Articles | Volume 23, issue 1
https://doi.org/10.5194/acp-23-611-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-611-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
16 Jan 2023
Research article |
| 16 Jan 2023
| 16 Jan 2023
Impact of aging on the sources, volatility, and viscosity of organic aerosols in Chinese outflows
Tingting Feng
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Chinese Academy of Sciences University, Beijing 100049, China
Guangdong-Hong Kong-Macao, Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
Yingkun Wang
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Chinese Academy of Sciences University, Beijing 100049, China
Guangdong-Hong Kong-Macao, Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Guangdong-Hong Kong-Macao, Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
State Environmental Protection Key Laboratory of Formation and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China
Ming Zhu
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Chinese Academy of Sciences University, Beijing 100049, China
Guangdong-Hong Kong-Macao, Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
Wei Song
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Guangdong-Hong Kong-Macao, Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
Wei Chen
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Chinese Academy of Sciences University, Beijing 100049, China
Guangdong-Hong Kong-Macao, Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
Yanyan Sang
Tai'an Environmental Protection Bureau, Tai'an, Shandong 271000, China
Zheng Fang
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Chinese Academy of Sciences University, Beijing 100049, China
Guangdong-Hong Kong-Macao, Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Chinese Academy of Sciences University, Beijing 100049, China
Guangdong-Hong Kong-Macao, Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
Hua Fang
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Chinese Academy of Sciences University, Beijing 100049, China
Guangdong-Hong Kong-Macao, Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
now at: School of Ecology and Environment, Anhui Normal University, Wuhu, Anhui 241000, China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Chinese Academy of Sciences University, Beijing 100049, China
Guangdong-Hong Kong-Macao, Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
Institute of Mass Spectrometry and Atmospheric Environment, Jinan University, Guangzhou 510632, China
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Shan Huang
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Min Shao
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Xiaofeng Huang
Key Laboratory for Urban Habitat Environmental Science and Technology, School of Environment and Energy, Peking University Shenzhen Graduate School, Shenzhen 518055, China
Lingyan He
Key Laboratory for Urban Habitat Environmental Science and Technology, School of Environment and Energy, Peking University Shenzhen Graduate School, Shenzhen 518055, China
Young Ro Lee
School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA 30332, USA
Lewis Gregory Huey
School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA 30332, USA
Francesco Canonaco
Paul Scherrer Institute, Laboratory of Atmospheric Chemistry, 5232 Villigen PSI, Switzerland
Datalystica Ltd., Park innovAARE, 5234 Villigen, Switzerland
Andre S. H. Prevot
Paul Scherrer Institute, Laboratory of Atmospheric Chemistry, 5232 Villigen PSI, Switzerland
Xinming Wang
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Chinese Academy of Sciences University, Beijing 100049, China
Guangdong-Hong Kong-Macao, Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Chinese Academy of Science, Guangzhou 510640, China
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Cited
8 citations as recorded by crossref.
- Changes in Physicochemical Properties of Organic Aerosol During Photochemical Aging of Cooking and Burning Emissions W. Xu et al. 10.1029/2022JD037911
- Linking Precursors and Volatility of Ambient Oxygenated Organic Aerosols Using Thermal Desorption Measurement and Machine Learning X. Wang et al. 10.1021/acsestair.4c00076
- Molecular Insights into Gas–Particle Partitioning and Viscosity of Atmospheric Brown Carbon Q. Xie et al. 10.1021/acs.est.4c05650
- Elucidating ozone and PM2.5 pollution in the Fenwei Plain reveals the co-benefits of controlling precursor gas emissions in winter haze C. Lin et al. 10.5194/acp-23-3595-2023
- Chemical characterization and sources of background aerosols in the eastern Mediterranean K. Florou et al. 10.1016/j.atmosenv.2024.120423
- Simulated phase state and viscosity of secondary organic aerosols over China Z. Zhang et al. 10.5194/acp-24-4809-2024
- A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system T. Pan et al. 10.5194/amt-17-4915-2024
- The characterization of ambient levoglucosan in Beijing during summertime: Dynamic variation and source contributions under strong cooking influences J. Wang et al. 10.1016/j.jes.2024.08.029
8 citations as recorded by crossref.
- Changes in Physicochemical Properties of Organic Aerosol During Photochemical Aging of Cooking and Burning Emissions W. Xu et al. 10.1029/2022JD037911
- Linking Precursors and Volatility of Ambient Oxygenated Organic Aerosols Using Thermal Desorption Measurement and Machine Learning X. Wang et al. 10.1021/acsestair.4c00076
- Molecular Insights into Gas–Particle Partitioning and Viscosity of Atmospheric Brown Carbon Q. Xie et al. 10.1021/acs.est.4c05650
- Elucidating ozone and PM2.5 pollution in the Fenwei Plain reveals the co-benefits of controlling precursor gas emissions in winter haze C. Lin et al. 10.5194/acp-23-3595-2023
- Chemical characterization and sources of background aerosols in the eastern Mediterranean K. Florou et al. 10.1016/j.atmosenv.2024.120423
- Simulated phase state and viscosity of secondary organic aerosols over China Z. Zhang et al. 10.5194/acp-24-4809-2024
- A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system T. Pan et al. 10.5194/amt-17-4915-2024
- The characterization of ambient levoglucosan in Beijing during summertime: Dynamic variation and source contributions under strong cooking influences J. Wang et al. 10.1016/j.jes.2024.08.029
Latest update: 21 Nov 2024
Short summary
To investigate the impact of aging processes on organic aerosols (OA), we conducted a comprehensive field study at a continental remote site using an on-line mass spectrometer. The results show that OA in the Chinese outflows were strongly influenced by upwind anthropogenic emissions. The aging processes can significantly decrease the OA volatility and result in a varied viscosity of OA under different circumstances, signifying the complex physiochemical properties of OA in aged plumes.
To investigate the impact of aging processes on organic aerosols (OA), we conducted a...
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