Articles | Volume 25, issue 21 
            
                
                    
            
            
            https://doi.org/10.5194/acp-25-14205-2025
                    © Author(s) 2025. This work is distributed under 
the Creative Commons Attribution 4.0 License.
                the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-25-14205-2025
                    © Author(s) 2025. This work is distributed under 
the Creative Commons Attribution 4.0 License.
                the Creative Commons Attribution 4.0 License.
Differentiation of primary and secondary marine organic aerosol with machine learning
Baihua Chen
                                            State Key Laboratory of Advanced Environmental Technology, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen, China
                                        
                                    Lu Lei
                                            School of Physics, Centre for Climate & Air Pollution Studies, Ryan Institute, University of Galway, Galway, Ireland
                                        
                                    Emmanuel Chevassus
                                            School of Physics, Centre for Climate & Air Pollution Studies, Ryan Institute, University of Galway, Galway, Ireland
                                        
                                    
                                            State Key Laboratory of Advanced Environmental Technology, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen, China
                                        
                                    Ling Zhen
                                            State Key Laboratory of Advanced Environmental Technology, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen, China
                                        
                                    Haobin Zhong
                                            State Key Laboratory of Advanced Environmental Technology, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen, China
                                        
                                    Lin Wang
                                            State Key Laboratory of Advanced Environmental Technology, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen, China
                                        
                                    Chunshui Lin
                                            State Key Laboratory of Loess and Quaternary Geology and Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, China
                                        
                                    Ru-Jin Huang
                                            State Key Laboratory of Loess and Quaternary Geology and Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, China
                                        
                                    Darius Ceburnis
                                            School of Physics, Centre for Climate & Air Pollution Studies, Ryan Institute, University of Galway, Galway, Ireland
                                        
                                    Colin O'Dowd
                                            School of Physics, Centre for Climate & Air Pollution Studies, Ryan Institute, University of Galway, Galway, Ireland
                                        
                                    Jurgita Ovadnevaite
CORRESPONDING AUTHOR
                                            
                                    
                                            School of Physics, Centre for Climate & Air Pollution Studies, Ryan Institute, University of Galway, Galway, Ireland
                                        
                                    Data sets
Cloud condensation nuclei and hygroscopic growth measurement at Mace Head from 2009 to 2010 W. Xu et al. https://doi.org/10.17632/3dx6pnx869.1
Short summary
                    This study uses machine learning to separate marine primary organic aerosol (POA) and secondary organic aerosol (SOA) from 1 decade of high-resolution data. POA averages 51 % of marine organic aerosols annually, peaking at 63 % in summer. A support vector regression model, validated via fuzzy clustering and Monte Carlo simulations, identifies seasonal patterns of POA linked to biological activity. We found diverse impacts of marine POA and SOA on the aerosol hygroscopicity and mixing state.
                    This study uses machine learning to separate marine primary organic aerosol (POA) and secondary...
                    
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