Articles | Volume 23, issue 10
https://doi.org/10.5194/acp-23-5993-2023
https://doi.org/10.5194/acp-23-5993-2023
Research article
 | 
01 Jun 2023
Research article |  | 01 Jun 2023

Collision-sticking rates of acid–base clusters in the gas phase determined from atomistic simulation and a novel analytical interacting hard-sphere model

Huan Yang, Ivo Neefjes, Valtteri Tikkanen, Jakub Kubečka, Theo Kurtén, Hanna Vehkamäki, and Bernhard Reischl

Viewed

Total article views: 1,457 (including HTML, PDF, and XML)
HTML PDF XML Total Supplement BibTeX EndNote
1,202 220 35 1,457 81 38 28
  • HTML: 1,202
  • PDF: 220
  • XML: 35
  • Total: 1,457
  • Supplement: 81
  • BibTeX: 38
  • EndNote: 28
Views and downloads (calculated since 25 Jan 2023)
Cumulative views and downloads (calculated since 25 Jan 2023)

Viewed (geographical distribution)

Total article views: 1,457 (including HTML, PDF, and XML) Thereof 1,430 with geography defined and 27 with unknown origin.
Country # Views %
  • 1
1
 
 
 
 
Latest update: 06 May 2024
Download
Short summary
We present a new analytical model for collision rates between molecules and clusters of arbitrary sizes, accounting for long-range interactions. The model is verified against atomistic simulations of typical acid–base clusters participating in atmospheric new particle formation (NPF). Compared to non-interacting models, accounting for long-range interactions leads to 2–3 times higher collision rates for small clusters, indicating the necessity of including such interactions in NPF modeling.
Altmetrics
Final-revised paper
Preprint