Articles | Volume 25, issue 22
https://doi.org/10.5194/acp-25-16775-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-25-16775-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Is the summer aerosol over the Arctic controlled by regional atmospheric circulation or ice conditions? Trends and future implications
Caroline Leck
CORRESPONDING AUTHOR
Department of Meteorology and Bert Bolin Centre for Climate Research, Stockholm University, Stockholm, 106 91, Sweden
Jost Heintzenberg
Leibniz Institute for Tropospheric Research, Leipzig, 04318, Germany
Tiina Nygård
Finnish Meteorological Institute, PB 503, Helsinki, 00101, Finland
Tuomas Naakka
Finnish Meteorological Institute, PB 503, Helsinki, 00101, Finland
Related authors
Ines Bulatovic, Julien Savre, Michael Tjernström, Caroline Leck, and Annica M. L. Ekman
Atmos. Chem. Phys., 23, 7033–7055, https://doi.org/10.5194/acp-23-7033-2023, https://doi.org/10.5194/acp-23-7033-2023, 2023
Short summary
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We use numerical modeling with detailed cloud microphysics to investigate a low-altitude cloud system consisting of two cloud layers – a type of cloud situation which was commonly observed during the summer of 2018 in the central Arctic (north of 80° N). The model generally reproduces the observed cloud layers and the thermodynamic structure of the lower atmosphere well. The cloud system is maintained unless there are low aerosol number concentrations or high large-scale wind speeds.
Ines Bulatovic, Adele L. Igel, Caroline Leck, Jost Heintzenberg, Ilona Riipinen, and Annica M. L. Ekman
Atmos. Chem. Phys., 21, 3871–3897, https://doi.org/10.5194/acp-21-3871-2021, https://doi.org/10.5194/acp-21-3871-2021, 2021
Short summary
Short summary
We use detailed numerical modelling to show that small aerosol particles (diameters ~25–80 nm; so-called Aitken mode particles) significantly influence low-level cloud properties in the clean summertime high Arctic. The small particles can help sustain clouds when the concentration of larger particles is low (<10–20 cm-3). Measurements from four different observational campaigns in the high Arctic support the modelling results as they indicate that Aitken mode aerosols are frequently activated.
André Welti, E. Keith Bigg, Paul J. DeMott, Xianda Gong, Markus Hartmann, Mike Harvey, Silvia Henning, Paul Herenz, Thomas C. J. Hill, Blake Hornblow, Caroline Leck, Mareike Löffler, Christina S. McCluskey, Anne Marie Rauker, Julia Schmale, Christian Tatzelt, Manuela van Pinxteren, and Frank Stratmann
Atmos. Chem. Phys., 20, 15191–15206, https://doi.org/10.5194/acp-20-15191-2020, https://doi.org/10.5194/acp-20-15191-2020, 2020
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Ship-based measurements of maritime ice nuclei concentrations encompassing all oceans are compiled. From this overview it is found that maritime ice nuclei concentrations are typically 10–100 times lower than over continents, while concentrations are surprisingly similar in different oceanic regions. The analysis of the influence of ship emissions shows no effect on the data, making ship-based measurements an efficient strategy for the large-scale exploration of ice nuclei concentrations.
Tuomas Naakka, Daniel Köhler, Kalle Nordling, Petri Räisänen, Marianne Tronstad Lund, Risto Makkonen, Joonas Merikanto, Bjørn H. Samset, Victoria A. Sinclair, Jennie L. Thomas, and Annica M. L. Ekman
Atmos. Chem. Phys., 25, 8127–8145, https://doi.org/10.5194/acp-25-8127-2025, https://doi.org/10.5194/acp-25-8127-2025, 2025
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The effects of warmer sea surface temperatures and decreasing sea ice cover on polar climates have been studied using four climate models with identical prescribed changes in sea surface temperatures and sea ice cover. The models predict similar changes in air temperature and precipitation in the polar regions in a warmer climate with less sea ice. However, the models disagree on how the atmospheric circulation, i.e. the large-scale winds, will change with warmer temperatures and less sea ice.
Elena Shevnina, Timo Vihma, Miguel Potes, and Tuomas Naakka
EGUsphere, https://doi.org/10.5194/egusphere-2025-1964, https://doi.org/10.5194/egusphere-2025-1964, 2025
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The study first estimated the summertime evaporation over lakes located in coastal Antarctica with direct (eddy-covariance) measurements collected during two austral summers (December–January) in 2017–2018 and 2019–2020. The lake evaporation was on average 1.6 mm d-1 in the ice break-up period, and it doubled in the ice free period. The bulk aerodynamic method with a site-specific transfer coefficient of moisture well reproduced the observed day-to-day variations in evaporation over lakes.
Daniel Köhler, Petri Räisänen, Tuomas Naakka, Kalle Nordling, and Victoria A. Sinclair
Weather Clim. Dynam., 6, 669–694, https://doi.org/10.5194/wcd-6-669-2025, https://doi.org/10.5194/wcd-6-669-2025, 2025
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We study the impacts of globally increasing sea surface temperatures and sea ice loss on the atmosphere in wintertime. In future climates, the jet stream shifts southward over the North Atlantic and extends further over Europe. Increasing sea surface temperatures drives these changes. The region of high activity of low-pressure systems is projected to move east towards Europe. Future increasing sea surface temperatures and sea ice loss contribute with similar magnitude to the eastward shift.
Tiina Nygård, Lukas Papritz, Tuomas Naakka, and Timo Vihma
Weather Clim. Dynam., 4, 943–961, https://doi.org/10.5194/wcd-4-943-2023, https://doi.org/10.5194/wcd-4-943-2023, 2023
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Despite the general warming trend, wintertime cold-air outbreaks in Europe have remained nearly as extreme and as common as decades ago. In this study, we identify six principal cold anomaly types over Europe in 1979–2020. We show the origins of various physical processes and their contributions to the formation of cold wintertime air masses.
Ines Bulatovic, Julien Savre, Michael Tjernström, Caroline Leck, and Annica M. L. Ekman
Atmos. Chem. Phys., 23, 7033–7055, https://doi.org/10.5194/acp-23-7033-2023, https://doi.org/10.5194/acp-23-7033-2023, 2023
Short summary
Short summary
We use numerical modeling with detailed cloud microphysics to investigate a low-altitude cloud system consisting of two cloud layers – a type of cloud situation which was commonly observed during the summer of 2018 in the central Arctic (north of 80° N). The model generally reproduces the observed cloud layers and the thermodynamic structure of the lower atmosphere well. The cloud system is maintained unless there are low aerosol number concentrations or high large-scale wind speeds.
Elena Shevnina, Miguel Potes, Timo Vihma, Tuomas Naakka, Pankaj Ramji Dhote, and Praveen Kumar Thakur
The Cryosphere, 16, 3101–3121, https://doi.org/10.5194/tc-16-3101-2022, https://doi.org/10.5194/tc-16-3101-2022, 2022
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The evaporation over an ice-free glacial lake was measured in January 2018, and the uncertainties inherent to five indirect methods were quantified. Results show that in summer up to 5 mm of water evaporated daily from the surface of the lake located in Antarctica. The indirect methods underestimated the evaporation over the lake's surface by up to 72 %. The results are important for estimating the evaporation over polar regions where a growing number of glacial lakes have recently been evident.
Silvia Becagli, Elena Barbaro, Simone Bonamano, Laura Caiazzo, Alcide di Sarra, Matteo Feltracco, Paolo Grigioni, Jost Heintzenberg, Luigi Lazzara, Michel Legrand, Alice Madonia, Marco Marcelli, Chiara Melillo, Daniela Meloni, Caterina Nuccio, Giandomenico Pace, Ki-Tae Park, Suzanne Preunkert, Mirko Severi, Marco Vecchiato, Roberta Zangrando, and Rita Traversi
Atmos. Chem. Phys., 22, 9245–9263, https://doi.org/10.5194/acp-22-9245-2022, https://doi.org/10.5194/acp-22-9245-2022, 2022
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Measurements of phytoplanktonic dimethylsulfide and its oxidation products in the Antarctic atmosphere allow us to understand the role of the oceanic (sea ice melting, Chl α and dimethylsulfoniopropionate) and atmospheric (wind direction and speed, humidity, solar radiation and transport processes) factors in the biogenic aerosol formation, concentration and characteristic ratio between components in an Antarctic coastal site facing the polynya of the Ross Sea.
Stephen M. Platt, Øystein Hov, Torunn Berg, Knut Breivik, Sabine Eckhardt, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Markus Fiebig, Rebecca Fisher, Georg Hansen, Hans-Christen Hansson, Jost Heintzenberg, Ove Hermansen, Dominic Heslin-Rees, Kim Holmén, Stephen Hudson, Roland Kallenborn, Radovan Krejci, Terje Krognes, Steinar Larssen, David Lowry, Cathrine Lund Myhre, Chris Lunder, Euan Nisbet, Pernilla B. Nizzetto, Ki-Tae Park, Christina A. Pedersen, Katrine Aspmo Pfaffhuber, Thomas Röckmann, Norbert Schmidbauer, Sverre Solberg, Andreas Stohl, Johan Ström, Tove Svendby, Peter Tunved, Kjersti Tørnkvist, Carina van der Veen, Stergios Vratolis, Young Jun Yoon, Karl Espen Yttri, Paul Zieger, Wenche Aas, and Kjetil Tørseth
Atmos. Chem. Phys., 22, 3321–3369, https://doi.org/10.5194/acp-22-3321-2022, https://doi.org/10.5194/acp-22-3321-2022, 2022
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Here we detail the history of the Zeppelin Observatory, a unique global background site and one of only a few in the high Arctic. We present long-term time series of up to 30 years of atmospheric components and atmospheric transport phenomena. Many of these time series are important to our understanding of Arctic and global atmospheric composition change. Finally, we discuss the future of the Zeppelin Observatory and emerging areas of future research on the Arctic atmosphere.
Tiina Nygård, Michael Tjernström, and Tuomas Naakka
Weather Clim. Dynam., 2, 1263–1282, https://doi.org/10.5194/wcd-2-1263-2021, https://doi.org/10.5194/wcd-2-1263-2021, 2021
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Temperature and humidity profiles in the Arctic atmosphere in winter are affected by both the large-scale dynamics and the local processes, such as radiation, cloud formation and turbulence. The results show that the influence of different large-scale flows on temperature and humidity profiles must be viewed as a progressing set of processes. Within the Arctic, there are notable regional differences in how large-scale flows affect the temperature and specific humidity profiles.
Ines Bulatovic, Adele L. Igel, Caroline Leck, Jost Heintzenberg, Ilona Riipinen, and Annica M. L. Ekman
Atmos. Chem. Phys., 21, 3871–3897, https://doi.org/10.5194/acp-21-3871-2021, https://doi.org/10.5194/acp-21-3871-2021, 2021
Short summary
Short summary
We use detailed numerical modelling to show that small aerosol particles (diameters ~25–80 nm; so-called Aitken mode particles) significantly influence low-level cloud properties in the clean summertime high Arctic. The small particles can help sustain clouds when the concentration of larger particles is low (<10–20 cm-3). Measurements from four different observational campaigns in the high Arctic support the modelling results as they indicate that Aitken mode aerosols are frequently activated.
André Welti, E. Keith Bigg, Paul J. DeMott, Xianda Gong, Markus Hartmann, Mike Harvey, Silvia Henning, Paul Herenz, Thomas C. J. Hill, Blake Hornblow, Caroline Leck, Mareike Löffler, Christina S. McCluskey, Anne Marie Rauker, Julia Schmale, Christian Tatzelt, Manuela van Pinxteren, and Frank Stratmann
Atmos. Chem. Phys., 20, 15191–15206, https://doi.org/10.5194/acp-20-15191-2020, https://doi.org/10.5194/acp-20-15191-2020, 2020
Short summary
Short summary
Ship-based measurements of maritime ice nuclei concentrations encompassing all oceans are compiled. From this overview it is found that maritime ice nuclei concentrations are typically 10–100 times lower than over continents, while concentrations are surprisingly similar in different oceanic regions. The analysis of the influence of ship emissions shows no effect on the data, making ship-based measurements an efficient strategy for the large-scale exploration of ice nuclei concentrations.
Cited articles
Alexander, L. V., Uotila, P., Nicholls, N., and Lynch, A.: A New Daily Pressure Dataset for Australia and Its Application to the Assessment of Changes in Synoptic Patterns during the Last Century, J. Climate, 23, 1111–1126, https://doi.org/10.1175/2009jcli2972.1, 2010.
Arrigo, K. R., Perovich, D. K., Pickart, R. S., Brown, Z. W., van Dijken, G. L., Lowry, K. E., Mills, M. M., Palmer, M. A., Balch, W. M., Bahr, F., Bates, N. R., Benitez-Nelson, C., Bowler, B., Brownlee, E., Ehn, J. K., Frey, K. E., Garley, R., Laney, S. R., Lubelczyk, L., Mathis, J., Matsuoka, A., Mitchell, B. G., Moore, G. W. K., Ortega-Retuerta, E., Pal, S., Polashenski, C. M., Reynolds, R. A., Schieber, B., Sosik, H. M., Stephens, M., and Swift, J. H.: Massive Phytoplankton Blooms Under Arctic Sea Ice, Science, 336, 1408–1408, https://doi.org/10.1126/science.1215065, 2012.
Aslam, S. N., Michel, C., Niemi, A., and Underwood, G. J. C.: Patterns and drivers of carbohydrate budgets in ice algal assemblages from first year Arctic sea ice, Limnol. Oceanogr., 61, 919–937, https://doi.org/10.1002/lno.10260, 2016.
Baccarini, A., Karlsson, L., Dommen, J., Duplessis, P., Vüllers, J., Brooks, I. M., Saiz-Lopez, A., Salter, M., Tjernström, M., Baltensperger, U., Zieger, P., and Schmale, J.: Frequent new particle formation over the high Arctic pack ice by enhanced iodine emissions, Nature Communications, 11, 4924, https://doi.org/10.1038/s41467-020-18551-0, 2020a.
Baccarini, A., Schmale, J., and Dommen, J.: Concentration of particles larger than 2.5 nm collected during the Arctic Ocean 2018 expedition, Bolin Centre Database [data set], https://doi.org/10.17043/oden-ao-2018-aerosol-ucpc-1, 2020b.
Beck, L. J., Sarnela, N., Junninen, H., Hoppe, C. J. M., Garmash, O., Bianchi, F., Riva, M., Rose, C., Peräkylä, O., Wimmer, D., Kausiala, O., Jokinen, T., Ahonen, L., Mikkilä, J., Hakala, J., He, X.-C., Kontkanen, J., Wolf, K. K. E., Cappelletti, D., Mazzola, M., Traversi, R., Petroselli, C., Viola, A. P., Vitale, V., Lange, R., Massling, A., Nøjgaard, J. K., Krejci, R., Karlsson, L., Zieger, P., Jang, S., Lee, K., Vakkari, V., Lampilahti, J., Thakur, R. C., Leino, K., Kangasluoma, J., Duplissy, E.-M., Siivola, E., Marbouti, M., Tham, Y. J., Saiz-Lopez, A., Petäjä, T., Ehn, M., Worsnop, D. R., Skov, H., Kulmala, M., Kerminen, V.-M., and Sipilä, M.: Differing Mechanisms of New Particle Formation at Two Arctic Sites, Geophysical Research Letters, 48, e2020GL091334, https://doi.org/10.1029/2020GL091334, 2021.
Bowman, J. S. and Deming, J. W.: Elevated bacterial abundance and exopolymers in saline frost flowers and implications for atmospheric chemistry and microbial dispersal, Geophysical Research Letters, 37, https://doi.org/10.1029/2010GL043020, 2010.
Bulatovic, I., Igel, A. L., Leck, C., Heintzenberg, J., Riipinen, I., and Ekman, A. M. L.: The importance of Aitken mode aerosol particles for cloud sustenance in the summertime high Arctic – a simulation study supported by observational data, Atmos. Chem. Phys., 21, 3871–3897, https://doi.org/10.5194/acp-21-3871-2021, 2021.
Carmack, E. and Wassmann, P.: Food webs and physical–biological coupling on pan-Arctic shelves: Unifying concepts and comprehensive perspectives, Progress in Oceanography, 71, 446-477, https://doi.org/10.1016/j.pocean.2006.10.004, 2006.
Comiso, J.: Fundamental Characteristics of the Polar Oceans and Their Sea Ice Cover, in: Polar Oceans from Space, Springer New York, New York, NY, 19–71, https://doi.org/10.1007/978-0-387-68300-3, 2010.
Covert, D. S., Wiedensohler, A., Aalto, P., Heintzenberg, J., McMurry, P. H., and Leck, C.: Aerosol number size distributions from 3 to 500 nm diameter in the arctic marine boundary layer during summer and autumn, Tellus, 48B, 197–212, 1996.
Deming, J. W. and Young, J. N.: The Role of Exopolysaccharides in Microbial Adaptation to Cold Habitats, in: Psychrophiles: From Biodiversity to Biotechnology, edited by: Margesin, R., Springer International Publishing, Cham, 259–284, https://doi.org/10.1007/978-3-319-57057-0 12, 2017.
Ding, Q., Schweiger, A., L'Heureux, M., Battisti, D. S., Po-Chedley, S., Johnson, N. C., Blanchard-Wrigglesworth, E., Harnos, K., Zhang, Q., Eastman, R., and Steig, E. J.: Influence of high-latitude atmospheric circulation changes on summertime Arctic sea ice, Nature Clim. Change, 7, 289–295, https://doi.org/10.1038/nclimate3241, 2017.
Duplessis, P., Karlsson, L., Baccarini, A., Wheeler, M., Leaitch, W. R., Svenningsson, B., Leck, C., Schmale, J., Zieger, P., and Chang, R. Y.-W.: Highly hygroscopic aerosols facilitate summer and early-autumn cloud formation at extremely low concentrations over the central Arctic Ocean, Journal of Geophysical Research: Atmospheres, 129, e2023JD039159, https://doi.org/10.1029/2023JD039159, 2024.
Galley, R. J., Else, B. G. T., Geilfus, N. X., Hare, A. A., Isleifson, D., Barber, D. G., and Rysgaard, S.: Imaged brine inclusions in young sea ice – Shape, distribution and formation timing, Cold Reg. Sci. Technol., 111, 39–48, https://doi.org/10.1016/j.coldregions.2014.12.011, 2015.
Good, S.: Global Ocean OSTIA Sea Surface Temperature and Sea Ice Analysis, EU Copernicus Marine Service Information 80 (CMEMS), Marine Data Store (MDS) [data set], https://doi.org/10.48670/moi-00165, 2022.
Heintzenberg, J. and Leck, C.: The summer aerosol in the central Arctic 1991–2008: did it change or not?, Atmos. Chem. Phys., 12, 3969–3983, https://doi.org/10.5194/acp-12-3969-2012, 2012.
Heintzenberg, J., Leck, C., Birmili, W., Wehner, B., Tjernström, M., and Wiedensohler, A.: Aerosol number-size distributions during clear and fog periods in the summer high Arctic: 1991, 1996, and 2001, Tellus, 58B, 41–50, 2006.
Heintzenberg, J., Leck, C., and Tunved, P.: Potential source regions and processes of aerosol in the summer Arctic, Atmos. Chem. Phys., 15, 6487–6502, https://doi.org/10.5194/acp-15-6487-2015, 2015.
Hersbach, H., Bell, B., Berrisford, P., Hirahara, S., Horányi, A., Muñoz-Sabater, J., Nicolas, J., Peubey, C., Radu, R., Schepers, D., Simmons, A., Soci, C., Abdalla, S., Abellan, X., Balsamo, G., Bechtold, P., Biavati, G., Bidlot, J., Bonavita, M., De Chiara, G., Dahlgren, P., Dee, D., Diamantakis, M., Dragani, R., Flemming, J., Forbes, R., Fuentes, M., Geer, A., Haimberger, L., Healy, S., Hogan, R. J., Hólm, E., Janisková, M., Keeley, S., Laloyaux, P., Lopez, P., Lupu, C., Radnoti, G., de Rosnay, P., Rozum, I., Vamborg, F., Villaume, S., and Thépaut, J.-N.: The ERA5 global reanalysis, Q. J. Roy. Meteorol. Soc., 146, 1999–2049, https://doi.org/10.1002/qj.3803, 2020.
Hersbach, H., Bell, B., Berrisford, P., Biavati, G., Horányi, A., Muñoz Sabater, J., Nicolas, J., Peubey, C., Radu, R., Rozum, I., Schepers, D., Simmons, A., Soci, C., Dee, D., and Thépaut, J.-N.: ERA5 hourly data on single levels from 1940 to present, Copernicus Climate Change Service (C3S) Climate Data Store (CDS) [data set], https://doi.org/10.24381/cds.adbb2d47, 2023.
Hewitson, B. C. and Crane, R. G.: Self-organizing maps: applications to synoptic climatology, Climate Research, 22, 13–26, 2002.
Kanamitsu, M.: Description of the NMC Global Data Assimilation and Forecast System, Weather Forecasting, 4, 335–342, https://doi.org/10.1175/1520-0434(1989)004<0335:DOTNGD>2.0.CO;2, 1989.
Karl, M., Gross, A., Leck, C., and Pirjola, L.: Intercomparison of dimethylsulfide oxidation mechanisms for the marine boundary layer: Gaseous and particulate sulfur constituents, J. Geophys. Res., 112, D15304, https://doi.org/10.1029/2006JD007914, 2007.
Karl, M., Leck, C., Coz, E., and Heintzenberg, J.: Marine nanogels as a source of atmospheric nanoparticles in the high Arctic, Geophysical Research Letters, 40, 3738–3743, https://doi.org/10.1002/grl.50661, 2013.
Karlsson, L., Baccarini, A., Duplessis, P., Baumgardner, D., Brooks, I. M., Chang, R. Y.-W., Dada, L., Dällenbach, K. R., Heikkinen, L., Krejci, R., Leaitch, W. R., Leck, C., Partridge, D. G., Salter, M. E., Wernli, H., Wheeler, M. J., Schmale, J., Zieger, P.: Physical and chemical properties of cloud droplet residuals and aerosol particles during the Arctic Ocean 2018 expedition, Journal of Geophysical Research, Atmospheres, 127, 1–20, https://doi.org/10.1029/2021JD036383, 2022.
Karlsson, L. and Zieger, P.: Aerosol particle number size distribution data collected during the Arctic Ocean 2018 expedition, Bolin Centre Database [data set], https://doi.org/10.17043/oden-ao-2018-aerosol-dmps-1, 2020.
Kerminen, V.-M. and Leck, C.: Sulfur chemistry over the Central Arctic Ocean in summer: Gas to particulate transformation, J. Geophys. Res., 106, 32087–32100, 2001.
Kohonen, T.: Self-Organizing Maps, Springer-Verlag, 501 pp., https://doi.org/10.1007/978-3-642-56927-2, 2001.
Lawler, M. J., Saltzman, E. S., Karlsson, L., Zieger, P., Salter, M., Baccarini, A., Schmale, J., and Leck, C.: New Insights Into the Composition and Origins of Ultrafine Aerosol in the Summertime High Arctic, Geophys. Res. Lett., 48, e2021GL094395, https://doi.org/10.1029/2021GL094395, 2021.
Leck, C. and Bigg, E. K.: Biogenic particles in the surface microlayer and overlaying atmosphere in the central Arctic Ocean during summer, Tellus, 57B, 305–316, 2005a.
Leck, C. and Bigg, E. K.: Evolution of the marine aerosol – A new perspective, Geophys. Res. Lett., 32, https://doi.org/10.1029/2005GL023651, 2005b.
Leck, C. and Bigg, E. K.: New particle formation of marine biological origin, Aerosol Sci. Technol., 44, 570–577, 2010.
Leck, C. and Bigg, E. K.: Aerosol production over remote marine areas – A new route, Geophys. Res. Lett., 23, 3577–3581, 1999.
Leck, C. and Persson, C.: The central Arctic Ocean as a source of dimethyl sulfide: Seasonal variability in relation to biological activity, Tellus, 48B, 156–177, 1996a.
Leck, C. and Persson, C.: Seasonal and short-term variability in dimethyl sulfide, sulfur dioxide and biogenic sulfur and sea salt aerosol particles in the arctic marine boundary layer, during summer and autumn, Tellus, 48B, 272–299, 1996b.
Leck, C. and Svensson, E.: Importance of aerosol composition and mixing state for cloud droplet activation over the Arctic pack ice in summer, Atmos. Chem. Phys., 15, 2545–2568, https://doi.org/10.5194/acp-15-2545-2015, 2015.
Leck, C., Bigg, E. K., Covert, D. S., Heintzenberg, J., Maenhaut, W., Nilsson, E. D., and Wiedensohler, A.: Overview of the atmospheric research program during the International Arctic Ocean Expedition of 1991 (IAOE-91) and its scientific results, Tellus, 48B, 136–155, 1996.
Leck, C., Nilsson, E. D., Bigg, E. K., and Bäcklin, L.: The atmospheric program on the Arctic Ocean Expedition 1996 (AOE-96): An overview of scientific goals, experimental approach, and instruments, J. Geophys. Res., 106, 32051–32067, 2001.
Leck, C., Norman, M., Bigg, E. K., and Hillamo, R.: Chemical composition and sources of the high Arctic aerosol relevant for cloud formation, J. Geophys. Res., 107, https://doi.org/10.1029/2001JD001463, 2002.
Leck, C., Tjernström, M., Matrai, M. P., Swietlicki, E., and Bigg, E. K.: Can Marine Micro-organisms Influence Melting of the Arctic Pack Ice?, EOS, 85, 25–26, 2004.
Leck, C., Matrai, P., Perttu, A.-M., and Gårdfeldt, K.: Expedition report: SWEDARTIC Arctic Ocean 2018, Swedish, Polar Research Secretariat, Stockholm, ISBN 978-991-519-3671-3670, 2019.
Lee, M.-H. and Kim, J.-H.: The Role of Synoptic Cyclones for the Formation of Arctic Summer Circulation Patterns as Clustered by Self-Organizing Maps, Atmosphere, 10, 474, https://doi.org/10.3390/atmos10080474, 2019.
Mauritsen, T., Sedlar, J., Tjernström, M., Leck, C., Martin, M., Shupe, M., Sjogren, S., Sierau, B., Persson, P. O. G., Brooks, I. M., and Swietlicki, E.: An Arctic CCN-limited cloud-aerosol regime, Atmos. Chem. Phys., 11, 165–173, https://doi.org/10.5194/acp-11-165-2011, 2011.
Meier, W. N., Hovelsrud, G. K., van Oort, B. E. H., Key, J. R., Kovacs, K. M., Michel, C., Haas, C., Granskog, M. A., Gerland, S., Perovich, D. K., Makshtas, A., and Reist, J. D.: Arctic sea ice in transformation: A review of recent observed changes and impacts on biology and human activity, Rev. Geophys., 52, 185–217, https://doi.org/10.1002/2013RG000431, 2014.
Mortin, J., Svensson, G., Graversen, R. G., Kapsch, M.-L., Stroeve, J. C., and Boisvert, L. N.: Melt onset over Arctic sea ice controlled by atmospheric moisture transport, Geophysical Research Letters, 43, 6636–6642, https://doi.org/10.1002/2016GL069330, 2016.
Nilsson, E. D. and Barr, S.: Effcts of synoptic patterns on atmospheric chemistry and aerosols during the Arctic Ocean Expedition 1996, J. Geophys. Res., 106, 32069–32086, 2001.
Nilsson, E. D. and Leck, C.: A pseudo-Lagrangian study of the sulfur budget in the remote Arctic marine boundary layer, Tellus B, 54, 213–230, 2002.
Nygård, T., Graversen, R. G., Uotila, P., Naakka, T., and Vihma, T.: Strong Dependence of Wintertime Arctic Moisture and Cloud Distributions on Atmospheric Large-Scale Circulation, J. Climate, 32, 8771–8790, https://doi.org/10.1175/JCLI-D-19-0242.1, 2019.
Nygård, T., Tjernström, M., and Naakka, T.: Winter thermodynamic vertical structure in the Arctic atmosphere linked to large-scale circulation, Weather Clim. Dynam., 2, 1263–1282, https://doi.org/10.5194/wcd-2-1263-2021, 2021.
Ogren, J. A. and Heintzenberg, J.: Parametric aerosol sampling at low concentration levels, Report AA-1, Department of Meteorology, Stockholm University, 11 pp., ISSN 1101-4814, 1990.
Orellana, M. V., Matrai, P. A., Leck, C., Rauschenberg, C. D., Lee, A. M., and Coz, E.: Marine microgels as a source of cloud condensation nuclei in the high Arctic, Proceedings of the National Academy of Sciences, 108, 13612–13617, 2011.
Orellana, M. V., Hansell, D. A., Matrai, P. A., and Leck, C.: Marine Polymer-Gels' Relevance in the Atmosphere as Aerosols and CCN, Gels, 7, 185, https://doi.org//10.3390/gels7040185, 2021.
Perovich, D. K. and Richter-Menge, J. A.: Surface characteristics of lead ice, Journal of Geophysical Research: Oceans, 99, 16341–16350, https://doi.org/10.1029/94JC01194, 1994.
Polyakov, I. V., Ingvaldsen, R. B., Pnyushkov, A. V., Bhatt, U. S., Francis, J. A., Janout, M., Kwok, R., and Skagseth, Ø.: Fluctuating Atlantic inflows modulate Arctic atlantification, Science, 381, 972–979, https://doi.org/10.1126/science.adh5158, 2023.
Rantanen, M., Karpechko, A. Y., Lipponen, A., Nordling, K., Hyvärinen, O., Ruosteenoja, K., Vihma, T., and Laaksonen, A.: The Arctic has warmed nearly four times faster than the globe since 1979, Communications Earth & Environment, 3, 168, https://doi.org/10.1038/s43247-022-00498-3, 2022.
Rigor, I. G., Colony, R. L., and Martin, S.: Variations in Surface Air Temperature Observations in the Arctic, 1979–97, J. Climate, 13, 896–914, https://doi.org/10.1175/1520-0442(2000)013<0896:VISATO>2.0.CO;2, 2000.
Saiz-Lopez, A., Blaszczak-Boxe, C. S., and Carpenter, L. J.: A mechanism for biologically induced iodine emissions from sea ice, Atmos. Chem. Phys., 15, 9731–9746, https://doi.org/10.5194/acp-15-9731-2015, 2015.
Serreze, M. C. and Barrett, A. P.: The Summer Cyclone Maximum over the Central Arctic Ocean, J. Climate, 21, 1048–1065, https://doi.org/10.1175/2007JCLI1810.1, 2008.
Stein, A. F., Draxler, R. R., Rolph, G. D., Stunder, B. J. B., Cohen, M. D., and Ngan, F.: NOAA's HYSPLIT Atmospheric Transport and Dispersion Modeling System, B. Am. Meteorol. Soc., 96, 2059–2077, https://doi.org/10.1175/BAMS-D-14-00110.1, 2015.
Thomas, M. A., Devasthale, A., and Nygård, T.: Influence of springtime atmospheric circulation types on the distribution of air pollutants in the Arctic, Atmos. Chem. Phys., 21, 16593–16608, https://doi.org/10.5194/acp-21-16593-2021, 2021.
Thomdike, A. S. and Cheung, J. Y.: A IDJEX measurements of sea ice motion 11 April 1975 to 14 May 1976, AIDJEX Bull., 35, 1–149, 1977.
Timmermans, M.-L. and Marshall, J.: Understanding Arctic Ocean Circulation: A Review of Ocean Dynamics in a Changing Climate, Journal of Geophysical Research: Oceans, 125, e2018JC014378, https://doi.org/10.1029/2018JC014378, 2020.
Titchner, H. A. and Rayner, N. A.: The Met Office Hadley Centre sea ice and sea surface temperature data set, version 2: 1. Sea ice concentrations, J. Geophys. Res., 119, 2864–2889, https://doi.org/10.1002/2013JD020316, 2014.
Tjernström, M., Birch, C. E., Brooks, I. M., Shupe, M. D., Persson, P. O. G., Sedlar, J., Mauritsen, T., Leck, C., Paatero, J., Szczodrak, M., and Wheeler, C. R.: Meteorological conditions in the central Arctic summer during the Arctic Summer Cloud Ocean Study (ASCOS), Atmos. Chem. Phys., 12, 6863–6889, https://doi.org/10.5194/acp-12-6863-2012, 2012.
Tjernström, M., Leck, C., Birch, C. E., Bottenheim, J. W., Brooks, B. J., Brooks, I. M., Bäcklin, L., Chang, R. Y.-W., de Leeuw, G., Di Liberto, L., de la Rosa, S., Granath, E., Graus, M., Hansel, A., Heintzenberg, J., Held, A., Hind, A., Johnston, P., Knulst, J., Martin, M., Matrai, P. A., Mauritsen, T., Müller, M., Norris, S. J., Orellana, M. V., Orsini, D. A., Paatero, J., Persson, P. O. G., Gao, Q., Rauschenberg, C., Ristovski, Z., Sedlar, J., Shupe, M. D., Sierau, B., Sirevaag, A., Sjogren, S., Stetzer, O., Swietlicki, E., Szczodrak, M., Vaattovaara, P., Wahlberg, N., Westberg, M., and Wheeler, C. R.: The Arctic Summer Cloud Ocean Study (ASCOS): overview and experimental design, Atmos. Chem. Phys., 14, 2823–2869, https://doi.org/10.5194/acp-14-2823-2014, 2014.
Twomey, S.: Pollution and the planetary albedo, Atmos. Environ., 8, 1251–1256, 1974.
Vüllers, J., Achtert, P., Brooks, I. M., Tjernström, M., Prytherch, J., Burzik, A., and Neely III, R.: Meteorological and cloud conditions during the Arctic Ocean 2018 expedition, Atmos. Chem. Phys., 21, 289–314, https://doi.org/10.5194/acp-21-289-2021, 2021.
Wassmann, P. and Reigstad, M.: Future Arctic Ocean Seasonal Ice Zones and Implications for Pelagic-Benthic Coupling, Oceanography, 24, 220–231, 2011.
Whitby, E. and McMurry, P. H.: Modal aerosol dynamics modeling, Aerosol Sci. Technol., 27, 673–688, 1997.
Short summary
Five summer cruises of the Swedish icebreaker Oden in the inner Arctic in 1990, 1996, 2001, 2008, and 2018 provided a unique dataset on the seasonal distribution of atmospheric aerosol. Coupling these data with the seasonal sea ice distribution strongly indicated a regional biogenic aerosol source during late summer and early autumn freeze-up conditions. Given the expected further warming of the Arctic, we hypothesize an increase in biogenic aerosol in late summer and autumn.
Five summer cruises of the Swedish icebreaker Oden in the inner Arctic in 1990, 1996, 2001,...
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