Articles | Volume 25, issue 15
https://doi.org/10.5194/acp-25-8785-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-25-8785-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Light scattering and microphysical properties of atmospheric bullet rosette ice crystals
Shawn W. Wagner
CORRESPONDING AUTHOR
Institute of Meteorology and Climate Research – Atmospheric Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
now at: Department of Atmospheric Sciences, University of North Dakota, Grand Forks, North Dakota, United States
Martin Schnaiter
Institute of Meteorology and Climate Research – Atmospheric Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
schnaiTEC GmbH, Wuppertal, Germany
now at: Institute for Atmospheric and Environmental Research, University of Wuppertal, Wuppertal, Germany
Guanglang Xu
Institute of Meteorology and Climate Research – Atmospheric Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
now at: Institute for Advanced Study, Shenzhen University, Shenzhen, China
Franziska Rogge
Institute of Meteorology and Climate Research – Atmospheric Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
previously published under the name Franziska Nehlert
Institute of Meteorology and Climate Research – Atmospheric Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
now at: Institute for Atmospheric and Environmental Research, University of Wuppertal, Wuppertal, Germany
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Adrian Hamel, Martin Schnaiter, Masa Saito, Robert Wagner, and Emma Järvinen
EGUsphere, https://doi.org/10.5194/egusphere-2025-3515, https://doi.org/10.5194/egusphere-2025-3515, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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The depolarisation ratio of ice clouds is commonly measured by satellites and ground-based instruments to learn about ice particle shapes. In our cloud chamber experiments, we found that for small ice crystals, the depolarisation ratio is more strongly influenced by particle size than by nano-scale structure. The measured trends could be reproduced with numerical simulations. This result helps improve the interpretation of remote sensing data and the accuracy of light scattering models.
Adrian Hamel, Massimo del Guasta, Carl Schmitt, Christophe Genthon, Emma Järvinen, and Martin Schnaiter
EGUsphere, https://doi.org/10.5194/egusphere-2025-3598, https://doi.org/10.5194/egusphere-2025-3598, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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We measured the size and shape of small ice particles in the dry and cold atmosphere of inland Antarctica. We observed that particles originating near the surface are smaller than those falling from higher altitudes. Inland Antarctic particles of frozen fog occur at lower concentrations and are less complex than those observed in an urban, polluted environment. These findings help to improve Antarctic climate models and to accurately interpret satellite observations of the polar atmosphere.
Emma Järvinen and Franz Martin Schnaiter
EGUsphere, https://doi.org/10.5194/egusphere-2025-3065, https://doi.org/10.5194/egusphere-2025-3065, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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We studied high-level ice clouds in the Arctic and mid-latitudes using measurements from a research aircraft. By simultaneously recording the size and shape of individual ice particles and how they scatter light, we found that these clouds reflect more sunlight than commonly assumed in climate models. Our results improve understanding of cloud optical properties and help reduce uncertainties in climate predictions.
Marco Zanatta, Pia Bogert, Patrick Ginot, Yiwei Gong, Gholam Ali Hoshyaripour, Yaqiong Hu, Feng Jiang, Paolo Laj, Yanxia Li, Claudia Linke, Ottmar Möhler, Harald Saathoff, Martin Schnaiter, Nsikanabasi Silas Umo, Franziska Vogel, and Robert Wagner
Aerosol Research Discuss., https://doi.org/10.5194/ar-2025-12, https://doi.org/10.5194/ar-2025-12, 2025
Revised manuscript accepted for AR
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Back carbon is an atmospheric pollutant from combustion, contributes to the Arctic warming. However, its properties change as it travels through the atmosphere, affecting its impact. We recreated Arctic transport conditions in a laboratory to study how black carbon evolves over time. Our findings show that temperature and altitude strongly influence its transformation, providing key insights for improving climate models and understanding Arctic pollution.
Marco Zanatta, Stephan Mertes, Olivier Jourdan, Regis Dupuy, Emma Järvinen, Martin Schnaiter, Oliver Eppers, Johannes Schneider, Zsófia Jurányi, and Andreas Herber
Atmos. Chem. Phys., 23, 7955–7973, https://doi.org/10.5194/acp-23-7955-2023, https://doi.org/10.5194/acp-23-7955-2023, 2023
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Black carbon (BC) particles influence the Arctic radiative balance. Vertical measurements of black carbon were conducted during the ACLOUD campaign in the European Arctic to study the interaction of BC with clouds. This study shows that clouds influence the vertical variability of BC properties across the inversion layer and that multiple activation and transformation mechanisms of BC may occur in the presence of low-level, persistent, mixed-phase clouds.
Emma Järvinen, Franziska Nehlert, Guanglang Xu, Fritz Waitz, Guillaume Mioche, Regis Dupuy, Olivier Jourdan, and Martin Schnaiter
Atmos. Chem. Phys., 23, 7611–7633, https://doi.org/10.5194/acp-23-7611-2023, https://doi.org/10.5194/acp-23-7611-2023, 2023
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The Arctic is warming faster than other regions. Arctic low-level mixed-phase clouds, where ice crystals and liquid droplets co-exist, are thought to have an important role in Arctic warming. Here we show airborne measurements of vertical distribution of liquid and ice particles and their relative abundance. Ice particles are found in relative warm clouds, which can be explained by multiplication of existing ice crystals. However, the role of ice particles in redistributing sun light is minimal.
Robert Wagner, Alexander D. James, Victoria L. Frankland, Ottmar Möhler, Benjamin J. Murray, John M. C. Plane, Harald Saathoff, Ralf Weigel, and Martin Schnaiter
Atmos. Chem. Phys., 23, 6789–6811, https://doi.org/10.5194/acp-23-6789-2023, https://doi.org/10.5194/acp-23-6789-2023, 2023
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Polar stratospheric clouds (PSCs) play an important role in the depletion of stratospheric ozone. They can consist of different chemical species, including crystalline nitric acid hydrates. We found that mineral dust or meteoric ablation material can efficiently catalyse the formation of a specific phase of nitric acid dihydrate crystals. We determined predominant particle shapes and infrared optical properties of these crystals, which are important inputs for remote sensing detection of PSCs.
Franz Martin Schnaiter, Claudia Linke, Eija Asmi, Henri Servomaa, Antti-Pekka Hyvärinen, Sho Ohata, Yutaka Kondo, and Emma Järvinen
Atmos. Meas. Tech., 16, 2753–2769, https://doi.org/10.5194/amt-16-2753-2023, https://doi.org/10.5194/amt-16-2753-2023, 2023
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Light-absorbing particles from combustion processes are important contributors to climate warming. Their highly variable spectral light absorption properties need to be monitored in the field. Commonly used methods show measurement artefacts that are difficult to correct. We introduce a new instrument that is based on the photoacoustic effect. Long-term operation in the Finnish Arctic demonstrates the applicability of the new instrument for unattended light absorption monitoring.
Fritz Waitz, Martin Schnaiter, Thomas Leisner, and Emma Järvinen
Atmos. Chem. Phys., 22, 7087–7103, https://doi.org/10.5194/acp-22-7087-2022, https://doi.org/10.5194/acp-22-7087-2022, 2022
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Riming, i.e., the accretion of small droplets on the surface of ice particles via collision, is one of the major uncertainties in model prediction of mixed-phase clouds. We discuss the occurrence (up to 50% of particles) and aging of rimed ice particles and show correlations of the occurrence and the degree of riming with ambient meteorological parameters using data gathered by the Particle Habit Imaging and Polar Scattering (PHIPS) probe during three airborne in situ field campaigns.
Julia Schneider, Kristina Höhler, Robert Wagner, Harald Saathoff, Martin Schnaiter, Tobias Schorr, Isabelle Steinke, Stefan Benz, Manuel Baumgartner, Christian Rolf, Martina Krämer, Thomas Leisner, and Ottmar Möhler
Atmos. Chem. Phys., 21, 14403–14425, https://doi.org/10.5194/acp-21-14403-2021, https://doi.org/10.5194/acp-21-14403-2021, 2021
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Homogeneous freezing is a relevant mechanism for the formation of cirrus clouds in the upper troposphere. Based on an extensive set of homogeneous freezing experiments at the AIDA chamber with aqueous sulfuric acid aerosol, we provide a new fit line for homogeneous freezing onset conditions of sulfuric acid aerosol focusing on cirrus temperatures. In the atmosphere, homogeneous freezing thresholds have important implications on the cirrus cloud occurrence and related cloud radiative effects.
Janne Lampilahti, Hanna E. Manninen, Tuomo Nieminen, Sander Mirme, Mikael Ehn, Iida Pullinen, Katri Leino, Siegfried Schobesberger, Juha Kangasluoma, Jenni Kontkanen, Emma Järvinen, Riikka Väänänen, Taina Yli-Juuti, Radovan Krejci, Katrianne Lehtipalo, Janne Levula, Aadu Mirme, Stefano Decesari, Ralf Tillmann, Douglas R. Worsnop, Franz Rohrer, Astrid Kiendler-Scharr, Tuukka Petäjä, Veli-Matti Kerminen, Thomas F. Mentel, and Markku Kulmala
Atmos. Chem. Phys., 21, 12649–12663, https://doi.org/10.5194/acp-21-12649-2021, https://doi.org/10.5194/acp-21-12649-2021, 2021
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We studied aerosol particle formation and growth in different parts of the planetary boundary layer at two different locations (Po Valley, Italy, and Hyytiälä, Finland). The observations consist of airborne measurements on board an instrumented Zeppelin and a small airplane combined with comprehensive ground-based measurements.
Fritz Waitz, Martin Schnaiter, Thomas Leisner, and Emma Järvinen
Atmos. Meas. Tech., 14, 3049–3070, https://doi.org/10.5194/amt-14-3049-2021, https://doi.org/10.5194/amt-14-3049-2021, 2021
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A major challenge in the observations of mixed-phase clouds remains the phase discrimination and sizing of cloud droplets and ice crystals, especially for particles with diameters smaller than 0.1 mm. Here, we present a new method to derive the phase and size of single cloud particles using their angular-light-scattering information. Comparisons with other in situ instruments in three case studies show good agreement.
Cited articles
Abdelmonem, A., Järvinen, E., Duft, D., Hirst, E., Vogt, S., Leisner, T., and Schnaiter, M.: PHIPS–HALO: the airborne Particle Habit Imaging and Polar Scattering probe – Part 1: Design and operation, Atmos. Meas. Tech., 9, 3131–3144, https://doi.org/10.5194/amt-9-3131-2016, 2016. a, b
Bailey, M. P. and Hallett, J.: A Comprehensive Habit Diagram for Atmospheric Ice Crystals: Confirmation from the Laboratory, AIRS II, and Other Field Studies, J. Atmos. Sci., 66, 2888–2899, https://doi.org/10.1175/2009JAS2883.1, 2009. a, b, c, d
Baker, B. and Lawson, R. P.: Improvement in Determination of Ice Water Content from Two-Dimensional Particle Imagery. Part I: Image-to-Mass Relationships, J. Appl. Meteorol. Clim., 45, 1282–1290, https://doi.org/10.1175/JAM2398.1, 2006. a
Baran, A. J.: From the single-scattering properties of ice crystals to climate prediction: A way forward, Atmos. Res., 112, 45–69, https://doi.org/10.1016/j.atmosres.2012.04.010, 2012. a
Baran, A. J. and Francis, P. N.: On the radiative properties of cirrus cloud at solar and thermal wavelengths: A test of model consistency using high-resolution airborne radiance measurements, Q. J. Roy. Meteor. Soc., 130, 763–778, https://doi.org/10.1256/qj.03.151, 2004. a
Baran, A. J. and Labonnote, L. C.: On the reflection and polarisation properties of ice cloud, J. Quant. Spectrosc. Ra., 100, 41–54, https://doi.org/10.1016/j.jqsrt.2005.11.062, 2006. a
Baran, A. J., Hill, P., Furtado, K., Field, P., and Manners, J.: A Coupled Cloud Physics–Radiation Parameterization of the Bulk Optical Properties of Cirrus and Its Impact on the Met Office Unified Model Global Atmosphere 5.0 Configuration, J. Climate, 27, 7725–7752, https://doi.org/10.1175/JCLI-D-13-00700.1, 2014. a
Baran, A. J., Hill, P., Walters, D., Hardiman, S. C., Furtado, K., Field, P. R., and Manners, J.: The Impact of Two Coupled Cirrus Microphysics–Radiation Parameterizations on the Temperature and Specific Humidity Biases in the Tropical Tropopause Layer in a Climate Model, J. Climate, 29, 5299–5316, https://doi.org/10.1175/JCLI-D-15-0821.1, 2016. a
Brown, P. R. A. and Francis, P. N.: Improved Measurements of the Ice Water Content in Cirrus Using a Total-Water Probe, J. Atmos. Ocean. Tech., 12, 410–414, https://doi.org/10.1175/1520-0426(1995)012<0410:IMOTIW>2.0.CO;2, 1995. a
Cole, B. H., Yang, P., Baum, B. A., Riedi, J., and C.-Labonnote, L.: Ice particle habit and surface roughness derived from PARASOL polarization measurements, Atmos. Chem. Phys., 14, 3739–3750, https://doi.org/10.5194/acp-14-3739-2014, 2014. a
Cotton, R. J., Field, P. R., Ulanowski, Z., Kaye, P. H., Hirst, E., Greenaway, R. S., Crawford, I., Crosier, J., and Dorsey, J.: The effective density of small ice particles obtained from in situ aircraft observations of mid-latitude cirrus, Q. J. Roy. Meteor. Soc., 139, 1923–1934, https://doi.org/10.1002/qj.2058, 2013.
Erfani, E. and Mitchell, D. L.: Developing and bounding ice particle mass- and area-dimension expressions for use in atmospheric models and remote sensing, Atmos. Chem. Phys., 16, 4379–4400, https://doi.org/10.5194/acp-16-4379-2016, 2016. a
Fridlind, A. M., Atlas, R., van Diedenhoven, B., Um, J., McFarquhar, G. M., Ackerman, A. S., Moyer, E. J., and Lawson, R. P.: Derivation of physical and optical properties of mid-latitude cirrus ice crystals for a size-resolved cloud microphysics model, Atmos. Chem. Phys., 16, 7251–7283, https://doi.org/10.5194/acp-16-7251-2016, 2016. a, b, c, d, e, f, g, h, i, j, k, l, m, n, o
Heymsfield, A. J. and Iaquinta, J.: Cirrus Crystal Terminal Velocities, J. Atmos. Sci., 57, 916–938, https://doi.org/10.1175/1520-0469(2000)057<0916:CCTV>2.0.CO;2, 2000. a
Heymsfield, A. J., Lewis, S., Bansemer, A., Iaquinta, J., Miloshevich, L. M., Kajikawa, M., Twohy, C., and Poellot, M. R.: A General Approach for Deriving the Properties of Cirrus and Stratiform Ice Cloud Particles, J. Atmos. Sci., 59, 3–29, https://doi.org/10.1175/1520-0469(2002)059<0003:AGAFDT>2.0.CO;2, 2002. a, b
Heymsfield, A. J., Bansemer, A., Schmitt, C., Twohy, C., and Poellot, M. R.: Effective Ice Particle Densities Derived from Aircraft Data, J. Atmos. Sci., 61, 982–1003, https://doi.org/10.1175/1520-0469(2004)061<0982:EIPDDF>2.0.CO;2, 2004. a
Hogan, R. J., Tian, L., Brown, P. R. A., Westbrook, C. D., Heymsfield, A. J., and Eastment, J. D.: Radar Scattering from Ice Aggregates Using the Horizontally Aligned Oblate Spheroid Approximation, J. Appl. Meteorol. Clim., 51, 655–671, https://doi.org/10.1175/JAMC-D-11-074.1, 2012. a
Järvinen, E., Jourdan, O., Neubauer, D., Yao, B., Liu, C., Andreae, M. O., Lohmann, U., Wendisch, M., McFarquhar, G. M., Leisner, T., and Schnaiter, M.: Additional global climate cooling by clouds due to ice crystal complexity, Atmos. Chem. Phys., 18, 15767–15781, https://doi.org/10.5194/acp-18-15767-2018, 2018. a
Järvinen, E., van Diedenhoven, B., Magee, N., Neshyba, S., Schnaiter, M., Xu, G., Jourdan, O., Delene, D., Waitz, F., Lolli, S., and Kato, S.: Ice Crystal Complexity and Link to the Cirrus Cloud Radiative Effect, in: Clouds and Their Climatic Impacts, American Geophysical Union (AGU), 47–85, https://doi.org/10.1002/9781119700357.ch3, 2023. a
Jones, S. H., King, M. D., and Ward, A. D.: Determining the unique refractive index properties of solid polystyrene aerosol using broadband Mie scattering from optically trapped beads, Phys. Chem. Chem. Phys., 15, 20735–20741, https://doi.org/10.1039/C3CP53498G, 2013. a
Krämer, M., Rolf, C., Luebke, A., Afchine, A., Spelten, N., Costa, A., Meyer, J., Zöger, M., Smith, J., Herman, R. L., Buchholz, B., Ebert, V., Baumgardner, D., Borrmann, S., Klingebiel, M., and Avallone, L.: A microphysics guide to cirrus clouds – Part 1: Cirrus types, Atmos. Chem. Phys., 16, 3463–3483, https://doi.org/10.5194/acp-16-3463-2016, 2016. a
Lawson, R. P., Baker, B. A., Zmarzly, P., O'Connor, D., Mo, Q., Gayet, J.-F., and Shcherbakov, V.: Microphysical and Optical Properties of Atmospheric Ice Crystals at South Pole Station, J. Appl. Meteorol. Clim., 45, 1505–1524, https://doi.org/10.1175/JAM2421.1, 2006. a
Lawson, R. P., Jensen, E., Mitchell, D. L., Baker, B., Mo, Q., and Pilson, B.: Microphysical and radiative properties of tropical clouds investigated in TC4 and NAMMA, J. Geophys. Res.-Atmos., 115, D00J08, https://doi.org/10.1029/2009JD013017, 2010. a
Lawson, R. P., Woods, S., Jensen, E., Erfani, E., Gurganus, C., Gallagher, M., Connolly, P., Whiteway, J., Baran, A. J., May, P., Heymsfield, A., Schmitt, C. G., McFarquhar, G., Um, J., Protat, A., Bailey, M., Lance, S., Muehlbauer, A., Stith, J., Korolev, A., Toon, O. B., and Krämer, M.: A Review of Ice Particle Shapes in Cirrus formed In Situ and in Anvils, J. Geophys. Res.-Atmos., 124, 10049–10090, https://doi.org/10.1029/2018JD030122, 2019. a, b, c, d, e, f
Liou, K. N.: Influence of Cirrus Clouds on Weather and Climate Processes: A Global Perspective, Mon. Weather Rev., 114, 1167–1199, https://doi.org/10.1175/1520-0493(1986)114<1167:IOCCOW>2.0.CO;2, 1986. a
Liou, K.-N. and Yang, P.: Light Scattering by Ice Crystals: Fundamentals and Applications, Cambridge University Press, Cambridge, https://doi.org/10.1017/CBO9781139030052, 2016. a
Liou, K. N., Yang, P., Takano, Y., Sassen, K., Charlock, T., and Arnott, W.: On the radiative properties of contrail cirrus, Geophys. Res. Lett., 25, 1161–1164, https://doi.org/10.1029/97GL03508, 1998. a
Liu, C., Lee Panetta, R., and Yang, P.: The effects of surface roughness on the scattering properties of hexagonal columns with sizes from the Rayleigh to the geometric optics regimes, J. Quant. Spectrosc. Ra., 129, 169–185, https://doi.org/10.1016/j.jqsrt.2013.06.011, 2013. a
Liu, C., Panetta, R. L., and Yang, P.: The effective equivalence of geometric irregularity and surface roughness in determining particle single-scattering properties, Opt. Express, 22, 23620–23627, https://doi.org/10.1364/OE.22.023620, 2014. a
Lynch, D. K.: Cirrus clouds: Their role in climate and global change, Acta Astronaut., 38, 859–863, https://doi.org/10.1016/S0094-5765(96)00098-7, 1996. a
Macke, A., Mueller, J., and Raschke, E.: Single Scattering Properties of Atmospheric Ice Crystals, J. Atmos. Sci., 53, 2813–2825, https://doi.org/10.1175/1520-0469(1996)053<2813:SSPOAI>2.0.CO;2, 1996. a, b, c, d
McCorquodale, M. W. and Westbrook, C. D.: TRAIL part 2: A comprehensive assessment of ice particle fall speed parametrisations, Q. J. Roy. Meteor. Soc., 147, 605–626, https://doi.org/10.1002/qj.3936, 2021. a
Mie, G.: Beiträge zur Optik trüber Medien, speziell kolloidaler Metallösungen, Ann. Phys.-Berlin, 330, 377–445, https://doi.org/10.1002/andp.19083300302, 1908. a
Mitchell, D. L.: Use of Mass- and Area-Dimensional Power Laws for Determining Precipitation Particle Terminal Velocities, J. Atmos. Sci., 53, 1710–1723, https://doi.org/10.1175/1520-0469(1996)053<1710:UOMAAD>2.0.CO;2, 1996. a
Paltridge, G. W.: Cloud-radiation feedback to climate, Q. J. Roy. Meteor. Soc., 106, 895–899, https://doi.org/10.1002/qj.49710645018, 1980. a
Ren, T., Li, D., Muller, J., and Yang, P.: Sensitivity of Radiative Flux Simulations to Ice Cloud Parameterization over the Equatorial Western Pacific Ocean Region, J. Atmos. Sci., 78, 2549–2571, https://doi.org/10.1175/JAS-D-21-0017.1, 2021. a
Sassen, K., Wang, Z., and Liu, D.: Global distribution of cirrus clouds from CloudSat/Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) measurements, J. Geophys. Res.-Atmos., 113, D00A12, https://doi.org/10.1029/2008JD009972, 2008. a
Schmitt, C. G. and Heymsfield, A. J.: On the Occurrence of Hollow Bullet Rosette– and Column-Shaped Ice Crystals in Midlatitude Cirrus, J. Atmos. Sci., 64, 4514–4519, https://doi.org/10.1175/2007JAS2317.1, 2007. a, b
Schnaiter, M., Järvinen, E., Abdelmonem, A., and Leisner, T.: PHIPS-HALO: the airborne particle habit imaging and polar scattering probe – Part 2: Characterization and first results, Atmos. Meas. Tech., 11, 341–357, https://doi.org/10.5194/amt-11-341-2018, 2018. a, b, c
Schön, R., Schnaiter, M., Ulanowski, Z., Schmitt, C., Benz, S., Möhler, O., Vogt, S., Wagner, R., and Schurath, U.: Particle Habit Imaging Using Incoherent Light: A First Step toward a Novel Instrument for Cloud Microphysics, J. Atmos. Ocean. Tech., 28, 493–512, https://doi.org/10.1175/2011JTECHA1445.1, 2011. a
Stubenrauch, C. J., Rossow, W. B., Kinne, S., Ackerman, S., Cesana, G., Chepfer, H., Girolamo, L. D., Getzewich, B., Guignard, A., Heidinger, A., Maddux, B. C., Menzel, W. P., Minnis, P., Pearl, C., Platnick, S., Poulsen, C., Riedi, J., Sun-Mack, S., Walther, A., Winker, D., Zeng, S., and Zhao, G.: Assessment of Global Cloud Datasets from Satellites: Project and Database Initiated by the GEWEX Radiation Panel, B. Am. Meteorol. Soc., 94, 1031–1049, https://doi.org/10.1175/BAMS-D-12-00117.1, 2013. a
Stubenrauch, C. J., Feofilov, A. G., Protopapadaki, S. E., and Armante, R.: Cloud climatologies from the infrared sounders AIRS and IASI: strengths and applications, Atmos. Chem. Phys., 17, 13625–13644, https://doi.org/10.5194/acp-17-13625-2017, 2017. a
Thermo Fisher Scientific: https://www.thermofisher.com/search/browse/category/us/en/90220126, last access: 1 June 2024. a
Um, J. and McFarquhar, G. M.: Single-Scattering Properties of Aggregates of Bullet Rosettes in Cirrus, J. Appl. Meteorol. Clim., 46, 757–775, https://doi.org/10.1175/JAM2501.1, 2007. a, b
Um, J. and McFarquhar, G. M.: Dependence of the single-scattering properties of small ice crystals on idealized shape models, Atmos. Chem. Phys., 11, 3159–3171, https://doi.org/10.5194/acp-11-3159-2011, 2011. a, b, c
van Diedenhoven, B.: Variation of Ice Microphysical Properties With Temperature and Humidity at Tops of Convective Clouds, Geophys. Res. Lett., 48, e2021GL093673, https://doi.org/10.1029/2021GL093673, 2021. a, b
Wagner, S. W., Schnaiter, M., Xu, G., Nehlert, F., and Järvinen, E.: Bullet Rosette Light Scattering and Microphysical Data from CIRRUS-HL, in: Atmospheric Chemistry and Physics, Zenodo [data set], https://doi.org/10.5281/zenodo.15343726, 2025. a
Warren, S. G.: Optical constants of ice from the ultraviolet to the microwave, Appl. Optics, 23, 1206–1225, https://doi.org/10.1364/AO.23.001206, 1984. a
Weickmann, H. K.: Die Eisphase in der Atmosphäre, Berichte Deutsch Wetterdienstes, US Zone, 6, 3–54, 1949. a
White, F. M.: Viscous Fluid Flow, 3rd edn., McGraw Hill, New York, NY, 656 pp., ISBN 0072402318, 2005. a
Wylie, D. P., Menzel, W. P., Woolf, H. M., and Strabala, K. I.: Four Years of Global Cirrus Cloud Statistics Using HIRS, J. Climate, 7, 1972–1986, https://doi.org/10.1175/1520-0442(1994)007<1972:FYOGCC>2.0.CO;2, 1994. a
Xu, G., Waitz, F., Wagner, S., Nehlert, F., Schnaiter, M., and Järvinen, E.: Toward Better Constrained Scattering Models for Natural Ice Crystals in the Visible Region, J. Geophys. Res.-Atmos., 128, e2022JD037604, https://doi.org/10.1029/2022JD037604, 2023. a, b
Yang, P. and Liou, K. N.: Geometric-optics–integral-equation method for light scattering by nonspherical ice crystals, Appl. Optics, 35, 6568–6584, https://doi.org/10.1364/AO.35.006568, 1996. a
Yang, P. and Liou, K. N.: Single-scattering properties of complex ice crystals in terrestrial atmosphere, Contributions to Atmospheric Physics, 71, 223–248, 1998. a
Yang, P., Zhang, Z., Kattawar, G. W., Warren, S. G., Baum, B. A., Huang, H.-L., Hu, Y. X., Winker, D., and Iaquinta, J.: Effect of Cavities on the Optical Properties of Bullet Rosettes: Implications for Active and Passive Remote Sensing of Ice Cloud Properties, J. Appl. Meteorol. Clim., 47, 2311–2330, https://doi.org/10.1175/2008JAMC1905.1, 2008. a, b, c, d, e, f, g, h, i, j, k
Yang, P., Bi, L., Baum, B. A., Liou, K.-N., Kattawar, G. W., Mishchenko, M. I., and Cole, B.: Spectrally Consistent Scattering, Absorption, and Polarization Properties of Atmospheric Ice Crystals at Wavelengths from 0.2 to 100 µm, J. Atmos. Sci., 70, 330–347, https://doi.org/10.1175/JAS-D-12-039.1, 2013. a, b
Yang, P., Liou, K. N., Bi, L., Liu, C., Yi, B., and Baum, B. A.: On the radiative properties of ice clouds: Light scattering, remote sensing, and radiation parameterization, Adv. Atmos. Sci., 32, 32–63, https://doi.org/10.1007/s00376-014-0011-z, 2015. a
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An important parameter for calculation of the impact of cirrus clouds on climate is the asymmetry parameter. The asymmetry parameter captures the degree to which light is scattered by individual ice crystals towards the ground rather than reflected upwards to space. The measurements presented in this study show that, for a common type of ice crystal called bullet rosettes, cirrus clouds may be far more efficient at reflecting sunlight than is typically assumed in the radiative transfer models used to represent the role of clouds in climate.
An important parameter for calculation of the impact of cirrus clouds on climate is the...
Short summary
Understanding the interaction between cirrus clouds and solar radiation is critical for modeling the Earth's climate. A common crystal type found in cirrus clouds is the bullet rosette. Here, atmospheric bullet rosettes measured from jet aircraft are analyzed for their morphological and radiative properties. Atmospheric bullet rosettes are found to be more morphologically complex than previously assumed. This complexity has a significant impact on their radiative properties.
Understanding the interaction between cirrus clouds and solar radiation is critical for modeling...
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