Articles | Volume 26, issue 1
https://doi.org/10.5194/acp-26-391-2026
© Author(s) 2026. This work is distributed under the Creative Commons Attribution 4.0 License.
Atmospheric lifetime of sulphur hexafluoride (SF6) and five other trace gases in the BASCOE model driven by three reanalyses
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- Final revised paper (published on 08 Jan 2026)
- Supplement to the final revised paper
- Preprint (discussion started on 13 Aug 2025)
- Supplement to the preprint
Interactive discussion
Status: closed
Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor
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RC1: 'Comment on egusphere-2025-3597', Anonymous Referee #1, 10 Sep 2025
- AC1: 'Reply on RC1', Sarah Vervalcke, 17 Dec 2025
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RC2: 'Comment on egusphere-2025-3597', Anonymous Referee #2, 01 Oct 2025
- AC2: 'Reply on RC2', Sarah Vervalcke, 17 Dec 2025
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AR – Author's response | RR – Referee report | ED – Editor decision | EF – Editorial file upload
AR by Sarah Vervalcke on behalf of the Authors (17 Dec 2025)
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ED: Publish subject to technical corrections (17 Dec 2025) by Jens-Uwe Grooß
AR by Sarah Vervalcke on behalf of the Authors (18 Dec 2025)
Author's response
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This paper describes the results of an update to the BASCOE model to include detailed SF6 chemistry in the mesosphere. The lifetime of SF6 as well as of five other trace gases are calculated from the model output and they all generally agree well with previous lifetime estimates. This suggests that the SF6 chemistry implemented in BASCOE is at least sufficient to represent the main loss processes of SF6 and that it is then primarily the model transport that will determine the SF6 lifetime. The SF6 lifetime is shown to vary considerably with different reanalysis data sets driving the model but the lifetimes still agree within uncertainties. The accurate representation of SF6 chemistry in BASCOE is an important advancement in assessing model transport compared to observations.
The paper is well written and the results are described clearly. The topic is appropriate for ACP and so I suggest publication with consideration of the minor comments listed below.
Minor comments:
Line 24: I would suggest replacing ‘General’ with ‘Chemistry-‘.
Table 1: The entries in this table are somewhat confusing and repetitive. It doesn’t seem like you need the fifth column with the Data Versions since they’re all the same. Maybe just state the versions in the table header. Also, the ‘Agreement’ and ‘Notes and References’ columns sometimes overlap in their content and frequently include the subjective term ‘Good’ that isn’t necessarily helpful. The ‘Compared instruments’ and Data versions’ columns seem to have conflicting versions. For instance, for SF6 the ACE V2.2 and V5.3 are listed. I would suggest trimming this table down to the basic information and make sure it isn’t repetitive or conflicting.
Line 131 ‘parameterized’ is misspelled
Fig. 7: The y-axis scales here seem much too large, it’s difficult to see any features. Maybe that’s the point but it seems like you could at least go to +/-30%. It also might be helpful to indicate the instrument differences for each species by dashed lines for instance.