Articles | Volume 17, issue 22
https://doi.org/10.5194/acp-17-13891-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-17-13891-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Insight into the in-cloud formation of oxalate based on in situ measurement by single particle mass spectrometry
Guohua Zhang
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Resources Utilization and Protection, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR
China
Qinhao Lin
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Resources Utilization and Protection, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR
China
University of Chinese Academy of Sciences, Beijing 100039, PR China
Long Peng
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Resources Utilization and Protection, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR
China
University of Chinese Academy of Sciences, Beijing 100039, PR China
Yuxiang Yang
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Resources Utilization and Protection, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR
China
University of Chinese Academy of Sciences, Beijing 100039, PR China
Yuzhen Fu
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Resources Utilization and Protection, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR
China
University of Chinese Academy of Sciences, Beijing 100039, PR China
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Resources Utilization and Protection, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR
China
Mei Li
Institute of Mass Spectrometer and Atmospheric Environment, Jinan
University, Guangzhou 510632, PR China
Duohong Chen
State Environmental Protection Key Laboratory of Regional Air
Quality Monitoring, Guangdong Environmental Monitoring Center, Guangzhou
510308, PR China
Jianxin Chen
Shaoguan Environmental Monitoring Center, Shaoguan 512026, PR China
Zhang Cai
John and Willie Leone Family Department of Energy and Mineral
Engineering, Pennsylvania State University, University Park, PA 16802,
USA
Xinming Wang
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Resources Utilization and Protection, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR
China
Ping'an Peng
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Resources Utilization and Protection, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR
China
Guoying Sheng
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Resources Utilization and Protection, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, PR
China
Zhen Zhou
Institute of Mass Spectrometer and Atmospheric Environment, Jinan
University, Guangzhou 510632, PR China
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- The reductions of oxalate and its precursors in cloud droplets relative to wet particles Q. Lin et al. 10.1016/j.atmosenv.2020.117632
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- Oxalate Formation Enhanced by Fe-Containing Particles and Environmental Implications G. Zhang et al. 10.1021/acs.est.8b05280
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We first reported the size-resolved mixing state of oxalate in the cloud droplet residual, the cloud interstitial, and cloud-free particles by single particle mass spectrometry. Individual particle analysis provides unique insight into the formation and evolution of oxalate during in-cloud processing. The data show that in-cloud aqueous reactions dramatically improved the formation of oxalate from organic acids that were strongly associated with the aged biomass burning particles.
We first reported the size-resolved mixing state of oxalate in the cloud droplet residual, the...
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