Articles | Volume 17, issue 12
https://doi.org/10.5194/acp-17-7567-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-7567-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
22 Jun 2017
Research article |
| 22 Jun 2017
Observations of bromine monoxide transport in the Arctic sustained on aerosol particles
Peter K. Peterson
Department of Chemistry, University of Michigan, Ann Arbor, MI, USA
Denis Pöhler
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
Holger Sihler
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
Max Planck Institute for Chemistry, Mainz, Germany
Johannes Zielcke
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
Stephan General
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
Udo Frieß
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
Ulrich Platt
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
Max Planck Institute for Chemistry, Mainz, Germany
William R. Simpson
Department of Chemistry and Biochemistry and Geophysical Institute, University of Alaska Fairbanks, Fairbanks, Alaska, USA
Son V. Nghiem
Jet Propulsion Laboratory, California Institute of Technology, Pasadena, CA, USA
Paul B. Shepson
Department of Chemistry, Department of Earth, Planetary, and Atmospheric Sciences, and Purdue Climate Change
Research Center, Purdue University, West Lafayette, IN, USA
Brian H. Stirm
School of Aviation and Transportation Technology, Purdue University, West Lafayette, IN, USA
Suresh Dhaniyala
Department of Mechanical and Aeronautical Engineering, Clarkson University, Potsdam, NY, USA
Thomas Wagner
Max Planck Institute for Chemistry, Mainz, Germany
Dana R. Caulton
Department of Civil and Environmental Engineering, Princeton University, Princeton, NJ, USA
Jose D. Fuentes
Department of Meteorology, The Pennsylvania State University, University Park, PA, USA
Department of Chemistry, University of Michigan, Ann Arbor, MI, USA
Department of Earth and Environmental Sciences, University of Michigan, Ann Arbor, MI, USA
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- Comparison of model and ground observations finds snowpack and blowing snow aerosols both contribute to Arctic tropospheric reactive bromine W. Swanson et al. 10.5194/acp-22-14467-2022
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- Global retrieval of stratospheric and tropospheric BrO columns from the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM) on board the Suomi-NPP satellite H. Chong et al. 10.5194/amt-17-2873-2024
- Reactive bromine in the low troposphere of Antarctica: estimations at two research sites C. Prados-Roman et al. 10.5194/acp-18-8549-2018
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- Modelling wintertime sea-spray aerosols under Arctic haze conditions E. Ioannidis et al. 10.5194/acp-23-5641-2023
- Study of an Arctic Cyclone-Induced Bromine Explosion Event in Ny-Ålesund, Svalbard D. Chen et al. 10.2139/ssrn.4045479
- Surface Propensity of Aqueous Atmospheric Bromine at the Liquid–Gas Interface I. Gladich et al. 10.1021/acs.jpclett.0c00633
- Time-dependent 3D simulations of tropospheric ozone depletion events in the Arctic spring using the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) M. Herrmann et al. 10.5194/acp-21-7611-2021
- An unexpected large continental source of reactive bromine and chlorine with significant impact on wintertime air quality X. Peng et al. 10.1093/nsr/nwaa304
- Impacts of Arctic oil field NOx emissions on downwind bromine chemistry: insights from 5 years of MAX-DOAS observations P. Peterson et al. 10.1039/D4FD00164H
- Springtime Bromine Activation over Coastal and Inland Arctic Snowpacks P. Peterson et al. 10.1021/acsearthspacechem.8b00083
- Technical note: Sublimation of frozen CsCl solutions in an environmental scanning electron microscope (ESEM) – determining the number and size of salt particles relevant to sea salt aerosols L. Vetráková et al. 10.5194/acp-23-4463-2023
- Atmospheric particle abundance and sea salt aerosol observations in the springtime Arctic: a focus on blowing snow and leads Q. Chen et al. 10.5194/acp-22-15263-2022
- Horizontal and vertical structure of reactive bromine events probed by bromine monoxide MAX-DOAS W. Simpson et al. 10.5194/acp-17-9291-2017
- Multiphase Reactive Bromine Chemistry during Late Spring in the Arctic: Measurements of Gases, Particles, and Snow D. Jeong et al. 10.1021/acsearthspacechem.2c00189
- Application of Satellite‐Based Detections of Arctic Bromine Explosion Events Within GEOS‐Chem P. Wales et al. 10.1029/2022MS003465
- Processes Controlling the Composition and Abundance of Arctic Aerosol M. Willis et al. 10.1029/2018RG000602
- Link Between Arctic Tropospheric BrO Explosion Observed From Space and Sea‐Salt Aerosols From Blowing Snow Investigated Using Ozone Monitoring Instrument BrO Data and GEOS‐5 Data Assimilation System S. Choi et al. 10.1029/2017JD026889
- Direct detection of atmospheric atomic bromine leading to mercury and ozone depletion S. Wang et al. 10.1073/pnas.1900613116
- Snowpack measurements suggest role for multi-year sea ice regions in Arctic atmospheric bromine and chlorine chemistry P. Peterson et al. 10.1525/elementa.352
- Source mechanisms and transport patterns of tropospheric bromine monoxide: findings from long-term multi-axis differential optical absorption spectroscopy measurements at two Antarctic stations U. Frieß et al. 10.5194/acp-23-3207-2023
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- Long-term time series of Arctic tropospheric BrO derived from UV–VIS satellite remote sensing and its relation to first-year sea ice I. Bougoudis et al. 10.5194/acp-20-11869-2020
- Modelling the coupled mercury-halogen-ozone cycle in the central Arctic during spring S. Ahmed et al. 10.1525/elementa.2022.00129
- Microphysics of the aqueous bulk counters the water activity driven rate acceleration of bromide oxidation by ozone from 289–245 K J. Edebeli et al. 10.1039/C8EM00417J
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- Evaluating the impact of blowing-snow sea salt aerosol on springtime BrO and O3 in the Arctic J. Huang et al. 10.5194/acp-20-7335-2020
- Tropospheric Halogen Photochemistry in the Rapidly Changing Arctic K. Pratt 10.1016/j.trechm.2019.06.001
- Tropospheric bromine monoxide vertical profiles retrieved across the Alaskan Arctic in springtime N. Brockway et al. 10.5194/acp-24-23-2024
- Simulating tropospheric BrO in the Arctic using an artificial neural network I. Bougoudis et al. 10.1016/j.atmosenv.2022.119032
- Chemical characterization of sub-micron aerosols over the East Sea (Sea of Japan) A. Loh et al. 10.1016/j.scitotenv.2022.159173
- The Role of Snow in Controlling Halogen Chemistry and Boundary Layer Oxidation During Arctic Spring: A 1D Modeling Case Study S. Ahmed et al. 10.1029/2021JD036140
- Investigation of meteorological conditions and BrO during ozone depletion events in Ny-Ålesund between 2010 and 2021 B. Zilker et al. 10.5194/acp-23-9787-2023
- Particle aging and aerosol–radiation interaction affect volcanic plume dispersion: evidence from the Raikoke 2019 eruption L. Muser et al. 10.5194/acp-20-15015-2020
- Global Observations of Tropospheric Bromine Monoxide (BrO) Columns From TROPOMI Y. Chen et al. 10.1029/2023JD039091
- Snowmelt onset hinders bromine monoxide heterogeneous recycling in the Arctic J. Burd et al. 10.1002/2017JD026906
41 citations as recorded by crossref.
- Comparison of model and ground observations finds snowpack and blowing snow aerosols both contribute to Arctic tropospheric reactive bromine W. Swanson et al. 10.5194/acp-22-14467-2022
- Study of an Arctic blowing snow-induced bromine explosion event in Ny-Ålesund, Svalbard D. Chen et al. 10.1016/j.scitotenv.2022.156335
- Dynamics of gaseous oxidized mercury at Villum Research Station during the High Arctic summer J. Pernov et al. 10.5194/acp-21-13287-2021
- Global retrieval of stratospheric and tropospheric BrO columns from the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM) on board the Suomi-NPP satellite H. Chong et al. 10.5194/amt-17-2873-2024
- Reactive bromine in the low troposphere of Antarctica: estimations at two research sites C. Prados-Roman et al. 10.5194/acp-18-8549-2018
- Measurements of Tropospheric Bromine Monoxide Over Four Halogen Activation Seasons in the Canadian High Arctic K. Bognar et al. 10.1029/2020JD033015
- Modelling wintertime sea-spray aerosols under Arctic haze conditions E. Ioannidis et al. 10.5194/acp-23-5641-2023
- Study of an Arctic Cyclone-Induced Bromine Explosion Event in Ny-Ålesund, Svalbard D. Chen et al. 10.2139/ssrn.4045479
- Surface Propensity of Aqueous Atmospheric Bromine at the Liquid–Gas Interface I. Gladich et al. 10.1021/acs.jpclett.0c00633
- Time-dependent 3D simulations of tropospheric ozone depletion events in the Arctic spring using the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) M. Herrmann et al. 10.5194/acp-21-7611-2021
- An unexpected large continental source of reactive bromine and chlorine with significant impact on wintertime air quality X. Peng et al. 10.1093/nsr/nwaa304
- Impacts of Arctic oil field NOx emissions on downwind bromine chemistry: insights from 5 years of MAX-DOAS observations P. Peterson et al. 10.1039/D4FD00164H
- Springtime Bromine Activation over Coastal and Inland Arctic Snowpacks P. Peterson et al. 10.1021/acsearthspacechem.8b00083
- Technical note: Sublimation of frozen CsCl solutions in an environmental scanning electron microscope (ESEM) – determining the number and size of salt particles relevant to sea salt aerosols L. Vetráková et al. 10.5194/acp-23-4463-2023
- Atmospheric particle abundance and sea salt aerosol observations in the springtime Arctic: a focus on blowing snow and leads Q. Chen et al. 10.5194/acp-22-15263-2022
- Horizontal and vertical structure of reactive bromine events probed by bromine monoxide MAX-DOAS W. Simpson et al. 10.5194/acp-17-9291-2017
- Multiphase Reactive Bromine Chemistry during Late Spring in the Arctic: Measurements of Gases, Particles, and Snow D. Jeong et al. 10.1021/acsearthspacechem.2c00189
- Application of Satellite‐Based Detections of Arctic Bromine Explosion Events Within GEOS‐Chem P. Wales et al. 10.1029/2022MS003465
- Processes Controlling the Composition and Abundance of Arctic Aerosol M. Willis et al. 10.1029/2018RG000602
- Link Between Arctic Tropospheric BrO Explosion Observed From Space and Sea‐Salt Aerosols From Blowing Snow Investigated Using Ozone Monitoring Instrument BrO Data and GEOS‐5 Data Assimilation System S. Choi et al. 10.1029/2017JD026889
- Direct detection of atmospheric atomic bromine leading to mercury and ozone depletion S. Wang et al. 10.1073/pnas.1900613116
- Snowpack measurements suggest role for multi-year sea ice regions in Arctic atmospheric bromine and chlorine chemistry P. Peterson et al. 10.1525/elementa.352
- Source mechanisms and transport patterns of tropospheric bromine monoxide: findings from long-term multi-axis differential optical absorption spectroscopy measurements at two Antarctic stations U. Frieß et al. 10.5194/acp-23-3207-2023
- On the dynamics of ozone depletion events at Villum Research Station in the High Arctic J. Pernov et al. 10.5194/acp-24-13603-2024
- Lake Spray Aerosol Incorporated into Great Lakes Clouds N. Olson et al. 10.1021/acsearthspacechem.9b00258
- Arctic tropospheric ozone: assessment of current knowledge and model performance C. Whaley et al. 10.5194/acp-23-637-2023
- Implementation and Impacts of Surface and Blowing Snow Sources of Arctic Bromine Activation Within WRF‐Chem 4.1.1 L. Marelle et al. 10.1029/2020MS002391
- Long-term time series of Arctic tropospheric BrO derived from UV–VIS satellite remote sensing and its relation to first-year sea ice I. Bougoudis et al. 10.5194/acp-20-11869-2020
- Modelling the coupled mercury-halogen-ozone cycle in the central Arctic during spring S. Ahmed et al. 10.1525/elementa.2022.00129
- Microphysics of the aqueous bulk counters the water activity driven rate acceleration of bromide oxidation by ozone from 289–245 K J. Edebeli et al. 10.1039/C8EM00417J
- Fostering multidisciplinary research on interactions between chemistry, biology, and physics within the coupled cryosphere-atmosphere system J. Thomas et al. 10.1525/elementa.396
- MAX-DOAS measurements of NO2, SO2, HCHO, and BrO at the Mt. Waliguan WMO GAW global baseline station in the Tibetan Plateau J. Ma et al. 10.5194/acp-20-6973-2020
- Evaluating the impact of blowing-snow sea salt aerosol on springtime BrO and O3 in the Arctic J. Huang et al. 10.5194/acp-20-7335-2020
- Tropospheric Halogen Photochemistry in the Rapidly Changing Arctic K. Pratt 10.1016/j.trechm.2019.06.001
- Tropospheric bromine monoxide vertical profiles retrieved across the Alaskan Arctic in springtime N. Brockway et al. 10.5194/acp-24-23-2024
- Simulating tropospheric BrO in the Arctic using an artificial neural network I. Bougoudis et al. 10.1016/j.atmosenv.2022.119032
- Chemical characterization of sub-micron aerosols over the East Sea (Sea of Japan) A. Loh et al. 10.1016/j.scitotenv.2022.159173
- The Role of Snow in Controlling Halogen Chemistry and Boundary Layer Oxidation During Arctic Spring: A 1D Modeling Case Study S. Ahmed et al. 10.1029/2021JD036140
- Investigation of meteorological conditions and BrO during ozone depletion events in Ny-Ålesund between 2010 and 2021 B. Zilker et al. 10.5194/acp-23-9787-2023
- Particle aging and aerosol–radiation interaction affect volcanic plume dispersion: evidence from the Raikoke 2019 eruption L. Muser et al. 10.5194/acp-20-15015-2020
- Global Observations of Tropospheric Bromine Monoxide (BrO) Columns From TROPOMI Y. Chen et al. 10.1029/2023JD039091
1 citations as recorded by crossref.
Discussed (final revised paper)
Latest update: 16 Jul 2025
Short summary
High-spatial-resolution aircraft measurements in the Arctic showed the sustained transport of reactive bromine in a lofted layer via heterogeneous reactions on aerosol particles. This process provides an explanation for free tropospheric reactive bromine and the significant spatial extent of satellite-observed bromine monoxide. The knowledge gained herein improves our understanding of the fate and transport of atmospheric pollutants in the Arctic.
High-spatial-resolution aircraft measurements in the Arctic showed the sustained transport of...
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Final-revised paper
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