Articles | Volume 22, issue 10
https://doi.org/10.5194/acp-22-6449-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-6449-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Measurement report
| 
19 May 2022
Measurement report |
| 19 May 2022
| 19 May 2022
Measurement report: Optical properties and sources of water-soluble brown carbon in Tianjin, North China – insights from organic molecular compositions
Junjun Deng
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Hao Ma
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Xinfeng Wang
Environment Research Institute, Shandong University, Jinan 250100, China
Shujun Zhong
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Zhimin Zhang
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Jialei Zhu
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Yanbing Fan
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Libin Wu
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Xiaodong Li
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Lujie Ren
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Chandra Mouli Pavuluri
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Xiaole Pan
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Zifa Wang
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Kimitaka Kawamura
Chubu Institute for Advanced Studies, Chubu University, Kasugai 487-8501, Japan
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
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Cited
30 citations as recorded by crossref.
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- Chemical and Light-Absorption Properties of Water-Soluble Organic Aerosols in Northern California and Photooxidant Production by Brown Carbon Components W. Jiang et al. 10.1021/acsearthspacechem.3c00022
- Compositional and optical characteristics of aqueous brown carbon and HULIS in the eastern Indo-Gangetic Plain using a coupled EEM PARAFAC, FT-IR and 1H NMR approach S. Dey & S. Sarkar 10.1016/j.scitotenv.2024.171084
- Water-soluble brown carbon in PM2.5 at two typical sites in Guanzhong Basin: Optical properties, sources, and implications X. Li et al. 10.1016/j.atmosres.2022.106499
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- Seasonal characterization of chemical and optical properties of water-soluble organic aerosol in Beijing B. You et al. 10.1016/j.scitotenv.2024.172508
- Compositions and sources of fluorescent water-soluble and water-insoluble organic aerosols H. Ma et al. 10.1016/j.scitotenv.2024.174627
- Impact of biogenic secondary organic aerosol (SOA) loading on the molecular composition of wintertime PM2.5 in urban Tianjin: an insight from Fourier transform ion cyclotron resonance mass spectrometry S. Zhong et al. 10.5194/acp-23-2061-2023
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- Measurement report: Brown carbon aerosol in polluted urban air of the North China Plain – day–night differences in the chromophores and optical properties Y. Gong et al. 10.5194/acp-23-15197-2023
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- Research progress on secondary formation, photosensitive reaction mechanism and human health effects of chromophoric brown carbon B. Chen et al. 10.1016/j.jes.2024.04.003
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- Diurnal variations in primary and secondary organic aerosols in an eastern China coastal city: The impact of land-sea breezes Q. Zhang et al. 10.1016/j.envpol.2023.121016
- Measurement report: Changes in light absorption and molecular composition of water-soluble humic-like substances during a winter haze bloom-decay process in Guangzhou, China C. Zou et al. 10.5194/acp-23-963-2023
- Seasonal and Day–Night Variations in Carbonaceous Aerosols and Their Light-Absorbing Properties in Guangzhou, China J. Su et al. 10.3390/atmos14101545
- Insights into dissolved organics in non-urban areas - Optical properties and sources F. Yu et al. 10.1016/j.envpol.2023.121641
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- Effects of aerosol water content and acidity on the light absorption of atmospheric humic-like substances in winter T. Tang et al. 10.1016/j.chemosphere.2023.140796
- Stable Isotopes Reveal Photoreduction of Particle-Bound Mercury Driven by Water-Soluble Organic Carbon during Severe Haze K. Zhang et al. 10.1021/acs.est.2c01933
- Molecular composition of Beijing PM2.5 Brown carbon associated with fluorescence revealed by gas chromatography time-of-flight mass spectrometry and parallel factor analysis J. Cao et al. 10.1016/j.atmosenv.2024.120670
- The water-insoluble organic carbon in PM2.5 of typical Chinese urban areas: light-absorbing properties, potential sources, radiative forcing effects, and a possible light-absorbing continuum Y. Mo et al. 10.5194/acp-24-7755-2024
- Brown Carbon from Photo-Oxidation of Glyoxal and SO2 in Aqueous Aerosol D. De Haan et al. 10.1021/acsearthspacechem.3c00035
- Water-Soluble Brown Carbon in Pm2.5 at Two Typical Sites in Guanzhong Basin: Optical Properties, Sources, and Implications X. Li et al. 10.2139/ssrn.4192603
- Continuous Measurement and Molecular Compositions of Atmospheric Water‐Soluble Brown Carbon in the Nearshore Marine Boundary Layer of Northern China: Secondary Formation and Influencing Factors H. Li et al. 10.1029/2023JD038565
29 citations as recorded by crossref.
- Optical Properties of Individual Tar Balls in the Free Troposphere S. Mathai et al. 10.1021/acs.est.3c03498
- Variations in optical properties of water- and methanol-soluble organic carbon in PM2.5 in Tianjin and Handan over the Wintertime of 2018–2020 H. Chen et al. 10.1016/j.atmosres.2024.107332
- Chemical and Light-Absorption Properties of Water-Soluble Organic Aerosols in Northern California and Photooxidant Production by Brown Carbon Components W. Jiang et al. 10.1021/acsearthspacechem.3c00022
- Compositional and optical characteristics of aqueous brown carbon and HULIS in the eastern Indo-Gangetic Plain using a coupled EEM PARAFAC, FT-IR and 1H NMR approach S. Dey & S. Sarkar 10.1016/j.scitotenv.2024.171084
- Water-soluble brown carbon in PM2.5 at two typical sites in Guanzhong Basin: Optical properties, sources, and implications X. Li et al. 10.1016/j.atmosres.2022.106499
- Technical note: Chemical composition and source identification of fluorescent components in atmospheric water-soluble brown carbon by excitation–emission matrix spectroscopy with parallel factor analysis – potential limitations and applications T. Cao et al. 10.5194/acp-23-2613-2023
- Measurement report: Optical characterization, seasonality, and sources of brown carbon in fine aerosols from Tianjin, North China: year-round observations Z. Dong et al. 10.5194/acp-24-5887-2024
- Atmospheric humic-like substances (HULIS) in Chongqing, Southwest China: Abundance, light absorption properties, and potential sources T. Tang et al. 10.1016/j.atmosres.2023.107016
- Seasonal characterization of chemical and optical properties of water-soluble organic aerosol in Beijing B. You et al. 10.1016/j.scitotenv.2024.172508
- Compositions and sources of fluorescent water-soluble and water-insoluble organic aerosols H. Ma et al. 10.1016/j.scitotenv.2024.174627
- Impact of biogenic secondary organic aerosol (SOA) loading on the molecular composition of wintertime PM2.5 in urban Tianjin: an insight from Fourier transform ion cyclotron resonance mass spectrometry S. Zhong et al. 10.5194/acp-23-2061-2023
- Characterizing water-soluble brown carbon in fine particles in four typical cities in northwestern China during wintertime: integrating optical properties with chemical processes M. Zhong et al. 10.5194/acp-23-12609-2023
- Light-absorbing properties of polar- and non-polar brown carbon fractions of aerosols in Delhi A. Alang et al. 10.1016/j.atmosres.2023.107073
- Measurement report: Brown carbon aerosol in polluted urban air of the North China Plain – day–night differences in the chromophores and optical properties Y. Gong et al. 10.5194/acp-23-15197-2023
- Chromophores and chemical composition of brown carbon characterized at an urban kerbside by excitation–emission spectroscopy and mass spectrometry F. Jiang et al. 10.5194/acp-22-14971-2022
- Research progress on secondary formation, photosensitive reaction mechanism and human health effects of chromophoric brown carbon B. Chen et al. 10.1016/j.jes.2024.04.003
- A Review on Brown Carbon Aerosol in China: From Molecular Composition to Climate Impact X. Cao et al. 10.1007/s40726-024-00293-y
- Photoaging of phenolic secondary organic aerosol in the aqueous phase: evolution of chemical and optical properties and effects of oxidants W. Jiang et al. 10.5194/acp-23-7103-2023
- Diurnal variations in primary and secondary organic aerosols in an eastern China coastal city: The impact of land-sea breezes Q. Zhang et al. 10.1016/j.envpol.2023.121016
- Measurement report: Changes in light absorption and molecular composition of water-soluble humic-like substances during a winter haze bloom-decay process in Guangzhou, China C. Zou et al. 10.5194/acp-23-963-2023
- Seasonal and Day–Night Variations in Carbonaceous Aerosols and Their Light-Absorbing Properties in Guangzhou, China J. Su et al. 10.3390/atmos14101545
- Insights into dissolved organics in non-urban areas - Optical properties and sources F. Yu et al. 10.1016/j.envpol.2023.121641
- Optical properties and molecular composition of wintertime atmospheric water-soluble organic carbon in different coastal cities of eastern China H. Chen et al. 10.1016/j.scitotenv.2023.164702
- Effects of aerosol water content and acidity on the light absorption of atmospheric humic-like substances in winter T. Tang et al. 10.1016/j.chemosphere.2023.140796
- Stable Isotopes Reveal Photoreduction of Particle-Bound Mercury Driven by Water-Soluble Organic Carbon during Severe Haze K. Zhang et al. 10.1021/acs.est.2c01933
- Molecular composition of Beijing PM2.5 Brown carbon associated with fluorescence revealed by gas chromatography time-of-flight mass spectrometry and parallel factor analysis J. Cao et al. 10.1016/j.atmosenv.2024.120670
- The water-insoluble organic carbon in PM2.5 of typical Chinese urban areas: light-absorbing properties, potential sources, radiative forcing effects, and a possible light-absorbing continuum Y. Mo et al. 10.5194/acp-24-7755-2024
- Brown Carbon from Photo-Oxidation of Glyoxal and SO2 in Aqueous Aerosol D. De Haan et al. 10.1021/acsearthspacechem.3c00035
- Water-Soluble Brown Carbon in Pm2.5 at Two Typical Sites in Guanzhong Basin: Optical Properties, Sources, and Implications X. Li et al. 10.2139/ssrn.4192603
Latest update: 16 Jul 2024
Short summary
Light-absorbing brown carbon (BrC) plays an important role in climate change and atmospheric chemistry. Here we investigated the seasonal and diurnal variations in water-soluble BrC in PM2.5 in the megacity Tianjin in coastal China. Results of the source apportionments from the combination with organic molecular compositions and optical properties of water-soluble BrC reveal a large contribution from primary bioaerosol particles to BrC in the urban atmosphere.
Light-absorbing brown carbon (BrC) plays an important role in climate change and atmospheric...
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