State Key Laboratory of Severe Weather, Key Laboratory of
Atmospheric Chemistry of CMA, Institute of Atmospheric Composition, Chinese
Academy of Meteorological Sciences, Beijing 100081, China
State Key Laboratory of Severe Weather, Key Laboratory of
Atmospheric Chemistry of CMA, Institute of Atmospheric Composition, Chinese
Academy of Meteorological Sciences, Beijing 100081, China
National Observation and Research Station of Coastal Ecological
Environments in Macao, Macao Environmental Research Institute, Macau
University of Science and Technology, Macao SAR 999078, China
Jian Zhang
State Key Laboratory of Severe Weather, Key Laboratory of
Atmospheric Chemistry of CMA, Institute of Atmospheric Composition, Chinese
Academy of Meteorological Sciences, Beijing 100081, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan Tyndall Centre, Institute of Atmospheric Sciences, Fudan University,
Shanghai, China
Center for Excellence in Urban Atmospheric Environment, Institute
of Urban Environment, Chinese Academy of Science, Xiamen, China
Shanghai Institute of Eco-Chongming (SIEC), No. 3663 Northern
Zhongshan Road, Shanghai 200062, China
Lei Zhang
State Key Laboratory of Severe Weather, Key Laboratory of
Atmospheric Chemistry of CMA, Institute of Atmospheric Composition, Chinese
Academy of Meteorological Sciences, Beijing 100081, China
State Key Laboratory of Severe Weather, Key Laboratory of
Atmospheric Chemistry of CMA, Institute of Atmospheric Composition, Chinese
Academy of Meteorological Sciences, Beijing 100081, China
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WRF/CUACE was used to assess the cloud chemistry contribution in China. Firstly, the CUACE cloud chemistry scheme was found to reproduce well the cloud processing and consumption of H2O2, O3, and SO2, as well as the increase of sulfate. Secondly, during cloud availability in December under a heavy pollution episode, sulfate production increased 60–95 % and SO2 was reduced by over 80 %. This study provides a way to analyze the phenomenon of overestimation of SO2 in many chemical transport models.
WRF/CUACE was used to assess the cloud chemistry contribution in China. Firstly, the CUACE cloud...
