Articles | Volume 24, issue 23
https://doi.org/10.5194/acp-24-13317-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-24-13317-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Opinion: Challenges and needs of tropospheric chemical mechanism development
Institute of Chemistry, University Clermont Auvergne, CNRS, 63000 Clermont-Ferrand, France
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, Heslington, York, YO10 5DD, United Kingdom
National Centre for Atmospheric Science, University of York, Heslington, York, YO10 5DD, United Kingdom
Bernard Aumont
Univ Paris Est Créteil and Université Paris Cité, CNRS, LISA, 94010 Créteil, France
William P. L. Carter
College of Engineering Center for Environmental Research and Technology (CE-CERT), University of California, Riverside, CA 92521, USA
Max McGillen
Institut de Combustion, Aérothermique, Réactivité Environnement (ICARE), CNRS, 1C Avenue de la Recherche Scientifique, CEDEX 2, 45071 Orléans, France
Abdelwahid Mellouki
Institut de Combustion, Aérothermique, Réactivité Environnement (ICARE), CNRS, 1C Avenue de la Recherche Scientifique, CEDEX 2, 45071 Orléans, France
University Mohammed VI Polytechnic (UM6P), Lot 660, Hay Moulay Rachid Ben Guerir, 43150, Morocco
John Orlando
Atmospheric Chemistry Observations and Modeling Lab, National Center for Atmospheric Research, P.O. Box 3000, Boulder, CO 80307, USA
Bénédicte Picquet-Varrault
Univ Paris Est Créteil and Université Paris Cité, CNRS, LISA, 94010 Créteil, France
Paul Seakins
School of Chemistry, University of Leeds, Leeds, LS2 9JT, United Kingdom
William R. Stockwell
Department of Physics, University of Texas at El Paso, El Paso, TX, USA
Luc Vereecken
Institute of Climate and Energy Systems ICE-3: Troposphere, Forschungszentrum Jülich GmbH, 52425 Jülich, Germany
Timothy J. Wallington
Center for Sustainable Systems, School for Environment and Sustainability, University of Michigan, Ann Arbor MI 48109, USA
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- Enhancing 72-Hour air quality forecasting with an observation-driven deep learning chemistry transport model S. Li & J. Xing 10.1016/j.envint.2025.109689
- Development of a Relative Rate Technique to Measure Criegee Intermediate Reactivity P. Wang et al. 10.1021/acs.estlett.5c00372
- A perspective on the reactions of organic peroxy radicals with HO2 N. Illmann 10.1039/D5EA00023H
- Practical atmospheric photochemical kinetics for undergraduate teaching and research J. D'Souza Metcalf et al. 10.1039/D5SU00681C
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Latest update: 09 Oct 2025
Executive editor
This paper is written by experts in the field and addresses new tropospheric chemical mechanism developments. It shows how new analytical methods, instrumentation and cheminformatics methods have led to the identification of key processes and knowledge gaps in our understanding of chemical mechanisms, both in the gas phase and condensed phases. The opinion paper presents a perspective on these developments in the present and future, and outlines new directions. This opinion will be a very valuable contribution for the community and I am convinced it will be frequently read and cited.
This paper is written by experts in the field and addresses new tropospheric chemical mechanism...
Short summary
Chemical mechanisms describe the chemical processes in atmospheric models that are used to describe the changes in the atmospheric composition. Therefore, accurate chemical mechanisms are necessary to predict the evolution of air pollution and climate change. The article describes all steps that are needed to build chemical mechanisms and discusses the advances and needs of experimental and theoretical research activities needed to build reliable chemical mechanisms.
Chemical mechanisms describe the chemical processes in atmospheric models that are used to...
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