14-4507-2021
10 citations as recorded by crossref.
- Survival of newly formed particles in haze conditions R. Marten et al. 10.1039/D2EA00007E
- What controls the observed size-dependency of the growth rates of sub-10 nm atmospheric particles? J. Kontkanen et al. 10.1039/D1EA00103E
- Role of sesquiterpenes in biogenic new particle formation L. Dada et al. 10.1126/sciadv.adi5297
- Combining instrument inversions for sub-10 nm aerosol number size-distribution measurements D. Stolzenburg et al. 10.1016/j.jaerosci.2021.105862
- Improved counting statistics of an ultrafine differential mobility particle size spectrometer system D. Stolzenburg et al. 10.5194/amt-16-2471-2023
- Revisiting matrix-based inversion of scanning mobility particle sizer (SMPS) and humidified tandem differential mobility analyzer (HTDMA) data M. Petters 10.5194/amt-14-7909-2021
- Global modeling of aerosol nucleation with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs) X. Shao et al. 10.5194/acp-24-11365-2024
- Assessing pH- and temperature-dependence in the aqueous phase partitioning of organic acids and bases in the atmosphere O. Driessen & J. Murphy 10.1039/D5EA00034C
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
- Opinion: Should high-resolution differential mobility analyzers be used in mainstream aerosol studies? J. Fernandez de la Mora 10.5194/ar-2-21-2024
Latest update: 30 Oct 2025
Short summary
                    Measuring the rate at which aerosol particles are formed is of importance for understanding climate change. We present an analysis method based on Kalman smoothing, which retrieves new particle formation and growth rates from size-distribution measurements. We apply it to atmospheric simulation chamber experiments and show that it agrees well with traditional methods. In addition, it provides reliable uncertainty estimates, and we suggest instrument design optimisation for signal processing.
                    Measuring the rate at which aerosol particles are formed is of importance for understanding...
                    
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