Articles | Volume 19, issue 2
https://doi.org/10.5194/acp-19-1357-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-19-1357-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Possible heterogeneous chemistry of hydroxymethanesulfonate (HMS) in northern China winter haze
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA 02138, USA
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA 02138, USA
Weiqi Xu
State Key Laboratory of Atmospheric Boundary Physics and Atmospheric
Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
State Key Laboratory of Atmospheric Boundary Physics and Atmospheric
Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
Center for Excellence in Regional Atmospheric Environment, Institute
of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
Douglas R. Worsnop
Aerodyne Research, Inc., Billerica, MA 01821, USA
John T. Jayne
Aerodyne Research, Inc., Billerica, MA 01821, USA
Yuzhong Zhang
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA 02138, USA
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA 02138, USA
Mei Li
Institute of Mass Spectrometer and Atmospheric Environment, Jinan
University, Guangzhou 510632, China
Guangdong Provincial Engineering Research Center for Online Source
Apportionment System of Air Pollution, Guangzhou 510632, China
Zhen Zhou
Institute of Mass Spectrometer and Atmospheric Environment, Jinan
University, Guangzhou 510632, China
Guangdong Provincial Engineering Research Center for Online Source
Apportionment System of Air Pollution, Guangzhou 510632, China
Chunlei Cheng
Institute of Mass Spectrometer and Atmospheric Environment, Jinan
University, Guangzhou 510632, China
Guangdong Provincial Engineering Research Center for Online Source
Apportionment System of Air Pollution, Guangzhou 510632, China
Yibing Lv
China National Environmental Monitoring Center, Beijing 100012, China
Ying Wang
State Key Laboratory of Severe Weather & Key Laboratory for
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing 100081, China
Wei Peng
State Key Laboratory of Severe Weather & Key Laboratory for
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing 100081, China
Xiaobin Xu
State Key Laboratory of Severe Weather & Key Laboratory for
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing 100081, China
Nan Lin
Department of Earth System Science, Tsinghua University, Beijing
100084, China
Yuxuan Wang
Department of Earth and Atmospheric Sciences, University of Houston,
Houston, TX 77004, USA
Shuxiao Wang
School of Environment, Tsinghua University, Beijing 100084, China
J. William Munger
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA 02138, USA
Daniel J. Jacob
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA 02138, USA
Michael B. McElroy
CORRESPONDING AUTHOR
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA 02138, USA
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- Carbonyl Compounds Regulate Atmospheric Oxidation Capacity and Particulate Sulfur Chemistry in the Coastal Atmosphere M. Zhao et al. 10.1021/acs.est.4c03947
- Integration of field observation and air quality modeling to characterize Beijing aerosol in different seasons J. Liu et al. 10.1016/j.chemosphere.2019.125195
- Responses of gaseous sulfuric acid and particulate sulfate to reduced SO2 concentration: A perspective from long-term measurements in Beijing X. Li et al. 10.1016/j.scitotenv.2020.137700
- Sulfate formation is dominated by manganese-catalyzed oxidation of SO2 on aerosol surfaces during haze events W. Wang et al. 10.1038/s41467-021-22091-6
- Deactivating Effect of Hydroxyl Radicals Reactivity by Sulfate and Sulfite Functional Groups in Aqueous Phase─Atmospheric Implications for Small Organosulfur Compounds D. Lai et al. 10.1021/acsestair.4c00033
- Significant Biogenic Source of Oxygenated Volatile Organic Compounds and the Impacts on Photochemistry at a Regional Background Site in South China X. Lyu et al. 10.1021/acs.est.4c05656
- Study on the assimilation of the sulphate reaction rates based on WRF-Chem/DART C. Huang et al. 10.1007/s11430-023-1153-9
- Heterogeneous interactions between SO<sub>2</sub> and organic peroxides in submicron aerosol S. Wang et al. 10.5194/acp-21-6647-2021
- Global modeling of heterogeneous hydroxymethanesulfonate chemistry S. Song et al. 10.5194/acp-21-457-2021
- A Review on Laboratory Studies and Field Measurements of Atmospheric Organic Aerosol Hygroscopicity and Its Parameterization Based on Oxidation Levels Y. Kuang et al. 10.1007/s40726-020-00164-2
- Comparative Study of Particulate Organosulfates in Contrasting Atmospheric Environments: Field Evidence for the Significant Influence of Anthropogenic Sulfate and NOx Y. Wang et al. 10.1021/acs.estlett.0c00550
- Assessment of the impacts of cloud chemistry on surface SO2 and sulfate levels in typical regions of China J. Lu et al. 10.5194/acp-23-8021-2023
- Critical Roles of Surface-Enhanced Heterogeneous Oxidation of SO2 in Haze Chemistry: Review of Extended Pathways for Complex Air Pollution Z. Zhang et al. 10.1007/s40726-023-00287-2
- Wintertime Formation of Large Sulfate Particles in China and Implications for Human Health Q. Zhang et al. 10.1021/acs.est.3c05645
- Evaluation and sensitivity analysis of the ecosystem service functions of haze absorption by green space based on its quality in China P. Zhang et al. 10.3897/natureconservation.40.23017
- Opinion: Atmospheric multiphase chemistry – past, present, and future J. Abbatt & A. Ravishankara 10.5194/acp-23-9765-2023
- Quantifying the Influences of PM2.5 and Relative Humidity on Change of Atmospheric Visibility over Recent Winters in an Urban Area of East China X. Sun et al. 10.3390/atmos11050461
- Fine particulate matter (PM<sub>2.5</sub>) trends in China, 2013–2018: separating contributions from anthropogenic emissions and meteorology S. Zhai et al. 10.5194/acp-19-11031-2019
- Catalytic role of formaldehyde in particulate matter formation E. Dovrou et al. 10.1073/pnas.2113265119
- Significant Conversion of Organic Sulfur from Hydroxymethanesulfonate to Inorganic Sulfate and Peroxydisulfate Ions upon Heterogeneous OH Oxidation D. Lai et al. 10.1021/acs.estlett.3c00472
- Complex Interplay Between Organic and Secondary Inorganic Aerosols With Ambient Relative Humidity Implicates the Aerosol Liquid Water Content Over India During Wintertime A. Gopinath et al. 10.1029/2021JD036430
- Chemical and optical characterization of aqueous secondary organic aerosol generated by reaction of pyruvaldehyde with sodium sulfite M. Zhu et al. 10.1016/j.apr.2024.102124
- Overview of the Alaskan Layered Pollution and Chemical Analysis (ALPACA) Field Experiment W. Simpson et al. 10.1021/acsestair.3c00076
- Hygroscopicity and cloud condensation nucleation activities of hydroxyalkylsulfonates C. Peng et al. 10.1016/j.scitotenv.2022.154767
- A review of aerosol chemistry in Asia: insights from aerosol mass spectrometer measurements W. Zhou et al. 10.1039/D0EM00212G
- Quantitative Determination of Hydroxymethanesulfonate (HMS) Using Ion Chromatography and UHPLC-LTQ-Orbitrap Mass Spectrometry: A Missing Source of Sulfur during Haze Episodes in Beijing L. Wei et al. 10.1021/acs.estlett.0c00528
- Varying Drivers of 2013–2017 Trends in PM2.5 Pollution over Different Regions in China Y. Tao et al. 10.3390/atmos15070789
- A theoretical study on the formation and oxidation mechanism of hydroxyalkylsulfonate in the atmospheric aqueous phase D. Zhang et al. 10.1039/C9RA05193G
- Influence of organic aerosol molecular composition on particle absorptive properties in autumn Beijing J. Cai et al. 10.5194/acp-22-1251-2022
- Contribution of hydroxymethanesulfonate (HMS) to severe winter haze in the North China Plain T. Ma et al. 10.5194/acp-20-5887-2020
- Significant contribution of organics to aerosol liquid water content in winter in Beijing, China X. Jin et al. 10.5194/acp-20-901-2020
- Chemical transport models often underestimate inorganic aerosol acidity in remote regions of the atmosphere B. Nault et al. 10.1038/s43247-021-00164-0
- Determination of Urban Formaldehyde Emission Ratios in the Shanghai Megacity Y. Liu et al. 10.1021/acs.est.3c06428
- Theoretical investigation of a potentially important formation pathway of organosulfate in atmospheric aqueous aerosols K. Chen & J. Zhao 10.1038/s41598-020-61968-2
- Secondary inorganic aerosol during heating season in a megacity in Northeast China: Evidence for heterogeneous chemistry in severe cold climate region Y. Cheng et al. 10.1016/j.chemosphere.2020.127769
- Multiphase Reactions between Organic Peroxides and Sulfur Dioxide in Internally Mixed Inorganic and Organic Particles: Key Roles of Particle Phase Separation and Acidity M. Yao et al. 10.1021/acs.est.3c04975
- Aerosol chemical component: Simulations with WRF-Chem and comparison with observations in Nanjing T. Sha et al. 10.1016/j.atmosenv.2019.116982
- Hydroxymethanesulfonate and Sulfur(IV) in Fairbanks Winter During the ALPACA Study K. Dingilian et al. 10.1021/acsestair.4c00012
- Spatial-Temporal Variation in Health Impact Attributable to PM2.5 and Ozone Pollution in the Beijing Metropolitan Region of China M. Huo et al. 10.3390/atmos13111813
- Fast oxidation of sulfur dioxide by hydrogen peroxide in deliquesced aerosol particles T. Liu et al. 10.1073/pnas.1916401117
- Source and Chemistry of Hydroxymethanesulfonate (HMS) in Fairbanks, Alaska J. Campbell et al. 10.1021/acs.est.2c00410
- Global Importance of Hydroxymethanesulfonate in Ambient Particulate Matter: Implications for Air Quality J. Moch et al. 10.1029/2020JD032706
- Production and Reactions of Organic Molecules in Clouds of Venus J. Spacek et al. 10.1021/acsearthspacechem.3c00261
- Investigation of factors controlling PM2.5 variability across the South Korean Peninsula during KORUS-AQ C. Jordan et al. 10.1525/elementa.424
- Sulfate formation during heavy winter haze events and the potential contribution from heterogeneous SO<sub>2</sub> + NO<sub>2</sub> reactions in the Yangtze River Delta region, China L. Huang et al. 10.5194/acp-19-14311-2019
- Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds A. Tilgner et al. 10.5194/acp-21-13483-2021
- Ambient fine particulate matter and ozone pollution in China: synergy in anthropogenic emissions and atmospheric processes Y. Jiang et al. 10.1088/1748-9326/aca16a
- Aerosol pH and chemical regimes of sulfate formation in aerosol water during winter haze in the North China Plain W. Tao et al. 10.5194/acp-20-11729-2020
- Insight into wet scavenging effects on sulfur and nitrogen containing organic compounds in urban Beijing C. Zhang et al. 10.1038/s41612-024-00756-5
- Fast sulfate formation from oxidation of SO2 by NO2 and HONO observed in Beijing haze J. Wang et al. 10.1038/s41467-020-16683-x
- Uptake of Water‐soluble Gas‐phase Oxidation Products Drives Organic Particulate Pollution in Beijing G. Gkatzelis et al. 10.1029/2020GL091351
- Secondary aerosol formation in winter haze over the Beijing-Tianjin-Hebei Region, China D. Shang et al. 10.1007/s11783-020-1326-x
- Predicting hygroscopic growth of organosulfur aerosol particles using COSMOtherm Z. Li et al. 10.5194/acp-24-11717-2024
- Persistent Heavy Winter Nitrate Pollution Driven by Increased Photochemical Oxidants in Northern China X. Fu et al. 10.1021/acs.est.9b07248
- Heterogeneous sulfate aerosol formation mechanisms during wintertime Chinese haze events: air quality model assessment using observations of sulfate oxygen isotopes in Beijing J. Shao et al. 10.5194/acp-19-6107-2019
- Stringent Emission Controls Are Needed to Reach Clean Air Targets for Cities in China under a Warming Climate R. Wang et al. 10.1021/acs.est.1c08403
- Modelling of sulfur chemistry in a fog episode in northern China and implication for the efficacy of SO2 emission control L. Yuan et al. 10.1016/j.atmosenv.2024.120409
- Positive Feedback between Partitioning of Carbonyl Compounds and Particulate Sulfur Formation during Haze Episodes H. Shen et al. 10.1021/acs.est.4c07278
- Origin and transformation of ambient volatile organic compounds during a dust-to-haze episode in northwest China Y. Xue et al. 10.5194/acp-20-5425-2020
- Measurement report: Impact of cloud processes on secondary organic aerosols at a forested mountain site in southeastern China Z. Zhang et al. 10.5194/acp-24-8473-2024
- Interactions between aerosol organic components and liquid water content during haze episodes in Beijing X. Li et al. 10.5194/acp-19-12163-2019
- Multiphase Reactions between Secondary Organic Aerosol and Sulfur Dioxide: Kinetics and Contributions to Sulfate Formation and Aerosol Aging M. Yao et al. 10.1021/acs.estlett.9b00657
- Unraveling a New Chemical Mechanism of Missing Sulfate Formation in Aerosol Haze: Gaseous NO2 with Aqueous HSO3–/SO32– J. Yang et al. 10.1021/jacs.9b08503
- Multiphase Oxidation of Sulfur Dioxide in Aerosol Particles: Implications for Sulfate Formation in Polluted Environments T. Liu et al. 10.1021/acs.est.0c06496
- Hydroxymethanesulfonate formation as a significant pathway of transformation of SO2 H. Zhang et al. 10.1016/j.atmosenv.2022.119474
- Responses of decline in air pollution and recovery associated with COVID-19 lockdown in the Pearl River Delta S. Wang et al. 10.1016/j.scitotenv.2020.143868
- Marine sources of formaldehyde in the coastal atmosphere H. Shen et al. 10.1016/j.scib.2024.09.024
- Multiple Sulfur Isotopic Evidence for Sulfate Formation in Haze Pollution X. Han et al. 10.1021/acs.est.3c05072
- Multi-Scale Effects of Meteorological Conditions and Anthropogenic Emissions on PM2.5 Concentrations over Major Cities of the Yellow River Basin J. Zhang et al. 10.3390/ijerph192215060
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Short summary
Chemistry responsible for sulfate production in northern China winter haze remains mysterious. We propose a potentially key pathway through the reaction of formaldehyde and sulfur dioxide that has not been accounted for in previous studies. The special atmospheric conditions favor the formation and existence of their complex, hydroxymethanesulfonate (HMS).
Chemistry responsible for sulfate production in northern China winter haze remains mysterious....
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