Articles | Volume 18, issue 1
https://doi.org/10.5194/acp-18-467-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-467-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Secondary organic aerosol formation from ambient air in an oxidation flow reactor in central Amazonia
Brett B. Palm
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Dept. of Chemistry, University of Colorado, Boulder, CO, USA
Suzane S. de Sá
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA, USA
Douglas A. Day
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Dept. of Chemistry, University of Colorado, Boulder, CO, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Dept. of Chemistry, University of Colorado, Boulder, CO, USA
Weiwei Hu
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Dept. of Chemistry, University of Colorado, Boulder, CO, USA
Roger Seco
Dept. of Earth System Science, University of California, Irvine, CA, USA
Steven J. Sjostedt
Earth System Research Laboratory, National Oceanic and Atmospheric
Administration, Boulder, CO, USA
Jeong-Hoo Park
National Center for Atmospheric Research, Boulder, CO, USA
now at: Climate and Air Quality Research Department, National
Institute of Environmental Research (NIER), Incheon, 22689, Republic of
Korea
Alex B. Guenther
Dept. of Earth System Science, University of California, Irvine, CA, USA
Div. of Atmospheric Sciences & Global Change, Pacific Northwest
National Laboratory, Richland, WA, USA
Saewung Kim
Dept. of Earth System Science, University of California, Irvine, CA, USA
Joel Brito
Institute of Physics, University of São Paulo, São Paulo, Brazil
now at: Laboratory for Meteorological Physics (LaMP), Université
Clermont Auvergne, 63000 Clermont-Ferrand, France
Florian Wurm
Institute of Physics, University of São Paulo, São Paulo, Brazil
Paulo Artaxo
Institute of Physics, University of São Paulo, São Paulo, Brazil
Ryan Thalman
Environmental and Climate Sciences Department, Brookhaven National
Laboratory, Upton, NY, USA
now at: Department of Chemistry, Snow College, Richfield, UT, USA
Jian Wang
Environmental and Climate Sciences Department, Brookhaven National
Laboratory, Upton, NY, USA
Lindsay D. Yee
Department of Environmental Science, Policy, and Management,
University of California, Berkeley, CA, USA
Rebecca Wernis
Department of Civil and Environmental Engineering, University of
California, Berkeley, CA, USA
Gabriel Isaacman-VanWertz
Department of Environmental Science, Policy, and Management,
University of California, Berkeley, CA, USA
now at: Department of Civil and Environmental Engineering, Virginia
Tech, Blacksburg, VA, USA
Allen H. Goldstein
Department of Environmental Science, Policy, and Management,
University of California, Berkeley, CA, USA
Department of Civil and Environmental Engineering, University of
California, Berkeley, CA, USA
Yingjun Liu
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA, USA
now at: Department of Environmental Science, Policy, and
Management, University of California, Berkeley, CA, USA
Stephen R. Springston
Environmental and Climate Sciences Department, Brookhaven National
Laboratory, Upton, NY, USA
Rodrigo Souza
University of the State of Amazonas, Manaus, Brazil
Matt K. Newburn
Environmental and Molecular Sciences Laboratory, Pacific Northwest
National Laboratory, Richland, WA, USA
M. Lizabeth Alexander
Environmental and Molecular Sciences Laboratory, Pacific Northwest
National Laboratory, Richland, WA, USA
Scot T. Martin
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA, USA
Department of Earth and Planetary Sciences, Harvard University,
Cambridge, MA, USA
Jose L. Jimenez
CORRESPONDING AUTHOR
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Dept. of Chemistry, University of Colorado, Boulder, CO, USA
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- Final revised paper (published on 17 Jan 2018)
- Supplement to the final revised paper
- Preprint (discussion started on 30 Aug 2017)
- Supplement to the preprint
Interactive discussion
Status: closed
Status: closed
AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment
- Printer-friendly version
- Supplement
- RC1: 'Review of Palm et al., "Secondary organic aerosol formation from ambient air in an oxidation flow reactor in central Amazonia"', Anonymous Referee #1, 02 Oct 2017
- RC2: 'Review of "Secondary organic aerosol formation from ambient air in an oxidation flow reactor in central Amazonia"', Anonymous Referee #2, 09 Nov 2017
- AC1: 'Response to reviewers for “Secondary organic aerosol formation from ambient air in an oxidation flow reactor in central Amazonia”', Brett B. Palm, 06 Dec 2017
Peer-review completion
AR: Author's response | RR: Referee report | ED: Editor decision
AR by Brett B. Palm on behalf of the Authors (06 Dec 2017)
Author's response
Manuscript
ED: Publish as is (06 Dec 2017) by Thomas Karl
AR by Brett B. Palm on behalf of the Authors (07 Dec 2017)
Short summary
Ambient air was oxidized by OH or O3 in an oxidation flow reactor during both wet and dry seasons in the GoAmazon2014/5 campaign to study secondary organic aerosol (SOA) formation. We investigated how much biogenic, urban, and biomass burning sources contributed to the ambient concentrations of SOA precursor gases and how their contributions changed diurnally and seasonally. SOA yields and hygroscopicity of organic aerosol in the oxidation flow reactor were also studied.
Ambient air was oxidized by OH or O3 in an oxidation flow reactor during both wet and dry...
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