Articles | Volume 25, issue 12
https://doi.org/10.5194/acp-25-6197-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-25-6197-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
25 Jun 2025
Research article |
| 25 Jun 2025
| 25 Jun 2025
Toward a learnable Artificial Intelligence Model for Aerosol Chemistry and Interactions (AIMACI) based on the Multi-Head Self-Attention algorithm
Zihan Xia
Deep Space Exploration Laboratory/School of Earth and Space Sciences/CMA-USTC Laboratory of Fengyun Remote Sensing/State Key Laboratory of Fire Science/Institute of Advanced Interdisciplinary Research on High-Performance Computing Systems and Software, University of Science and Technology of China, Hefei, China
Chun Zhao
CORRESPONDING AUTHOR
Deep Space Exploration Laboratory/School of Earth and Space Sciences/CMA-USTC Laboratory of Fengyun Remote Sensing/State Key Laboratory of Fire Science/Institute of Advanced Interdisciplinary Research on High-Performance Computing Systems and Software, University of Science and Technology of China, Hefei, China
Laoshan Laboratory, Qingdao, China
CAS Center for Excellence in Comparative Planetology, University of Science and Technology of China, Hefei, China
Zining Yang
Deep Space Exploration Laboratory/School of Earth and Space Sciences/CMA-USTC Laboratory of Fengyun Remote Sensing/State Key Laboratory of Fire Science/Institute of Advanced Interdisciplinary Research on High-Performance Computing Systems and Software, University of Science and Technology of China, Hefei, China
Qiuyan Du
Deep Space Exploration Laboratory/School of Earth and Space Sciences/CMA-USTC Laboratory of Fengyun Remote Sensing/State Key Laboratory of Fire Science/Institute of Advanced Interdisciplinary Research on High-Performance Computing Systems and Software, University of Science and Technology of China, Hefei, China
Jiawang Feng
Deep Space Exploration Laboratory/School of Earth and Space Sciences/CMA-USTC Laboratory of Fengyun Remote Sensing/State Key Laboratory of Fire Science/Institute of Advanced Interdisciplinary Research on High-Performance Computing Systems and Software, University of Science and Technology of China, Hefei, China
Chen Jin
Deep Space Exploration Laboratory/School of Earth and Space Sciences/CMA-USTC Laboratory of Fengyun Remote Sensing/State Key Laboratory of Fire Science/Institute of Advanced Interdisciplinary Research on High-Performance Computing Systems and Software, University of Science and Technology of China, Hefei, China
Jun Shi
School of Computer Science and Technology, University of Science and Technology of China, Hefei, 230026, China
Hong An
Laoshan Laboratory, Qingdao, China
School of Computer Science and Technology, University of Science and Technology of China, Hefei, 230026, China
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Zhiyuan Hu, Chun Zhao, Jianping Huang, L. Ruby Leung, Yun Qian, Hongbin Yu, Lei Huang, and Olga V. Kalashnikova
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Kai Zhang, Chun Zhao, Hui Wan, Yun Qian, Richard C. Easter, Steven J. Ghan, Koichi Sakaguchi, and Xiaohong Liu
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Y. Feng, V. R. Kotamarthi, R. Coulter, C. Zhao, and M. Cadeddu
Atmos. Chem. Phys., 16, 247–264, https://doi.org/10.5194/acp-16-247-2016, https://doi.org/10.5194/acp-16-247-2016, 2016
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S. Yu, R. Mathur, J. Pleim, D. Wong, R. Gilliam, K. Alapaty, C. Zhao, and X. Liu
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H. Wan, P. J. Rasch, K. Zhang, Y. Qian, H. Yan, and C. Zhao
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C. Zhao, X. Liu, Y. Qian, J. Yoon, Z. Hou, G. Lin, S. McFarlane, H. Wang, B. Yang, P.-L. Ma, H. Yan, and J. Bao
Atmos. Chem. Phys., 13, 10969–10987, https://doi.org/10.5194/acp-13-10969-2013, https://doi.org/10.5194/acp-13-10969-2013, 2013
C. Zhao, S. Chen, L. R. Leung, Y. Qian, J. F. Kok, R. A. Zaveri, and J. Huang
Atmos. Chem. Phys., 13, 10733–10753, https://doi.org/10.5194/acp-13-10733-2013, https://doi.org/10.5194/acp-13-10733-2013, 2013
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Related subject area
Subject: Aerosols | Research Activity: Machine Learning | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
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Hourly elemental carbon (EC) and NOx were continuously measured for 5 years (2016–2020) at a sampling site near a highway in western Shanghai. We use a machine learning model to rebuild the measured EC and NOx, and a business-as-usual (BAU) scenario was assumed in 2020 and compared with the measured EC and NOx.
Jin Feng, Yanjie Li, Yulu Qiu, and Fuxin Zhu
Atmos. Chem. Phys., 23, 375–388, https://doi.org/10.5194/acp-23-375-2023, https://doi.org/10.5194/acp-23-375-2023, 2023
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It is important to use weather data to estimate aerosol concentrations. Here, a weather index for aerosol concentration based on deep learning was developed, linking weather and short-term variations in aerosol concentrations over China. The index provides better performance than chemical transport model simulation and other data-based estimation approaches. It can be used as a robust tool for estimating daily variations in aerosol concentrations.
Yu Lin, Leiming Zhang, Qinchu Fan, He Meng, Yang Gao, Huiwang Gao, and Xiaohong Yao
Atmos. Chem. Phys., 22, 16073–16090, https://doi.org/10.5194/acp-22-16073-2022, https://doi.org/10.5194/acp-22-16073-2022, 2022
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In this study, we analyzed 7-year (from May 2014 to April 2021) concentration data of six criteria air pollutants (PM2.5, PM10, O3, NO2, CO and SO2) as well as the sum of NO2 and O3 in six cities in South China. Three different analysis methods were used to identify emission-driven interannual variations and perturbations from varying weather conditions. In addition, a self-developed method was further introduced to constrain analysis uncertainties.
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Short summary
Traditional numerical schemes of aerosol chemistry and interactions (ACI) in atmospheric models are computationally costly and are often simplified or omitted, introducing uncertainties. We use an AI scheme to achieve fast, accurate, and stable end-to-end simulation for full ACI within an atmospheric model, replacing numerical schemes. This innovation is expected to enhance the accuracy and efficiency of ACI simulations in climate models that would otherwise neglect or simplify ACI processes.
Traditional numerical schemes of aerosol chemistry and interactions (ACI) in atmospheric models...
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